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At least 577 records · Page 32

Dry coupled magnetostrictive transducers for robotic inspection of dry storage casks - 15304

The lack of a national repository for used nuclear fuel has lead to the usage of dry storage casks as the de facto long term storage solution, the usage of which is prevalent throughout the United States. Furthermore, as shown in figure 3, the usage of dry storage is only expected to increase over time. Because these casks were originally intended as only an interim measure, there is an urgent need to develop methods to monitor their structural health over the long-term. Additionally, when concerns about the susceptibility of these casks to cracking is considered, the need for inspection becomes even more apparent. The use of robotic devices to inspect the interior of these casks for signs of damage has been proposed, but in order for this to be realized, advances in sensing technology must occur. We develop a novel type of transducer for non-destructive evaluation to aid in these efforts. We construct a prototype sensor, demonstrate simple defect detection with it, and present a design for an inspection robot equipping these transducers. Ultrasonic inspection is a well known method of non-destructive evaluation which works by measuring the response of ultrasonic waves propagating through a material. In through-transmission inspection, a transmitter and receiver are used to generate and detect waves in the material to be inspected. The presence of a crack or defect in the material will scatter some of the transmitted wave's energy, reducing the strength of the response at the receiver. Magnetostrictive transducers are often used to generate and detect guided waves. These transducers depend on the magnetostrictive effect, where certain materials will deform in the presence of a magnetic field. The typical construction of one of these transducers is shown in figure 5, consisting of a magnetostrictive foil, meandering coil, and a biasing magnet. Materials typically used for the foil include Fe-Co and Terfenol-D. For wave generation, a high-frequency alternating current is supplied to the coil of the transducer, which generates an oscillating magnetic field that causes the foil to deform. For reception, the inverse occurs: deformation of the foil results in a current in the coil that can be detected. The deformation of the foil is usually coupled to the material to be inspected with an adhesive, and waves are transmitted through this bond. Obviously, an inspection robot cannot have its sensors bound to the surface of the cask. A robot is being designed for inspection, and it must deal with many challenges inside the cask, including tight confines, right-angle transitions, high temperatures, and radiation. For our initial design, we consider only the geometrical constraints, and present a design for a prototype that can be assembled from COTS components. The robot needs to be articulated to navigate the bends in the cask, so each wheel is individually actuated. The robot is controlled via a tether, which also supplies electrical power and compressed air. For localization, ultrasonic range-finders and a camera are equipped. Using the basic transducer, we experimented with various configurations of materials and geometry. In order to gather relevant data, we used force sensitive resistors to measure applied force, and a Matec computer system to generate and measure ultrasonic waves. A testing rig was constructed to simulate the geometrical constraints of the interior of the cask, and we experimented using deadweights, a pneumatic cylinder, and an air bladder to apply the force. It was discovered early in the testing process that the performance of the transducer was very sensitive to the alignment of the components, and the method by which the foil was attached. To maximize performance, we designed an enclosure that would hold the components in alignment while still allowing the foil to float. To test the effectiveness of our new transducer, we cut circular holes of varying diameter in 2 mm aluminum plate, and measured the response across them. It can be seen that there is a clear relationship between the strength of the received signal and the force applied, and to a lesser extent, the size of the defect. This design performs adequately as a proof of concept, and a more precisely fabricated enclosure should further increase the accuracy of its measurements.

42 ENGINEERING↗

Effect of Ferrimagnetic Cr{sub 2}S{sub 3} on AC Susceptibility and Superconducting Properties of YBa{sub 2}Cu{sub 3}O{sub 7−δ}

