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At least 577 records · Page 32

Moiré trions in MoSe 2 /WSe 2 heterobilayers

Transition metal dichalcogenide moiré bilayers with spatially periodic potentials have emerged as a highly tunable platform for studying both electronic and excitonic phenomena. The power of these systems lies in the combination of strong Coulomb interactions with the capability of controlling the charge number in a moiré potential trap. Electronically, exotic charge orders at both integer and fractional fillings have been discovered. However, the impact of charging effects on excitons trapped in moiré potentials is poorly understood. Here, we report the observation of moiré trions and their doping-dependent photoluminescence polarization in H-stacked MoSe 2 /WSe 2 heterobilayers. We find that as moiré traps are filled with either electrons or holes, new sets of interlayer exciton photoluminescence peaks with narrow linewidths emerge about 7 meV below the energy of the neutral moiré excitons. Circularly polarized photoluminescence reveals switching from co-circular to cross-circular polarizations as moiré excitons go from being negatively charged and neutral to positively charged. Furthermore, this switching results from the competition between valley-flip and spin-flip energy relaxation pathways of photo-excited electrons during interlayer trion formation. Our results offer a starting point for engineering both bosonic and fermionic many-body effects based on moiré excitons.

36 MATERIALS SCIENCE↗

Energetic charged-particle phenomena in the Jovian magnetosphere - First results from the Ulysses COSPIN collaboration

The Ulysses spacecraft made the first exploration of the region of Jupiter's magnetosphere at high Jovigraphic latitudes on the dusk side and reached higher magnetic latitudes on the day side than any previous mission to Jupiter. The cosmic and solar particle investigations (COSPIN) instrumentation achieved a remarkably well integrated set of observations of energetic charged particles in the energy ranges of about 1 to 170 megaelectron volts for electrons and 0.3 to 20 megaelectron volts for protons and heavier nuclei. The new findings include an apparent polar cap region in the northern hemisphere in which energetic charged particles following Jovian magnetic field lines may have direct access to the interplanetary medium; high-energy electron bursts on the dusk side that are apparently associated with field-aligned currents and radio burst emissions; persistence of the global 10-hour relativistic electron 'clock' phenomenon throughout Jupiter's magnetosphere; on the basis of charged-particle measurements, apparent dragging of magnetic field lines at large radii in the dusk sector toward the tail; and consistent outflow of megaelectron volt electrons and large-scale departures from corotation for nucleons.

Simpson, J. A.↗

Fingerprinting fractons with pump-probe spectroscopy

We demonstrate how pump-probe techniques enable specific spectroscopic diagnostics of fracton phases of matter by studying lineon-planon braiding in the paradigmatic X-cube model. Our discussion builds on previous works probing anyonic exchange statistics in conventional spin liquids, but the extension to fracton phases reveals qualitatively different phenomena due to the restricted mobility of fractionalized excitations. A key feature is that nearby planons can form an emergent bound state by accessing different planes via alternative pairing configurations. We show that this bound state qualitatively modifies the long-time linear and nonlinear responses, leading to an asymptotic linear-in-𝑡 behavior for the pump-probe signal 𝜒 𝑍𝑍𝑋 . By contrast, swapping the pump and probe polarizations produces a nonlinear response 𝜒 𝑋𝑋𝑍 that is asymptotically 𝑡 independent. This asymmetry reflects the fact that the two species of fractionalized excitations live in different spatial dimensions. Thus the pump-probe signals studied here are sensitive to (i) nontrivial braiding statistics in three dimensions, (ii) the existence of bound states among fractionalized excitations, and (iii) the one-dimensional mobility of lineons. Furthermore, our results therefore provide spectroscopic signatures that distinguish fracton phases from conventional topologically ordered spin liquids.

braiding↗

Surveys of the earth's resources and environment by satellites

The potential and promise of observing the earth from the vantage point of space is discussed. The systematic surveying of processes and phenomena occurring on the surface of the earth by Landsat 1 and Nimbus 5 is considered to be useful in the following areas: assessment of water resources; mineral and petroleum exploration; land use planning; crop, forest, and rangeland inventory; assessment of flood, earthquake, and other environmental hazards; monitoring coastal processes; environmental effects of industrial effluents and of air pollution; mapping the distribution and types of ice covering the earth's polar caps and global soil moisture distributions.

