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Primary and secondary ice production: interactions and their relative importance

A discrepancy of up to 5 orders of magnitude between ice crystal and ice nucleating particle (INP) number concentrations was found in the measurements, indicating the potentially important role of secondary ice production (SIP) in the clouds. However, the interactions between primary and SIP processes and their relative importance remain unexplored. In this study, we implemented five different ice nucleation schemes as well as physical representations of SIP processes (i.e., droplet shattering during rain freezing, ice-ice collisional break-up, and rime splintering) in the Community Earth System Model version 2 (CESM2). We ran CESM2 in the single column mode for model comparisons with the DOE Atmospheric Radiation Measurement (ARM) Mixed-Phase Arctic Cloud Experiment (M-PACE) observations. We found that the model experiments with aerosol-aware ice nucleation schemes and SIP processes yield the best simulation results for the M-PACE single-layer mixed-phase clouds. We further investigated the relative importance of ice nucleation and SIP to ice number and cloud phase as well as interactions between ice nucleation and SIP in the M-PACE single-layer mixed-phase clouds. Our results show that SIP contributes 80 % to the total ice formation and transforms ~30 % of pure liquid-phase clouds simulated in the model experiments without considering SIP into mixed-phase clouds. The SIP is not only a result of ice crystals produced from ice nucleation, but also competes with the ice nucleation by reducing the number concentrations of cloud droplets and cloud-borne dust INPs. Conversely, strong ice nucleation also suppresses SIP by glaciating mixed-phase clouds and thereby reducing the amount of precipitation particles (rain and graupel).

54 ENVIRONMENTAL SCIENCES↗

Atmosphere-Biosphere Interaction Study (Field Campaign Report)

The objective of this campaign was to collect hyperspectral reflectance measurements and complementary optical and infrared data of land surface (i.e., vegetation and soil) throughout the growing season (i.e., from March to September) at high temporal frequency (e.g., < 30 minutes). To collect the measurements, the EcoSpec system, a tower-based sensor system housing seven optical and infrared sensors that was developed at Argonne National Laboratory, was deployed to the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility Southern Great Plains (SGP) atmospheric observatory (within the crop, south of the eddy correlation flux measurement system [ECOR] tower). The EcoSpec system consists of a spectroradiometer having 2,151 channels (350–2,500 nm), red-greenblue (RGB) camera, diffuse radiometer, thermal infrared (TIR) sensors, albedometers, Photochemical Reflectance Index (PRI) sensors, Normalized Difference Vegetation Index (NDVI) sensors, and wetness sensor. The system is designed to collect an array of land surface measurements, including hyperspectral reflectance of plants and soils, RGB photos capturing contextual information of land surface, radiant temperature of sky and land surface, incoming and reflected shortwave radiation, and incoming radiation components (direct and diffuse) as frequent as every minute from up to 12 discrete positions around the tower. This would allow us to capture inherent heterogeneity of the terrestrial ecosystem and to obtain representative spectral signatures of the plant and soil surfaces via averaging those measurements. The SGP site provides advanced atmospheric and other physical measurements that are essential for our investigation of ecosystem functions using hyperspectral reflectance measurements of land surfaces. Located in the mid-latitudes, the SGP site exhibits dynamic seasonality and a wide range of meteorological variability and flux properties that make it ideal for studying interactions between near-surface atmosphere and biosphere across a range of environmental conditions. The atmosphere, plants, and soil control terrestrial carbon and water cycles. To make more accurate climate forecasts, researchers need to understand ecosystem dynamics at the biosphere–atmosphere interface. Even though our ability to forecast ecosystem dynamics and climate at both the regional and global scales has advanced significantly, we still do not know how local phenomena affecting water and carbon fluxes—such as diurnal variations—interrelate with large-scale atmospheric/climate phenomena, and vice versa. The lack of a more thorough understanding of ecosystem dynamics and climate interactions is a key knowledge gap for the improvement of earth system models (ESMs).

