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Low-energy enhancement of the magnetic dipole radiation in odd-mass lanthanides

We compute the magnetic dipole (M1) $\gamma$-ray strength functions ($\gamma$SF) for the odd-mass lanthanides $^{\textrm{143-151}}$Nd and $^{\textrm{147-153}}$Sm using the shell-model Monte Carlo method in combination with the static-path approximation and the maximum-entropy method. In particular, we quantify the statistical uncertainties in the calculated M1 $\gamma$SFs and show that they are under control for the excitation energies relevant to the experiments despite a Monte Carlo sign problem that originates in the projection onto an odd number of neutrons. We identify a low-energy enhancement (LEE) in the M1 $\gamma$SFs of these odd-mass lanthanides, which was recently observed experimentally in some of them. We also find a scissors mode resonance (SR) in the strongly deformed isotopes. We observe that the decrease in the LEE strength with neutron number along an isotopic chain is compensated for by an increase in the SR strength in the deformed nuclei. Furthermore, we compare our results with recent experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Electromagnetic Radiation from Cosmic-Ray Scatterings on Relic Neutrinos

Cosmic-ray scatterings on the cosmic neutrino background induce a flux of gamma-rays and X-rays from boosted meson decays and charged lepton processes. Here we present the first estimate of this flux and its cumulative cosmological contribution. Confronting expectations with Fermi-LAT diffuse gamma-ray data, we find a limit on the cosmic neutrino background overdensity at the level of $η\lesssim 2 \times 10^{4}$ for a lightest neutrino mass of $m_ν\gtrsim0.1$ eV, orders of magnitude stronger than current direct laboratory probes, and comparable to constraints on the cosmic neutrino background obtained with IceCube. We further show that X-ray synchrotron emission from cascade electron-positron pairs in intergalactic magnetic fields provides a complementary, albeit weaker, constraint. We discuss how anisotropic signatures and future gamma-ray data from CTA could further improve bounds on the relic neutrino overdensity, approaching in sensitivity the $Λ$CDM expected density.

Herrera, Gonzalo [MIT, MKI; Harvard U.] (ORCID:000↗

Angular Correlation Date Measurements with the GeRMAC system

Advanced modeling and simulation efforts have improved at Idaho National Laboratory in recent years with a solid foundation of experimental results. Current computational methods represent significant modeling capabilities but are limited by the accuracy and availability of nuclear data. The creation of pre- and post-processing software tools to address these limitations is fundamental to the improvement of nuclear science modeling capacities. One aspect of predictive modeling tools deals with gamma-rays emitted from radionuclides, including fissile or fissionable material, fission products, or activation products, produced in reactor experiments or other neutron environments. The resulting radionuclides decay in unique ways, providing complications upon measurement as a result of random and cascade, or true, coincidence summing. These effects are not easily quantified during modeling efforts of gamma-ray source terms., The germanium rotational measurements for angular correlation (GeRMAC) system was built to quantify the relative angles for gamma rays emitted by radionuclides of interest to investigate true coincidence, or cascade, summing as well as the nuclear energy levels of decay schemes of interest. Proof of concept studies utilize a series of laboratory check sources to provide validity, and it will soon be used to perform the same measurements for fission products of interest. The resulting data can be used to implement into a Monte Carlo code, such as Geant4, to provide more precise gamma-ray source terms following irradiations of materials.

73 - NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Searching for velocity-dependent dark matter annihilation signals from extragalactic halos

For this work, we consider gamma-ray signals of dark matter annihilation in extragalactic halos in the case where dark matter annihilates from a p-wave or d-wave state. In these scenarios, signals from extragalactic halos are enhanced relative to other targets, such as the Galactic Center or dwarf spheroidal galaxies, because the typical relative speed of the dark matter is larger in extragalactic halos. We perform a mock data analysis of gamma rays produced by dark matter annihilation in halos detected by the Sloan Digital Sky Survey. We include a model for uncorrelated galactic and extragalactic gamma ray backgrounds, as well as a simple model for backgrounds due to astrophysical processes in the extragalactic halos detected by the survey. We find that, for models which are still allowed by other gamma ray searches, searches of extragalactic halos with the current Fermi exposure can produce evidence for dark matter annihilation, though it is difficult to distinguish the p-wave and d-wave scenarios. With a factor 10x larger exposure, though, discrimination of the velocity-dependence is possible.

