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At least 595 records · Page 33

Evaluation of the Los Alamos Nuclear Material Packaging Risk Ranking Method

Repackaging nuclear material into robust containers to protect workers and the public has been ongoing at LANL and around the DOE complex for nearly two decades. The number of containers at LANL is around 5,000; limited resources for repackaging material has led to extended repackaging campaigns and the need to prioritize repackaging. Various methodologies have been used to prioritize the repackaging efforts and to demonstrate progress in risk reduction over time (e.g., Boerigter, 1997). The 2000-1 DNFSB recommendation recognized the limited DOE resources for repackaging, and acknowledged the need to “prioritize and schedule tasks to be undertaken with available funds according to consideration of risks.” Later, in DNFSB recommendation 2005-1, in addition to recommending that DOE develop a packaging standard, the Board recommended that “Characterization information should also be used to develop a surveillance program prioritized according to expected material and container risk (including, for example, material type, material form, and the age and type of container).” In response to requests and recommendations from the DOE and DNSFB to prioritize according to worker risk, a risk ranking method based on the potential consequence of dropping a container from 3 meters was developed in 2007 (Smith, 2007) and updated in 2014 (Hoffman, 2014). Various LANL implementation plans for repackaging were developed over the years using this methodology (Stone, 2014). Currently, this method is utilized in conjunction with an algorithm to mitigate programmatic risk to prioritize container repackaging and material processing (Prochnow, 2015). The purpose of this study is to document how the current risk ranking method works, how it is used and potential limitations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

National Security Research Center

Born out of a need to make LANL Weapons Program archival material available to scientists and engineers. Material is the result of decades of consolidation of mini-libraries and mini archives at LANL. Latest consolidation brought together LANL’s digital archives and physical archives. Houses 75+ years of nuclear weapons research, designs, procedures, videos, photos, and other reports.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

National Security Research Center

Born from the need to make LANL Weapons Program archival material available to scientists and engineers. Material is the end result of decades of consolidation of mini libraries and mini archives at LANL. Latest consolidation brought together LANL’s digital archives and physical archives. Houses 75+ years of nuclear weapons research, designs, procedures, videos, photos, and other report.

99 GENERAL AND MISCELLANEOUS↗

Community Conversation [Slides]

Our employees are the reason we kept up so much vital work during the pandemic. LANL is responsible for important R&D work for the nation and our scope is growing. COVID has taught us there are many ways to leverage technology to work effectively. Our researchers are making important contributions to nuclear security, climate change, environmental remediation, and fuel cell technology. LANL played a key leadership role in the pandemic by identifying mutations, predicting spread, and providing decision support. LANL has exciting news and changes on the horizon.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

Tensile Property and Lifetime Prediction for Low-Temperature Aged Uranium-Niobium Alloys

Thermal aging models and lifetime predictions for uranium-niobium (U-Nb) alloys were created using an approach similar to those previously employed. Lifetime estimates for generic U-6Nb components were thus updated; the reported value being 800 years. This update represents a small change in lifetime vs. that of the 2012 assessment (540 years). This lifetime estimate emerged from consideration of several model fits specific to the aging datasets and properties chosen. Aging was quantified using quasi-static tensile properties measured on specimens artificially aged for up to 10 years. The major change relative to the most recent 2012 LANL assessment was that a more comprehensive body of U-Nb literature data was mined, in addition to being augmented by the latest LANL and UK AWE data. The tensile data compilation was published separately (LANL report LA-14493, December 2016). Recognizing the chemical banding of industrially produced U-6Nb, models were developed for the mid-range (6 wt.%) and extrema (4 and 8 wt.%) compositions. Lifetime estimates were calculated for all three alloy classes (4, 6, 8 wt.% nominal) and two measures of total tensile elongation (TE) to failure, namely TE-ext. — extensometer method, and TE-NCD — normalized crosshead displacement method. The conservative assumption was made that whichever composition (4, 6, or 8 wt.% Nb) and property (TE-ext or TE-NCD) was the first to cross the ductility failure threshold would limit the lifetime of the entire component. Tensile strength properties did not figure into the lifetime predictions, but could be useful as age-sensitive diagnostics and were also modeled. Of these, only first yield strength is expected to show a change at 40°C aging vs. time = 0 over the ~100-year timespan of engineering interest. Second yield strength evolves more slowly, and ultimate tensile strength slower still. Among all the models, the apparent activation energies for aging were mostly in the narrow 29– 37 kcal/mol range, which is close to that for diffusion of Nb in gamma-uranium. This agreement may be coincidental. The data from recent long-term aging studies substantially improved the model fit quality and robustness of the lifetimes. Appendices document sensitivity studies of the model fits and lifetimes with respect to using more limited datasets. These results highlight the limitations of relying solely on data from scattered literature studies and smaller datasets more generally.