54 ENVIRONMENTAL SCIENCES↗

Solid-State, High Energy 2-Micron Laser Development for Space-Based Remote Sensing

Lidar (light detection and ranging) remote sensing enjoys the advantages of excellent vertical and horizontal resolution; pointing capability; a signal source independent from natural light; and control and knowledge of transmitted wavelength, pulse shape, and polarization and received polarization. Lidar in space is an emerging technology now being developing to fit applications where passive sensors cannot meet current measurement requirements. Technical requirements for space lidar are more demanding than for ground-based or airborne systems. Perhaps the most distinguishing characteristics of space lidars are the environmental requirements. Space lidar systems must be specially designed to survive the mechanical vibration loads of launch and operate in the vacuum of space where exposure to ionizing radiation limits the electronic components available. Finally, space lidars must be designed to be highly reliable because they must operate without the need for repair or adjustment. Lifetime requirements tend to be important drivers of the overall system design. The maturity of the required technologies is a key to the development of any space lidar system. NASA entered a new era in the 1990 s with the approval of several space-based remote sensing missions employing laser radar (lidar) techniques. Following the steps of passive remote sensing and then active radar remote sensing, lidar sensors were a logical next step, providing independence from natural light sources, and better spatial resolution and smaller sensor size than radar sensors. The shorter electromagnetic wavelengths of laser light also allowed signal reflectance from air molecules and aerosol particles. The smaller receiver apertures allowed the concept of scanning the sensor field of view. However, technical problems with several space-based lidar missions during that decade led to concern at NASA about the risk of lidar missions. An external panel was convened to make recommendations to NASA. Their report in 2000 strongly advocated that NASA maintain in-house laser and lidar capability, and that NASA should work to lower the technology risk for all future lidar missions. A multi-Center NASA team formulated an integrated NASA strategy to provide the technology and maturity of systems necessary to make Lidar/Laser systems viable for space-based study and monitoring of the Earth's atmosphere. In 2002 the NASA Earth Science Enterprise (ESE) and Office of Aerospace Technology (OAT) created the Laser Risk Reduction Program (LRRP) and directed NASA Langley Research Center (LaRC) and Goddard Space Flight Center to carry out synergistic and complementary research towards solid-state lasers/lidars developments for space-based remote sensing applications.

Singh, Upendra N.↗

Accelerated Climate Model for Energy (ACME): Ocean and Sea-Ice Processes

The primary goal of this project was to understand the role of the ocean and sea-ice components in the evolution of the climate in both a high-resolution fully-coupled 1850 preindustrial control and present day transient climate simulations run using the Energy Exascale Earth System Model (E3SM), formerly known as the Accelerated Climate Model for Energy (ACME). Two distinct approaches to the initialization of the present day transients were tested: in the first, an ensemble of three transients used atmospheric reanalysis forced 0.1-degree ocean/sea-ice states, while a fourth transient was branched off the preindustrial control. Biases from the control were inherited by its successor transient, in particular, sea surface temperatures (SSTs) at high latitudes were too warm and too much northward meridional heat transport occurred in the North Atlantic Ocean. SSTs in the Northern Hemisphere and Atlantic meridional heat transport increased in the transients initialized from the ocean/sea-ice simulation over a 40-50 year period to largely resemble the transient branched off the control simulation. Excessive absorbed solar radiation (ASR) is considered to be responsible for the SST biases as well as the formation of mode waters in lighter density classes than in reality both in the Southern Ocean and the North Atlantic Ocean subtropical gyre. These mode waters ventilate the thermocline waters to the north of their formation sites explaining the excessive Atlantic meridional heat transport and some of the warming in the high-latitude North Atlantic Ocean after multiple decades.

