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At least 613 records · Page 34

Using Remote Sensing to Monitor the Spring Phenology of Acadia National Park Across Elevational Gradients

Greenup dates and their responses to elevation and temperature variations across the mountains of Acadia National Park are monitored using remote sensing data, including Landsat 8 surface reflectances (at a 30-m spatial resolution) and VIIRS reflectances adjusted to a nadir view (gridded at a 500-m spatial resolution), during the 2013–2016 growing seasons. The 30-m resolution provides a better scale for studying the phenology variation across elevational gradients than the 500-m resolution, as greenup dates monitored at 30-m scale have better agreement with leaf-out dates recorded in the field alongside the north–south-oriented hiking trails on three of the park’s tallest mountains (466 m, 418 m, and 380 m), and can provide landcover-specific analysis. The spring phenology responses to temperature and elevation vary among different spatial scales. Greenup dates of Acadia National Park monitored at 30-m scale show a weak advancing trend with higher spring temperature, while greenup dates monitored at 500 m show a weak delaying trend. The species mix within landcover at 30-m scale could weaken the advancing trend detected at field observation level. The landcover mix and elevation variation within 500-m scale could alter the spring phenology response to spring temperature variation. Greenup dates monitored at both 30-m and 500-m scales vary among different elevational zones, aspects, landcovers, and years. However, the relationship between greenup dates and elevation is rather weak.

Yan Liu↗

Topological Relationship–Based Flow Direction Modeling: Mesh–Independent River Networks Representation

River networks are important features in surface hydrology. However, accurately representing river networks in spatially distributed hydrologic and Earth system models is often sensitive to the model's spatial resolution. Specifically, river networks are often misrepresented because of the mismatch between the model's spatial resolution and river network details, resulting in significant uncertainty in the projected flow direction. In this study, we developed a topological relationship-based river network representation method for spatially distributed hydrologic models. This novel method uses (a) graph theory algorithms to simplify real-world vector-based river networks and assist in mesh generation; and (b) a topological relationship-based method to reconstruct conceptual river networks. The main advantages of our method are that (a) it combines the strengths of vector-based and DEM raster-based river network extraction methods; and (b) it is mesh-independent and can be applied to both structured and unstructured meshes. This method paves a path for advanced terrain analysis and hydrologic modeling across different scales.

54 ENVIRONMENTAL SCIENCES↗

Associated Particle Imaging of Neutron Inelastic Scatter: 3-D Reconstruction, Capabilities, and Challenges

Associated particle imaging (API) offers unique advantages for 3-D imaging of neutron inelastic scatter, including single-view tomographic imaging and data acquisition when access is limited to only one side of the interrogated object. However, widespread adoption of neutron inelastic scatter imaging has been impeded by several inherent challenges, most prominently spatial resolution, self-attenuation, and statistical noise. Here, in this work, the capabilities and challenges of neutron inelastic scatter imaging are investigated. Instead of focusing on a single imaging application, we identify imaging principles that hold for various neutron inelastic scatter imaging techniques. The primary challenges for 3-D imaging are characterized. The inherent spatial resolution in the time-of-flight (TOF) dimension is derived based on the known system timing resolution and scan geometry. Three reconstruction algorithms are described and demonstrated, including the introduction of modern iterative reconstruction incorporating a physics-based system model. Simulation is leveraged to demonstrate imaging capability with varying coincidence count levels and system timing resolution. An example of measured data with both back-scatter and forward-scatter detector positioning is presented. System design characteristics and their effects on image quality are identified. The imaging framework presented in this article has the potential to facilitate growth of 3-D neutron inelastic scatter API by identifying applications that are a good match for the technique and by targeting system development resources toward the requirements of a specific imaging task.

Associated particle imaging (API)↗

Performance of a triple-GEM detector with capacitive-sharing 3-coordinate (X–Y–U)-strip anode readout

