Fast, Radiation Tolerant Detector for Thermal Neutrons
Explore the source record for details and available documents.
SEARCH · Engineering Papers
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
Explore the source record for details and available documents.
Explore the source record for details and available documents.
Explore the source record for details and available documents.
Explore the source record for details and available documents.
The International Atomic Energy Agency (IAEA) has obligations to apply safeguards to nuclear material and facilities within States subject to IAEA safeguards agreements. As a result of these obligations, safeguards will need to be applied to Generation IV reactors, including liquid fueled molten salt reactors (MSRs), if they are deployed in States with safeguards agreements. Recently, the IAEA has noted that a growing number of Member States are showing interest in MSR technology. This has been accompanied by an increase in short term development and deployment activities relating to MSRs. To ensure MSRs can be safeguarded effectively and efficiently upon possible future deployment, safeguards approaches and techniques need to be investigated now.
Explore the source record for details and available documents.
Systems codes require fast, simplified models to rapidly evaluate fusion power plant concepts, but neutronics analyses are often a computational bottleneck. Here, to address this, surrogate models for key neutronics responses have been developed using 3-D neutronics-ready models built with the open-source code ParaStell from a database of stellarator equilibria. Neutronics responses such as tritium breeding ratio (TBR), nuclear heating, and neutron-induced radiation damage displacements per atom (dpa) were simulated using OpenMC. Through sensitivity analysis and symbolic regression (SR), simple power-law formulas were derived connecting these neutronics responses to global stellarator parameters, including fusion power, plasma surface area, and plasma elongation. Validation shows these formulas can predict the simulation results with low error, enabling quick and accurate assessment of neutronics requirements in stellarator design exploration activities with systems codes.
The neutrons sublibrary aims to describe nuclear reactions between incident neutron particles and different nuclei. For ENDF/B-VIII.1, many neutron files were re-evaluated or received major changes. A new 239Pu evaluation was jointly-produced by IAEA, LANL, LLNL and ORNL bringing important updates to fission neutron multiplicity, Prompt Fission Neutron Spectrum, resonance and fast regions. Around one third of the new neutron evaluations were performed as part of the INDEN collaboration, including 16,18 O, 19 F, 28,29,30 Si, 63,65 Cu, 50,51,52,53,54 Cr, 55 Mn, 54,56,57 Fe, 139 La, 233,235,238 U, 240,241 Pu. Important non-INDEN evaluations include 234,236 U, 206,207,208 Pb, 181 Ta, 88 Sr, 140,142 Ce, Pt and Dy isotopes, and many others. Also, dosimetry reactions from IRDFF-II were adopted for many materials.
In inertial confinement fusion experiments at the National Ignition Facility, asymmetries are probed by a variety of neutron diagnostics, including neutron imaging systems, real-time neutron activation diagnostics (RTNADs), and neutron spectrometers. It is often useful to generate synthetic data based on these diagnostics to validate and tune models. However, current methods of doing so using Monte Carlo particle tracing are time-consuming. In this paper, an ultra-fast method is presented for generating synthetic neutron images, RTNAD data, and spectrometry data using line integrals and 3D convolutions. While it does not contain as much physics as particle tracing codes, it is thousands of times faster and produces nearly identical data. This enables analysis techniques that depend on generating large amounts of synthetic data, which will prove very useful for the study of asymmetries going forward.
