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At least 577 records · Page 32

Dependence of marine stratocumulus reflectivities on liquid water paths

Simple parameterizations that relate cloud liquid water content to cloud reflectivity are often used in general circulation climate models to calculate the effect of clouds in the earth's energy budget. Such parameterizations have been developed by Stephens (1978) and by Slingo and Schrecker (1982) and others. Here researchers seek to verify the parametric relationship through the use of simultaneous observations of cloud liquid water content and cloud reflectivity. The column amount of cloud liquid was measured using a microwave radiometer on San Nicolas Island following techniques described by Hogg et al., (1983). Cloud reflectivity was obtained through spatial coherence analysis of Advanced Very High Resolution Radiometer (AVHRR) imagery data (Coakley and Beckner, 1988). They present the dependence of the observed reflectivity on the observed liquid water path. They also compare this empirical relationship with that proposed by Stephens (1978). Researchers found that by taking clouds to be isotropic reflectors, the observed reflectivities and observed column amounts of cloud liquid water are related in a manner that is consistent with simple parameterizations often used in general circulation climate models to determine the effect of clouds on the earth's radiation budget. Attempts to use the results of radiative transfer calculations to correct for the anisotropy of the AVHRR derived reflectivities resulted in a greater scatter of the points about the relationship expected between liquid water path and reflectivity. The anisotropy of the observed reflectivities proved to be small, much smaller than indicated by theory. To critically assess parameterizations, more simultaneous observations of cloud liquid water and cloud reflectivities and better calibration of the AVHRR sensors are needed.

Coakley, James A., Jr.↗

STS-53 Space Shuttle mission report

The STS-53 Space Shuttle Program Mission Report provides a summary of the Orbiter, External Tank (ET), Solid Rocket Booster/Redesigned Solid Rocket Motor (SRB/RSRM), and the Space Shuttle Main Engine (SSME) subsystems performance during the fifty-second flight of the Space Shuttle Program, and the fifteenth flight of the Orbiter vehicle Discovery (OV-103). In addition to the Orbiter, the flight vehicle consisted of an ET, which was designated as ET-49/LWT-42; three SSME's, which were serial numbers 2024, 2012, and 2017 in positions 1, 2, and 3, respectively; and two SRB's, which were designated BI-055. The lightweight RSRM's that were installed in each SRB were designated 360L028A for the left SRB, and 360L028B for the right SRB. The primary objective of this flight was to successfully deploy the Department of Defense 1 (DOD-1) payload. The secondary objectives of this flight were to perform the operations required by the Glow Experiment/Cryogenic Heat Pipe Experiment Payload (GCP); the Hand-Held, Earth-Oriented, Real-Time, Cooperative, User-Friendly, Location-Targeting and Environmental System (HERCULES); the Space Tissue Loss (STL); the Battlefield Laser Acquisition Sensor Test (BLAST); the Radiation Monitoring Equipment-III (RME-III); the Microcapsules in Space-1 (MIS-1); the Visual Function Tester-2 (VFT-2); the Cosmic Radiation Effects and Activation Monitor (CREAM); the Clouds Logic to Optimize Use of Defense Systems-1A (CLOUDS-1A); the Fluids Acquisition and Resupply Experiment (FARE); and the Orbital Debris Radar Calibration Spheres (ODERACS). In addition to presenting a summary of subsystem performance, this report also discusses each Orbiter, ET, SSME, SRB, and RSRM in-flight anomaly in the applicable section of the report. Listed in the discussion of each anomaly is the officially assigned tracking number as published by each Project Office in their respective Problem Tracking List. All times given in this report are in Greenwich mean time (G.m.t.) as well as mission elapsed time (MET).

Fricke, Robert W., Jr.↗

Improvements of an ice-phase microphysics parameterization for use in numerical simulations of tropical convection

It is important to properly simulate the extent and ice water content of tropical anvil clouds in numerical models that explicitly include cloud formation because of the significant effects that these clouds have on the radiation budget. For this reason, a commonly used bulk ice-phase microphysics parameterization was modified to more realistically simulate some of the microphysical processes that occur in tropical anvil clouds. Cloud ice growth by the Bergeron process and the associated formation of snow were revised. The characteristics of graupel were also modified in accord with a previous study. Numerical simulations of a tropical squall line demonstrate that the amount of cloud ice and the extent of anvil clouds are increased to more realistic values by the first two changes.

