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At least 577 records · Page 32
All sourcesNASA NTRSDOE OSTI
DOE OSTI2013

3D Reconstruction of Biological Organization and Mineralization in Sediment Attached Biofilms During Uranium Bioremediation

Of central interest in this study were microbial communities attached to sediment particles and in associated groundwater. Are the communities similar? What do the organisms look like and how do they associated with each other? Research was conducted on samples collected from the Department of Energy's (DOE) Rifle Integrated Field Research Challenge (IFRC) site in Rifle, Colorado, USA. This site served first as a test case for in situ bioremediation via biostimulation, and more recently as a location for studying the role of microbial communities in the carbon and other linked biogeochemical cycles. We addressed the question of the nature of planktonic to sediment-attached microbial communities using field and laboratory experimental studies with a range of methods that provide 2- and 3-dimensional topological information coupled to information about chemical speciation, organism type, and activity levels. The research leveraged data from metagenomics and proteomics analyses that obtained through parallel work at the Rifle site in the context of the IFRC. In this project we integrated characterization methods with extensive genomic sequence information and associated environmental data to better understand the processes that occur within groundwater and sediment-attached communities. Notable is the range of characterization methods, including scanning transmission x-ray microscopy (STXM), micro-EXAFS/XANES and microdiffraction and 2D and 3D cryo-electron tomographic analysis, and high-resolutino transmission electron microscope (HRTEM) analysis to characterize these natural microbial communities. A cryo-TEM work was unique because samples for electron microscopic characterization were cryo-plunged directly on site immediately after sampling. This step minimizes post-collection alterations, including cell damages and change of redox state. Among many achievements documented in publications listed at the end of this report, we highlight the following: 1) The development of a platform for routine correlative cryogenic microscopy and spectroscopy with samples prepared on-site. 2) The determination of which organisms dominate planktonic and biofilm communities in the subsurface. 3) Identification of microorganism-mineral associations and discovery of a novel mechanism that sustains activity of iron-reducing bacteria. 4) The detection of bacteria from the OP11-OD1-WWE3 (etc.) radiation and elucidation of their remarkable structural organization by cryog-TEM cryo-electron tomograhpy (cryo-ET). 5) Extensive analysis of biofilms and documentation of the association of cells and Se minerals. 6) The comparison of expressed c-type cytochromes between pure cultures of G. bemidjiensis and related field populations, provided insight into possible molecular mechanisms for U(VI) reduction in the aquifer. At least sixteen publications will result from this project (partial support), which provide both graduate student and post doctoral training.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2018

Maximizing the habitat restoration potential of controlled releases at hydropower dams; Understanding impacts of hydrograph form on sediment transport

Regulation of streamflow for hydropower often alters natural hydrographs, commonly reducing peak flows, increasing baseflows, and increasing ramping rates. Simultaneously, reservoirs typically trap sediment, reducing the supply to the reach downstream of the dam. These changes to the flow regime and sediment supply impact channel morphology and sediment transport processes in ways that reduce the diversity and suitability of instream habitat. A variety of restoration approaches have attempted to mitigate for some of these changes and a growing number include releases of high flows designed to mimic key characteristics of the pre-regulation hydrograph. One example is the Trinity River, CA, where the addition of augmentation gravel to the channel has been combined with high flows designed to restore portions of the pre-regulation hydrograph to improve channel conditions for spawning fish on the Trinity River, CA. Another example is the high-flow experiments on the Colorado River through the Grand Canyon that aim to restore eroding sand bars that not only provide habitat but camping for rafting groups. More projects that restore portions of the pre-regulation hydrograph are likely in the future because the Federal Energy Regulatory Commission (FERC) requires habitat mitigation efforts in the relicensing process for hydropower facilities. However, the outcomes of these costly restoration efforts are often hard to predict because little is known about how hydrograph form actually impacts channel morphology and bedload transport in rivers. Here we summarize the results of two flume experiments designed to investigate the impacts of hydrograph form on the morphology of a channel bar and bedload transport processes. The first experiment primarily investigated the impacts of hydrograph recession rate on the morphology of a channel-bar in a sand bed channel. Additional runs examined the combined effects of hydrograph recession and a dense patch of vegetation on bar form. The second flume experiment investigated bedload transport processes in an armored, gravel bed channel during hydrographs with varying form. It documented total bedload flux for a hydrograph, bedload flux rates, persistence of the coarse armor surface, and changes in bed surface structure. Both experiments observed links between hydrograph form and the resulting bar morphology or bedload transport processes, providing insight into ways that high flow hydrographs can be designed to better facilitate restoration goals downstream of hydropower facilities.