The concept of capacitive-sharing readout, described in detail in a previous study, offers the possibility for the development of high-performance three-coordinates (X--Y--U)-strip readout for Micro Pattern Gaseous Detectors (MPGDs) using simple standard PCB fabrication techniques. Capacitive-sharing (X--Y--U)-strip readout allows simultaneous measurement of the Cartesian coordinates x and y of the position of the particles together with a third coordinate u along the diagonal axis in a single readout PCB. This provides a powerful tool to address multiple-hit ambiguity and enable pattern recognition capabilities in moderate particle flux environment of collider or fixed target experiments in high energy physics HEP) and nuclear physics (NP). We present in this paper the performance of a 10 cm × 10 cm triple-GEM detector with capacitive-sharing (X--Y--U)-strip anode readout. Spatial resolutions of the order of $\sigma_{x}^{res}$ = 71.6 $\pm$ 0.8 $\mu$m for X-strips, $\sigma_{y}^{res}$ = 56.2 $\pm$ 0.9 $\mu$m for Y-strips and $\sigma_{u}^{res}$ = 75.2 $\pm$ 0.9 $\mu$m for U-strips have been obtained at a beam test at Thomas Jefferson National Accelerator Facility (Jefferson Lab). Modifications of the readout design of future prototypes to improve the spatial resolution and challenges in scaling to large-area MPGDs are discussed.

(X-Y-U) strip↗

Numerical experiments on consistent horizontal and vertical resolution for atmospheric models and observing systems

Simple numerical experiments are performed in order to determine the effects of inconsistent combinations of horizontal and vertical resolution in both atmospheric models and observing systems. In both cases, we find that inconsistent spatial resolution is associated with enhanced noise generation. A rather fine horizontal resolution in a satellite data observing system seems to be excessive when combined with the usually available relatively coarse vertical resolution. Using different strength horizontal filters, adjusted in such a way as to render the effective horizontal resolution more consistent with vertical resolution for the observing system, may result in improvement of the analysis accuracy. However, the increase of vertical resolution for a satellite data observing system is desirable. For the conventional data observing system with better vertically resolved data, the results are different in that little or no horizontal filtering is needed to make spatial resolution more consistent for the system. The obtained experimental estimates of consistent vertical and effective horizontal resolution are in a general agreement with consistent resolution estimates previously derived theoretically by the authors.

Fox-Rabinovitz, Michael S.↗

Laboratory-Based Micro-X-ray Computed Tomography of Energy Materials at Idaho National Laboratory

Abstract The Idaho National Laboratory (INL) has implemented laboratory-based micro-X-ray computed tomography in a laboratory equipped for the examination of highly radioactive samples. This capability provides nondestructive three-dimensional volumetric information on samples to inform subsequent traditional destructive examinations as well as real-world inputs for high-fidelity scientific modeling. Samples can be imaged with spatial resolutions ranging from several hundred nm/voxel up to ~ 100 µm/voxel. The best usable spatial resolution achieved to date is 384 nm/voxel with this instrument, while the highest radiological dose rate of a sample imaged is ~ 60 R/h β/γ on contact. Advanced data analysis, including custom tomographic reconstruction and segmentation methods, have also been developed to support this capability. In addition to traditional digital X-ray radiography and tomography, this instrument is also able to visualize in situ tensile and compression testing as well as perform diffraction contrast tomography. This work describes the X-ray computed tomography post-irradiation examination capabilities at INL, as well as detailing a variety of applications this instrument has examined.

36 MATERIALS SCIENCE↗

Measurement of temperature and density fluctuations in turbulence using an ultraviolet laser

Noninvasive measurement of density and temperature fluctuations in turbulent air flow was examined. The approach used fluorescence of oxygen molecules which are selectively excited by a tunable vacuum ultraviolet laser beam. The strength of the fluorescence signal and its dependence on laser wavelength vary with the density and temperature of the air in the laser beam. Because fluorescence can be detected at 90 degrees from the beam propagation direction, spatial resolution in three dimensions, rather than path-integrated measurements can be achieved. With spatial resolutions of the order of a millimeter and at supersonic air velocities it is necessary to perform each measurement in a time of the order of a microsecond; this is possible by by using laser pulses of ten nanosecond duration. In this method atmospheric O2 is excited by the emission of a tunable ArF excimer laser, and the fluorescence, which spans the 210 to 420 range, is detected by an ultraviolet phototube.

