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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Probing the Magnetosheath Boundaries Using Interstellar Boundary Explorer (IBEX) Orbital Encounters

Inside the magnetosheath, the IBEX-Hi energetic neutral atom (ENA) imager measures a distinct background count rate that is more than 10 times the typical heliospheric ENA emissions observed when IBEX is outside the magnetosheath. The source of this enhancement is magnetosheath ions of solar wind (SW) origin that deflect around the Earth's magnetopause (MP), scatter and neutralize from the anti-sunward part of the IBEX-Hi sunshade, and continue into the instrument as neutral atoms, behaving indistinguishably from ENAs emitted from distant plasma sources. While this background pollutes observations of outer heliospheric ENAs, it provides a clear signature of IBEX crossings over the magnetospheric boundaries. In this study, we investigate IBEX encounters with the magnetosheath boundaries using ~8 yr of orbital data, and we determine the MP and bow shock (BS) locations derived from this background signal. We find 280 BS crossings from X GSE ~ 11 R e to X GSE ~ –36 R e and 241 MP crossings from X GSE ~ 6 R e to X GSE ~ –48 R e . We compare IBEX BS and MP crossing locations to those from IMP-8, Geotail, Cluster, Magion-4, ISEE, and Magnetospheric Multiscale Mission, and we find that IBEX crossing locations overlap with the BS and MP locations inferred from these other data sets. In this paper, we demonstrate how IBEX can be used to identify magnetosheath crossings, and extend boundary observations well past the terminator, thus further constraining future models of magnetosheath boundaries. Furthermore, we use the IBEX data set to show observational evidence of near-Earth magnetotail squeezing during periods of strong interplanetary magnetic field B y .

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2004

Science Questions for the Post-SIRTF and Herschel Era

The contents include the following: 1. SIRTF. Long wavelength surveys planned for SIRTF. Galaxy Discovery Rates for Future Missions. Impact of SIRTF s Improved Resolution at 160um: Resolving the Background. 2. Polarimetry. Submillimeter Polarimetry - The State of Play. Magnetic Vectors Across the Orion Molecular Cloud Core. Neutral and Ionized Molecular Spectral Lines. Variation of Polarization With Wavelength. The Polarization Spectrum. Submillimeter Polarimetry - Looking Ahead. 3.Confusion. Confusion at 500, 600 micron. 4. Extragalactic Science. Do Massive Black Holes and Galaxy Bulges form Together? 5. Galactic Science. Can We See the First Generations of Stars and Metal Formation? The Birth of Planets and the Origins of Life. Spatial Resolution at 100 microns. Far-ir/Sub-mm Transitions of Linear Carbon Clusters. Predicted Spectra of Glycine.

Werner, Michael↗
NASA NTRS2024

Unveiling the Journey of A Highly Inclined CME: Insights from the March 13, 2012, Event With 110° Longitudinal Separation

Context. A fast (∼2000 km s -1 ) and wide (>110°) coronal mass ejection (CME) erupted from the Sun on March 13, 2012. Its interplanetary counterpart was detected in situ two days later by STEREO-A and near-Earth spacecraft, such as ACE, Wind, and Cluster. We suggest that at 1 au the CME extended at least 110° in longitude, with Earth crossing its east flank and STEREO-A crossing its- west flank. Despite their separation, measurements from both positions showed very similar in situ CME signatures. The solar source region where the CME erupted was surrounded by three coronal holes (CHs). Their locations with respect to the CME launch site were east (negative polarity), southwest (positive polarity) and west (positive polarity). The solar magnetic field polarity of the area covered by each CH matches that observed at 1 au in situ. Suprathermal electrons at each location showed mixed signatures with only some intervals presenting clear counter streaming flows as the CME transits both locations. The strahl population coming from the shortest magnetic connection of the structure to the Sun showed more intensity. Aims. The aim of this work is to understand the propagation and evolution of the CME and its interaction with the surrounding CHs, to explain the similarities and differences between the observations at each spacecraft, and report what one of the most longitudinal expanded CME structures measured in situ would be. Methods. Known properties of the large-scale structures from a variety of catalogues and previous studies were used to have a better overview of this particular event. In addition, multipoint observations were used to reconstruct the 3D geometry of the CME and determine the context of the solar and heliospheric conditions before the CME eruption and during its propagation. The graduated cylindrical shell model (GCS) was used to reproduce the orientation, size and speed of the structure with a simple geometry. Also, the Drag-Based Model (DBM) was utilised to understand the conditions of the interplanetary medium better in terms of the drag undergone by the structure while propagating in different directions. Finally, a comparative analysis of the different regions of the structure through the different observatories was carried out in order to directly compare the in situ plasma and magnetic field properties at each location. Results. The study presents important findings regarding the in situ measured CME on March 15, 2012, detected at a longitudinal separation of 110° in the ecliptic plane despite its initial inclination being around 45° when erupted (March 13). This suggests that the CME may have deformed and/or rotated, allowing it to be observed near its legs with spacecraft at a separation angle greater than 100°. The CME structure interacted with high-speed streams generated by the surrounding CHs. The piled-up plasma in the sheath region exhibited an unexpected correlation in magnetic field strength despite the large separation in longitude. In situ observations reveal that at both locations there was a flank encounter – where the spacecraft crossed the first part of the CME – then encountered ambient solar wind, and finally passed near the legs of the structure. Conclusions. A scenario covering all evidence is proposed for both locations with a general view of the whole structure and solar wind conditions. Also, the study shows the necessity of having multipoint observations of large-scale structures in the heliosphere.

