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At least 631 records · Page 35

Remote sensing of smoke, clouds, and radiation using AVIRIS during SCAR experiments

During the past two years, researchers from several institutes joined together to take part in two SCAR experiments. The SCAR-A (Sulfates, Clouds And Radiation - Atlantic) took place in the mid-Atlantic region of the United States in July, 1993. remote sensing data were acquired with the Airborne Visible Infrared Imaging Spectrometer (AVIRIS), the MODIS Airborne Simulator (MAS), and a RC-10 mapping camera from an ER-2 aircraft at 20 km. In situ measurements of aerosol and cloud microphysical properties were made with a variety of instruments equipped on the University of Washington's C-131A research aircraft. Ground based measurements of aerosol optical depths and particle size distributions were made using a network of sunphotometers. The main purpose of SCAR-A experiment was to study the optical, physical and chemical properties of sulfate aerosols and their interaction with clouds and radiation. Sulfate particles are believed to affect the energy balance of the earth by directly reflecting solar radiation back to space and by increasing the cloud albedo. The SCAR-C (Smoke, Clouds And Radiation - California) took place on the west coast areas during September - October of 1994. Sets of aircraft and ground-based instruments, similar to those used during SCAR-A, were used during SCAR-C. Remote sensing of fires and smoke from AVIRIS and MAS imagers on the ER-2 aircraft was combined with a complete in situ characterization of the aerosol and trace gases from the C-131A aircraft of the University of Washington and the Cesna aircraft from the U.S. Forest Service. The comprehensive data base acquired during SCAR-A and SCAR-C will contribute to a better understanding of the role of clouds and aerosols in global change studies. The data will also be used to develop satellite remote sensing algorithms from MODIS on the Earth Observing System.

Gao, Bo-Cai↗

Atmospheric processing and aerosol aging responsible for observed increase in absorptivity of long-range-transported smoke over the southeast Atlantic

Biomass burning aerosol (BBA) from agricultural fires in southern Africa contributes about one-third of the global carbonaceous aerosol load. These particles have strong radiative effects in the southeast Atlantic (SEA), which depend in part on the radiative contrast between the aerosol layer in the free troposphere (FT) and the underlying cloud layer. However, there is large disagreement in model estimates of aerosol-driven climate forcing due to uncertainties in the vertical distribution, optical properties, and life cycle of these particles. This study applies a novel method combining remote sensing observations with regional model outputs to investigate the aging of the BBA and its impact on the optical properties during transatlantic transport from emission sources in Africa to the SEA. Results show distinct variations in extinction Ångström exponent (EAE) and single-scattering albedo (SSA) as aerosols age. Near the source, fresh aerosols are characterized by low mean SSA (0.84) and high EAE (1.85), indicating smaller, highly absorbing particles. By isolating marine contributions from the total column during BBA transport across the SEA, our analysis reveals an initial decrease in BBA absorptivity, with mean FT SSA of 0.87 after 6–7 d, followed by increased absorptivity with mean FT SSA of 0.84 after 10 d, suggesting enhanced absorption due to chemical aging. These findings indicate that BBA becomes more absorbing during extended transport across the SEA, with implications for reducing model uncertainties. Our remote-sensing-based results agree well with previous in situ studies and offer new insights into aerosol–radiation interactions and the energy balance over the SEA.

