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At least 595 records · Page 33

Measurements of Atmospheric CO2 Column in Cloudy Weather Conditions using An IM-CW Lidar at 1.57 Micron

This study evaluates the capability of atmospheric CO2 column measurements under cloudy conditions using an airborne intensity-modulated continuous-wave integrated-path-differential-absorption lidar operating in the 1.57-m CO2 absorption band. The atmospheric CO2 column amounts from the aircraft to the tops of optically thick cumulus clouds and to the surface in the presence of optically thin clouds are retrieved from lidar data obtained during the summer 2011 and spring 2013 flight campaigns, respectively.

Lin, Bing↗

Surface Pressure Dependencies in the GEOS-Chem-Adjoint System and the Impact of the GEOS-5 Surface Pressure on CO2 Model Forecast

In the GEOS-Chem Adjoint (GCA) system, the total (wet) surface pressure of the GEOS meteorology is employed as dry surface pressure, ignoring the presence of water vapor. The Jet Propulsion Laboratory (JPL) Carbon Monitoring System (CMS) research team has been evaluating the impact of the above discrepancy on the CO2 model forecast and the CO2 flux inversion. The JPL CMS research utilizes a multi-mission assimilation framework developed by the Multi-Mission Observation Operator (M2O2) research team at JPL extending the GCA system. The GCA-M2O2 framework facilitates mission-generic 3D and 4D-variational assimilations streamlining the interfaces to the satellite data products and prior emission inventories. The GCA-M2O2 framework currently integrates the GCA system version 35h and provides a dry surface pressure setup to allow the CO2 model forecast to be performed with the GEOS-5 surface pressure directly or after converting it to dry surface pressure.

Lee, Meemong↗

Interactions Between Temperature and Intercellular CO2 Concentration in Controlling Leaf Isoprene Emission Rates

Plant isoprene emissions have been linked to several reaction pathways involved in atmospheric photochemistry. Evidence exists from a limited set of past observations that isoprene emission rate (I(sub s)) decreases as a function of increasing atmospheric CO2 concentration, and that increased temperature suppresses the CO2 effect. We studied interactions between intercellular CO2 concentration (C(sub I)) and temperature as they affect I(sub s) in field-grown hybrid poplar trees in one of the warmest climates on earth - the Sonoran Desert of the southwestern United States. We observed an unexpected midsummer down regulation of I(sub s) despite the persistence of relatively high temperatures. High temperature suppression of the I(sub s):C(sub I) relation occurred at all times during the growing season, but sensitivity of I(sub s) to increased C(sub I) was greatest during the midsummer period when I(subs) was lowest. We interpret the seasonal down regulation of I(sub s) and increased sensitivity of I(sub s) to C(sub I) as being caused by weather changes associated with the onset of a regional monsoon system. Our observations on the temperature suppression of the I(sub s):C(sub I) relation are best explained by the existence of a small pool of chloroplastic inorganic phosphate, balanced by several large, connected metabolic fluxes, which together, determine the C(sub I) and temperature dependencies of phosphoenolpyruvate import into the chloroplast.

Monson, Russell K.↗

Changes in the Structure and Propagation of the MJO with Increasing CO2

Changes in the Madden-Julian Oscillation (MJO) with increasing CO2 concentrations are examined using the Goddard Institute for Space Studies Global Climate Model (GCM). Four simulations performed with fixed CO2 concentrations of 0.5, 1, 2 and 4 times pre-industrial levels using the GCM coupled with a mixed layer ocean model are analyzed in terms of the basic state, rainfall and moisture variability, and the structure and propagation of the MJO.The GCM simulates basic state changes associated with increasing CO2 that are consistent with results from earlier studies: column water vapor increases at approximately 7.1% K(exp -1), precipitation also increases but at a lower rate (approximately 3% K(exp -1)), and column relative humidity shows little change. Moisture and rainfall variability intensify with warming. Total moisture and rainfall variability increases at a rate that is similar to that of the mean state change. The intensification is faster in the MJO-related anomalies than in the total anomalies, though the ratio of the MJO band variability to its westward counterpart increases at a much slower rate. On the basis of linear regression analysis and space-time spectral analysis, it is found that the MJO exhibits faster eastward propagation, faster westward energy dispersion, a larger zonal scale and deeper vertical structure in warmer climates.