methods: data analysis↗
NASA NTRS1976

The relation of metal composition to rock type for clasts in Apollo 16 soils

The moderately magnetic fractions of soils from a bright ray of South Ray Crater and from the continuous ejecta of North Ray Crater are described. The clasts in these fractions are classified as agglutinate, ANT melt rocks, glassy melt rocks, and ANT hornfels/breccia. Determinations are made of the Ni-Co and P contents of single-phase metal grains in the clasts. It is found that most of these grains have compositions in the meteoritic range and that the compositions tend to cluster at about 6% Ni. A significant amount of Fe-rich metal is also detected in some clasts along with a clear P-enrichment in metal from one soil sample. Meteoritic contamination of lunar metal having compositions in or close to the meteoritic range is considered. A model involving nine separate factors is proposed as an explanation of the observed metal compositions.

Hewins, R. H.↗
DOE OSTI2022

Atomic-Level Structure of Mesoporous Hexagonal Boron Nitride Determined by High-Resolution Solid-State Multinuclear Magnetic Resonance Spectroscopy and Density Functional Theory Calculations

Mesoporous hexagonal boron nitride (p-BN) has received significant attention over the last decade as a promising candidate for water cleaning/pollutant removal and hydrogen storage applications. In this work, high-resolution solid-state NMR spectroscopy and plane-wave density-functional theory (DFT) calculations are used to obtain an atomic-level description of p-BN. 1 H– 15 N or 1 H– 14 N heteronuclear (HETCOR) correlation experiments recorded with either conventional NMR at room temperature or dynamic nuclear polarization surface-enhanced spectroscopy (DNP-SENS) at ca. 100 K reveal NB 2 H, NBH 2 , NBH 3 + species residing on the edges of BN sheets. Ultra-high field 35.2 T 11 B NMR spectroscopy was used to resolve 11 B NMR signals from BN 3 , BN 2 O x (OH) 1–x (x = 0–1), BNO x (OH) 2–x (x = 0–2), BO x (OH) 3–x (x = 0–3), and BO x (OH) 4–x – (x = 0–4). Importantly, 2D 11 B dipolar double-quantum–single-quantum homonuclear correlation spectra reveal that many pore/defect sites are composed of boron oxide/hydroxide clusters connected to the BN framework through BN 2 O units. 1D and 2D 11 B{ 15 N} HETCOR NMR experiments, in addition to plane-wave DFT calculations of nine different structural models, further confirm the assignment of all NMR signals. The detailed structure determination of the pore and edge/defect sites within p-BN should further enable the rational design and development of next-generation p-BN-based materials. In addition, the techniques outlined here should be applicable to determine structure within other porous and/or boron-based materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1992

The Galactic center wind

The combined effect of winds from a cluster of stars in the central 0.8 pc of the Galaxy is modeled as uniform power and mass input over the central region. The flow becomes supersonic outside the central region, and the expected decrease in pressure is in approximate accord with observations. The pressure variations on a larger scale suggest that the Galactic center wind passes through a shock front at a radius of a few pc, leading to a shocked wind bubble on a scale of 100 pc. The tangential magnetic field can come to dominate the pressure in the shocked wind flow even if the energy density of the magnetic field in the initial wind is only 0.1 percent of the wind kinetic energy density. The magnetic region produced in this way may be related to some of the apparently magnetized structures observed in the central region of the Galaxy.

