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At least 613 records · Page 34

A variational method for the calculation of dynamic polarizabilities and two-photon transition moments - The dressed molecule approach

The solution of the time-dependent Schroedinger equation of the molecule + radiation field system is analyzed. A quantized radiation field is used. The relationship between the oscillatory wave function and the dressed state wave function is established, the oscillatory wave function being the solution if the radiation field is turned on at t = 0 and the dressed state being the stationary solution satisfying the boundary condition only if the field is present at t = negative infinity. In general, the oscillatory wave function can be expressed using a complete set of dressed states. However, in the presence of a nonresonant radiation field, the system is well represented by a single dressed state. Molecular properties such as dynamic polarizabilities and two-photon transition moments can be deduced from the dressed state wave function instead of the oscillatory wave function as in previous methods. Because of its stationary character, the dressed state is more amenable to approximate calculations. A CI method is developed for this purpose. The CI matrix is simple in form and can be readily constructed using existing computer codes. The present method can also be adapted to calculate other optical properties.

Huo, W. M.↗

Rotationally resolved electron-photon coincidence study of H2(d 3 Pi u) excitation

The three normalized Stokes' parameters characterizing the decay of the electron impact excited d 3 Pi u (V1=O, N1=1) rotational level of H2 were determined in an electron-photon coincidence experiment at 25 eV impact energy and 60 deg scattering angle. The low degree of polarization (coherence) which was observed could be caused by both the averaging over the magnetic sublevels of the ground state of the target and the fine and hyperfine relaxation process. The average angular momentum transfer perpendicular to the scattering plane from the electrons to the molecules was found to be near zero in this excitation process.

Mcconkey, J. W.↗

New formalism for two-photon quantum optics. I - Quadrature phases and squeezed states. II - Mathematical foundation and compact notation

A new formalism for analyzing two-photon devices, such as parametric amplifiers and phase-conjugate mirrors, is proposed in part I, focusing on the properties and the significance of the quadrature-phase amplitudes and two-mode squeezed states. Time-stationary quasi-probability noise is also detailed for the case of Gaussian noise, and uncertainty principles for the quadrature-phase amplitudes are outlined, as well as some important properties of the two-mode states. Part II establishes a mathematical foundation for the formalism, with introduction of a vector notation for compact representation of two-mode properties. Fundamental unitary operators and special quantum states are also examined with an emphasis on the two-mode squeezed states. The results are applied to a previously studied degenerate limit (epsilon = 0).

Caves, C. M.↗

Theoretical study relating the two-photon absorption cross section to the susceptibility controlling four-wave mixing

A theory that it is necessary to extract a two-photon absorption cross section from a mixing signal is developed. The dependence of the cross section on the third-order susceptibility is shown and both the mixing signal and reference signal dependences on the susceptibility are given. Techniques to process the measured value of the susceptibility and relate it to the cross section are developed and limits of validity are established. Finally, a comparison is made between the expression for the cross section presently reported and values given elsewhere.

Burris, J.↗

Observations of barium ion jets in the magnetosphere using Doppler imaging systems and very sensitive imaging systems using imaging photon detectors

Observations of four shaped charge releases from rockets launched from Alaska are described. Results demonstrate that imaging and Doppler imaging instruments, based on exploiting the imaging photon detector, provide additional insight into the motion and development of low intensity targets such as the fast ion jets produced by shaped charge releases. It is possible to trace the motion of fast ion jets to very great distances, of the order of 50,000 km, outward along the Earth's magnetic field, when the conditions are suitable for the outward (upward) motion and/or acceleration of such ion jets. It is shown that ion jets, which fade below the lower sensitivity threshold of previous instruments, do not always disappear. There is no evidence of an abrupt field-aligned shear-type acceleration.