79 ASTRONOMY AND ASTROPHYSICS↗

Simple and Scalable Streaming: The GRETA Data Pipeline

The Gamma Ray Energy Tracking Array (GRETA) is a state of the art gamma-ray spectrometer being built at Lawrence Berkeley National Laboratory to be first sited at the Facility for Rare Isotope Beams (FRIB) at Michigan State University. A key design requirement for the spectrometer is to perform gamma-ray tracking in near real time. To meet this requirement we have used an inline, streaming approach to signal processing in the GRETA data acquisition system, using a GPU-equipped computing cluster. The data stream will reach 480 thousand events per second at an aggregate data rate of 4 gigabytes per second at full design capacity. We have been able to simplify the architecture of the streaming system greatly by interfacing the FPGA-based detector electronics with the computing cluster using standard network technology. A set of highperformance software components to implement queuing, flow control, event processing and event building have been developed, all in a streaming environment which matches detector performance. Prototypes of all high-performance components have been completed and meet design specifications.

Cromaz, Mario↗

Simulated Performance of the Micro-Pocket Fission Detector in the Advanced Test Reactor Critical Facility

The Micro-Pocket Fission Detector (MPFD) is a small-form–factor real-time fission chamber. MPFD performance has been simulated in the Advanced Test Reactor Critical Facility (ATRC), located at Idaho National Laboratory (INL). Here, the neutron and gamma-ray flux profiles and magnitudes were simulated using Monte Carlo N-Particle (MCNP) in the near-core B-8 irradiation position. These simulations were performed at 69 discrete axial locations inside the B-8 position for three separate orientations of the nearby hafnium outer shim control cylinders and at a power level of 700 Wth. The resulting neutron and gamma-ray flux values were used to determine the MPFD response for various fissile masses and detector gas pressures. The optimal gas-operating pressure was determined to be between 30 and 60 psig. The required fissile-layer mass was determined to be between 1–2 µg of 235 U. Additionally, the gamma-ray to fission-fragment interaction rate was determined to be 4.42 × 10 -3 with average energy deposition for gamma rays and fission fragments in 30 psig argon gas to be 1 keV and 9.5 MeV, respectively.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Neutrino point source searches for dark matter spikes

Any dark matter spikes surrounding black holes in our Galaxy are sites of significant dark matter annihilation, leading to a potentially detectable neutrino signal. In this paper we examine 10-10 5 M ⊙ black holes associated with dark matter spikes that formed in early minihalos and still exist in our Milky Way Galaxy today, in light of neutrino data from the ANTARES and IceCube detectors. In various regions of the sky, we determine the minimum distance away from the solar system that a dark matter spike must be in order to have not been detected as a neutrino point source for a variety of representative dark matter annihilation channels. Given these constraints on the distribution of dark matter spikes in the Galaxy, we place significant limits on the formation of the first generation of stars in early minihalos — stronger than previous limits from gamma-ray searches in Fermi Gamma-Ray Space Telescope data. The larger black holes considered in this paper may arise as the remnants of Dark Stars after the dark matter fuel is exhausted; thus neutrino observations may be used to constrain the properties of Dark Stars. The limits are particularly strong for heavier WIMPs. For WIMP masses ~ 5TeV, we show that ≲ 10 % of minihalos can host first stars that collapse into BHs larger than 10 3 M ⊙ .