54 ENVIRONMENTAL SCIENCES↗

Mineralogy and Astrobiology Detection Using Laser Remote Sensing Instrument

A multispectral instrument based on Raman, laser-induced fluorescence (LIF), laser-induced breakdown spectroscopy (LIBS), and a lidar system provides high-fidelity scientific investigations, scientific input, and science operation constraints in the context of planetary field campaigns with the Jupiter Europa Robotic Lander and Mars Sample Return mission opportunities. This instrument conducts scientific investigations analogous to investigations anticipated for missions to Mars and Jupiter's icy moons. This combined multispectral instrument is capable of performing Raman and fluorescence spectroscopy out to a >100 m target distance from the rover system and provides single-wavelength atmospheric profiling over long ranges (>20 km). In this article, we will reveal integrated remote Raman, LIF, and lidar technologies for use in robotic and lander-based planetary remote sensing applications. Discussions are focused on recently developed Raman, LIF, and lidar systems in addition to emphasizing surface water ice, surface and subsurface minerals, organics, biogenic, biomarker identification, atmospheric aerosols and clouds distributions, i.e., near-field atmospheric thin layers detection for next robotic-lander based instruments to measure all the above-mentioned parameters. OCIS codes: (120.0280) Remote sensing and sensors; (130.0250) Optoelectronics; (280.3640) Lidar; (300.2530) Fluorescence, laser-induced; (300.6450) Spectroscopy, Raman; (300.6365) Spectroscopy, laser induced breakdown

Abedin, M. Nurul↗

Investigating the Spatial and Temporal Limitations for Remote Sensing of Wildfire Smoke Using Satellite and Airborne Imagers During FIREX_AQ

Starting from point sources, wildfire smoke is important in the global aerosol system. The ability to characterize smoke near-source is key to modeling smoke dispersion and predicting air quality. With hemispheric views and 10-min refresh, imagers in Geostationary (GEO) orbit have advantages monitoring smoke over once-per-day sensors in low-earth orbit (LEO). However, both can be inadequate in capturing the characteristics of smoke plumes close to their sources due to too-coarse spatial resolution (both detector and product resolution), too-sparse temporal resolution (from LEO sensors), and too-conservative masking. In addition to satellite observations, the Fire Influence on Regional to Global Environments and Air Quality experiment offered sub-orbital enhanced-MODIS Airborne Simulator (eMAS) imagery at 50 m pixel resolution—including multiple eMAS flight tracks over individual fires in short time periods. It provided opportunity to explore smoke plume characterization at various spatial and temporal scales and quantify the limitations of space sensors for describing smoke magnitude near source as well as its temporal evolution. Here we applied modified aerosol algorithm to different imagers, relaxing its masking to estimate smoke's aerosol optical depth (AOD) as close as possible to its source. We found that GEO sensors with nominal 1 km spatial resolution can match the much finer resolution eMAS retrieved mean plume AOD, as long as the retrieval spatial resolution is finer than the width of the plumes. However, the plume's maximum AOD may be drastically underestimated by satellite products.

remote sensing↗

Observation and Quantification of Aerosol Outflow from Southern Africa Using Spaceborne Lidar

Biomass burning in Africa provides a prolific source of aerosols that are transported from the source region to distant areas, as far away as South America and Australia. Models have long predicted the primary outflow and transport routes. Over time, field studies have validated the basic production and dynamics that underlie these transport patterns. In more recent years, the advancement of spaceborne active remote sensing techniques has allowed for more detailed verification of the models and, importantly, verification of the vertical distribution of the aerosols in the transport regions, particularly with respect to westerly transport over the Atlantic Ocean. The Cloud-Aerosol Transport System (CATS) lidar on the International Space Station has detection sensitivity that provides observations that support long-held theories of aerosol transport from the African subcontinent over the remote Indian Ocean and as far downstream as Australia.

Lidar↗

The Amazon River‐Breeze Circulation Limits Detection of Aerosol‐Cloud Interactions in Warm Clouds

