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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2013

Super-resolving quantum radar: Coherent-state sources with homodyne detection suffice to beat the diffraction limit

There has been much recent interest in quantum metrology for applications to sub-Raleigh ranging and remote sensing such as in quantum radar. For quantum radar, atmospheric absorption and diffraction rapidly degrades any actively transmitted quantum states of light, such as N00N states, so that for this high-loss regime the optimal strategy is to transmit coherent states of light, which suffer no worse loss than the linear Beer's law for classical radar attenuation, and which provide sensitivity at the shot-noise limit in the returned power. We show that coherent radar radiation sources, coupled with a quantum homodyne detection scheme, provide both longitudinal and angular super-resolution much below the Rayleigh diffraction limit, with sensitivity at shot-noise in terms of the detected photon power. Our approach provides a template for the development of a complete super-resolving quantum radar system with currently available technology.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2011

High-Energy Calibration of a BGO Detector of the GLAST Burst Monitor

The understanding of the instrumental response of the GLAST Burst Monitor BGO detectors at energies above the energy range which is accessible by common laboratory radiation sources (< 4.43 MeV), is important, especially for the later cross-calibration with the LAT response in the overlap region between {approx}20 MeV to 30 MeV. In November 2006 the high-energy calibration of the GBM-BGO spare detector was performed at the small Van-de-Graaff accelerator at SLAC. High-energy gamma-rays from excited {sup 8}Be* (14.6 MeV and 17.5 MeV) and {sup 16}O* (6.1 MeV) were generated through (p, {gamma})-reactions by irradiating a LiF-target. For the calibration at lower energies radioactive sources were used. The results, including spectra, the energy/channel-relation and the dependence of energy resolution are presented.

43 PARTICLE ACCELERATORS↗
DOE OSTI2011

Controlled Co(II) Doping of Zinc Oxide Nanocrystals

Dopants are non-native atoms commonly used to modify the properties of bulk semiconductors. In this paper we demonstrate that by controlling the addition of cobalt(II) to growing zinc oxide nanocrystals (ZnO NCs) it is possible to modulate the resulting properties. We show that the environment of cobalt may be controlled by varying the synthetic conditions, mainly through varying the time of dopant-precursor addition and concentration. These conditions prove critical to the resulting Co(II) configuration, which affects both the luminescent and photocatalytic properties of the ZnO NCs. Presynthetic doping with 2% Co(II) results in a 98% quenching of the visible emission of ZnO, whereas the same quantity doped post synthesis results in only a 60% quenching. The environment of cobalt in the ZnO wurtzite lattice is identified through UV-vis spectroscopy. The wurtzite structure of the ZnO lattice for all nanocrystalline species is confirmed through X-ray diffraction patterns obtained from a synchrotron radiation source. Postsynthetically doped Co(II) in ZnO NC is demonstrated to have potential applications as an 'on-off' sensor, as exemplified with nitric oxide.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2011

Ultrarelativistic nanoplasmonics as a route towards extreme-intensity attosecond pulses

The generation of ultrastrong attosecond pulses through laser-plasma interactions offers the opportunity to surpass the intensity of any known laboratory radiation source, giving rise to new experimental possibilities, such as quantum electrodynamical tests and matter probing at extremely short scales. Here we demonstrate that a laser irradiated plasma surface can act as an efficient converter from the femto- to the attosecond range, giving a dramatic rise in pulse intensity. Although seemingly similar schemes have been described in the literature, the present setup differs significantly from the previous attempts. We present a model describing the nonlinear process of relativistic laser-plasma interaction. This model, which is applicable to a multitude of phenomena, is shown to be in excellent agreement with particle-in-cell simulations. The model makes it possible to determine a parameter region where the energy conversion from the femto- to the attosecond regime is maximal. Based on the study we propose a concept of laser pulse interaction with a target having a groove-shaped surface, which opens up the potential to exceed an intensity level of 10{sup 26} W/cm{sup 2} and observe effects due to nonlinear quantum electrodynamics with upcoming laser sources.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2011

Theoretical analysis of the possibilities of Zernike phase contrast method in hard X rays for nondestructive imaging of micropipes in a silicon carbide single crystal

