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At least 631 records · Page 35
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Anthracene clusters and the interstellar infrared emission features

The unidentified infrared bands are ubiquitous in the interstellar medium and typically attributed to emission from neutral and ionized polycyclic aromatic hydrocarbons (or PAHs). The contribution of neutral PAH clusters to these bands has been impossible to determine due to a paucity of infrared spectral data. Here we investigated neutral clusters of the three-ring PAH anthracene using FTIR absorption spectroscopy of anthracene matrix-isolated at varying concentrations in solid argon. In order to determine likely cluster structures of the embedded molecules, we also calculated theoretical absorption spectra for the anthracene monomer through hexamer using density functional theory with a dispersion correction (DFT-D). The DFT-D calculations have been calibrated for the anthracene dimer using the second-order Møller-Plesset approach. Because there is some support for the hypothesis that three or four-ring PAHs are present in the Red Rectangle nebula, we discuss the application of our results to this nebula in particular as well as to the interstellar infrared emission in general.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

First time-dependent study of H{sub 2} and H{sub 3}{sup +} ortho-para chemistry in the diffuse interstellar medium: Observations meet theoretical predictions

The chemistry in the diffuse interstellar medium (ISM) initiates the gradual increase of molecular complexity during the life cycle of matter. A key molecule that enables build-up of new molecular bonds and new molecules via proton donation is H{sub 3}{sup +}. Its evolution is tightly related to molecular hydrogen and thought to be well understood. However, recent observations of ortho and para lines of H{sub 2} and H{sub 3}{sup +} in the diffuse ISM showed a puzzling discrepancy in nuclear spin excitation temperatures and populations between these two key species. H{sub 3}{sup +}, unlike H{sub 2}, seems to be out of thermal equilibrium, contrary to the predictions of modern astrochemical models. We conduct the first time-dependent modeling of the para-fractions of H{sub 2} and H{sub 3}{sup +} in the diffuse ISM and compare our results to a set of line-of-sight observations, including new measurements presented in this study. We isolate a set of key reactions for H{sub 3}{sup +} and find that the destruction of the lowest rotational states of H{sub 3}{sup +} by dissociative recombination largely controls its ortho/para ratio. A plausible agreement with observations cannot be achieved unless a ratio larger than 1:5 for the destruction of (1, 1)- and (1, 0)-states of H{sub 3}{sup +} is assumed. Additionally, an increased cosmic-ray ionization rate to 10{sup –15} s{sup –1} further improves the fit whereas variations of other individual physical parameters, such as density and chemical age, have only a minor effect on the predicted ortho/para ratios. Thus, our study calls for new laboratory measurements of the dissociative recombination rate and branching ratio of the key ion H{sub 3}{sup +} under interstellar conditions.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Ulysses observations of magnetic waves due to newborn interstellar pickup ions. II. Application of turbulence concepts to limiting wave energy and observability

The low-frequency magnetic waves that arise from the isotropization of newborn interstellar pickup ions (PUIs) are reasonably well described by linear and quasi-linear kinetic theory in so far as those theories predict the wave frequency and polarization in the spacecraft frame. Those theories fail to describe the scarce observability of the waves. Quasilinear theory predicts that the wave power should accumulate over long periods of time as the relatively weak kinetic instability slowly adds power to the observed spectrum. At the same time it has been argued that the same wave energy must serve as a secondary source of thermal ion heating in the outer heliosphere once the initial turbulence is depleted. To the extent that turbulent transport of the wave energy acts against the spectrally confined accumulation of wave energy, turbulence should be a limiting factor in observability. We argue that turbulence does limit the observability of the waves and we use turbulence theory to predict the observed wave energy. We compare this prediction against a database of 502 wave observations attributed to newborn interstellar PUIs observed by the Ulysses spacecraft.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Interstellar scintillation of the double pulsar J0737–3039

We report a series of observations of the interstellar scintillation (ISS) of the double pulsar J0737–3039 over the course of 18 months. As in earlier work, the basic phenomenon is the variation in the ISS caused by the changing transverse velocities of each pulsar, the ionized interstellar medium (IISM), and the Earth. The transverse velocity of the binary system can be determined both by very long baseline interferometry and timing observations. The orbital velocity and inclination is almost completely determined from timing observations, but the direction of the orbital angular momentum is not known. Since the Earth's velocity is known, and can be compared with the orbital velocity by its effect on the timescale of the ISS, we can determine the orientation Ω of the pulsar orbit with respect to equatorial coordinates (Ω = 65 ± 2°). We also resolve the ambiguity (i = 88.°7 or 91.°3) in the inclination of the orbit deduced from the measured Shapiro delay by our estimate i = 88.°1 ± 0.°5. This relies on the analysis of the ISS over both frequency and time, and provides a model for the location, anisotropy, turbulence level, and transverse phase gradient of the IISM. We find that the IISM can be well-modeled during each observation, typically of a few orbital periods, but its turbulence level and mean velocity vary significantly over the 18 months.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Paramagnetic alignment of small grains: A novel method for measuring interstellar magnetic fields

