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At least 613 records · Page 34

High Pressure Sensing and Dynamics Using High Speed Fiber Bragg Grating Interrogation Systems

Fiber Bragg gratings (FBGs) are developing into useful sensing tools for measuring high pressure dynamics in extreme environments under shock loading conditions. Approaches using traditional diode array coupled FBG interrogation systems are often limited to readout speeds in the sub-MHz range. For shock wave physics, required detection speeds approaching 100 MHz are desired. We explore the use of two types of FBG sensing systems that are aimed at applying this technology as embedded high pressure probes for transient shock events. Both approaches measure time resolved spectral shifts in the return light from short (few mm long) uniform FBGs at 1550 nm. In the first approach, we use a fiber coupled spectrometer to demultiplex spectral channels into an array (up to 12) of single element InGaAs photoreceivers. By monitoring the detectors during a shock impact event with high speed recording, we are able to track the pressure induced spectral shifting in FBG down to a time resolution of 20 ns. In the second approach, developed at the Special Technologies Lab, a coherent mode-locked fiber laser is used to illuminate the FBG sensor. After the sensor, wavelength-to-time mapping is accomplished with a chromatic dispersive element, and entire spectra are sampled using a single detector at the modelocked laser repetition rate of 50 MHz. By sampling with a 12 GHz InGaAs detector, direct wavelength mapping in time is recorded, and the pressure induced FBG spectral shift is sampled at 50 MHz. Here, the sensing systems are used to monitor the spectral shifts of FBGs that are immersed into liquid water and shock compressed using explosives. In this configuration, the gratings survive to pressures approaching 50 kbar. We describe both approaches and present the measured spectral shifts from the shock experiments.

fiber Bragg grating sensors, shockwave diagnostics↗

Broadband Laser Ranging: Signal Analysis and Interpretation

Broadband laser ranging (BLR) is essentially a spectral interferometer used to infer distance to a moving target. The light source is a mode-locked fiber laser, and chromatic dispersion maps the spectral interference pattern into the time domain, yielding chirped beat signals at the detector. A BLR record is a sequence of these chirped signals, representing consecutive target positions. To infer distance to a target, each underlying pulse envelope must be consistently registered and subtracted despite environmentally-induced variability. Then, nonlinear transformation of the phase is applied to remove the chirp, an FFT is performed to determine the peak frequency of the de-chirped signal, and a calibration factor relating de-chirped frequency to distance results in target position. This article discusses these analysis steps are in detail.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

SU-E-T-526: On the Linearity, Stability and Beam Energy Dependence of CdSe Quantum Dots as Scintillating Probes

Purpose: Structure and energy transfer mechanisms confer colloidal quantum dots (cQDs) interesting properties, among them their potential as scintillators. CdSe multi-shell cQDs in powder were investigated under photons irradiation. The purpose of this work is to characterize signal to dose linearity, stability with time and to quantify the dependence of their light output with beam energy. Methods: The cQDs are placed at the extremity of a non-scintillating plastic collecting fiber, with the other extremity connected to an Apogee U2000C CCD camera. The CCD camera collects the fluorescence light from irradiated cQDs from which the delivered dose is extracted. This signal is corrected for Cerenkov contamination at MV energies using the chromatic technique. The detector was irradiated with two devices: Xstrahl 200 orthovoltage unit for 120, 180 and 220 kVp and a Varian Clinac iX for 6 and 23 MV. Results: Linear output response with varying dose is observed for all beam energies with R2 factors > 0,999. Reproducibility measurements were performed at 120 kVp: the same set-up was irradiated at different time intervals (one week and three months). The results showed only a small relative decrease of light output of 3,2 % after a combine deposited dose of approximately 95 Gy. CdSe nanocrystals response has been studied as a function of beam energy. The output increases with decreasing energy from 120 kVp to 6 MV and increase again for 23 MV. This behavior could be explained in part by the cQDs high-Z composition. Conclusion: The fluorescence light output of CdSe cQDs was found to be linear as a function of dose. The results suggest stability of the scintillation output of cQDs over time. The specific composition of cQDs is the main cause of the observed energy dependence. We will further look into particle beam dependence of the cQDs. Bourse d'excellence aux etudes graduees du CRC (Centre de Recherche sur le Cancer, Universite Laval) Bourse d'excellence aux etudes graduees du CRC (Centre de Recherche sur le Cancer, Universite Laval)