36 MATERIALS SCIENCE↗

Accelerate M-TIP on GPUs and deploy to Summit and NERSC-9 (against simulated data) WBS 2.2.4.05 ExaFEL, Milestone ADSE13-199

We evaluated the orientation matching step in the M-TIP SPI workflow for potential offloading to accelerators. We ported the code to GPUs, benchmarked it, optimized and down-selected the best versions. The accelerated version of the orientation matching code that was developed at LANL (LANL GPU v3) is 34-55X faster than sequential, 2.4-4.9X faster than the fastest OpenMP open source version we found (FAISS OpenMP) and 1.5-4X faster than the fastest GPU open source version we found (FAISS GPU). Summit single-node GPU versions were somewhat faster than Cori GPU. Image size plays a role; mid-range image sizes take more time. The LANL CUDA multi-node, multi-GPU implementation shows mostly linear strong scaling. I/O also plays a large role; splitting data into parts improves read time and burst buffers dramatically improve read times. This work will be integrated into the M-TIP workflow as part of the next milestone ADSE13-193.

97 MATHEMATICS AND COMPUTING↗

Evaluation report on the Thermo Scientific TruDose (neutron,gamma) EPD3

This report summarizes an evaluation study on the Thermo Scientific TruDose n/γ EPD3 by LANL’s RP-SVS group. Two EPD3s were received for assessment (SNs 7500100 and 7500108) along with an EPD3 desktop reader. The evaluation included intercomparisons with Thermo’s N2 EPD which is in wide circulation at LANL but is no longer commercially available. A favourable assessment of the TruDose EPD3 would help support it as a viable option to replace the N2 EPD. The data and observations included in this report could also serve as the basis of a Technical Basis Document for the use of the EPD3 at LANL.

61 RADIATION PROTECTION AND DOSIMETRY↗

Structural Health Monitoring: Using an Autoencoder to Identify Damage in a Bolted Joint [Capstone Project]

Los Alamos National Laboratory (LANL) is an important fixture in the United States Department of Energy’s (DOE) National Nuclear Security Agency (NNSA) complex. LANL is one of the largest national laboratories in the country, and the laboratory’s primary mission is to support the nation’s nuclear stockpile. The lab functions as a design agencies for the NNSA and performs extensive testing on weapons as part of that mission. The shock and vibration test team at LANL utilizes electrodynamic shaker systems for important qualification testing in support of the laboratory’s mission. Modern engineering relies heavily on bolted joints to connect two objects. During these shaker tests, engineers depend on bolted joints to secure the test article to a fixture and the fixture to the table. The test article may be hazardous and contain high explosives which could create a safety issue if a bolted joint failed. A loss of preload in a bolt will affect the way energy is input to the system and may introduce nonlinearities as the joint opens and closes. The loss of preload can create challenges controlling the test and make acquired signals useless. Being able to monitor preload within bolted joints during testing can improve the quality of the data and keep workers safe.

42 ENGINEERING↗

238 PuO 2 In Vitro Lung Dissolution Rate and Particle Size Determination for Material Involved in the June 8, 2020 Incident at the Los Alamos National Laboratory PF-4 Facility

As part of the LANL response to the June 8, 2020 238 PuO 2 inhalation exposure incident in PF-4, the Nuclear and Radiochemistry Group (C-NR) was asked to assist in determining the lung dissolution rate and particle size distribution of the airborne material. These material characteristics, along with urine and fecal bioassay data, are used by the Radiation Protection Services (RP-SVS) internal dosimetrists to refine dose estimates for exposed workers. Similar to previous studies, an in vitro lung dissolution rate study was performed to assess how fast 238 Pu is cleared from the lungs. Given that PuO 2 is a relatively insoluble material, it dissolves very slowly and requires in vitro studies of 100 or more days to estimate dissolution rates. This report details the results of a 100 day in vitro dissolution rate study and the particle size characteristics of 238 PuO 2 collected on an air filters during the incident. Results show that the 238 PuO 2 involved in this incident has behavior comparable to PuO 2 from previous in vitro studies, with approximately 1% of material dissolving quickly, and 99% of the material dissolving very slowly, with a half-time of approximately 120 years. This is somewhat slower than what was determined in a previous study of LANL 238 PuO 2 , which had an experimental dissolution half-time of 3 years, but significantly faster than 3000 years measured for 239 PuO 2 . Particle size distribution measurements indicate that particle sizes range from 0.10 µm – 6 µm, with most < 2 µm, which is reasonable based on our understanding of the process history of the 238 PuO 2 . Particle size, specific surface area, calcining temperature, specific activity, and age all are known factors that can impact the dissolution rate of refractory materials, however, there are too few studies to quantify the exact influence of these parameters on a measured dissolution rate. The results of this study add to that knowledge base, and provide new insights into the dissolution rates for this LANL process-specific 238 PuO 2 material.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗

