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NASA NTRS2010

A Global Modeling Study on Carbonaceous Aerosol Microphysical Characteristics and Radiative Effects

Recently, attention has been drawn towards black carbon aerosols as a short-term climate warming mitigation candidate. However the global and regional impacts of the direct, indirect and semi-direct aerosol effects are highly uncertain, due to the complex nature of aerosol evolution and the way that mixed, aged aerosols interact with clouds and radiation. A detailed aerosol microphysical scheme, MATRIX, embedded within the GISS climate model is used in this study to present a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative effects. Our best estimate for net direct and indirect aerosol radiative flux change between 1750 and 2000 is -0.56 W/m2. However, the direct and indirect aerosol effects are quite sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative flux change can vary between -0.32 to -0.75 W/m2 depending on these carbonaceous particle properties at emission. Taking into account internally mixed black carbon particles let us simulate correct aerosol absorption. Absorption of black carbon aerosols is amplified by sulfate and nitrate coatings and, even more strongly, by organic coatings. Black carbon mitigation scenarios generally showed reduced radiative fluxeswhen sources with a large proportion of black carbon, such as diesel, are reduced; however reducing sources with a larger organic carbon component as well, such as bio-fuels, does not necessarily lead to a reduction in positive radiative flux.

Bauer, S. E.↗

NASA NTRS2011

Observational Evidence of Aerosol Enhancement of Lightning Activity and Convective Invigoration

Lightning activity over the West Pacific Ocean east of the Philippines is usually much less frequent than over the nearby maritime continents. However, in 2005 the Lightning Imaging Sensor (LIS) aboard the TRMM satellite observed anomalously high lightning activity in that area. In the same year the Moderate resolution Imaging Spectroradiometer (MODIS) measured anomalously high aerosol loading. The high aerosol loading was traced to volcanic activity, and not to any factor linked to meteorology, disentangling the usual convolution between aerosols and meteorology. We show that in general lightning activity is tightly correlated with aerosol loadings at both inter-annual and biweekly time scales. We estimate that a approximately 60% increase in aerosol loading leads to more than 150% increase in lightning flashes. Aerosols increase lightning activity through modification of cloud microphysics. Cloud ice particle sizes are reduced and cloud glaciation is delayed to colder temperature when aerosol loading is increased. TRMM precipitation radar measurements indicate that anomalously high aerosol loading is associated with enhanced cloud mixed phase activity and invigorated convection over the maritime ocean. These observed associations between aerosols, cloud microphysics, morphology and lightning activity are not related to meteorological variables or ENSO events. The results have important implications for understanding the variability of lightning and resulting aerosol-chemistry interactions.

Yuan, Tianle↗

NASA NTRS2012

Critical Reflectance Derived from MODIS: Application for the Retrieval of Aerosol Absorption over Desert Regions

Aerosols are tiny suspended particles in the atmosphere that scatter and absorb sunlight. Smoke particles are aerosols, as are sea salt, particulate pollution and airborne dust. When you look down at the earth from space sometimes you can see vast palls of whitish smoke or brownish dust being transported by winds. The reason that you can see these aerosols is because they are reflecting incoming sunlight back to the view in space. The reason for the difference in color between the different types of aerosol is that the particles arc also absorbing sunlight at different wavelengths. Dust appears brownish or reddish because it absorbs light in the blue wavelengths and scatters more reddish light to space, Knowing how much light is scattered versus how much is absorbed, and knowin~ that as a function of wavelength is essential to being able to quantify the role aerosols play in the energy balance of the earth and in climate change. It is not easy measuring the absorption properties of aerosols when they are suspended in the atmosphere. People have been doing this one substance at a time in the laboratory, but substances mix when they are in the atmosphere and the net absorption effect of all the particles in a column of air is a goal of remote sensing that has not yet been completely successful. In this paper we use a technique based on observing the point at which aerosols change from brightening the surface beneath to darkening it. If aerosols brighten a surface. they must scatter more light to space. If they darken the surface. they must be absorbing more. That cross over point is called the critical reflectance and in this paper we show that critical reflectance is a monotonic function of the intrinsic absorption properties of the particles. This parameter we call the single scattering albedo. We apply the technique to MODIS imagery over the Sahara and Sahel regions to retrieve the single scattering albedo in seven wavelengths, compare these retrievals to ground-based retrievals from AERONET instruments and compute error bars on each retrieval. The results show that we can retrieve single scattering albedo for pure dust to within +/-0.02 and mixtures of dust and smoke to within +/-0.03. No other space based instrument has achieved a retrieval of single scattering albedo that spans the spectrum from 0.47 microns to 2.13 microns and produces regional maps of aerosol absorption showing gradients and changes. Applied in a more operational fashion, such information will narrow uncertainties in estimating aerosol forcing on climate.