The possibilities of using Zernike phase contrast in hard X rays for imaging micropipes in a silicon carbide single crystal are analyzed by numerical simulation. Calculations are performed for the experimental conditions characteristic of third-generation synchrotron radiation sources. A scheme is considered where the focusing element is a parabolic refracting lens and the phase-shifting element is mounted at the point of the source image. It is shown that micropipe cross sections by a beam with a longitudinal diameter reaching 10 {mu}m are imaged by the lens without distortions. At the same time, the lens makes it possible to magnify the image several tens of times. The cross sections that are significantly elongated along the beam are imaged with artifacts; however, their structure can also be recovered. It is shown that polychromaticity of radiation does not significantly affect the object imaging.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2010

A Miniature Maxthal Furnace for X-ray Spectroscopy and Scattering Experiments up to 1200 degrees C

We have built a new small furnace to perform high temperature studies up to 1200 deg. C in vacuum or in oxygen atmosphere. This furnace was originally used as a catalytic reactor optimized for the in situ X-ray Absorption Spectroscopy experiments on beamline ID24. It has now been redesigned for use on the ESRF beamline ID01 for in situ Grazing Incidence Small Angle X-ray Scattering experiments. For these experiments high mechanical stability of the sample holder is necessary to keep the alignment of the sample during heating.

43 PARTICLE ACCELERATORS↗
DOE OSTI2018

Synthesis of radially aligned nano-rutile modified with Au and Ni for the photodegradation of methyl orange

Radially aligned nano-rutile (RANR) was synthesized using the hydrothermal technique. The RANR structure was formed by the radial aggregation of nanorods with an average width of 9 nm. The radii of RANR ranged between 1.2–1.6 μm. Au and Ni (0.5–10 wt.%) nanoparticles were deposited on the tips of RANR by the deposition-precipitation method using urea. The UV–vis DRS spectrum of RANR had a band edge at 3.2 eV, whereas those of Ni-RANR and Au-RANR were characterized by reflectance peaks that extended into the visible part of the spectrum, with Au-RANR having an SPR peak at 2.25 eV. Photoluminescence studies showed that loading RANR with Ni and Au reduced the recombination rate of the charge carriers. The photodegradation efficiency of the various materials was tested on methyl orange using solar simulator radiation source. RANR was the least efficient material, followed by Ni-RANR composites, with Au-RANR composites having the highest activity.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2010

Application of laser photothermal spectroscopy for standoff detection of trace explosive residues on surfaces

Laser photothermal methods of standoff detection of trace explosive residues on surfaces are considered. The analysis is restricted to the most promising methods: photoacoustic spectroscopy, deflection spectroscopy, and IR photothermal imaging of objects under resonant irradiation. Particular attention is paid to the choice of radiation sources and detectors. Comparative analysis of the existing standoff detection methods for explosive particles on the object surface is performed. Prospects of laser photothermal spectroscopy in this field are discussed. (review)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2019

Regular Microstructures Based on Polyethylene Terephthalate Films

A method for forming regular dielectric and metallic microstructures based on polyethylene terephthalate films irradiated with a synchrotron radiation source through a mask with subsequent etching. To study their geometric parameters, scanning electron microscopy was used.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2012

Optimization of the Coherent Intensity from Multi-Segment Undulators by Phase Matching

The use of inline insertion devices at third-generation synchrotron radiation sources can result in destructive interference effects if the relative phase between the devices is not properly adjusted. The destructive interference can strongly affect the emission spectrum and coherent wavefront of a compound insertion device. We simulate the photon source generated by a dual-inline elliptically polarizing undulator (EPU) situated in a low-{beta} straight section of the planned NSLS-II storage ring and show that a magnetic chicane with adjustable field integral can be used to phase-match the devices. Furthermore, we show that the maximum coherent intensity is delivered by a focusing x-ray beamline if the chicane is adjusted to phase-match the off-axis and red-shifted radiation. Such a system will be installed at the coherent soft x-ray (CSX) beamline of the NSLS-II in order to provide the highest possible coherent flux for coherent soft x-ray scattering experiments.