Chevalier, Roger A.↗
DOE OSTI2023

An in-silico NMR laboratory for nuclear magnetic shieldings computed via finite fields: Exploring nucleus-specific renormalizations of MP2 and MP3

Here we developed and implemented a method-independent, fully numerical, finite difference approach to calculating nuclear magnetic resonance shieldings, using gauge-including atomic orbitals. The resulting capability can be used to explore non-standard methods, given only the energy as a function of finite-applied magnetic fields and nuclear spins. For example, standard second-order Møller-Plesset theory (MP2) has well-known efficacy for 1H and 13C shieldings and known limitations for other nuclei such as 15N and 17O. It is, therefore, interesting to seek methods that offer good accuracy for 15N and 17O shieldings without greatly increased compute costs, as well as exploring whether such methods can further improve 1H and 13C shieldings. Using a small molecule test set of 28 species, we assessed two alternatives: κ regularized MP2 (κ-MP2), which provides energy-dependent damping of large amplitudes, and MP2.X, which includes a variable fraction, X, of third-order correlation (MP3). The aug-cc-pVTZ basis was used, and coupled cluster with singles and doubles and perturbative triples [CCSD(T)] results were taken as reference values. Our κ-MP2 results reveal significant improvements over MP2 for 13C and 15N, with the optimal κ value being element-specific. κ-MP2 with κ = 2 offers a 30% rms error reduction over MP2. For 15N, κ-MP2 with κ = 1.1 provides a 90% error reduction vs MP2 and a 60% error reduction vs CCSD. On the other hand, MP2.X with a scaling factor of 0.6 outperformed CCSD for all heavy nuclei. These results can be understood as providing renormalization of doubles amplitudes to partially account for neglected triple and higher substitutions and offer promising opportunities for future applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Exotic bonding interactions and coexistence of chemically distinct periodic lattice distortions in the charge density wave compound TaTe2

The superstructure of TaTe 2 is examined by total high-energy x-ray scattering and large-scale structure modeling over a broad temperature range. At room temperature, it features double zigzag chains of Ta atoms exhibiting metallic bonding. The chains are sandwiched between planes of weakly interacting Te atoms. Below 170 K, the chains appear broken to “butterflylike” clusters and single zigzag chains of covalently bonded Te atoms emerge while Ta-Te interactions remain largely ionic. This is a rare example of a charge density wave compound stabilized by bonding that is a mix of covalent, ionic, and metallic character giving rise to chemically distinct periodic lattice distortions. We argue that the formation of periodic lattice distortions in the Te sublattice in addition to those in the Ta sublattice favors charge delocalization, which may explain the unusually diminished resistivity and increased magnetic susceptibility exhibited by the low-temperature charge density wave phase of TaTe 2 . The effect may be common for 5d transition metal chalcogenides containing Te because of the extended electronic orbitals of the constituent atoms.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1990

Spectra, composition, and interactions of nuclei with magnet interaction chambers

Emulsion chambers will be flown in the Astromag Facility to measure the cosmic ray composition and spectra to 10 exp 15 eV total energy and to definitively study the characteristics of nucleus-nucleus interactions above 10 exp 12 eV/n. Two configurations of emulsion chambers will be flown in the SCIN/MAGIC experiment. One chamber has an emulsion target and a calorimeter similar to those recently flown on balloons for composition and spectra measurements. The other has an identical calorimeter and a low-density target section optimized for performing rigidity measurements on charged particles produced in interactions. The transverse momenta of charged and neutral mesons, direct hadronic pairs from resonance decays and interference effects, and possible charge clustering in high-density states of matter will be studied.

Parneil, T. A.↗
NASA NTRS2020

Chandra and XMM-Newton Observations of A2256: Cold Fronts, Merger Shocks, and Constraint on the IC Emission

We present the results of deep Chandra and XMM-Newton observations of a complex merging galaxy cluster Abell 2256 (A2256) that hosts a spectacular radio relic (RR).The temperature and metallicity maps show clear evidence of a merger between the western subcluster (SC) and the primary cluster (PC). We detect five X-ray surface brightness edges. Three of them near the cluster center are cold fronts (CFs): CF1is associated with the infalling SC; CF2 is located in the east of the PC; and CF3 is to the west of the PC core. The other two edges at cluster outskirts are shock fronts(SFs): SF1 near the RR in the NW has Mach numbers derived from the temperature and the density jumps, respectively, of MT=1.62±0.12andMρ=1.23±0.06; SF2 in the SE has MT=1.54±0.05andMρ=1.16±0.13. In the region of the RR, there is no evidence for the correlation between X-ray and radio substructures, from which we estimate an upper limit for the inverse-Compton emission, and therefore set a lower limit on the magnetic field (∼450 kpc from PC center) of B>1.0μG for a single power-law electron spectrum or B>0.4μG for a broken power-law electron spectrum. We propose a merger scenario including a PC, an SC, and a group. Our merger scenario accounts for the X-ray edges, diffuse radio features, and galaxy kinematics, as well as projection effects.