Wells, Kelley C.↗

NASA NTRS2011

Advancements in the Representation of Cloud-Aerosol Microphysics in the GEOS-5 AGCM

Despite numerous challenges, the physical parameterization of cloud-aerosol interactions in atmospheric GCMs has become a top priority for advancement because of our need to simulate and understand past, current, and future indirect effects of aerosols on clouds. The challenges stem from the involvement of wide range of cloud-scale dynamics and aerosol activation physical processes. Cloud dynamics modulate cloud areal extent and condensate, while aerosol activation depends on aerosol mass load, size distribution, internal mixing state, and nucleating properties, and ultimately determines cloud optical properties via particle sizes. Both macro- and micro-scale processes are obviously important for cloud-radiation interactions. We will present the main features of cloud microphysical properties in the GEOS- 5 Atmospheric GCM (AGCM) as simulated by the McRAS-AC (Microphysics of Clouds with Relaxed Arakawa-Schubert and Aerosol-Cloud interaction) scheme. McRAS-AC uses Fountoukis and Nenes (2005) aerosol activation for liquid clouds, and has an option for either Liu and Penner (2005) or Barahona and Nenes (2008, 2009) aerosol activation for ice clouds. Aerosol loading (on-line or climatological) comes from GOCART, with an assumed log-normal size distribution. Other features of McRAS-AC are level-by-level cloud-scale thermodynamics, and Seifert-Beheng (2001)-type precipitation microphysics, particularly from moist convection. Results from Single-Column Model simulations will be shown to demonstrate how cloud radiative properties, lifetimes, and precipitation are influenced by different parameterization assumptions. Corresponding fields from year-long simulations of the full AGCM will also be presented with geographical distributions of cloud effective particle sizes compared to satellite retrievals. While the primary emphasis will be on current climate, simulation results with perturbed aerosol loadings will also be shown to expose the radiative sensitivity of the microphysical parameterization.

Lee, D.↗

NASA NTRS2011

Comment on "'Elevated Heat Pump' Hypothesis for the Aerosol-Monsoon Hydroclimate Link: 'Grounded' in Observations?" by S. Nigam and M. Bollasina

In their recent paper, Nigam and Bollasina [2010] (hereinafter NB) claimed to have found observational evidences that are at variance with the elevated heat pump (EHP) hypothesis regarding the possible impacts of absorbing aerosols on the South Asian summer monsoon [Lau et al., 2006; Lau and Kim, 2006]. We found NB's arguments and inferences against the EHP hypothesis flawed, stemming from their own out of context interpretation of the hypothesis. NB argued that the simultaneous negative correlation of aerosol with rainfall, and correlations with other quantities in May, are evidence against the EHP hypothesis. Their argument cannot be justified. First, Lau and Kim [2006] (hereinafter LK06) never stated that the main rainfall response to EHP is in May. Second, the EHP is about responses of the entire Indian monsoon system that are nonlocal in space and time with respect to the aerosol forcing. As shown in Figure 4 of LK06, while the aerosol anomalies are strongest in April-May, the strongest rainfall response is in June-July, with the enhanced rainfall fed by an induced thermally driven circulation which brings additional moisture from the ocean to the Indian subcontinent. Third, the increased rainfall over the Bay of Bengal as shown in Figure 1a of NB and the increased low-level convergence in Figure 1f of NB do not necessarily reflect responses associated with EHP but rather the large ]scale circulation that provides the buildup of the aerosols before the onset of the monsoon rainfall over India. Because aerosol can only accumulate where there is little or no washout by rain, the negative correlation is a necessary condition for increased atmospheric loading of aerosols. For the same reason, the spatial distributions of rainfall and aerosol generally are offset with each other, i.e., high aerosol in regions of low rainfall. This is evident in Figure 1, which shows the climatological mean of the MODIS aerosol optical depth (AOD), and TRMM rainfall over India in May. The maximum AOD is found over the Indo-Gangetic Plain and the desert regions of northwest India and Pakistan

