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At least 613 records · Page 34

Pollutant Formation in Monodisperse Fuel Spray Combustion

The combustion of liquid sprays represents an extremely important class of combustion processes. In the transition region, encompassing droplet sizes in the range of 25-80 micron diameter, the mixing and evaporation processes are both incomplete at the flame front and burning occurs in a combined diffusive and premixed fashion. Under these conditions, the relative importance of heterogeneous and homogeneous effects in dominating the combustion process is switched and gives rise to a number of interesting phenomena. NO (sub x) formation in monodisperse spray combustion was investigated with the following specific objectives: (1) to quantitatively determine the effect of droplet size, number density, etc. on NO sub x formation in monodisperse fuel spray combustion; and (2) to isolate the important physical and chemical phenomena in NO sub x formation in these combustion systems.

Cernansky, N. P.↗

Mechanisms by which heat release affects the flow field in a chemically reacting, turbulent mixing layer

The mechanisms by which heat release affects the fluid dynamics in a turbulent reacting mixing layer are studied by direct numerical simulation. In agreement with previous laboratory experiments, the heat release is observed to lower the rate at which the mixing layer grows and to reduce the rate at which chemical products are formed. The baroclinic torque and thermal expansion in the mixing layer are shown to produce changes in the flame vortex structure that act to produce more diffuse vortices than in the constant density case, resulting in lower rotation rates of fluid elements. Previously unexplained anomalies observed in the mean velocity profiles of reacting jets and mixing layers are shown to result from vorticity generation by baroclinic torques. The density reductions also lower the generation rates of turbulent kinetic energy and the turbulent shear stresses, resulting in less turbulent mixing of fluid elements. Calculations of the energy in the various wave numbers show that the heat release has a stabilizing effect on the growth rates of individual modes. A linear stability analysis of a simlified model problem confirms this, showing that low density fluid in the mixing region will result in a shift of the frequency of the unstable modes to lower wave numbers (longer wavelengths). The growth rates of the unstable modes decrease, contributing to the slower growth of the mixing layer.

Riley, J. J.↗

The use of direct numerical simulation in the study of turbulent, chemically-reacting flows

Full turbulence simulations are used here to study the effects of chemical heat release on the large-scale structures in turbulent mixing layers. In agreement with laboratory results, it is found that the heat release lowers the rate at which the mixing layer grows and reduces the rate at which chemical products are formed. The baroclinic torque and thermal expansion in the mixing layer produce changes in the flame vortex structure that act to produce more diffuse vortices than in the constant density case, resulting in lower rotation rates of the large-scale structures. Previously unexplained anomalies observed in the mean velocity profiles of reacting jets and mixing layer are shown to result from vorticity generation by baroclinic torques. Calculations of the energy in the various wavenumbers shows that the heat release has a stabilizing effect on the growth rate of individual modes. This methodology can be applied for Reynolds numbers less than several hundred and for Damkoehler numbers less than about ten.

Riley, J. J.↗

Combustion of Two-Component Miscible Droplets in Reduced Gravity

This paper presents recent theoretical and experimental results from an ongoing research program that deals with reduced-gravity combustion of bi-component droplets initially in the mm size range or larger. The primary objectives of the research are to study the effects of droplet internal flows, thermal and solutal Marangoni stresses, and species volatility differences on liquid species transport and overall combustion phenomena (e.g., gas-phase unsteadiness, burning rates, sooting, radiation, and extinction). The research program utilizes a reduced-gravity environment so that buoyancy effects are rendered negligible. Use of large droplets also facilitates visualization of droplet internal flows, which is important to this research. This program is a continuation of extensive ground based experimental and theoretical research on bi-component droplet combustion which has been ongoing for several years. The focal point of this research program is a flight experiment (Bi-Component Droplet Combustion Experiment, BCDCE). This flight experiment is still under development. However, supporting ground studies have been performed, and preliminary data have been obtained from flight experiments (Fiber Supported Droplet Combustion Experiment, FSDC-1 and FSDC-2). These flight experiments were performed during the STS-73/USML-2 and STS-94/MSL- I missions. In the experiments, droplets composed of low- and high-volatility species are burned. The low-volatility components are initially present in small amounts. As combustion of a droplet proceeds, the liquid surface mass fraction of the low-volatility component will increase with time, resulting in a sudden and temporary decrease in droplet burning rates as the droplet rapidly heats to temperatures close to the boiling point of the low-volatility component. This decrease in burning rates causes a sudden and temporary contraction of the flame. The decrease in burning rates and the flame contraction can be observed experimentally. Measurements of burning rates as well as the onset time for flame contraction allow effective liquid-phase species diffusivities to be calculated, e.g., using asymptotic theory. A goal of the research is to relate effective liquid species diffusivities to droplet internal flow characteristics. Droplet internal flows will be visualized in future flight and ground-based experiments.