79 ASTRONOMY AND ASTROPHYSICS↗

Isotopic Analysis using FRAM [Slides]

FRAM is an isotopic analysis code nominally designed for plutonium and uranium. It stands for Fixed-energy Response-function Analysis with Multiple efficiencies. It has self-calibration using several gamma-ray peaks and can analyze gamma ray data from 30keV to >1MeV of HPGe, CdTe, or LaBr3 detector. The key difference between the MGA family of codes (from LLNL) and FRAM is the use of user-editable analysis parameters in the latter.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Progress Towards Microcalorimeter Gamma Spectroscopy Analysis for Nuclear Fuel Separations

The High Efficiency and Resolution Microcalorimeter Spectrometer, 400 pixels (HERMES-400) is an ultra-high resolution gamma-ray spectrometer at Idaho National Laboratory’s Materials and Fuels Complex. HERMES-400 is intended to enable precise nondestructive analysis of advanced fuel cycle materials. Key upgrades and repairs of the instrument were performed this year to improve performance. First, the fourth and final microcalorimeter detector module was installed, meeting the milestone for its integration into the system. Operation with all four modules enables higher detector efficiency than any previous microcalorimeter gamma-ray system. Second, a thinner magnetic shield was installed. This shields the sensitive microcalorimeter pixels from stray magnetic fields while allowing transmission of lower-energy gamma rays, which are important to isotopic analysis. Finally, the cryostat, which provides cooling of the modules to their operating temperature, was found to have a helium coolant leak, which was repaired. HERMES-400 is in a stable state to perform repeated, long-term gamma-ray measurements with good detector efficiency and energy resolution. In FY25, irradiated TRISO fuel and salts from advanced electrochemical recycling techniques are candidates for microcalorimeter measurements. A final upgrade of the magnetic shielding and vibration damping of the system is also planned to maximize the system performance.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

The Mini Astrophysical MeV Background Observatory (MAMBO) CubeSat mission

The origin of the cosmic diffuse gamma-ray (CDG) background in the 0.3 – 30 MeV energy range is a mystery that has persisted for over 40 years. The Mini Astrophysical MeV Background Observatory (MAMBO) is a CubeSat mission concept motivated by the fact that, since the MeV CDG is relatively bright, only a small detector is required to make highquality measurements of it. Indeed, the sensitivity of space-based gamma-ray instruments to the CDG is limited not by size, but by the locally generated instrumental background produced by interactions of energetic particles in spacecraft materials. Comparatively tiny CubeSat platforms provide a uniquely quiet environment relative to previous gamma-ray science missions. The MAMBO mission will provide the best measurements ever made of the MeV CDG spectrum and angular distribution, utilizing two key innovations: 1) low instrumental background on a 12U CubeSat platform; and 2) an innovative shielded spectrometer design that simultaneously measures signal and background. We describe the MAMBO instrument and mission concept in detail, including simulations and laboratory measurements demonstrating the key measurement concept.

Astronomy and astrophysics↗

Remote Radiation Sensing Using Aerial and Ground Platforms

Remote sensing of ionizing radiation has a significant role in waste management, nuclear material management and nonproliferation, and radiation safety. Robotic platforms can surpass the number of tasks that are achieved by humans. With this technique, the operator's radiation exposure can be decreased. Remote sensing allows for the evaluation and monitoring of radiological contamination. Gamma-ray and neutron sensors were integrated onto the robotic platforms. This approach allows for the radiation sensor data to be dynamically tracked and mapped thus enabling further analysis of the radiation flux in temporal and spatial domains. The goal is to complete scheduled tasks while the robot is being irradiated. To achieve this, electronic components must be shielded and radiation hardened. CZT Detector: Cadmium Zinc Telluride (CZT) detector technology has been a promising solution for gamma-ray and x-ray measurements. Detector data is transferred to the Odroid minicomputer that controls and powers the module via the USB. Robot Operating System (ROS) was utilized for data acquisition and data fusion. The Mariscotti method was employed for the spectrum analysis. A function was programmed in ROS for the automatic identification of photopeaks. CLYC Detector: A Cs{sub 2}LiYCl{sub 6}:Ce{sup 3+} (CLYC) detector was used for simultaneous medium-resolution gamma-ray measurements and neutron counting. A 2.54 cm diameter photomultiplier tube (PMT) was equipped with a high voltage supply and a miniature digitizer. Gamma-ray excitation: fast core-to-valence luminescence (CVL) with 1 ns decay constant, and prompt Ce{sup 3+} emission with 50 ns decay constant. Neutron excitation: slow cerium self-trapped excitation (Ce{sup 3+} STE), 1000 ns decay constant. Radiation Source Localization: Maximum Likelihood Estimation (MLE) and gradient-based methods were used to locate the position of a radiation source based on measured radiation intensities. Multi-Particle Transport Code FLUKA: Estimation of radiation damage of the electronic components is important in order to optimize the robot's operational time while it is irradiated. Displacement per atom (DPA) represents the radiation damage in materials exposed to the ionizing radiation. Various shielding layers of different thickness t were analyzed (< 5% statistical error). The model of the controller of the UAS was designed in FLUKA. Conclusion: CZT and CLYC detectors were integrated onto the robotic platforms. Radiation source localization and contour mapping using robotic platforms were studied. Functions for data analysis and fusion were developed in ROS. FLUKA code was utilized to analyze DPA values. Layers of low-density and high-density materials were used to shield the UAS electronics.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Measuring the neutrino-oxygen neutral current quasielastic cross section using the accelerator neutrino neutron interaction experiment