Krueger, Steven K.↗

The MODIS Aerosol Algorithm: Critical Evaluation and Plans for Collection 6

For ten years the MODIS aerosol algorithm has been applied to measured MODIS radiances to produce a continuous set of aerosol products, over land and ocean. The MODIS aerosol products are widely used by the scientific and applied science communities for variety of purposes that span operational air quality forecasting in estimates o[ clear-sky direct radiative effects over ocean and aerosol-cloud interactions. The products undergo continual evaluation, including self-consistency checks and comparisons with highly accurate ground-based instruments. The result of these evaluation exercises is a quantitative understanding of the strengths and weaknesses of the retrieval, where and when the products are accurate and the situations where and when accuracy degrades. We intend 10 present results of the most recent critical evaluations including the first comparison of the over ocean products against the shipboard aerosol optical depth measurements of the Marine Aerosol Network (MAN), the demonstration of the lack of sensitivity to size parameter in the over land products and identification of residual problems and regional issues. While the current data set is undergoing evaluation, we are preparing for the next data processing, labeled Collection 6. Collection 6 will include transparent Quality Flags, a 3 km aerosol product and the 500m resolution cloud mask used within the aerosol n:bicvu|. These new products and adjustments to algorithm assumptions should provide users with more options and greater control, as they adapt the product for their own purposes.

Remer, Lorraine↗

Improved Determination of Surface and Atmospheric Temperatures Using Only Shortwave AIRS Channels

AIRS was launched on EOS Aqua on May 4, 2002, together with AMSU-A and HSB, to form a next generation polar orbiting infrared and microwave atmospheric sounding system. AIRS is a grating spectrometer with a number of linear arrays of detectors with each detector sensitive to outgoing radiation in a characteristic frequency v(sub i) with a spectral band pass delta v(sub i) of roughly v(sub i) /1200. AIRS contains 2378 spectral channels covering portions of the spectral region 650 cm(exp -1) (15.38 gm) - 2665 cm(exp -1)' (3.752 micrometers). These spectral regions contain significant absorption features from two CO2 absorption bands, the 15 micrometer (longwave) CO2 band, and the 4.3 micrometer (shortwave) CO, absorption band. There are also two atmospheric window regions, the 12 micrometerm - 8 micrometer (longwave) window, and the 4.17 micrometer - 3.75 micrometer (shortwave) window. Historically, determination of surface and atmospheric temperatures from satellite observations was performed using primarily observations in the longwave window and CO2 absorption regions. One reason for this was concerns about the effects, during the day, of reflected sunlight and non-Local Thermodynamic Equilibrium (non-LTE) on the observed radiances in the shortwave portion of the spectrum. According to cloud clearing theory, more accurate soundings of both surface skin and atmospheric temperatures can be obtained under partial cloud cover conditions if one uses the longwave channels to determine cloud cleared radiances R(sub i) for all channels, and uses R(sub i) only from shortwave channels in the determination of surface and atmospheric temperatures. This procedure is now being used by the AIRS Science Team in preparation for the AIRS Version 6 Retrieval Algorithm. This paper describes how the effects on the radiances of solar radiation reflected by clouds and the Earth's surface, and also of non-LTE, are accounted for in the analysis of the data. Results are presented for both daytime and nighttime conditions showing improved surface and atmospheric soundings under partial cloud cover resulted from not using R(sub i) in the retrieval process for any longwave channels sensitive to cloud effects. This improvement is made possible because AIRS NEDT in the shortwave portion of the spectrum is extremely low.

Susskind,Joel↗

Optimizing energy yield of monolithic perovskite/silicon tandem solar cells in real-world Conditions: The impact of luminescent coupling

Efficient light management is key to maximizing power conversion efficiency (PCE) in monolithic perovskite/silicon tandem solar cells. Achieving peak efficiency requires closely matched current generation in all junctions, especially in integrated configurations. However, real-world conditions vary significantly due to factors such as sunlight spectrum, diffuse-to-direct sunlight ratio, angular distribution of light, subcell temperature coefficients, and ground reflection. This study introduces a comprehensive optical and device simulation to optimize perovskite/silicon tandem cells, considering experimental luminescent coupling (LC) efficiency and its dependence on working conditions, alongside variations in radiative recombination, effect of temperature on absorptivity spectra, and cloud cover. Our results show potential energy yield improvements of up to 1.4 % with LC, based on current perovskite radiative recombination records, and up to 4 % with direct bandgap materials. Although radiative recombination's dependence on excitation intensity reduces output power and requires thicker absorbers, LC compensates for these losses. LC also lowers the optimized bandgap for the perovskite top cell from 1.72 eV to 1.64–1.68 eV, or even lower in regions with redshifted irradiance. Additionally, optimization revealed that thinner silicon bottom cells require a higher perovskite top cell bandgap, impacting the balance between fabrication cost and cell stability.