Massey, G. A.↗

Aircraft-based radiometric imaging of tropospheric temperature and precipitation using the 118.75-GHz oxygen resonance

Passive microwave imaging of O2 emissions using the 118.75-GHz resonance has been investigated for tropospheric and stratospheric remote sensing of atmospheric temperature and precipitation. An imaging millimeter-wave spectrometer (MTS) using eight double-sideband channels centered around the 118.75-GHz resonance, and including a fixed-beam 53.65-GHz radiometer and video camera was constructed. The MTS collected data during 33 flights of the NASA-ER-2 high-altitude aircraft in 1986 during GALE and Cohmex, yielding the first high-spatial-resolution microwave images of atmospheric O2 brightness. The isolated 118-GHz line offers higher spatial resolution and precipitation sensitivity than O2 lines in the 5-mm band near 60 GHz. The brightness temperature perturbations of clouds in nonprecipitating regions are typically twice as large in the 118-GHz channels. However, observations over cirrus anvils show that the 118-GHz brightnesses are not adversely sensitive to some optically opaque cloud cover. Thus these channels are expected to be useful for temperature sounding in the presence of clouds, although retrieval ambiguities can result from variations in the water-vapor profile and surface emissivity.

Gasiewski, A. J.↗

Deep Mapping of Small Solar System Bodies with Galactic Cosmic Ray Secondary Particle Showers

We will investigate the use of galactic cosmic ray (GCR) secondary particles to probe the deep interiors of small solar system bodies (SSBs), including comets, asteroids, and geologic structures on the surfaces of airless bodies. Applications include solar system science, planetary defense, and resource utilization. Our Phase I study demonstrated that muons, the long-range charged component of GCR showers, can penetrate SSBs up to a km in diameter, providing information on their interior structure. Muons produced in Earth’s atmosphere have been applied to image the interior of large objects for science and engineering. In Phase I, we found that the production of muons in the solid surfaces of airless bodies is much smaller than in Earth’s atmosphere. Nevertheless, the flux of transmitted muons is sufficient to detect inclusions within an asteroid or comet in a reasonable amount of time, ranging from hours to weeks, depending on the size of the SSB and the density contrast, position and size of the inclusion. For asteroids and comets, large density variations (e.g., porous soil or ice versus solid rock) are relatively easy to detect. The intrinsic spatial resolution of muon radiography (“muography”) is on the scale of a few meters. The spatial resolution that can be achieved in practice depends on signal intensity and integration time (counting statistics), the angular resolution of the muon tracker (hodoscope) and details of data reduction and analysis methodology. Our Phase II project will assess remaining unknowns for the application of muography to determining the interior structure of SSBs, assess risks for implementation, and provide a roadmap for development of SSB muography beyond the NIAC program. To achieve our objectives, we will focus on four interrelated tasks: Task1) Signal and background characterization: Characterize the production and transmission of muons and secondary particle backgrounds made by cosmic ray showers in SSBs; and near-surface features from radiographic and tomographic data; Task2) Imaging studies: Develop methods to determine the density structure of SSB interiors and near-surface features from radiographic and tomographic data; Task3) Instrument design: Using simulations and bench-top laboratory experiments, investigate specific concepts for the design of compact hodoscopes and components; Task4) Synthesis: Combine the results of the first three tasks to determine the range of applicability of the method, identify the steps needed for maturation of the concept, and explore concepts for a pilot muography mission.

Prettyman, Thomas H.↗

Complexity Reduction Methods for Large-Scale Spatially Explicit Biofuels Network Design

The size and complexity of energy system optimization models have increased significantly in recent years, driven by the availability of high-resolution spatial data. We present complexity reduction and solution methods that enable us to efficiently represent high-resolution spatial data in the network design of large-scale energy systems. We aim to reduce the size and enhance the computational efficiency of network design models without sacrificing solution accuracy. Specifically, we first present how to aggregate highly granular data into larger resolutions without averaging out their specific properties through a composite-curve-based approach and then develop a method to linearly represent these curves. Second, we utilize a general clustering method to determine groups of geographically proximate biomass fields and establish a single transportation arc for all of them, reducing the number of transportation-related variables while maintaining an accurate representation of the system. Finally, we introduce a two-step algorithm that decomposes large-scale network design problems into two smaller, more manageable subproblems. We demonstrate the application of our methods using a case study of switchgrass-to-biofuels network design in the eight states of the U.S. Midwest, using realistic and highly explicit spatial data.

