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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Results of the Collaborative International Evaluated Library Organization (CIELO) Project

Simulation of nuclear systems requires complete data that represents the relevant nuclear physics. This requires many types of experimental measurements, theoretical physics, semi-empirical models and software systems, as well as experts to integrate and guide the process. This discipline is collectively known as nuclear data, and separate programmes within various European countries, the USA, Japan, Russia, and other OECD Nuclear Energy Agency (NEA) member countries have been operating for many decades. The NEA Working Party on International Nuclear Data Evaluation Co-operation (WPEC) exists to improve the quality and completeness of nuclear data by bringing together representatives of the major nuclear data evaluation projects of NEA member countries and selected Invitees. The Sub- and Expert Groups of the WPEC typically focus on specific technical topics, while the Collaborative International Evaluated Library Organisation Pilot Project (CIELO) was established to generate complete evaluations for a selection of the most important isotopes for criticality in nuclear technologies: 235,238 U, 239 Pu, 56 Fe, 16 O and 1 H.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Collaborative Research: Understanding Sheaths and Presheaths in Magnetized and Unmagnetized Plasmas

The common states of matter on Earth are solids, liquids and gases. Putting energy into gases can result in the 4th state of matter known as plasma, which consists of electrically charged particles (electrons and ions, both positive and negative) and neutral atoms and molecules. While uncommon on the Earth, plasma makes up more than 99% of the visible matter in the universe. Where plasma comes in contact with material boundaries, a thin region near the plasma boundary usually forms to isolate the plasma from the boundary. This thin region is called the plasma sheath. Experiments performed under aimed at improving our understanding of plasma sheaths and associated phenomena as fundamental to understanding all bounded plasmas. Plasma studied in this work are similar to those used in plasma applications such as the etching of semiconducting materials to make computer chips, in plasma space propulsion satellite engines, and used in experimental plasma fusion devices. The majority of experimental studies were carried out at the University of Wisconsin-Madison in close collaboration with Dr. Severn at the University of San Diego (USD), where most of diagnostic development for laser-induced fluorescence (LIF) measurements were carried out. USD is primarily an undergraduate institution. The award made possible outreach activities that promoted engagement of undergraduate students with diverse backgrounds in science, technology, engineering and mathematics (STEM) disciplines.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Collaborative Research: Improved Efficiency and Coupling of the Radiation Code in the ACME Earth System Model (Final Report)

The complexity of radiative transfer, its importance to the exchange of energy in the climate system, and its high computational cost establishes importance of an accurate and efficient radiative transfer parameterization for climate simulation. Previous work by the proposing team at AER led to the development of the radiation code, RRTMG, which has been widely accepted by the global modeling community as a fast and accurate advancement over the previous generation of radiation codes. It has been in use in the NCAR CESM for many years, and it has been implemented in the initial version the DOE E3SM model. However, its computational cost remains high relative to other components in part due to its complexity and to its inefficient use of modern optimization strategies, and this project helped address this limitation for the code’s application in E3SM. Under other funding, the Investigators of this project led an effort to develop a high-performance broadband radiation code, called RTE+RRTMGP, which is a completely restructured code that will take advantage of modern computational capabilities to enhance its performance while retaining the strengths and accuracy of the original code. Designed to perform over a range of computer architectures, RTE+RRTMGP makes extensive use of Fortran 2003 features to improve both its efficiency and its use of memory. RTE+RRTMGP is expected to be adopted in the next generation of RTE+RRTMGP. This project allowed for advancements to the code’s computational capabilities and adding new and enhanced features. This included revising RTE+RRTMGP to run on GPU processors, analysis of and improvements to the code’s timing, modifying the gas optics in RRTMGP to increase the code’s accuracy, extensive validation of computed fluxes, heating rates and forcings, generating a cloud optical property and vertical sampling capabilities for RTE+RRTMGP, implementing a fast and accurate longwave scattering capability, and groundwork for the inclusion of a capability to specify solar variability. Many of the accomplishment in this project necessitated significant collaboration with the E3SM development team. The result of this project was optimization of a key physical component (radiative transfer calculations) of E3SM, directly supporting E3SM’s overarching global modeling objectives. More broadly, this project provided overall advancements in the use of radiative transfer calculations in atmospheric modeling and simulation, particularly for climate.

