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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

High burn-up spent nuclear fuel vibration integrity study - 15134

The Oak Ridge National Laboratory (ORNL) has developed the cyclic integrated reversible-bending fatigue tester (CIRFT) approach to successfully demonstrate the controllable fatigue fracture of high burnup (HBU) spent nuclear fuel (SNF) in a normal vibration mode. CIRFT enables examination of the underlying mechanisms of SNF system dynamic performance. Due to the inhomogeneous composite structure of the SNF system, the detailed mechanisms of pellet-pellet and pellet-clad interactions and the stress concentration effects at the pellet-pellet interface cannot be readily obtained from a CIRFT system measurement. Therefore, finite element analyses (FEAs) are being used to complement the experimental work by estimating values of local stresses and strains from the measured global moment-curvature. These results and their implications will be used for further investigation. Major findings of CIRFT on the HBU SNF are as follows: - The degree of bonding between pellets, as well as the bonding between pellets and clad in the SNF system plays an important role in the vibration performance of SNF. - Fuel structure contributes to SNF system stiffness. - There are significant variations in stress and curvature of SNF systems during vibration cycles resulting from segment pellet and clad interactions. - SNF failure initiates at the pellet-pellet interface region and appears to be spontaneous. (authors)

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DOE OSTI2016

Immediate Dismantling of a Large Fleet of LWR NPPs: Consequences for Spent Fuel and Waste Management - 16027

The experience feedback shows that the complete dismantling of one Light Water Reactor (LWR) unit is an activity now globally well under control (reactor pressure vessel and its internals removal and cutting included). However some specific industrial difficulties may arise in view of the dismantling of numerous LWR units simultaneously. Indeed more than 300 LWR units are currently operated worldwide, which have been commissioned these last 50 years. So in some countries, many units may be permanently shut down over a period of few years in the next decades. Such a situation addresses the issue of the overall management of large quantities of spent nuclear fuel (SNF) and decommissioning waste for the concerned units. For example, in France, the legislative and regulatory framework for the nuclear facilities favors their dismantling 'as soon as possible' after their permanent shutdown which implies as well to limit the duration of the transition period from operation to decommissioning. Furthermore 58 LWR units have been commissioned between 1977 and 1999 in France - on average more than 2 units per year. In this context, the operator (Electricite de France - EDF) plans to remove quickly the SNF then to perform dismantling actions immediately after the permanent shutdown of the LWR units. One issue is to remove the SNF from all the relevant units, even if this removal is simultaneous in many units (permanently shut down or still under operation). Similar issue has to be taken into account regarding the management of the radioactive waste (RW) produced by the dismantling and clean-up actions, notably the RW that cannot be disposed of in a near surface repository. One method followed by the French technical support organization (Institut de Radioprotection et de Surete Nucleaire - IRSN) to analyze these issues is the use of estimates of flows of SNF and RW. These estimates are based notably on a phasing-scenario and a planning template defined for the decommissioning of the units of one nuclear power plant (NPP) and coupled to an overall schedule for phase out all the units of the fleet. The estimates relative to the next decades can be compared to the current experience feedback of flows of SNF and RW for units under operation, in order to identify risks when facing decommissioning. The risks highlighted are driven by key parameters (as duration of the main dismantling actions) of the estimates which can be adapted to minimize their impact. On this basis, it is possible to identify the key-factors to dismantle each unit of NPPs and phase out the fleet regarding SNF and RW management. It is noteworthy that this work needs to be done in any case upstream the studies and the implementation of dismantling actions. Finally it can be underlined that another issue is the human resources (staff, skills and knowledge) necessary to perform all the decommissioning actions, but this aspect is not addressed in the present paper. (authors)

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DOE OSTI2016

Enhanced Performance Assessment Models for Generic Deep Geologic Repositories for High-Level Waste and Spent Nuclear Fuel - 16223