Lau, K. M.↗

NASA NTRS2012

Satellite-Based Evidence of Wavelength-Dependent Aerosol Absorption in Biomass Burning Smoke Inferred from Ozone Monitoring Instrument

We provide satellite-based evidence of the spectral dependence of absorption in biomass burning aerosols over South America using near-UV measurements made by the Ozone Monitoring Instrument (OMI) during 2005-2007. In the current near-UV OMI aerosol algorithm (OMAERUV), it is implicitly assumed that the only absorbing component in carbonaceous aerosols is black carbon whose imaginary component of the refractive index is wavelength independent. With this assumption, OMI-derived aerosol optical depth (AOD) is found to be significantly over-estimated compared to that of AERONET at several sites during intense biomass burning events (August-September). Other well-known sources of error affecting the near-UV method of aerosol retrieval do not explain the large observed AOD discrepancies between the satellite and the ground-based observations. A number of studies have revealed strong spectral dependence in carbonaceous aerosol absorption in the near-UV region suggesting the presence of organic carbon in biomass burning generated aerosols. A sensitivity analysis examining the importance of accounting for the presence of wavelength-dependent aerosol absorption in carbonaceous particles in satellite-based remote sensing was carried out in this work. The results convincingly show that the inclusion of spectrally-dependent aerosol absorption in the radiative transfer calculations leads to a more accurate characterization of the atmospheric load of carbonaceous aerosols.

Jethva, H.↗

NASA NTRS2012

Comparison of Aerosol Classification From Airborne High Spectral Resolution Lidar and the CALIPSO Vertical Feature Mask

Knowledge of aerosol composition and vertical distribution is crucial for assessing the impact of aerosols on climate. In addition, aerosol classification is a key input to CALIOP aerosol retrievals, since CALIOP requires an inference of the lidar ratio in order to estimate the effects of aerosol extinction and backscattering. In contrast, the NASA airborne HSRL-1 directly measures both aerosol extinction and backscatter, and therefore the lidar ratio (extinction-to-backscatter ratio). Four aerosol intensive properties from HSRL-1 are combined to infer aerosol type. Aerosol classification results from HSRL-1 are used here to validate the CALIOP aerosol type inferences.

Burton, Sharon P.↗

NASA NTRS2009

Case Studies of Aerosol Remote Sensing in the Vicinity of Clouds

Studying the spatial variability of aerosol properties in the vicinity of clouds is essential to our ability to determine aerosol direct and indirect effects on climate. In this paper, we describe aerosol observations collected near cloud edges by an airborne Sun photometer over dark ocean waters. Focusing on case studies of aerosol measurements near eight cloud edges within a dissipating stratiform cloud deck, we compare the airborne Sun photometer observations to retrievals of aerosol properties using the standard Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol algorithm applied to 500-m-resolution MODIS spectral reflectances. We find a persistent, spectrally neutral increase in the Sun photometer-derived aerosol optical depth (AOD) of up to 10% (0.015) in the 2-km distances closest to the edges of several distinct clouds. At midvisible wavelengths, the MODIS AOD retrievals show similar increases toward cloud edges, although a larger increase in AOD is found in the MODIS along-scan direction. At shortwave infrared (SWIR) wavelengths (1240-2130 nm), the MODIS-derived AOD increases near cloud edges are of the order of 0.03 and as such three times as large as the Sun photometer-derived values. Hence, in contrast to recently discussed bluing of aerosols near cloud edges, i.e., a preferential apparent increase in the visible reflectances of clear-sky pixels due to 3-D radiative transfer effects in the vicinity of clouds, we find a reddening of aerosols in the MODIS 500-m-resolution aerosol retrievals near clouds. This reddening in our study can be traced to larger absolute increases in SWIR reflectances when compared to visible reflectances near clouds, which in turn seem to stem from larger electronic cross talk in the MODIS SWIR bands (5-7). We note that the lack of bluing in our MODIS observations is likely due to the small geometric and optical thicknesses of the clouds considered.