Superconductivity and magnetism are mutually exclusive phenomena. This work was carried out to investigate the effect of ferrimagnetic Cr{sub 2}S{sub 3} addition on YBa{sub 2}Cu{sub 3}O{sub 7−δ} superconductor. The solid-state reaction method was used to prepare YBa{sub 2}Cu{sub 3}O{sub 7−δ} (Cr{sub 2}S{sub 3}){sub x} (x = 0 to 0.3 wt%). The samples were characterized by using the four-probe method to measure the electrical resistivity and AC susceptibility to measure the critical temperature, T{sub cχ} and critical current density at the peak temperature T{sub p} of the complex susceptibility, J{sub c}(T{sub p}). The x-ray diffraction (XRD) method was used to determine the phase and structure of the sample. Field emission electron microscopy (FESEM) was used to determine the microstructure. The x = 0.05 sample showed the highest onset transition temperature, T{sub c−onset} (93 K), zero-resistance temperature, T{sub c−zero} (89 K), T{sub cχ} (93 K) and T{sub p} (86 K). Addition of Cr{sub 2}S{sub 3} did not affect the orthorhombic structure. However, the addition of Cr{sub 2}S{sub 3} for x ≥ 0.10 showed some impurity peaks in the XRD patterns. The grain size decreased with Cr{sub 2}S{sub 3} addition. Cr{sub 2}S{sub 3} improved the intergrain coupling and flux pinning as indicated by the increase in J{sub c}(T{sub p}) and T{sub p}. These results are compared with other magnetic and non-magnetic materials addition to YBa{sub 2}Cu{sub 3}O{sub 7−δ}.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Generation of circularly polarized radiation from a compact plasma-based extreme ultraviolet light source for tabletop X-ray magnetic circular dichroism studies

Generation of circularly polarized light in the extreme ultraviolet (EUV) spectral region (about 25 eV–250 eV) is highly desirable for applications in spectroscopy and microscopy but very challenging to achieve in a small-scale laboratory. We present a compact apparatus for generation of linearly and circularly polarized EUV radiation from a gas-discharge plasma light source between 50 eV and 70 eV photon energy. In this spectral range, the 3p absorption edges of Fe (54 eV), Co (60 eV), and Ni (67 eV) offer a high magnetic contrast often employed for magneto-optical and electron spectroscopy as well as for magnetic imaging. We simulated and designed an instrument for generation of linearly and circularly polarized EUV radiation and performed polarimetric measurements of the degree of linear and circular polarization. Furthermore, we demonstrate first measurements of the X-ray magnetic circular dichroism at the Co 3p absorption edge with a plasma-based EUV light source. Our approach opens the door for laboratory-based, element-selective spectroscopy of magnetic materials and spectro-microscopy of ferromagnetic domains.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A Novel Fluorescent Nanoparticle for Sensitive Detection of Cry1Ab Protein In Vitro and In Vivo

Here, we report the synthesis and characterization of CoFe{sub 2}O{sub 4} doping Ag{sub 2}S dendrimer-modified nanoparticles (CoFe{sub 2}O{sub 4}-Ag{sub 2}S DMNs) in Cry1Ab protein detection and imaging. The near-infrared Ag{sub 2}S quantum dots were first prepared by using the thermal decomposition method, followed by modification of the water-soluble quantum dots using the method of solvent evaporation and ligand exchange, and finally the fluorescent magnetic bifunctional nanoparticles were obtained by binding with CoFe{sub 2}O{sub 4}. As-prepared CoFe{sub 2}O{sub 4}-Ag{sub 2}S DMNs were characterized by fluorescence (FL) spectroscopy and transmission electron microscopy (TEM). Results showed that Ag{sub 2}S DMNs could sensitively detect Cry1Ab both in vitro and in vivo. In vitro, the enhanced FL intensity as a function of the concentration is notably consistent with the Langmuir binding isotherm equation in the range of 0–200 ng/mL of Cry1Ab proteins. The detection limit of this method was found to be 0.2 ng/mL. Meanwhile, the fluorescence wavelength was extended to the second near-infrared range (NIR-II, 1.0~1.4 μm), which enables in vivo imaging. This study highlights the importance of NIR QDs doping magnetic materials as a new method to trace Bacillus thuringiensis (Bt) in insects and their potential applications in in vivo NIR tissue imaging.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Large linear magnetoresistance in a GaAs/AlGaAs heterostructure