14 SOLAR ENERGY↗

Radiative properties of cirrus clouds inferred from broadband measurements during FIRE

It is well known that clouds are significant modulators of weather and climate because of their effects on the radiation field and thus on the energy balance of the earth atmosphere system. As a result, the accurate prediction of weather and climate depends to a significant degree on the accuracy with which cloud radiation interactions can be described. The broadband radiative and microphysical properties of five cirrus cloud systems are reported, as observed from the NCAR Sabreliner during the FIRE first Cirrus IFO, in order to better understand cirrus cloud-radiation interactions. A broadband infrared (BBIR) radiative transfer model is used to deduce BBIR absorption coefficients in order to assess the impact of the cirrus clouds on infrared radiation. The relationships of these absorption coefficients to temperature and microphysical characteristics are explored.

Smith, William L., Jr.↗

Influence of Aerosol Embedded in Shallow Cumulus Cloud Fields on the Surface Solar Irradiance

Ubiquitous shallow cumulus clouds are associated with complex variability in surface solar irradiance (SSI). Aerosol embedded in the cloud field typically has a much smaller overall radiative effect, but can significantly perturb the shape of the SSI probability density function (PDF). These perturbations have important implications for several applications that utilize SSI, but are poorly quantified and are the subject of this study. Multiple cases of shallow cumulus cloud fields with embedded aerosol are simulated at the Southern Great Plains Atmospheric Observatory using large eddy simulation (LES). The LES-derived cloud and aerosol fields are then ingested into Monte Carlo three-dimensional (3D) radiative transfer to simulate SSI. We find a variety of perturbations to the SSI PDF that depend on aerosol presence and optical properties. The processes leading to these perturbations include extinction of the direct beam that often increases from the clear-sky region toward cloud edge due to aerosol hygroscopic growth, and scattering of radiation by aerosol into cloud shadows. The ability to predict the SSI PDF in the presence of aerosol is assessed by adding three representative aerosol optical properties into an existing machine learning framework. We show that machine learning accurately predicts the SSI PDF across a wide range of conditions with negligible computational expense. Importance metrics reveal the relatively high influence of aerosol optical properties in making the predictions. These new findings highlight the important role that aerosol plays in SSI variability for highly 3D cloud-aerosol environments and provides a computationally efficient route forward for its simulation.

3D radiative transfer↗

Cloud adjustments from large-scale smoke–circulation interactions strongly modulate the southeastern Atlantic stratocumulus-to-cumulus transition