13 HYDRO ENERGY↗
DOE OSTI2017

DETERMINING THE TRIBUTARY SEDIMENT CONTRIBUTION TO EXPERIMENTAL FLOOD DEPOSITS ON THE COLORADO RIVER IN MARBLE CANYON, GRAND CANYON, ARIZONA

A multivariate sediment fingerprint was used in a Bayesian mixing model to determine the source contribution to experimental flood deposits along the Colorado River in the Marble Canyon reach of Grand Canyon, AZ. This study provides an independent evaluation, complementary to previous sediment mass balance and morphological studies, of the degree to which sand from the Paria River, the primary source of sand in Marble Canyon, has supplemented total sand storage since upstream dam closure in 1963. Samples of endmember and downstream mixed populations of sand were analyzed using portable XRF to measure the concentration of eleven major and trace elements, from which 55 elemental ratios were calculated. A principal components analysis consolidated those ratios eligible for use in the fingerprint into a multivariate signature used in the mixing model, MixSIAR. Twenty flood deposits from 14 sites in Marble Canyon from the 2013 and 2014 controlled floods were sampled. Six individual mixing models, using sediment fingerprints unique to each of six half-phi grain size fractions returned the percentage of sand, in each size fraction of each deposit, that was sourced from the Paria River. Paria contribution averaged 33.8 ± 4.1% in deposits from the 2013 flood, and 54.7 ± 4.3% in deposits from the 2014 flood. Individual grain size samples ranged 4.9 – 73.1% in 2013 and 9.1 – 90.2% in 2014. In general, iii the four median grain size fractions (90 – 355 μm) in both years have the highest Paria contribution; low Paria contribution in the finest 63 – 90 μm) fraction suggests significant contribution by an unaccounted-for third endmember, likely minor tributaries. The coarsest fraction, 355 – 500 μm, is the only grain size to show a trend in Paria contribution with distance traveled downstream, suggesting a transport-related fractionation effect. Overall scatter in the results speaks to the spatial heterogeneity of intra-rapid storage pools throughout the reach and their capacity, as well as the effects of local hydraulic variability between eddy deposition zones where sandbars form. Mass balance calculations determine that under conditions of constant or decreasing total storage since 1963, approximately 20-30% of the annual Paria flux would need to be retained within Marble Canyon each year to reach the observed concentration of Paria sand. From these results, we conclude that HFEs are conditionally sustainable given frequent enough occurrence to maintain sandbar deposit storage.

13 HYDRO ENERGY↗
DOE OSTI2022

PARTICLE RESOLVED DNS STUDY OF TURBULENCE EFFECTS ON HYPORHEIC MIXING IN RANDOMLY PACKED SEDIMENT BEDS

Pore-resolved direct numerical simulations (DNS) are used to investigate the interactions between stream-water flow turbulence and groundwater flow through a porous sediment bed in the hyporheic zone. Two permeability Reynolds numbers (2.56 and 5.17), representative of aquatic systems and representing ratio of permeability to viscous length scales, were simulated to understand its influence on the momentum exchange at the sediment-water interface (SWI). A doubleaveraging methodology is used to compute the Reynolds stresses, form-induced stresses, and pressure fluctuations. It is observed that both shear layer and turbulent shear stress penetration increases with ReK. Reynolds and form-induced bed-normal stresses increase with ReK. The peak values of the form-induced stresses for the lower (2.56) and higher (5.17) ReK happen within the top layer of the sediment bed. The sum of turbulent and form-induced pressure fluctuations, analyzed at their respective zero-displacement planes, are statistically similar and can be well approximated by a t location-scale distribution fit providing with a model that could potentially be used to impose boundary conditions at the SWI in reach scale simulations.

