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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Why Seeding Works When Nucleation Barriers Vanish

This paper explains why seeds can speed up crystallization even when the formation of new crystal nuclei is not the slow step. In zeolite synthesis, local crystalline order can form relatively early, but the material may still appear poorly crystalline by X-ray diffraction because many small crystallites are misoriented and lack long-range coherence. Using coarse-grained molecular simulations, the study showed that seeds help solve this coherence problem. Rather than primarily lowering a nucleation barrier, seeds impose a common orientation on nearby growing crystallites, allowing them to merge into larger, better aligned domains. This accelerates the development of X-ray-detectable crystallinity even if the total amount of locally ordered material has not changed much. The work changes how induction times in zeolite synthesis should be interpreted: the delay before X-ray crystallinity appears can reflect the time needed to build long-range structural coherence, not simply the time needed to form crystalline material. This provides a new explanation for why seeding is effective in growth-limited crystallization and offers design principles for controlling crystallization rate and crystal quality.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Integrated quantum optical phase sensor in thin film lithium niobate

Abstract The quantum noise of light, attributed to the random arrival time of photons from a coherent light source, fundamentally limits optical phase sensors. An engineered source of squeezed states suppresses this noise and allows phase detection sensitivity beyond the quantum noise limit (QNL). We need ways to use quantum light within deployable quantum sensors. Here we present a photonic integrated circuit in thin-film lithium niobate that meets these requirements. We use the second-order nonlinearity to produce a squeezed state at the same frequency as the pump light and realize circuit control and sensing with electro-optics. Using 26.2 milliwatts of optical power, we measure (2.7 ± 0.2)% squeezing and apply it to increase the signal-to-noise ratio of phase measurement. We anticipate that photonic systems like this, which operate with low power and integrate all of the needed functionality on a single die, will open new opportunities for quantum optical sensing.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Lightwave-electronic harmonic frequency mixing

Electronic frequency mixers are fundamental building blocks of electronic systems. Harmonic frequency mixing in particular enables broadband electromagnetic signal analysis across octaves of spectrum using a single local oscillator. However, conventional harmonic frequency mixers do not operate beyond hundreds of gigahertz to a few terahertz. If extended to the petahertz scale in a compact and scalable form, harmonic mixers would enable field-resolved optical signal analysis spanning octaves of spectra in a monolithic device without the need for frequency conversion using nonlinear crystals. Here, we demonstrate lightwave-electronic harmonic frequency mixing beyond 0.350 PHz using plasmonic nanoantennas. We demonstrate that the mixing process enables complete, field-resolved detection of spectral content far outside that of the local oscillator, greatly extending the range of detectable frequencies compared to conventional heterodyning techniques. Our work has important implications for applications where optical signals of interest exhibit coherent femtosecond-scale dynamics spanning multiple harmonics.

Science & Technology - Other Topics↗
DOE OSTI2023

Hard x-ray – optical four-wave mixing using a split-and-delay line

New, hard x-ray free electron lasers (FEL) produce intense femtosecond-to-attosecond pulses at angstrom wavelengths, giving access to the fundamental spatial and temporal scales of matter. These revolutionary light sources open the door to applying the suite of nonlinear, optical spectroscopy methods at hard x-ray photon energies. Nonlinear spectroscopy with hard x-rays can allow for measuring the coherence properties of short wavelength excitations with atomic specificity and for understanding how high energy excitations couple to other degrees of freedom in atomic, molecular or condensed-phase systems. As a step in this direction, here we present hard x-ray, optical four-wave mixing (4WM) measurements done at 9.8 keV at the split-and-delay line at the x-ray correlation spectroscopy (XCS) hutch of the Linac Coherent Light Source (LCLS). In this work, we create an x-ray transient grating (TG) from a pair of crossing x-ray beams and diffract optical laser pulses at 400 nm from the TG. The key technical advance here is being able to independently vary the delays of the x-ray pulses. Measurements were made in 3 different solid samples: bismuth germinate (BGO), zinc oxide (ZnO) and yttrium aluminum garnet (YAG). The resulting phase-matched, 4WM signal is measured in two different ways: by varying the x-ray, x-ray pulse delay which can reveal both material and light source coherence properties and also by varying the optical laser delay with respect to the x-ray TG to study how the x-ray excitation couples to the optical properties. Although no coherent 4WM signal was seen in these measurements, the absence of this signal gives important information on experimental requirements for detecting this in future work. Also, our laser-delay scans, although not a new measurement, were applied to different materials than in past work and reveal new examples x-ray induced lattice dynamics in solids. This work represents a key step towards extending nonlinear optics and time-resolved spectroscopy into the hard x-ray regime.

