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All sources NASA NTRS DOE OSTI

DOE OSTI2020

The role of turbulent fluctuations in aerosol activation and cloud formation

Aerosol indirect effects are one of the leading contributors to cloud radiative properties relevant to climate. Aerosol particles become cloud droplets when the ambient relative humidity (saturation ratio) exceeds a critical value, which depends on the particle size and chemical composition. In the traditional formulation of this problem, only average, uniform saturation ratios are considered. Using experiments and theory, we examine the effects of fluctuations, produced by turbulence. Our measurements, from a multiphase, turbulent cloud chamber, show a clear transition from a regime in which the mean saturation ratio dominates to one in which the fluctuations determine cloud properties. The laboratory measurements demonstrate cloud formation in mean-subsaturated conditions (i.e., relative humidity <100%) in the fluctuation-dominant activation regime. The theoretical framework developed to interpret these measurements predicts a transition from a mean- to a fluctuation-dominated regime, based on the relative values of the mean and standard deviation of the environmental saturation ratio and the critical saturation ratio at which aerosol particles activate or become droplets. The theory is similar to the concept of stochastic condensation and can be used in the context of the atmosphere to explore the conditions under which droplet activation is driven by fluctuations as opposed to mean supersaturation. Overall, it provides a basis for future development of cloud droplet activation parameterizations that go beyond the internally homogeneous parcel calculations that have been used in the past.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1990

Relationship between the longwave cloud radiative forcing at the surface and the top of the atmosphere

In order to achieve global coverage, any surface radiation climatology has to be based on satellite observations. In the last decade several schemes have been devised to obtain the surface solar insolation from top of the atmosphere reflected solar radiation. More recently, attempts have been made to infer the components of longwave radiation at the surface from satellite sounder data using a radiative transfer model. In addition to the radiative transfer scheme, these methods require assumptions about the effective emitting temperature of cloud tops and bases. Modeling studies have shown that although there are strong correlations between the solar upwelling radiative flux and surface flux, this is not true of the longwave. However, if the clear sky component is considered separately such that the cloud longwave forcing at the top and at the surface are compared, a slightly different picture emerges. During the FIRE Cirrus IFO, surface radiation measurements were made at several sites and coincident satellite overpass data was also collected. It may be possible to extract the longwave cloud radiative forcing at the top and surface from these data. If relationships are verifiable by observations, this information can be useful for the extraction of the surface longwave radiation from satellite data. The radiative transfer schemes used to convert upwelling spectral radiances into a downwelling longwave radiation can provide the clear sky component. The cloud radiative forcing at the top of the atmosphere can then modify the surface fluxes according to relationships shown. It should be noted that this procedure may be considered only for temporal averages and not for instantaneous deductions of surface fluxes. This would be most useful in compiling monthly mean regional climatologies of the surface longwave fluxes.

HARSHVARDHAN↗

DOE OSTI2022

Physics-guided machine learning for improved accuracy of the National Solar Radiation Database

The National Solar Radiation Database (NSRDB) provides high-resolution spatiotemporal solar irradiance data for the entire globe. The NSRDB uses a two-step Physical Solar Model (PSM) to compute the effects of clouds and other atmospheric variables on the solar radiation reaching the surface of the Earth. Physical and optical cloud properties are fundamental inputs to the PSM and are derived from the National Oceanic and Atmospheric Administration's Geostationary Operational Environmental Satellites. This paper describes recent improvements to the NSRDB driven by physics-guided machine learning methods for cloud property retrieval. The impacts of these new methods on the NSRDB irradiance data are validated using an extensive set of ground measurement sites, showing significant improvement for all sites. We report on average, the mean absolute percentage error for global horizontal irradiance and direct normal irradiance show reductions of 2.16 and 3.95 percentage points respectively for all daylight conditions, 5.92 and 17.39 percentage points respectively for cloudy conditions, and 9.00 and 22.59 percentage points respectively for gap-filled cloudy conditions. These new methods will help improve the quality and accuracy of the irradiance and cloud data in the NSRDB.