Karra, Shashank↗
DOE OSTI2017

A Global Data Analysis for Representing Sediment and Particulate Organic Carbon Yield in Earth System Models

Although sediment yield (SY) from water erosion is ubiquitous and its environmental consequences are well recognized, its impacts on the global carbon cycle remain largely uncertain. This knowledge gap is partly due to the lack of soil erosion modeling in Earth System Models (ESMs), which are important tools used to understand the global carbon cycle and explore its changes. As such, this study analyzed sediment and particulate organic carbon yield (CY) data from 1081 and 38 small catchments (0.1-200 km 2 ), respectively, in different environments across the globe. Using multiple statistical analysis techniques, we explored environmental factors and hydrological processes important for SY and CY modeling in ESMs. Our results show clear correlations of high SY with traditional agriculture, seismicity and heavy storms, as well as strong correlations between SY and annual peak runoff. These highlight the potential limitation of SY models that represent only interrill and rill erosion because shallow overland flow and rill flow have limited transport capacity due to their hydraulic geometry to produce high SY. Further, our results suggest that SY modeling in ESMs should be implemented at the event scale to produce the catastrophic mass transport during episodic events. Several environmental factors such as seismicity and land management that are often not considered in current catchment-scale SY models can be important in controlling global SY. Our analyses show that SY is likely the primary control on CY in small catchments and a statistically significant empirical relationship is established to calculate SY and CY jointly in ESMs.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

Injectivity Evaluation for Offshore CO 2 Sequestration in Marine Sediments

Global and regional climate change caused by greenhouse gases emissions has stimulated interest in developing various technologies (such as carbon dioxide (CO 2 ) geologic sequestration in brine reservoirs) to reduce the concentrations of CO 2 in the atmosphere. Our study develops a statistical framework to identify gravitational CO 2 trapping processes and to quantitatively evaluate both CO 2 injectivity (or storage capacity) and leakage potential from marine sediments which exhibit heterogeneous permeability and variable thicknesses. Here, we focus on sets of geostatistically-based heterogeneous models populated with fluid flow parameters from several reservoir sites in the U.S. Gulf of Mexico (GOM). A computationally efficient uncertainty quantification study was conducted with results suggesting that permeability heterogeneity and anisotropy, seawater depth, and sediment thickness can all significantly impact CO 2 flow and trapping. Large permeability/porosity heterogeneity can enhance gravitational, capillary, and dissolution trapping, which acts to deter CO 2 upward migration and subsequent leakage onto the seafloor. When log permeability variance is 5, self-sealing with heterogeneity-enhanced gravitation trapping can be achieved even when water depth is 1.2 km. This extends the previously identified self-sealing condition that water depth be greater than 2.7 km. Our results have yielded valuable insight into the conditions under which safe storage of CO 2 can be achieved in offshore environments. The developed statistical framework is general and can be adapted to study other offshore sites worldwide.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

WHONDRS Surface Water and Sediment Non-Purgeable Organic Carbon and FTICR-MS across Glacial Features in Svalbard 2021 (v3)

This dataset supports a broader study examining land-atmosphere gas exchange associated with permafrost and glaciers in Svalbard. The dataset provides geochemistry and organic matter characterization data generated from surface water and sediment. Samples were collected from 8 spatially diverse sites across central Svalbard and also from a more comprehensive temporal and spatial study within one glacial catchment area throughout one summer melt season. Related data were collected and will be published separately in collaboration with Yde and Kleber.This data package was originally published in September 2022. It was updated in March 2023 (v2; new and modified files), and July 2025 (v3; modified files). See the change history section in the readme for details.For details on how to navigate data packages generated by this project, see https://data.ess-dive.lbl.gov/portals/PNNLRiverCorridorSFA/About. This dataset is comprised of one main data folder containing (1) file-level metadata; (2) data dictionary; (3) field metadata; (4) dissolved organic carbon (DOC; measure as non-purgeable organic carbon; NPOC); (5) surface water sampling protocol; (6) sediment extraction protocol; (7) readme; (8) methods codes; (9) international generic sample number (IGSN) mapping file; and (10) folder of high resolution characterization of organic matter via 7 and 12 Tesla (7T and 12T) Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) generated through the Environmental Molecular Sciences Laboratory (EMSL; https://www.pnnl.gov/environmental-molecular-sciences-laboratory). The FTICR folder contains two subfolders containing the 7T and 12T .xml data files and another subfolder containing instructions for using Formularity (https://omics.pnl.gov/software/formularity) and an R script to process the data based on the user's specific needs. All files are .csv, .pdf, .R, .ref, or .xml.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Laboratory time series moisture manipulative experiment from sediment across San Antonio, Texas: time series aerobic respiration and geochemistry

