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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Spinon Confinement and a Sharp Longitudinal Mode in Yb 2 Pt 2 Pb in Magnetic Field

Here, the fundamental excitations in an antiferromagnetic chain of spins-1/2 are spinons, de-confined fractional quasiparticles that when combined in pairs, form a triplet excitation continuum. In an Ising-like spin chain the continuum is gapped and the ground state is Neel ordered. Here, we report high resolution neutron scattering experiments, which reveal how a magnetic field closes this gap and drives the spin chains in Yb 2 Pt 2 Pb to a critical, disordered Luttinger-liquid state. In Yb 2 Pt 2 Pb the effective spins-1/2 describe the dynamics of large, Ising-like Yb magnetic moments, ensuring that the measured excitations are exclusively longitudinal, which we find to be well described by time-dependent density matrix renormalization group calculations. The inter-chain coupling leads to the confinement of spinons, a condensed matter analog of quark confinement in quantum chromodynamics. Insensitive to transverse fluctuations, our measurements show how a gapless, dispersive longitudinal mode arises from confinement and evolves with magnetic order.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Oriented nanometric aggregates of partially inverted zinc ferrite: One-step processing and tunable high-frequency magnetic properties

In this work, it is demonstrated that the in situ growth of oriented nanometric aggregates of partially inverted zinc ferrite can potentially pave a way to alter and tune magnetocrystalline anisotropy that, in turn, dictates ferromagnetic resonance frequency (f{sub FMR}) by inducing strain due to aggregation. Furthermore, the influence of interparticle interaction on magnetic properties of the aggregates is investigated. Mono-dispersed zinc ferrite nanoparticles (<5 nm) with various degrees of aggregation were prepared through decomposition of metal-organic compounds of zinc (II) and iron (III) in an alcoholic solution under controlled microwave irradiation, below 200 °C. The nanocrystallites were found to possess high degree of inversion (>0.5). With increasing order of aggregation in the samples, saturation magnetization (at 5 K) is found to decrease from 38 emu/g to 24 emu/g, while coercivity is found to increase gradually by up to 100% (525 Oe to 1040 Oe). Anisotropy-mediated shift of f{sub FMR} has also been measured and discussed. In essence, the result exhibits an easy way to control the magnetic characteristics of nanocrystalline zinc ferrite, boosted with significant degree of inversion, at GHz frequencies.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

In-plane angular dependence of the spin-wave nonreciprocity of an ultrathin film with Dzyaloshinskii-Moriya interaction

The nonreciprocal propagation of spin waves in an ultrathin Pt/Co/Ni film has been measured by Brillouin light scattering. The frequency nonreciprocity, due to the interfacial Dzyaloshinskii-Moriya interaction (DMI), has a sinusoidal dependence on the in-plane angle between the magnon wavevector and the applied magnetic field. The results, which are in good agreement with analytical predictions reported earlier, yield a value of the DMI constant which is the same as that obtained previously from a study of the magnon dispersion relations. We have demonstrated that our magnon-dynamics based method can experimentally ascertain the DMI constant of multilayer thin films.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1988

Conditions for the validity of unmagnetized-plasma theory in describing weakly magnetized plasmas

The application of the unmagnetized-plasma theory to the derivation of the expression for the dielectric tensor for weakly magnetized plasmas is examined. The analysis of Baldwin et. al. (1969) is employed to determine the conditions under which the magnetic effects on the dielectric tensor of a plasma are small. The relation between wave and plasma parameters and the plasma distribution function is studied. Axisymmetric distribution functions in magnetized plasma are considered. The derived conditions are analyzed in terms of resonance ellipses of the cyclotron maser theory. Examples are presented in which the conditions are applied to a nonrelativistic Maxwellian distribution and the dispersion and instability of Langmuir and Bernstein waves in weakly magnetized plasma. The data reveal that the conditions under which the magnetic field can be completely neglected depend on the forms of the distribution function.