14 SOLAR ENERGY↗

DOE OSTI2020

Revisiting particle dry deposition and its role in radiative effect estimates

Wet and dry deposition remove aerosols from the atmosphere, and these processes control aerosol lifetime and thus impact climate and air quality. Dry deposition is a significant source of aerosol uncertainty in global chemical transport and climate models. Dry deposition parameterizations in most global models were developed when few particle deposition measurements were available. However, new measurement techniques have enabled more size-resolved particle flux observations. We combined literature measurements with data that we collected over a grassland in Oklahoma and a pine forest in Colorado to develop a dry deposition parameterization. We find that relative to observations, previous parameterizations overestimated deposition of the accumulation and Aitken mode particles, and underestimated in the coarse mode. These systematic differences in observed and modeled accumulation mode particle deposition velocities are as large as an order of magnitude over terrestrial ecosystems. As accumulation mode particles form most of the cloud condensation nuclei (CCN) that influence the indirect radiative effect, this model-measurement discrepancy in dry deposition alters modeled CCN and radiative forcing. We present a revised observationally driven parameterization for regional and global aerosol models. Using this revised dry deposition scheme in the Goddard Earth Observing System (GEOS)-Chem chemical transport model, we find that global surface accumulation-mode number concentrations increase by 62% and enhance the global combined anthropogenic and natural aerosol indirect effect by −0.63 W m −2 . Our observationally constrained approach should reduce the uncertainty of particle dry deposition in global chemical transport models.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1977

Analytical prediction of moisture absorption/desorption in resin matrix composites exposed to aircraft environments

The moisture absorption/desorption behavior of resin matrix composites was mathematically modeled by classical diffusion theory using an effective diffusion coefficient. Good agreement was found between calculated moisture content and published data for T300/5208 graphite fiber reinforced epoxy matrix composite. Weather Bureau data for Langley Air Force Base and Norfolk, Va., were used to calculate the amount of moisture a T300/5208 composite panel would contain if exposed outdoors. Results obtained by using average monthly weather data for several high aircraft usage locations around the world suggest that, except for desert areas, geographical locations should have only minimal effect on the moisture absorption level reached in composites. Solar radiation data together with cloud and wind information were included in the analysis to estimate an effective temperature of the composite panel during ground exposure.

Unnam, J.↗

DOE OSTI2026

SPARTAN and IMPROVE Comparison Experiment (SPICE) Interim Campaign Report

SPICE (the SPARTAN and IMPROVE Comparison Experiment) aims to obtain and quantify comparisons between aerosol PM 2.5 mass concentration measurements from the University of Oklahoma (OU) Surface Particulate Matter Network (SPARTAN) station and the U.S. Environmental Protection Agency (EPA) Interagency Monitoring of Protected Visual Environments (IMPROVE) station hosted by the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) User Facility at ARM’s Southern Great Plains (SGP) observatory in Oklahoma. Aerosols—both natural and anthropogenic—affect human populations in multiple ways. Much of ARM’s research focuses on how aerosols influence weather and climate through their optical and radiative effects, as well as their impacts on clouds and precipitation. However, aerosols also pose direct risks to humans and other organisms through inhalation, with the severity of health impacts depending on particle size, chemical composition, and duration of exposure. The IMPROVE network was established by the U.S. EPA to monitor air quality, including visible clarity as well as total and chemically speciated aerosol mass concentrations. The ARM SGP site hosts the IMPROVE SOGP station. Separately, the SPARTAN network operates a globally distributed set of stations similar to IMPROVE but with an emphasis on remote deployment and semi-autonomous operation for use beyond the borders of the United States (IMPROVE only operates within the U.S.). The University of Oklahoma operates a SPARTAN station. To establish confidence in the OU SPARTAN instrumentation and measurement protocol relative to the EPA-certified IMPROVE station, the OU SPARTAN station is currently deployed at SGP in close proximity to the IMPROVE SOGP station. The SPICE campaign was envisioned as a contiguous calendar-year effort for 2025 to capture seasonal variation in mass loading as well as composition. However, independent of the SPICE campaign, the SPARTAN network adopted a new filter construction part-way through the year, interrupting our contiguous data set. Thus, to obtain a contiguous data set with a uniform consistent configuration, SPICE desires an extension through 2026.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

