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At least 613 records · Page 34

Numerical Simulations of Flow-Induced Deflections in MITR LEU Fuel Plate Due to Channel Size Disparity

The hydromechanical stability of the fuel plates in parallel coolant channels of a Materials Testing Reactor (MTR) fuel element design is of great importance to the safety of research and test reactors. Previous analytical, experimental, and numerical efforts focused on parallel channels with the same or similar size; also, in the prior numerical simulations, the fuel plate was often assumed to be perfectly flat. This work presents the results of a fluid-structure interaction simulation performed to evaluate the flow-induced deflections of the fuel plates in the low-enriched uranium (LEU, <20 wt% 235 U) fuel element design for the conversion (from highly enriched uranium) of the Massachusetts Institute of Technology Reactor (MITR-II, also referred to as MITR). Various manufacturing and assembly tolerances of the MITR LEU elements are considered in the analysis, and the effects of channel size disparity, nonideal plate shape, and flow rate uncertainty are investigated. Results show that, for all cases analyzed, the deflection occurs toward the larger channel, and the change in any channel stripe remains small (less than 0.021 mm) compared to fabrication tolerances. In addition to simulation work, a hydraulic performance test of the MITR LEU fuel element is currently planned to support conversion to the use of LEU fuel.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Influence of Microstructure on the Absorption of Tritium into Gold-Plated 316 Stainless Steel

The interaction of tritium with metal surfaces is the initial step in the overall absorption of tritium by the substrate metal. As a result, limiting the adsorption of tritium to the surface may effectively reduce the quantity of tritium absorbed by a metal when it is in contact with tritium gas. To limit tritium adsorption, many tritium users electroplate gold onto the substrate metal. The gold layer is expected to reduce tritium adsorption, and subsequently absorption, by reducing water adsorption. The present work shows a comparison between tritium inventories in nonplated 316 stainless steel to the inventories in 316 stainless-steel samples electroplated with gold by various commercial vendors and laboratories. Of the various gold-plated samples, only one type of plating shows ~25% reduction in tritium inventory, relative to non-plated steel samples. The degree of tritium absorption appears to be significantly influenced by the porosity, texture, and completeness of the gold layer. Incomplete and/or porous layers lead to increased absorption, while gold layers with smaller surface features lead to similar tritium inventories as non-plated samples. Furthermore, reduced tritium absorption was observed only for complete gold layers with small surface features.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Atomistic modeling of LiF microstructure ionic conductivity and its influence on nucleation and plating

We report the formation and degradation of the solid electrolyte interphase (SEI) and its underlying transport properties play an essential role in the overall performance of lithium-ion batteries. This paper presents classical molecular dynamics studies on polycrystalline inorganic lithium fluoride (LiF) layers to model and predict the SEI transport properties. The ionic conductivity is obtained from the lithium-ion diffusivity in polycrystalline structures of LiF using the Nernst-Einstein relation. The predicted molecular dynamics data are used in a continuum scale phase-field model to evaluate the plating kinetics under fast charging conditions. The analysis emphasizes that the SEI ionic conductivity properties impact the plating dynamics, where SEI's low ion conductivity value is prone to large plating and subsequent capacity degradation. The combination of atomic and continuum scale studies shown herein lays a foundation to tune in SEI transport properties to decrease the amount of lithium plating and improve the performance of fast-charging batteries.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Comparison of Planar and Tubular Flow Field Plates for Proton Exchange Membrane Fuel Cells (PEMFCs) through Simulation

Proton exchange membrane fuel cells are excellent clean energy alternatives to current non-renewable energy sources. Bipolar plates are a key component of these fuel cells and directly responsible for their performance. Traditional bipolar plates are created in a planar form, but recent research has revealed a novel tubular design that performs similarly to conventional plates. Here, this study compares traditional planar designs with tubular ones. The finite element ANSYS software was used to determine and visualize velocity and pressure distributions of fluid flow through the bipolar plate channels.