Molten salt fission reactors (MSR) have been suggested for lunar and planetary surface power systems. They have the advantage of operating at high temperature, for efficient thermal-electrical conversion, low pressure, long-lived with high nuclear fuel burnup. MSR are often designed to breed fissile 233U from natural 232Th by neutron capture and decay via: 232Th(n,)233Th(,)233Pa(,)233U Unfortunately, this process requires 233Pa isotope separation and segregation to decay to 233U. This requirement prevents additional neutron capture that interferes with 233U breeding. Instead, Wooley’s sub-critical, fast fission, molten salt reactor would use externally generated tokamak fusion neutrons1,2 to fission all actinides.We propose a simpler fusion-fast-fission sub-critical reactor that generates fast neutrons in situ from lattice confinement fusion (LCF) to fission fertile and fissile actinides. This hybrid reactor doesn't require enriched 235U fissile pins to initiate fis-sion reactions, nor 233Pa separation and segregation during operation. Like Wooley’s, this hybrid reactor “burns” natural uranium (238U) or thorium (232Th) which avoids uranium enrichment and additional fissile material launch safety and security costs. The LCF neutron source is initiated by bremsstrahlung photoneutrons (Fig. 1)3 or isotopic neutron sources in electron-screened lattices (Fig. 2)4,5. Alternatively, the electrolytic Pd-deuterium co-deposition6protocol fast fissions7 both 232Th and 238U. However, an aqueous electrolyte-based system, without pressurization similar to conventional pressurized water fission reactors, is incapable of high temperatures due to the boiling point of the electrolyte slightly over 100 C. Molten salts can be used instead as was demonstrated at the University of Hawaii8 using a variety of Ni and Pd cathodes in lithiated, hydrided and deuterated salts. These salts have melting points often exceeding 500C making them suitable to efficiently produce electrical power9 through either Advanced Stirling Genera-tors (< 100 kWe) or closed-Brayton Cycle (> 100 kWe). This hybrid reactor could power a wide range of lunar or Martian applications from unmanned in-struments, to charging vehicles and entire facilities such as human habitats or in situ resource utilization. The power conversion cycles are Carnot Cycle limited, but generally 30% efficient at best. However, waste heat on the moon or Mars is important to surviving either two-week lunar nights or Martian nights as well as providing process heat for mineral extraction and “living off the land”
Advanced battery characterization using neutron and X-ray-based imaging modalities is crucial to reveal fundamental degradation modes of lithium-ion batteries (LIBs). Taking advantage of the sensitivity of neutrons to some low-Z (Li) and X-rays to high-Z materials (Cu), here we demonstrate the viability of simultaneous neutron and X-ray tomography (NeXT) as a non-destructive imaging platform for ex-situ 3D visualization of graphite electrode degradation following extreme fast charging (XFC). In addition, we underscore the benefits of the simultaneous of NeXT by combining the neutron and X-ray tomography data from the same sample location for material identification and segmentation of one pristine and two XFC-cycled graphite electrodes (9C charge for 450 cycles). Our ex-situ results and methodology development pave the way for the design of NeXT-friendly LIB geometries that will allow operando and/or in-situ 3D visualization of electrode degradation during XFC.
Fast-ion losses need to be monitored to avoid damage to plasma facing components. In existing experimental devices, the scintillator-based fast-ion loss detector (FILD) is the most advanced diagnostic for measuring fast-ion losses. However, FILDs provide only local information about the losses. Infrared (IR) thermography can be used as a complementary tool for more global monitoring of the deposition of fast-ion losses on the wall, at the expense of no velocity-space resolution. IR cameras measure the temperature of the plasma facing components. This measurement, determined by a combined effect of the thermal plasma, radiation, neutrons and fast-ion losses, can be decomposed to infer the fast-ion load on the tokamak wall. In this manuscript, a workflow to estimate fast-ion losses via IR thermography is applied to the MAST-U spherical tokamak, using a 1D approximation to extract the experimental heat flux on the FILD front face from IR data. To numerically estimate the different contributions to this total heat flux, the field-line tracing environment SMITER is used to calculate the thermal plasma contribution, the orbit-following Monte-Carlo code ASCOT to estimate the fast-ion losses, and bolometry measurements for the radiation. To validate the workflow, two discharges, L-mode plasmas with low MHD activity, were executed using on and off-axis beams, respectively. The experimentally and numerically estimated heat flux are of the same order of magnitude for the on-axis heated scenario, with a strong dependence of the estimated fast-ion losses contribution on the fit to the kinetic profiles used as input. This is also true for the off-axis heated scenario, where the total numerically estimated heat flux is 2.1 or 1.3 times higher than the maximum experimentally estimated heat flux, depending on the ASCOT input used.
