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Technical Documents for Gateway for Accelerated Innovation in Nuclear (GAIN)

The Gateway for Accelerated Innovation in Nuclear (GAIN) provides the nuclear energy community with access to the technical, regulatory, and financial support necessary to move new or advanced nuclear reactor designs toward commercialization. GAIN provides the nuclear community with a single point of access to the broad range of capabilities (i.e., people, facilities, materials, and data) across the U.S. Department of Energy (DOE) complex and its National Lab capabilities. The Fast Flux Test Facility (FFTF) is the most recent liquid metal reactor (LMR) to be designed, constructed, and operated by DOE. The 400-MWt sodium-cooled, fast-neutron flux reactor plant was designed for irradiation testing of nuclear reactor fuels and materials for liquid metal fast breeder reactors. Following the demise of the breeder reactor program in the United States, FFTF continued to play a key role in providing a test bed for demonstrating performance of advanced fuel designs and demonstrating operation, maintenance, and safety of advanced liquid metal reactors. The FFTF Program provides valuable information for potential follow-on reactor projects in the areas of plant system and component design, component fabrication, fuel design and performance, reactor control, prototype testing, and site construction. This report provides documents related to three important aspects of FFTF design and operation: 1) irradiation behavior of structural alloys and absorber materials, 2) thermohydraulics of rod bundles (i.e., coolant mixing), and 3) natural circulation heat transfer in the areas of modeling and validation. These technical documents are believed to be of interest to the nuclear industry and in particular to designers of new liquid metal reactors.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

FFTF Acceptance and Startup Testing for GAIN

The Fast Flux Test Facility (FFTF) is the most recent liquid metal reactor (LMR) to be designed, constructed, and operated by the U.S. Department of Energy (DOE). The 400-MWt sodium-cooled, fast-neutron flux reactor plant was designed for irradiation testing of nuclear reactor fuels and materials for liquid metal fast breeder reactors. Following the demise of the breeder reactor program in the United States, FFTF continued to play a key role in providing a test bed for demonstrating performance of advanced fuel designs and demonstrating operation, maintenance, and safety of advanced liquid metal reactors. FFTF operations ceased in April 1992 after a determination by DOE that no combination of proposed missions was financially feasible over a ten-year period. The reactor is currently deactivated and in a long-term surveillance and maintenance (S&M) mode. This report provides information on the extensive and rigorous process that was used to conduct turnover from construction followed by acceptance and startup testing of the FFTF. This paper is in support of the Gateway for Accelerated Innovation in Nuclear (GAIN), which provides the nuclear energy community with access to the technical, regulatory, and financial support necessary to move new or advanced nuclear reactor designs toward commercialization while ensuring the continued safe, reliable, and economic operation of the existing nuclear fleet. The information obtained from the design, startup, and operation of the FFTF provides valuable insight for follow-on reactor projects, such as the Versatile Test Reactor (VTR), in the areas of plant system and component design, component fabrication, fuel design and performance, prototype testing, site construction, reactor startup and operations, and reactor deactivation and decommissioning (D&D). The focus of this report is on the process used to startup the FFTF and to ensure that operations could be conducted efficiently and safely. A reference section is provided of documents detailing the successful turnover and testing process implemented for startup of the reactor and its supporting systems. The documents listed can be retrieved upon request and are believed useful for future reactor startup endeavors.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Advanced Monitoring and Control in the ANL METL Facility Using an Engineering Digital Twin

The potential benefits of using an engineering digital twin to achieve greater autonomy for monitoring and control functions in advanced reactors was investigated for the Mechanisms Engineering Test Loop (METL) liquid sodium facility at Argonne National Laboratory. The METL sodium purification system served as a representative system as it requires significant human in-the-loop interaction to accomplish its design function. The objective was to demonstrate how real-time operation could be automated while preserving oversight of the operator for ensuring that the system design functions are met. A digital twin model of the purification system was developed for both the cold trap purification loop and plugging meter diagnostic loop using information from the METL piping and instrumentation diagram (P&ID). Automated monitoring and diagnosis of component degradation in the METL facility was demonstrated in tests using the PRO-AID health monitoring software with the digital twin model incorporated in the library of components. Component failures were introduced and were successfully diagnosed in real time. These tests serve to demonstrate an advanced monitoring capability able to differentiate sensor degradation from component degradation, to generate a rank ordering of probabilities of different failure mechanisms that serves to circumvent the false alarm problem with current anomaly detection methods, and how facility monitoring can be transformed from anomaly detection to identification of a specific fault. Automated control of the purification system was demonstrated through simulations that exercised a model predictive controller designed using the digital twin model. Results of these simulations compared favorably with experimental data showing very good reference tracking response with negligible overshoot. In conclusion, these pilot tests and simulations successfully demonstrated the use of a digital twin for improved automation of monitoring and control. It was shown how the digital twin enables switching between control modes from cold trap operation where impurities are removed to plugging meter operation where impurity concentrations are measured.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