This dataset supports a broader study examining the effects of wetting and drying on hyporheic zone respiration. The dataset provides data generated from a laboratory moisture manipulation experiment. The contents include time series aerobic respiration and moisture; dissolved oxygen; sediment geochemistry data; and field metadata (including qualitative information on instream and river corridor characteristics). Samples were collected as part of the WHONDRS Allison Veach collaboration (AV1). The data package associated with the AV1 study is available at https://data.ess-dive.lbl.gov/datasets/doi:10.15485/2529428. AV1 sampling occurred across 7 perennial and 7 intermittent streams in San Antonio, Texas. Each stream/site was visited both in summer during base flow (July-September 2023) and winter during peak flow (January-February 2024). This study uses subsamples from a subset of AV1 samples. The original field samples were labeled as AV1_###. Subsequent subsamples for this study were labeled as EV_###. The labels from the field samples and the EV subsamples can be mapped directly based on the digits following the prefix and underscore (i.e., EV_001 is a subsample from AV1_001). See the critical details section below for more details on sample naming. For details on how to navigate data packages generated by this project, see https://data.ess-dive.lbl.gov/portals/PNNLRiverCorridorSFA/About. This dataset is comprised of one main data folder containing (1) file-level metadata; (2) data dictionary; (3) field metadata; (4) readme; (5) field protocol; and a (6) a subfolder with sediment sample data from the incubation experiment. The sample data subfolder contains (1) effect size; (2) iron (II); (3) gravimetric moisture; (4) respiration rates; (5) raw dissolved oxygen values and plots; (6) specific conductance; (7) pH; (8) temperature; (9) a summary containing mean, median, and standard deviation values of each data type for each treatment (wet and dry); and (10) methods codes. All files are .csv or.pdf.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Seasonal hyporheic dynamics control coupled microbiology and geochemistry in Colorado River sediments

Riverbed microbial communities play an oversized role in many watershed ecosystem functions, including the processing of organic carbon, cycling of nitrogen, and alterations to metal mobility. The structure and activity of microbial assemblages depend in part on geochemical conditions set by river-groundwater exchange or hyporheic exchange. In order to assess how seasonal changes in river-groundwater mixing affect these populations in a snowmelt-dominated fluvial system, vertical sediment and pore water profiles were sampled at three time points at one location in the hyporheic zone of the Colorado River and analyzed by using geochemical measurements, 16S rRNA gene sequencing, and ecological modeling. Oxic river water penetrated deepest into the subsurface during peak river discharge, while under base flow conditions, anoxic groundwater dominated shallower depths. Over a 70 cm thick interval, riverbed sediments were therefore exposed to seasonally fluctuating redox conditions and hosted microbial populations statistically different from those at both shallower and deeper locations. Additionally, microbial populations within this zone were shown to be the most dynamic across sampling time points, underlining the critical role that hyporheic mixing plays in constraining microbial abundances. Given such mixing effects, we anticipate that future changes in river discharge in mountainous, semiarid western U.S. watersheds may affect microbial community structure and function in riverbed environments, with potential implications for biogeochemical processes in riparian regions.

16S rRNA↗
DOE OSTI2019

Pollution and Risk of PAHs in Surface Sediments from the Tributaries and Their Relation to Anthropogenic Activities, in the Main Urban Districts of Chongqing City, Southwest China

Concentrations, sources and risk of 16 priority polycyclic aromatic hydrocarbons (PAHs) were investigated in surface sediments from 19 representative tributaries in a regional scale of Chongqing City. The total concentration of 16 PAHs (ΣPAHs) ranged from 221 to 3205 ng g{sup −1} with a mean of 1055 ng g{sup −1}. Most tributaries of the Jialing River exhibited significantly higher ΣPAHs concentrations (mean 1864 ng g{sup −1}) compared to those flowing into the Yangtze River (mean 787 ng g{sup −1}). Isomeric ratio and hierarchical clustering analysis showed combustion may impact sedimentary PAHs at most center sites of the City, while PAHs at most sites were mixed of petrogenic and pyrogenic sources. Toxicity equivalency concentration for carcinogenic PAH were 2–4 times more than the Dutch limit. More comprehensive assessment of safety is suggested to reduce environmental risk of PAHs in sediments.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Evaluation of coal-associated sediments, wastes, and AMD sludge in the Southern Appalachian Basin as feedstock materials for REE and Li recovery