Smoke from southern Africa blankets the southeastern Atlantic Ocean from June to October, producing strong and competing aerosol radiative effects. Smoke effects on the transition between overcast stratocumulus and scattered cumulus clouds are investigated along a Lagrangian (air-mass-following) trajectory in regional climate and large eddy simulation models. Results are compared with observations from three recent field campaigns that took place in August 2017: ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES), CLouds and Aerosol Radiative Impacts and Forcing: Year 2017 (CLARIFY), and Layered Atlantic Smoke Interactions with Clouds (LASIC). The case study is set up around the joint ORACLES–CLARIFY flight that took place near Ascension Island on 18 August 2017. Smoke sampled upstream on an ORACLES flight on 15 August 2017 likely entrained into the marine boundary layer later sampled during the joint flight. The case is first simulated with the WRF-CAM5 regional climate model in three distinct setups: (1) FireOn, in which smoke emissions and any resulting smoke–cloud–radiation interactions are included; (2) FireOff, in which no smoke emissions are included; (3) RadOff, in which smoke emissions and their microphysical effects are included but aerosol does not interact directly with radiation. Over the course of the Lagrangian trajectory, differences in free tropospheric thermodynamic properties between FireOn and FireOff are nearly identical to those between FireOn and RadOff, showing that aerosol–radiation interactions are primarily responsible for the free tropospheric effects. These effects are non-intuitive: in addition to the expected heating within the core of the smoke plume, there is also a “banding” effect of cooler temperature (~1–2 K) and greatly enhanced moisture (>2 g kg -1 ) at the plume top. This banding effect is caused by a vertical displacement of the former continental boundary layer in the free troposphere in the FireOn simulation resulting from anomalous diabatic heating due to smoke absorption of sunlight that manifests primarily as a few hundred meters per day reduction in large-scale subsidence over the ocean. A large eddy simulation (LES) is then forced with free tropospheric fields taken from the outputs for the WRF-CAM5 FireOn and FireOff runs. Cases are run by selectively perturbing one variable (e.g., aerosol number concentration, temperature, moisture, vertical velocity) at a time to better understand the contributions from different indirect (microphysical), “large-scale” semi-direct (above-cloud thermodynamic and subsidence changes), and “local” semi-direct (below-cloud smoke absorption) effects. Despite a more than 5-fold increase in cloud droplet number concentration when including smoke aerosol concentrations, minimal differences in cloud fraction evolution are simulated by the LES when comparing the base case with a perturbed aerosol case with identical thermodynamic and dynamic forcings. A factor of 2 decrease in background free tropospheric aerosol concentrations from the FireOff simulation shifts the cloud evolution from a classical entrainment-driven “deepening–warming” transition to trade cumulus to a precipitation-driven “drizzle-depletion” transition to open cells, however. The thermodynamic and dynamic changes caused by the WRF-simulated large-scale adjustments to smoke diabatic heating strongly influence cloud evolution in terms of both the rate of deepening (especially for changes in the inversion temperature jump and in subsidence) and in cloud fraction on the final day of the simulation (especially for the moisture “banding” effect). Such large-scale semi-direct effects would not have been possible to simulate using a small-domain LES model alone.

54 ENVIRONMENTAL SCIENCES↗

The Influence of Thermodynamic Phase on the Retrieval of Mixed-Phase Cloud Microphysical and Optical Properties in the Visible and Near Infrared Region

Cloud microphysical and optical properties are inferred from the bidirectional reflectances simulated for a single-layered cloud consisting of an external mixture of ice particles and liquid droplets. The reflectances are calculated with a rigorous discrete ordinates radiative transfer model and are functions of the cloud effective particle size, the cloud optical thickness, and the values of the ice fraction in the cloud (i.e., the ratio of ice water content to total water content). In the present light scattering and radiative transfer simulations, the ice fraction is assumed to be vertically homogeneous; the habit (shape) percentage as a function of ice particle size is consistent with that used for the Moderate Resolution Imaging Spectroradiometer (MODIS) operational (Collection 4 and earlier) cloud products; and the surface is assumed to be Lambertian with an albedo of 0.03. Furthermore, error analyses pertaining to the inference of the effective particle sizes and optical thicknesses of mixed-phase clouds are performed. Errors are calculated with respect to the assumption of a cloud containing solely liquid or ice phase particles. The analyses suggest that the effective particle size inferred for a mixed-phase cloud can be underestimated (or overestimated) if pure liquid phase (or pure ice phase) is assumed for the cloud, whereas the corresponding cloud optical thickness can be overestimated (or underestimated).

Lee, Joonsuk↗

Study of the consistency of climatological products of Nimbus-7

The study, in addition to investigating the consistency of climatological products from Nimbus-7 Earth Radiation Budget and Temperature Humidity Infrared Radiometer experiments, focussed on the climatological analysis of the specified regions of the Earth. The climatological study consisted of the effects of various types of clouds on the net radiation, albedos, and emitted radiation. In addition to a correlational study for determining consistency level of data, a population study of the regions was formulated and conducted. The regions under this study were formed by clustering the target areas using the criteria of climatological conditions such as geography, ocean, and land. Research is limited to tropics from 18 deg north to 18 deg south. A correlational study indicates that there is high positive correlation between high clouds and albedo, and a reduced negative correlation between albedo and net radiation.