The Accelerator Neutrino Neutron Interaction Experiment (ANNIE) is a 26-ton gadolinium-doped water Cherenkov detector located on-axis to Fermilab’s Booster Neutrino Beam (BNB). ANNIE is uniquely positioned to perform high-statistics measurements of neutrino-nucleus interactions in water, benefiting from a large neutrino flux due to a short (100-meter) baseline. A central focus of ANNIE’s physics program is the measurement of both charged current (CC) and neutral current (NC) cross sections on water, including neutral current quasielastic (NCQE) and CC-inclusive channels. The NCQE measurement is particularly critical for constraining uncertainties in rare-event searches such as the Diffuse Supernova Neutrino Background (DSNB), where atmospheric $\nu$NCQE interactions constitute a significant and poorly constrained background. This dissertation presents a measurement of the flux-averaged neutrino-oxygen neutral current quasielastic ($\nu$NCQE) cross section using $2.573 \times 10^{20}$~POT of BNB exposure from the 2022 and 2023 beam years. The $\nu$NCQE interaction is identified through the primary $\gamma$-rays produced by nuclear de-excitation of the residual $^{15}$N$^*$ or $^{15}$O$^*$ nucleus following nucleon knockout from $^{16}$O. A dedicated Monte Carlo (MC) re-tuning campaign was conducted using an americium-beryllium (AmBe) calibration source, Michel electrons from stopped muons, and throughgoing dirt muons originating upstream of the detector. This multi-sample approach provided a wide-ranging $\mathcal{O}(\text{MeV})$--$\mathcal{O}(\text{GeV})$ dataset for tuning the simulated detector response, which was subsequently validated against AmBe neutron and Michel electron data for use in the $\nu$NCQE analysis. A dedicated laser calibration campaign was carried out to reduce timing uncertainties across the PMT system, enabling reconstruction of the BNB bunch substructure with sufficient resolution to serve as a background rejection tool. By selecting events in-time with individual neutrino bunches, beam-correlated $\nu$NCQE events are separated from diffuse and accelerator-induced backgrounds, notably skyshine neutrons and externally-originating events, that would otherwise dominate traditional charge-based selections within a small-scale, surface-level, short-baseline detector. A data-driven estimation of the skyshine neutron and external background rates was performed and incorporated into the systematic uncertainty budget. The flux-averaged $\nu$NCQE cross section on oxygen is measured to be $1.57 \pm 0.06\,(\text{stat.})$ $^{+0.91}_{-0.67}\,(\text{syst.})$ $\times 10^{-38}\ \text{cm}^{2}$. A full systematic budget is constructed by propagating uncertainties in the secondary hadronic interaction modeling, background cross section normalizations, detector response, neutrino flux, and the primary $\gamma$-ray emission probabilities from oxygen nuclear de-excitation. An idealized de-excitation model, constructed from existing measurements in the literature is developed to benchmark the predictions of the \textsc{GENIE} event generator. A comparison reveals that \textsc{GENIE} systematically overpredicts the primary $\gamma$-ray emission probability from oxygen de-excitation by a factor of $1.49\times$ for $E_\gamma > 6$~MeV and $3.07\times$ in the $3$--$6$~MeV band. This comparison motivates the dominant systematic uncertainty in this analysis, where a conservative uncertainty of $^{+39.9\%}_{-0\%}$ on the primary $\gamma$-ray signal prediction is assigned. The ANNIE result is consistent with and complementary to existing flux-averaged $\nu$NCQE cross section measurements from T2K and Super-Kamiokande, providing an independent measurement with a different detector, neutrino beam, and analysis methodology. Looking ahead, an upgrade to the ANNIE DAQ infrastructure enabling continuous extended readout will allow a complementary $\nu$NCQE neutron multiplicity measurement, directly relevant to constraining the NCQE background in DSNB searches, competitive with the recent T2K measurement at SK-Gd. The planned Super-SANDI upgrade, deploying a large Water-based Liquid Scintillator (WbLS) volume, will further extend ANNIE's reach to hadronic final states and exclusive NC channels, and enable joint measurements with liquid argon detectors sharing the BNB beamline ahead of DUNE and Hyper-Kamiokande.

