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At least 649 records · Page 36

Facile Measurement of the Rotation of a Single Optically Trapped Nanoparticle Using the Diagonal Ratio of a Quadrant Photodiode

Optical tweezers are a powerful tool for exploring physical properties of particles in various environments through analysis of their dynamics in a trapping potential. Analysis of the trapped particle's position is often done using interferometric back-focal-plane detection microscopy in which interference between the trapping laser and the light interacting with the trapped particle is projected on a quadrant photo-diode (QPD). The QPD measurements are almost universally the voltage ratios between the transverse components of the detector (left/right; up/down) that are calibrated to ascertain particle positions and orientations (i.e., rotation). In this paper, we demonstrate how measuring the diagonal ratio of the QPD allows tracking the spinning and orbital motion of optically trapped objects with enhanced sensitivity compared to the conventional transverse ratio and reveals additional information about particle dynamics. The diagonal ratio "balances" the signal from opposite sides of the QPD, allowing common mode noise reduction and increased measurement sensitivity of the rotating nanospheres at frequencies from below 200 Hz to above 15 kHz. We show that the variability in particle rotation rates is due to slight differences in the aspect ratio of the nanoparticles. We also measure in situ a gradual acceleration in the spinning frequency of trapped nanoparticles due to photothermal shedding of surface ligands and the resulting decrease of rotational friction in solution. The accelerating particles spin at rates exceeding 30 kHz and are eventually "optically printed" onto the glass coverslip on top of the liquid cell enclosure. The diagonal ratio is a simple, readily available, and powerful enabler for measuring rotational dynamics with a 5-fold sensitivity increase over conventional QPD measurements. This affords opportunities for controlling the orientational dynamics of trapped nanoparticles, which is crucial for various applications, including nanoscale mechanical motors.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Dynamics of skyrmion contraction and expansion in a magnetic film

Contraction and expansion of skyrmions in ferromagnetic films are investigated. In centrosymmetric systems, the dynamics of a collapsing skyrmion is driven by dissipation. The collapse time has a minimum on the damping constant. In systems with broken inversion symmetry, the evolution of skyrmions toward equilibrium size is driven by the Dzyaloshinskii–Moriya interaction. As a result, expressions describing the time dependence of the skyrmion size are derived and their implications for skyrmion-based information processing are discussed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Covalency in Fe 2 O 3 and FeO: Consequences for XPS satellite intensity

The covalent character of the interaction between the metal cation and the oxygen ligands has been examined for two Fe oxides with different nominal oxidation states, Fe(II)O, and Fe(III) 2 O 3 . The covalent character is examined for the initial, ground state configuration and for the ionic states involving the removal of a shallow core, Fe 3p, and a deep core, Fe 2p, electron. The covalency is assessed based on novel theoretical analyses of wave functions for the various cases. It is found that the covalency is considerably different for different oxidation states and for different ionized and non-ionized configurations. The changes in covalency for the ions are shown to be responsible for important changes in relaxation energies for X-Ray Photoelectron Spectroscopy (XPS) spectra and in the intensity lost from main XPS peaks to shake satellites. While these consequences are not observables themselves, they are important for the interpretation of the XPS spectra, in particular, for efforts to extract stoichiometries of these iron oxides from XPS data. This is a finding likely applicable across various 3d transition metal oxide materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

On the circularly polarized luminescence of individual triplet sublevels

Here, we discuss the possibility of using circularly polarized luminescence (CPL) as a tool to probe individual triplet spin sublevels that are populated nonadiabatically following photoexcitation. This study is motivated by a mechanism proposed for chirality-induced spin selectivity in which coupled electronic-nuclear dynamics may lead to a non-statistical population of the three triplet sublevels in chiral systems. We find that low-temperature CPL should aid in quantifying the exact spin state/s populated through coupled electronic-nuclear motion in chiral molecules.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Laser cooling of atoms at narrow optical transitions in fields with a polarisation gradient