54 ENVIRONMENTAL SCIENCES↗

Polarity Asymmetries in Rocket‐Triggered Lightning

Abstract The dissonant development of positive and negative lightning leaders is a central question in atmospheric electricity. It is also the likely root cause of other reported asymmetries between positive and negative lightning flashes, including the ones regarding: stroke multiplicity, recoil activity, leader velocities, and emission of energetic radiation. In an effort to contrast lightning leaders of different polarities, we highlight the staggering differences between two rocket‐triggered lightning flashes. The flash beginning with upward positive leaders exhibits an initial continuous current stage followed by multiple sequences of dart leaders and return strokes. On the other, in its opposite‐polarity counterpart, the upward development of negative leaders is by itself the entire flash. As a result, the flash with negative leaders is faster, briefer, transfers less charge to the ground, has lower currents, and smaller spatial extent. We conclude by presenting a discussion on the three fundamental leader propagation modes.

54 ENVIRONMENTAL SCIENCES↗

X-Band CubeSat Communication System Demonstration

Today's CubeSats mostly operate their communications at UHF- and S-band frequencies. UHF band is presently crowded, thus downlink communications are at lower data rates due to bandwidth limitations and are unreliable due to interference. This research presents an end-to-end robust, innovative, compact, efficient and low cost S-band uplink and X-band downlink CubeSat communication system demonstration between a balloon and a Near Earth Network (NEN) ground system. Since communication systems serve as umbilical cords for space missions, demonstration of this X-band communication system is critical for successfully supporting current and future CubeSat communication needs. This research has three main objectives. The first objective is to design, simulate, and test a CubeSat S- and X-band communication system. Satellite Tool Kit (STK) dynamic link budget calculations and HFSS Simulations and modeling results have been used to trade the merit of various designs for small satellite applications. S- and X-band antennas have been tested in the compact antenna test range at Goddard Space Flight Center (GSFC) to gather radiation pattern data. The second objective is simulate and test a CubeSat compatible X-band communication system at 12.5Mbps including S-band antennas, X-band antennas, Laboratory for Atmospheric and Space Physics (LASP) /GSFC transmitter and an S-band receiver from TRL-5 to TRL-8 by the end of this effort. Different X-band communication system components (antennas, diplexers, etc.) from GSFC, other NASA centers, universities, and private companies have been investigated and traded, and a complete component list for the communication system baseline has been developed by performing analytical and numerical analysis. This objective also includes running simulations and performing trades between different X-band antenna systems to optimize communication system performance. The final objective is to perform an end-to-end X-band CubeSat communication system demonstration between a balloon and/or a sounding rocket and a Near Earth Network (NEN) ground system. This paper presents CubeSat communication systems simulation results, analysis of X-band and S-band antennas and RF front-end components, transceiver design, analysis and optimization of space-to-ground communication performance, subsystem development, as well as the test results for an end-to-end X-band CubeSat communication system demonstration. The outcome of this work will be used to pave the way for next generation NEN-compatible X-band CubeSat communication systems to support higher data rates with more advanced modulation and forward error correction (FEC) coding schemes, and to support and attract new science missions at lower cost. It also includes an abbreviated concept of operations for CubeSat users to utilize the NEN, starting from first contact with NASA's communication network and continuing through on-orbit operations.

NEN↗

Understanding Biomass Burning Aerosol via Integrated Analyses of Aerosol Mass Spectrometry Data from DOE Campaigns and ACRF Long Term Measurements