25 ENERGY STORAGE↗

Characterization of Tri-lab Tantalum Plate

This report provides a detailed characterization Tri-lab Tantalum (Ta) plate jointly purchased from HCStark Inc. by Sandia, Los Alamos and Lawrence Livermore National Laboratories. Data in this report was compiled from series of material and properties characterization experiments carried out at Sandia (SNL) and Los Alamos (LANL) Laboratories through a leveraged effort funded by the C2 campaign. Results include microstructure characterization detailing the crystallographic texture of the material and an increase in grain size near the end of the rolled plate. Mechanical properties evaluations include, compression cylinder, sub-scale tension specimen, micohardness and instrumented indentation testing. The plate was found to have vastly superior uniformity when compare with previously characterized wrought Ta material. Small but measurable variations in microstructure and properties were noted at the end, and at the top and bottom edges of the plate.

Buchheit, Thomas E.↗

Internal (Annular) and Compressible External (Flat Plate) Turbulent Flow Heat Transfer Correlations.

Here we provide a discussion regarding the applicability of a family of traditional heat transfer correlation based models for several (unit level) heat transfer problems associated with flight heat transfer estimates and internal flow heat transfer associated with an experimental simulation design (Dobranich 2014). Variability between semi-empirical free-flight models suggests relative differences for heat transfer coefficients on the order of 10%, while the internal annular flow behavior is larger with differences on the order of 20%. We emphasize that these expressions are strictly valid only for the geometries they have been derived for e.g. the fully developed annular flow or simple external flow problems. Though, the application of flat plate skin friction estimate to cylindrical bodies is a traditional procedure to estimate skin friction and heat transfer, an over-prediction bias is often observed using these approximations for missile type bodies. As a correction for this over-estimate trend, we discuss a simple scaling reduction factor for flat plate turbulent skin friction and heat transfer solutions (correlations) applied to blunt bodies of revolution at zero angle of attack. The method estimates the ratio between axisymmetric and 2-d stagnation point heat transfer skin friction and Stanton number solution expressions for sub-turbulent Reynolds numbers %3C1x10 4 . This factor is assumed to also directly influence the flat plate results applied to the cylindrical portion of the flow and the flat plate correlations are modified by

42 ENGINEERING↗

IER-297 CED-2: Final Design for Thermal/Epithermal eXperiments with Jemima Plates with Polyethylene and Hafnium

This report presents the final design (CED-2) for IER-297, and focuses on 15 critical configurations using highly enriched uranium (HEU) Jemima plates moderated by polyethylene with and without hafnium diluent. The goal of the U.S. Nuclear Criticality Safety Program’s Thermal/Epithermal eXperiments (TEX) is to design and conduct new critical experiments to address high priority nuclear data needs from the nuclear criticality safety and nuclear data communities, with special emphasis on intermediate energy (0.625 eV – 100 keV) assemblies that can be easily modified to include various high priority diluent materials. The TEX (IER 184) CED-1 Report [1], completed in 2012, demonstrated the feasibility of meeting the TEX goals with two existing NCSP fissile assets, plutonium Zero Power Physics Reactor (ZPPR) plates and highly enriched uranium (HEU) Jemima plates. The first set of TEX experiments will focus on using the plutonium ZPPR plates with polyethylene moderator and tantalum diluents.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

MLEP-Fail calibration for 1/8 inch thick cast plate of 17-4 steel.

The purpose of the work presented in this memo was to calibrate the Sierra material model Multilinear Elastic-Plastic Hardening Model with Failure (MLEP-Fail) for 1/8 inch thick cast plate of 17-4 steel. The calibration approach is essentially the same as that recently used in a previous memo using data from smooth and notched tensile specimens. The notched specimens were manufactured with three notch radii R = 1=8, 1/32 and 1/64 inches. The dimensions of the smooth and notched specimens are given in the prints in Appendix A. Two cast plates, Plate 3 and Plate 4, with nominally identical properties were considered.