NRIC FY 2025 Collaboration Initiatives Annual Report

The National Reactor Innovation Center (NRIC) is a national program established by the U.S. Department of Energy (DOE) in 2019 and led by Idaho National Laboratory (INL). Its mission is to work with industry and national laboratories to bridge the gap between concept, demonstration, and commercialization of advanced nuclear technology. NRIC works to inspire stakeholders and the public, empower innovators, and deliver successful outcomes through efficient collaboration and coordination with partners. NRIC is partnered with industry to accelerate the demonstration and deployment of advanced nuclear technology using DOE’s national laboratory infrastructure and expertise. NRIC’s vision is to establish four new experimental facilitates and two large reactor test beds for integrated technology demonstrators and experimentation by 2028 and complete two advanced nuclear technology tests by 2030.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Post-irradiation Heating Tests of As-Irradiated AGR-3/4 TRISO Fuel Compacts

Four post-irradiation heating tests of fuel compacts from the U.S. Advanced Gas Reactor (AGR)-3/4 irradiation experiment were completed. In addition to tristructural isotropic (TRISO)-coated driver fuel, each compact contained designed-to-fail (DTF) particles with fuel kernels coated only in pyrocarbon so as to simulate exposed kernels. Tests at 1600/1700°C, 1400°C, and 1200°C were performed to measure fission product release as a function of time and temperature. Silver release was highest in the 1200°C test, supporting the observation that silver release rates are highest in the 1100–1300°C range. Compared to tests of AGR-1 compacts with no exposed kernels, the Cs-134 and Kr-85 releases were noticeably higher in AGR-3/4. The exposed kernels’ contributions to Eu and Sr release are inconclusive, due to the difficulty in distinguishing among the combined effects of higher irradiation temperatures in these particular AGR-3/4 compacts, the presence of the DTF particles, and the Fuel Accident Condition Simulator (FACS) test temperatures. These data can be used to make inferences about fission product retention in exposed kernels as a function of time and temperature.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Perspectives on Potential Advanced Construction Technologies for Nuclear Energy

NRIC Enables Nuclear Reactor Tests & Demonstrations Authorized by the Nuclear Energy Innovation Capabilities Act (NEICA) DOE-Office of Nuclear Energy; INL Nuclear Science & Tech Partner with industry to bridge the gap between research and commercial deployment Leverage national lab expertise and infrastructure

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

SCALE depletion capabilities for molten salt reactors and other liquid-fueled systems

Nuclear reactor systems that use fuel dissolved in a liquid have the potential for enhanced safety characteristics, improved fuel-cycle outcomes, and more efficient isotope-production configurations. In these reactor systems, the fueled liquid may simultaneously undergo irradiation, physical and chemical removal processes, and fueling. The modeling and simulation of this transmutation and decay with material additions and removals is an ongoing research area. An accurate simulation tool is critical to the reactor and fuel-cycle design, reactor deployment, and source-term characterization for these advanced reactor systems. The work described herein involved implementing, testing, and applying the capability to perform reactor physics simulations within the Oak Ridge National Laboratory-developed SCALE suite for nuclear systems analyses and design, leveraging much of its pedigree in quality-assurance and reactor-analysis capabilities. The functionalities to simulate irradiation with material feeds and removals had been added in ORIGEN, and the TRITON reactor physics sequence was extended to calculate the total removed material and track external nonirradiated mixtures to estimate separate processing or waste streams. Results from these capabilities align with analytical expectations obtained from ORIGEN for simplified test cases and with expectations for a molten salt reactor application. This implementation, available with the SCALE 6.3 release, provides for a more efficient and accurate material accountability methodology, allowing for the characterization, design, and analysis of the complete isotopic material inventory of advanced liquid-fueled systems for a variety of applications.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Assessment of ASI-developed Sensors for Inclusion in METL Testing

The Advanced Sensors and Instrumentation (ASI) program facilitates the development of new sensors for both conventional and advanced reactors. Advanced reactor concepts utilize coolants other than light water, such as molten salts, liquid sodium, and high-temperature helium. Qualification of sensors developed for these advanced reactors is complicated by the relatively small number of facilities available that can provide relevant testing conditions (e.g., temperature, flow, and coolant chemistry). This report identifies sensors that were developed under the ASI program and may be tested in one available testbed: the Mechanisms Engineering Test Loop (METL) at Argonne National Laboratory (ANL), a non-nuclear liquid sodium flow facility.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A Practical Approach to Starting Fission Surface Power Development