Acceptance Testing of the Scorpius Sweep Magnet

A beam-dump magnet for Scorpius has been defined by LANL and designed and built by Radiabeam Technologies. Initial verification of the Radiabeam design used a magnetic field model provided by Radiabeam and analyzed by LANL tools during September 2021. Simulations indicated that the design was sufficient to meet deflection requirements to protect sensitive equipment in the case of a failed target. In January 2022, the magnet was fabricated and Radiabeam conducted measurements of the magnetic field as a function of position. The measurements deviate somewhat from the simulation. In particular, the peak magnetic field is 10-15% smaller in magnitude than expected from simulation. This note compares the magnetic field measurements to simulation and to measurements of the existing DARHT magnet, which was designed for the same purpose. We show a comparison of the measured beam deflection performance between Scorpius and DARHT and show updated results of LANL’s electron beam tracking code using the Scorpius measurements. Using field measurements we find that the DARHT magnet will deflect a 19.6 MeV electron beam by 46.6° and the Scorpius magnet will deflect by 44.6°. These results show that the as-built Scorpius magnet has met design requirements for beam deflection.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Physical Sciences Vistas: Perspectives on Excellence in Community Relations (Issue 1, 2022)

This is the first 2022 issue of Physical Sciences Vistas, with a focus on “excellence in community relations.” The achievements in this area help LANL realize the goal of being "recognized as a force for good" and promotes the lab's "strategic objectives of nuclear deterrence, threat reduction, technical leadership, and trustworthy operations." Some of the highlights in this issue include LANL's new outreach program, featuring interactive travel labs, outstanding achievements in pollution prevention and how LANL is "supporting opportunities for Indigenous women in physics."

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

NorthStar Facility Target Fab and Flow Testing - FY 21

The facility target fabrication and flow testing activity will consist of flow tests using the blower system at LANL to test the disk holder and target, both redesigned by the NorthStar prime contractor. The housing and transition system delivering helium cooling to the disc holder and target will be fabricated and tested at LANL facilities. The tests will include pressure drop versus flow measurements through the target and housing, optical flow diagnostics and fiber optic imaging of the disc stack. The pressure drop measurements will be compared to CFD simulations to verify the latter, the optical flow diagnostics will be used to determine whether modifications made to the housing and target holder allow sufficient flow through the bottom of the housing to adequately cool it and the fiber optics will be used to image the discs during operation as a proof of concept of the diagnostic, to be used at NorthStar facilities during preproduction testing. The work is a Partial Fulfillment of the Deliverable Requirement for NorthStar Facility Target Fab and Flow Testing and Production Target Testing Support by LANL

42 ENGINEERING↗

PDQ Users Manual. Manual Version 2, for PDQ Code Version 1.20

PDQ is a tool for the management of the input and execution of batch jobs for simulation codes that use a text based input system. It accomplishes this goal by operating at two levels. First, it takes input file templates (commonly known at LANL as input deck templates) and creates multiple instantiations by performing substitutions of data from table files into symbols (variables) found in the template. Second, it provides commands to submit the created files to the SLURM batch system for execution. These two activities taken together produce a whole that is greater than the sum of its parts and provides an elegant way of executing studies across multiple similar simulations while minimizing the risk of typographical errors in the input files. PDQ was originally developed as a job management system called XVS by Jeff McAninch while he was at LANL. Besides the capabilities described here, XVS had many other features specific for interactions with particular simulation codes. After Jeff’s departure, maintenance of XVS was taken over by Rendell Carver; he added some new features as well as kept it functioning as the batch system at LANL was changed from LSF to MOAB to SLURM. In 2017, Rob Pelak decided to develop a different version that removed the additional features (many of which were rendered obsolete with the retirement of the simulation code or batch system that they supported) and produced a cleaner “bare bones” version of XVS. A few other behaviors of XVS that Rob found irksome were altered. Rob gave the resulting code a new name: PDQ. In 2022 Danielle McDermott developed a version that runs under Python 3.X. As suggested by Rob, she used the python2to3 utility to identify most changes. Given that PDQ continues to operate with Python version 2.7 we have advanced the version number to 1.20.