Chong Ge↗
DOE OSTI2020

Preface

Crystallization via nonclassical pathways is important during the formation of minerals in nature and has become a popular method to synthesize advanced materials on both laboratory and industrial scales. Unlike classical crystal growth pathways via monomer-by-monomer addition, crystallization via nonclassical pathways such as particle-by-particle attachment can form bigger crystals more quickly. Many materials prepared via non-classical crystallization have been applied in various fields such as energy, catalysis, environment, biomedicine, optics, electrics, and magnetics. Understanding nonclassical crystallization pathways could provide new insights on design and synthesize novel materials. This ACS Book series aims to provide updated information on fundamental nonclassical crystallization research, including theory and experiments. It’s also designed for experienced researchers to reinforce their knowledge on the scopes of development of new techniques, especially state-of-the-art in situ characterization tools, to understand mechanisms of crystallization via nonclassical pathways. Topics that would be covered in this book series include: (1) nonclassical nucleation; (2) cluster assembly; (3) particlebased crystallization; (4) crystal formation from amorphous intermedium phases; (5) biomineralization via nonclassical pathways; (6) theoretical developments to simulate nonclassical crystallization; (7) observation of the nonclassical crystallization pathways via various characterization techniques; and (8) the application of nonclassical crystallization. Volume I of the Nonclassical Crystallization Book Series will cover a broad range of topics about nucleation, assembly, observation, and applications of nonclassical crystallization.

Zhang, Xin↗
DOE OSTI2022

Colossal piezoresistance in narrow-gap Eu 5 In 2 Sb 6

Piezoresistance, the change of the electrical resistance (R) of a material in response to an applied mechanical stress (σ), is the driving principle of electromechanical devices such as strain gauges, accelerometers, and cantilever force sensors. Enhanced piezoresistance has been traditionally observed in two classes of uncorrelated materials: nonmagnetic semiconductors and composite structures. In this study, we report the discovery of a remarkably large piezoresistance in Eu 5 In 2 Sb 6 single crystals, wherein anisotropic metallic clusters naturally form within a semiconducting matrix due to electronic interactions. Eu 5 In 2 Sb 6 shows a highly anisotropic piezoresistance, and uniaxial pressure along [001] of only 0.4 GPa leads to a resistivity drop of >99.95%, which results in a colossal piezoresistance factor of 5000×10 –11 Pa –1 . Our result not only reveals the role of interactions and phase separation in the realization of colossal piezoresistance, but it also highlights a route to multifunctional devices with large responses to both pressure and magnetic field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2003

Studies of Atomic Free Radicals Stored in a Cryogenic Environment

Impurity-Helium Solids are porous gel-like solids consisting of impurity atoms and molecules surrounded by thin layers of solid helium. They provide an ideal medium for matrix isolation of free radicals to prevent recombination and store chemical energy. In this work electron spin resonance, nuclear magnetic resonance, X-ray diffraction, and ultrasound techniques have all been employed to study the properties of these substances. Detailed studies via electron spin resonance of exchange tunneling chemical reactions involving hydrogen and deuterium molecular and atomic impurities in these solids have been performed and compared with theory. Concentrations of hydrogen approaching the quantum solid criterion have been produced. Structured studies involving X ray diffraction, ultrasound, and electron spin resonance have shown that the impurities in impurity helium solids are predominantly contained in impurity clusters, with each cluster being surrounded by thin layers of solid helium.

Lee, David M.↗
DOE OSTI2021

Hierarchical excitations from correlated spin tetrahedra on the breathing pyrochlore lattice

The hierarchy of the coupling strengths in a physical system often engenders an effective model at low energies where the decoupled high-energy modes are integrated out. Here, using neutron scattering, we show that the spin excitations in the breathing pyrochlore lattice compound CuInCr 4 S 8 are hierarchical and can be approximated by an effective model of correlated tetrahedra at low energies. At higher energies, intratetrahedron excitations together with strong magnon-phonon couplings are observed, which suggests the possible role of the lattice degree of freedom in stabilizing the spin tetrahedra. Finally, our work illustrates the spin dynamics in CuInCr 4 S 8 and demonstrates a general effective-cluster approach to understand the dynamics on the breathing-type lattices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2026