58 GEOSCIENCES↗
DOE OSTI2019

Sodium Fire Collaborative Study Progress (CNWG FY 2019)

This report discusses the progress on the collaboration between Sandia National Laboratories (Sandia) and Japan Atomic Energy Agency (JAEA) on the sodium fire research in fiscal year 2019. First, the current sodium pool fire model in MELCOR, which is adapted from CONTAIN-LMR code, is discussed. The associated sodium fire input requirements are also presented. A proposed model improvement developed at Sandia is discussed. Finally, the validation study of the sodium pool fire model in MELCOR carried out by a JAEA's staff is described. To validate this model, a JAEA sodium pool fire experiment (F7-1 test) is used. A preliminary calculation is performed using a modified MELCOR model from a previous experiment simulation. The results of the calculation are discussed as well as suggestions for improvement. Finally, recommendations are made for new MELCOR simulations for next fiscal year, 2020.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

CEA/DAM - CEA/DEN - LANL - IAEA - IPHC Collaboration Meeting on Nuclear Data, Nuclear Reaction Theories, and Machine Learning (Summary Report)

Dupuis hosted our biennial CEA/NNSA collaboration meeting, and Kawano and Lovell of LANL and Tamagno of CEA/DEN (Cadarache) visited CEA/DAM to discuss current issues and further developments in nuclear reaction modeling, nuclear data evaluation, and relevant programs of modern computer science, especially the machine learning technology. The discussions included topics of our common interest such as neutron inelastic scattering, capture, and fission, with particular emphasis on the actinide nuclear data evaluations. We report briefly the summary of our discussions. We also had a half-day video meeting with Capote of IAEA and Kerveno of IPHC to discuss nuclear reactions on actinides.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Fracture Toughness Properties of Tritium Charged and Aged Stainless Steels: SRNL and SNL Collaboration Test Plan and 2018 Results

Forged stainless steels are used as the materials of construction for tritium reservoirs. During service, tritium diffuses into the reservoir walls and radioactively decays to helium-3. Tritium and decay helium cause a higher propensity for cracking which could lead to a tritium leak or failure of a tritium reservoir. Fracture toughness properties are needed for designing tritium reservoirs and evaluating the long-term effects of tritium on their structural properties. A key result of prior studies is that the long-term cracking resistance of stainless steels in tritium service depends greatly on the interaction between decay helium and the steels’ forged microstructure. Designers and modelers at Sandia National Laboratories (SNL) have identified key gaps in the data available on material performance in tritium. Thus, a collaborative plan and schedule of tests have been developed with SRNL and SNL to fill these gaps using a range of tensile test and fracture mechanics test geometries, at stockpile relevant temperatures. These studies target the fundamental deformation mechanisms and the influence of tritium-decay-helium on their behavior. This report outlines the goals of each program and describes the sample test matrices and experimental conditions. This report fulfills the requirements for a portion of the Enhanced Surveillance Campaign (ESC) FY19 Level 2 milestone 6725 to deliver an annual report on the aging studies of reservoir materials.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Engineered Barrier System R&D and International Collaborations – LANL (FY20): Spent Fuel and Waste Disposition