97 MATHEMATICS AND COMPUTING↗

2021 Radionuclide Air Emissions Report for Los Alamos National Laboratory, Revised October 2022

Provided is a revision to the Calendar Year 2021 Radionuclide Air Emissions Report for the Los Alamos National Laboratory (LANL). This report is a regulatory compliance deliverable for LANL under the Radionuclide NESHAP, 40 CFR 61 Subpart H. The revised report is needed to correct an error identified regarding generation of wind data files. These wind data files are used for plume modeling as part of calculating off-sites doses from monitored radionuclide air emissions sources. The error resulted from a software update by LANL’s meteorology team after new towers were added to the tower network. As a result of this error, incorrect wind frequencies were assigned to the different stability classes. This slightly affected the plume model calculations and subsequent off-site dose determinations for analyses using these wind files.

2021 Radionuclide, Air Emissions↗

W.A.T.E.R. Water Assessment & Technical Efficiency Report

Water use at Los Alamos National Laboratory (LANL) has become a top priority due to New Mexico’s arid climate. LANL is taking steps to reduce its current water footprint and become a national leader in water efficiency. LANL used approximately 271 million gallons of water in FY 2021. Despite the large water footprint, the Lab has reduced its water use by 2% each year since a 2007 baseline. To continue this positive trend of water conservation, the water management team at Utilities & Infrastructure – Operations Support & Improvement (UI-OSI) studied water usage across campus and developed several water reduction strategies.

54 ENVIRONMENTAL SCIENCES↗

Hierarchical Division and Clustering of Group Structures

When using multigroup neutron transport models, it is important to choose a suitable group structure due to the impact on runtime and accuracy. Group structures at LANL have been largely pared down to a handful of commonly used group structures, such as the LANL-30 and LANL-70 group structures. By identifying the key boundaries for a given problem, more insight can be gained into why the commonly used group structures are accurate and when they are inaccurate. This work focuses on using hierarchical division and agglomeration methods to identify the most critical boundaries in these group structures, using the ICSBEP HEU-MET-FAST-001-001 benchmark as a case study.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Traditional Forensic Examinations on Bulk Special Nuclear Material

The Federal Bureau of Investigation (FBI) Laboratory at Quantico, Virginia is responsible for the forensic examination of radiological evidence and evidence contaminated with radioactive materials. Due to these unique hazards and the necessary specialized safety protocols, the FBI has developed a network of Partner Laboratories (PLs) across the United States of America to support conventional forensic examinations of radiological evidence and evidence contaminated with radioactive materials. In support of this, the FBI Laboratory has established the Hazardous Evidence Analysis Team (HEAT), a group of qualified forensic examiners, scientists, technicians, and photographers who can deploy to laboratories outside of the FBI Laboratory at Quantico, VA to perform conventional forensics on evidence containing/contaminated with hazardous materials. One of the FBI’s PLs, the United States Department of Energy’s Los Alamos National Laboratory (LANL), in Los Alamos, New Mexico, has unique facilities, personnel, and procedures to secure, safely handle, and process significant quantities of special nuclear material (SNM). While LANL’s procedures for working with SNM are well established, working with SNM under evidentiary controls is not. Close cooperation between LANL and FBI HEAT is required due to FBI policies on evidence handling, as well as the challenges associated with the exploitation and preservation of conventional forensics (fingerprints, trace evidence, and photography) on SNM evidence.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Principles of Biosafety

Biological safety, or biosafety, means containment principles, technologies and practices that are implemented to prevent unintentional exposure to pathogens and toxins, or their accidental release. This report is a training course for Biosafety with these features and objectives: Topics associated with biological safety, including basic terms, definitions, and approaches to biological safety; regulations, consensus guidance and standards for biological safety; safety requirements for working with biological materials at Los Alamos National Laboratory (LANL); containment requirements for biological materials at LANL; and, emergency response requirements for biological materials at LANL.

99 GENERAL AND MISCELLANEOUS↗