Shaw, B. D.↗

Bi-Component Droplet Combustion in Reduced Gravity

This research deals with reduced-gravity combustion of bi-component droplets initially in the mm size range or larger. The primary objectives of the research are to study the effects of droplet internal flows, thermal and solutal Marangoni stresses, and species volatility differences on liquid species transport and overall combustion phenomena (e.g., gas-phase unsteadiness, burning rates, sooting, radiation, and extinction). The research program utilizes a reduced-gravity environment so that buoyancy effects are rendered negligible. Use of large droplets also facilitates visualization of droplet internal flows, which is important for this research. In the experiments, droplets composed of low- and high-volatility species are burned. The low-volatility components are initially present in small amounts. As combustion of a droplet proceeds, the liquid surface mass fraction of the low-volatility component will increase with time, resulting in a sudden and temporary decrease in droplet burning rates as the droplet rapidly heats to temperatures close to the boiling point of the low-volatility component. This decrease in burning rates causes a sudden and temporary contraction of the flame. The decrease in burning rates and the flame contraction can be observed experimentally. Measurements of burning rates as well as the onset time for flame contraction allow effective liquid-phase species diffusivities to be calculated, e.g., using asymptotic theory. It is planned that droplet internal flows will be visualized in future flight and ground-based experiments. In this way, effective liquid species diffusivities can be related to droplet internal flow characteristics. This program is a continuation of extensive ground based experimental and theoretical research on bi-component droplet combustion that has been ongoing for several years. The focal point of this program is a flight experiment (Bi-Component Droplet Combustion Experiment, BCDCE). This flight experiment is under development. However, supporting studies have been performed. Because of space limitations, only some of the research performed over the last two years (since the 5th Microgravity Combustion Workshop) is summarized here.

Shaw, B. D.↗

Flame Propagation in Low-Intensity Turbulence under Microgravity Conditions

The goal of the research is to understand the influences of the hydrodynamic instability on premixed-flame propagation. It is known that coupling between flame and flow-field dynamics in association with the hydrodynamic instability may lead to flame-generated turbulence, flame acceleration and enhancement of burning rates. As a result of such hydrodynamic coupling the transition from initially planar or wrinkled laminar flames to fast turbulent flames or detonations is possible, even when diffusive-thermal effects associated with non-unity reactant Lewis numbers are not destabilizing. It is important to identify methods of suppressing the hydrodynamic instability so as to insure fire safety, particularly in space.

Aldredge, R. C.↗

Bi-Component Droplet Combustion in Reduced Gravity

This research deals with reduced-gravity combustion of bi-component droplets initially in the mm size range or larger. The primary objectives of the research are to study the effects of droplet internal flows, thermal and solutal Marangoni stresses, and species volatility differences on liquid species transport and overall combustion phenomena (e.g., gas-phase unsteadiness, burning rates, sooting, radiation, and extinction). The research program utilizes a reduced-gravity environment so that buoyancy effects are rendered negligible. Use of large droplets also facilitates visualization of droplet internal flows, which is important for this research. In the experiments, droplets composed of low- and high-volatility species are burned. The low-volatility components are initially present in small amounts. As combustion of a droplet proceeds, the liquid surface mass fraction of the low-volatility component will increase with time, resulting in a sudden and temporary decrease in droplet burning rates as the droplet rapidly heats to temperatures close to the boiling point of the low-volatility component. This decrease in burning rates causes a sudden and temporary contraction of the flame. The decrease in burning rates and the flame contraction can be observed experimentally. Measurements of burning rates as well as the onset time for flame contraction allow effective liquid-phase species diffusivities to be calculated, e.g., using asymptotic theory. It is planned that droplet internal flows will be visualized in flight and ground-based experiments. In this way, effective liquid species diffusivities can be related to droplet internal flow characteristics. This program is a continuation of extensive ground based experimental and theoretical research on bi-component droplet combustion that has been ongoing for several years. The focal point of this program is a flight experiment (Bi-Component Droplet Combustion Experiment, BCDCE). This flight experiment is under development. However, supporting ground-based studies have been performed. This ground-based research is summarized below.