09 BIOMASS FUELS↗

Nanoscale Antiferromagnetic Domain Imaging using Full-Field Resonant X-ray Magnetic Diffraction Microscopy

The physical properties of magnetic materials frequently depend not only on the microscopic spin and electronic structures, but also on the structures of mesoscopic length scales that emerge, for instance, from domain formations, or chemical and/or electronic phase separations. However, experimental access to such mesoscopic structures is currently limited, especially for antiferromagnets with net zero magnetization. Here, full-field microscopy and resonant magnetic X-ray diffraction are combined to visualize antiferromagnetic (AF) domains of the spin–orbit Mott insulator Sr 2 IrO 4 with area over ≈0.1 mm 2 and with spatial resolution as high as ≈150 nm. With the unprecedented wide field of views and high spatial resolution, an intertwining of two AF domains on a length comparable to the measured average AF domain wall width of 545 nm is revealed. This mesoscopic structure comprises a substantial portion of the sample surface, and thus can result in a macroscopic response unexpected from its microscopic magnetic structure. In particular, the symmetry analysis presented in this work shows that the inversion symmetry, which is preserved by the microscopic AF order, becomes ill-defined at the mesoscopic length scale. We report this result underscores the importance of this novel technique for a thorough understanding of the physical properties of antiferromagnets.

36 MATERIALS SCIENCE↗

Probing molecular vibrations by monochromated electron microscopy

Chemical bonds fundamentally determine molecular properties and are prevalently characterized by various spectroscopic means such as infrared and Raman spectroscopies. However, the spatial resolution of these conventional approaches is insufficient to reveal nanoscale features. Recently, monochromated electron energy-loss spectroscopy (EELS) in the transmission electron microscope achieved a groundbreaking energy resolution of a few millielectronvolts and enabled direct observation of molecular vibrational spectrum with unmatched spatial resolution. Vibrational EELS is widely applicable to both organic and inorganic matter in the solid state or liquid phase. In this study, we introduce recent advancements and key concepts of this method, compare with other spectroscopic techniques, and discuss future developments for potential applications in research fields centered on catalysts, polymers, and live cells.

Vibrational Spectroscopy↗

4D Imaging of ZnO-Coated Nanoporous Al 2 O 3 Aerogels by Chemically Sensitive Ptychographic Tomography: Implications for Designer Catalysts

The 3D chemical structure (4D spectromicroscopy) of nanoporous Al 2 O 3 aerogels coated with ZnO by atomic layer deposition (ALD) was studied by multienergy scanning transmission X-ray microscopy. These materials are representative of a class of designer catalysts in which the nanoporous support is prepared separately from the active catalyst material, which is subsequently introduced by ALD, thereby allowing independent optimization of the morphology, chemistry, and spatial distribution of the support and catalyst. The samples studied were prepared by Ga ion and Xe plasma focused ion beam (FIB) milling as well as drop casting from water suspension. Zn L and Al K edge spectra of six samples with three different ZnO loadings were measured to investigate how loading and different sample preparation methods affect the 3D distribution of the ZnO and Al 2 O 3 . Scanning transmission X-ray microscopy (STXM) and ptychographic imaging at two energies each at the Zn L 3 and Al K edge were measured. The ptychography data were analyzed by using the SHARP reconstruction code to generate quantitative 2D chemical maps of the Al 2 O 3 and the ZnO. The STXM and ptychography maps were then measured at a sequence of tilt angles, covering up to 160° of rotation. The 3D structure of the ZnO and Al 2 O 3 was derived from the tilt series data by tomographic reconstruction using a compressed sensing algorithm. A twodimensional spatial resolution (half-period) of 6 nm, measured by Fourier ring correlation, and a 3D spatial resolution (half-period) of 9 nm, measured by Fourier shell correlation, were achieved when using the COSMIC beamline at the Advanced Light Source (ALS). The results show that for all of the ZnO loadings studied there is nonuniform coverage of the ZnO on the Al 2 O 3 aerogel framework. In addition, we found that both FIB methods create sample artifacts, although the distortion was less with Xe plasma than Ga ion FIB.

36 MATERIALS SCIENCE↗

From zonal to nodal capacity expansion planning: Spatial aggregation impacts on a realistic test-case

Solving power system capacity expansion planning (CEP) problems at realistic spatial resolutions is computationally challenging. Thus, a common practice is to solve CEP over zonal models with low spatial resolution rather than over full-scale nodal power networks. Due to improvements in solving large-scale stochastic mixed integer programs, these computational limitations are becoming less relevant, and the assumption that zonal models are realistic and useful approximations of nodal CEP is worth revisiting. Here, this work is the first to conduct a systematic computational study on the assumption that spatial aggregation can reasonably be used for ISO-scale CEP. By considering a realistic, large-scale test network based on the state of California with over 8000 buses, we find that well-designed small spatial aggregations can yield good approximations but that coarser zonal models may result in large distortions of investment decisions, e.g., capacity under-investment of up to 41% for the lowest resolution model considered.

