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A Note on the Nomenclature in Neutron Multiplicity Mathematics

The purpose of this technical note is to consolidate the notations used for describing parameters that pertain to neutron multiplicity mathematics relevant to various applications including nonproliferation, international safeguards, and criticality safety among others. The nomenclatures used in these techniques vary widely depending on the origin of the work and their applications. We aim here to consolidate many of the previously used notations in a single document to enhance past, present, and future technical exchanges pertaining to neutron multiplicity. This will help avoid confusion in future publications and will facilitate wider application-independent advancements and utility of peer-reviewed findings. A brief introduction and history of neutron multiplicity counting is presented, followed by a summary of commonly used techniques in a variety of different applications. In each section, we present the notations used in previous publications for the reader’s reference.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

MULTIPLICITY AND PERIOD DISTRIBUTION OF POPULATION II FIELD STARS IN SOLAR VICINITY

We examine a sample of 223 F, G, and early K metal-poor subdwarfs ([m/H] < -1) with high proper motions ({mu}>0.''2 yr{sup -1}) at distances of up to 250 pc from the Sun. By means of our own speckle interferometric observations conducted on the 6 m Bolshoi Azimuthal Telescope of the Special Astrophysical Observatory of the Russian Academy of Sciences, and the spectroscopic and visual data taken from the literature, we determine the frequency of binary and multiple systems in this sample. The ratio of single, binary, triple, and quadruple systems among 221 primary components of the sample is 147:64:9:1. We show that the distribution of orbital periods of binary and multiple subdwarfs is asymmetric in the range of up to P = 10{sup 10} days, and has a maximum at P = 10{sup 2}-10{sup 3} days, which differs from the distribution, obtained for the thin disk G dwarfs. We estimated the number of undetected companions in our sample. Comparing the frequency of binary subdwarfs in the field and in the globular clusters, we show that the process of halo field star formation by the means of destruction of globular clusters is very unlikely in our Galaxy. We discuss the multiplicity of old metal-poor stars in nearby stellar streams.

79 ASTRONOMY AND ASTROPHYSICS↗

THE SOLAR NEIGHBORHOOD. XXVIII. THE MULTIPLICITY FRACTION OF NEARBY STARS FROM 5 TO 70 AU AND THE BROWN DWARF DESERT AROUND M DWARFS

We report on our analysis of Hubble Space Telescope/NICMOS snapshot high-resolution images of 255 stars in 201 systems within {approx}10 pc of the Sun. Photometry was obtained through filters F110W, F180M, F207M, and F222M using NICMOS Camera 2. These filters were selected to permit clear identification of cool brown dwarfs through methane contrast imaging. With a plate scale of 76 mas pixel{sup -1}, NICMOS can easily resolve binaries with subarcsecond separations in the 19.''5 Multiplication-Sign 19.''5 field of view. We previously reported five companions to nearby M and L dwarfs from this search. No new companions were discovered during the second phase of data analysis presented here, confirming that stellar/substellar binaries are rare. We establish magnitude and separation limits for which companions can be ruled out for each star in the sample, and then perform a comprehensive sensitivity and completeness analysis for the subsample of 138 M dwarfs in 126 systems. We calculate a multiplicity fraction of 0.0{sup +3.5}{sub -0.0}% for L companions to M dwarfs in the separation range of 5-70 AU, and 2.3{sup +5.0}{sub -0.7}% for L and T companions to M dwarfs in the separation range of 10-70 AU. We also discuss trends in the color-magnitude diagrams using various color combinations and present astrometry for 19 multiple systems in our sample. Considering these results and results from several other studies, we argue that the so-called brown dwarf desert extends to binary systems with low-mass primaries and is largely independent of primary mass, mass ratio, and separations. While focusing on companion properties, we discuss how the qualitative agreement between observed companion mass functions and initial mass functions suggests that the paucity of brown dwarfs in either population may be due to a common cause and not due to binary formation mechanisms.

79 ASTRONOMY AND ASTROPHYSICS↗

OBSERVATIONS OF HIERARCHICAL SOLAR-TYPE MULTIPLE STAR SYSTEMS

Twenty multiple stellar systems with solar-type primaries were observed at high angular resolution using the PALM-3000 adaptive optics system at the 5 m Hale telescope. The goal was to complement the knowledge of hierarchical multiplicity in the solar neighborhood by confirming recent discoveries by the visible Robo-AO system with new near-infrared observations with PALM-3000. The physical status of most, but not all, of the new pairs is confirmed by photometry in the Ks band and new positional measurements. In addition, we resolved for the first time five close sub-systems: the known astrometric binary in HIP 17129AB, companions to the primaries of HIP 33555, and HIP 118213, and the companions to the secondaries in HIP 25300 and HIP 101430. We place the components on a color–magnitude diagram and discuss each multiple system individually.