General circulation models simulate negative liquid water path–droplet number correlations, but anthropogenic aerosols still increase simulated liquid water path

General circulation models' (GCMs) estimates of the liquid water path adjustment to anthropogenic aerosol emissions differ in sign from other lines of evidence. This reduces confidence in estimates of the effective radiative forcing of the climate by aerosol–cloud interactions (ERFaci). The discrepancy is thought to stem in part from GCMs' inability to represent the turbulence–microphysics interactions in cloud-top entrainment, a mechanism that leads to a reduction in liquid water in response to an anthropogenic increase in aerosols. In the real atmosphere, enhanced cloud-top entrainment is thought to be the dominant adjustment mechanism for liquid water path, weakening the overall ERFaci. We show that the latest generation of GCMs includes models that produce a negative correlation between the present-day cloud droplet number and liquid water path, a key piece of observational evidence supporting liquid water path reduction by anthropogenic aerosols and one that earlier-generation GCMs could not reproduce. However, even in GCMs with this negative correlation, the increase in anthropogenic aerosols from preindustrial to present-day values still leads to an increase in the simulated liquid water path due to the parameterized precipitation suppression mechanism. This adds to the evidence that correlations in the present-day climate are not necessarily causal. We investigate sources of confounding to explain the noncausal correlation between liquid water path and droplet number. These results are a reminder that assessments of climate parameters based on multiple lines of evidence must carefully consider the complementary strengths of different lines when the lines disagree.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1972

The infrared spectrum of Jupiter - Structure and radiative properties of the clouds.

A model of the structure and radiative properties of the Jovian clouds is described that is inhomogeneous both laterally and vertically. Radiative transfer calculations are presented which include cloud effects and show that the model can account for available observations at all wavelengths.

Taylor, F. W.↗

NASA NTRS1981

Remote sensing of sea surface temperature in the 3.7 micron CO2 band

The main sources of error in remote sensing of sea surface temperature are discussed. The interfering effects of reflected solar radiation, reflected thermal flux, clouds and haze and atmospheric attenuation are examined. The components of measured sea surface radiances, such as clear column radiance, surface emission, atmospheric emission, reflected thermal downward flux, and reflection of solar flux, are analytically presented. The use of the 3.7 micron region window to obtain the radiance to four percent accuracy is discussed. The advantages to be obtained by the use of narrow bandpass channels are assessed.

Chahine, M. T.↗

NASA NTRS1989

A study of the effect of synoptic scale processes in GCM modelling

Research was conducted to help modeling groups at NASA to develop better weather forecasting and general circulation models (GCM) for activities relating to the meteorological uses of satellite data. The focus was on the physical processes that were being simulated by models: radiative effects and latent heat release associated with clouds; orographic influences; and heat transfer at the ocean and ice surfaces. An attempt was made to deduce the role of diabatic heating in North Atlantic cyclogenesis and in the global heat budget. Inferences were made in four studies: heat budget statistics from GCM assimilations; dynamics of north Atlantic cyclones; Cage-type energy budget calculations; and grid scale cloud formation. Mechanisms that were responsible for the variability and structure of the atmospheric on a hemispheric scale were studied by a hybrid of statistical analysis and theoretical modeling. Variability and structure are both related to synoptic scale processes through baroclinic and barotropic energy transformations.