Development of an enhanced performance assessment (PA) capability for geologic disposal of spent nuclear fuel and high-level waste has been ongoing for several years in the U.S. repository program. The new Generic Disposal System Analysis (GDSA) modeling and software framework is intended to be flexible enough to evolve through the various phases of repository activities, beginning with generic PA activities in the current Concept Evaluation phase to site-specific PA modeling in the Repository Development phase. The GDSA Framework utilizes modern software and hardware capabilities by being based on open-source software architecture and being configured to run in a massively parallel, high-performance computing (HPC) environment. It consists of two main components, the open-source Dakota uncertainty sampling and analysis software and the PFLOTRAN reactive multi-phase flow and transport simulator. Reference cases or 'generic repositories' have been, and are being developed, based on typical properties for potential salt, clay, and granite host-rock formations and corresponding engineered design concepts for each medium. Past simulations have focused on a generic repository in bedded-salt host rock, while the most recent research has focused on a reference case for a typical clay/shale host rock. A variety of single-realization (i.e., deterministic) and multi-realization (probabilistic) results for the new clay reference case are presented, including an analysis of the effects of heat generation on repository performance, assuming a 100-year out-of-reactor commercial SNF waste form. Order-of-magnitude differences between predicted radionuclide concentrations in thermal versus isothermal simulations imply that mechanistic, coupled-process modeling in three-dimensional (3-D) domains can be important for building confidence in post-closure performance assessments. (authors)

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DOE OSTI2016

Examining Supply Chain Resilience for the Inter-modal Shipment of Spent Nuclear Fuel and High Level Radioactive Materials - 16309

The U.S. Department of Energy (DOE) has a significant programmatic interest in the safe and secure routing and transportation of Spent Nuclear Fuel (SNF) and High Level Waste (HLW) in the United States, including shipments entering the country from locations outside U.S borders. In any shipment of SNF/HLW, there are multiple 'chains'; a jurisdictional chain as the material moves between jurisdictions (state, federal, tribal, administrative), a physical supply chain (which mode), as well as a custody chain (which stakeholder is in charge/possession) of the materials being transported. Given these interconnected networks, there lies vulnerabilities, whether in lack of communication between interested stakeholders or physical vulnerabilities such as interdiction. By identifying key links and nodes as well as administrative weaknesses, decisions can be made to 'harden' the physical network and improve communication between stakeholders. This paper examines the parallel chains of oversight and custody as well as the chain of stakeholder interests for the shipments of SNF/HLW and the potential impacts on systemic resiliency. Using the Crystal River shutdown location as well as a hypothetical international shipment brought into the United States, this paper illustrates the parallel chains and maps them out visually. (authors)

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DOE OSTI2016

Perspective of Dry Interim Storage of spent nuclear fuel (SNF) in Germany - 16504

According to article 6 of the German Atomic Energy Act, storage of nuclear fuel requires a license granted by the competent authority in this field, which is the Federal Office of Radiation Protection (BfS). In 1995 a license to store spent nuclear fuel (SNF) and vitrified high level waste (HAW) for the interim storage facility in Gorleben was granted. Dry Interim storage at the NPP sites in its current form started in 2002 in the interim storage facility next to the NPP Lingen. Since this time each NPP erected its own storage facility and three central storage facilities have been built. All of these facilities use dry storage in metallic dual purpose casks (DPCs). The actual storage licenses for SNF and the HAW (which is stored in Gorleben and Rubenow) are limited to 40 years after closing the transport and storage cask. The first license to expire will be the storage license for the interim storage facility in Gorleben in the year 2035. During the last two years in Germany preparatory consultations to restart the process towards finding a repository took place, organised by a commission. This commission consists out of members of the scientific community, religious parties, social communities and environmental organizations as well as members of federal states governments and members of the German parliament (Bundestag). Recently the commission decided to extend its working period until summer 2016. Taking this background into account the BfS plans to intensify its research into extended interim storage with respect to potential material degradation leading to interference with safety functions (e.g. neutron shielding material). This includes topics like ageing of gasket materials which are already studied in ongoing experiments (e.g. at the Federal Institute for Materials Research and Testing) as well as studies of long term relaxation processes. Because of the need for transportation towards a repository another important field is the behaviour of the inventory under mechanical loads. For SNF, first calculations showed that because of the lower decay heat load after 60 years due to hydride reorientation the cladding might become much less ductile. (authors)

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DOE OSTI2016

Spent Nuclear Fuel Management and Disposal in Finland - Status and Lessons Learned at the End of 2015 - 16507