Adames, Angel F.↗

Frequency Stabilization of DFB Laser Diodes at 1572 nm for Spaceborne Lidar Measurements of CO2

We report a fiber-based, pulsed laser seeder system that rapidly switches among 6 wavelengths across atmospheric carbon dioxide (CO2) absorption line near 1572.3 nm for measurements of global CO2 mixing ratios to 1-ppmv precision. One master DFB laser diode has been frequency-locked to the CO2 line center using a frequency modulation technique, suppressing its peak-to-peak frequency drifts to 0.3 MHz at 0.8 sec averaging time over 72 hours. Four online DFB laser diodes have been offset-locked to the master laser using phase locked loops, with virtually the same sub-MHz absolute accuracy. The 6 lasers were externally modulated and then combined to produce the measurement pulse train.

Numata, Kenji↗

Validation of Regional CO2 Concentrations in the ECMWF Real-Time Analysis and Carbon-Tracker Reanalysis with Airborne Observations from ACT-A Field Campaign

Through verifying against hundreds of hours of airborne in-situ measurements from the NASA-sponsored Atmospheric Carbon and Transport – America (ACT-A) field campaign, this study systematically examines the regional uncertainties and biases of the carbon dioxide (CO2) concentrations from two of the state-of-the-art global analysis products, namely the real-time analysis from the European Center (EC) for Medium Range Forecasting and NOAA’s near real-time Carbon Tracker (CT) reanalysis. It is found that both the EC and CT-NRT analyses agree reasonably well with the independent ACT-A flight-level CO2 measurements in the free troposphere but the uncertainties are considerably larger in the boundary layer during both the summer months of 2016 and the winter months of 2017. There are also strong variabilities in accuracy and bias between seasons, and across three different subregions in the United States (Mid-Atlantic, Midwest and South). Overall, the analysis uncertainties of the EC and CT-NRT analyses in terms of root-mean square deviations against airborne data are comparable to each other, both of which are between 1-2 ppm in the free troposphere but can be as large as 10 ppm near the surface, which are grossly consistent with the difference between the two analyses. The current study not only provides systematic uncertainty estimates for both analysis products over North America but also demonstrated that these two independent estimates can be used to approximate the overall regional CO2 analysis uncertainties. Both statistics are important in future studies in quantifying the uncertainties of regional carbon concentration and flux estimates, as well as in assessing the impact of regional transport through more refined regional modeling and analysis systems.

Chen, Hans W.↗

CO2 Removal for the International Space Station – 4-Bed Molecular Sieve Material Selection and System Design

Efforts over the past three years have focused on the study of candidate sorbent materials for use in a 4BMS molecular sieve system. The accumulation of knowledge has been invaluable for further decisions and for reflecting on the conclusions of past decisions. The goal of the next generation CO2 removal system is continuous, failure-free operation for nearly 20,000 hours, but no complex life support system has yet reached this lofty goal. In addition to reliability, CO2 removal performance improvements have been intensively studied. The achievements toward this end include highly detailed isotherm measurements which drive system simulations as well as testing physical design improvements. Looking back on the successes and failures of past systems, correlating data from long-duration tests, and carefully projecting future results are all needed for the success of the next system. This work intends to reveal the path we have taken and illuminate the steps to come for CO2 removal life support with the 4BCO2 flight demonstration.

Cmarik, Gregory E.↗

Changes in Tropical Clouds and Atmospheric Circulation Associated with Rapid Adjustment Induced by Increased Atmospheric CO2 – A Multiscale Modeling Framework Study

The radiative heating increase due to increased CO2 concentration is the primary source for the rapid adjustment of atmospheric circulation and clouds. In this study, we investigate the rapid adjustment resulting from doubling of CO2 and its physical mechanism using a multiscale modeling framework (MMF). The MMF includes an advanced higher-order turbulence closure in its cloud-resolving model component and simulates realistic shallow and deep cloud climatology and boundary layer turbulence. The rapid adjustment over the tropics is characterized by 1) reduced ascent and descent strengths over the ocean, 2) increased lower tropospheric stability (LTS) over the subsidence region, 3) shoaling of planetary boundary layers over the ocean, 4) increased deep convection over lands and shift of cloud coverage from the ocean to lands, and 5) reduced sensible (SH) and latent heat (LH) fluxes over the oceanic deep convective regions. Unlike conventional general circulation models and another MMF, a reduction in the global-mean shortwave cloud radiative cooling is not simulated, due to the increase in low clouds at lower altitudes over the ocean, resulting from reduced cloud-top entrainment due to strengthened inversion. Changes in regional circulation play a key role in cloud changes and shift of cloud coverage to lands. Weaker energy transport resulting from water vapor and cloud CO2 masking effects reduces the upward motion and convective clouds in the oceanic regions. The ocean-land transports are linked to the partitioning of surface SH and LH fluxes that increases humidity over lands and enhances deep convection over the tropical lands.