Biomass burning (BB) is one of the largest sources of aerosol particles in the atmosphere and a significant source of trace gases important to atmospheric chemistry. Organic aerosols from biomass burning sources (BBOA) are an important but poorly characterized component of the earth’s climate system. BBOA composition and life cycle processes are associated with enormous complexities and contribute significantly to model uncertainties. Hence it is important to improve the ability to simulate the concentration and properties (chemical, optical, and hygroscopic) of BBOA and the atmospheric aging processes that affect these properties. Here, we propose to analyze ambient data collected from the DOE Biomass Burning Observation Project (BBOP) field campaign and from a long term measurement site of the Atmospheric Radiation Measurement (ARM) program – the Southern Great Plains (SGP), where transported BB plumes and elevated BBOA episodes were frequently observed. This project is aimed at 1) gaining detailed, quantitative understanding of the chemical and physical properties of BBOA and their chemical changes during atmospheric aging via advanced analysis of aerosol measurement data acquired at the summit of Mt. Bachelor (MBO) during the BBOP campaign and through integration with concurrent measurements of trace gases, particle properties, and meteorological conditions performed at MBO and from the G-1 aircraft; 2) gaining better understanding of BBOA properties and its roles in radiative forcing via analysis of routine data from the ARM long-term measurement sites; and 3) integrating the results from 1) and 2) into a global database of aerosol mass spectrometry and collaborate with modelers on evaluating and improving numerical model performance as part of the ASR program.

54 ENVIRONMENTAL SCIENCES↗

2021 Annual Report: Atmospheric Radiation Measurement

In fiscal year 2021 (FY2021), the COVID-19 pandemic continued to have an impact on activities within the Atmospheric Radiation Measurement (ARM) user facility. Travel was limited, which affected field activities and forced the continuation of virtual meetings. However, the ability to travel expanded significantly through the year, bringing some return to normalcy, and throughout the year, there was a great deal of activity dedicated to advancing the facility. Because of COVID, ARM twice delayed the TRacking Aerosol Convection interactions ExpeRiment (TRACER) in the Houston, Texas, area. Originally planned to launch in the spring, TRACER started October 1, 2021, one month after the Surface Atmosphere Integrated Field Laboratory (SAIL) campaign began near Crested Butte, Colorado. ARM teams worked onsite and remotely to make sure both campaigns could launch on this new schedule that was set early in the year. Data from SAIL and TRACER will be critical to improving earth system models, each contributing to different sets of issues. SAIL measurements will provide insights into how precipitation forms and water travels through the Upper Colorado River Basin. TRACER scientists want to know whether tiny atmospheric particles can influence the severity of thunderstorms. In October 2020, the Multidisciplinary Drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition ended after 13 months. MOSAiC data from ARM and other organizations are already helping scientists better understand how ice, atmosphere, and ocean systems are connected in the central Arctic. This report discusses some early investigations from MOSAiC, along with other ARM campaigns and activities generating prolific research. In this report, you will also learn how research activities moved forward during the pandemic at ARM’s fixed-location atmospheric observatories. There were important science applications from measurements across the facility. ARM spent a significant amount of FY2021 looking back—and ahead. In November 2020, ARM had its Triennial Review. This review is held every three years to evaluate ARM’s effectiveness in science, operations, and management. Overall, the reviewers had positive feedback regarding the breadth and impact of science activities using ARM data and the way ARM strives to meet changing user needs. The reviewers also provided some recommendations for strengthening ARM going forward. Incorporating feedback from the review, we finalized an updated Decadal Vision document that will help guide ARM priorities in the coming years. This report describes the four themes driving ARM’s Decadal Vision.