42 ENGINEERING↗

Fuel Plate Surface Temperature in a Fully-Uncovered Fuel Assembly after a Loss-of-Coolant Accident in an MTR-Type Research Reactor

A methodology and model that were developed in the 1960s for calculating the peak fuel temperature in an MTR fuel assembly in a reactor core that has been fully-uncovered in a hypothetical loss-of-coolant accident (LOCA) are revived and updated in this report. The semi-empirical one-node model is based on experiments on fuel elements for the Oak Ridge Research Reactor (ORR) and the Low Intensity Testing Reactor (LITR) that were done in the 1950s and 1960s at the Oak Ridge National Laboratory. The peak plate temperature in 18 LOCA tests in the ORR and two of 24 tests in the LITR, calculated using the model, are compared with experiments. The original model was used in LOCA analyses for the Omega West Reactor (OWR) at Los Alamos National Laboratory with HEU fuel and for three cores of the University of Virginia Reactor (UVAR) with both HEU and LEU fuels. The LOCA analyses for UVAR using this model were accepted for licensing purposes by the US Nuclear Regulatory Commission for an assembly containing 12 HEU fuel plates in 1970, an assembly containing 18 HEU fuel plates in 1984, and an assembly containing 22 LEU silicide fuel plates in 1994. The analyses done for the OWR and UVAR are repeated here and compared with data in the original reports in order to establish the validity of the model revived in this report. The model is then used in a subsequent LOCA analysis for the HEU and LEU cores of the RPI MTR-type reactor in Portugal. It can also be applied to other MTR-type reactors with designs similar to the LITR.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Characterization of the Sub-mm Delay Plates for the IOTA Optical-Stochastic-Cooling Experiment

This note describes the methods used to measure the thickness profile of the glass plates used in the optical-delay line of the Optical Stochastic Cooling (OSC) experiment at the Fermilab’s IOTA ring. The plates have a nominal thickness of 250 μm and the measurement was performed to verify the nominal thickness and determine its variation over the entire plate surface. All the available plates were characterized and the impact of the thickness variation on the radiation wave front was found to be negligible using wave-optics simulation.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Effect of Lateral Conduction in a Rectangular Fuel Plate and Optimum Stripe Widths for the OPAL Reactor

The impetus for this work is the Proliferation Resistance Optimization (PRO-X) program, which was created by the National Nuclear Security Administration (NNSA) of the US Department of Energy (DOE) to provide a framework for developing reactor designs that minimize the production of special nuclear materials while maximizing performance for peaceful uses. The Argentine company INVAP and Argonne National Laboratory collaborated to share knowledge and expertise regarding the thermal analysis of research reactors. Working together, they designed a series of test problems based on the Open Pool Australian Light Water (OPAL) reactor, whose fuel is in the form of flat plates cooled by water flowing through narrow rectangular channels. ANL used their PLTEMP/ANL code. INVAP used their TERMIC code (and its new multi-plate version, TERMIC-MP). Then, INVAP and ANL compared the two sets of results. 1-D models were used during the collaboration since for research reactor analysis, largely 1-D thermal-hydraulics models are commonly used because they are simple to apply and technically defendable. The collaboration between the two organizations aims for improvements in thermal-hydraulic models. Improvements to methods and models can reduce modeling uncertainties and excessive conservatism, allowing greater reactor performance without reducing predicted safety margins. Therefore, these improvements potentially expand the design space, making additional designs feasible, which, in turn, may achieve better fuel utilization and proliferation resistance in the designs. This report provides justification for the lateral node size (stripe width) chosen for the 1-D computer models during the collaboration. The lateral heat conduction in OPAL fuel plates is evaluated using the two-dimensional conduction capability of PLTEMP/ANL to determine a representative hot-stripe width that can be conservatively used for one-dimensional steady-state thermal-hydraulic analysis. Basically, a representative hot-stripe width needs to be selected so that the actual heat flux averaged over this stripe width is greater than or equal to the maximum heat flux obtained by the two-dimensional analysis. Detailed results in this report show that a hot-stripe width of 8.125 mm can be conservatively used for the one-dimensional thermal-hydraulics analysis of all plates. Therefore, eight equal stripes (8.125 mm each) are recommended to be modeled in the MCNP and PLTEMP/ANL full core models of the OPAL reactor.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Preliminary Design of Critical Experiments Involving Commercially Available B 4 C Neutron Absorber Plates with Low-Enriched UO 2 Fuel [Slides]