Robinson, P. A.↗
DOE OSTI2022

Simultaneous measurement of the exchange parameter and saturation magnetization using propagating spin waves

The exchange interaction in ferromagnetic ultra thin films is a critical parameter in magnetization-based storage and logic devices, yet the accurate measurement of it remains a challenge. While a variety of approaches are currently used to determine the exchange parameter, each has its limitations, and good agreement among them has not been achieved. To date, neutron scattering, magnetometry, Brillouin light scattering, spin-torque ferromagnetic resonance spectroscopy, and Kerr microscopy have all been used to determine the exchange parameter. Here, we present a method that exploits the wavevector selectivity of Brillouin light scattering to measure the spin wave dispersion in both the backward volume and Damon–Eshbach orientations. The exchange, saturation magnetization, and magnetic thickness are then determined by a simultaneous fit of both dispersion branches with general spin wave theory without any prior knowledge of the thickness of a magnetic “dead layer.” In this study, we demonstrate the strength of this technique for ultrathin metallic films, typical of those commonly used in industrial applications for magnetic random-access memory.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

ABINIT: Overview and focus on selected capabilities

ABINIT is probably the first electronic-structure package to have been released under an open-source license about 20 years ago. It implements density functional theory, density-functional perturbation theory (DFPT), many-body perturbation theory (GW approximation and Bethe–Salpeter equation), and more specific or advanced formalisms, such as dynamical mean-field theory (DMFT) and the “temperature-dependent effective potential” approach for anharmonic effects. Relying on planewaves for the representation of wavefunctions, density, and other space-dependent quantities, with pseudopotentials or projector-augmented waves (PAWs), it is well suited for the study of periodic materials, although nanostructures and molecules can be treated with the supercell technique. The present article starts with a brief description of the project, a summary of the theories upon which ABINIT relies, and a list of the associated capabilities. It then focuses on selected capabilities that might not be present in the majority of electronic structure packages either among planewave codes or, in general, treatment of strongly correlated materials using DMFT; materials under finite electric fields; properties at nuclei (electric field gradient, Mössbauer shifts, and orbital magnetization); positron annihilation; Raman intensities and electro-optic effect; and DFPT calculations of response to strain perturbation (elastic constants and piezoelectricity), spatial dispersion (flexoelectricity), electronic mobility, temperature dependence of the gap, and spin-magnetic-field perturbation. The ABINIT DFPT implementation is very general, including systems with van der Waals interaction or with noncollinear magnetism. Community projects are also described: generation of pseudopotential and PAW datasets, high-throughput calculations (databases of phonon band structure, second-harmonic generation, and GW computations of bandgaps), and the library libpaw. ABINIT has strong links with many other software projects that are briefly mentioned.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

Calculations of structural, elastic, electronic, magnetic and phonon properties of FeNiMnAl by the first principles

The electronic, elastic and dynamical properties of the quaternary alloy FeNiMnAl have been investigated using a pseudopotential plane wave method within the generalized gradient approximation (GGA). We determined the lattice parameters and the bulk modulus B. In addition, the elastic properties such as elastic constans (C{sub 11}, C{sub 12} and C{sub 44}), the shear modulus G, the young modulus E, the poisson's ratio σ and the B/G ratio are also given. The FeNiMnAl Heusler alloy exhibit a ferromagnetic half-metallic behavior with the total magnetic moment of 4.02 μ{sub B}. The phonon dispersion of FeNiMnAl has been performed using the density functional theory and the direct method with 2×2×2 supercell.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2013

SOLAR MAGNETIC TRACKING. IV. THE DEATH OF MAGNETIC FEATURES

The removal of magnetic flux from the quiet-Sun photosphere is important for maintaining the statistical steady state of the magnetic field there, for determining the magnetic flux budget of the Sun, and for estimating the rate of energy injected into the upper solar atmosphere. Magnetic feature death is a measurable proxy for the removal of detectable flux, either by cancellation (submerging or rising loops, or reconnection in the photosphere) or by dispersal of flux. We used the SWAMIS feature tracking code to understand how nearly 2 Multiplication-Sign 10{sup 4} magnetic features die in an hour-long sequence of Hinode/SOT/NFI magnetograms of a region of the quiet Sun. Of the feature deaths that remove visible magnetic flux from the photosphere, the vast majority do so by a process that merely disperses the previously detected flux so that it is too small and too weak to be detected, rather than completely eliminating it. The behavior of the ensemble average of these dispersals is not consistent with a model of simple planar diffusion, suggesting that the dispersal is constrained by the evolving photospheric velocity field. We introduce the concept of the partial lifetime of magnetic features, and show that the partial lifetime due to Cancellation of magnetic flux, 22 hr, is three times slower than previous measurements of the flux turnover time. This indicates that prior feature-based estimates of the flux replacement time may be too short, in contrast with the tendency for this quantity to decrease as resolution and instrumentation have improved. This suggests that dispersal of flux to smaller scales is more important for the replacement of magnetic fields in the quiet Sun than observed bipolar cancellation. We conclude that processes on spatial scales smaller than those visible to Hinode dominate the processes of flux emergence and cancellation, and therefore also the quantity of magnetic flux that threads the photosphere.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Protected fermionic zero modes in periodic gauge fields