47 OTHER INSTRUMENTATION↗
NASA NTRS1983

Simultaneous observation of rotational coherent Stokes Raman scattering and coherent anti-Stokes Raman scattering in air and nitrogen

Rotational coherent Stokes Raman scattering (CSRS) and coherent anti-Stokes Raman scattering (CARS) in air and in nitrogen were observed simultaneously by using broadband generation and detection. In the broadband technique used, the entire CARS and CSRS spectrum was generated in a single laser pulse; the CSRS and CARS signals were dispersed by a spectrograph and detected simultaneously by an optical multichannel analyzer. A three-dimensional phase-matching geometry was used to achieve spatial resolution of the CSRS and CARS beams from the input beams. Under resonant conditions, similar experiments may provide a means of investigating the possible interaction between the CSRS and CARS processes in driving the rotational levels.

Snow, J. B.↗
NASA NTRS1990

Windshear detection and avoidance - Airborne systems survey

Functional requirements for airborne windshear detection and warning systems are discussed in terms of the threat posed to civil aircraft operations. A preliminary set of performance criteria for predictive windshear detection and warning systems is defined. Candidate airborne remote sensor technologies based on microwave Doppler radar, Doppler laser radar (lidar), and infrared radiometric techniques are discussed in the context of overall system requirements, and the performance of each sensor is assessed for representative microburst environments and ground clutter conditions. Preliminary simulation results demonstrate that all three sensors show potential for detecting windshear, and provide adequate warning time to allow flight crews to avoid the affected area or escape from the encounter. Radar simulation and analysis show that by using bin-to-bin automatic gain control, clutter filtering, limited detection range, and suitable antenna tilt management, windshear from wet microbursts can be accurately detected. Although a performance improvement can be obtained at higher radar frequency, the baseline X-band system also detected the presence of windshear hazard for a dry microburst. Simulation results of end-to-end performance for competing coherent lidar systems are presented.

Bowles, Roland L.↗
NASA NTRS1984

Differential detection of Gaussian MSK in a mobile radio environment

Minimum shift keying with Gaussian shaped transmit pulses is a strong candidate for a modulation technique that satisfies the stringent out-of-band radiated power requirements of the mobil radio application. Numerous studies and field experiments have been conducted by the Japanese on urban and suburban mobile radio channels with systems employing Gaussian minimum-shift keying (GMSK) transmission and differentially coherent reception. A comprehensive analytical treatment is presented of the performance of such systems emphasizing the important trade-offs among the various system design parameters such as transmit and receiver filter bandwidths and detection threshold level. It is shown that two-bit differential detection of GMSK is capable of offering far superior performance to the more conventional one-bit detection method both in the presence of an additive Gaussian noise background and Rician fading.

Simon, M. K.↗
DOE OSTI2024

Precision-controlled ultrafast electron microscope platforms. A case study: Multiple-order coherent phonon dynamics in 1T-TaSe2 probed at 50 fs–10 fm scales

We report on the first detailed beam tests attesting the fundamental principle behind the development of high-current-efficiency ultrafast electron microscope systems where a radio frequency (RF) cavity is incorporated as a condenser lens in the beam delivery system. To allow for the experiment to be carried out with a sufficient resolution to probe the performance at the emittance floor, a new cascade loop RF controller system is developed to reduce the RF noise floor. Temporal resolution at 50 fs in full-width-at-half-maximum and detection sensitivity better than 1% are demonstrated on exfoliated 1T-TaSe2 system under a moderate repetition rate. To benchmark the performance, multi-terahertz edge-mode coherent phonon excitation is employed as the standard candle. The high temporal resolution and the significant visibility to very low dynamical contrast in diffraction signals via high-precision phase-space manipulation give strong support to the working principle for the new high-brightness femtosecond electron microscope systems.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS2000