Increased aerosol concentrations can brighten low-level clouds and extend their lifetimes, but aerosol–cloud interactions (ACI) remain highly uncertain and difficult to quantify. We show that part of this uncertainty is caused by topographical influences on clouds, that is, those arising from land–water contrasts. This is demonstrated using satellite retrievals in regions with extensive river networks, such as the Amazon Basin. 15 years of MODerate resolution Imaging Spectroradiometer (MODIS) satellite data show cloud formation over the Amazon River basin is suppressed by 26% with warm low clouds above the river exhibiting a 22% smaller droplet effective radius and 18% higher droplet concentration ($N_d$) compared to adjacent land clouds. Thus, clouds above the river may appear polluted but are actually influenced by river-breeze circulations driven by the thermal contrast between the river and the surrounding land. These responses are robust in both wet and dry seasons, and tests using an improved MODIS retrieval product show cloud differences are unlikely due to retrieval artifacts. In situ measurements from the Green Ocean Amazon Experiment (GoAmazon) confirm that $N_d$ is elevated above rivers and are also higher when carbon monoxide concentrations are elevated near the large city of Manaus. Lagrangian airmass tracking over Manaus shows that regional-scale river-breeze circulations impact $N_d$ as much as the urban aerosol plume, complicating ACI attribution and highlighting the need to isolate land-surface effects to assess ACI in continental regions.

Aerosol-Cloud Interactions↗

Remote Sensing by Spaceborne Lidar Aided by Surface Returns

Spaceborne lidar offers the possibility of global mapping of clouds and atmospheric aerosols. Mapping of cloud-top heights, multiple layers of thin clouds and the depth of the planetary boundary layer (PBL), given sufficient aerosols, are applications that should be fairly easy to accomplish from space with even a modest lidar system. However, the constraints imposed on spaceborne lidar by large ranging distances, limited available power/weight, and fast moving platforms present significant challenges to achieving more quantitative retrievals such as extracting aerosol extinction profiles, PBL optical depths and cloud optical depths. Ways to take advantage of the strong signals available from ground/sea reflections to improve upon atmospheric aerosol and cloud retrievals as well as to distinguish certain surface types are explored.

Reagan, J. A.↗

Effects of Whitecaps on Satellite-Derived Ocean Color

During the 3.25 years of the project, various aspects of satellite ocean-color remote sensing were investigated, including effect of whitecaps on atmospheric correction, validity of aerosol models, and evaluation of ocean-color products. Algorithms to estimate pigment concentration and photo-synthetically active radiation (PAR) were developed, and studies of geophysical phenomena, such as the 1998 Asian Dust event, were performed. The influence of solar radiation absorption by phytoplankton on mixed layer dynamics, ocean circulation, and climate was also investigated. The project's results and findings are described.

Frouin, Robert↗

The 1996 Subsonic Aircraft: Contrail and Cloud Effects Special Study

During April 1996 NASA, in conjunction with the DOE, will sponsor a multi-aircraft field campaign to better understand the microphysical and radiative properties of cirrus clouds, the origins of ice nuclei and cloud condensation nuclei in the upper troposphere, and the possible role that the commercial subsonic aircraft fleet might play in altering cloud or aerosol properties. The NASA ER-2 aircraft will be used as a remote sensing platform, while the NASA DC-8 aircraft will be used as an in situ measurement platform. In situ observations will include a full set of size distribution measurements from nano-meter to millimeter sizes, ice water content measurements, gas phase and condensed phase chemical measurements, ice crystal optical phase function measurements, lidar observations of cloud top and cloud base, and atmospheric state measurement. The ER-2 will have lidar, microwave ice water path measurements, as well as visible and infrared spectral measurement. In this presentation the highlights of the mission will be presented. The goal will be to address fundamental questions such as the mode of nucleation of cirrus clouds, the composition of the nuclei on which cirrus form, the degree to which aircraft impact cirrus cloud properties.

