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Digital Inject Book is a software program designed to generate and managed simulated data for radiation detectors, used to increase the realism of training where real radiation sources are impractical, expensive, or simply not available.
BNL has started growing CdZnTeSe crystals for room-temperature radiation detector applications. The addition of Se to CdTe reduces the concentration of secondary phases and sub-grain boundary networks. The addition of Zn increases the energy band gap. Material characterization to understand the limiting factors of radiation detection material and to improve the properties continues to be a core element of an extensive R&D program at the LBNL’s ALS and BNL’s NSLS-II synchrotron facilities. ALS’s Beamline 3.3.2 is available for 60% of its beamtime and allows us to perform both White Beam X-ray Diffraction Topography and Micron Scale X-ray Detector Mapping. The latter technique is extremely useful when measuring scintillators because it allows us to subtract contributions from the variability in the counting statistics, and also the fluctuations due to delta electrons, and non-proportionality. BNL has recently developed a new type of thermal neutron detector using pad technology in combination with 3 He gas operated in ionization mode. The new detector is used for coded aperture thermal neutron imaging.
The Majorana Collaboration is building the Majorana Demonstrator, a 60 kg array of high purity germanium detectors housed in an ultra-low background shield at the Sanford Underground Laboratory in Lead, SD. The Majorana Demonstrator will search for neutrinoless double-beta decay of 76Ge while demonstrating the feasibility of a tonne-scale experiment. It may also carry out a dark matter search in the 1-10 GeV/c² mass range. We have found that customized Broad Energy Germanium (BEGe) detectors produced by Canberra have several desirable features for a neutrinoless double-beta decay experiment, including low electronic noise, excellent pulse shape analysis capabilities, and simple fabrication. We have deployed a customized BEGe, the Majorana Low-Background BEGe at Kimballton (MALBEK), in a low-background cryostat and shield at the Kimballton Underground Research Facility in Virginia. This paper will focus on the detector characteristics and measurements that can be performed with such a radiation detector in a low-background environment.
The time dependent thermal equations of two types of conical radiation detectors are discussed and solved for a step function application of radiation parallel to the axis of the cases. The first type has a heat sink at the base and the second has the vertex buried in a heat sink to a variable proportion of its total height. It is found that the first case has the lower sensitivity and better time response. The time response of the second case is improved by more deeply burying the vertex, but to the detriment of sensitivity. At no value of this inclusion can both a superior sensitivity and time response be achieved for the second case.
Photoelectric detectors and their operation are described, with emphasis on photomultipliers, infrared radiation detectors, and photoelectric photometers.
A solid-state radiation detector includes a pattern of conductive metal on a zinc oxide substrate. The pattern provides an arrangement of interdigitated electrode fingers. The wide band gap substrate is sensitive to UV light, which can cause a conductivity change in the substrate. The electrode fingers are configured to sense a difference in substrate conductivity resulting from UV light. The detector has a fast response time, which enables it to detect Cherenkov light. The compact detector provides savings on size, weight, and required power. Thus, the solid-state detector can be used to replace photomultiplier tubes in Cherenkov detectors. The features of the novel detector allow for an improved system to detect and monitor UV radiation, especially during deep space missions.
While calibrating a High Purity Germanium (HPGe) Radiation Detector for Xenon-133 (133Xe) the process of random summing occurs which leads to excess counts in the 160.6keV peak from random summing of the 81keV photons at the 162keV energy. Multiple samples of 133Xe with varying levels of radioactivity were assayed to determine a relationship between the occurrence of random summing and the net area of the 160.6keV peak. When the calculated efficiencies in the 160.6keV peak were compared to the theoretical efficiency obtained from a multi-energy calibration at 160.6keV, the amount of random summing could be estimated as excess observed efficiency and correlated to the sample activity. While a trend is apparent in the data, the mechanisms that contribute to the trend are still being studied so the data can be accurately correlated.
Most common ionizing radiation detectors typically rely on one of two general methods: collection of charge generated by the radiation, or collection of light produced by recombination of excited species. Substantial efforts have been made to improve the performance of materials used in these types of detectors, e.g. to raise the operating temperature, to improve the energy resolution, timing or tracking ability. However, regardless of the material used, all these detectors are limited in performance by statistical variation in the collection efficiency, for charge or photons. We examine three alternative schemes for detecting ionizing radiation that do not rely on traditional direct collection of the carriers or photons produced by the radiation. The first method detects refractive index changes in a resonator structure. The second looks at alternative means to sense the chemical changes caused by radiation on a scintillator-type material. The final method examines the possibilities of sensing the perturbation caused by radiation on the transmission of a RF transmission line structure. Aspects of the feasibility of each approach are examined and recommendations made for further work.