Rees, D.↗

Double photon excitation of high-Rydberg atoms as a long-lived submillimeter detector

A method and apparatus for detecting submillimeter or IR radiation is disclosed. A rare gas, such as xenon, is supplied at its ground state via a pressurized cylinder and an adjustable leak valve into a cryogenically cooled detection area. The ground state of xenon is double photon excited to a particularized level of the Rydberg series by a resonance lamp and a laser. The doubly excited gas is then further excited by the radiation to be measured. A field ionization and an ion measurement indicative of the radiation intensity is achieved.

Chutjian, A. N.↗

The joint NASA/Goddard-University of Maryland research program in charged particle and high energy photon detector technology

Progress made in the following areas is discussed: low energy ion and electron experiments; instrument design for current experiments; magnetospheric measurement of particles; ion measurement in the earth plasma sheet; abundance measurement; X-ray data acquisition; high energy physics; extragalactic astronomy; compact object astrophysics; planetology; and high energy photon detector technology.

Source record↗

A two-photon laser-induced fluorescence field instrument for ground-based and airborne measurements of atmospheric NO

This paper reports on a new two-photon laser-induced fluorescence (TP-LIF) sensor capable of making routine measurements at the few parts per trillion volume level. This direct spectroscopic detection method has been demonstrated to be a reliable instrument while performing both on the ground and in the air. As currently designed it is unique in being 'signal' rather than 'signal-to-noise' limited. The latter characteristic enables the TP-LIF sensor to make atmospheric measurements of NO under environmental conditions that might normally be considered unsuitable for a laser technique. These include clouds, rain, and, in general, high-atmospheric-aerosol loading conditions. Of special interest is the insensitivity of the TP-LIF NO instrument to changes in pressure while operating in the troposphere. This characteristic has enabled this sensor to be used to record real-time altitude profiles of NO. Future improvements should make possible two measurement opportunities: (1) NO flux measurements via the airborne eddy-correlation method and (2) nitrogen isotopic distribution measurements (e.g., (N-15)(0-16) versus (N-14)(0-16) as a means of identifying specific NO(x) sources.

Bradshaw, J. D.↗

A cooled avalanche photodiode with high photon detection probability

An avalanche photodiode has been operated as a photon-counting detector with 2 to 3 times the sensitivity of currently-available photomultiplier tubes. APD (avalanche photodiodes) detection probabilities that exceed 27% and approach 50% have been measured at an optimum operating temperature which minimizes noise. The sources of noise and their dependence on operating temperature and bias voltage are discussed.

Robinson, D. L.↗

Two-photon laser-induced fluorescence detection of OH

The TP-LIF OH sensor is based on the principle that a molecule having multiple energy states, all of which are bonding, can be pumped into the highest state with the resulting fluorescence being blue-shifted relative to all pumping wavelengths. In this way, one can successfully discriminate against virtually all noise sources in the system using long wavelength blocking filters in conjunction with solar-blind photomultiplier tubes. Thus, these systems tend to be signal limited rather than signal-to-noise limited as is true of the SP-LIF technique as well as other conventional analytical methods. The trick to achieving the above sampling scheme, with high efficiency, is in the use of high photon fluxes of short time duration. Obviously, the latter type of light source is fulfilled nicely by available pulsed lasers. From an operational point of view, however, this laser source needs to be tunable. The latter characteristic permits extremely high selectivity for the detection of a diatomic or simple polyatomic molecule by taking advantage of the high-resolution spectroscopic features of these type species.

Davis, D. D.↗

Transient response of Ge:Be and Ge:Zn FIR photoconductors under low background photon flux conditions

An experimental study of the transient behavior of Ge:Be and Ge:Zn photoconductors to changes in photon flux rates has been performed under the low background flux conditions (10 to the 8th photon/s) typical of astronomy and astrophysics applications. A characteristic transient behavior with time constants ranging from 0.1 to greater than 5 s has been observed in both materials when the shallow levels are very closely compensated. The detector response consists of both a fast and a slow component. The amplitude of the slow component can be up to 10 times greater than the initial fast component. It has been established that this phenomenon cannot be explained by current models of carrier sweep-out or dielectric relaxation. The transient behavior has been characterized as a function of temperature, electric field, photoconductive gain and material parameters.