Shaw, B. D.↗

Bi-Component Droplet Combustion in Reduced Gravity

This research deals with reduced-gravity combustion of bi-component droplets initially in the mm size range or larger. The primary objectives of the research are to study the effects of droplet internal flows, thermal and solutal Marangoni stresses, and species volatility differences on liquid species transport and overall combustion phenomena (e.g., gas-phase unsteadiness, burning rates, sooting, radiation, and extinction). The research program utilizes a reduced gravity environment so that buoyancy effects are rendered negligible. Use of large droplets also facilitates visualization of droplet internal flows, which is important for this research. In the experiments, droplets composed of low- and high-volatility species are burned. The low-volatility components are initially present in small amounts. As combustion of a droplet proceeds, the liquid surface mass fraction of the low-volatility component will increase with time, resulting in a sudden and temporary decrease in droplet burning rates as the droplet rapidly heats to temperatures close to the boiling point of the low-volatility component. This decrease in burning rates causes a sudden and temporary contraction of the flame. The decrease in burning rates and the flame contraction can be observed experimentally. Measurements of burning rates as well as the onset time for flame contraction allow effective liquid-phase species diffusivities to be calculated, e.g., using asymptotic theory. It is planned that droplet internal flows will be visualized in flight and ground-based experiments. In this way, effective liquid species diffusivities can be related to droplet internal flow characteristics. This program is a continuation of extensive ground-based experimental and theoretical research on bi-component droplet combustion that has been ongoing for several years. The focal point of this program is a flight experiment (Bi-Component Droplet Combustion Experiment, BCDCE). This flight experiment is under development. However, supporting ground-based studies have been performed. Some of the most recent ground-based research is summarized.

Shaw, Benjamin D.↗

Methanol Droplet Combustion in Oxygen-Inert Environments in Microgravity

The Flame Extinguishment (FLEX) experiment that is currently underway in the Combustion Integrated Rack facility onboard the International Space Station is aimed at understanding the effects of inert diluents on the flammability of condensed phase fuels. To this end, droplets of various fuels, including alkanes and alcohols, are burned in a quiescent microgravity environment with varying amounts of oxygen and inert diluents to determine the limiting oxygen index (LOI) for these fuels. In this study we report experimental observations of methanol droplets burning in oxygen-nitrogen-carbon dioxide and oxygen-nitrogen-helium gas mixtures at 0.7 and 1 atmospheric pressures. The initial droplet size varied between approximately 1.5 mm and 4 mm to capture both diffusive extinction brought about by insufficient residence time at the flame and radiative extinction caused by excessive heat loss from the flame zone. The ambient oxygen concentration varied from a high value of 30% by volume to as low as 12%, approaching the limiting oxygen index for the fuel. The inert dilution by carbon dioxide and helium varied over a range of 0% to 70% by volume. In these experiments, both freely floated and tethered droplets were ignited using symmetrically opposed hot-wire igniters and the burning histories were recorded onboard using digital cameras, downlinked later to the ground for analysis. The digital images yielded droplet and flame diameters as functions of time and subsequently droplet burning rate, flame standoff ratio, and initial and extinction droplet diameters. Simplified theoretical models correlate the measured burning rate constant and the flame standoff ratio reasonably well. An activation energy asymptotic theory accounting for time-dependent water dissolution or evaporation from the droplet is shown to predict the measured diffusive extinction conditions well. The experiments also show that the limiting oxygen index for methanol in these diluent gases is around 12% to 13% oxygen by volume.

Nayagam, Vedha↗

A study of the propagation, dynamics, and extinguishment of cellular flames using microgravity techniques

The characteristics of premixed gas flames in mixtures with low Lewis numbers, free of natural convection effects, were investigated and found to be dominated by diffusive-thermal instabilities. For sufficiently reactive mixtures, cellular structures resulting from these instabilities were observed and found to spawn new cells in regular patterns. For less reactive mixtures, cells formed shortly after ignition but did not spawn new cells; instead these cells evolved into a flame structure composed of stationary, apparently stable spherical flamelets. As a result of these phenomena, well-defined flammability limits were not observed. The experimental results are found to be in qualitative agreement with a simple analytical model based on the interaction of heat release due to chemical reaction, differential diffusion of thermal energy and mass, flame front curvature, and heat losses due to gas radiation.