Doran, Steven [Iowa State U.]↗

Combined dark matter search towards dwarf spheroidal galaxies with Fermi -LAT, HAWC, H.E.S.S., MAGIC, and VERITAS

Dwarf spheroidal galaxies (dSphs) are excellent targets for indirect dark matter (DM) searches using gamma-ray telescopes because they are thought to have high DM content and a low astrophysical background. The sensitivity of these searches is improved by combining the observations of dSphs made by different gamma-ray telescopes. We present the results of a combined search by the most sensitive currently operating gamma-ray telescopes, namely: the satellite-borne Fermi -LAT telescope; the ground-based imaging atmospheric Cherenkov telescope arrays H.E.S.S., MAGIC, and VERITAS; and the HAWC water Cherenkov detector. Individual datasets were analyzed using a common statistical approach. Results were subsequently combined via a global joint likelihood analysis. We obtain constraints on the velocity-weighted cross section 〈σv〉 for DM self-annihilation as a function of the DM particle mass. This five-instrument combination allows the derivation of up to 2-3 times more constraining upper limits on 〈σv〉 than the individual results over a wide mass range spanning from 5 GeV to 100 TeV. Depending on the DM content modeling, the 95% confidence level observed limits reach 1.5×10 -24 cm 3 s -1 and 3.2×10 -25 cm 3 s -1 , respectively, in the τ + τ - annihilation channel for a DM mass of 2 TeV.

79 ASTRONOMY AND ASTROPHYSICS↗

Detecting and characterizing special nuclear material for nuclear nonproliferation applications

Abstract There is an urgent need for new, better instrumentation and techniques for detecting and characterizing special nuclear material (SNM), i.e., highly enriched uranium and plutonium. The development of improved instruments and techniques requires experiments performed with the SNM itself, which is of limited availability. This paper describes the findings of experiments performed at the National Criticality Experiments Research Center conducted using new instruments and techniques on unclassified, kg-quantity SNM objects. These experiments, performed in the framework of the Department of Energy, National Nuclear Security Administration Consortium for Monitoring, Technology, and Verification, focused on detecting, characterizing, and localizing SNM samples with masses ranging from 3.3 to 13.8 kg, including plutonium and highly enriched uranium using prototype detectors and techniques. The work demonstrates SNM detection and characterization using recently-developed prototype detection systems. Specifically, we present new results in passive detection and imaging of plutonium and uranium objects using gamma-ray and dual particle (fast neutron and gamma-ray) imaging. We also present a new analysis of the delayed neutron emissions during active interrogation of uranium using a neutron generator.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Hazma: a python toolkit for studying indirect detection of sub-GeV dark matter