In November 2015 the Finnish Government approved and the Parliament ratified Posiva's 2012 License Application for Construction of a mined, deep geological repository for the spent nuclear fuel (SNF) at the Olkiluoto site in the Eurajoki municipality based upon recommendations provided by the Finnish Radiation Safety Authority (STUK), international expert groups and long-standing local support. The preceding siting process began in 1983 and it included disposal-concept selection (KBS-3V), 'consent-based' site selection and large-scale in-situ tests conducted in an underground research laboratory, the ONKALO, situated ∼440 m below the mean Sea level immediately adjacent to the planned repository at the Olkiluoto site. At the end of 2015, the Finnish SNF repository is projected to open in 2024 as the first of its kind. Four related lessons learned in Finland during the past 30 years are: 1. The selection of potentially-suitable sites for geological disposal of SNF proved to be more difficult and more time consuming than initially envisioned. 2. The siting of nuclear facilities has evolved from being mainly a radionuclide containment and isolation challenge to becoming a critical moving-target, socio-political challenge governing progress with majority local acceptance being a fundamental imperative. 3. Public and political acceptance and support are strongly linked to the competency, credibility and transparency of the involved organisations and the maturity/pedigree of the proposed disposal concept. 4. Timely sharing lessons learned and conducting selective collaborations with other countries proved to be successful keys to timely and cost-effectively obtain and maintain public and political acceptance and support. (authors)

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DOE OSTI2016

Development of an Execution Strategy Analysis (ESA) Capability and Tool for the Management of Spent Nuclear Fuel (SNF) - 16575

An Execution Strategy Analysis (ESA) capability and tool are being developed to evaluate alternative execution strategies for future deployment of a consolidated Interim Storage Facility using a consent-based siting process per the Administration's Strategy for the Management and Disposal of Used Nuclear Fuel and High-Level Radioactive Waste (Strategy). Application of an ESA approach not only leverages but also goes beyond traditional project analysis tools. The ESA tool allows for ongoing performance assessment of the evolving project execution plan that takes into account significant assumptions, risks, and uncertainties throughout the project lifecycle. The ESA process and tool will be used to support the development of plans, budgets, and alternative execution/implementation strategies for meeting the goals of the Strategy. This paper describes the development of the ESA capability and tool and identifies the value of applying such a capability in implementing a long-term strategy for managing spent nuclear fuel and high-level radioactive waste. (authors)

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DOE OSTI2016

Development of a U.S. Rail Transport Capability for Spent Nuclear Fuel and High-Level Waste - 16623

The U.S. Department of Energy, Office of Nuclear Energy (DOE-NE) is laying the groundwork for implementing an integrated nuclear waste management system. This includes preparing for future large-scale transport of spent nuclear fuel (SNF) and high-level radioactive waste (HLW) since transport will be a necessary component of an integrated waste management system. DOE continues to plan and develop options for the design of an integrated nuclear waste management disposition system. A significant destination-independent component of this integrated system is a rail transport capability for SNF and HLW. This paper provides an overview of the current DOE-NE effort related to designing and fabricating prototype rail cars. (authors)

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DOE OSTI2017

Fuel pin zoning to improve the accuracy of the palisades spent fuel pool criticality analysis

Most PWR spent fuel pool criticality analyses assume that the burnup is uniformly distributed among the fuel pins in the assembly. This assumption is accurate for PWR cores that have the typical small inter-assembly gap. The Palisades reactor core, however, is different in that it uses cruciform control rods in between fuel assemblies. Every interior assembly has two sides having a wide water gap and two sides having a narrow water gap. After depleting under these conditions, the pins near the wide water gap will have a higher burnup than the pins in the center. If the burnup is distributed uniformly among the pins, the resulting k calculation will be conservative but excessively so. The excess conservatism was found to be on the order of 1% in k. For this analysis, SCALE 6.1 depletion with TRITON is used followed by the CSAS5 module for the Palisades pool analysis. Several burnup zoning arrangements (uniform enrichment) were investigated ranging from 3 zones to as many as 19 zones. The 19 zone analysis agreed well with a CASMO analysis where every pin was its own depletion zone. It was found that 8 fuel zones gave essentially the same result as 19 zones with less complexity. The depletion calculation using 8 fuel zones instead of a single zone is more complicated but the resulting k calculation no longer has the excessive conservatism seen in a one zone model. (authors)