The Prometheus Power and Propulsion Program has been reformulated to address NASA needs relative to lunar and Mars exploration. Emphasis has switched from the Jupiter Icy Moons Orbiter (JIMO) flight system development to more generalized technology development addressing Fission Surface Power (FSP) and Nuclear Thermal Propulsion (NTP). Current NASA budget priorities and the deferred mission need date for nuclear systems prohibit a fully funded reactor Flight Development Program. However, a modestly funded Advanced Technology Program can and should be conducted to reduce the risk and cost of future flight systems. A potential roadmap for FSP technology development leading to possible flight applications could include three elements: 1) Conceptual Design Studies, 2) Advanced Component Technology, and 3) Non-Nuclear System Testing. The Conceptual Design Studies would expand on recent NASA and DOE analyses while increasing the depth of study in areas of greatest uncertainty such as reactor integration and human-rated shielding. The Advanced Component Technology element would address the major technology risks through development and testing of reactor fuels, structural materials, primary loop components, shielding, power conversion, heat rejection, and power management and distribution (PMAD). The Non-Nuclear System Testing would provide a modular, technology testbed to investigate and resolve system integration issues.

Mason, Lee S.↗

Latent Pitfalls in Microstructure-Based Modeling for Thermally Aged 9Cr-1Mo-V Steel (Grade 91)

A case study was conducted on a mechanistic model development that predicted tensile strength deterioration with thermal aging of 9Cr-1Mo-V steel in supporting the 60-year design life expected for advanced nuclear reactors. For property prediction beyond practical testing times, mechanistic modeling is highly desired, as it taps into the physics of structure–property relationships and therefore can generate reliable results for extrapolation. Meanwhile, as mechanistic models are often complicated, reflecting the intricacy of microstructure and strengthening mechanisms, pitfalls that are difficult to detect often exist. Here, this paper discusses latent pitfalls that are common in mechanistic modeling or specific in this 9Cr-1Mo-V case development through using the American Society of Mechanical Engineers verification and validation in computational solid mechanics (ASME V&V 10) standard for evaluating credibility of modeling in materials engineering. Suggestions are also made for enhancing reliability of microstructure-based modeling.

36 MATERIALS SCIENCE↗

Infrastructure and Testing Needs for Molten Salt Reactor Safeguards

Molten salt reactors (MSRs) are an attractive advanced reactor technology because of their increased fuel utilization and efficiency, the ease of fueling, and the potential to use alternative fuel cycles, including thorium and breeder/burner scenarios. Since an MSR has never been domestically operated for commercial electricity production, minimal infrastructure exists to support performance and materials testing, reactor licensing (including research, test, and operating reactors), and technology development in general. These factors could present challenges for the commercialization of the proposed design technology. Several research and development efforts and investments have begun to identify and supplement the infrastructure to accommodate the molten salt concept, including the United States Department of Energy Office of Nuclear Energy Molten Salt Reactor Program. This report reviews safeguards technology and domestic infrastructure to support the evaluation of nuclear safeguards (primarily material control and accounting) measures and approaches for salt-fueled MSRs. Recommendations for potential priority infrastructure investments, including safeguards measurement test beds and future research, are presented.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Testing of Instrumentation and Control Sensors and Cables for Small Modular Reactors

As advanced reactor concepts like small modular reactors (SMRs) progress towards design maturity and commercial deployment, it is important to assess their instrumentation and control (I&C) system sensors and cables to assure their safe, reliable, and efficient operation throughout their service lifetimes. The I&C system of any nuclear power plant (NPP) is the central nervous system of the plant and is made up of field devices such as sensors which are connected via cables to analog and/or digital systems. These systems are responsible for control and/or protection of the plant. The performance of I&C sensors and cables is dependent on several factors, including plant operating conditions. In particular, the plant operation can affect the static (accuracy) and dynamic (response) performance of the sensor, whereas the surrounding ambient environment can impact the remaining useful life of the cables, connectors, and other associated components within I&C sensor circuits.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Fast Reactor Database Utilization for Qualification of Metallic Fuel Forms