Airborne Coherent Lidar for Advanced In-Flight Measurements (ACLAIM) Flight Testing of the Lidar Sensor

The purpose of the ACLAIM program is ultimately to establish the viability of light detection and ranging (lidar) as a forward-looking sensor for turbulence. The goals of this flight test are to: 1) demonstrate that the ACLAIM lidar system operates reliably in a flight test environment, 2) measure the performance of the lidar as a function of the aerosol backscatter coefficient (beta), 3) use the lidar system to measure atmospheric turbulence and compare these measurements to onboard gust measurements, and 4) make measurements of the aerosol backscatter coefficient, its probability distribution and spatial distribution. The scope of this paper is to briefly describe the ACLAIM system and present examples of ACLAIM operation in flight, including comparisons with independent measurements of wind gusts, gust-induced normal acceleration, and the derived eddy dissipation rate.

Soreide, David C.↗
DOE OSTI2022

Resolution of 100 photons and quantum generation of unbiased random numbers

Macroscopic quantum phenomena, such as observed in superfluids and superconductors, have led to promising technological advancements and some of the most important tests of fundamental physics. At present, quantum detection of light is mostly relegated to the microscale, where avalanche photodiodes are very sensitive to distinguishing single-photon events from vacuum but cannot differentiate between larger photon-number events. Beyond this, the ability to perform measurements to resolve photon numbers is highly desirable for a variety of quantum information applications including computation, sensing, and cryptography. True photon-number resolving detectors do exist, but they are currently limited to the ability to resolve on the order of 10 photons, which is too small for certain proposals. In this work, we extend photon measurement into the mesoscopic regime by implementing a detection scheme based on multiplexing highly quantum-efficient transition-edge sensors to accurately resolve photon numbers between zero and 100. Further, we then demonstrate the use of our system by implementing a quantum random number generator with no inherent bias. This method is based on sampling a coherent state in the photon-number basis and is robust against environmental noise, phase and amplitude fluctuations in the laser, loss and detector inefficiency as well as eavesdropping. Beyond true random number generation, our detection scheme serves as a means to implement quantum measurement and engineering techniques valuable for photonic quantum information processing.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Time-resolved biphase signatures of quadratic nonlinearity observed in coupled Alfvén eigenmodes on the DIII-D tokamak

We report the detection of nonstationary quadratic coupling between toroidicity-induced Alfvén eigenmodes (TAEs) on sub-millisecond time scales. Identification of phase coherency between multiple TAEs and nonlinearly generated modes is facilitated by wavelet-based bicoherence analysis of time-series from inductive coils, taken from a DIII-D discharge heated by neutral beam injection (NBI). Characterization of nonlinear three-wave interaction is inferred by stationary local bispectrum phase (biphase) and confirmed via bandpass filtering. Biphase dynamics associated with prominent bispectral features are well-resolved in time and consistent with transient quadratic coupling. Onset and duration of nonlinearity are correlated with enhanced amplitude of participating TAEs; coincident changes in amplitude are observed for modes at difference frequency |f TAE,1 - f TAE,2 |.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Generation and control of phase-locked Bessel beams with a persistent noninterfering region

We present, to the best of our knowledge, a novel method for the generation of multiple Bessel-like (Bessel–Gauss) beams with tilted wavefronts whose optical phases can be controlled independently. In the far field multiple field-free regions develop that are persistent to interference effects and the optical phase. The extent of these field-free regions can be controlled through the tilt angle of the wavefront with a theoretical maximum resolution of 0.1 mrad. Experimentally we employ a spatial light modulator, a lens, and an axicon, each suitable for narrow-band (continuous-wave) and broadband operation. Because of the simplicity in the optical elements, the number of noninterfering Bessel-like beams can be scaled on demand for applications that require multiple sources for coherent imaging or multiple intense beams over a controllable region with the added benefit of a field-free region for detection. Here, for reasons of clarity, we characterized two beams.