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DOE OSTI2018

ENRESA's Spent Nuclear Fuel and Special Waste Database - 18115

Empresa Nacional de Residuos Radiactivos S.A. (ENRESA, by its initials in Spanish) Spent Nuclear Fuel (SNF) and Special Waste (SW) database development was initiated in a common effort between ENRESA and UNESA (the Spanish Association of the Electricity Industry) as a consequence of new regulatory requirements in the frame of radioactive waste management plans. Although these requirements were only mandatory for operators of nuclear power plants, ENRESA deemed necessary to have a centralized database which collected the data from the plant operators. The most relevant features of this database are: - The information collected covers not only the general characteristics of the SNF and SW but also the operation details needed for their characterization. - An application, named Gestion de Elementos Combustibles y Residuos Especiales (GECYRE, by its initials in Spanish) has been implemented for easing the queries and the generation of predefined reports. - An agile data transfer scheme, based on XML files, is used for an effective communication between ENRESA and the operators. The database is currently in production phase since 2014. During this phase it has demonstrated its effectiveness as an information repository to address the SNF and SW interim storage projects in Spain foreseen in the near future. (authors)

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DOE OSTI2018

Update on Development of a U.S. Rail Transport Capability for Spent Nuclear Fuel and High-Level Waste - 18518

The U.S. Department of Energy, Office of Nuclear Energy (DOE-NE) is laying the groundwork for implementing an integrated nuclear waste management system. This includes preparing for future large-scale transport of spent nuclear fuel (SNF) and high-level radioactive waste (HLW) since transport will be a necessary component of an integrated waste management system. This paper provides an overview of the progress to date, and discussion of the path forward related to designing, fabricating and testing prototype railcars for rail transport of SNF from commercial nuclear power reactor sites when a receiving site becomes operational. (authors)

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DOE OSTI2016

Cataloguing Past Incidents in Transporting Spent Nuclear Fuel

Shipments of spent nuclear fuel (SNF) and high level radioactive waste (HLW) have a history of more than 50 years, during which tens of thousands of tons of material have been transported in tens of thousands of shipments worldwide. The vast majority of these have been completed without incident. This safety record has been made possible by establishing robust regulatory requirements for the casks used in transport, studying past shipments and incidents, and improving equipment and procedures to lessen the probability and impacts of future events. The authors recently collected a wide array of publicly available information on transportation incidents involving SNF and HLW worldwide. This presented a challenge, as no international or US databases currently exist which are dedicated to SNF and HLW transportation incidents. Thus, sources for this research included national database reports from nations that publish them; technical reports and archival journal papers focused on the solutions to particular transportation problems; and news reports of SNF and HLW transportation incidents, including transportation accidents and protests of shipments. Based on the survey of past transportation incidents, of which several representative descriptions are included in this paper, the authors conclude that (1) the casks in which SNF and HLW are shipped are able to contain their radioactive cargoes in severe accidents because of their robust construction and their being in compliance with regulatory requirements; and (2) most incidents in transporting SNF and HLW have been minor ones, primarily resulting from procedural compliance deficiencies. Furthermore, recent incidents suggest that public information and engagement challenges outweigh technical challenges in SNF and HLW transportation, since the most significant challenges surrounding shipments in recent years have been the results of public demonstrations and protests. This paper discusses some SNF and HLW transportation incidents, as well as the process used in cataloguing them. In general, there have been few transportation incidents worldwide in the history of transporting SNF and HLW. The transportation of SNF and HLW has an excellent safety record; by learning from past incidents, shippers of SNF and HLW can continue to make safe shipments while avoiding mistakes made in the past. Despite the safe and successful record of SNF and HLW transportation, information on its record is not easy to find. Few incidents are detailed as thoroughly as the truck accident that occurred in 1971. Several anti-nuclear organizations publish pamphlets that make reference to transportation accidents involving radioactive material and imply that transporting SNF and HLW is an intrinsically dangerous activity whose history is fraught with accidents. The absence of a clear, complete, official record on transportation incidents allows these claims to continue to be unanswered and uncorrected. For these reasons, it would be beneficial to develop a database detailing incidents involving SNF and HLW internationally. (authors)

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DOE OSTI2016

Risk-Informed Maritime Spent Fuel Transportation

South Korea is facing a shortage of Spent Nuclear Fuel (SNF) storage space. The country generates approximately 760 metric tons of SNF annually out of its 23 Nuclear Power Plants (NPPs). Until any terminal solutions of the back-end fuel cycle is decided, there exists the need to relocate these SNF assemblies from relatively packed storage pools to the more vacant ones. Since NPPs in South Korea are situated at coastal sites, the maritime mode of transportation is more practical for this purpose in comparison to land and air ones. The primary risk factors in this transportation mode, based on the data collected by the Korea Maritime Institute from 1981 until 2013, are ship collision and engine damage. However, because ship collision may initiate other accident types such as sinking, fire or engine damage, it may be considered as the most hazardous event. It is therefore a significant interest to calculate the likelihood of this event. This paper proposes a risk assessment methodology on the maritime SNF transportation in the form of the quantification of ship collision probability. To demonstrate the applicability of the methodology, a transportation case study in South Korea is presented. (authors)