This project addresses the need for real time monitoring of actinide concentrations for spent fuel reprocessing utilizing alpha spectroscopy. This project specifically focuses on spent fuel reprocessing with the pyroprocessing technique that uses high temperature molten salt. Pyroprocessing uses molten salt such as lithium chloride and potassium chloride to separate out uranium and plutonium from spent fuel. To prevent any possible diversion of high purity plutonium in this process, monitoring of the actinide concentrations within the refinery are essential for safeguards and non-proliferation efforts. Alpha spectroscopy enables the identification and quantification of actinide isotopic concentrations. However, current assay methods involving intrusive sampling and ex-suit measurement require weeks to provide accurate information. A near real-time and in-situ measurement system is required to quickly quantify actinide isotopic concentrations within the salt. Semiconductor radiation detectors provide a compact, high energy resolution option for completing these measurement needs. Silicon carbide (SiC) has been shown to operate effectively at high temperatures and high chemical stability in the molten salt environment. 4H-SiC Schottky diode alpha particle detectors were fabricated and tested to determine their alpha spectroscopy capabilities. The detectors need to operate at the elevated temperatures, survive the molten salt environment, be radiation hard, and have sufficient energy resolution under all these conditions to determine isotopic concentrations. Along with the detector, a method of producing samples of the actinides in the salt is required. To produce a thin film of the actinides on the detector, which is a necessity for alpha spectroscopy, electrodeposition can be used. Electrodeposition uses an electric potential difference to selectively deposit uranium or other actinides from the salt using an anode and cathode. Deposition of the material directly onto the sensor would produce a thin film of material that would enable materials accountability measurements to be taken in real time.
This project aims to invent, model, and prototype mixed-material scintillator systems (MMSSs), a new class of radiation detectors that use heterogenous internal structures of different scintillating materials to detect additional properties of radiation. These internal structures can be produced using additive manufacture (3D printing) of scintillator, a currently emerging application of additive manufacture technology. MMSSs combine the low cost and complexity of conventional scintillation detectors with capabilities currently only available in more expensive and complex detectors. By identifying promising MMSS designs, this project will enable a new class of detectors to meet DNN’s mission needs for SNM detection.
CsPbBr3 perovskite semiconductors have emerged as a leading candidate for nextgeneration radiation detectors because of their exceptional charge transport properties, defect tolerance, and record-breaking sensitivity and energy resolution. Their long-term stability, however, is hindered by electrode-driven electrochemical decomposition, which is accelerated by moisture- and oxygen-assisted ion migration during operation. Here, we investigated organic and inorganic encapsulation strategies as both environmental barriers and means to suppress interfacial degradation pathways. Atomic layer deposition (ALD) of Al2O3 provided a conformal passivation layer that blocked environmental ingress, suppressed ionic diffusion, reduced leakage current, enhanced energy resolution and expanded the operational electric-field window beyond 5 kV∙cm1 . By contrast, organic encapsulants such as paraffin wax and polystyrene slowed moisture diffusion but did not suppress interfacial reactions, with wax extending stability to over 90 days. These results show that ALD-Al2O3 suppresses dominant interfacial degradation pathways, enabling stable, high-field operation and advancing the practical deployment of CsPbBr3 γ-ray detectors.
The design of large area transition radiation detectors for highly relativistic particles can be greatly simplified if plastic foam radiators are employed. Using electron beams with energies 1-9 GeV at the Cornell synchrotron, we have studied the properties of a large variety of transition radiators consisting of commercially available foam materials. In most cases, a measurable transition radiation signal has been observed, but only a few materials have been found to be suitable for practical purposes. The observed radiation yield is in these cases very similar to that of equivalent multifoil radiators. A detailed discussion is given of the particle detection efficiency that can be obtained with high yield foam radiators.
The Cosmic Ray Nuclei (CRN) detector was designed to measure elemental composition and energy spectra of cosmic radiation nuclei ranging from lithium to iron. CRN was flown as part of Spacelab 2 in 1985, and consisted of three basic components: a gas Cerenkov counter, a transition radiation detector, and plastic scintillators. The results of the experiment indicate that the relative abundance of elements in this range, traveling at near relativistic velocities, is similar to those reported at lower energy.
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The application of Cd0.9Zn0.1Te (CZT) single crystals, the primary choice for high-resolution, room-temperature compact gamma-ray detectors in the field of medical imaging and homeland security for the past three decades, is limited by the high cost of production and maintenance due to low detector grade crystal growth yield. The recent advent of its quaternary successor, Cd0.9Zn0.1Te1−ySey (CZTS), has exhibited remarkable crystal growth yield above 90% compared to that of ~33% for CZT. The inclusion of Se in appropriate stoichiometry in the CZT matrix is responsible for reducing the concentration of sub-grain boundary (SGB) networks which greatly enhances the compositional homogeneity and growth yield. SGB networks also host defect centers responsible for charge trapping, hence their reduced concentration ensures minimized charge trapping. Indeed, CZTS single crystals have shown remarkable improvement in electron charge transport properties and energy resolution over CZT detectors. However, our studies have found that the overall charge transport in CZTS is still limited by the hole trapping. In this article, we systematically review the advances in the CZTS growth techniques, its performance as room-temperature radiation detector, and the role of defects and their passivation studies needed to improve the performance of CZTS detectors further.
This project aimed to invent, model, and prototype architected multimaterial scintillator systems (AMSSs), a new class of radiation detectors that use heterogenous internal structures of different scintillating materials to detect additional properties of radiation. These internal structures can be produced using additive manufacture (AM, i.e. 3D printing) of scintillator, a currently emerging application of additive manufacture technology. AMSSs combine the low cost and complexity of conventional scintillation detectors with capabilities currently only available in more expensive and complex detectors. By identifying promising AMSS designs, this project enabled a new class of detectors to meet DNN’s mission needs for SNM detection.
Sterilizable solid state - scintillation crystal nuclear radiation detector for deep space missions