54 ENVIRONMENTAL SCIENCES↗

A review of coarse mineral dust in the Earth system

Mineral dust particles suspended in the atmosphere span more than three orders of magnitude in diameter, from <0.1 µm to more than 100 µm. This wide size range makes dust a unique aerosol species with the ability to interact with many aspects of the Earth system, including radiation, clouds, hydrology, atmospheric chemistry, and biogeochemistry. This review focuses on coarse and super-coarse dust aerosols, which we respectively define as dust particles with a diameter of 2.5–10 µm and 10–62.5 µm. We review several lines of observational evidence indicating that coarse and super-coarse dust particles are transported farther than previously expected and that the abundance of these particles is substantially underestimated in current global models. We synthesize previous studies that used observations, theories, and model simulations to highlight the impacts of coarse and super-coarse dust aerosols on the Earth system, including their effects on dust-radiation interactions, dust-cloud interactions, atmospheric chemistry, and biogeochemistry. Specifically, coarse and super-coarse dust aerosols produce a net positive direct radiative effect (warming) at the top of the atmosphere and can modify temperature and water vapor profiles, influencing the distribution of clouds and precipitation. In addition, coarse and super-coarse dust aerosols contribute a substantial fraction of ice-nucleating particles, especially at temperatures above –23 °C. They also contribute a substantial fraction to the available reactive surfaces for atmospheric processing and the dust deposition flux that impacts land and ocean biogeochemistry by supplying important nutrients such as iron and phosphorus. Furthermore, we examine several limitations in the representation of coarse and super-coarse dust aerosols in current model simulations and remote-sensing retrievals. Because these limitations substantially contribute to the uncertainties in simulating the abundance and impacts of coarse and super-coarse dust aerosols, we offer some recommendations to facilitate future studies. Overall, we conclude that an accurate representation of coarse and super-coarse properties is critical in understanding the impacts of dust aerosols on the Earth system.

54 ENVIRONMENTAL SCIENCES↗

Latest Development in Radiative Transfer Models and Retrieval Algorithms Using Principal Components

The radiative transfer model (RTMs) has a wide range of applications in satellite remote sensing and atmospheric radiation applications. However, millions of line-by-line (LBL) radiative transfer calculations at fine monochromatic frequencies are needed in order to properly calculate spectral contributions of water vapor and trace gases in the atmosphere in infrared and solar spectral regions. Therefore, fast and accurate RTMs are needed to efficiently process large amount of satellite data. A Principal Component-based Radiative Transfer Model (PCRTM) was first developed in 2004 at NASA Langley Research Centre to fulfil this need. By using PC-compression, one can reduce the data dimension significantly while maintaining original information content. The PCRTM can directly compute PC-scores and their derivatives with respect to retrieved parameters. The PCRTM can simulate the top-of-atmosphere (TOA) radiance or reflectance spectra from 0.250 µm (400000 cm-1) to 2000 µm (50 cm-1) with several orders of magnitude faster speed as compared to a LBL RTM. It is also extremely accurate compared to LBL RTM benchmarks (0.03 K RMS error in IR and 0.05% in solar). The PCRTM model has been developed for hyperspectral sensors such as AIRS, CrIS, IASI, NAST-I, SHIS, FIRST, and CLARREO-IR in thermal IR spectral region and CLARREO-Solar, CPF, TEMPO, EMIT, OMI, and SCIAMACHY in solar spectral region. The PCRTM accuracy has been demonstrated via RTM intercomparisons and with real satellite observations from AIRS, CrIS, IASI, SCHIAMACHY, and EMIT etc. In this presentation, we will describe two PCRTM-based inversion algorithms to retrieve atmospheric temperature, water vapor, and trace gas profiles, as well as cloud and surface properties from hyperspectral sounders such as AIRS, CrIS, IASI, and NAST-I. The first one is called Single Fieldof-view Sounder Atmospheric Product (SiFSAP) algorithm. It provides L2 products with 9-times higher area spatial resolution as compared to current cloud-clearing sounder algorithms. The SiFSAP L2 and L3 products are available at NASA's Goddard Earth Sciences Data and Information Services Center (GES DISC) for public access. The second inversion algorithm is called Climate Fingerprinting Atmospheric Product (ClimFiSP) algorithm. It is designed to produce high quality climate products (trends, anomalies, daily, and monthly profiles of temperature, water vapor, traces, clouds, and surface properties) from multiple satellite sensors such AIRS on Aqua and CrIS on multiple satellites. This product will be available at NASA GES DISC later this year. The PCRTMbased high fidelity simulators for CLARREO and CPF have been used for sensor performance trade studies, algorithm development, and inter-satellite calibrations. We have also used PCRTM generated TOA radiance spectra to train an AI-based algorithm and successfully retrieved cloud properties from EMIT solar hyperspectral imagers.