36 MATERIALS SCIENCE↗
DOE OSTI2010

High Heat Load Diamond Monochromator Project at ESRF

Due to its outstanding thermal properties, diamond is an attractive alternative to silicon as a monochromator material for high intensity X-ray beams. To date, however, the practical applications have been limited by the small size and relatively poor crystallographic quality of the crystals available. The ESRF Diamond Project Group has studied the perfection of diamonds in collaboration with industry and universities. The group has also designed and tested different stress-free mounting techniques to integrate small diamonds into larger X-ray optical elements. We now propose to develop a water-cooled Bragg-Bragg double crystal monochromator using diamond (111) crystals. It will be installed on the ESRF undulator beamline, ID06, for testing under high heat load. This monochromator will be best suited for the low energy range, typically from {approx}3.4 keV to 15 keV, due to the small size of the diamonds available and the size of the beam footprint. This paper presents stress-free mounting techniques studied using X-ray diffraction imaging, and their thermal-mechanical analysis by finite element modelling, as well as the status of the ID06 monochromator project.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2010

The High Energy Materials Science Beamline (HEMS) at PETRA III

The HEMS Beamline at the German high-brilliance synchrotron radiation storage ring PETRA III is fully tunable between 30 and 250 keV and optimized for sub-micrometer focusing. Approximately 70 % of the beamtime will be dedicated to Materials Research. Fundamental research will encompass metallurgy, physics and chemistry with first experiments planned for the investigation of the relationship between macroscopic and micro-structural properties of polycrystalline materials, grain-grain-interactions, and the development of smart materials or processes. For this purpose a 3D-microsctructure-mapper has been designed. Applied research for manufacturing process optimization will benefit from high flux in combination with ultra-fast detector systems allowing complex and highly dynamic in-situ studies of micro-structural transformations, e.g. during welding processes. The beamline infrastructure allows accommodation of large and heavy user provided equipment. Experiments targeting the industrial user community will be based on well established techniques with standardized evaluation, allowing full service measurements, e.g. for tomography and texture determination. The beamline consists of a five meter in-vacuum undulator, a general optics hutch, an in-house test facility and three independent experimental hutches working alternately, plus additional set-up and storage space for long-term experiments. HEMS is under commissioning as one of the first beamlines running at PETRA III.

43 PARTICLE ACCELERATORS↗
DOE OSTI2019

Dynamics of Spatially Inhomogeneous Spin Polarization of Nonequilibrium Conduction Electrons in Magnetic Transitions

The equation of the dynamics of the magnetic moment motion that has been averaged over the ensemble of nonequilibrium spin-injected electrons in a ferromagnetic transition in the presence of exchange interaction, interaction with an external electromagnetic field, and a thermostat has been obtained taking into account the spatial inhomogeneity of the charge carrier distribution. It has been shown that taking into account the spatial inhomogeneity of the charge carrier distribution in the equation of the dynamics of the magnetic moment motion allows for describing the various processes of electron transfer in the magnetic transition. The probability of quantum transitions of electrons with opposite spin directions, which determine spin relaxation in interaction with a thermostat, has been estimated. It has been shown that the anisotropy of the radiation medium is determined not only by the anisotropy of the sd-exchange tensor, but also by the additional anisotropy that is caused by the electron impulse derivatives of this tensor. The considered phenomena have a great potential for the detection of new effects and development of new devices based on them, including compact tunable radiation sources in the terahertz frequency range, which is obviously difficult to generate.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2011

NSLS-II X-Ray Diagnostics Development

NSLS-II x-ray diagnostics will provide continuous online data of electron beam dimensions, which will be used to derive electron beam emittance and energy spread. It will also provide information of electron beam tilt for coupling evaluation. X-ray diagnostics will be based on imaging of bending magnet and three-pole wiggler synchrotron radiation sources. Diagnostics from three-pole wiggler source will be used to derive particles energy spread. Beta and dispersion functions will have to be evaluated for emittance and particles energy spread calculations. Due to small vertical source sizes imaging need to be performed in x-ray energy range. X-ray optics with high numerical aperture, such as compound refractive lens, will be used to achieve required spatial resolution. Optical setups with different magnifications in horizontal and vertical directions fill be employed to deal with large aspect ratio of the source. X-ray diagnostics setup will include x-ray imaging optics, monochromatization, x-ray imaging and recording components.