Conclusions of this presentation conclude that the experiment is feasible with at least 10 critical configurations, and low expected benchmark uncertainty. Potential high impact for the understanding of commercially used neutron absorber plates. Next steps are to think about other configurations: rod pitch, other rods – Finalize plate support, uncertainty study. Additionally, the potential use of IER-441 central test region to safely place the plate in the core. Next steps include the Determination of the neutron absorber plate characterization path and the Potential SINBAD benchmark of neutron transmission measurements.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Alternate Methods for Cleaning Zirconium Plate

The United States High Performance Research Reactor Conversion Program identified the need to transition from highly enriched uranium fuel to lowly enriched uranium fuel for high power research and civil reactors. One of the fuel configurations selected for these reactors was a uranium (U) foil alloyed with 10% molybdenum (Mo). The U-10Mo fuel foil was then covered with a zirconium (Zr) interlayer and pressed into an aluminum cladding. Idaho National Laboratory prescribed a need to remove surface oxidation on the Zr prior to bonding it with U-10Mo fuel foil. To determine the best method of oxidation removal, a variety of polishing methods, including hand polishing with a diamond paste or Scotch-Brite™ pads, mechanically wet-polishing with abrasive belts, and chemical etching with hydrofluoric/nitric acid mixtures, were investigated on pre-polished Zircaloy 702 sheets purchased directly from the manufacturer. No change in surface roughness was detected using any of these methods relative to the as-received material. In fact, scanning electron microscopy detected grit from hand polishing with Amplex Grade 30 waste soluble diamond paste and Scotch-Brite™ pads. Visible staining was found, and fluorine detected via X-ray photoelectron spectroscopy on the flash etching samples. These contaminants were not seen on the as-received material. In addition to the need to remove the oxide layer on the Zr prior to co-rolling, there are concerns that the Neolube debonding agent on the co-rolling can may contaminate the Zr surface after co-rolling. The experimental results found that zirconium in contact with Neolube coated steel plates was easily cleaning with ethanol wiping after heat treated and no carbide inclusions remained on the surface. Overall, all cleaning methods tested did not significantly change the surface roughness of the plates or reduce the oxide layer present on the zirconium. Carbon was found on all the samples, before and after cleaning, except for the flash etch samples which detected fluorine instead. The insignificant changes seen in the cleaned plates relative to the as received plates question the need for cleaning prior to rolling. Further investigation in the requirements for cleaning at this step is recommended. Current methods for cleaning the surface after hot rolling with alcohol appear sufficient. After hot rolling, if Neolube does peel off the can and onto the zirconium coated foil surface, a dry abrasive or diamond paste polish is not recommended due to the chance of abrasive being embedded into the surface. However, the ability of an etchant to lift the lubricant off the zirconium surface indicates that a spot etch method could work to clean specific spots where Neolube is present, if the need arises.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Electropolishing of a Full-Sized U-10Mo Plate