Toon, Owen B.↗

Application of the CALIOP Layer Product to Evaluate the Vertical Distribution of Aerosols Estimated by Global Models: AeroCom Phase I Results

The CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) layer product is used for a multimodel evaluation of the vertical distribution of aerosols. Annual and seasonal aerosol extinction profiles are analyzed over 13 sub-continental regions representative of industrial, dust, and biomass burning pollution, from CALIOP 2007-2009 observations and from AeroCom (Aerosol Comparisons between Observations and Models) 2000 simulations. An extinction mean height diagnostic (Z-alpha) is defined to quantitatively assess the models' performance. It is calculated over the 0-6 km and 0-10 km altitude ranges by weighting the altitude of each 100 m altitude layer by its aerosol extinction coefficient. The mean extinction profiles derived from CALIOP layer products provide consistent regional and seasonal specificities and a low inter-annual variability. While the outputs from most models are significantly correlated with the observed Z-alpha climatologies, some do better than others, and 2 of the 12 models perform particularly well in all seasons. Over industrial and maritime regions, most models show higher Z-alpha than observed by CALIOP, whereas over the African and Chinese dust source regions, Z-alpha is underestimated during Northern Hemisphere Spring and Summer. The positive model bias in Z-alpha is mainly due to an overestimate of the extinction above 6 km. Potential CALIOP and model limitations, and methodological factors that might contribute to the differences are discussed.

Aerosols and particles↗

Laboratory for Atmospheres Instrument Systems Report

Studies of the atmospheres of our solar system's planets including our own require a comprehensive set of observations, relying on instruments on spacecraft, aircraft, balloons, and on the surface. These instrument systems perform one or both of the following: 1) provide information leading to a basic understanding of the relationship between atmospheric systems and processes, and 2) serve as calibration references for satellite instrument validation. Laboratory personnel define requirements, conceive concepts, and develop instrument systems for spaceflight missions, and for balloon, aircraft, and ground-based observations. Balloon and airborne platforms facilitate regional measurements of precipitation, cloud systems, and ozone from high-altitude vantage points, but still within the atmosphere. Such platforms serve as stepping-stones in the development of space instruments. Satellites provide nearly global coverage of the Earth with spatial resolutions and repetition rates that vary from system to system. The products of atmospheric remote sensing are invaluable for research associated with water vapor, ozone, trace gases, aerosol particles, clouds, precipitation, and the radiative and dynamic processes that affect the climate of the Earth. These parameters also provide the basic information needed to develop models of global atmospheric processes and weather and climate prediction. Laboratory scientists also participate in the design of data processing algorithms, calibration techniques, and the data processing systems.

Platnick, Steven E.↗

Raman Lidar (RL) Instrument Handbook

The Raman lidar at the ARM Climate Research Facility (ACRF) Southern Great Plains (SGP) Central Facility (SGPRL) is an active, ground-based laser remote sensing instrument that measures height and time resolved profiles of water vapor mixing ratio and several cloud- and aerosol-related quantities. The system is a non-commercial custom-built instrument developed by Sandia National Laboratories specifically for the ARM Program. It is fully computer automated, and will run unattended for many days following a brief (~5-minute) startup period. The self-contained system (requiring only external electrical power) is housed in a climate-controlled 8’x8’x20’ standard shipping container.

54 ENVIRONMENTAL SCIENCES↗

Multipurpose Spectroradiometer for Satellite Instrument Calibration and Zenith Sky Remote Sensing Measurements

In the early 1990s a series of surface-based direct sun and zenith sky measurements of total column ozone were made with SBUV/2 flight models and the SSBUV Space Shuttle instrument in Boulder, Colorado which were compared with NOAA Dobson Instrument direct sun observations and TOMS instrument overpass observations of column ozone. These early measurements led to the investigation of the accuracy of derived total column ozone amounts and aerosol optical depths from zenith sky observations. Following the development and availability of radiometrically stable IAD narrow band interference filter and nitrided silicon photodiodes a simple compact multifilter spectroradiometer was developed which can be used as a calibration transfer standard spectroradiometer (CTSS) or as a surface based instrument remote sensing instruments for measurements of total column ozone and aerosol optical depths. The total column ozone derived from zenith sky observations agrees with Dobson direct sun AD double wavelength pair measurements and with TOMS overpass ozone amounts within uncertainties of about 1%. When used as a calibration transfer standard spectroradiometer the multifilter spectroradiometer appears to be capable of establishing instrument radiometric calibration uncertainties of the order of 1% or less relative to national standards laboratory radiometric standards.