It is well known that macroscopically normalizable zero-energy wave functions of spin-$\frac{1}{2}$ particles in a two-dimensional inhomogeneous magnetic field are spin-polarized and exactly calculable with degeneracy equaling the number of flux quanta linking the whole system. Here, extending this argument to massless Dirac fermions subjected to magnetic fields that have zero net flux but are doubly periodic in real space, we show that there exist only two Bloch-normalizable zero-energy eigenstates, one for each spin flavor. This result is immediately relevant to graphene multilayer systems subjected to doubly periodic strain fields, which at low energies enter the Hamiltonian as periodic pseudogauge vector potentials. Furthermore, we explore various related settings including nonlinearly dispersing band structure models and systems with singly periodic magnetic fields.

36 MATERIALS SCIENCE↗
DOE OSTI2016

MAGNETIC FIELD OF THE VELA C MOLECULAR CLOUD

We have performed extensive near-infrared ( JHK {sub s}) imaging polarimetry toward the Vela C molecular cloud, which covers the five high-density sub-regions (North, Centre-Ridge, Centre-Nest, South-Ridge, and South-Nest) with distinct morphological characteristics. The obtained polarization vector map shows that three of these sub-regions have distinct plane-of-the-sky (POS) magnetic-field characteristics according to the morphological characteristics. (1) In the Centre-Ridge sub-region, a dominating ridge, the POS magnetic field is mostly perpendicular to the ridge. (2) In the Centre-Nest sub-region, a structure having a slightly extended nest of filaments, the POS magnetic field is nearly parallel to its global elongation. (3) In the South-Nest sub-region, which has a network of small filaments, the POS magnetic field appears to be chaotic. By applying the Chandrasekhar–Fermi method, we derived the POS magnetic field strength as ∼70–310 μ G in the Centre-Ridge, Centre-Nest, and South-Ridge sub-regions. In the South-Nest sub-region, the dispersion of polarization angles is too large to apply the C-F method. Because the velocity dispersion in this sub-region is not greater than those in the other sub-regions, we suggest that the magnetic field in this sub-region is weaker than those in other sub-regions. We also discuss the relationship between the POS magnetic field (configuration and strength) and the cloud structure of each sub-region.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Finite temperature properties of uranium mononitride

Uranium mononitride (UN) is a promising nuclear fuel that combines the advantageous properties of readily used UO 2 and uranium alloys, such as high melting temperature and high uranium density, and thermal conductivity, respectively. A better understanding of UN behavior at operating temperatures can be obtained from finite temperature data, such as elastic properties. To get this information, ab initio molecular dynamics (AIMD) simulations were performed at five different temperatures using constant volume (NVT) and constant pressure (NPT) ensembles. Initially, the performance of PBE functional in reproducing experimental crystallographic properties and magnetic ordering is assessed. The finite temperature phonon dispersions are calculated using NVT simulation results, which show a softening of the phonon modes with increasing temperature. The NPT results are used to obtain the thermal expansion of UN and finite temperature electronic properties. The calculated thermal expansion is compared with our measurements using neutron diffraction. Additionally, the temperature dependent elastic properties of UN are evaluated using the strain-stress method in AIMD simulations, indicating that UN becomes softer and more compressible with increasing temperature. Also, the calculated Young’s modulus slope is in very good agreement with the experiment. The finite temperature heat capacity and electronic thermal conductivity are calculated from AIMD simulations, which are in better agreement with the experiment than the heat capacity and thermal conductivity calculated using the structures relaxed at 0K. Finally, the thermal diffusivity from AIMD has opposite temperature dependence compared to experimental results, which we argued comes from the underestimated electronic thermal conductivity.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2020

Stability of a tokamak plasma with diffuse toroidal rotation

The present work considers the stability of a high- $\beta$ , large aspect ratio, circular plasma with diffuse profiles for the safety factor and the angular toroidal frequency (López & Guazzotto, Phys. Plasmas , vol. 24, 032501). An application of the Frieman–Rotenberg formalism results in a system of scalar eigenmode equations whose coupling is retained at the plasma–vacuum transition but is disregarded across the plasma column, which is a standard practice. The solution technique consists of a multidimensional shooting method for the poloidal harmonics; robust initial guesses are constructed by solving the dispersion relation in the static scenario with vanishing magnetic shear. Flow shear appears as a high- $\beta$ toroidal contribution, and we illustrate its destabilizing influence on $n=1$ external kink modes in the presence of ideal and resistive walls. Internal resonances are avoided by means of the selection of appropriate equilibrium parameters. The stabilizing influence of a finite positive average magnetic shear is also exemplified.