We present a novel method to measure the strength of interstellar magnetic fields using ultraviolet (UV) polarization of starlight that is in part produced by weakly aligned, small dust grains. We begin with calculating the degrees of the paramagnetic alignment of small (size a ∼ 0.01 μm) and very small (a ∼ 0.001 μm) grains in the interstellar magnetic field due to the Davis-Greenstein relaxation and resonance relaxation. To calculate the degrees of paramagnetic alignment, we use Langevin equations and take into account various interaction processes essential for the rotational dynamics of small grains. We find that the alignment of small grains is necessary to reproduce the observed polarization in the UV, although the polarization arising from these small grains is negligible at the optical and infrared (IR) wavelengths. Based on fitting theoretical models to observed extinction and polarization curves, we find that the best-fit model for the case with the peak wavelength of polarization λ{sub max} < 0.55 μm requires a higher degree of alignment of small grains than for the typical case with λ{sub max} = 0.55 μm. We interpret the correlation between the systematic increase of the UV polarization relative to maximum polarization (i.e., of p(6 μm{sup –1})/p{sub max}) with λ{sub max}{sup −1} for cases of low λ{sub max} by appealing to the higher degree of alignment of small grains. We utilize the correlation of the paramagnetic alignment of small grains with the magnetic field strength B to suggest a new way to measure B using the observable parameters λ{sub max} and p(6 μm{sup –1})/p{sub max}.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

A theoretical study on the interstellar synthesis of H{sub 2}NCS{sup +} and HNCSH{sup +} cations

HNCS and NCSH molecules, recently discovered in the interstellar medium, are likely formed via the dissociative recombination of H{sub 2}NCS{sup +} or HNCSH{sup +} isomeric ions. Interstellar synthesis of the latter is discussed on theoretical grounds. The analysis of relevant potential energy surfaces suggests a key role for chemical processes in which CSH{sup +} or HCS{sup +} cations (most likely formed in CS+H{sub 3}{sup +} collisions) react with NH{sub 2} or NH{sub 3}. The astrochemical kinetic database (kida.uva.2011), appended with 7 sulfur-bearing molecules and 48 corresponding reactions, has been applied to model the evolution of HNCS, NCSH, and their cationic precursors in a quiescent molecular cloud. Based on the model and on spectroscopic predictions, for an object like TMC-1, we expect the total intensity of H{sub 2}NCS{sup +} microwave lines to be comparable to that observed for HSCN. Theoretically derived molecular parameters, of interest for radio spectroscopy, are given for the most stable cations sharing the H{sub 2}NCS{sup +} stoichiometry.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

A high-resolution study of near-infrared diffuse interstellar bands

We present high-resolution echelle spectroscopic observations of the two near-infrared (NIR) diffuse interstellar bands (DIBs) at 13175 Å and 11797.5 Å. The DIBs have been observed in a number of diffuse interstellar medium sightlines that exhibit a wide range of visual extinctions. Band profiles are similar to those seen in narrow DIBs, clearly asymmetric and can be closely fitted in most cases using two simple Gaussian components. Gaussian fits were generally found to be more successful than fits based on a multiple-cloud model using a template DIB profile. For a sample of nine objects in which both bands are observed, the strength of both NIR DIBs generally increases with A(V), and we report a correlation between the two observed bands over a large A(V) range and widely separated lines of sight. The strength of the two bands is also compared against those of two visual DIBs and the diffuse ISM aliphatic dust absorption feature at 3.4 μm previously detected in the same sightlines. We find that the NIR DIBs do not exhibit notable (anti)correlations with either. Implications of these observations on possible DIB carrier species are discussed.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