Critical minerals (CM) such as rare earth elements (REE+) and Lithium (Li) are essential to technological innovation, energy transitions, global economic and defense security, necessitating the search for unconventional resources and efficient recovery methods to avert supply chain disruptions. Here, this study evaluates coal-associated sediments (underclay and roof rock) and wastes from the Pennsylvanian Pottsville Formation of the Southern Appalachian Basin (SAB) as potential feedstocks for CM recovery. A total of 34 samples (15 underclays, 12 roof rocks, 5 Acid Mine Drainage (AMD) sludges, and 2 coal mining wastes) were characterized using XRD, XRF, ICP-MS, and μ-XRF analytical methods. The REE+ and Li concentrations of these materials ranged from 46.8 to 334.4 ppm and from 11.1 to 519 ppm, respectively, with one underclay sample (Hendrix 3456) yielding the highest values for both. Bulk mineralogy for all samples was dominated by aluminosilicate clay phases, particularly illite and kaolinite. All samples exhibited REY def, rel% values >26% and C outl indices that ranged from 0.69 to 0.94, classifying their REE ore potential as Category II (Promising) as defined by Seredin and Dai (2012). Extractability tests (EPA method 3051 A) yielded low REE+ and Li recoveries, with maximum values of 3.3% and 3.6%, respectively, suggesting associations with resistant minerals like clay and phosphates. Elemental mapping indicates that REE+ is associated with phosphate, whereas statistical analysis suggests that REE+ are associated with aluminosilicates, suggesting heterogeneous associations or minimal phosphate contribution. Li also correlated positively with Al 2 O 3 , indicating an aluminosilicate host. This study highlights the potential of coal-associated sediments in the SAB.

Clay minerals↗
DOE OSTI2014

Cytotoxicity of TiO{sub 2} nanoparticles towards freshwater sediment microorganisms at low exposure concentrations

There is a persistent need to assess the effects of TiO{sub 2} nanoparticles on the aquatic ecosystem owing to their increasing usage in consumer products and risk of environmental release. The current study is focused on TiO{sub 2} nanoparticle-induced acute toxicity at sub-ppm level (≤1 ppm) on the three different freshwater sediment bacterial isolates and their consortium under two different irradiation (visible light and dark) conditions. The consortium of the bacterial isolates was found to be less affected by the exposure to the nanoparticles compared to the individual cells. The oxidative stress contributed considerably towards the cytotoxicity under both light and dark conditions. A statistically significant increase in membrane permeability was noted under the dark conditions as compared to the light conditions. The optical and fluorescence microscopic images showed aggregation and chain formation of the bacterial cells, when exposed to the nanoparticles. The electron microscopic (SEM, TEM) observations suggested considerable damage of cells and bio-uptake of nanoparticles. The exopolysaccrides (EPS) production and biofilm formation were noted to increase in the presence of the nanoparticles, and expression of the key genes involved in biofilm formation was studied by RT-PCR. - Highlights: • Toxicity of NPs towards freshwater sediment bacteria at sub-ppm concentrations. • Decreased toxicity of the nanoparticles in the consortium of microorganisms. • Enhanced bacterial resistance through EPS and biofilm formation in the presence of NPs. • Considerable surface damage of cells and internalization of NPs. • Gene expression analyses related to biofilm formation in the presence of NPs.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Enantio-selective molecular dynamics of (±)-o,p-DDT uptake and degradation in water-sediment system