Temporal and spatial separations between spin glass and short-range order

Broken-symmetry-induced order parameters account for many phenomena in physics. For spin glasses, this framework dictates the theoretical construction, whereas experiments have only established dynamical behaviors but not the physical entity. Experimental techniques have limitations when the spin glass is probed as an isolated state. Here, we create an evolution from a long-range order using well-controlled non-magnetic substitution on a sublattice. Neutron magnetic diffuse scattering of pico-second timescale reveals that the dynamics of short- and long-range order formation are not affected by disorder, but their spatial ranges are. Across all specimens, the inflection point of spin correlation length’s temperature dependence fully matches with the peak in heat capacity, while spin glass can freeze at millisecond timescale either above or below this characteristic temperature of spin-order formation. Our results identify the spin glass as single, uncorrelated spins at domain walls between spin clusters, and an uncorrelated coexistence of the two.

Dronova, Margarita G [Okinawa Institute of Science↗
NASA NTRS2020

Chandra and XMM-Newton Observations of A2256: Cold Fronts, Merger Shocks, and Constraint on the IC Emission

We present the results of deep Chandra and XMM-Newton observations of a complex merging galaxy cluster Abell 2256 (A2256) that hosts a spectacular radio relic (RR). The temperature and metallicity maps show clear evidence of a merger between the western subcluster (SC) and the primary cluster (PC). We detect five X-ray surface brightness edges. Three of them near the cluster center are cold fronts (CFs): CF1 is associated with the infalling SC; CF2 is located in the east of the PC; and CF3 is to the west of the PC core. The other two edges at cluster outskirts are shock fronts(SFs): SF1 near the RR in the NW has Mach numbers derived from the temperature and the density jumps, respectively, of MT=1.62±0.12 and Mρ=1.23±0.06; SF2 in the SE has MT=1.54±0.05 and Mρ=1.16±0.13. In the region of the RR, there is no evidence for the correlation between X-ray and radio substructures, from which we estimate an upper limit for the inverse-Compton emission, and therefore set a lower limit on the magnetic field (∼450 kpc from PC center) of B>1.0μG for a single power-law electron spectrum or B>0.4μG for a broken power-law electron spectrum. We propose a merger scenario including a PC, an SC, and a group. Our merger scenario accounts for the X-ray edges, diffuse radio features, and galaxy kinematics, as well as projection effects.

Chong Ge↗
DOE OSTI2026

Investigation of the isoscalar monopole response in the proton-rich nucleus 14 O

Deuteron inelastic scattering on 14 O was measured in inverse kinematics using an active-target time projection chamber and a magnetic spectrograph. The experimental technique enabled precise measurements of deuteron recoiling particles in coincidence with beam-like fragments detected in the spectrograph focal plane. The double differential cross section was reconstructed for scattering angles of 3–6 degrees and excitation energies up to 26 MeV. The monopole strength distribution was obtained from the data using a multipole decomposition analysis. The results were compared to quasiparticle random-phase approximation (QRPA) and generator coordinate method (GCM) calculations. The QRPA calculation accurately describes experimental data in the energy range of 13 to 26 MeV. GCM calculations assuming a 12 C (g . s .) + p + p cluster configuration were used to determine the 0 + strength in 14 O below 13 MeV. The monopole transition strength of these cluster states provides a good description of the experimental distribution in the 9–11 MeV region, while the 0$^{+}_{2}$ state accounts for only a small fraction of the experimental strength around 6 MeV.

Active target↗
NASA NTRS1983

Radio and X-ray observations of the radio halo source in A1367

Radio and X-ray observations of the 'radio halo' in A1367 are presented. The radio spectral index distribution is derived combining data at 610 and 1415 MHz taken with the Westerbork Synthesis Radio Telescope (WSRT). A high-resolution Very Large Array (VLA) map allows us to discriminate between the extended cluster emission and a triple radio source associated with a background stellar object (most probably a QSO) which appears projected onto it. X-ray observations taken with the high-resolution imager on board the Einstein satellite reveal an X-ray source associated with this background object. A second weak X-ray enhancement is found projected onto the extended radio component. Inverse Compton scattering of the synchrotron-emitting particles provides a possible interpretation of such a source. The presence of large-scale magnetic fields and particle acceleration due to the turbulent motion of galaxies through the intergalactic medium is discussed in relationship to the observed peculiarities of the galaxies found in this region.

Gavazzi, G.↗