Herman, Gerald F.↗

NASA NTRS1990

Calculations of atmospheric radiative flux profiles

Results are presented of experiments with a diagnostic approach to the radiation budget by using all available data sets to describe the properties of the atmosphere, clouds, and surface at each time and place, together with a radiative transfer model that calculates the radiative fluxes using this information. Each parameter in the calculations is represented explicitly, so that improved data sets can be easily substituted. The model and data are combined to calculate profiles of radiative fluxes, including individual flux components, heating/cooling rates, as well as top-of-atmosphere and surface radiation budget components. The advantage of this explicit approach is that all contributions to the radiation budget can be diagnosed separately; in particular, cloud-radiative feedbacks can be isolated from the effects of other atmospheric and surface changes.

Rossow, William B.↗

NASA NTRS1990

Is there a cirrus small particle radiative anomaly?

Earlier studies of fundamental radiative properties of cirrus clouds suggest the presence of a significant radiative effect produced by small ice crystals of sizes below the detection thresholds of currently available in situ probes. This paper examines visible versus IR radiation relationships to explain the nature and implications of the cirrus small-particle radiative anomaly. It is concluded that the apparent phenomenon of cirrus small particle radiative anomaly is likely due to the approximate treatment of the radiative properties of actual cirrus particles.

Sassen, Kenneth↗

NASA NTRS1993

Earth observing scanning polarimeter

Climate forcing by tropospheric aerosols is receiving increased attention because of the realization that the climate effects may be large, while our knowledge of global aerosol characteristics and temporal changes is very poor. Tropospheric aerosols cause a direct radiative forcing due simply to their scattering and absorption of solar radiation, as well as an indirect effect as cloud condensation nuclei which can modify the shortwave reflectivity of clouds. Sulfate aerosols tend to increase planetary albedo through both the direct and indirect effects; a cooling due to anthropogenic sulfate aerosols has been estimated of order 1 W/sq m, noting that this is similar in magnitude to the present anthropogenic greenhouse gas warming. Other aerosols, including those from biomass burning and wind-blown desert dust are also of potential climatic importance. At present, the only global monitoring of tropospheric aerosols is a NOAA operational product, aerosol optical thickness, obtained using channel-1 (0.58-0.68 mu m) radiances from the AVHRR. With this single channel radiance data, one must use an approach which is based on the inferred excess of reflected radiance owing to scattering by the aerosols over that expected from theoretical calculations. This approach is suited only for situations where the surface has a low albedo that is well known a priori. Thus, the NOAA operational product is restricted to coverage over the ocean at AVHRR scan angles well away from sun glint, and aerosol changes are subject to confusion with changes caused by either optically thin or subpixel clouds. Because optically thin aerosols have only a small effect on the radiance, accurate measurements for optical thickness less than 0.1 (which is a typical background level) are precluded. Moreover, some of the largest and most important aerosol changes are expected over land. The Earth Observing Scanning Polarimeter (EOSP) instrument, based upon design heritage and analysis techniques developed for planetary missions, will retrieve tropospheric aerosol characteristics from measurements of multispectral radiance and polarization. Moreover, the same radiance and polarization measurements will also provide very precise information on cloud properties and maps of surface characteristics for cloud-free regions. These capabilities also give EOSP the unique ability to discriminate aerosol from clouds and surface.

Travis, Larry↗

NASA NTRS2008

The Influence of Radiation on Ice Crystal Spectrum in the Upper Troposphere

This theoretical study is carried out to investigate the effect of radiation on ice crystal spectrum in the upper troposphere. First, an explicit expression is obtained for the ice crystal growth rate that takes account of radiative and kinetic effects. Second, the expression is used to quantitatively analyze how radiation broadens the ice crystal spectrum and then reveal a new precipitation mechanism in the upper troposphere and the stratosphere. Third, the radiative effect is used to explain the subvisual clouds near the tropopause.