60 APPLIED LIFE SCIENCES↗

SU-E-T-44: A Micro-Raman Spectroscopy Study of the Dose-Dependence of EBT3 GafChromicTM Films for Quantifying the Degree of Molecular Polymerization

Purpose: Radiochromic films, such as the poly-diacetylene-based EBT3 GafChromic{sup TM} films (Ashland Specialty Ingredients, Wayne, NY, USA), are widely used for dosimetry applications because of their clear energy independence, high spatial resolution, near tissue equivalence and easy handling. The films undergo a slight color change by radiation-induced polymerization of diacetylene monomers. But more importantly, the film becomes optically less transparent with increasing radiation dose, with a saturation starting between 10 and 20 Gy, i.e. a common SBRT dose level. In contrast to the chromatic properties, less attention has been given to the underlying molecular mechanism that induces this partial color change and strongly reduces the transparency. Therefore, the current work investigates the variation of the molecular composition of the active layer of EBT3 films for an SBRT dose range. Method: Uncoated EBT3 films were irradiated with a 6 MV photon beam using dose levels between 0 and 20 Gy. The relative variation of the polymer content as a function of the applied radiation dose was studied using micro-Raman spectroscopy. Raman spectroscopy with a 633 nm probe laser incident on the active layer allowed to identify the film constituents and to estimate the amount of poly-diacetylenes from the intensities of the unique molecular vibrations of the molecule. Results: The normalized intensity of all polymeric vibrations, and most notably the polymeric triple and double carbon-carbon bonds at 2058 cm{sup −1} and 1446 cm{sup −1} respectively, increase with increasing dose up to a saturation level starting at about 10 Gy, indicating a corresponding increase and saturation of the amount of polymers. This molecular saturation process is the main cause of the non-linear dose response (i.e. a transparency reduction) and of the limited dose range of the studied films. Conclusion: Raman spectroscopy provides new and more fundamental insights in the mechanism of the dose-dependence of EBT3 films. This work was funded by the Research Foundation - Flanders (FWO)

60 APPLIED LIFE SCIENCES↗

Draft Genome Sequences for Two Metal-Reducing Pelosinus fermentans Strains Isolated from a Cr(VI) Contaminated Site and for Type Strain R7

Pelosinus fermentans 16S rRNA gene sequences have been reported from diverse geographical sites since the recent isolation of the type strain. We present the genome sequence of the P. fermentans type strain R7 (DSM 17108) and genome sequences for two new strains with different abilities to reduce iron, chromate, and uranium.

59 BASIC BIOLOGICAL SCIENCES↗

RcaE-Dependent Regulation of Carboxysome Structural Proteins Has a Central Role in Environmental Determination of Carboxysome Morphology and Abundance in Fremyella diplosiphon

Carboxysomes are proteinaceous subcellular compartments, or bacterial organelles, found in cyanobacteria that consist of a protein shell surrounding a core primarily composed of the enzyme ribulose-1,5-biphosphate carboxylase/oxygenase (RuBisCO) that is central to the carbon dioxide-concentrating mechanism (CCM) and carbon fixation. Whereas significant insights have been gained regarding the structure and synthesis of carboxysomes, limited attention has been given to how their size, abundance, and protein composition are regulated to ensure optimal carbon fixation in dynamic environments. Given the centrality of carboxysomes in photosynthesis, we provide an analysis of the role of a photoreceptor, RcaE, which functions in matching photosynthetic pigmentation to the external environment during complementary chromatic acclimation and thereby optimizing photosynthetic efficiency, in regulating carboxysome dynamics. Our data highlight a role for RcaE in perceiving external light cues and regulating carboxysome structure and function and, thus, in the cellular capacity for carbon fixation and organismal fitness.