79 ASTRONOMY AND ASTROPHYSICS↗

MULTIPLE INVERSE COMPTON SCATTERINGS AND THE BLAZAR SEQUENCE

The high frequency component in blazars is thought to be due to inverse Compton scattered radiation. Recent observations by Fermi-LAT are used to evaluate the details of the scattering process. A comparison is made between the usually assumed single scattering scenario and one in which multiple scatterings are energetically important. In the latter case, most of the radiation is emitted in the Klein-Nishina limit. It is argued that several of the observed correlations defining the blazar sequence are most easily understood in a multiple scattering scenario. Observations indicate also that, in such a scenario, the blazar sequence is primarily governed by the energy density of relativistic electrons rather than that of the seed photons. The pronounced X-ray minimum in the spectral energy distribution often observed in the most luminous blazars is discussed. It is shown how this feature can be accounted for in a multiple scattering scenario by an extension of standard one-zone models.

79 ASTRONOMY AND ASTROPHYSICS↗

MULTIPLE STAR FORMATION TO THE BOTTOM OF THE INITIAL MASS FUNCTION

The frequency and properties of multiple star systems offer powerful tests of star formation models. Multiplicity surveys over the past decade have shown that binary properties vary strongly with mass, but the functional forms and the interplay between frequency and semimajor axis remain largely unconstrained. We present the results of a large-scale survey of multiplicity at the bottom of the initial mass function in several nearby young associations, encompassing 78 very low mass members observed with Keck laser guide star adaptive optics. Our survey confirms the overall trend observed in the field for lower-mass binary systems to be less frequent and more compact, including a null detection for any substellar binary systems with separations wider than {approx}7 AU. Combined with a Bayesian re-analysis of existing surveys, our results demonstrate that the binary frequency and binary separations decline smoothly between masses of 0.5 M{sub Sun} and 0.02 M{sub Sun }, though we cannot distinguish the functional form of this decline due to a degeneracy between the total binary frequency and the mean binary separation. We also show that the mass ratio distribution becomes progressively more concentrated at q {approx} 1 for declining masses, though a small number of systems appear to have unusually wide separations and low-mass ratios for their mass. Finally, we compare our results to synthetic binary populations generated by smoothed particle hydrodynamic simulations, noting the similarities and discussing possible explanations for the differences.

79 ASTRONOMY AND ASTROPHYSICS↗

NUMERICAL SIMULATIONS OF MULTIPLE SCATTERING OF THE f-MODE BY FLUX TUBES

We use numerical simulations to study the absorption and phase shift of surface-gravity waves caused by groups of magnetic flux tubes. The dependence of the scattering coefficients on the distance between the tubes and their positions is analyzed for several cases with two or three flux tubes embedded in a quiet Sun atmosphere. The results are compared with those obtained neglecting completely or partially multiple scattering effects. We show that multiple scattering has a significant impact on the absorption measurements and tends to reduce the phase shift. We also consider more general cases of ensembles of randomly distributed flux tubes, and we have evaluated the effects on the scattering measurements of changing the number of tubes included in the bundle and the average distance between flux tubes. We find that for the longest wavelength incoming waves, multiple scattering enhances the absorption, and its efficiency increases with the number of flux tubes and the reduction of the distance between them.