Redemann, Jens↗

NASA NTRS1973

Comparison of Lidar and In-Situ Measurements of Stratospheric Aerosols

This paper will present the results of a comparative study conducted in Laramie, Wyoming, during the summer and fall of 1972, as part of the Department of Transportation's Climatic Impact Assessment Program (ClAP). The study included independent, and nearly simultaneous, measurements of stratospheric aerosols using a LIDAR system and a balloon-borne in-situ particle counter. The LIDAR provides a remote measurement of volume backscatter (aerosols and molecules) in a narrow wavelength region centered at the ruby wavelength (6943R); whereas the balloon-borne in-situ counter measures aerosol concentration by counting aerosols greater than approx. 0.30 microns in diameter as they are pumped through a chamber and scatter white light forward into photo-detectors. The comparison of measurements that will be discussed using the two techniques involves formulating the LIDAR data so that it is compatible with the counter data. The formulation includes separation of the scattering due to aerosols from the total and displaying this in terms of aerosol scattering function. Aerosol scattering function is proportional to aerosol concentration if the aerosol parameters, such as size distribution and composition, are constant with altitude. In separating the aerosol scattering from the total, the need for real atmospheric number density over the Standard Atmosphere is also discussed.

Melfi, S. H.↗

NASA NTRS2016

Validation and Expected Error Estimation of Suomi-NNP VIIRS Aerosol Optical Thickness and Angstrom Exponent with AERONET

The new-generation polar-orbiting operational environmental sensor, the Visible Infrared Imaging Radiometer Suite (VIIRS) on board the Suomi National Polar-orbiting Partnership (S-NPP) satellite, provides critical daily global aerosol observations. As older satellite sensors age out, the VIIRS aerosol product will become the primary observational source for global assessments of aerosol emission and transport, aerosol meteorological and climatic effects, air quality monitoring, and public health. To prove their validity and to assess their maturity level, the VIIRS aerosol products were compared to the spatiotemporally matched Aerosol Robotic Network (AERONET)measurements. Over land, the VIIRS aerosol optical thickness (AOT) environmental data record (EDR) exhibits an overall global bias against AERONET of 0.0008 with root-mean-square error(RMSE) of the biases as 0.12. Over ocean, the mean bias of VIIRS AOT EDR is 0.02 with RMSE of the biases as 0.06.The mean bias of VIIRS Ocean Angstrom Exponent (AE) EDR is 0.12 with RMSE of the biases as 0.57. The matchups between each product and its AERONET counterpart allow estimates of expected error in each case. Increased uncertainty in the VIIRS AOT and AE products is linked to specific regions, seasons, surface characteristics, and aerosol types, suggesting opportunity for future modifications as understanding of algorithm assumptions improves. Based on the assessment, the VIIRS AOT EDR over land reached Validated maturity beginning 23 January 2013; the AOT EDR and AE EDR over ocean reached Validated maturity beginning 2 May 2012, excluding the processing error period 15 October to 27 November 2012. These findings demonstrate the integrity and usefulness of the VIIRS aerosol products that will transition from S-NPP to future polar-orbiting environmental satellites in the decades to come and become the standard global aerosol data set as the previous generations missions come to an end.

Huang, Jingfeng↗

NASA NTRS2018

Improving the Performance of the OMPS Limb Profiling Instrument in Monitoring Aerosols in the Post-Pinatubo Stratosphere

The OMPS Limb Profiling (LP) instrument was launched on NOAA's Suomi NPP (SNPP) weather satellite in October 2011. The instrument measures limb-scattered radiation in the ultraviolet, visible and NIR wavelengths with high vertical resolution (~2 km) and relatively dense spatial and temporal sampling (several thousand measurements/day covering the entire sunlit globe). These measurements have very high sensitivity to stratospheric aerosols due to long path of the incoming solar photons through the aerosol layer. However, unlike the recently launched ISS/SAGE III that directly measures extinction of solar/lunar radiation by gases and particles along the line of sight (LOS) of the instrument, information content of OMPS LP measurements is complex. It consists of solar radiation singly scattered and attenuated by aerosols, air, and trace gases along the LOS of the instrument, as well as diffuse upwelling radiation from the lower atmosphere that also gets scattered and attenuated into the LOS. To unscramble this complex signal one needs to have good knowledge of aerosol size distribution (ASD) and their complex refractive index. We will describe our recent efforts in constraining the ASD parameters by analyzing in-situ balloon data from Laramie, Wyoming; aerosol microphysical model data from CARMA; and spectral information provided by OMPS LP. We will also discuss our proposed methodology to reï¬ne this information by adjusting the microphysical properties of the aerosols to make data from various occultation and scattering instruments internally consistent. This is a generalized version of the technique employed by AERONET in which solar extinction data are combined with scattered radiation measured by the almucantar technique to determine aerosol particle shape, complex refractive index and size distribution. We suggest that such closure studies are essential to develop confidence in space-based data to validate aerosol microphysical models, such as CARMA, and aerosol chemistry- transport models, such as GOCART, and for estimating radiative forcing due to stratospheric aerosols in both volcanic and quiescent time periods.