Heath, Donald F.↗

A State-of-the-Art Experimental Laboratory for Cloud and Cloud-Aerosol Interaction Research

The state of the art for predicting climate changes due to increasing greenhouse gasses in the atmosphere with high accuracy is problematic. Confidence intervals on current long-term predictions (on the order of 100 years) are so large that the ability to make informed decisions with regard to optimum strategies for mitigating both the causes of climate change and its effects is in doubt. There is ample evidence in the literature that large sources of uncertainty in current climate models are various aerosol effects. One approach to furthering discovery as well as modeling, and verification and validation (V&V) for cloud-aerosol interactions is use of a large "cloud chamber" in a complimentary role to in-situ and remote sensing measurement approaches. Reproducing all of the complex interactions is not feasible, but it is suggested that the physics of certain key processes can be established in a laboratory setting so that relevant fluid-dynamic and cloud-aerosol phenomena can be experimentally simulated and studied in a controlled environment. This report presents a high-level argument for significantly improved laboratory capability, and is meant to serve as a starting point for stimulating discussion within the climate science and other interested communities.

Fremaux, Charles M.↗

A Network for Standardized Ocean Color Validation Measurements

The Aerosol Robotic Network (AERONET) was developed to support atmospheric studies at various scales with measurements from worldwide distributed autonomous sunphotometers [Holben et al. 1998]. AERONET has now extended its support to marine applications through the additional capability of measuring the radiance emerging from the sea with modified sun-photometers installed on offshore platforms like lighthouses, navigation aids, oceanographic and oil towers. The functionality of this added network component called AERONET - Ocean Color (AERONET-OC), has been verified at different sites and deployment structures over a four year testing phase. Continuous or occasional deployment platforms (see Fig. 1) included: the Acqua Alta Oceanographic Tower (AAOT) of the Italian National Research Council in the northern Adriatic Sea since spring 2002; the Martha s Vineyard Coastal Observatory (MVCO) tower of the Woods Hole Oceanographic Institution in the Atlantic off the Massachusetts coast for different periods since spring 2004; the TOTAL Abu-Al-Bukhoosh oil Platform (AABP, shown through an artistic rendition in Fig. 1) in the Persian (Arabian) Gulf in fall 2004; the Gustaf Dal n Lighthouse Tower (GDLT) of the Swedish Maritime Administration in the Baltic Sea in summer 2005; and the platform at the Clouds and the Earth's Radiant Energy System (CERES) Ocean Validation Experiment (COVE) site located in the Atlantic Ocean off the Virginia coast since fall 2005. Data collected during the network testing phase, confirm the capability of AERONET-OC to support the validation of marine optical remote sensing products through standardized measurements of normalized water-leaving radiance, LWN, and aerosol optical thickness, a, at multiple coastal sites.

Zibordi, Giuseppe↗

Optical depth measurements and atmospheric correction of remotely sensed data for FIFE

Data derived from an airborne tracking-sun photometer are used to provide quantitative corrections for atmospheric effects in remotely sensed data. The atmospheric correction involves the validation of radiometric and atmospheric measurements and the application of single scattering approximation which permits the separation of Rayleigh scattering from aerosol scattering. Sun-photometer data are used to generate plots of spectral optical depths, aerosol size distributions, aerosol phase functions, and aerosol single-scattering albedos. The atmospheric correction model and the atmospheric optical properties are incorporated into a program which is applied to two flightlines of data. Atmospheric corrections tested on remotely sensed data permitted the removal of limb brightening, although the results require verification by means of ground measurements.