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DOE OSTI2016

Proposed Muon Radiography Method for Spent Fuel Cask Interrogation

Multiple scattering muon radiography is a technique that was developed at Los Alamos National Laboratory (LANL) to detect high Z material using cosmic ray muons as a radiation source. As a result,there has been considerable interest in using the technique to radiograph nuclear waste inside of storage casks. Recently,the technique has been used to interrogate the inside of a MC-10 dry fuel cask at Idaho National Laboratory (INL).This is the only technique that has been successful in imaging the interior of a spent fuel cask.The measurement was performed with the LANL Mini Muon Tracker (MMT), composed of two super-modules of drift tubes and readout electronics placed on each side of the fuel cask. The final result was a one dimensional histogram (projection) that showed areal scattering density within the cask binned according to horizontal position within the cask. While successful, the MMT is not designed for an optimal measurement of a fuel cask. The MMT only covers a limited solid angle around the cask and needs to be orientated so as to be aligned with the grid of stored fuel bundles. Even when properly aligned, the resulting areal scattering density projection indicates that a fuel bundle within a column is missing, but is ambiguous as to which row is lacking the fuel bundle. This paper discusses a potential new detector and analytical technique that may be used to better radiograph the nuclear material inside of a storage cask. (authors)

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DOE OSTI2019

Factors Influencing the Evaluation of Spent Fuel Rail Routes - 19010

The U.S. Department of Energy (DOE) is considering use of rail transport for future shipments of commercial spent nuclear fuel (SNF) from where it currently resides to storage or disposal facilities. Rail carriers transporting in commerce certain quantities of 'rail security sensitive materials,' including SNF, face a regulatory requirement from the U.S. Department of Transportation to perform route risk assessments on an annual basis. In performing these assessments, each affected rail carrier must take into consideration twenty-seven different route factors, and document its rationale for selecting preferred and alternative routes on the basis of the safety and security risk analysis results. The major freight rail carriers operating in the U.S. have invested in the development of a proprietary tool, for rail carrier use only, to assist them in making route selections. This tool utilizes operations data input by each affected rail carrier in conjunction with geographic information systems (GIS) data to represent proximate risk factors, to be integrated and assigned to individual points and segments on the railroad network. Separate safety and security risk values are generated for each rail route under consideration. These values are then placed on an equivalent scoring basis and summed together to allow direct comparison between different route options and to rank order each route in terms of its relative attractiveness. Each affected rail carrier files an annual report for evaluation by the Federal Railroad Administration (FRA) that documents its route risk assessment approach and analysis results. DOE has developed its own decision-support tool, Stakeholder Tool for Assessing Radioactive Transportation (START), which is capable of generating and analyzing routing options for transporting SNF by rail in addition to other freight modes. To better understand how affected rail carriers are likely to route SNF shipments in accordance with regulatory requirements and those route factors likely to be most influential in impacting DoE's evaluation of alternative SNF rail routes, a study was undertaken by DOE with the following objectives: - Review the shipment routes that have been historically used by rail carriers to move high hazard materials, including SNF; - Identify the physical, operational and proximate characteristics (attributes) associated with the rail segments that comprise these routes; - Evaluate the relationships between these attributes; - Make suggestions for how to streamline the factors used in DoE's rail route evaluations; - Contrast these relationships with how the factors are used by the rail carriers in applying their tool This paper describes the study approach, analysis results, and implications for rail route selection methodology. Differences between this evaluation and railroad industry information about rail route assessments are also discussed. (authors)

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DOE OSTI2019

Support of UJV Rez, a. s. for Shipments of Spent Nuclear Fuel Within the M3 Program - 19035