43 PARTICLE ACCELERATORS↗
DOE OSTI2016

Cosmological simulations of early black hole formation: halo mergers, tidal disruption, and the conditions for direct collapse

Gravitational collapse of a massive primordial gas cloud is thought to be a promising path for the formation of supermassive black holes in the early universe. We study conditions for the so-called direct collapse (DC) black hole formation in a fully cosmological context. We combine a semianalytic model of early galaxy formation with halo merger trees constructed from dark matter N-body simulations. We locate a total of 68 possible DC sites in a volume of 20 h{sup −1} Mpc on a side. We then perform hydrodynamics simulations for 42 selected halos to study in detail the evolution of the massive clouds within them. We find only two successful cases where the gas clouds rapidly collapse to form stars. In the other cases, gravitational collapse is prevented by the tidal force exerted by a nearby massive halo, which otherwise should serve as a radiation source necessary for DC. Ram pressure stripping disturbs the cloud approaching the source. In many cases, a DC halo and its nearby light source halo merge before the onset of cloud collapse. When the DC halo is assembled through major mergers, the gas density increases rapidly to trigger gravitational instability. Based on our cosmological simulations, we conclude that the event rate of DC is an order of magnitude smaller than reported in previous studies, although the absolute rate is still poorly constrained. It is necessary to follow the dynamical evolution of a DC cloud and its nearby halo(s) in order to determine the critical radiation flux for DC.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

Dynamic Control over Mega-Ampere Electron Currents in Metals Using Ionization-Driven Resistive Magnetic Fields

The possibility of dynamically shaping mega-ampere electron currents generated in solids by ultraintense laser pulses in various conductor materials has been investigated. By tuning the target ionization dynamics, which depends both on the target material properties and on the input electron beam characteristics, we can control the growth of resistive magnetic fields that feedback on the current transport. As a result, collimation, hollowing, or filamentation of the electron beam can all be obtained. These results are beneficial for applications such as the production of secondary particles and radiation sources and fast ignition of inertial confinement fusion.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Low-coherence terahertz tomography based on spatially separated counterpropagating beams with allowance for probe radiation absorption in the medium

This paper analyses low-coherence tomography of absorbing media with the use of spatially separated counterpropagating object and reference beams. A probe radiation source based on a broadband terahertz (THz) generator that emits sufficiently intense THz waves in the spectral range 90 – 350 μm and a prism spectroscope that separates out eight narrow intervals from this range are proposed for implementing this method. This allows media of interest to be examined by low-coherence tomography with counterpropagating beams in each interval. It is shown that, according to the Rayleigh criterion, the method is capable of resolving inhomogeneities with a size near one quarter of the coherence length of the probe radiation. In addition, the proposed tomograph configuration allows one to determine the average surface asperity slope and the refractive index and absorption coefficient of inhomogeneities 180 to 700 mm in size, and obtain spectra of such inhomogeneities in order to determine their chemical composition. (laser applications and other topics in quantum electronics)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2015

The spectral imaging facility: Setup characterization

The SPectral IMager (SPIM) facility is a laboratory visible infrared spectrometer developed to support space borne observations of rocky bodies of the solar system. Currently, this laboratory setup is used to support the DAWN mission, which is in its journey towards the asteroid 1-Ceres, and to support the 2018 Exo-Mars mission in the spectral investigation of the Martian subsurface. The main part of this setup is an imaging spectrometer that is a spare of the DAWN visible infrared spectrometer. The spectrometer has been assembled and calibrated at Selex ES and then installed in the facility developed at the INAF-IAPS laboratory in Rome. The goal of SPIM is to collect data to build spectral libraries for the interpretation of the space borne and in situ hyperspectral measurements of planetary materials. Given its very high spatial resolution combined with the imaging capability, this instrument can also help in the detailed study of minerals and rocks. In this paper, the instrument setup is first described, and then a series of test measurements, aimed to the characterization of the main subsystems, are reported. In particular, laboratory tests have been performed concerning (i) the radiation sources, (ii) the reference targets, and (iii) linearity of detector response; the instrumental imaging artifacts have also been investigated.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