A study on the neutron production from single and double gas puff Z-pinches on the CESZAR linear transformer driver with ~0.45 MA current and 170 ns rise time is presented. Total neutron yield measurements made with a LaBr activation detector are compared for three configurations, using a double nozzle setup. When a single, hollow, deuterium gas shell was used, reliable implosions could only be attained at higher load mass than the optimal value to match implosion time with the driver rise time, with neutron yields of ~10 6 per pulse. The use of a double gas puff configuration with a deuterium center jet allowed a reduction in the shell density and operation closer to machine-matched conditions, recording up to (4.1 ± 0.3) × 10 7 neutrons/pulse when either Kr or D 2 was used in the shell. For a comparable mass and implosion time, using a higher atomic-number gas in the outer shell results in more unstable plasma surface and smaller plasma radius at the location of instability bubbles, which, however, do not seem to consistently correlate with a higher neutron yield. Comparing implosion dynamics with models and neutron yields with literature scaling suggests that the machine current is not well coupled to the plasma during the final stages of compression. Optimizing current and energy coupling to the pinched plasma is critical to improving performance, particularly in low-impedance drivers.
The direct Urca process of rapid neutrino emission can occur in nonuniform nuclear pasta phases that are expected in the inner crusts of neutron stars. Here, the periodic potential for a nucleon in nuclear pasta allows momentum conservation to be satisfied for direct Urca reactions. We improve on earlier work by modeling a rich variety of pasta phases (gnocchi, waffle, lasagna, and anti-spaghetti) with large-scale molecular dynamics simulations. We find that the neutrino luminosity due to direct Urca reactions in nuclear pasta can be 3 to 4 orders of magnitude larger than that from the modified Urca process in the NS core. Thus neutrino radiation from pasta could dominate radiation from the core and this could significantly impact the cooling of neutron stars.
At a spallation neutron source, neutron pulses of varying energies are generated, and the detection of neutrons by instrument detectors is recorded as time-of-flight from the emission of the neutron pulse to its arrival at specific detector pixels with high time resolution. The flight path of neutrons from the moderator to the sample and then to the detector must be precisely calibrated at the detector-pixel level using standard powders, so the neutron events from all pixels can be time-focused to produce high-resolution diffraction patterns. Modern time-of-flight neutron diffractometers at spallation neutron sources are equipped with two-dimensional detectors with millimeter-scale pixelations. The number of pixels in a diffraction instrument can reach millions, which makes a single-pixel-level calibration process time-consuming or even impossible with conventional refinement or fitting approaches. Here we present a machine-learning-aided calibration process using a train-and-predict approach, in which machine learning models are trained on the relationship between an individual pixel time-of-flight diffraction pattern and its diffraction constant. These models use a portion of the available pixels for training, and a good model then predicts the diffraction constants precisely and rapidly for large sets of pixel diffraction patterns.
Explore the source record for details and available documents.
Explore the source record for details and available documents.
Previous measurements of neutron energy using fast plastic scintillators while operating the Fusion Z Pinch Experiment (FuZE) constrained the energy of any yield-producing deuteron beams to less than 4.65 keV. FuZE has since been operated at increasingly higher input power, resulting in increased plasma current and larger fusion neutron yields. A detailed experimental study of the neutron energy isotropy in these regimes applies more stringent limits to possible contributions from beam-target fusion. The FuZE device operated at -25 kV charge voltage has resulted in average plasma currents of 370 kA and D–D fusion neutron yields of $4\times10^7 \pm 4\times10^6$ neutrons per discharge. Measurements of the neutron energy isotropy under these operating conditions demonstrates the energy of deuteron beams is less than $7.4 \pm 5.6^\mathrm{(stat)} \pm 3.7^\mathrm{(syst)}$ keV. Characterization of the detector response has reduced the number of free parameters in the fit of the neutron energy distribution, improving the confidence in the forward-fit method. Gamma backgrounds have been measured and the impact of these contributions on the isotropy results have been studied. Additionally, a time dependent measurement of the isotropy has been resolved for the first time, indicating increases to possible deuteron beam energies at late times. This suggests the possible growth of m = 0 instabilities at the end of the main radiation event but confirms that the majority of the neutron production exhibits isotropy consistent with thermonuclear origin.