Physics↗
DOE OSTI2023

Signatures of fractional quantum anomalous Hall states in twisted MoTe 2

The interplay between spontaneous symmetry breaking and topology can result in exotic quantum states of matter. A celebrated example is the quantum anomalous Hall (QAH) state, which exhibits an integer quantum Hall effect at zero magnetic field owing to intrinsic ferromagnetism. In the presence of strong electron–electron interactions, fractional QAH (FQAH) states at zero magnetic field can emerge. These states could host fractional excitations, including non-Abelian anyons—crucial building blocks for topological quantum computation9. Here we report experimental signatures of FQAH states in a twisted molybdenum ditelluride (MoTe 2 ) bilayer. Magnetic circular dichroism measurements reveal robust ferromagnetic states at fractionally hole-filled moiré minibands. Using trion photoluminescence as a sensor, we obtain a Landau fan diagram showing linear shifts in carrier densities corresponding to filling factor v = −2/3 and v = −3/5 ferromagnetic states with applied magnetic field. These shifts match the Streda formula dispersion of FQAH states with fractionally quantized Hall conductance of ${\sigma }_{xy}=-\,\frac{2}{3}\frac{{e}^{2}}{h}$ and ${\sigma }_{xy}=-\,\frac{3}{5}\frac{{e}^{2}}{h}$ , respectively. Moreover, the v = −1 state exhibits a dispersion corresponding to Chern number −1, consistent with the predicted QAH state. In comparison, several non-ferromagnetic states on the electron-doping side do not disperse, that is, they are trivial correlated insulators. The observed topological states can be electrically driven into topologically trivial states. Our findings provide evidence of the long-sought FQAH states, demonstrating MoTe 2 moiré superlattices as a platform for exploring fractional excitations.

Quantum Hall↗
DOE OSTI2016

Magnetic moment collapse induced axial alternative compressibility of Cr 2 TiAlC 2 at 420 GPa from first principle

The electronic structure and thermo-dynamical properties of Cr 2 TiAlC 2 are studied by first principles under pressure. The obtained results observed that the ferromagnetic order is the most stable ground state and the magnetic moment will collapse at about 50GPa. As a result, the lattice a axis becomes stiffer above about 420GPa, ultimately presenting the same axial compressibility trends with those of nonmagnetic compounds Mo2TiAlC2 and hypothetical Cr2TiAlC2. The elastic constants and phonon dispersion curves demonstrate the structural stability during the disappearance of magnetic moment and occurrence of axial alternative compressibility. The density of states and energy band calculations confirmed the existence of magnetic moment of Cr2TiAlC2 at 0GPa and disappearance at high pressures above 50GPa. Evolutions of magnetic moment collapse with pressure are confirmed by a variety of properties. The obtained grüneisen parameter and thermal expansion coefficients show the maximum value among the known MAX phases, to date and to the author’s knowledge.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2011

Particle acceleration by circularly and elliptically polarised dispersive Alfven waves in a transversely inhomogeneous plasma in the inertial and kinetic regimes