PCRTM↗

Multi-Year Electric Field Study at the North Slope of Alaska (OYESNSA) Field Campaign Report

The Global Electric Circuit (GEC) of the atmosphere provides a unique perspective on Earth’s changing climate. Monitoring this global electrical signature provides details of the global nature of electrified clouds and thunderstorms. The North Slope of Alaska (NSA) is a unique location for collecting these electric field measurements. Besides being at the opposite pole from many previous electric field measurements taken at Russia’s Vostok station in Antarctica, this site provides a rare opportunity to use other instruments at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) User Facility’s NSA observatory at Utqiaġvik (formerly known as Barrow), such as the Ka-band ARM Zenith Radar (KAZR), upward-facing micropulse lidar (MPL), vertical profile of meteorological measures, and other aerosol measurements. Since 2017, Texas A&M University at Corpus Christi (TAMUCC) has established an observational instrument package, including CS110 electric fields and anemometer, at ARM’s NSA observatory at Utqiaġvik. This enabled the unique opportunity to not only provide information about the global signature of the GEC, but also the physical inputs to the local electric field, by analyzing the physical properties of the simultaneous cloud, wind, and aerosol properties occurring with the vertical electric field.

54 ENVIRONMENTAL SCIENCES↗

Multi-Year Electric Field Study at the North Slope of Alaska (OYESNSA) Field Campaign Report

The Global Electric Circuit (GEC) of the atmosphere provides a unique perspective on Earth’s changing climate. Monitoring this global electrical signature provides details of the global nature of electrified clouds and thunderstorms. The North Slope of Alaska (NSA) is a unique location for collecting these electric field measurements. Besides being at the opposite pole from many previous electric field measurements taken at Russia’s Vostok station in Antarctica, this site provides a rare opportunity to use other instruments at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) User Facility’s NSA observatory at Utqiaġvik (formerly known as Barrow), such as the Ka-band ARM Zenith Radar (KAZR), upward-facing micropulse lidar (MPL), vertical profile of meteorological measures, and other aerosol measurements. Since 2017, Texas A&M University at Corpus Christi (TAMUCC) has established an observational instrument package, including CS110 electric fields and anemometer, at ARM’s NSA observatory at Utqiaġvik. This enabled the unique opportunity to not only provide information about the global signature of the GEC, but also the physical inputs to the local electric field, by analyzing the physical properties of the simultaneous cloud, wind, and aerosol properties occurring with the vertical electric field.

54 ENVIRONMENTAL SCIENCES↗

Assessing the climate impact of an improved volcanic sulfate aerosol representation in E3SM

Accurately simulating historical surface temperature variations is essential for evaluating climate models, yet many struggle to reproduce the mid-20th-century temperature trends associated with significant volcanic eruptions. This study examines the impact of volcanic sulfate aerosol representation on these biases using the Energy Exascale Earth System Model (E3SM). The standard CMIP6 protocol prescribes volcanic forcing through radiative perturbations, omitting volcanic aerosol–cloud interactions (VACIs). Here, we implement an emission-based approach with an updated volcanic eruption inventory that directly incorporates volcanic sulfur dioxide (SO 2 ) emissions, enabling a more process-based representation of volcanic forcing. This approach leads to improved surface temperature variability and a modest reduction in cold biases between 1940 and 1980 compared to the CMIP6 setup. Additionally, we assess cloud property responses to a more realistic volcanic sulfate aerosol representation, which weakens cloud-induced cooling during periods of lower volcanic activity. However, despite these refinements, a significant temperature cold bias remains, indicating that further improvements in atmospheric chemistry, aerosol microphysics, cloud processes, and model parameterizations are needed to fully resolve this issue in E3SM.