BENZENE FORMATION ON INTERSTELLAR ICY MANTLES CONTAINING PROPARGYL ALCOHOL

Propargyl alcohol (CHCCH{sub 2}OH) is a known stable isomer of the propenal (CH{sub 2}CHCHO) molecule that was reported to be present in the interstellar medium (ISM). At astrochemical conditions in the laboratory, icy layers of propargyl alcohol grown at 85 K were irradiated by 2 keV electrons and probed by a Fourier Transform InfraRed spectrometer in the mid-infrared (IR) region, 4000-500 cm{sup –1}. Propargyl alcohol ice under astrochemical conditions was studied for the first time; therefore, IR spectra of reported amorphous (85 K) and crystalline (180 K) propargyl alcohol ices can be used to detect its presence in the ISM. Moreover, our experiments clearly show benzene (C{sub 6}H{sub 6}) formation to be the major product from propargyl alcohol irradiation, confirming the role of propargyl radicals (C{sub 3}H{sub 3}) formed from propargyl alcohol dissociation that was long expected based on theoretical modeling to effectively synthesize C{sub 6}H{sub 6} in the interstellar icy mantles.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

THE INFLUENCE OF SUPERNOVA REMNANTS ON THE INTERSTELLAR MEDIUM IN THE LARGE MAGELLANIC CLOUD SEEN AT 20-600 μm WAVELENGTHS

We present the analysis of supernova remnants (SNRs) in the Large Magellanic Cloud (LMC) and their influence on the environment at far-infrared (FIR) and submillimeter wavelengths. We use new observations obtained with the Herschel Space Observatory and archival data obtained with the Spitzer Space Telescope, to make the first FIR atlas of these objects. The SNRs are not clearly discernible at FIR wavelengths; however, their influence becomes apparent in maps of dust mass and dust temperature, which we constructed by fitting a modified blackbody to the observed spectral energy distribution in each sightline. Most of the dust that is seen is pre-existing interstellar dust in which SNRs leave imprints. The temperature maps clearly reveal SNRs heating surrounding dust, while the mass maps indicate the removal of 3.7{sub −2.5}{sup +7.5} M {sub ☉} of dust per SNR. This agrees with the calculations by others that significant amounts of dust are sputtered by SNRs. Under the assumption that dust is sputtered and not merely pushed away, we estimate a dust destruction rate in the LMC of 0.037{sub −0.025}{sup +0.075} M {sub ☉} yr{sup –1} due to SNRs, yielding an average lifetime for interstellar dust of 2{sub −1.3}{sup +4.0}×10{sup 7} yr. We conclude that sputtering of dust by SNRs may be an important ingredient in models of galactic evolution, that supernovae may destroy more dust than they produce, and that they therefore may not be net producers of long lived dust in galaxies.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

THE COMPOSITION OF INTERSTELLAR GRAINS TOWARD ζ OPHIUCHI: CONSTRAINING THE ELEMENTAL BUDGET NEAR THE DIFFUSE-DENSE CLOUD TRANSITION

We investigate the composition of interstellar grains along the line of sight toward ζ Ophiuchi, a well-studied environment near the diffuse-dense cloud transition. A spectral decomposition analysis of the solid-state absorbers is performed using archival spectroscopic observations from the Spitzer Space Telescope and Infrared Space Observatory. We find strong evidence for the presence of sub-micron-sized amorphous silicate grains, principally comprised of olivine-like composition, with no convincing evidence of H{sub 2}O ice mantles. However, tentative evidence for thick H{sub 2}O ice mantles on large (a ≈ 2.8 μm) grains is presented. Solid-state abundances of elemental Mg, Si, Fe, and O are inferred from our analysis and compared to standard reference abundances. We find that nearly all of the Mg and Si atoms along the line of sight reside in amorphous silicate grains, while a substantial fraction of the elemental Fe resides in compounds other than silicates. Moreover, we find that the total abundance of elemental O is largely inconsistent with the adopted reference abundances, indicating that as much as ∼156 ppm of interstellar O is missing along the line of sight. After taking into account additional limits on the abundance of elemental O in other O-bearing solids, we conclude that any missing reservoir of elemental O must reside on large grains that are nearly opaque to infrared radiation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

The effect of selective desorption mechanisms during interstellar ice formation

Major components of ices on interstellar grains in molecular clouds—water and carbon oxides—occur at various optical depths. This implies that selective desorption mechanisms are at work. An astrochemical model of a contracting low-mass molecular cloud core is presented. Ice was treated as consisting of the surface and three subsurface layers (i.e., sublayers). Photodesorption, reactive desorption, and indirect reactive desorption were investigated. The latter manifests itself through desorption from H+H reaction on grains. Desorption of shallow subsurface species was also included. Modeling results suggest the existence of a “photon-dominated ice” during the early phases of core contraction. Subsurface ice is chemically processed by interstellar photons, which produces complex organic molecules (COMs). Desorption from the subsurface layer results in high COM gas-phase abundances at A{sub V} = 2.4–10 mag. This may contribute toward an explanation for COM observations in dark cores. It was found that photodesorption mostly governs the onset of ice accumulation onto grains. Reaction-specific reactive desorption is efficient for small molecules that form via highly exothermic atom-addition reactions. Higher reactive desorption efficiency results in lower gas-phase abundances of COMs. Indirect reactive desorption allows for closely reproducing the observed H{sub 2}O:CO:CO{sub 2} ratio toward a number of background stars. Presumably, this can be done by any mechanism whose efficiency fits with the sequence CO⩾CO{sub 2}≫H{sub 2}O. After the freeze-out has ended, the three sublayers represent chemically distinct parts of the mantle. The likely A{sub V} threshold for the appearance of CO ice is 8–10.5 mag. The lower value is supported by observations.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