Bhartia, P. K.↗

NASA NTRS2018

Results from ORACLES-2016: Observed Biomass Burning Aerosol Properties over the Southeast Atlantic Ocean and the Relationship to Meteorology

The Southeast Atlantic Ocean (SEA), with seasonal biomass burning (BB) smoke plumes overlying persistent stratocumulus cloud deck, offers an excellent natural laboratory to make the observations necessary to understand the complexities of aerosol-cloud-radiation interactions. The first field deployment of the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) campaign was conducted in September of 2016 out of Walvis Bay, Namibia. During this deployment, two NASA aircraft (a P-3 and an ER-2) were flown with a suite of aerosol, cloud, radiation, and meteorological instruments for remote-sensing and in-situ observations. In this talk, I will first present results from an intercomparison of the different instrument retrievals for the 2016 flights, with a specific focus on the measures of aerosol absorption. In ORACLES, data collected by eight different instrument teams are used to derive aerosol properties over this region by independent methods. We focus on the single scattering albedo (SSA), a measure of the relative absorption versus total extinction by aerosols, as the main comparable property between all methods. I will also discuss comparisons of the retrieved aerosol absorption parameters, as well as the agreement and the variability seen between different instruments, and spatially over the study region. Another important factor in understanding aerosol radiative effects is how the magnitude of these effects may be modified by meteorological conditions. I will next describe observations collected from the P-3 aircraft (from near-surface up to 6-7 kilometers) which show a strong correlation between the in-situ pollution indicators (carbon monoxide and aerosol properties) and atmospheric water vapor content, seen at all altitudes above the boundary layer. This condition is seen to persist over all flights, with minimal detrainment during advection from the continental source. In exploring the potential causal factors behind and implications of this relationship, we see indications that convective dynamics over the continent likely contribute to this elevated signal, but neither meteorological reanalysis nor trajectory analysis fully capture the magnitude and vertical structure of the observed elevated signal. Finally, I will discuss the radiative implications of the observed correlations, a topic of ongoing analysis in ORACLES: understanding the mechanisms which cause water vapor to covary with plume strength is important to quantifying the radiative effects (direct and semi-direct) of biomass burning aerosol in the region.

Pistone, Kristina↗

NASA NTRS2018

CALIPSO Lidar Level 3 Aerosol Profile Product: Version 3 Algorithm Design

The CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) level 3 aerosol profile product reports globally gridded, quality-screened, monthly mean aerosol extinction profiles retrieved by CALIOP (the Cloud-Aerosol Lidar with Orthogonal Polarization). This paper describes the quality screening and averaging methods used to generate the version 3 product. The fundamental input data are CALIOP level 2 aerosol extinction profiles and layer classification information (aerosol, cloud, and clear-air). Prior to aggregation, the extinction profiles are quality-screened by a series of filters to reduce the impact of layer detection errors, layer classification errors, extinction retrieval errors, and biases due to an intermittent signal anomaly at the surface. The relative influence of these filters are compared in terms of sample rejection frequency, mean extinction, and mean aerosol optical depth (AOD). The “extinction QC flag” filter is the most influential in preventing high-biases in level 3 mean extinction, while the “misclassified cirrus fringe” filter is most aggressive at rejecting cirrus misclassified as aerosol. The impact of quality screening on monthly mean aerosol extinction is investigated globally and regionally. After applying quality filters, the level 3 algorithm calculates monthly mean AOD by vertically integrating the monthly mean quality-screened aerosol extinction profile. Calculating monthly mean AOD by integrating the monthly mean extinction profile prevents a low bias that would result from alternately integrating the set of extinction profiles first and then averaging the resultant AOD values together. Ultimately, the quality filters reduce level 3 mean AOD by −24 and −31 % for global ocean and global land, respectively, indicating the importance of quality screening.

Tackett, Jason L.↗

NASA NTRS2019

Can OMPS and VIIRS Be Used as a Single Virtual Sensor for Aerosol Retrieval?