59 BASIC BIOLOGICAL SCIENCES↗

IR challenges and the machine detector interface at FCC-ee

The FCC-ee, with its unprecedented luminosity goal and high energy reach, creates challenges and requires solutions to many issues in order to produce a realistic design for the complex machine detector interface. The interaction region design for the FCC-ee adopts the crab-waist collision scheme and proposes an elegant local chromaticity correction system. An asymmetric layout of nearby dipoles suppresses the critical energy of synchrotron radiation incoming to the detector at the interaction point to a maximum value of 100 keV. The main challenge of the FCC-ee machine detector interface design is to combine the many conflicting accelerator and 2 T detector constraints, aiming for the optimal trade-off choices that simultaneously allow for a best machine performance in terms of integrated luminosity and data taking efficiency. Much of the success of the FCC-ee will be related to the interaction region design, as a result of the ingredients coming from areas of accelerator physics, mechanical engineering and detector optimization.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

A conceptual design of circular Higgs factory

Similar to a super B-factory, a circular Higgs factory (CHF) will require strong focusing systems near the interaction points and a low-emittance lattice in the arcs to achieve a factory luminosity. At electron beam energy of 125 GeV, beamstrahlung effects during the collision pose an additional challenge to the collider design. In particular, a large momentum acceptance at the 2% level is necessary to retain an adequate beam lifetime. This turns out to be the most challenging aspect in the design of a CHF. In this paper, an example will be provided to illustrate the beam dynamics in a CHF, emphasizing the chromatic optics. Basic optical modules and advanced analysis will be presented. Most importantly, we will show that 2% momentum aperture is achievable.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Chromium-Free Coating for Al Alloy Corrosion Protection Based on a Novel Ti/Mg Oxyfluoride

Chromium-free corrosion protection of aluminum alloys comparable to that of chromates (Cr(VI)) is demonstrated using a TiF 6 2– fluoro-anion-based coating recipe containing boric acid and a Mg salt. Boric acid drove TiF 6 2– hydrolysis enabling up to micrometer-scale thick coatings. The Mg salt led to deposition of a novel crystalline phase Ti/Mg oxyfluoride coating with an approximate composition of Ti 5 MgO 7 F 8 . Corrosion protection performance was characterized by polarization resistance measurements during immersion in 5% aqueous NaCl solution and neutral salt fog exposure following ASTM B.117. The performance is discussed in terms of the presence of fluoride in the coating enabling active behavior during its gradual depletion (in corrosion environments) toward a final composition approaching TiO 2 . This active corrosion protection mechanism may be more generally applicable for transition metal-based coatings that do not have high oxidation state oxo-anions, but do have stable fluoro-anions.

36 MATERIALS SCIENCE↗

era-opt

An algorithm to reduce the enumeration of possible metamers to be examined from multi-primary LED systems when searching (optimizing) for combinations with particular chromaticity characteristics.

Baxter, DouglasJ↗

Human perceptions of colour rendition vary with average fidelity, average gamut, and gamut shape

An experiment was conducted to evaluate how subjective impressions of color quality vary with changes in average fidelity, average gamut, and gamut shape (which considers the specific hues that are saturated or desaturated). Twenty-eight participants each evaluated 26 lighting conditions—created using four, seven-channel, tunable LED luminaires—in a 3.1 m by 3.7 m room filled with objects selected to cover a range of hue, saturation, and lightness. IES TM-30 fidelity index (Rf) values ranged from 64 to 93, IES TM-30 gamut index (Rg¬) values from 79 to 117, and IES TM-30 Rcs,h1 values (a proxy for gamut shape) from -19% to 26%. All lighting conditions delivered the same nominal illuminance and chromaticity. Participants were asked to rate each condition on eight point semantic differential scales for saturated-dull, normal-shifted, and like-dislike. They were also asked one multiple choice question, classifying the condition as saturated, dull, normal, or shifted. The findings suggest that gamut shape is more important than average gamut for human preference, where reds play a more important role than other hues. Additionally, average fidelity alone is a poor predictor of human perceptions, although Rf was somewhat better than CIE Ra. The most preferred source had a CIE Ra value of 68, and 9 of the top 12 rated products had a CIE Ra value of 73 or less, which indicates that the commonly used criteria of CIE Ra ≥ 80 may be excluding a majority of preferred light sources.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Data for Physiological Controls on Carbon Fluxes and Biomass Production in Miscanthus: Insights From a Process- Based Agroecosystem Model