Zeng, Xiping↗

NASA NTRS2012

Remote Measurement of Pollution-A 40-Year Langley Retrospective: Aerosols and Clouds - Part 2

A workshop was convened in 1971 by the National Aeronautics and Space Administration (NASA) on the Remote Measurement of Pollution (RMOP), and the findings and recommendations of its participants are in a NASA Special Publication (NASA SP-285). The three primary workshop panels and their chairmen were focused on trace gas species (Will Kellogg), atmospheric particulates or aerosols (Verner Suomi), and water pollution (Gifford Ewing). Many of the workshop participants were specialists in the techniques that might be employed for regional to global-scale, remote measurements of the atmospheric parameters from Earth-orbiting satellites. In 2011 the author published a 40-year retrospective (or Part I) of the instrumental developments that were an outgrowth of the RMOP panel headed by Will Kellogg, i.e., on atmospheric temperature and gaseous species. The current report (or Part II) is an analogous retrospective of the vision of the panel led by Verner Suomi for the measurement of particulates (or aerosols) and clouds and for their effects on Earth s radiation budget. The class of measurement techniques includes laser radar or lidar, solar occultation, limb emission and scattering, nadir-viewing photometry or radiometry, and aerosol polarimetry. In addition, the retrospective refers to the scientific imperatives that led to those instrument developments of 1971-2010. Contributions of the atmospheric technologists at the Langley Research Center are emphasized, and their progress is placed in the context of the parallel and complementary work from within the larger atmospheric science community.

Remsberg, Ellis E.↗

NASA NTRS2024

General Circulation Models Simulate Negative Liquid Water Path–Droplet Number Correlations, but Anthropogenic Aerosols Still Increase Simulated Liquid Water Path

General circulation models↗

NASA NTRS1993

Radiative feedback of polar stratospheric clouds on Antarctic temperatures

A one-dimensional time marching radiative transfer model has been used to investigate the potential effects of polar stratospheric clouds (PSCs) on winter and spring temperatures in the Antarctic lower stratosphere. High, middle, and low PSC amounts were specified from lidar backscatter profiles and were chosen to represent the likely range of PSC amounts present in the Antarctic region. The computed effects of the PSCs on temperatures depend strongly on the surface temperature and on the extent of tropospheric cloudiness, and range from a maximum increase of 6 K for a high amount of PSCs over a warm surface and clear troposphere to a maximum decrease of 2 K for a high amount of PSCs over a cold surface and a troposphere with high clouds. The average effect is unlikely to be more than a 1 or 2 K temperature change.

Rosenfeld, Joan E.↗

NASA NTRS1994

Coolness in the tropical Pacific during an El Nino episode

The response of radiation budgets to changes in water vapor and clouds in an El Nino episode is investigated using the analyzed sea surface temperature (SST) and satellite-derived clouds and the earth radiation budgets for the tropical Pacific (30 deg N-30 deg S, 100 deg E-100 deg W). Analyses are performed for April 1985 and April 1987. The former is a non-El Nino year and the latter is an El Nino year. Compared to April 1985, when the SST over the central and eastern equatorial Pacific is approximately 2 C lower, the high-level cloudiness in April 1987 increases in the central and eastern equatorial Pacific. Corresponding to the increase in cloudiness, the outgoing longwave radiation and the net downward solar radiation at the top of the atmosphere decrease. The patterns of these changes are reversed in the western tropical Pacific and the Northern Hemispheric (NH) subsidence region centered at approximately 20 deg N, indicating an eastward shift of the convection center from the maritime continents to the central equatorial Pacific and a strengthened NH Hadley circulation. The earth-atmosphere system in the region receives less radiative energy by 4 W/sq m in the warmer month of April 1987 than in the month of April 1985, which is primarily caused by a reduced atmospheric clear sky greenhouse effect in the NH tropical Pacific in April 1987. Clouds have strong effects on both the IR and solar radiation, but the net effect on the radiation budget at the top of the atmopshere changes only slightly between April 1985 and April 1987. The results are consistent with Lindzen's hypothesis that reduced upper-tropospheric water vapor in the vicinity of the enhanced convection region produces cooling that counteracts warming in the Tropics.

Chou, Ming-Dah↗