Xu, Kuan-Man↗

Modeling Electrolytic Conversion of Metabolic CO2 and Optimizing a Macrofluidic Electrochemical Reactor for Advanced Closed Loop Life Support Systems

The International Space Station (ISS) is currently equipped with a complex, heavy, and power consuming system that recovers approximately 50% of O2 from metabolic CO2. Future long duration missions will require a sustainable and highly efficient system capable of yielding a minimum of 75% O2 recovery. A Macrofluidic Electrochemical Reactor (MFECR) technology development effort is currently underway at NASA Marshall Space Flight Center (MSFC) to significantly increase current O2 recovery efficiency and reduce complexity of the system. This paper presents a comprehensive multi-physic 3D model developed at MSFC on CO2 conversion to O2 and C2H4 at standard conditions via MFECR. The 3D spatial domain of the model is a replica of the actual MFECR’s 3D drawing generated for the MFECR fabrication and operated to recover O2 from CO2 yielding C2H4 as byproduct. Electrochemical (EC) physics that includes EC multicomponent reaction mechanisms, mass transport, and current density distributions is coupled in the model with all the other physics phenomena involved in the process, such as free and porous fluid flow, multicomponent mass transfer, heat transfer, and DC electrical current generation along with Joule heating effect. The authors plan to use experimental results to validate this comprehensive and rigorous model and build a reliable simulator that will not only assist the authors on the MFECR design but also optimize its operation.

Dominguez, Jesus A.↗

Power Optimization of Cryogenic CO2 Deposition Capture in Deep Space

An extremely reliable cabin air revitalization system is needed for human deep space exploration missions. Deep space offers an environmental temperature close to 4 Kelvin. This low environmental temperature enables heat rejection for systems that are thermally power-intensive, i.e. CO2 cold surface deposition (CDep). The CDep system relies on phase change temperatures of air components to deposit CO2 onto a cold surface. The cold surface can be generated utilizing cryocoolers, including Stirling and Reverse Brayton, or deep space environmental temperature. This paper presents a numerical study on a power optimization of cold surface generation via a cryocooler or thermal radiator. An example system for each type is presented. However, a hybrid system would not only reduce power required to remove CO2, but also increase redundancy and reliability of the air revitalization system.

Pranav Jagtap↗

Optimizing CO2 Washout in the Exploration Extravehicular Mobility Unit

CO2 Washout refers to the suit’s ability to remove exhaled metabolic waste gases from the helmet before the crewmember’s next consecutive inhale. Efficient removal of such waste gases is paramount as it prevents crewmember fatigue as well as hypoxia. A variety of hardware and conditions inside the suit contribute to the efficiency at which CO2 washout occurs including (but not limited to) the shape of the helmet bubble, crewmember head position, breathing type and metabolic rate, the configuration of the oxygen vent inside the helmet, etc. While designing the oxygen vent inside the helmet of the Extravehicular Mobility Unit (xEMU) both nominal and contingency scenarios were considered in order to optimize CO2 washout. During nominal Extravehicular Activity (EVA), the pressure gradient created by the vent loop inlets located in the arms and legs of the Pressure Garment Subsystem (PGS) aids in washout by pulling the metabolic waste out of the helmet. However, in the event that a contingency scenario occurs, where the flow of oxygen to the crewmember, or the removal of metabolic waste is disrupted, the primary oxygen regulator fails open and removal of waste is no longer performed by the vent loop, but rather by the Low Flow Purge Valve (LFPV) located in the helmet. The paper to follow will provide an overview of the analysis, design, and testing performed to optimize washout for both nominal and contingency scenarios for the most current design iteration of the xEMU.

Margot Steely↗

Evaluating China's fossil-fuel CO2 emissions from a comprehensive dataset of nine inventories