Rodnova, Zhanna↗
NASA NTRS1978

Long wavelength radar for geological analysis in vegetated terrain

In contrast to shorter wavelength radars, the range of returns from vegetated surfaces is appreciably less at L-band frequencies. However, the evaluation of differences in image quality due to changes in operational frequency is hindered by several system dissimilarities. In particular, a comparison of the Ka, X- and L-band radar imagery is difficult because of differences in 'effective' resolution. Though the physical resolution of these systems may be somewhat comparable, the inherent averaging of the real aperture systems (X-and Ka-) provides an apparent wider range of gray tones. This effect is related to the fact that at a scale where the resolution cell is discernable, the coherent scintillation of 'speckle' of the synthetic aperture L-band system masks tonal variations. This mismatch of effective resolution impedes detection of small changes in gray tone and makes subtle boundary changes less distinct.

Macdonald, H. C.↗
NASA NTRS1985

Semiconductor Laser Phased Array

Oscillations synchronized and modulated individually for beam steering. Phased array of GaAs infrared lasers put out powerful electronically-steerable coherent beam. Fabricated as integrated circuit on GaAs chip, new device particularly suited to optical communications, optical data processing and optical detection and ranging systems.

Katz, J.↗
NASA NTRS1987

Distribution of whistler mode bursts at Venus

Several thousand impulsive whistler mode noise bursts were detected by the Pioneer Venus wave instrument during the first 10 seasons with nightside traversals at low altitudes. The altitude distribution for these events shows that essentially all of the bursts were detected when the orbiter was less than 2000 km above the planet, suggesting that the varying plasma conditions could not maintain coherent whistler mode field-aligned guidance over greater distances. Within the 2000-km range, the distribution of the number of events versus altitude shows that there are two distinct subregions. These results are interpreted in terms of two types of whistler mode propagation from sources below the ionosphere.

Scarf, F. L.↗
NASA NTRS1996

Global Single and Multiple Cloud Classification with a Fuzzy Logic Expert System

An unresolved problem in remote sensing concerns the analysis of satellite imagery containing both single and multiple cloud layers. While cloud parameterizations are very important both in global climate models and in studies of the Earth's radiation budget, most cloud retrieval schemes, such as the bispectral method used by the International Satellite Cloud Climatology Project (ISCCP), have no way of determining whether overlapping cloud layers exist in any group of satellite pixels. Coakley (1983) used a spatial coherence method to determine whether a region contained more than one cloud layer. Baum et al. (1995) developed a scheme for detection and analysis of daytime multiple cloud layers using merged AVHRR (Advanced Very High Resolution Radiometer) and HIRS (High-resolution Infrared Radiometer Sounder) data collected during the First ISCCP Regional Experiment (FIRE) Cirrus 2 field campaign. Baum et al. (1995) explored the use of a cloud classification technique based on AVHRR data. This study examines the feasibility of applying the cloud classifier to global satellite imagery.

Welch, Ronald M.↗
NASA NTRS1999

A Search for Short-Period Accreting Pulsars with BATSE

Accreting X-ray pulsar systems can be detected and monitored by the BATSE Pulsar Monitor at full sensitivity only above the Nyquist period of 2.048 s, since it uses the DISCLA data type. Systems with shorter periods than 2 s can be observed, but with a reduced sensitivity, since only the aliased power is measured. While persistent sources in the period range below that have been found by earlier spacecraft, transient systems may still be undiscovered, due to limited time coverage of the galactic plane with all-sky instruments. BATSE data with a time resolution of 31 ms (PSR single-sweep mode) has been collected for four energy channels spanning 20-50 keV , at scheduled times for particular detectors and detector combinations which view the galactic plane. The data spans Nov 1993 to present, with a typical exposure of 15000 s per day to approximately 1/8 of the plane. An accelerated FFT-based search is in progress on these data. Data are segmented into approximately 300 second intervals, barycentered for 3 possible source directions spaced by 30 degrees about the detector normal, with the time series accelerated for each of 15 steps, each spaced by 5 x 10(exp -5). To avoid loss of coherence due to system orbital velocities, FFTs are averaged over each 1/4 day interval separately. Results of this search are presented, including examples of detection of Her X-1, Cen X-3, and other pulsars.

Wilson, R. B.↗