54 ENVIRONMENTAL SCIENCES↗

HIRM v1.0: a hybrid impulse response model for climate modeling and uncertainty analyses

Simple climate models (SCMs) are frequently used in research and decision-making communities because of their flexibility, tractability, and low computational cost. SCMs can be idealized, flexibly representing major climate dynamics as impulse response functions, or process-based, using explicit equations to model possibly nonlinear climate and Earth system dynamics. Each of these approaches has strengths and limitations. Here we present and test a hybrid impulse response modeling framework (HIRM) that combines the strengths of process-based SCMs in an idealized impulse response model, with HIRM's input derived from the output of a process-based model. This structure enables the model to capture some of the major nonlinear dynamics that occur in complex climate models as greenhouse gas emissions transform to atmospheric concentration to radiative forcing to climate change. As a test, the HIRM framework was configured to emulate the total temperature of the simple climate model Hector 2.0 under the four Representative Concentration Pathways and the temperature response of an abrupt 4 times CO 2 concentration step. HIRM was able to reproduce near-term and long-term Hector global temperature with a high degree of fidelity. Additionally, we conducted two case studies to demonstrate potential applications for this hybrid model: examining the effect of aerosol forcing uncertainty on global temperature and incorporating more process-based representations of black carbon into a SCM. The open-source HIRM framework has a range of applications including complex climate model emulation, uncertainty analyses of radiative forcing, attribution studies, and climate model development.

54 ENVIRONMENTAL SCIENCES↗

Abrupt reduction in shipping emission as an inadvertent geoengineering termination shock produces substantial radiative warming

Abstract Human activities affect the Earth’s climate through modifying the composition of the atmosphere, which then creates radiative forcing that drives climate change. The warming effect of anthropogenic greenhouse gases has been partially balanced by the cooling effect of anthropogenic aerosols. In 2020, fuel regulations abruptly reduced the emission of sulfur dioxide from international shipping by about 80% and created an inadvertent geoengineering termination shock with global impact. Here we estimate the regulation leads to a radiative forcing of $$+0.2\pm 0.11$$ + 0.2 ± 0.11 Wm −2 averaged over the global ocean. The amount of radiative forcing could lead to a doubling (or more) of the warming rate in the 2020 s compared with the rate since 1980 with strong spatiotemporal heterogeneity. The warming effect is consistent with the recent observed strong warming in 2023 and expected to make the 2020 s anomalously warm. The forcing is equivalent in magnitude to 80% of the measured increase in planetary heat uptake since 2020. The radiative forcing also has strong hemispheric contrast, which has important implications for precipitation pattern changes. Our result suggests marine cloud brightening may be a viable geoengineering method in temporarily cooling the climate that has its unique challenges due to inherent spatiotemporal heterogeneity.

54 ENVIRONMENTAL SCIENCES↗

The uncertain role of rising atmospheric CO 2 on global plant transpiration

As CO 2 concentration in the atmosphere rises, there is a need for improved physical understanding of its impact on global plant transpiration. This knowledge gap poses a major hurdle in robustly projecting changes in the global hydrologic cycle. For this reason, here we review the different processes by which atmospheric CO 2 concentration affects plant transpiration, the several uncertainties related to the complex physiological and radiative processes involved, and the knowledge gaps which need to be filled in order to improve predictions of plant transpiration. Additionally, although there is a high degree of certainty that rising CO 2 will impact plant transpiration, the exact nature of this impact remains unclear due to complex interactions between CO 2 and climate, and key aspects of plant morphology and physiology. The interplay between these factors has substantial consequences not only for future climate and global vegetation, but also for water availability needed for sustaining the productivity of terrestrial ecosystems. Future changes in global plant transpiration in response to enhanced CO 2 are expected to be driven by water availability, atmospheric evaporative demand, plant physiological processes, emergent plant disturbances related to increasing temperatures, and the modification of plant physiology and coverage. Considering the universal sensitivity of natural and agricultural systems to terrestrial water availability we argue that reliable future projections of transpiration is an issue of the highest priority, which can only be achieved by integrating monitoring and modeling efforts to improve the representation of CO 2 effects on plant transpiration in the next generation of earth system models.