The United States Department of Energy’s Spent Fuel and Waste Disposition (SFWD) program is investigating the design and safety function of generic nuclear geologic repositories in a variety of geologic settings (salt, argillite, and crystalline rock). Different configurations and loadings of spent nuclear fuel and waste within disposal canisters are also being investigated, some of which have the potential to generate repository temperatures higher than previously considered (i.e., temperatures >100ºC) by foreign and domestic concepts. This report expands on engineered barrier material stability in a high temperature crystalline rock repository through high temperature hydrothermal experiments. Experiments were designed to develop engineered barrier system (EBS) concepts in a hightemperature crystalline environment in 1) bentonite-Grimsel Granodiorite interactions, 2) bentonite-cement reactions, and 3) interaction between waste canister materials and bentonite. Experiment results are applied to understanding long-term repository performance in terms of radionuclide isolation. One hydrothermal experiment was completed in the rocking autoclaves at LANL in FY-20: IEBS-6 (Grimsel Granodiorite + Wyoming bentonite + cured ordinary Portland cement + Grimsel Granodiorite synthetic groundwater, 250ºC/150 bar, 8 weeks). Several other experiments were planned but were delayed due to the COVID-19 pause in laboratory work. In addition, some characterization of the reaction products of experiments conducted in FY-20 was prevented by COVID-19. Mineral phase chemistry was not measured via electron microprobe analyses for IEBS-6. Quantitative X-ray diffraction results from IEBS-6 and HBT-1 were not completed. The missing analyses and discussion of the results will be included in next year’s report. New characterization that was completed includes scanning electron microscopy of reaction products from IEBS-6, quantitative X-ray diffraction results are presented from IEBS-1 through IBES-5, preliminary scanning electron microscope images and chemical analyses for IEBS-6, X-ray diffraction of the clay fraction from all experiments, measurement/imaging of mineral growth on the surface of steel coupons. Major observations pertaining to bentonite stability in a Grimsel Granodiorite environment include the stability of Na-montmorillonite at 250°C, the formation of trace CSH phases, and the formation of bentonite colloids on experiment cooling. The addition of a cured chip of Portland cement to the bentonite-Grimsel system results in slightly higher pH values and the formation of diverse secondary mineral phases that were not observed in the previous experiments (e.g., analcime, garronite, CSH phases). The new characterization efforts related to the interaction of stainless-steel coupons and bentonite clay focused on thickness and mineralogy of phases that formed at the steel surface. In Wyoming bentonite + Grimsel Granodiorite systems, newly formed minerals at the bentonitesteel coupon interface included alteration of the outermost steel edge to Fe,Cr-oxide phases, followed by Fe-rich phyllosilicates (Fe-saponite, chlorite) and interbedded Fe,Cr,Ni-sulfide phases (pentlandite). Hydrothermal experiments were completed to assess uranium-carbonate complexation at conditions relevant to high-temperature disposal. Autoclave solubility experiments were conducted at 150 to 250ºC with a range of carbonate and uranium concentrations. The experiment results were characterized via situ UV-Visible spectroscopy and synchrotron-based in situ XAS techniques. Results show a significant decrease in the stability of uranyl-carbonate complexes at temperatures above 100ºC along with the precipitation of uranium oxides. Further, at T > 200ºC, results show that uranyl-hydroxyl complexes control solubility of uranium instead of the previously predicted uranyl-carbonate species. These results are significant for understanding the mobility of uranium in the EBS, which will likely contain carbonate-rich fluids. International research efforts focused on three main areas: 1) participation in international conferences, 2) building collaborations with foreign repository programs, and 3) the initiation of an experimental program to complement the full-scale HotBENT test at the Grimsel test site. This experiment included Wyoming bentonite + low carbon steel + Grimsel Granodiorite synthetic groundwater and was run at the planned maximum temperature of the HotBENT test (200°C). Complete characterization of reaction products was hindered by disruptions to laboratory work but will be reported in the next FY. The experimental results obtained in FY-20 continue to document the wide-ranging effects of bulk composition and pressure-temperature conditions in the mineralogical and geochemical evolution of a high-temperature repository environment. Concepts developed will be used to inform models of long-term material stability in a generic crystalline rock-hosted repository.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2020

Collaboration with USACyS for Signals Manipulation

Savannah River National Laboratory has been investing into cybersecurity capabilities since 2019. Cybersecurity has been a rapidly growing area for the CSRA in general and has included the consolidation of Cyber and Electronic Warfare units at Fort Gordon. This consolidation has been driven by the convergence of cyberwarfare and electronic warfare as the technologies underpinning Army Cyber Command’s vision of Information Warfare. This convergence, investment by SRNL into cybersecurity for critical infrastructure, and the desire for collaboration between the Army and SRNL has resulted in an opportunity for SRNL to develop R&D capabilities in electronic warfare that will complement SRNL’s cybersecurity efforts. Discussions between SRNL and the U.S. Army Cyber School (USACyS) has identified a general gap in ICS training lab capability in which both entities could contribute to solve. It is proposed to design and architecture that meets this need.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2020

Collaborative Research: Polymer Macrocycles: A novel topology to control dynamics of rubbery materials