Ronney, Paul D.↗

Stability of a premixed flame in stagnation-point flow against general disturbances

Previously, the stability of a premixed flame in a stagnation flow was discussed for a restricted class of disturbances that are self-similar to the basic undisturbed flow; thus, flame fronts with corrugations only in the cross stream direction were considered. Here, we consider a more general class of three-dimensional flame front perturbations which also permits corrugations in the streamwise direction. It is shown that, because of the stretch experienced by the flame, the hydrodynamic instability is limited only to disturbances of short wavelength. If in addition diffusion effects have a stabilizing influence, as would be the case of mixtures with Lewis number greater than one, a stretched flame could be absolutely stable. Instabilities occur when the Lewis number is below some critical value less than one. Neutral stability boundaries are presented in terms of the Lewis number, the strain rate, and the appropriate wavenumbers. Beyond the stability threshold, the two-dimensional self-similar modes always grow first. However, if disturbances of long wavelength are excluded, it is possible for the three-dimensional modes to be the least stable one. Accordingly, the pattern that will be observed on the flame front, at the onset of instability, will consist of either ridges in the direction of stretch or the more common three-dimensional cellular structure.

Jackson, Thomas L.↗

Flame characteristics of a NASA contra swirler module

The structure of unconfined flames stabilized on a NASA contra-swirl can has been examined. The structure depends on reference velocity and fuel-air ratio, and photographic illustrations of representative examples of each flame type are shown. A highly compact flame is obtained over a narrow band of fuel-air ratios, within the total range over which flames may be stabilized, at high reference velocity (27.8 m/s). The compact structure can only be obtained with careful fuel nozzle location. Chemical concentration profiles, temperature profiles and sodium chloride seeding experiments all confirm the visual impression of compactness. A flame with 50% greater fuel throughput has a much less compact structure, which is reflected in lower maximum temperature, much more complex chemical concentration distributions and a more diffuse recirculation boundary as observed by sodium chloride seeding than in the compact flame. Each of these flames has not only an evident axial recirculation core but also a toroidal recirculation region over the bluff region between the inner and outer swirlers. In contrast, laser Doppler velocimetry measurements carried out on a flame with lower reference velocity (5.65 m/s) do not indicate the presence of a secondary recirculation region in this flame.

Thompson, D.↗

Effects of pressure gradients on turbulent premixed flames

The influence of a constant acceleration on a turbulent premixed flame is studied by direct numerical simulation. This acceleration induces a mean pressure gradient across the flame brush, leading to a modification of the turbulent flame structure due to differential buoyancy mechanisms between heavy cold fresh and light hot burnt gases. Such a pressure gradient may be encountered in practical applications in ducted flames. A favorable pressure gradient, i.e. the pressure decreases from unburnt to burnt gases, is found to decrease the flame wrinkling, the flame brush thickness, and the turbulent flame speed. A favorable pressure gradient also promotes counter-gradient turbulent transport. On the other hand, adverse pressure gradients tend to increase the flame brush thickness and turbulent flame speed, and promote classical gradient turbulent transport. The balance equation for the turbulent flux of the Favre averaged progress variable is also analyzed. The first results show that the fluctuating pressure term, cannot be neglected as generally assumed in models. Simple models assuming that a high mean pressure gradient may only be balanced by the cross-dissipation term seem too approximate. This analysis has to be continued to compare simulation data and closure schemes proposed for the transport equation. The analysis developed by Veynante et al.(1995) has been extended to imposed acceleration and mean pressure gradients. A simple model for the turbulent flux is proposed and validated from simulation data. Then, a modified criterion is derived to delineate between counter-gradient and gradient turbulent diffusion. In fact, counter-gradient diffusion may occur in most practical applications, especially for ducted flames.

Veynante, D.↗

Interferometer Development for Study of Interactions between Flames on Parallel Solid Surfaces

The interactions between flames spreading over parallel solid sheets of paper are being studied in normal gravity and in microgravity. This geometry provides interesting opportunities to study the interaction of radiative and diffusive transport mechanisms on the spread process. These transport mechanisms are changed when the flame interacts with other flames. Most practical heterogeneous combustion processes involve interacting discrete burning fuel elements, consequently, the study of these interactions is of practical significance. Owing largely to this practical importance, flame interactions have been an area of active research, however microgravity research has been largely limited to droplets. Consideration of flame spread over parallel solid surfaces has been limited to 1-g studies. To study the conductive transport in these flames, an interferometer system has been developed for use in the drop tower. The system takes advantage of a single beam interferometer: Point Diffraction Interferometry (PDI) which uses a portion of the light through the test section to provide the reference beam. Like other interferometric and Schlieren systems, it is a line of sight measurement and is subject to the usual edge and concentration effects. The advantage over Schlieren and shearing interferometry systems is that the fringes are lines of constant index of refraction rather than of its gradient so the images are more readily interpreted. The disadvantage is that it is less able to accommodate a range of temperature gradients.