Highlights: • Simultaneous molecular uptake and degradation of (±)-o,p-DDT. • Both uptake and degradation of (-)-enantiomer are higher than (+)-o,p- DDT. • Both uptake and degradation are liable for removal of (±)-o,p-DDT from nature. • Uptake plays crucial role for removal of (±)-o,p-DDT from nature. Enantio-selective molecular dynamics of (±)-o,p-DDT uptake and degradation in water-sediment system is described. Both uptake and degradation processes of (-)-o,p-DDT were slightly higher than (+)-o,p-DDT enantiomer. The optimized parameters for uptake were 7.0 μg L{sup −1} concentration of o,p-DDT, 60 min contact time, 5.0 pH, 6.0 g L{sup −1} amount of reverine sediment and 25 °C temperature. The maximum degradation of both (-)- and (+)-o,p-DDT was obtained with 16 days, 0.4 μg L{sup −1} concentration of o,p-DDT, pH 7 and 35 °C temperature. Both uptake and degraded process followed first order rate reaction. Thermodynamic parameters indicated exothermic nature of uptake and degradation processes. Both uptake and degradation were slightly higher for (-)-enantiomer in comparison to (+)-enantiomer of o,p-DDT. It was concluded that both uptake and degradation processes are responsible for the removal of o,p-DDT from nature but uptake plays a crucial role. The percentage degradations of (-)- and (+)-o,p-DDT were 30.1 and 29.5, respectively. This study may be useful to manage o,p-DDT contamination of our earth's ecosystem.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

An experimental system and procedure of unsteady-state relative permeability test for gas hydrate-bearing sediments

Reliable estimations of the relative permeability of gas and water in hydrate-bearing sediments (HBS) and the dependency of the relative permeability on hydrate saturation are critical to predict the productivity of a hydrate reservoir. Yet, this remains poorly estimated owing to lack of experimental data associated with difficulties in conducting multiphase flow experiments in HBS. Recognizing the experimental challenges, this study intends to develop and validate a new experimental system and procedure of unsteady-state relative permeability test that can generate reliable and reproducible flow measurements in HBS. Furthermore, gas hydrate is considered as a part of solid matrix in the sediment, so one of the challenges is to maintain a constant hydrate saturation, which is achieved in this experimental study using tight pressure-temperature (P-T) control near the hydrate stability boundary. The measured differential pressure across the specimen, methane injection flow rate, and volume of displaced brine are used to calculate the relative permeability by adopting a conventional Buckley-Leverett theory-based interpretation method. Residual brine saturation calculated for the hydrate-bearing specimen is higher than that of hydrate-free specimen, presumably due to decrease in pore size, increase in heterogeneity of solid matrix, and increase in size distribution of solid matrix and pore in the presence of hydrates. Further studies are necessary to represent the results of the unsteady-state flow experiment in HBS with a gas hydrate-dependent relative permeability model.

03 NATURAL GAS↗
DOE OSTI2018

Physical property characteristics of gas hydrate-bearing reservoir and associated seal sediments collected during NGHP-02 in the Krishna-Godavari Basin, in the offshore of India

India’s National Gas Hydrate Program Expedition 02 (NGHP-02) was conducted to better understand geologic controls on gas hydrate occurrence and morphology, targeting coarse-grained sediments along the lower continental slope offshore eastern India. This study combines seismic, logging-while-drilling data, and a petroleum system approach to provide a regional geologic and lithologic context for: 1) gas hydrate morphology and distribution, and 2) effects of fine-grained sediments (clays and other grains smaller than 63µm) on gas production in NGHP-02 Area B in the Krishna-Godavari Basin. Area B seismic data show a buried anticline/syncline structure with strong reflectors, R1 and R2, that delineate two of the five lithologic units: Unit I (shallowest), II (R1), III, IV (R2) and V (below the bas of gas hydrate stability). Throughout Area B, gas hydrate morphology depends on its placement within these units. Specifically, core- and grain-scale measurements indicate fines content exerts a primary control on the gas hydrate distribution and morphology. Units I, II and III are generally fine-grained. On the anticline crest, these units host primarily grain-displacing gas hydrate veins linked to pore-occupying gas hydrate in thin, localized, coarser-grained deposits. Diatoms in Unit III increase porosity with depth, reaching ~70% where it contacts Unit IV, the gas hydrate reservoir associated with reflector R2. The Unit III lithology and porosity allow fluid and dissolved-phase methane to escape Unit IV and form gas hydrate in the fine-grained overburden. Within Unit IV, fine-grained layers are interbedded with coarser-grained gas hydrate reservoir sands, and the fines content even in the sands is high enough to impact hydraulic and mechanical properties during gas production. Fluid motion during gas production can mobilize fines, which can then clog pore throats, limiting production rates. In conclusion, pore-water freshening during gas hydrate dissociation can increase fines mobilization, particularly given the smectite identified in the fine-grained interbeds.