79 ASTRONOMY AND ASTROPHYSICS↗

SUB-STELLAR COMPANIONS AND STELLAR MULTIPLICITY IN THE TAURUS STAR-FORMING REGION

We present results from a large, high-spatial-resolution near-infrared imaging search for stellar and sub-stellar companions in the Taurus-Auriga star-forming region. The sample covers 64 stars with masses between those of the most massive Taurus members at ∼3 M {sub ☉} and low-mass stars at ∼0.2 M {sub ☉}. We detected 74 companion candidates, 34 of these reported for the first time. Twenty-five companions are likely physically bound, partly confirmed by follow-up observations. Four candidate companions are likely unrelated field stars. Assuming physical association with their host star, estimated companion masses are as low as ∼2 M {sub Jup}. The inferred multiplicity frequency within our sensitivity limits between ∼10-1500 AU is 26.3{sub −4.9}{sup +6.6}%. Applying a completeness correction, 62% ± 14% of all Taurus stars between 0.7 and 1.4 M {sub ☉} appear to be multiple. Higher order multiples were found in 1.8{sub −1.5}{sup +4.2}% of the cases, in agreement with previous observations of the field. We estimate a sub-stellar companion frequency of ∼3.5%-8.8% within our sensitivity limits from the discovery of two likely bound and three other tentative very low-mass companions. This frequency appears to be in agreement with what is expected from the tail of the stellar companion mass ratio distribution, suggesting that stellar and brown dwarf companions share the same dominant formation mechanism. Further, we find evidence for possible evolution of binary parameters between two identified sub-populations in Taurus with ages of ∼2 Myr and ∼20 Myr, respectively.

79 ASTRONOMY AND ASTROPHYSICS↗

The Auger Radioisotope Microscope: an instrument for characterization of Auger electron multiplicities and energy distributions

We describe a new instrument, the Argonne Auger Radioisotope Microscope (ARM), capable of characterizing the Auger electron (AE) emission of radionuclides, including candidates relevant in nuclear medicine. Our approach relies on event-by-event ion–electron coincidence, time-of-flight, and spatial readout measurement to determine correlated electron multiplicity and energy distributions of Auger decays. We present a proof-of-principle measurement with the ARM using x-ray photoionization of stable krypton beyond the K-edge and identify a bifurcation in the electron multiplicity distribution depending on the emission of K-LX electrons. Extension of the ARM to the characterization of radioactive sources of AE emissions is enabled by the combination of two recent developments: (1) cryogenic buffer gas beam technology to introduce Auger emitters into the detection region with well-defined initial conditions, and (2) large-area micro-channel plate detectors with multi-hit detection capabilities to simultaneously detect multiple electrons emitted in a single decay.

Auger emitters↗

Systematics of pre- and near-scission {alpha}-particle multiplicities in heavy-ion-induced fusion-fission reactions

The {alpha}-particle energy spectra have been measured in coincidence with fission fragments over a wide range of relative angles with respect to fragment emission direction in the {sup 11}B (62 MeV) + {sup 232}Th reaction. The {alpha}-particle multiplicity spectra have been fitted with moving source model to extract the precision ({alpha}{sub pre}) and near-scission ({alpha}{sub nse}) components. The present results, along with available data from the literature over a wide range of Z{sup 2}/A and the excitation energy of a compound system, have been analyzed to develop certain global features of the pre- and near-scission emission characteristics. It is seen that {alpha}{sub pre} values when normalized to E{sub CN}{sup 2.3} (E{sub CN} is the compound nucleus excitation energy) show a systematic linearly increasing trend with the {alpha}-particle emission Q value (Q{sub {alpha}}). The fraction of near-scission multiplicity is observed to be nearly the same at around 10% of the total precision multiplicity for all the systems.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A polarization-switch effect of silicon crystals under multiple-beam diffraction geometry

On the basis of rigorous dynamical-theory calculations, a complete X-ray polarization-switch effect of silicon crystals at the exact multiple-beam diffraction condition is demonstrated in this paper. The underlying physical mechanism of this unique phenomenon can be revealed using a simple multiple-wave propagation and interference model. The constructive and destructive interference of the multiple detoured-diffraction beams along the direction of the primary diffracted beam directly leads to the complete polarization switch. This phenomenon can be realized using both synchrotron and laboratory X-ray sources at many discrete wavelengths, and used to design a novel crystal-based polarizer to achieve a 90° polarization rotation.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DXRD : a user-friendly suite of two- and multiple-beam dynamical X-ray diffraction programs

The DXRD program suite consisting of a series of dynamical theory programs is introduced for computing dynamical X-ray diffraction from single crystals. Its interactive graphical user interfaces (GUIs) allow general users to make complicated calculations with minimal effort. It can calculate plane-wave Darwin curves of single crystals (or multiple crystals) for both the Bragg and Laue cases, including grazing-incidence diffraction and backward diffraction (with Bragg angles approaching 90°). It is also capable of simulating rocking curves for divergent incident X-ray beams with finite bandwidths. A unique feature of DXRD is that it provides a convenient GUI-based multiple-beam diffraction program that can accurately compute arbitrary N-beam diffraction of any geometry using a universal 4N × 4N matrix method. DXRD also provides a mapping program for plotting all the multiple-beam diffraction lines (monochromator glitches) in the azimuth–energy coordinate system. All these functions make DXRD a convenient and powerful software tool for designing crystal-based synchrotron/X-ray optics (monochromators, analyzers, polarizers, phase plates etc.) and for crystal characterization, X-ray spectroscopy and X-ray diffraction teaching.