Biomass crops serve as essential feedstocks for renewable energy and bioproducts and play a critical role in achieving lower emissions in the transportation sector. However, dedicated perennial biomass crops such as Miscanthus × giganteus (Miscanthus) remain underrepresented in process- based agroecosystem models, limiting robust evaluation of their economic and environmental performance. In this study, we developed a data- constrained representation of the sterile triploid Miscanthus (IL clone) within the process- based model ecosys, integrating global sensitivity analysis, ensemble simulation, and parameter calibration. Planting, harvesting, and fertilization practices consistent with field management were incorporated, and phenology was constrained using PhenoCam- derived Green Chromatic Coordinate (GCC) data. Using the Morris global sensitivity analysis method, we identified 11 key physiological parameters governing plant carbon, water, and nutrient relations, particularly processes associated with CO2 assimilation. We then conducted ensemble simulations by perturbing these parameters and calibrated the model against eddy covariance fluxes and field- measured biomass. Building on the calibrated operating state, parameter- response analyses show that different photosynthetic processes influence productivity in different ways. Protein allocation determines whether productivity increases toward a higher level, whereas electron transport capacity controls additional gains once protein allocation approaches saturation. These findings demonstrate that parameter importance depends on physiological context and on which photosynthetic processes remain limiting. Calibration and validation against observations show that ecosys can reliably reproduce carbon and water fluxes, as well as both above- and belowground biomass, with post- calibration GPP R2 improving from 0.67 to 0.95 during the calibration period and remaining high during validation (R2 = 0.95). These results provide a mechanistic foundation for regional simulations and sustainable bioenergy assessments.

Carbon↗

Scattering of an utlrashort laser pulse by a spherical air bubble

The scattering of an ultrashort laser pulse by an air bubble in water is investigated by means of the Lorenz-Mie theory and the Debye expansion. A 70 fs, 800 nm pulse is considered as a plane wave with a Gaussian temporal envelope. The transient response is treated with the theory derived from Gouesbet and Gréhan [ Part. Part. Syst. Charact. 17 , 213 –224 ( 2000 ) ], taking now into account chromatic dispersion and absorption of water. It is observed that contrary to the case of water droplet in air, the Debye modes p ≥ 1 start their transient scattering at the same time and the same angle (≈90 ° ) and for a large size parameter, they differentiate as time elapses. A parametric study on the size parameter and the spatial extension of the pulse is performed to identify regimes where the different Debye mode are distinguishable in time. Dependence on the scattering angle is also treated. Finally, by considering pulse chirp, it is shown that the laser/bubble distance has an influence on the separability of modes p = 0 and p = 1.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Kerr-lens mode-locked Cr:ZnS oscillator reaches the spectral span of an optical octave

We report, to the best of our knowledge, the first super-octave femtosecond polycrystalline Cr:ZnS laser at the central wavelength 2.4 µm. The laser is based on a non-polarizing astigmatic X-folded resonator with normal incidence mounting of the gain element. The chromatic dispersion of the resonator is controlled with a set of dispersive mirrors within one third of an optical octave over 2.05–2.6 µm range. The resonator’s optics is highly reflective in the range 1.8–2.9 µm. The components of the oscillator’s output spectrum at the wavelengths 1.6 µm and 3.2 µm are detected at –60 dB with respect to the main peak. Average power of few-cycle Kerr-lens mode-locked laser is 1.4 W at the pulse repetition frequency 79 MHz. That corresponds to 22% conversion of cw radiation of Er-doped fiber laser, which we used for optical pumping of the Cr:ZnS oscillator.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Ultrabroadband flying-focus using an axiparabola-echelon pair