03 NATURAL GAS↗
DOE OSTI2016

The transport of suspended sediment in the wake of a marine hydrokinetic turbine: Simulations via a validated Discrete Random Walk (DRW) model

The interaction of sediment with Marine Hydrokinetic (MHK) Turbines is studied via turbulent flow simulation coupled with a model for particle dynamics. The Discrete Random Walk (DRW) model is commonly used for simulations of particle dispersion in environmental flows. A method to improve the accuracy of the DRW model in conjunction with RANS simulations of the flow around MHK turbines is presented. A key issues for the use of the DRW model in marine applications is identified, finding the right characteristic eddy lifetime scale, and a simple methodology based on G.I. Taylor's classical dispersion theory is develop to calibrate this physical model parameter. The model is validated against experiments in the literature and the physics of suspended sediment transport in the wake of an MHK turbine is studied with this improved method. The qualitative changes observed in the particle trajectories agree well with theoretical and empirical observations and the quantitive trends allow for comparison of multiple particle cases under different flow conditions, confirming that this implementation of CFD can become a powerful tool to select the most challenging cases, among the thousands of potential studies on the environmental effects of MHK energy, for further study with experiments and pilot projects.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Multistage Triaxial Tests on Laboratory-Formed Methane Hydrate-Bearing Sediments

A sound understanding of the geomechanical behavior of hydrate–bearing sediments (HBSs) is essential not only for assessing reservoir and wellbore stability during methane gas production but also for projecting the impact of global warming on the stability of geological settings that contain hydrates. This study experimentally investigated the geomechanical responses of laboratory–formed methane–HBS to triaxial shearing under drained conditions. The hydrate pore habit formed in the sediments is noncontact–cementing, which is different from contact–cementing or grain–coating hydrate pore habits formed when the excessive gas method is used. The multistage triaxial test method, which shears a single specimen under different confinements, was employed to examine its applicability in measuring geomechanical properties of the HBS. Conventional single–stage triaxial tests were also performed to serve as baselines. The results show that both the strength and stiffness of HBS increase with increased hydrate saturation and confining stress. Shear dilatancy increases with increased hydrate saturation and decreased confining stress. The peak strength and peak/postpeak shear dilation measured using the multistage tests are comparable to those using the single–stage tests. However, the stiffness measured in later stress stages in the multistage tests was enhanced by the stress–strain history of earlier stages. Therefore, the multistage test offers an efficient way of measuring the strength and volumetric response of the HBS with a much smaller number of specimens than the single–stage test. As a result, this benefits the geomechanical characterization of the HBS, as obtaining the pressure cores is extremely costly and preparing lab samples is usually sophisticated and time consuming.

58 GEOSCIENCES↗
DOE OSTI2026

Inundation and Sediment Supply Predict Annual but Not Centennial Carbon Accumulation in Tidal Wetlands Across Land‐Use Types

Despite growing interest in the contributions of tidal wetlands to natural climate solutions, data remain scarce on how land use affects their carbon accumulation rates (CAR). Additionally, environmental factors driving the large observed variability in CAR among sites are poorly understood. To address these knowledge gaps, we measured short-term (∼1 year) and long-term (∼100 years) CAR using feldspar marker horizons, 210 Pb profiles, and surface elevation tables from 39 sites in seven estuaries in Oregon and Washington, USA. Sites varied in wetland type (tidal marsh, tidal swamp, nontidal pasture), land-use history (reference, restored, and disturbed), and salinity (fresh to polyhaline). Across both timescales, CAR was lowest in disturbed pastures and highest in restored marshes, reflecting patterns in sediment accretion rates. Short-term CAR exceeded long-term CAR by approximately 50% on average and was only weakly correlated with long-term CAR, with differences among hydrogeomorphic setting. Short-term CAR was well predicted by summer inundation frequency and relative sediment load, together explaining 60% of variance, whereas long-term CAR was poorly predicted by contemporary environmental conditions. These findings highlight the importance of aligning predictor and response timescales when modeling blue carbon dynamics, and reinforce the climate mitigation potential of tidal wetland restoration.

land use and land cover change↗