Wrigley, R. C.↗

Satellite-Surface Perspectives of Air Quality and Aerosol-Cloud Effects on the Environment: An Overview of 7-SEAS BASELInE

The objectives of 7-SEASBASELInE (Seven SouthEast Asian Studies Biomass-burning Aerosols and Stratocumulus Environment: Lifecycles and Interactions Experiment) campaigns in spring 2013-2015 were to synergize measurements from uniquely distributed ground-based networks (e.g., AERONET (AErosol RObotic NETwork)), MPLNET ( NASA Micro-Pulse Lidar Network)) and sophisticated platforms (e.g.,SMARTLabs (Surface-based Mobile Atmospheric Research and Testbed Laboratories), regional contributing instruments), along with satellite observations retrievals and regional atmospheric transport chemical models to establish a critically needed database, and to advance our understanding of biomass-burning aerosols and trace gases in Southeast Asia (SEA). We present a satellite-surface perspective of 7-SEASBASELInE and highlight scientific findings concerning: (1) regional meteorology of moisture fields conducive to the production and maintenance of low-level stratiform clouds over land; (2) atmospheric composition in a biomass-burning environment, particularly tracers-markers to serve as important indicators for assessing the state and evolution of atmospheric constituents; (3) applications of remote sensing to air quality and impact on radiative energetics, examining the effect of diurnal variability of boundary-layer height on aerosol loading; (4) aerosol hygroscopicity and ground-based cloud radar measurements in aerosol-cloud processes by advanced cloud ensemble models; and (5) implications of air quality, in terms of toxicity of nanoparticles and trace gases, to human health. This volume is the third 7-SEAS special issue (after Atmospheric Research, vol. 122, 2013; and Atmospheric Environment, vol. 78, 2013) and includes 27 papers published, with emphasis on air quality and aerosol-cloud effects on the environment. BASELInE observations of stratiform clouds over SEA are unique, such clouds are embedded in a heavy aerosol-laden environment and feature characteristically greater stability over land than over ocean, with minimal radar surface clutter at a high vertical spatial resolution. To facilitate an improved understanding of regional aerosol-cloud effects, we envision that future BASELInE-like measurement modeling needs fall into two categories: (1) efficient yet critical in-situ profiling of the boundary layer for validating remote-sensing retrievals and for initializing regional transport chemical and cloud ensemble models; and (2) fully utilizing the high observing frequencies of geostationary satellites for resolving the diurnal cycle of the boundary layerheight as it affects the loading of biomass-burning aerosols, air quality and radiative energetics.

AERONET↗

The ATTO-Campina site: A new observatory for tropical convection and gas-aerosol-cloud-precipitation interactions in the Amazon

We present results from ATTO-Campina, a new permanent observational site in central Amazon, about 4 km from the ATTO towers. Operational since 2020, ATTO-Campina characterizes atmospheric, cloud and rainfall properties through remote sensing. The goal is to provide continuous, complementary measurements to the ATTO towers, addressing the rainforest’s complex gas-aerosol-cloud-precipitation dynamics. Using a 3.5-year dataset, we classified convective clouds into three types: shallow cumulus (ShCu), congestus (Con) or (Deep) clouds. The shallow-to-deep transition takes about three hours, starting with ShCu formation at 11:00 local time. The accumulated rainfall peak follows at about 16:00. Only weak downdrafts are present in the upper troposphere where previous studies indicate new particle formation (NPF) occurrence. Strong downdrafts are mostly limited to heights below 5 km. Con and Deep convective days have higher concentrations of ultrafine aerosol and lower concentrations of accumulation-mode particles compared to ShCu. Convective clouds also significantly modify gas mixing ratios. Deep convective clouds are associated with high near-surface O3, consistent with downward transport from the midtroposphere. Our results showcase the added detail achieved by integrating data from the ATTO towers and ATTO-Campina sites. Together, these sites support better understanding of interconnected gas-aerosol-cloud-precipitation processes in the Amazon and their evolution under climate change.

54 ENVIRONMENTAL SCIENCES↗