Flying-focus pulses promise to revolutionize laser-driven secondary sources by decoupling the trajectory of the peak intensity from the native group velocity of the medium over distances much longer than a Rayleigh range. Previous demonstrations of the flying focus have either produced an uncontrolled trajectory or a trajectory that is engineered using chromatic methods that limit the duration of the peak intensity to picosecond scales. Here we demonstrate a controllable ultrabroadband flying focus using a nearly achromatic axiparabola-echelon pair. Spectral interferometry using an ultrabroadband superluminescent diode was used to measure designed super- and subluminal flying-focus trajectories and the effective temporal pulse duration as inferred from the measured spectral phase. The measurements demonstrate that a nearly transform- and diffraction-limited moving focus can be created over a centimeter-scale—an extended focal region more than 50 Rayleigh ranges in length. This ultrabroadband flying-focus and the novel axiparabola-echelon configuration used to produce it are ideally suited for applications and scalable to >100 TW peak powers.

47 OTHER INSTRUMENTATION↗

Referenceless, grating-based, single shot X-ray phase contrast imaging with optimized laser-driven K-α sources

With its ability to efficiently probe low-Z materials, X-ray phase imaging methods have recently raised high interest in multiple fields from biology and medical applications to high energy density (HED) physics. Initially developed with synchrotron light and X-ray tubes, we present a novel grating based Talbot X-ray deflectometer (TXD) diagnostic that was coupled with laser-generated K-α X-ray sources. The multi-terawatt laser (I > 1 × 10 14 W cm -2 ) was used as a testbed for diagnostic development. It was found that X-ray source chromaticity plays an important role in TXD. Indeed, the broadband spectrum of laser-generated X-ray sources may strongly impact image quality and thus diagnostic performance. We qualified X-ray emission from different laser-produced sources and determined laser, target, and deflectometer parameters that optimize TXD performance. We present the first results of referenceless grating-based X-ray imaging at high-power laser facilities and discuss the implications of this new development in HED research.

47 OTHER INSTRUMENTATION↗

Disordered spontaneously buckled optical gratings for improved lighting applications

Technologies for directing daylight deeper within a building space are highly sought after for energy efficiency applications in order to offset artificial lighting costs and to improve workplace productivity via the use of natural light. Vertical window coatings that can perform this task by redistributing sunlight deeper into a space are especially attractive as they are significantly more straightforward to incorporate into a wide variety of architectures as well as to retrofit into existing facades as compared to roof-based skylights or bulky horizontal daylight shelf type options. The potential energy savings are even greater when one takes into account the fact that such technologies would mitigate harsh glare, allowing window shades to be open for longer portions of the day. However, low-cost and readily scalable techniques are essential for widespread adoption of these window coating technologies. Here, we describe a potentially low-cost method to create a window coating that could enhance daylight penetration, requiring only a thin film of polymeric material deposited on an elastomeric substrate. The resulting structure is a disordered, spontaneously buckled optical grating that spreads incident light without noticeable chromatic dispersion due to its stochastic patterning. The described method has the potential to improve energy efficiency and while maintaining acceptable optical clarity.

De Vetter, Brent M.↗

Investigation of Tail-dominated Instability in the Fermilab Recycler Ring

In our recent operational run, a single bunch, tail-dominated instability was observed in the Fermilab Recycler ring. This instability exclusively occurs in the vertical plane when the chromaticity is close to zero. In this study, we conduct a detailed analysis of this instability under different operational parameters. We investigate the impact of space charge on the head-tail motion and propose potential interpretations of the underlying mechanism of the instability. Moreover, we explore methods to mitigate this instability in the future.

43 PARTICLE ACCELERATORS↗