China's fossil-fuel CO2 (FFCO2) emissions accounted for approximately 28 % of the global total FFCO2 in 2016. An accurate estimate of China's FFCO2 emissions is a prerequisite for global and regional carbon budget analyses and the monitoring of carbon emission reduction efforts. However, significant uncertainties and discrepancies exist in estimations of China's FFCO2 emissions due to a lack of detailed traceable emission factors (EFs) and multiple statistical data sources. Here, we evaluated China's FFCO2 emissions from nine published global and regional emission datasets. These datasets show that the total emissions increased from 3.4 (3.0–3.7) in 2000 to 9.8 (9.2–10.4) Gt CO2 per yr in 2016. The variations in these estimates were largely due to the different EF (0.491–0.746 t C per t of coal) and activity data. The large-scale patterns of gridded emissions showed a reasonable agreement, with high emissions being concentrated in major city clusters, and the standard deviation mostly ranged from 10 % to 40 % at the provincial level. However, patterns beyond the provincial scale varied significantly, with the top 5 % of the grid level accounting for 50 %–90 % of total emissions in these datasets. Our findings highlight the significance of using locally measured EF for Chinese coal. To reduce uncertainty, we recommend using physical CO2 measurements and use these values for dataset validation, key input data sharing (e.g., point sources), and finer-resolution validations at various levels.

Pengfei Han↗

Measuring Atmospheric CO2 Enhancements from the 2017 British Columbia 1 Wildfires Using a Lidar

During the summer 2017 ASCENDS/ABoVE airborne science campaign, the NASA Goddard CO2 Sounder lidar overflew smoke plumes from wildfires in the British Columbia, Canada. In the flight path over Vancouver Island on 8 August 2017, the column XCO2 retrievals from the lidar measurements at flight altitudes around 9 km showed an average enhancement of 4 ppm from the wildfires. A comparison of these enhancements with those from the Goddard Global Chemistry Transport model suggested that the modeled CO2 emissions from wildfires were underestimated by more than a factor of 2. A spiral-down validation performed at Moses Lake airport, Washington showed a bias of 0.1 ppm relative to in situ measurements and a standard deviation of 1 ppm in lidar XCO2 retrievals. The results show that future airborne campaigns and spaceborne missions with this type of lidar can improve estimates of CO2 emissions from wildfires and estimates of carbon fluxes globally.

Jianping Mao↗

3D Simulations of the Early Martian Hydrological Cycle Mediated by a H2-CO2 Greenhouse

For decades, the scientific community has been trying to reconcile abundant evidence for fluvialactivity on Noachian and early Hesperian Mars with the faint young Sun and reasonableconstraints on ancient atmospheric pressure and composition. Recently, the investigation of H2-CO2 collision-induced absorption has opened up a new avenue to warm Noachian Mars. We usethe ROCKE-3D global climate model to simulate plausible states of the ancient Martian climatewith this absorptive warming and reasonable constraints on surface paleopressure. We find that1.5-2 bar CO2-dominated atmospheres with ≥3% H2 can produce global mean surfacetemperatures above freezing, while also providing sufficient warming to avoid surfaceatmospheric CO2 condensation at 0°-45° obliquity. Simulations conducted with both moderntopography and a paleotopography, before Tharsis formed, highlight the importance of Tharsis asa cold trap for water on the planet. Additionally, we find that low obliquity (modern and 0°) ismore conducive to rainfall over valley network locations than high (45°) obliquity. PLAIN LANGUAGE SUMMARY Much evidence tells us that ancient Mars had liquid water on its surface. But reconciling thatwith the fainter young Sun and reasonable constraints on Mars' early atmosphere is challenging.We use a 3D global climate model with an atmosphere containing some amount of hydrogen (apossible greenhouse gas) to study Mars' early hydrological cycle and compare it to the geologicalevidence of surface liquid water billions of years ago. We find that hydrogen and carbon dioxidetogether in an atmosphere twice as thick as modern Earth can warm early Mars above thefreezing point of water and that a low axial tilt produces rainfall patterns that best match thegeologic evidence

Scott D Guzewich↗

Bone Metabolism During Strict Head-Down Tilt Bed Rest with and without CO2 Exposure

Spaceflight and spacecraft have many negative physiological effects on the human body. One such factor is the exposure to elevated levels of carbon dioxide (CO2). In fact, the CO2 levels on board the International Space Station (ISS) have often reached levels 10x higher than outdoor terrestrial levels (1). Among other effects of CO2, it is possible that this exposure alters bone metabolism, leading to an increase of bone tissue resorption and mineral efflux, thus jeopardizing bone fidelity and mission success. Bed rest is a common analog to simulate the effects of microgravity on bone as subjects are placed at a -6° head-down tilt (HDT) position which reduces the mechanical load on bone (2).