Dhuria, Harbans L.↗

Seasonality and Albedo Dependence of Cloud Radiative Forcing in the Upper Colorado River Basin

Mountains create and enhance their own clouds, which both scatter and absorb shortwave radiation from the sun and absorb and re-emit land surface and atmospheric longwave radiation. However, the impacts of clouds on the surface radiation balance in high elevation snowy mountain terrain are poorly explored. In this study, we use data collected by the SAIL field campaign and partner organizations in the upper elevations (2,880 m.a.s.l) of the Upper Colorado River Basin (UCRB) over a 21-month period from September 2021 to June 2023 to estimate Cloud Radiative Forcing (CRF) in the shortwave, longwave, and the net effect. Longwave warming effects dominate during the winter when snow albedos are high (0.8–0.9) and the background atmospheric precipitable water vapor is low (<0.5 cm), yielding a maximum monthly average net CRF of +34.7 W·m -2 , meaning that clouds increase the net radiation relative to clear skies during this time period. The sign of net CRF switches in the warm season as snow recedes, sun-angles increase, and the North American monsoon arrives, yielding a minimum monthly average net CRF of -47.6 W·m -2 with hourly minima of -600 W·m -2 . The sign of net CRF is typically positive, even at solar noon, when the surface is snow covered, except for a brief period over melting, low-albedo snow (0.5–0.6) impacted by dust impurities. Sensitivity tests elucidate the role of the surface albedo on the net CRF. The results suggest that net CRF will increase in magnitude and lead to a more persistent cooling effect on the surface net radiation budget as the snow cover declines.

54 ENVIRONMENTAL SCIENCES↗

Microwave radiative transfer through horizontally inhomogeneous precipitating clouds

Recent advances in cloud microphysical models have led to realistic three-dimensional distributions of cloud constituents. Radiative transfer schemes can make use of this detailed knowledge in order to study the effects of horizontal as well as vertical inhomogeneities within clouds. This study looks specifically at the differences between three-dimensional radiative transfer results and those obtained by plane parallel, independent pixel approximations in the microwave spectrum. A three-dimensional discrete ordinates method as well as a backward Monte Carlo method are used to calculate realistic radiances emerging from the cloud. Analyses between these models and independent pixel approximations reveal that plane parallel approximations introduce two distinct types of errors. The first error is physical in nature and is related to the fact that plane parallel approximations do not allow energy to leak out of dense areas into surrouding areas. In general, it was found that these errors are quite small for emission-dominated frequencies (37 GHz and lower) and that physical errors are highly pronounced only at scattering frequencies (85 GHz) where large deviations and biases up to 8 K averaged over the entire cloud were found. The second error is more geometric in nature and is related to the fact that plane parallel approximations cannot accommodate physical boundaries in the horizontal dimension for off-nadir viewing angles. The geometric errors were comparable in magnitude for all frequencies. Their magnitude, however, depends on a number of factors including the scheme used to deal with the edge, the nature of the surface, and the viewing angle.

Roberti, Laura↗

Sensitivity of Multispectral Imager Liquid Water Cloud Microphysical Retrievals to the Index of Refraction

A cloud property retrieved from multispectral imagers having spectral channels in the shortwave infrared (SWIR) and/or midwave infrared (MWIR) is the effective particle radius (CER), a radiatively relevant weighting of the cloud particle size distribution. The physical basis of the CER retrieval is the dependence of SWIR/MWIR cloud reflectance on the cloud particle single scattering absorption, which in turn depends on the complex index of refraction of bulk liquid water (or ice) in addition to the cloud particle size. There is a general consistency in the choice of the liquid water index of refraction by the cloud remote sensing community, largely due to the few available independent datasets and compilations. Here we examine the sensitivity of CER retrievals to the available laboratory index of refraction datasets in the SWIR and MWIR using the retrieval software package that produces NASA’s standard MODIS/VIIRS continuity cloud products. The sensitivity study incorporates two laboratory index of refraction datasets that include measurements at supercooled water temperatures, one in the SWIR [Kou et al., 1993] and one in the MWIR [Wagner et al., 2005]. Neither has been broadly utilized in the cloud remote sensing community. It is shown that these two new datasets can significantly change CER retrievals (e.g., 1-2 μm) relative to common datasets used by the community. Further, index of refraction data for a 265 K water temperature results in more consistent retrievals between the two spectrally distinct 2.2 μm atmospheric window channels on MODIS and VIIRS. As a result, the 265 K values from the SWIR and MWIR index of refraction datasets were adopted for use in the production version of the continuity cloud product. The results indicate the need to better understand temperature-dependent bulk water absorption and uncertainties in these spectral regions.