Dispersive Alfven waves (DAWs) offer, an alternative to magnetic reconnection, opportunity to accelerate solar flare particles in order to alleviate the problem of delivering flare energy to denser parts of the solar atmosphere to match x-ray observations. Here, we focus on the effect of DAW polarisation, left, right, circular and elliptical, in the different regimes inertial and kinetic, aiming to study these effects on the efficiency of particle acceleration. We use 2.5D particle-in-cell simulations to study how the particles are accelerated when DAW, triggered by a solar flare, propagates in the transversely inhomogeneous plasma that mimics solar coronal loop. (1) In the inertial regime, fraction of accelerated electrons (along the magnetic field) in the density gradient regions is {approx_equal}20% by the time when DAW develops three wavelengths and is increasing to {approx_equal}30% by the time when DAW develops thirteen wavelengths. In all considered cases, ions are heated in the transverse to the magnetic field direction and fraction of heated particles is {approx_equal}35%. (2) The case of right circular, left and right elliptical polarisation DAWs, with the electric field in the non-ignorable transverse direction exceeding several times that of in the ignorable direction, produce more pronounced parallel electron beams (with larger maximal electron velocities) and transverse ion beams in the ignorable direction. In the inertial regime, such polarisations yield the fraction of accelerated electrons 20%. In the kinetic regime, this increases to 35%. (3) The parallel electric field that is generated in the density inhomogeneity regions is independent of the electron-ion mass ratio and stays of the order 0.03 {omega}{sub pe}cm{sub e}/e which for solar flaring plasma parameters exceeds Dreicer electric field by eight orders of magnitude. (4) Electron beam velocity has the phase velocity of the DAW. Thus, electron acceleration is via Landau damping of DAWs. For the Alfven speeds of V{sub A} = 0.3c, the considered mechanism can accelerate electrons to energies circa 20 keV. (5) The increase of mass ratio from m{sub i}/m{sub e} = 16 to 73.44 increases fraction of accelerated electrons from 20% to 30-35% (depending on DAW polarisation). For the mass ratio m{sub i}/m{sub e} = 1836, the fraction of accelerated electrons would be >35%. (6) DAWs generate significant density and temperature perturbations that are located in the density gradient regions. DAWs propagating in the transversely inhomogeneous plasma can effectively accelerate electrons along the magnetic field and heat ions across it.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Maximal Cherenkov γ-radiation on Fermi-surface of compact stars

The quantum magnetohydrodynamic model is employed in this paper to study the extraordinary (XO) elliptically polarized electromagnetic wave dispersion in quantum plasmas with spin-1/2 magnetization and relativistic degeneracy effects, considering also the electron-exchange and quantum diffraction of electrons. From the lower and upper calculated XO-modes, it is observed that, for electrons on the surface of the Fermi-sphere, the lower XO-mode can excite the Cherenkov radiation by crossing the Fermi-line, with some proper conditions depending on the values of independent plasma parameters, such as the relativistic-degeneracy, the atomic-number of constituent ions, and the magnetic field strength. Particularly, a lower electron number-density and Cherenkov radiation frequency limits are found to exist, for instance, for given values of the plasma ions atomic-number and the magnetic field strength below which the radiation can not be excited by the electrons on the Fermi-surface. This lower density limit increases by decrease in the atomic-number but decreases with decrease in the strength of the ambient magnetic field. It is remarkable that in this research it is discovered that the maximal Cherenkov-radiation per unit-length (the energy radiated by superluminal electrons traveling through the dielectric medium) coincides with the plasma number-densities, which is present in compact stars with the maximal radiation frequency lying in the gamma-ray spectrum. Current study can provide an important plasma diagnostic tool for a wide plasma density range, be it the solid density, the warm dense matter, the inertial confined or the astrophysical compact plasmas and may reveal an important cooling mechanism for white dwarfs. Current findings may also answer the fundamental astrophysical question on the mysterious origin of intense cosmic gamma-ray emissions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

Excitation of the three principal spin waves in yttrium iron garnet using a wavelength-specific multi-element antenna

We report systematic measurements of the dispersion of long wavelength spin waves for the magnetic field along the three principal directions (supporting the forward volume, backward volume and Damon-Eshbach modes) of a 3.05 um thick yttrium iron garnet film on a lattice-matched (111) gadolinium gallium garnet substrate obtained using a lithographically patterned, multi-element, 50 um spatially-resonant, antenna.

36 MATERIALS SCIENCE↗
DOE OSTI2013

EXCITATION OF KINETIC ALFVEN WAVES BY DENSITY STRIATION IN MAGNETO-PLASMAS

Field-aligned density striation is one of the most common inhomogeneity phenomena in magneto-plasmas, such as in the solar coronal plasma and terrestrial auroral plasma. Kinetic Alfven waves (KAWs) can play an important role in the inhomogeneous heating of coronal magneto-plasmas as well as in the local acceleration of auroral energetic electrons. In this paper, we study the dispersion and instability of KAWs in a magneto-plasma with density striation structures. Results show that KAWs become unstable in the presence of the density striation and the corresponding instability has a maximal growth rate at the perpendicular wavelength close to the spatial scale of the density gradient. Related experimental phenomena in both laboratory and space plasmas are discussed. It is suggested that the excitation of KAWs by the density striation of magneto-plasmas can be of potential importance in understanding the physics of the formation of magneto-plasma filaments and their heating mechanisms, which are often present in the terrestrial auroral plasma, the solar coronal plasma, and other astrophysical plasmas.

79 ASTRONOMY AND ASTROPHYSICS↗