E R McGrath↗

Understanding Plant Nitrogen Form Preference Responses to Elevated CO2 Earth and Space Environments

Future long-duration missions to the International Space Station (ISS) and beyond will require a sustainable supply of food to support human crews. The spaceflight cabin environment often contains very high concentrations of CO2, and it is therefore crucial to understand plant responses to elevated CO2 (eCO2) environments. Much focus has been given to plant photosynthetic and performance parameters in response to eCO2, but studies on the effects of eCO2 on nitrogen uptake are poorly understood. Our previous work at The University of Sheffield, UK using novel stable isotope approaches has shown enhanced ammonium uptake and preference compared to nitrate at eCO2 in varieties of spring barley, hypothesized to be an indirect consequence of changes in photosynthesis and photorespiration. However, several varieties did not display altered preference under eCO2 and the universality of this response remains to be understood. In this NASA NPP project, several candidate crop species such as lettuce, radish and tomato will be screened using stable isotopes to assess whether N preference changes in favor of ammonium in response to eCO2 and whether this remains true at super-elevated CO2 (seCO2), which is often experienced on the ISS. Photosynthetic and related measurements will help to disentangle the relationship between these responses and photosynthesis. This work will enable the development of optimized nutrient regimes for candidate crops in space and in future Lunar and Martian habitats and will pave the way for selection of crop varieties adapted to an eCO2 and/or seCO2 environment. Moreover, this research will further our understanding of plant responses to the eCO2 environment brought about by climate change, allowing the development of future-proof crops that will help to maintain food security. This NPP Fellowship is funded by NASA Space Biology.

Luke Leslie Fountain↗

Understanding Plant Nitrogen Form Preference Responses to Elevated CO2 Earth and Spaceflight Cabin Environments

Future long-duration missions to the International Space Station (ISS) and beyond will require a sustainable supply of food to support human crews. The spaceflight cabin environment often contains very high concentrations of CO2, and it is therefore crucial to understand plant responses to elevated CO2 (eCO2) environments. Much focus has been given to plant photosynthetic and performance parameters in response to eCO2, but studies on the effects of eCO2 on nitrogen uptake are poorly understood. Our previous work at The University of Sheffield, UK using novel stable isotope approaches has shown enhanced ammonium uptake and preference compared to nitrate at eCO2 in varieties of spring barley, hypothesised to be an indirect consequence of changes in photosynthesis and photorespiration. However, several varieties did not display altered preference under eCO2 and the universality of this response remains to be understood. In this NASA NPP project, several candidate crop species such as lettuce, radish and tomato will be screened using stable isotopes to assess whether N preference changes in favor of ammonium in response to eCO2 and whether this remains true at super-elevated CO2 (seCO2), which is often experienced on the ISS. Photosynthetic and related measurements will help to disentangle the relationship between these responses and photosynthesis. This work will enable the development of optimized nutrient regimes for candidate crops in space and in future Lunar and Martian habitats and will pave the way for selection of crop varieties adapted to an eCO2 and/or seCO2 environment. Moreover, this research will further our understanding of plant responses to the eCO2 environment brought about by climate change, allowing the development of future-proof crops that will help to maintain food security. This NPP Fellowship is funded by NASA Space Biology.

Luke Fountain↗

Understanding Plant Nitrogen Form Preference Responses to Elevated CO2 Earth and Spaceflight Cabin Environments.

Future long-duration missions to the International Space Station (ISS) and beyond will require a sustainable supply of food to support human crews. The spaceflight cabin environment often contains very high concentrations of CO2, and it is therefore crucial to understand plant responses to elevated CO2 (eCO2) environments. Much focus has been given to plant photosynthetic and performance parameters in response to eCO2, but studies on the effects of eCO2 on nitrogen uptake are poorly understood. Our previous work at The University of Sheffield, UK using novel stable isotope approaches has shown enhanced ammonium uptake and preference compared to nitrate at eCO2 in varieties of spring barley, hypothesised to be an indirect consequence of changes in photosynthesis and photorespiration. However, several varieties did not display altered preference under eCO2 and the universality of this response remains to be understood. In this NASA NPP project, several candidate crop species such as lettuce, radish and tomato will be screened using stable isotopes to assess whether N preference changes in favor of ammonium in response to eCO2 and whether this remains true at super-elevated CO2 (seCO2), which is often experienced on the ISS. Photosynthetic and related measurements will help to disentangle the relationship between these responses and photosynthesis. This work will enable the development of optimized nutrient regimes for candidate crops in space and in future Lunar and Martian habitats and will pave the way for selection of crop varieties adapted to an eCO2 and/or seCO2 environment. Moreover, this research will further our understanding of plant responses to the eCO2 environment brought about by climate change, allowing the development of future-proof crops that will help to maintain food security. This NPP Fellowship is funded by NASA Space Biology.

space plant biology↗