Satellite earth observation of aerosols using a single sensor have been done for more than three decades. The retrieved global distribution of column integrated aerosol optical depth (AOD) has been refined with higher accuracy and finer resolutions. However, the other aerosol properties, such as aerosol absorption and aerosol height, haven not been mapped as extensively using passive sensors. The detectors sensitive to these properties (UV-based sensors such as Aura-OMI) lack the adequate visible channels to tease out the absorption, height and loading contributions. In addition, their spatial resolution is prone to frequent cloud contamination impacting aerosol loading retrievals using only these spectral ranges. However, the deployment of the VIIRS and OMPS-NM sensors on the same Suomi NPP platform provides a first opportunity to carry out retrievals of aerosol single scattering albedo (SSA) and AOD with little cloud contamination using an expanded spectral range from the UV to the near-IR wavelengths. After collocated VIIRS pixel within the large OMPS footprint during the high resolution OMPS observing mode, we compared the radiance from OMPS and VIIRS to ensure the calibration from individual sensors are comparable. Then a look up table (LUT) was created for a smoke case over central Africa. The LUT is generated using 10 channels from 0.357 to 2.1 micron with 44 combinations of aerosol models and 4 different aerosol heights. With CALIOP and AERONET observation nearby, the possibility of using OMPS and VIIRS radiance as a single virtual sensor to simultaneously and consistently retrieve AOD, SSA, and aerosol height is explored.

Shi, Yingxi↗

NASA NTRSDate not supplied

HSRL-2 Observations of Aerosol Variability and Mixing During Boundary Layer Evolution in Houston

The NASA Langley airborne multi-wavelength High Spectral Resolution Lidar (HSRL-2) provides vertical distribution of aerosol optical properties as ?curtains? of aerosol extinction, backscatter and depolarization along the flight track, plus intensive properties that are used to infer aerosol type and external mixing of types. Deployed aboard the NASA Langley King Air on the DISCOVER-AQ field mission in Houston in September 2013, HSRL-2 flew a pattern that included 18 ground sites, repeated four times a day, coordinated with a suite of airborne in situ measurements. The horizontally and vertically resolved curtains of HSRL-2 measurements give an unparalleled view of the spatial and temporal variability of aerosol, which provide broad context for interpreting other measurements and models. In Houston, HSRL-2 generally observed significant variability with distinct layering: boundary layer, residual layer, and frequent upper layers of smoke transported from the Mississippi Valley. The period from Sep. 11-14 is notable for a large aerosol build-up and persistent layers in the free troposphere. We investigate the aerosol properties and evolution using the vertically resolved HSRL-2 measurements, typing and mixture analysis techniques, and boundary layer detection. Between morning and afternoon overpasses, as the boundary layer grows, many distinctions between the layers are lost as the aerosols become mixed. As the boundary layer collapses overnight, the aerosols are cut off and are observed in a distinct residual layer the following day. HSRL-2 measurements of the upper smoke layers suggest slightly different properties each day as new smoke enters the region, while the morning boundary layer indicates more similarity in local emissions day-to-day. HSRL-2 intensive variables (indicators of aerosol type) reflect complex yet predictable mixing. We will present the analysis of aerosol mixtures, and explore the WRF-Chem chemical transport model along the HSRL-2 flight path.

Sharon P Burton↗

NASA NTRSDate not supplied

An Optimal Estimation Aerosol Retrieval Algorithm for Lidar-only and Combined Lidar Polarimeter Remote Sensors

Global measurements of aerosol vertical profile, composition, concentration, and size distribution are very important due to aerosol impacts on air quality, climate, clouds, and ocean ecosystems. We have developed a lidar-only and combined lidar and polarimeter algorithm to retrieve vertically-resolved profiles of aerosol microphysical properties. The new retrieval system is modular in design. It consists of three modules, a vertically-resolved aerosol profile retrieval module for lidar data, an aerosol and cloud/ocean retrieval module for polarimeter data, and a combined retrieval module for both lidar and polarimeter measurements. In addition to performing optimal estimation retrievals on various data sources, we have designed the system so that it can be used to carry out aerosol retrieval performance trade studies for various lidar and polarimeter configurations. For example, the retrieval system can take inputs from attenuated backscatter lidar at two wavelengths (e.g. CALIPSO like instrument), aerosol backscattering measured at two wavelengths and and aerosol extinction measured at one wavelength (HSRL-1), or aerosol backscattering measured at three wavelengths and aerosol extinction measured at two wavelengths (HSRL-1) (HSRL-2). We have applied the lidar-only algorithm to both simulated data and various field campaign data (DISCOVER-AQ, CHARMS, TCAP, and ORACLES). For polarimeter-only modules, we have done the same for SABOR, TCAP, NAAMES, and ORACLES data. We have applied the combined retrieval algorithm to ORACLES data. The simulated retrieval studies show that the combined lidar+polarimeter retrieval provides much higher information content relative to their individual counterparts for retrieving effective radius, particle concentrations, and absorption properties.