Nordberg, W.↗

Estimates of the wind speeds required for particle motion on Mars

Threshold wind speeds for setting particles into motion on Mars are estimated by evaluating experimentally observed threshold friction velocities and determining the ratio of this velocity to the threshold wind speed at the top of earth's atmospheric boundary layer (ABL). Turning angles between the direction of the wind at the top of the ABL and the wind stress at the surface are also estimated. Detailed consideration is given to the dependence of the threshold wind speed at the top of the ABL on particle diameter, surface pressure, air temperature, atmospheric stability and composition, surface roughness, and interparticle cohesion. The results are applied to interpret a number of phenomena that have been observed on Mars and are attributable to aeolian processes. It is shown that: (1) minimum threshold wind speeds of about 50 to 100 m/sec are required to cause particle motion on Mars under 'favorable' conditions; (2) particle motion should be infrequent and strongly correlated with proximity to small topographical features; (3) in general, particle motion occurs more readily at night than during the day, in winter polar areas than equatorial areas around noon, and for H2O or CO2 ice particles than for silicate particles; and (4) the boundary between saltating and suspendible particles is located at a particle diameter of about 100 microns.

Pollack, J. B.↗

Anomalous Magnetoelectric Coupling in the Paramagnetic State of a Chiral and Polar Magnet

Abstract Chiral magnets are excellent platforms for studying intertwined spin, charge, orbit, and lattice degrees of freedom in solid‐state materials. In this work, the anomalous magnetoelectric behavior in a chiral magnet K 2 Co 2 (SO 4 ) 3 is demonstrated using comprehensive experimental probes. This material adopts a P 2 1 3 chiral cubic structure at room temperature. Based on the results of high‐resolution synchrotron X‐ray diffraction, this study shows that the low‐temperature (<130 K) crystal structure is a P 2 1 monoclinic phase, both polar and chiral. Magnetic and thermodynamic measurements reveal highly frustrated magnetic interactions and possible non‐collinear antiferromagnetic ordering at an extremely low temperature ≈0.6 K. Critically, anomalous magnetoelectric correlations are experimentally detected in its paramagnetic temperature regime, which can arise from the synergetic interplay between magnetoelastic and piezoelectric effects. These findings thus indicate that K 2 Co 2 (SO 4 ) 3 is a unique material, displaying multiple emergent structural and magnetic phenomena. This is attributed to both its overall crystallographic symmetry and the fact that its magnetic ions are located at low‐symmetry sites.

Xu, Xianghan↗

Mapping causal pathways with structural modes fingerprint for perovskite oxides

Abstract Causality is innate to the determination of the fundamental mechanism controlling any physical phenomena. However, combining causality within the standard practices of computational modelling to understand structure-functionality connections is extremely rare. This work proposes a fingerprint based on key structural modes for ABO 3 -type perovskite oxides and its derivatives, combined with causal models, for predicting Kohn–Sham energies. Our study of causal models captures the inherent coupling between structural modes such as rotation, tilt and antiferroelectric displacements, responsible for phase transition, polarization, magnetization and metal–insulator transition, exhibited by these materials. Although developed for modelling specific functionality, this method is universally applicable to derive other functionalities and even different material classes while tracking hidden causal mechanisms via structural distortions.

42 ENGINEERING↗

Controlling magnetism and transport at perovskite cobaltite interfaces via strain-tuned oxygen vacancy ordering

Complex oxides such as perovskite cobaltites exhibit rich phenomena at interfaces due to the complex interplay between their structural, defect, electronic, and magnetic degrees of freedom. Here, we study this interplay here in the ferromagnetic metallic cobaltite La 1−𝑥 ⁢Sr 𝑥⁢ CoO 3−𝛿 , using specific substrates to vary both the heteroepitaxial strain (compressive vs tensile) and growth orientation ((001) vs (110)). Transmission electron microscopy, electron energy-loss spectroscopy, high-resolution X-ray diffraction, magnetometry, polarized neutron reflectometry, and electronic magnetotransport measurements are applied. Lattice mismatch and growth orientation are found to enable the precise control of interfacial oxygen vacancy ordering in La 1−𝑥⁢ Sr 𝑥 ⁢CoO 3−𝛿 , thus dictating strain relaxation and oxygen vacancy depth profiles, in turn controlling thickness-dependent magnetic and electronic properties. In particular, compressive strain and (110) orientations minimize deleterious magnetic/electronic dead layer effects, leading to the optimization of interfacial magnetism and transport. Strain and orientation tuning of oxygen vacancy ordering are thus established as powerful means to control physical properties at cobaltite-based interfaces, relevant to several fields.