The DOE Advanced Reactor Technologies program has supported efforts to recover and preserve metallic fuel data generated throughout the past fast reactor R&D programs. Those efforts are currently focused on establishing databases for information from the experiments conducted during the Integral Fast Reactor program including data generated at EBR-II, FFTF, and TREAT reactors, as well as out of pile transient testing data. These databases are essential for future licensing activities of metallic fuel based advanced fast reactors. This report describes the EBR-II Fuels Irradiation & Physics Database (FIPD) development, content updates, data qualification status, and user support. Future plans are also provided.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGC-2 Graphite Preirradiation Data Analysis Report

This report describes the specimen loading order and documents all preirradiation examination material property measurement data for graphite specimens contained within the Second Advanced Graphite Capsule (AGC 2) irradiation capsule. The AGC 2 capsule is the second in six planned irradiation capsules comprising the Advanced Graphite Creep (AGC) test series. The AGC test series is used to irradiate graphite specimens in order to garner quantitative data necessary for predicting the irradiation behavior and operating performance of new nuclear grade graphites. This testing will ascertain the in service behavior of the graphite for pebble bed and prismatic very high temperature reactor designs. Similar to the First Advanced Graphite Capsule (AGC 1) preirradiation examination report, material property tests were conducted on specimens from 18 nuclear grade graphite types. However, AGC 2 tested an increased number of specimens (i.e., 512) prior to loading them into the AGC 2 irradiation assembly. All AGC 2 specimen testing was conducted at Idaho National Laboratory from July 2009 to August 2010. This report also details the specimen loading methodology for graphite specimens inside the AGC 2 irradiation capsule. The AGC 2 capsule design requires “matched pair” creep specimens that have similar dose levels above and below the neutron flux profile mid plane. This provides similar specimens with and without an applied load. Analysis in this document utilizes the neutron flux profile calculated for the AGC 2 capsule design, the capsule dimensions, and the size (i.e., length) of the selected graphite specimens to create a stacking order that produces “matched pairs” of graphite specimens above and below the AGC 2 capsule elevation mid point, thus providing specimens with similar neutron dose levels.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Long-Term Thermal Aging Effect Evaluation for Grade 92 and 316L at The LWR Relevant Temperature

Life extension of the existing nuclear reactors imposes accumulated damages, such as higher fluences and longer periods of corrosion, to structural materials, which would result in significant challenges to the traditional reactor materials such as type 304 and 316 stainless steels. Advanced alloys with superior radiation resistance will increase safety margins, design flexibility, and economics for not only the life extension of the existing fleet but also new builds with advanced reactor designs. The Electric Power Research Institute (EPRI) initiated a collaboration with the Department of Energy (DOE) Light Water Reactor Sustainability (LWRS) Program on the Advanced Radiation Resistant Materials (ARRM) program, focused on developing and test degradation resistant alloys for light water reactor (LWR)- relevant environments. Based on a comprehensive microstructure and property screening, the ARRM program selected a total of five alloys (i.e., Grade 92, 310, 690, 718A, and 725), together with 316L and X-750 as references, for further investigations.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Elevated Temperature Graphite Mechanical Testing

High purity graphite will be used for core components within most High Temperature Reactor (HTR) designs. Several "high tech” industries currently utilize synthetic, high-purity, commercially available graphite components to fabricate photovoltaic cells, semi-conductors, optical fibers, and other high value electronic industry products. New advanced HTR designs are also interested in using these graphite grades for long-term, internal core component applications. Consequently, the US Department of Energy, Advanced Reactor Technologies (DOE-ART) program has spent several years testing different high purity graphite grades for potential use within these new nuclear reactor designs. A significant part of that effort has been in the development and improvement of American Society for Testing and Materials (ASTM) test standards specifically for nuclear graphite grades. Nearly all ASTM test standards have either been developed or improved by the DOE-ART program over the past 25 years. The ART program continues to assist in the development of new ASTM test standards in support of the future commercial HTR fleet currently being designed and built in the USA. The newest effort undertaken by ART is the development of high temperature mechanical testing practices that may be acceptable for a future ASTM test standard (or guide) for this critical material property measurement.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

FY20 Progress Report on FIPD Development and User Support

The DOE Advanced Reactor Technologies program has supported efforts to recover and preserve metallic fuel data generated throughout the past fast reactor R&D programs. Those efforts have focused on establishing databases for information from the experiments conducted during the Integral Fast Reactor program including data generated at EBR-II, FFTF, and TREAT reactors, as well as out of pile transient testing data. These databases are essential for future-licensing activities of metallic fuel based advanced fast reactors. This report describes the EBR-II Fuels Irradiation & Physics Database (FIPD) development, content updates, and user support during the current fiscal year (FY20). Future plans are also provided.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