Goldmeer, J. S.↗

Low velocity opposed-flow frame spread in a transport-controlled environment DARTFire

The overall objectives of the DARTFire project are to uncover the underlying physics and increase understanding of the mechanisms that cause flames to propagate over solid fuels against a low velocity of oxidizer flow in a low-gravity environment. Specific objectives are (1) to analyze experimentally observed flame shapes, measured gas-phase field variables, spread rates, radiative characteristics, and solid-phase regression rates for comparison with previously developed model prediction capability that will be continually extended, and (2) to investigate the transition from ignition to either flame propagation or extinction in order to determine the characteristics of those environments that lead to flame evolution. To meet the objectives, a series of sounding rocket experiments has been designed to exercise several of the dimensional, controllable variables that affect the flame spread process over PMMA in microgravity, i.e., the opposing flow velocity (1-20 cm/s), the external radiant flux directed to the fuel surface (0-2 W/cm(exp 2)), and the oxygen concentration of the environment (35-70%). Because radiative heat transfer is critical to these microgravity flame spread experiments, radiant heating is imposed, and radiant heat loss will be measured. These are the first attempts at such an experimental control and measurement in microgravity. Other firsts associated with the experiment are (1) the control of the low velocity, opposed flow, which is of the same order as diffusive velocities and Stefan flows; (2) state-of-the-art quantitative flame imaging for species-specific emissions (both infrared and ultraviolet) in addition to novel intensified array imaging to obtain a color image of the very dim, low-gravity flames.

West, Jeff↗

Diffusive and Radiative Transport in Fires Experiment: DARTFire

A low velocity, opposed-flow, flame spread experiment designed for execution on a sounding rocket is described. Early results of infrared and ultraviolet-visible imaging using video cameras and narrow band filters are described along with planned digital image data reduction. Measured and computed spread rates show that the classical thermal regime for flame spread over thick PMMA persists, for 50% O2, down to about 5 cm/s, at which point a transition to a microgravity regime in which radiation eventually leads to extinction in at least a quiescent environment. The microgravity regime of flame spread is then distinct from the thermal and kinetic regimes previously identified.

Olson, Sandra L.↗

Time-dependent computational studies of flames in microgravity

The research performed at the Center for Reactive Flow and Dynamical Systems in the Laboratory for Computational Physics and Fluid Dynamics, at the Naval Research Laboratory, in support of the NASA Microgravity Science and Applications Program is described. The primary focus was on investigating fundamental questions concerning the propagation and extinction of premixed flames in Earth gravity and in microgravity environments. The approach was to use detailed time-dependent, multispecies, numerical models as tools to simulate flames in different gravity environments. The models include a detailed chemical kinetics mechanism consisting of elementary reactions among the eight reactive species involved in hydrogen combustion, coupled to algorithms for convection, thermal conduction, viscosity, molecular and thermal diffusion, and external forces. The external force, gravity, can be put in any direction relative to flame propagation and can have a range of values. A combination of one-dimensional and two-dimensional simulations was used to investigate the effects of curvature and dilution on ignition and propagation of flames, to help resolve fundamental questions on the existence of flammability limits when there are no external losses or buoyancy forces in the system, to understand the mechanism leading to cellular instability, and to study the effects of gravity on the transition to cellular structure. A flame in a microgravity environment can be extinguished without external losses, and the mechanism leading to cellular structure is not preferential diffusion but a thermo-diffusive instability. The simulations have also lead to a better understanding of the interactions between buoyancy forces and the processes leading to thermo-diffusive instability.

Oran, Elaine S.↗

Numerical modeling of flame-balls in fuel-air mixtures

At low gravity, when buoyancy effects are small, flame-balls can be generated. These are stationary spherical structures whose existence appears to require a near-limit mixture, a small Lewis number and heat losses from radiation. It is our goal to combine computational modeling with existing experimental and theoretical studies (NASA) of these structures so that an improved understanding of flammability limits and near-limit phenomena will occur. The question of flammability limits is of fundamental importance and has long been examined. It is of great practical importance to predict, from first principles, a limit mixture strength that agrees with experimental values for the configuration at hand. Flame-balls provide an excellent configuration in which convective losses can be eliminated and the resulting stable solutions are produced from a diffusive, reactive and radiative balance. Although analytical modeling provides convincing evidence that the key physical ingredients of flame-balls have been identified, quantitative confirmation can only come from detailed numerical simulations. Our goal is to predict theoretically the mass fractions of the species and the temperature as functions of the independent coordinate r.

Smooke, Mitchell D.↗