The efficiency of the polarisation mechanisms of laser cooling of atoms is analysed using narrow optical transitions for which the recoil energy is greater than or comparable to the natural line width. By the example of atoms with the J{sub g} = 1 → J{sub e} = 2 optical transition (J{sub g} and J{sub e} are the total angular momenta of the ground and excited states) in the resonant light fields of σ{sub +} – σ{sub –} and lin⊥lin configurations, the analysis of the minimum achievable energies of laser-cooled atoms is performed. It is shown that the polarisation mechanisms of laser cooling under conditions of a significant influence of recoil effects become less efficient and do not lead to average kinetic energies of an ensemble of atoms below the Doppler limit. (paper)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Resonances of electromagnetically induced transparency and absorption in a light field of elliptically polarised waves

Electromagnetically induced transparency (EIT) and electromagnetically induced absorption (EIA) resonances excited by a strong two-frequency field are considered for various values of the total angular momenta of the ground (F{sub g}) and excited (F{sub e}) states at a degenerated optical closed transition F{sub g} → F{sub e}. The light field is formed by two co-propagating waves with arbitrary elliptical polarisations. The process of spontaneous transfer of anisotropy from the excited state to the ground state is shown to determine the formation of the EIA resonance at the transition F{sub g} = F → F{sub e} = F + 1. The results obtained generalise the classification of transitions into ‘bright’ (F{sub g} = F → F{sub e} = F + 1) and ‘dark’ (F{sub g} = F → F{sub e} = F and F{sub g} = F → F{sub e} = F – 1) transitions with respect to the direction of a subnatural resonance. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

The solenoidal large intensity device (SoLID) for JLab 12 GeV

The solenoidal large intensity device (SoLID) is a new experimental apparatus planned for Hall A at the Thomas Jefferson National Accelerator Facility (JLab). SoLID will combine large angular and momentum acceptance with the capability to handle very high data rates at high luminosity. With a slate of approved high-impact physics experiments, SoLID will push JLab to a new limit at the QCD intensity frontier that will exploit the full potential of its 12 GeV electron beam. In this paper, we present an overview of the rich physics program that can be realized with SoLID, which encompasses the tomography of the nucleon in 3D momentum space from semi-inclusive deep inelastic scattering, expanding the phase space in the search for new physics and novel hadronic effects in parity-violating DIS, a precision measurement of J/ψ production at threshold that probes the gluon field and its contribution to the proton mass, tomography of the nucleon in combined coordinate and momentum space with deep exclusive reactions, and more. To meet the challenging requirements, the design of SoLID described here takes full advantage of recent progress in detector, data acquisition and computing technologies. In addition, we outline potential experiments beyond the currently approved program and discuss the physics that could be explored should upgrades of CEBAF become a reality in the future.

3D imaging↗

Precision gyroscope from the helicity of light

We describe a gyroscope that measures rotation based on the effects of the rotation on the polarization of light. Rotation induces a differential phase shift in the propagation of left- and right-circularly polarized light and this phase shift can be measured in suitably designed interferometric setups. The signal in this setup is independent of the frequency of light, unlike various sources of noise such as vibrations, which cause phase shifts that depend on the frequency. Such vibrations are the practical limit on the sensitivity of conventional Sagnac-style optical interferometers that are typically used as gyroscopes. In the proposed setup, one can potentially mitigate this source of noise by simultaneously using two (or more) sources of light that have different frequencies. The signal in this setup scales with the total storage time of the light. Due to its frequency independence, it is thus most optimal to measure the signal using superconducting radio-frequency systems where the high finesse of the available cavities enables considerably longer storage times than is possible in an optical setup.