Understanding the dynamics of polymers of different topologies is an important field of study and one of the most important unanswered questions in this field is "how do circular polymers move," particularly in the melt state. New information suggests that molecular topology, specifically circular rings, impacts the response of materials in nanometer- scale confinement. The work performed here tackles these subjects through a collaboration in which specialists in polymer synthesis, polymer rheology and scattering methods, and in the physics of nanoconfinement work together to investigate the thermophysical behavior of circular macromolecules. The project goals are to use a novel synthesis method of "green" oxidative polymerization to produce high purity macrocycles and to investigate their linear viscoelastic behavior in order to fully characterize the dynamics of circular macromolecules to sizes that correspond to linear molecule entanglement densities higher than previously obtainable with synthetic polymers. Chemical chain end characterization and critical edge fractionation coupled with direct visualization of the prepared polymers through the use of polymer amplification methods are proposed in order to quantify the numbers of circular and linear molecules in each sample. The study of the linear viscoelastic response of blends of linear and circular molecules is also to be undertaken in the project. Nonlinear viscoelastic measurements, including extensional viscosity, are to be made. Strong differences in behavior between linear chains and circular ones also provides an important opportunity for new technology to break the "magic triangle" for tires: it is believed that improving one of the three key attributes - traction, wear, rolling resistance - necessarily sacrifices at least one of the others. Rubber made from cyclic polymers has the potential to break out of this triangle by reducing the so-called Payne effect in reinforced rubbers because circular macromolecules are less sensitive to nanoconfinement than their linear counterparts. The work has as one objective to characterize the impact of nanoconfinement on the behavior of large circular macromolecules. In addition, the dynamics of carbon black filled circular macromolecules are to be studied to test the hypothesis that the resulting rubbery materials will exhibit a reduced Payne effect.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2020

Collaborative Research: Improved Efficiency and Coupling of the Radiation Code in the ACME Earth System Model. Final Report

This final report details all work performed on the project by both project partners. This project provided support to properly couple RTE+RRTMGP, a high-performance broadband radiation code, within DOE’s Energy Exascale Earth System Model (E3SM). RTE+RRTMGP is a successor to the RRTMG radiation code, which has been widely accepted for its speed and accuracy by the global modeling community, and has been in use in the NCAR CESM for many years and was implemented in the initial version of E3SM. However, the computational cost of RRTMG remains high relative to other components in part due to its complexity and to its inefficient use of modern optimization strategies, issues that were rectified by the development of RTE+RRTMGP. Many of the accomplishment in this project necessitated significant collaboration with the E3SM development team. One focus of the project was to enhance the code’s optimization on the limited number of emerging computing systems on which the model is expected be used, including Many Integrated Core (MIC) architectures and Graphics Processing Unit (GPU) hardware. We also developed additional capabilities for RTE+RRTMGP that E3SM scientists identified as important for the planned applications of the model. The result of our project was optimization of a key physical component (radiative transfer calculations) of E3SM, directly supporting E3SM’s overarching global modeling objectives. More broadly, this project provided overall advancements in the use of radiative transfer calculations in atmospheric modeling and simulation, particularly for climate.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Collaborative Research: Understanding Nanoparticle-Plasma Interactions in Dusty Non-Thermal Plasmas by Nanoparticle Probes and Online Aerosol Characterization (Final Technical Report)

This report describes results from the University of Minnesota’s contribution to studies performed under the award DE-SC0018202 (principal Investigator: Christopher J. Hogan Jr.. This award is a collaborative research grant with support equally provided to Case Western Reserve University and to the University of Illinois (with principal investigator R. Mohan Sankaran). To date ten peer-reviewed published papers have resulted from the studies performed with University of Minnesota personnel contributing; this report describes the results of these studies as well as several unpublished studies, grouped into seven separate study types. The overarching goal of the carried out studies was to understand nanoparticle behavior and dynamics in non-thermal plasma synthesis reactors, specifically adapting aerosol measurement technology to provide online measurements of particle size, charge, and structure in plasma reactor systems.

42 ENGINEERING↗
DOE OSTI2021

Sodium Fire Collaborative Study Progress -- CNWG Fiscal Year 2020

This report discusses the progress on the collaboration between Sandia National Laboratories (Sandia) and Japan Atomic Energy Agency (JAEA) on the sodium fire research in fiscal year 2020. First, the current sodium pool fire model in MELCOR, which is adapted from CONTAIN-LMR code, is discussed. The associated sodium fire input requirements are also presented. These input requirements are flexible enough to permit further model development via control functions to enhance the current model without modifying the source code. The theoretical pool fire model improvement developed at Sandia is discussed. A control function model has been developed from this improvement. Then, the validation study of the sodium pool fire model in MELCOR carried out by both Sandia and JAEA’s staff is described. To validate this pool fire model with the enhancement, a JAEA sodium pool fire experiment (F7-1 test) is used. The results of the calculation are discussed as well as suggestions for further model improvement. Finally, recommendations are made for new MELCOR simulations for next fiscal year, 2021.