36 MATERIALS SCIENCE↗

In Situ Atmospheric Pressure Measurements in the Martian Southern Polar Region: Mars Volatiles and Climate Surveyor Meteorology Package on the Mars Polar Lander

Pressure observations are crucial for the success of the Mars Volatiles and Climate Surveyor (MVACS) Meteorology (MET) package onboard the Mars Polar Lander (MPL), due for launch early next year. The spacecraft is expected to land in December 1999 (L(sub s) = 256 degrees) at a high southern latitude (74 degrees - 78 degrees S). The nominal period of operation is 90 sols but may last up to 210 sols. The MVACS/MET experiment will provide the first in situ observations of atmospheric pressure, temperature, wind, and humidity in the southern hemisphere of Mars and in the polar regions. The martian atmosphere goes through a large-scale atmospheric pressure cycle due to the annual condensation/sublimation of the atmospheric CO2. Pressure also exhibits short period variations associated with dust storms, tides, and other atmospheric events. A series of pressure measurements can hence provide us with information on the large-scale state and dynamics of the atmosphere, including the CO2 and dust cycles as well as local weather phenomena. The measurements can also shed light on the shorter time scale phenomena (e.g., passage of dust devils) and hence be important in contributing to our understanding of mixing and transport of heat, dust, and water vapor.

Harri, A.-M.↗

Some dynamical design considerations for momentum biased spacecraft

This paper discusses some of the dynamical aspects that affect the attitude behavior of a spacecraft placed in a near earth polar orbit. The parameters such as atmospheric density variation, super-rotation of upper atmosphere, pitch equilibrium angle, and trim boom length selection to reduce pitch axis drift are considered. These parameters are studied with reference to two momentum biased satellities (Magsat and Dynamics Explorer-2) and the analyses are correlated with observed flight data. It is found that the design model of certain parameters has to be improved by including other phenomena so that flight data and the analytical model predictions have good correlations. The effects of mass imbalance on the orbital and nutational modes of the spacecraft attitude are discussed.

Sellappan, R. G.↗

Comparison of data from the Scanning Multifrequency Microwave Radiometer (SMMR) with data from the Advanced Very High Resolution Radiometer (AVHRR) for terrestrial environmental monitoring - An overview

Comparison between the microwave polarized difference temperature (MPDT) derived from 37 GHz band data and the normalized difference vegetation index (NDVI) derived from near-infrared and red bands, from several empirical investigations are summarized. These indicate the complementary character of the two measures in environmental monitoring. Overall the NDVI is more sensitive to green leaf activity, whereas the MPDT appears also to be related to other elements of the above-ground biomass. Monitoring of hydrological phenomena is carried out much more effectively by the MPDT. Further work is needed to explain spectral and temporal variation in MPDT both through modelling and field experiments.

Townshend, J. R. G.↗

A thermal model for the seasonal nitrogen cycle on Triton

The seasonal N2-cycle model presently used to characterize such observed phenomena on Triton as atmospheric pressure and surface albedo features at the time of the Voyager encounter incorporates diurnal and seasonal subsurface heat conduction, and can account for the heat capacity of N2 frost deposits. The results obtained by this model differ from those of previous studies in that they do not predict the seasonal freezing-out of the Triton atmosphere; even for a wide range of input parameters, the bright southern polar cap is seen as rather unlikely to be N2. The results support the microphysical arguments for the presence of either dark or smooth translucent N2 frosts on the Triton surface.

Hansen, Candice J.↗

Ultrafast Neuromorphic Dynamics Using Hidden Phases in the Prototype of Relaxor Ferroelectrics

Materials possessing multiple states are promising to emulate synaptic and neuronic behaviors. Their operation frequency, typically in or below the GHz range, however, limits the speed of neuromorphic computing. Ultrafast THz electric field excitation has been employed to induce nonequilibrium states of matter, called hidden phases in oxides. One may wonder if there are systems for which THz pulses can generate neuronic and synaptic behavior, via the creation of hidden phases. Using atomistic simulations, we discover that relaxor ferroelectrics can emulate all the key neuronic and memristive synaptic features. Their occurrence originates from the activation of many hidden phases of polarization order, resulting from the response of nanoregions to THz pulses. We find such phases further possess different dielectric constants, which is also promising for memcapacitor devices.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Advanced infrared astronomy