Xu Liu↗

NASA NTRSDate not supplied

Excessive Subsidence of the Southeast Atlantic Biomass Burning Aerosol Plume in the NASA Goddard Earth Observing System (GEOS) Model

Global models struggle to accurately represent the meteorological environment over the Southeast Atlantic Ocean, as evidenced by the poor representation of persistent marine stratocumulus decks off the west coast of southern Africa. This complex regime also experiences significant seasonal biomass burning aerosol plumes that are transported from southern Africa over the Atlantic Ocean, which gradually descend via large scale subsidence and interact radiatively and microphysically with the cloudy environment of the region. In comparisons to space borne lidar and aircraft observations we find that the NASA Goddard Earth Observing System (GEOS) model’s MERRA-2 aerosol and meteorology reanalysis shows that the aerosol plume descends too rapidly due to exaggerated large-scale downward vertical motion. This complicates the evaluation of aerosol properties utilizing aircraft observations collected throughout the ORACLES campaign as well as the model’s representation of the heating rate profiles due to the aerosol itself and its radiative interaction with the semi-permanent cloud deck typically located lower in altitude than the smoke. Two types of modeling experiments using GEOS will be presented to diagnose deficiencies in the model related to the excessive subsidence. Ensembles of free-running model simulations with and without radiatively active biomass burning aerosol will be used to quantify the impact of smoke on the atmospheric circulation. It will be demonstrated that heating within the aerosol layer results in self lofting through a reduction of the subsidence but did not alter the vertical placement or speed of the African Easterly jet. The amount of aerosol absorption required to eliminate the bias in the height of the aerosol plume through self-lofting will then be quantified. Finally, a second type of modeling experiment will be discussed in which the meteorology is constrained to observations. This will allow for biases in the height of the aerosol plume due to the general circulation model to be distinguished from biases that may be induced through the data assimilation process.

Allison Collow↗

NASA NTRSDate not supplied

Creating Seasonal Climatologies of Aerosol Lidar Ratios Over Ocean Using MODIS AOD Constrained Retrievals and GOCART Model Simulations

The current CALIPSO algorithms assign one lidar ratio (i.e., extinction-to-backscatter ratio; LR) value globally for each of the seven tropospheric aerosol types. In a future data products release, the CALIPSO project aims to improve these algorithms through the development of regional and seasonal LR climatologies. In this work, aerosol LRs are inferred through CALIOP backscatter profiles constrained by collocated aerosol optical depth (AOD) from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) data. This analysis is subsampled for those profiles that are cloud-free and contain only one CALIOP-classified aerosol type (e.g., marine). The CALIOP profiles are then collocated with aerosol volume fractions obtained through Goddard Chemistry Aerosol Radiation and Transport (GOCART) model simulations. In this poster, we show twelve-year (June 2006-August 2018) mean spatial distributions of inferred aerosol LRs for CALIOP-classified marine aerosols and how they correspond inversely with patterns of GOCART sea salt volume fraction (SSVF). Near land masses, smaller SSVFs and larger LRs are found (due to the influence of over-land aerosols). In the remote ocean regions (likely less impacted by over-land aerosols), larger SSVFs and smaller LRs are found. The developed relationship between the GOCART model SSVFs and MODIS AOD constrained LRs is used to create model-assisted seasonal LR maps. Additionally, we show maps of inferred LRs from constrained retrievals using the CALIPSO Ocean Derived Column Optical Depth (ODCOD) product and comparisons with those from the MODIS analyses. The technique demonstrated here benefits CALIPSO in the near-term, but similar methods can also be applied to the next generation space-based elastic backscatter lidars with collocated passive sensors, such as those of the upcoming NASA Atmosphere Observing System (AOS).

Travis Toth↗