We report non-saturating linear magnetoresistance (MR) in a two-dimensional electron system (2DES) at a GaAs/AlGaAs heterointerface in the strongly insulating regime. We achieve this by driving the gate voltage below the pinch-off point of the device and operating it in the non-equilibrium regime with high source-drain bias. Remarkably, the magnitude of MR is as large as 500% per Tesla with respect to resistance at zero magnetic field, thus dwarfing most non-magnetic materials which exhibit this linearity. Its primary advantage over most other materials is that both linearity and the enormous magnitude are retained over a broad temperature range (0.3 K to 10 K), thus making it an attractive candidate for cryogenic sensor applications.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Thermally driven topology in frustrated systems

Topological spin textures, such as magnetic skyrmions, have been extensively discussed in magnetic materials with broken inversion symmetry. Most of these textures are stable at low temperatures and form long-range orders. However, the topological nature of these textures, characterized by the index called topological charge, is actually persistent at elevated temperatures. In this work, the topological charge of a two-dimensional frustrated spin model with the Dzyaloshinskii-Moriya (DM) interaction was calculated by the Monte Carlo simulations. At finite temperatures, nontrivial topology driven by thermal fluctuation was discovered in a spin-disordered phase. Furthermore, this thermally driven topology is the dominant topology at low magnetic fields. The magnitude of topological charge is quadratic in the DM interaction and linear in the external magnetic field or uniaxial magnetic anisotropy. We also propose a real frustrated system, the Mn-Bi monolayer film, with large DM interaction to enable such thermally driven topology. A full phase diagram of this system has been explored.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Enabling ambient stability and quantum integration of organometallic magnonic ferrimagnets via atomic layer encapsulation

Magnons, the quanta of spin waves in magnetic materials, are promising for hybrid quantum systems by bridging electromagnetic and spin degrees of freedom. The organometallic ferrimagnet vanadium tetracyanoethylene (V[TCNE] x , x ≈ 2) is especially well-suited for quantum magnonics due to its low Gilbert damping and substrate versatility. However, its rapid chemical degradation in ambient conditions hinders practical applications. Incumbent encapsulation methods provide some protection, but are bulky, obscure intrinsic properties of V[TCNE] x , introduce thermal stress at cryogenic temperatures, and complicate microwave device integration. Here, we demonstrate that ultrathin alumina films deposited via low-temperature atomic layer deposition effectively protect V[TCNE] x by preserving its magnetic and magnonic properties following ambient exposure. The sub-100 nm transparent films also enable advanced spectroscopy, magnetometry, and cavity magnonic measurements that reveal the intrinsic properties of V[TCNE] x . This encapsulation strategy advances molecule-based quantum information science by providing a robust route toward scalable, monolithic integration in hybrid quantum technologies.

magnetic materials↗

Model Proposed to Calculate the Exchange Interaction in Ni/Pt Multilayers

The behavior of spin waves is mainly influenced by all parameters that characterize the magnetic material such as exchange interactions, surface and volume anisotropy effects, dipole interactions, and phase transitions and imperfections. In this article, we develop a simple calculation model based on a ferromagnetic anisotropic system that has allowed us to obtain numerical estimates for the Pt exchange interaction and the interlayer coupling force at various Ni/Pt multilayers.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

An efficient, movable single-particle detector for use in cryogenic ultra-high vacuum environments

A compact, highly efficient single-particle counting detector for ions of keV/u kinetic energy, movable by a long-stroke mechanical translation stage, has been developed at the Max-Planck-Institut für Kernphysik (Max Planck Institute for Nuclear Physics, MPIK). Both, detector and translation mechanics, can operate at ambient temperatures down to ∼10 K and consist fully of ultra-high vacuum compatible, high-temperature bakeable, and non-magnetic materials. The set-up is designed to meet the technical demands of MPIK’s Cryogenic Storage Ring. We present a series of functional tests that demonstrate full suitability for this application and characterise the set-up with regard to its particle detection efficiency.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Theory of unidirectional spin heat conveyer