Electropolishing is used to remove material from the surface of a metal using electric potential and current. U-10Mo fuel is produced from a low enriched uranium plate alloyed with 10% molybdenum (U-10Mo). Electropolishing is being considered in two steps of the process of fabricating this U-10Mo fuel. First, it could be used as a means initially improving the surface finish of the cast plate while removing smut from the casting process from the surface prior to homogenization. Second, it could be used again after homogenization to remove oxidation and continue to improve the surface finish prior to hot rolling. The purpose of this work is to demonstrate the process on full-size ingots and optimize the process. A depleted uranium U-10Mo plate was electropolished three times: the first two times were prior to homogenization and the third after a homogenization step. The first two polishes decreased the overall roughness, as measured by laser confocal microscopy. After each polish, a smoother and shinier blue-gold surface was left on the plate. Upon homogenization, the surface had a more matte appearance and the surface roughness increased back to the pre-homogenization values obtained prior to the initial polish. After electropolishing the homogenized pieces, the changes in surface roughness increased, as measured by laser confocal microscopy. The final polishing step was not long enough to return the surface roughness to pre-homogenization conditions, implying less polishing is needed before the homogenization versus afterwards. Heat generation during the polish was addressed by circulating the electrolyte solution through an external heat exchanger; however, solubility and anodization challenges require further study.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

HEU Pancake Plates

The HEU Pancake plates, formerly known as the Jemima plates, were procured in two batches. The first, consisting of the 15” plates, was ordered and produced by LANL in 1958. A second set, consisting of the 21” rings was ordered by LANL but produced by ORNL sometime in the 1960s. The plates were used at LACEF in experiments such as Big Ten and the Zeus series of experiments. In the mid-2000s, they were shipped to NCERC where they reside today. Since being at NCERC, they have been used in Zeus and TEX style experiments.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sensitivity calibration of a Carestream HPX-1 image plate scanner

There is a need to measure the sensitivity of the image plate scanners used to scan Z shot data. The Carestream HPX-1 image plate scanner was tested, and its performance was characterized to determine the system sensitivity in terms of signal per incident photon as a function of x-ray energy. A Manson source was used to simultaneously expose an Amptek x-ray multi-channel analyzer and image plates, allowing for a comparison of the counts as a function of energy to the signal recorded on the image plates. NIST-certified radioactive sources were used to assign an absolute sensitivity. Results indicate that the HPX-1 scanner response matches the shape of the modeled response, allowing for absolute scaling using NIST-certified radioisotope sources. The HPX-1 scanner shows a stable response with measurements taken over one week. In contrast, the sensitivity of the DITABIS scanner was characterized using the same approach, but it exhibits changes in its response that varied by more than 50% over the span of 4 days.

42 ENGINEERING↗

Increasing Radon Daughter Plate-out onto Superconducting Qubits

Radon daughter plate-out may pose a fundamental limitation to realizing large-scale superconducting quantum computers. Radon daughters plated-out onto a superconducting qubit chip can decay, releasing energy into the substrate, producing phonons. Phonon induced quasiparticles generate bit flip errors and reduce coherence times. We seek to increase plate-out on chips to enable future study of the impact of Radon on coherence times. In this project, we utilize COMSOL Multiphysics simulations to finalize design for a device to increase radon plate-out.

Kay, Dax [Northwestern U.]↗

Parametric Sensitivity Comparison of Simulation Models for Flyer Plate Impact Experiments

This paper compares the sensitivities of different modeling approaches for fundamental flyer plate impact experiments to variations of several input parameters. Two modeling approaches are used to model a copper flyer plate experiment: the CTH hydrodynamic code and the LS-DYNA code using the smoothed particle hydrodynamic (SPH) approach. Simulations using these two methods are compared to experimental data from a gas gun experiment in which a copper flyer plate impacted a copper target plate. The experiment was designed to cause spall in the target. Numerical simulations are conducted using typical input physics models including the Mie-Grüneisen equation of state, the Johnson-Cook compressive strength model, and a pressure cutoff (Pmin) model for tensile damage (spall). Effects of artificial viscosity, spall strength, and computational cell size are studied and discussed with the objective of improving the accuracy of these simulations.

CTH, smoothed particle hydrodynamics, SPH, Johnson↗