In 2005, UJV Rez, a. s. (UJV, the former Nuclear Research Institute Rez), Czech Republic joined the Russian Research Reactor Fuel Return (RRRFR) program under the US-Russian Global Threat Reduction Initiative (GTRI) (now Material Management and Minimization program, M{sup 3}). The primary goal of the program is to advance nuclear nonproliferation objectives encouraging eligible countries to convert their research reactors from highly enriched uranium (HEU) to low enriched uranium (LEU) fuel and eliminating stockpiles of HEU. UJV's daughter company, Research Centre Rez, operates the LVR-15 research reactor with output of 10 MWth, which has been in operation since 1957. After more than 50 years of operation of the reactor, a large amount of spent nuclear fuel (SNF) of Russian origin had been accumulated. The SKODA VPVR/M high capacity casks were used for SNF shipment from the LVR-15 research reactor back to the Russian Federation (RF). The cask has a capacity of 36 fuel assemblies, and 16 casks are available. This means that 576 FA can be transported in one shipment. Two SNF shipments of HEU and LEU SNF from UJV were realized in 2007 and 2013. After the shipments were completed, only LEU nuclear fuel remained on the territory of the Czech Republic. Proven to be an excellent and very sophisticated system for SNF transportation, the SKODA VPVR/M casks were further employed for SNF shipments from Bulgaria, Hungary, Poland, Ukraine, Belarus, Serbia, Vietnam, Uzbekistan and Georgia to Russia. Some shipments were carried out as air shipments with use of the TUK-145/C cask system developed in Russia that included the SKODA cask. In 2016, the new SKODA MNSR casks were developed on the base of the SKODA VPVR/M casks in the Czech Republic and currently are being employed in the shipments of HEU cores of Chinese Miniature Neutron Source Reactors (MNSR) to China. The TUK-145/C-MNSR cask system developed in Russia is used for air transportation. The shipment from Ghana was carried out in 2016; the shipment from Nigeria is under realization. Shipments from Syria, Iraq and Pakistan are planned. Sixteen shipments from eleven countries using a total of 109 SKODA casks have already been completed without any incident or accident and more than 3500 fuel assemblies or cores have been shipped to Russia and China. (authors)

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DOE OSTI2019

A Thermal Model for the Performance Analysis of Large Scale Spent Fuel Cooling Pond - 19173

This paper presents a thermal model for the performance analysis of a large scale cooling pond for the long term storage of spent nuclear fuel. The model has been developed using the knowledge gained from fundamental investigation using CFD and has been validated by comparing against reliable experimental and/or numerical data. It was then applied in the context of operation of a large scale pond to ascertain the sensitivity of various operational and environmental conditions. To develop the model, the water body along with the heating elements was considered as one zone and humid air inside the building as another zone, both of which are considered as well-mixed zones. Various input conditions namely, total heat load from the heat source, environmental temperature and relative humidity, ventilation rate, efficiency of the cooling tower, recirculation and make-up water flow rates have been programmed in the model. The statistical method AVONA has been used to assess the influence of the above variables. The results reveal that the efficiency of the cooling tower is the most influential parameter on the cooling performance of cooling pond within the considered values of heat load. It has also been found that the majority of the heat is taken by the recirculating water for very high heat load while the other modes of heat transfer are small but not insignificant. The model is capable of simulating the scenario of loss of cooling water and suggests that it can be used for managing a large pond efficiently as well as recovery from an accident situation. (authors)

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DOE OSTI2019

Development of Transient Coupled Chemical-Thermal-Fluids Simulation for Unsealed Aluminum-Clad Spent Nuclear Fuel Storage Canister - 19273

This study examines a preliminary three-dimensional (3D) multi-physics computational fluid dynamics (CFD) model of the unsealed canisters containing aluminum-clad spent nuclear fuel from INL's ATR in the irradiated fuel storage facility. This 3D CFD model considers fully resolved fuel plates in an unsealed canister with small mass exchange with surrounding air as time evolves in the simulation and contains a network of chemical reactions to consider due to several of the side reactions occurring in the presence of water vapor, nitrogen, oxygen and carbon dioxide rather than in helium backfilled DOE standard canisters. Prior to the CFD modeling, the full set of chemical reactions under these conditions was analyzed, reduced, and refit to a more manageable number of equations for the computational efficiency of the 3D CFD simulation. To deal with the long time-scale of interest for tracking the possible buildup of trace species such as nitric acid, NOx, and hydrogen, a segregated time stepping algorithm is used, wherein the velocity field is only updated periodically, and assumed to be in a pseudo steady state. This study first examines the theory of the model, workflow to establish radiolysis reaction network, and initial simulations of the evolutions of thermal fields, hydrogen gas and nitric acid concentrations within unsealed canisters in conditions relevant to the INL INTEC CPP-603 facility over a long period of time. (authors)

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