We theoretically investigate the unidirectional spin heat conveyer effect recently reported in the literature that emerges from the Damon-Eshbach spin wave on the surface of a magnetic material. We develop a simple phenomenological theory for heat transfer dynamics in a coupled system of phonons and the Damon-Eshbach spin wave, and demonstrate that there arises a direction-selective heat flow as a result of the competition between an isotropic heat diffusion by phonons and a unidirectional heat drift by the spin wave. The phenomenological approach can account for the asymmetric local temperature distribution observed in the experiment.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Distinct spin–lattice and spin–phonon interactions in monolayer magnetic CrI 3

In this study, we apply the density-functional theory to study various phases (including non-magnetic (NM), anti-ferromagnetic (AFM), and ferromagnetic (FM)) in monolayer magnetic chromium triiodide (CrI 3 ), a recently fabricated 2D magnetic material. It is found that: (1) the introduction of magnetism in monolayer CrI 3 gives rise to metal-to-semiconductor transition; (2) the electronic band topologies as well as the nature of direct and indirect band gaps in either AFM or FM phases exhibit delicate dependence on the magnetic ordering and spin–orbit coupling; and (3) the phonon modes involving Cr atoms are particularly sensitive to the magnetic ordering, highlighting distinct spin–lattice and spin–phonon coupling in this magnet. First-principles simulations of the Raman spectra demonstrate that both frequencies and intensities of the Raman peaks strongly depend on the magnetic ordering. The polarization dependent A 1g modes at 77 cm -1 and 130 cm -1 along with the E g mode at about 50 cm -1 in the FM phase may offer a useful fingerprint to characterize this material. Lastly, our results not only provide a detailed guiding map for experimental characterization of CrI 3 , but also reveal how the evolution of magnetism can be tracked by its lattice dynamics and Raman response.

36 MATERIALS SCIENCE↗

Natural circulation loop using liquid nitrogen for cryo-detection system

The natural circulation loop is designed for the cryogenic insert in a Fourier transform ion cyclotron resonance (FTICR) mass spectrometer. Sensitivity is the key parameter of a FTICR mass spectrometer and the cryo-cooling of the pre-amplifier can reduce the thermal noise level and thereby improve the signal-to-noise ratio. The pre-amplifier consisted of non-magnetic materials is thermally connected to the cooling loop which is passing through the flange maintaining ultra-high vacuum in the ion cell. The liquid nitrogen passes through inside of the loop to cool the pre-amplifier indirectly. At the end, a cryocooler is located to re-condense nitrogen vapor generated due to the heat from the pre-amplifier. The circulating fluid removes heat from the pre-amplifier and transports it to the cryocooler or heat sink. In this paper the natural circulation loop for cryogenic pre-amplifier is introduced for improving the sensitivity of cryo-detector. In addition, the initial cool-down of the system by a cryocooler is presented and the temperature of the radiation shield is discussed with respect to the thickness of shield and the thermal radiation load.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Stacking order dependence of inverse spin Hall effect and anomalous Hall effect in spin pumping experiments

The dependence of the measured DC voltage on the non-magnetic material (NM) in NM/CoFeB and CoFeB/NM bilayers is studied under ferromagnetic resonance conditions in a TE{sub 011} resonant cavity. The directional change of the inverse spin Hall effect (ISHE) voltage V{sub ISHE} for the stacking order of the bilayer can separate the pure V{sub ISHE} and the anomalous Hall effect (AHE) voltage V{sub AHE} utilizing the method of addition and subtraction. The Ta and Ti NMs show a broad deviation of the spin Hall angle θ{sub ISH}, which originates from the AHE in accordance with the high resistivity of NMs. However, the Pt and Pd NMs show that the kinds of NMs with low resistivity are consistent with the previously reported θ{sub ISH} values. Therefore, the characteristics that NM should simultaneously satisfy to obtain a reasonable V{sub ISHE} value in bilayer systems are large θ{sub ISH} and low resistivity.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A biosensor system using nickel ferrite nanoparticles