54 ENVIRONMENTAL SCIENCES↗

Atmospheric Variability Drives Anomalies in the Bering Sea Air–Sea Heat Exchange

Abstract High latitudes, including the Bering Sea, are experiencing unprecedented rates of change. Long-term Bering Sea warming trends have been identified, and marine heatwaves (MHWs), event-scale elevated sea surface temperature (SST) extremes, have also increased in frequency and longevity in recent years. Recent work has shown that variability in air–sea coupling plays a dominant role in driving Bering Sea upper-ocean thermal variability and that surface forcing has driven an increase in the occurrence of positive ocean temperature anomalies since 2010. In this work, we characterize the drivers of the anomalous surface air–sea heat fluxes in the Bering Sea over the period 2010–22 using ERA5 fields. We show that the surface turbulent heat flux dominates the net surface heat flux variability from September to April and is primarily a result of near-surface air temperature and specific humidity anomalies. The airmass anomalies that account for the majority of the turbulent heat flux variability are a function of wind direction, with southerly (northerly) wind advecting anomalously warm (cool), moist (dry) air over the Bering Sea, resulting in positive (negative) surface turbulent flux anomalies. During the remaining months of the year, anomalies in the surface radiative fluxes account for the majority of the net surface heat flux variability and are a result of anomalous cloud coverage, anomalous lower-tropospheric virtual temperature, and sea ice coverage variability. Our results indicate that atmospheric variability drives much of the Bering Sea upper-ocean temperature variability through the mediation of the surface heat fluxes during the analysis period. Significance Statement A long-term ocean warming trend and a recent increase in marine heatwaves in the Bering Sea have been identified. Previous work showed that anomalies in the exchange of heat between the ocean and the atmosphere were the primary driver of Bering Sea temperature variability, but the processes responsible for the heat exchange anomalies were unknown. In this work, we show that the atmosphere is the primary driver of anomalies in the Bering Sea air–sea heat exchange and therefore plays an important role in altering the thermal state of the Bering Sea. Our results highlight the importance of understanding more about how the ocean and the atmosphere interact at high latitudes and how this relationship will be affected by future climate change.

Hayden, Emily E. [a College of Earth, Ocean, and A↗

Rapid SACR Observations of Convection at Bankhead National Forest (RAPID) Field Campaign Report

Improving our representation of convective cell processes requires better quantification of convective clouds throughout their entire life cycle. This includes gaining a clearer understanding of the controls on key convective cloud properties, such as updraft intensity, particle size distributions, rainfall rates, and hydrometeor species. Our inability to improve convective cloud process modeling stems, in part, from a limited understanding of convective cell properties, particularly given how rapidly these storms evolve. This lack of detailed observations in the most intense and organized convective storms is especially significant, as large errors remain in representing these clouds, which are critical for severe weather prediction and Earth system model performance. Cloud and precipitation radars are essential tools for studying cloud microphysics and dynamics, particularly in deeper convective clouds. The recent U.S. Department of Energy Atmospheric Radiation Measurement (ARM) User Facility’s third Mobile Facility (AMF3) Bankhead National Forest (BNF) deployment provides a unique opportunity to investigate important land–atmosphere interactions, as well as the environmental controls on deep convective cloud processes, in a location favorable for frequent convection. We operate the X/Ka-band Scanning ARM Cloud Radar (X/Ka SACR) using a scan strategy optimized to capture these rapidly evolving clouds and their properties, thereby improving studies of deep convective cloud processes. This effort is strengthened by a complementary and coordinated partnership with ongoing university and multi-agency radar activities collocated in north Alabama—a unique opportunity to examine clouds and precipitation from a lifetime-centric perspective.

54 ENVIRONMENTAL SCIENCES↗