Haegel, N. M.↗

Gamma-ray burst spectra from photon-deficient Compton scattering by nonthermal electrons

Consideration is given to a model of gamma-ray burst sources based on repeated Compton scatterings of soft photons by relativistic nonthermal electrons. Relativistic electrons which are continuously produced in the source radiate the total power L supplied to them. Higher order Compton scatterings, which occur when L(soft) is much less than L make the model distinct. The spectrum having an X-ray energy index of about one results from the superposition of the spectral components from several orders of Compton scattering; the change of the slope at several hundred keV arises from the Klein-Nishina decline of the scattering cross section.

Zdziarski, Andrzej A.↗

High energy photon and particle luminosity from active nuclei

This paper describes a numerical calculation which follows the evolution of an initial photon and particle spectrum in an expanding, relativistic wind or jet, describes in particular the quasi-equilibrium distribution found for initial optical depths above 100 or so, and points out that this calculation may be relevant for the situation in luminous, compact nuclear sources.

Eilek, J. A.↗

Wedge and strip image readout systems for photon-counting detectors in space astronomy

EUV and far UV applications of wedge and strip anodes in photon-counting microchannel plate detector systems are discussed in light of performance data obtained as a result of EUV Explorer spacecraft open face detector and FAUST-Spacelab far UV sealed tube sensor calibrations. CsI quantum detection efficiencies of about 80 percent at 114 A and about 40 percent at 600 and 1300 A have been achieved; a position sensitivity of less than 10 microns is demonstrated, and the position resolution, image linearity, background rate, and flat-field characteristics are discussed.

Siegmund, O. H. W.↗

Uncertainty relations for light waves and the concept of photons

A Lorentz-covariant localization for light waves is presented. The unitary representation for the electromagnetic four-potential is constructed for a monochromatic light wave. A model for covariant superposition is constructed for light waves with different frequencies. It is therefore possible to construct a wave function for light waves carrying a covariant probability interpretation. It is shown that the time-energy uncertainty relation (Delta-t)(Delta-omega) = about 1 for light waves is a Lorentz-invariant relation. The connection between photons and localized light waves is examined critically.

Han, D.↗

Hybrid analog/digital, large format, photon counting detectors for astronomy

The development of a new microchannel plate photon-counting detector with an analog readout method based on a resistive anode is reported. This detector exhibits extremely high, stable electron gains of 10 to the 8th. At this gain, the spatial resolution is no longer primarily limited by the noise of the resistive anode, so that digital methods of readout, such as discrete conductors, lose their advantage. These detectors can be readily scaled to 40 mm and 70 mm formats to match plate scales of 2-m (and larger) telescopes. New, high speed digital electronics fully exploit the high spatial and time resolution made possible by gains of this level. Analysis of the theoretical performance of this detector shows that the major limitation to the spatial resolution is the proximity focus of the photocathode and the first microchannel plate. The detector has been mated to an echelle spectrograph developed.

Crocker, J.↗

Imaging by time-tagging photons with the multi-anode microchannel array detector system

The capability and initial use of the Multi-Anode Microchannel Array (MAMA) detector in the time-tag mode is reported. The detector hardware currently in use consists of a visible-light detector tube with a semitransparent photocathode proximity-focused to a high-gain curved-channel microchannel plate MCP. The photoevents are detected by a (256 x 1024)-pixel coincidence-anode array with pixel dimensions of 25 x 25 microns connected to charge-sensitive amplifiers and event-detection circuitry. In the time-lag mode, the detector delivers the pixel address and the time of arrival for each detected photon to an accuracy of 10 microns. The maximum count rate is limited by the speed of data-acquisition hardware. The MAMA detector in the time-lag mode is currently being evaluated in programs of astrometry and speckle imaging.

Timothy, J. G.↗