Bragg reflection↗

Alternatives to Helium-3 for Neutron Multiplicity Counters

Multiplicity counters are an example of a neutron detection system affected by the shortage of 3He. Efforts are underway to identify potential 3He neutron detector replacements for use in multiplicity counters. Boron-10 and 6Li based systems are two of the options being explored as near-term 3He alternatives for neutron multiplicity counters. Simulations of BF3, 10B-lined proportional counters and 6Li/ZnS(Ag) sheets in various configurations have been performed with the Monte Carlo particle transport code MCNPX and compared to simulations of existing 3He counters. The system performances are being compared using figure of merits that are the square or cube of the total system efficiency divided by the die-away time. Design considerations include developing a system with enough neutron detection material to achieve the highest possible efficiency, while simultaneously minimizing system size. Adequate moderation is required to thermalize the incident neutrons for increased counting efficiency but as the system size increases so will the die-away time (average lifetime of neutrons in the counter). The optimal moderator configuration is one for which the increase in neutron detection efficiency is not defeated by an increase in die-away time. Thus, the entire system performance must be evaluated with every configuration change. The simulation results will be validated against a bench-top demonstrator unit design based on the system identified through simulations as having the highest performance potential. Presented here are the simulation results with various configurations of BF3 filled proportional counters, 10B lined proportional counters and 6Li/ZnS(Ag) sheets, and preliminary bench-top measurements.

Alternatives to Helium-3 for Neutron Multiplicity ↗

Sixteen multiple-amplifier sensing charge-coupled devices and characterization techniques targeting the next generation of astronomical instruments

We present a candidate sensor for future spectroscopic applications, such as a Stage-5 Spectroscopic Survey Experiment or the Habitable Worlds Observatory. This type of charge-coupled device (CCD) sensor features multiple in-line amplifiers at its output stage allowing multiple measurements of the same charge packet, either in each amplifier or in the different amplifiers. Recently, the operation of an eight-amplifier sensor has been experimentally demonstrated, and we present the operation of a 16-amplifier sensor. This new sensor enables a noise level of ∼1 erms− with a single sample per amplifier. In addition, it is shown that sub-electron noise can be achieved using multiple samples per amplifier. In addition to demonstrating the performance of the 16-amplifier sensor, we aim to create a framework for future analysis and performance optimization of this type of detectors. New models and techniques are presented to characterize specific parameters, which are absent in conventional CCDs and Skipper CCDs: charge transfer between amplifiers and independent and common noise in the amplifiers and their processing.

16 multiple-amplifer sensing CCD (MAS-CCD)↗

Prompt Neutron Multiplicity Measurements with Portable Detectors

Mobile detection of kilogram quantities of special nuclear materials (SNM) during maritime transportation is a challenging problem for the U.S. Department of Homeland Security. Counting neutrons emitted by the SNM and partitioning them from background neutrons of multiple origins is the most effective passive means of detecting the SNM. Unfortunately, neutron detection, counting, and partitioning in a maritime environment is complex due to the presence of spallation neutrons (commonly known as “ship effect”) and to the complicated nature of the neutron scattering in that environment. This work studied the possibilities of building a prototype neutron detector using boron- 10 (10B) as the converter in a novel form factor called “straws” that would address the above problem by examining multiplicity distributions of neutrons originating from a fissioning source. Currently, commercially manufactured fission meters (FM) are available that separate cosmic neutrons from non-cosmic neutrons and quantitatively determine the strength of a fissioning source; however, these FMs use 3He, which is becoming increasingly difficult to procure; also the size and weight of a commercial FM is not conducive to manual neutron detection operations in a maritime environment. The current project may provide a near-term solution to the crisis that has arisen from the global scarcity of 3He by offering a viable alternative to the FM. The prototype detector provides a large-area, efficient, lightweight, more granular neutron responsive detection surface (to facilitate imaging) to ease the application of the new FMs. A novel prototype fission meter is being designed at National Security Technologies, LLC, using a thin uniform coating of 10B as neutron converter (only 1 micron thick) inside a large array of thin (4 mm diameter) copper tubes. The copper tubes are only 2-mil thick, and each holds the stretched anode wire under tension and high voltage. The tubes are filled with proportional counter gas (a mixture of 90% Ar and 10% CO2). The tubes operate in proportional counter mode and attract mobile charged particles (alpha-particles) created in the nuclear interaction 10B(n, a)7Li. Several MCNPX calculations covering the substantial design parameter space of neutron multiplicity detectors have been performed and are presented. Our detector’s thermal neutron detection efficiency is compared to two Ortec commercial products, the Fission Meter and Detective-EX. Pulse height spectra originating from the charged particles created in the nuclear reaction 10B(n, a) 7Li* + 2.310 MeV (94%) – excited state (1) and 10B(n, a) 7Li + 2.792 MeV (6%) – ground state (2) are examined, and the response to incident gamma rays are demonstrated.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Effect of the ultrasonic frequency on the multiple X-ray scattering from a LiNbO{sub 3} crystal modulated by a surface acoustic wave