47 OTHER INSTRUMENTATION↗

Stroboscopic x-ray diffraction microscopy of dynamic strain in diamond thin-film bulk acoustic resonators for quantum control of nitrogen-vacancy centers

Bulk-mode acoustic waves in a crystalline material exert lattice strain through the thickness of the sample, which couples to the spin Hamiltonian of defect-based qubits such as the nitrogen-vacancy (N-V) center defect in diamond. This mechanism has previously been harnessed for unconventional quantum spin control, spin decoherence protection, and quantum sensing. Bulk-mode acoustic wave devices are also important in the microelectronics industry as microwave filters. A key challenge in both applications is a lack of appropriate operando microscopy tools for quantifying and visualizing gigahertz-frequency dynamic strain. Here, in this work, we directly image acoustic strain within N-V center-coupled diamond thin-film bulk acoustic wave resonators using stroboscopic scanning hard x-ray diffraction microscopy at the Advanced Photon Source. The far-field scattering patterns of the nanofocused x-ray diffraction encode strain information entirely through the illuminated thickness of the resonator. These patterns have a real-space spatial variation that is consistent with the bulk strain’s expected modal distribution and a momentum-space angular variation from which the strain amplitude can be quantitatively deduced. We also perform optical measurements of strain-driven Rabi precession of of the N-V center spin ensemble, providing an additional quantitative measurement of the strain amplitude. As a result, we directly measure one of the six N-V spin-stress coupling parameters, 𝑏 =2.73⁢(2) MHz/GPa, by correlating these measurements at the same spatial position and applied microwave power. Our results demonstrate a unique technique for directly imaging ac lattice strain in micromechanical structures and provide a direct measurement of a fundamental constant for the N-V center defect spin Hamiltonian.

acoustic techniques↗

Large inverse Faraday effect for Rydberg states of free atoms and isolated donors in semiconductors

We report on the induction of magnetization in Rydberg systems by means of the inverse Faraday effect and propose the appearance of the effect in two such systems: Rydberg atoms proper and shallow dopants in semiconductors. Rydberg atoms are characterized by a large orbital radius. This large radius gives such excited states a large angular moment, which when driven with circularly polarized light translates to a large effective magnetic field $\mathscr{B}$ eff . We calculate this effect to generate effective magnetic fields of O⁡(1⁢ µ⁢T)×($\frac{ω}{1THz}$) -1 ⁢ ($\frac{\mathscr{I}}{10Wcm^{-2}}$)⁢n 4 in the Rydberg states of atoms such as Rb and Cs for off-resonant photon beams with frequency ω and intensity $\mathscr{I}$ expressed in units of the denominators and n the principal quantum number. Additionally, terahertz spectroscopy of phosphorus-doped silicon reveals a large cross section for excitation of shallow dopants to Rydberg-like states, which even for small n have the potential to be driven similarly with circularly polarized light to produce an even larger magnetization. Our theoretical calculations estimate $\mathscr{B}$ eff as O⁡(10 2 T) for Si:P with a beam intensity of 10 8 Wcm -2 .

36 MATERIALS SCIENCE↗

Many-body effects for the Mg 2s XPS of MgO

The energy separation of the higher lying cation XPS binding energies, BEs, for MgO is examined. It is shown that the Hartree–Fock BEs overestimate the separation of the Mg BE(2s) and BE(2p), because an important many-body effect is neglected in the determination of the Hartree–Fock BEs. Once the many-body effect is taken into account, there is good agreement between theory and the XPS measurement. The character of this atomic many-body effect is established in terms of a nearly degenerate configuration that is needed to describe the wavefunction when an Mg 2s electron is ionized. Further, the results provide additional evidence of the ionic character of the MgO crystal. Given the atomic character of the many-body effect, it is likely to apply also to the BE separations of other closed shell oxides.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

$\gamma$-ray angular correlations, distributions and linear polarization in tracking arrays

With $\gamma $-ray tracking arrays, the angular correlation and, especially, the linear polarization of $\gamma $ rays can be measured with high precision. However, because of the complexity of these spectrometers, measuring angular distributions is more involved. The techniques and associated formalisms were developed and established in the 1950s. The experimental setups of that era were relatively simple when compared to the advanced $\gamma $-ray tracking arrays available today. This paper aims to review and refine these techniques, unify the nomenclatures and, specifically, adapt them for use with the newest tracking arrays. In addition, new methods for producing the required response functions for these arrays are introduced.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