SWIFT ULTRAVIOLET OBSERVATIONS OF SUPERNOVA 2014J IN M82: LARGE EXTINCTION FROM INTERSTELLAR DUST

We present optical and ultraviolet (UV) photometry and spectra of the very nearby and highly reddened supernova (SN) 2014J in M82 obtained with the Swift Ultra-Violet/Optical Telescope (UVOT). Comparison of the UVOT grism spectra of SN 2014J with Hubble Space Telescope observations of SN2011fe or UVOT grism spectra of SN 2012fr are consistent with an extinction law with a low value of R{sub V} ∼1.4. The high reddening causes the detected photon distribution in the broadband UV filters to have a much longer effective wavelength than for an unreddened SN. The light curve evolution is consistent with this shift and does not show a flattening due to photons being scattered back into the line of sight (LOS). The light curve shapes and color evolution are inconsistent with a contribution scattered into the LOS by circumstellar dust. We conclude that most or all of the high reddening must come from interstellar dust. We show that even for a single dust composition, there is not a unique reddening law caused by circumstellar scattering. Rather, when considering scattering from a time-variable source, we confirm earlier studies that the reddening law is a function of the dust geometry, column density, and epoch. We also show how an assumed geometry of dust as a foreground sheet in mixed stellar/dust systems will lead to a higher inferred R{sub V}. Rather than assuming the dust around SNe is peculiar, SNe may be useful probes of the interstellar reddening laws in other galaxies.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

AN EXACT ANALYTICAL SOLUTION FOR THE INTERSTELLAR MAGNETIC FIELD IN THE VICINITY OF THE HELIOSPHERE

An analytical representation of the interstellar magnetic field in the vicinity of the heliosphere is derived. The three-dimensional field structure close to the heliopause is calculated as a solution of the induction equation under the assumption that it is frozen into a prescribed plasma flow resembling the characteristic interaction of the solar wind with the local interstellar medium. The usefulness of this analytical solution as an approximation to self-consistent magnetic field configurations obtained numerically from the full MHD equations is illustrated by quantitative comparisons.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

BROAD BALMER WINGS IN BA HYPER/SUPERGIANTS DISTORTED BY DIFFUSE INTERSTELLAR BANDS: FIVE EXAMPLES IN THE 30 DORADUS REGION FROM THE VLT-FLAMES TARANTULA SURVEY

Extremely broad emission wings at Hβ and Hα have been found in VLT-FLAMES Tarantula Survey data for five very luminous BA supergiants in or near 30 Doradus in the Large Magellanic Cloud. The profiles of both lines are extremely asymmetrical, which we have found to be caused by very broad diffuse interstellar bands (DIBs) in the longward wing of Hβ and the shortward wing of Hα. These DIBs are well known to interstellar but not to many stellar specialists, so that the asymmetries may be mistaken for intrinsic features. The broad emission wings are generally ascribed to electron scattering, although we note difficulties for that interpretation in some objects. Such profiles are known in some Galactic hyper/supergiants and are also seen in both active and quiescent Luminous Blue Variables (LBVs). No prior or current LBV activity is known in these 30 Dor stars, although a generic relationship to LBVs is not excluded; subject to further observational and theoretical investigation, it is possible that these very luminous supergiants are approaching the LBV stage for the first time. Their locations in the HRD and presumed evolutionary tracks are consistent with that possibility. The available evidence for spectroscopic variations of these objects is reviewed, while recent photometric monitoring does not reveal variability. A search for circumstellar nebulae has been conducted, with an indeterminate result for one of them.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