36 MATERIALS SCIENCE↗
DOE OSTI2018

International Collaboration Activities on Engineered Barrier Systems

International collaborations on nuclear waste disposal is an integral part of the Spent Fuel Waste Science and Technology (SFWST) campaign within the DOE Fuel Cycle and Technology (FCT) program. These engagements with international repository R&D programs provide key opportunities to participate in experiments with international partners on research investigations developing laboratory/field (underground research laboratories (URL) experiments) data of engineered barrier system (EBS) components (e.g., near-field) and characterization of transport phenomena in the host rock (e.g., far-field). The results of these field and laboratory experiments are used in the evaluation of coupled processes and the development of state-of-the-art simulation approaches to evaluate repository performance. Thermal heating from radionuclide decay in the waste canisters will increase temperature in the surrounding EBS driving chemical and transport processes in the near- and far-field domains of the repository. URL heater-tests for extended periods of times (e.g., years) provide key information and data of thermal effects on barrier responses to temperature and water saturation levels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2018

Progress of EBS International Collaborations (FY2018)

The SNL Engineered Barrier System (EBS) International activities were focused on two main collaborative efforts for FY18: 1) Benchmarking semi-analytical codes used for thermal analysis, and 2) Benchmarking of reactive transport codes (including PFLOTRAN) used for chemical evolution of cementitious EBS components. The former topic, was completed over the course of FY18, while the latter has just begun in the latter half of FY18 under the aegis of additional appropriations and scoped as "Additional FY18 Activities". This report contains a complete summary of Item #1, as well as a status update on the progress of Item #2.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2017

International Collaboration Activities on Engineered Barrier Systems

The Spent Fuel Waste Science and Technology (SFWST) campaign from the DOE Fuel Cycle and Technology (FCT) program has been engaging in international collaborations between repository R&D programs for nuclear waste disposal to leverage on the extensive research investigations and laboratory/field data of engineered barrier system (EBS) components (e.g., near-field) and characterization of transport phenomena in the host rock (e.g., far-field) processes from state-of-the-art underground research laboratories (URL) experiments. Thermal heating from radionuclide decay in the waste canisters will generate increases in temperature that will drive chemical and transport processes in the near- and far-field domains of the repository. URL sites provide the ideal setting to conduct heater test experiments to simulate the thermal effects of heat-generating nuclear waste in disposal galleries and surrounding host rock.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2021

International Collaborations Activities on Disposal in Argillite R&D: Characterization Studies and Modeling Investigations

This interim report is an update of ongoing experimental and modeling work on bentonite material described in Jové Colón et al. (2019, 2020) from past international collaboration activities. As noted in Jové Colón et al. (2020), work on international repository science activities such as FEBEX-DP and DECOVALEX19 is either no longer continuing by the international partners. Nevertheless, research activities on the collected sample materials and field data are still ongoing. Descriptions of these underground research laboratory (URL) R&D activities are described elsewhere (Birkholzer et al. 2019; Jové Colón et al. 2020) but will be explained here when needed. The current reports recent reactive-transport modeling on the leaching of sedimentary rock.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2020

A Proposed Common Model of Multi-phase Strength and Equation of State for a Tri-laboratory Collaboration (Working Draft 1.1)

The proposed simple common model for multiphase strength and EoS (CMMP) is meant to be sufficiently simple that each of the collaborating labs can share in a common starting point. Another objective is to start with relatively simple assumptions, which will not necessarily capture details of the physical processes, and incrementally add complexity in order to identify the minimal-needed technical detail. Through this co-evolution of model and experiment, we will better learn the importance of various theoretical approximations and where to invest future resources in experiment and model development. This simple framework is based on pressure and temperature equilibrium of all co-existing phases combined with deviatoric stress averaging through a volume fraction weighted ow stress and a volume fraction weighted shear modulus. Implementations of the framework based on equilibrium phase fractions (i.e. instantaneous kinetic rate) and for finite rate transition kinetics are proposed.

36 MATERIALS SCIENCE↗