MODIS↗

Aircraft-Measured Indirect Cloud Effects from Biomass Burning Smoke in the Arctic and Subarctic

The incidence of wildfires in the Arctic and subarctic is increasing; in boreal North America, for example, the burned area is expected to increase by 200-300% over the next 50-100 years, which previous studies suggest could have a large effect on cloud microphysics, lifetime, albedo, and precipitation. However, the interactions between smoke particles and clouds remain poorly quantified due to confounding meteorological influences and remote sensing limitations. Here, we use data from several aircraft campaigns in the Arctic and subarctic to explore cloud microphysics in liquid-phase clouds influenced by biomass burning. Median cloud droplet radii in smoky clouds were approx. 40- 60% smaller than in background clouds. Based on the relationship between cloud droplet number (N(liq)/ and various biomass burning tracers (BBt/ across the multi-campaign data set, we calculated the magnitude of subarctic and Arctic smoke aerosol-cloud interactions (ACIs, where ACI = (1/3) x dln(N(liq))/dln(BBt)) to be approx. 0.16 out of a maximum possible value of 0.33 that would be obtained if all aerosols were to nucleate cloud droplets. Interestingly, in a separate subarctic case study with low liquid water content (0.02 gm/cu m and very high aerosol concentrations (2000- 3000/ cu cm in the most polluted clouds, the estimated ACI value was only 0.05. In this case, competition for water vapor by the high concentration of cloud condensation nuclei (CCN) strongly limited the formation of droplets and reduced the cloud albedo effect, which highlights the importance of cloud feedbacks across scales. Using our calculated ACI values, we estimate that the smoke-driven cloud albedo effect may decrease local summertime short-wave radiative flux by between 2 and 4 W/sq m or more under some low and homogeneous cloud cover conditions in the subarctic, although the changes should be smaller in high surface albedo regions of the Arctic.We lastly explore evidence suggesting that numerous northern-latitude background Aitken particles can interact with combustion particles, perhaps impacting their properties as cloud condensation and ice nuclei.

cloud microphysics↗

Planning for the utilization of the PCDS in studying the interaction of clouds (ISCCP-C data) and the Earth radiation budget (ERBE data)

The Pilot Climate Data System (PCDS) affords an opportunity to analyze data from different but highly complementary data sets. Two of these highly complementary data sets supported by the PCDS are the International Satellite Cloud Climatology Project (ISCCP) and the Earth Radiation Budget Experiment (ERBE). Both data set sponsors are aware of the utility of one data set to the other, and both projects utilize gridded data on a 2.5 deg by 2.5 deg grid. The ISCCP data have been collected since July 1983, and the NOAA-9 data for ERBE have been collected for more than a year. Therefore, there is a good chance to use these temporally overlapping data sets to investigate hypothesized relationships. Changes in cloudiness affect both cloud albedo feedback (shortwave) and the greenhouse effect (longwave). The relative importance of the effects of clouds on albedo versus outgoing longwave radiation (OLR) in determining the radiation balance has long been a matter of controversy. Now, however, changes in cloud amount as observed by the ISCCPO can be correlated to corresponding changes in the albedo and changes in the OLR from ERBE. Monthly means can be utilized in all instances.

Jacobowitz, H.↗

Cloud, Aerosol, and Radiative Properties Over the Western North Atlantic Ocean

This study examines the atmospheric properties of weather states (WSs) derived from the International Satellite Cloud Climatology Project (ISCCP) over the Western North Atlantic Ocean. In particular, radiation and aerosol data corresponding to two sites in the study domain, Pennsylvania State University and Bermuda, were examined to characterize the atmospheric properties of the various satellite-derived WSs. At both sites, the fair weather WS was most prevalent, followed by the cirrus WS. Differences in the seasonality of the various WSs were observed at the two sites. Fractional sky cover and effective shortwave cloud transmissivity derived from ground-based radiation measurements were able to capture differences among the satellite-derived WSs. Speciated aerosol optical thicknesses (AOT) from the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) were used to investigate potential differences in aerosol properties among the WSs. The clear sky WS exhibited below-average seasonal values of AOT at both sites year-round, as well as relatively high rates of occurrence with low AOT events. In addition, the clear sky WS showed above-average contributions from dust and black carbon to the total AOT year-round. Finally, transitions between various WSs were examined under low, high, and mid-range AOT conditions. The most common pathway was for the WSs to remain in the same state after a 3 hr interval. Some WSs, such as midlatitude storms, deep convection, middle top, and shallow cumulus, were more prevalent as ending states under high AOT conditions. This work motivates examining differences in aerosol properties between WSs in other regions.

54 ENVIRONMENTAL SCIENCES↗