With several proposed MeV gamma-ray telescopes on the horizon, it is of paramount importance to perform accurate calculations of gamma-ray spectra expected from sub-GeV dark matter annihilation and decay. We present hazma, a python package for reliably computing these spectra, determining the resulting constraints from existing gamma-ray data, and prospects for upcoming telescopes. For high-level analyses, hazma comes with several built-in dark matter models where the interactions between dark matter and hadrons have been determined in detail using chiral perturbation theory. Additionally, hazma provides tools for computing spectra from individual final states with arbitrary numbers of light leptons and mesons, and for analyzing custom dark matter models. hazma can also produce electron and positron spectra from dark matter annihilation, enabling precise derivation of constraints from the cosmic microwave background

79 ASTRONOMY AND ASTROPHYSICS↗

Ultra-low-level measurements of airborne fission products from the Fukushima Daiichi reactor accident using high volume collection systems at Savannah River National Laboratory

For this study, ultra-low-level measurements of radionuclides in air have been conducted at the Savannah River National Laboratory (SRNL) to determine the atmospheric concentration of fission products released following the Fukushima Daiichi reactor accident on March 11, 2011. Air filter samples were acquired from two high-volume collection systems (a traditional filter-based system and an electrostatic precipitator-based system) to monitor airborne radionuclide concentrations in the period covering from 2 weeks to 3 years after the disaster. The world-wide spread of low-level concentrations of airborne fission products from the Fukushima event provided a unique opportunity to demonstrate SRNL's electrostatic particle collection technology and other improvements in environmental monitoring developed at the Savannah River Site (SRS). Detecting and analyzing the release allowed a comprehensive test of SRS systems for monitoring environmental radioactivity. Gamma-ray-emitting fission products ( 131,132 I, 134,136,137 Cs, and 129,132 Te) and cosmogenic isotopes ( 7 Be and 22 Na) in air were detected and quantified by high-resolution gamma-ray spectroscopy at concentrations as low as 0.07 μBq per standard cubic meter (SCM) (50 mBq total 137 Cs), while plutonium content was quantified by thermal ionization mass spectrometry (TIMS) at concentrations as low as 6.5 × 10 –21 g/SCM (3.0 fg 239+240 Pu). Isotope concentrations measured at SRNL from gamma-ray spectroscopy were compared to independent measurements from Chapel Hill, NC, located approximately 370 km (230 mi) NE of SRNL. Meteorological modeling was also used to predict radionuclide transport from the location of release to both measurement locations.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗

Inline gamma-spectrometry of fission product elements after rapid high-pressure ion chromatographic separation

Analysis of irradiated material shortly after irradiation can be non-trivial due to highly radioactive activation and fission isotopes increasing dead time in gamma-ray detection systems, often requiring a “cooling-period” between receipt of a sample and the subsequent analysis. A direct separation–detection method has been developed combining ion chromatography and inductively coupled mass spectrometry for rapid, low-level analysis of fission products; it cannot, however, detect certain short-lived species below the detection limit of the system. In this paper we report the implementation of an inline gamma-ray detector, which was added post-separation, pre-analysis, to test the quality and utility of elementally-isolated gamma-ray spectroscopy.

Inline gamma-ray detection↗

Recommended Nuclear Structure and Decay Data for A = 200 Isobars

Evaluated nuclear structure and decay data for all nuclei with mass number A = 200 ( 200 Os, 200 Ir, 200 Pt, 200 Au, 200 Hg, 200 Tl, 200 Pb, 200 Bi, 200 Po, 200 At, 200 Rn, and 200 Fr), are presented. All available experimental data are compiled and evaluated, and best values for level and gamma-ray energies, quantum numbers, lifetimes, gamma-ray intensities and transition probabilities, as well as other nuclear properties, are recommended. Inconsistencies and discrepancies that exist in the literature are discussed. A number of computer codes (https://www-nds.iaea.org/public/ensdf pgm/) developed by members of the NSDD network were used during the evaluation process. In conclusion, this work supersedes the earlier evaluation by F.G. Kondev and S. Lalkovski (2007Ko42), published in Nuclear Data Sheets 108, 1471 (2007).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