PRECURSORS TO INTERSTELLAR SHOCKS OF SOLAR ORIGIN

On or about 2012 August 25, the Voyager 1 spacecraft crossed the heliopause into the nearby interstellar plasma. In the nearly three years that the spacecraft has been in interstellar space, three notable particle and field disturbances have been observed, each apparently associated with a shock wave propagating outward from the Sun. Here, we present a detailed analysis of the third and most impressive of these disturbances, with brief comparisons to the two previous events, both of which have been previously reported. The shock responsible for the third event was first detected on 2014 February 17 by the onset of narrowband radio emissions from the approaching shock, followed on 2014 May 13 by the abrupt appearance of intense electron plasma oscillations generated by electrons streaming outward ahead of the shock. Finally, the shock arrived on 2014 August 25, as indicated by a jump in the magnetic field strength and the plasma density. Various disturbances in the intensity and anisotropy of galactic cosmic rays were also observed ahead of the shock, some of which are believed to be caused by the reflection and acceleration of cosmic rays by the magnetic field jump at the shock, and/or by interactions with upstream plasma waves. Comparisons to the two previous weaker events show somewhat similar precursor effects, although differing in certain details. Many of these effects are very similar to those observed in the region called the “foreshock” that occurs upstream of planetary bow shocks, only on a vastly larger spatial scale.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

ION IRRADIATION OF H{sub 2}-LADEN POROUS WATER-ICE FILMS: IMPLICATIONS FOR INTERSTELLAR ICES

To understand the effects of cosmic-ray (CR) impacts on interstellar icy grains immersed in H{sub 2} gas, we have irradiated porous water-ice films loaded with H{sub 2} with 100 keV H{sup +}. The ice films were exposed to H{sub 2} gas at different pressures following deposition and during irradiation. A net H{sub 2} loss is observed during irradiation due to competition between ion-induced sputtering and gas adsorption. The initial H{sub 2} loss cross-section, 4(1) × 10{sup −14} cm{sup 2}, was independent of film thickness, H{sub 2}, and proton fluxes. In addition to sputtering, irradiation also closes nanopores, trapping H{sub 2} in the film with binding that exceeds physical absorption energies. As a result, 2%–7% H{sub 2} is retained in the ice following irradiation to high fluences. We find that the trapped H{sub 2} concentration increases with decreasing Φ, the ratio of ion to H{sub 2} fluxes, suggesting that as high as 8% solid H{sub 2} can be trapped in interstellar ice by CR or stellar wind impacts.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2015

PROBING THE LOCAL BUBBLE WITH DIFFUSE INTERSTELLAR BANDS. III. THE NORTHERN HEMISPHERE DATA AND CATALOG

We present new high signal-to-noise ratio (S/N) observations of the diffuse interstellar bands (DIBs) in the Local Bubble and its surroundings. We observed 432 sightlines and obtain the equivalent widths of the λ5780 and λ5797 Å DIBs up to a distance of ∼200 pc. All of the observations were carried out using the Intermediate Dispersion Spectrograph on the 2.5 m Isaac Newton Telescope, during three years, to reach a minimum S/N of ∼2000. All of the λ5780 and λ5797 absorptions are presented in this paper and we tabulate the observed values of the interstellar parameters, λ5780, λ5797, Na ID{sub 1}, and Na ID{sub 2}, including the uncertainties.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

INTERSTELLAR NEUTRAL HELIUM IN THE HELIOSPHERE FROM IBEX OBSERVATIONS. I. UNCERTAINTIES AND BACKGROUNDS IN THE DATA AND PARAMETER DETERMINATION METHOD

This paper is one of three companion papers presenting the results of our in-depth analysis of the interstellar neutral helium (ISN He) observations carried out using IBEX-Lo during the first six Interstellar Boundary Explorer (IBEX) observation seasons. We derive corrections for losses due to the limited throughput of the interface buffer and determine the IBEX spin-axis pointing. We develop an uncertainty system for the data, taking into account the resulting correlations between the data points. This system includes uncertainties due to Poisson statistics, background, spin-axis determination, systematic deviation of the boresight from the prescribed position, correction for the interface buffer losses, and the expected Warm Breeze (WB) signal. Subsequently, we analyze the data from 2009 to examine the role of various components of the uncertainty system. We show that the ISN He flow parameters are in good agreement with the values obtained by the original analysis. We identify the WB as the principal contributor to the global χ{sup 2} values in previous analyses. Other uncertainties have a much milder role and their contributions are comparable to each other. The application of this uncertainty system reduced the minimum χ{sup 2} value 4-fold. The obtained χ{sup 2} value, still exceeding the expected value, suggests that either the uncertainty system may still be incomplete or the adopted physical model lacks a potentially important element, likely an imperfect determination of the WB parameters. The derived corrections and uncertainty system are used in the accompanying paper by Bzowski et al. in an analysis of the data from six seasons.

79 ASTRONOMY AND ASTROPHYSICS↗