NiFe{sub 2}O{sub 4} ferrite nanoparticles were synthesized by chemical co-precipitation method and the structural characteristics were investigated using X-ray diffraction technique, where single cubic phase formation of nanoparticles was confirmed. The average particle size of NiFe{sub 2}O{sub 4} was found to be 4.9 nm. Nanoscale magnetic materials are an important source of labels for biosensing due to their strong magnetic properties which are not found in biological systems. This property of the material was exploited and the fabrication of the NiFe{sub 2}O{sub 4} nanoparticle based biosensor was done in the form of a capacitor system, with NiFe{sub 2}O{sub 4} as the dielectric material. The biosensor system was tested towards different biological materials with the help of electrochemical workstation and the same was analysed through Cole-Cole plot of NiFe{sub 2}O{sub 4}. The performance of the sensor was determined based on its sensitivity, response time and recovery time.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Microstructure, Corrosion and Magnetic Behavior of an Aged Dual-Phase Stainless Steel

In the present work, the effect of the precipitation phenomena on corrosion and magnetic behavior of an aged dual-phase stainless steel was investigated. Aging treatment caused the precipitation of the σ phase, chromium carbides and secondary austenite, which was accompanied by the shifting of the δ/γ interfaces inside the δ ferrite grains. Aging between 700 and 850 °C strongly deteriorated the pitting corrosion resistance of the studied material. Magnetic investigation of the aged material using the vibration sample magnetic technique revealed the sensitivity of the intrinsic magnetic properties to the smallest microstructural change. This was confirmed by the Eddy current technique that led also to the evaluation of the aging-induced localized corrosion.

36 MATERIALS SCIENCE↗

Structural, magnetic and magnetocaloric properties of La{sub 0.65}Sr{sub 0.35}V{sub 0.1}Mn{sub 0.9}O{sub 3} perovskite

A new complex magnetic material La{sub 0.65}Sr{sub 0.35}V{sub 0.1}Mn{sub 0.9}O{sub 3}, suitable for the magnetic refrigeration, has been investigated. X-ray diffraction result showed that this compound had rhombohedral structure. The substitution of manganese with V leads to a decrease in the Curie temperature, T{sub C} from 378 K to 353 K. Using Arrott plots; it was found that the phase transition for this compound is of the second-order. The magnetocaloric study exposed a quite large value of the magnetic entropy change ∼ 1.56 J/kg K and the relative cooling power value of 67 J/kg at magnetic field variation of 1 T.

36 MATERIALS SCIENCE↗

Geometric control of magnetic domain morphology in electrodeposited Ni rich NiPt mesoscopic wires

In this paper, we study the electrodeposited Ni—Pt magnetic wires, exploring the mechanisms by which changes in geometry and composition influence the local magnetic structure. The samples were prepared by electrodeposition, their elemental composition was analyzed by energy dispersive X-ray spectroscopy, and phase analysis was carried out by an X-ray diffraction measurement. Magnetic force microscopy measurements, and magnetic force microscopy measurements in magnetic field were carried out to study the domain morphology of the prepared samples. Magnetization characteristics were measured via vibrating sample magnetometry mode of a superconducting quantum interference device. Here, the results were analyzed and compared with micromagnetic simulations. It is shown that a strong perpendicular magnetic anisotropy is responsible for the characteristic checkerboard-like surface magnetization patterns, which can be tuned by geometrical constriction and Ni content. Understanding these relationships provides insights into the design of magnetic materials with tailored properties for advanced applications, like magnetic sensors.

Binary alloy↗

CP2 skyrmions and skyrmion crystals in realistic quantum magnets

Abstract Magnetic skyrmions are nanoscale topological textures that have been recently observed in different families of quantum magnets. These objects are called CP 1 skyrmions because they are built from dipoles—the target manifold is the 1D complex projective space, CP 1 ≅ S 2 . Here we report the emergence of magnetic CP 2 skyrmions in a realistic spin-1 model, which includes both dipole and quadrupole moments. Unlike CP 1 skyrmions, CP 2 skyrmions can also arise as metastable textures of quantum paramagnets, opening a new road to discover emergent topological solitons in non-magnetic materials. The quantum phase diagram of the spin-1 model also includes magnetic field-induced CP 2 skyrmion crystals that can be detected with regular momentum- (diffraction) and real-space (Lorentz transmission electron microscopy) experimental techniques.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