The CO2 laser heterodyne spectrometer was used at the 3-m IRTF on Mauna Kea to make measurements of Mars during the 1984 opposition. Analysis of the observations of the mesospheric non-thermal emission demonstrated the existence of a warming of the Mars polar mesosphere, similar to the seasonal effects which are well known to occur at the Earth's mesopause. A search for CO2 and NH3 on Comet Halley was done with the new Kitt Peak system as well as with the IRTF heterodyne system. A Lamb-dip absorption cell was designed and constructed. Its use will allow extreme frequency stabilization of the laser local oscillator, which will greatly facilitate measurements of winds and dynamical phenomena. The Lamb-dip cell was used at Kitt Peak to study zonal and meridional winds in the atmosphere of Venus. Water vapor was detected in Comet Halley using Fourier transform spectrometer. The 2.65 micrometer upsilon sub 3 band was seen in emission, confirming non-thermal-equilibrium excitation models for comets. A study was made of the variability of Jovian ethane emission. The average volume mixing ratio of ethane in the Jovian stratosphere was found to be 3x10 to the -6 power, with the greatest variability seen in the auroral regions.

Mumma, M. J.↗

Understanding Geospace on a Grand Scale: The Global Ionoshphere/Thermosphere Constellation

We present the concept of a constellation of polar orbiting satellites equally spaced in longitude (local time) to systematically sample both the neutral and ionzed gas components of the Earth in circular orbits near 350 km, including their density, temperature, and velocities. The instrumentation would include techniques to measure the height of the ionospheric "F-peak" and its variations along the orbit. The number of satellites (l2? 24? 48?) and their configuration would be determined from modeling analysis and expected geophysical phenomena, including their drivers and characteristic time scales. Together with imaging data from separate satellites, the array of satellites with in situ probes would be expected to provide a new picture of (1) high latitude electrodynamics and atmospheric processes and associated coupling with magnetospheric mass and momentum input, (2) the response of the global ionosphere and thermosphere to magnetic storms, and (3) global neutral wind circulation patterns, neutral density structure, tides, planetary waves, and gravity waves. The comprehensive measurements gathered by the IT-Constellation envisioned here would provide a major leap forward in each of these areas, addressing global physical processes and providing fundamental, new knowledge of Geospace. In particular, by its very nature, the constellation addresses "system science", revealing how the ionosphere-thermosphere connects globally to the magnetosphere above and the troposphere below. We present this concept as the next logical step in observing the "whole" space environment using in situ probes in conjunction with imagers. We invite modelers to not only comment on this concept but also to become actively engaged in helping to define it.

Pfaff, Robert↗

Intrinsic donor-bound excitons in ultraclean monolayer semiconductors

The monolayer transition metal dichalcogenides are an emergent semiconductor platform exhibiting rich excitonic physics with coupled spin-valley degree of freedom and optical addressability. Here, we report a new series of low energy excitonic emission lines in the photoluminescence spectrum of ultraclean monolayer WSe 2 . These excitonic satellites are composed of three major peaks with energy separations matching known phonons, and appear only with electron doping. They possess homogenous spatial and spectral distribution, strong power saturation, and anomalously long population (>6 µs) and polarization lifetimes (>100 ns). Resonant excitation of the free inter- and intravalley bright trions leads to opposite optical orientation of the satellites, while excitation of the free dark trion resonance suppresses the satellites' photoluminescence. Defect-controlled crystal synthesis and scanning tunneling microscopy measurements provide corroboration that these features are dark excitons bound to dilute donors, along with associated phonon replicas. Our work opens opportunities to engineer homogenous single emitters and explore collective quantum optical phenomena using intrinsic donor-bound excitons in ultraclean 2D semiconductors.

36 MATERIALS SCIENCE↗

Pyroelectric thin films—Past, present, and future

Pyroelectrics are a material class that undergoes a change in polarization as the temperature of the system is varied. This effect can be utilized for applications ranging from thermal imaging and sensing to waste-heat energy conversion to thermally driven electron emission. Here, we review recent advances in the study and utilization of thin-film pyroelectrics. Leveraging advances in modeling, synthesis, and characterization has provided a pathway forward in one of the more poorly developed subfields of ferroelectricity. We introduce the complex physical phenomena of pyroelectricity, briefly explore the history of work in this space, and highlight not only new advances in the direct measurement of such effects but also how our ability to control thin-film materials is changing our understanding of this response. Finally, we discuss recent advances in thin-film pyroelectric devices and introduce a number of potentially new directions the field may follow in the coming years.

36 MATERIALS SCIENCE↗