24 POWER TRANSMISSION AND DISTRIBUTION↗

Machine learning reveals strong grid-scale dependence in the satellite N d –LWP relationship

The relationship between cloud droplet number concentration ( N d ) and liquid water path (LWP) is highly uncertain yet crucial for determining the impact of aerosol-cloud interactions (ACI) on Earth's radiation budget. The N d -LWP relationship is examined using a machine learning (ML) random forest model applied to five years of satellite data at grid resolutions ranging from 10° to 0.05° in 12 distinct regions. In the subtropics, the shape of the N d -LWP relationship switches from an inverted-V at 1° grid-resolution to an “M” shape at 0.1° resolution with decreased $\frac{\textrm{dln⁡LWP}}{\textrm{dln⁡}N_d}$ sensitivity. Tropical and midlatitude regions generally show a more positive sensitivity. Cloud sampling and filtering also influence this slope, wherein the exclusion of thin clouds, as commonly performed to reduce retrieval uncertainty, leads to strongly negative sensitivity across all regions. Precipitation is primarily responsible for driving the strength of the sensitivity, with strong positive slopes in raining clouds and negative and/or neutral responses found in non-raining clouds. A new method to compute radiative forcing from the ML model shows a robust Twomey radiative forcing across all regions and grid resolutions. However, LWP and cloud fraction adjustments to the radiative forcing, which are ∼50 % or smaller than the Twomey effect, decrease to negligible values with higher spatial resolution data. As Earth system models move toward higher spatial resolutions in the future, evaluating the LWP and CF adjustment contributions to the radiative forcing budget at these finer resolutions will be essential for evaluation and model development.

Aerosol-Cloud Interactions↗

Spatial structure, sampling design and scale in remotely-sensed imagery of a California savanna woodland

This article describes research related to sampling techniques for establishing linear relations between land surface parameters and remotely-sensed data. Predictive relations are estimated between percentage tree cover in a savanna environment and a normalized difference vegetation index (NDVI) derived from the Thematic Mapper sensor. Spatial autocorrelation in original measurements and regression residuals is examined using semi-variogram analysis at several spatial resolutions. Sampling schemes are then tested to examine the effects of autocorrelation on predictive linear models in cases of small sample sizes. Regression models between image and ground data are affected by the spatial resolution of analysis. Reducing the influence of spatial autocorrelation by enforcing minimum distances between samples may also improve empirical models which relate ground parameters to satellite data.

Mcgwire, K.↗

Sub-millimeter resolution SiPM-based neutron anger camera

Thermal and cold neutron beamlines require detector systems that have a high neutron efficiency, large active area, and good spatial resolution. One type of detector that has been implemented at beamlines at the Spallation Neutron Source (SNS) is a scintillator-based Anger camera that utilizes photomultiplier tubes (PMTs) as photodetectors. In this work, we present a new Anger camera design that replaces PMTs with silicon photomultipliers (SiPMs). This new design offers better resolution, less distortion, and more compactness than the previous cameras. A camera with active area of ~100 cm 2 was shown to have a spatial resolution better than 0.5 mm. Additionally, the use of SiPMs allows for use in strong magnetic fields, opening the possibility of additional experimental capabilities. In conclusion, prototype has been built that demonstrates vacuum-compatibility, as required for a proposed beamline for the Second Target Station at SNS.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Subnanometer Visualization of Spatially Varying Local Field Resonances that Drive Tip-Enhanced Optical Spectroscopy

Our knowledge of the electromagnetic fields that power modern nanoscale optical measurements, including (non)linear tip-enhanced Raman and photoluminescence, chiefly stems from numerical simulations. Aside from idealized in silico vs heterogeneous (nano)structures in the laboratory, challenges in quantitative descriptions of nanoscale light–matter interactions more generally stem from the very nature of the problem, which lies at the interface of classical and quantum theories. This is particularly the case in ultrahigh spatial resolution measurements that are sensitive to local optical field variations that take place on subnanometer length scales. Here this work approaches this challenge through extinction-based spectral nanoimaging experiments. We demonstrate <1 nm spatial resolution in hyperspectral extinction measurements that track spatially varying plasmon resonances. We describe the principles behind our experiments and highlight more general implications of our observations.

77 NANOSCIENCE AND NANOTECHNOLOGY↗