The effect of multiple scattering on the formation of the {theta}-2{theta} scan curves for a crystal modulated by a surface acoustic wave (SAW), depending on the ultrasonic frequency, has been investigated in the frame-work of the dynamical theory of X-ray diffraction. A model of a Rayleigh surface wave has been analyzed as applied to X-ray diffraction with allowance for the transverse and longitudinal elastic lattice strains. Using the example of the 127 Degree-Sign Y Prime cut of the LiNbO{sub 3} crystal, it is established that the effects of multiple scattering can be neglected for ultrasonic frequencies above 650 MHz; this finding significantly simplifies the numerical calculations of X-ray diffraction from a crystal modulated by a short-wavelength SAW. A comparative quantitative analysis of the experimental data on synchrotron scattering from the 127 Degree-Sign Y Prime cut of a LiNbO{sub 3} crystal modulated by a 952-MHz SAW have been performed, both taking into account and neglecting the effects of multiple scattering. It is shown that the computation time can be reduced by 2 to 3 orders of magnitude.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Simulations of neutron multiplicity measurements with MCNP-PoliMi.

The heightened focus on nuclear safeguards and accountability has increased the need to develop and verify simulation tools for modeling these applications. The ability to accurately simulate safeguards techniques, such as neutron multiplicity counting, aids in the design and development of future systems. This work focuses on validating the ability of the Monte Carlo code MCNPX-PoliMi to reproduce measured neutron multiplicity results for a highly multiplicative sample. The benchmark experiment for this validation consists of a 4.5-kg sphere of plutonium metal that was moderated by various thicknesses of polyethylene. The detector system was the nPod, which contains a bank of 15 3He detectors. Simulations of the experiments were compared to the actual measurements and several sources of potential bias in the simulation were evaluated. The analysis included the effects of detector dead time, source-detector distance, density, and adjustments made to the value of {nu}-bar in the data libraries. Based on this analysis it was observed that a 1.14% decrease in the evaluated value of {nu}-bar for 239Pu in the ENDF-VII library substantially improved the accuracy of the simulation.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

MPACT Fast Neutron Multiplicity System Prototype Development

This document serves as both an FY2103 End-of-Year and End-of-Project report on efforts that resulted in the design of a prototype fast neutron multiplicity counter leveraged upon the findings of previous project efforts. The prototype design includes 32 liquid scintillator detectors with cubic volumes 7.62 cm in dimension configured into 4 stacked rings of 8 detectors. Detector signal collection for the system is handled with a pair of Struck Innovative Systeme 16-channel digitizers controlled by in-house developed software with built-in multiplicity analysis algorithms. Initial testing and familiarization of the currently obtained prototype components is underway, however full prototype construction is required for further optimization. Monte Carlo models of the prototype system were performed to estimate die-away and efficiency values. Analysis of these models resulted in the development of a software package capable of determining the effects of nearest-neighbor rejection methods for elimination of detector cross talk. A parameter study was performed using previously developed analytical methods for the estimation of assay mass variance for use as a figure-of-merit for system performance. A software package was developed to automate these calculations and ensure accuracy. The results of the parameter study show that the prototype fast neutron multiplicity counter design is very nearly optimized under the restraints of the parameter space.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