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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 577 records · Page 32

Seven-core fibre Raman laser with intercore coupling

This paper reports results of a study aimed at producing a Raman fibre laser based on a multicore fibre with high-reflectivity fibre Bragg gratings inscribed in its peripheral cores using femtosecond laser pulses. We present spectral and power characteristics of a Raman laser whose output power at a wavelength of 1090 nm is 2.5 W. The laser emission linewidth has been shown to decrease as a result of the reduction in nonlinear effects owing to the larger effective mode area in the multicore fibre in comparison with a standard single-mode fibre Raman laser. (paper)

36 MATERIALS SCIENCE↗

Plasma decay of nanosecond pulsed laser-produced Ar and Ar–H 2 O sparks at atmospheric pressure

Time-resolved diagnostics were applied to investigate free-electron properties in nanosecond laser-produced discharges generated in atmospheric pressure Ar and in Ar–3%H 2 O. The discharges were generated using 23 ns, 1064 nm laser pulses. Broadband plasma imaging and laser Thomson scattering were combined with optical emission spectroscopy, with particular emphasis on the Stark broadening of the H α and H β lines. The plasma exhibited a bright emission that persists for up to 30–40 µs after breakdown. Plasma emission was then followed by a very weak glow emission that persisted for up to 19 ms after breakdown. Peak electron number density of ∼2 × 10 17 cm −3 and electron temperature of ∼7 eV were measured. An excellent agreement between both techniques was obtained regarding absolute electron number densities. The inferred free-electron temporal decay dynamics are consistent with processes dominated by hydrodynamic expansion and two- and three-body electron–ion recombination. These results provide benchmark data for modeling nanosecond laser discharges and demonstrate the reliability of combining Thomson scattering with Stark broadening in atmospheric laser sparks.

Thomson scattering↗

Simulation studies of the interaction of laser radiation with additively manufactured foams

The interaction of laser radiation with foams of various porosities and low densities has been the subject of several numerical and experimental studies. In all cases, the modeling of low-Z under-dense foams as uniform gases of equivalent average density using standard radiation-hydrodynamics codes has resulted in heat-front velocities that are considerably faster than those observed experimentally. It has been theoretically conjectured that this difference may be attributed to the breakdown of the foam’s morphology, leading to a dynamics of filament expansion where the ion and electron energy partitions are significantly different from those calculated using the uniform gas model. We found that 3D computer simulations employing a disconnected representation of the foam’s microstructure which allowed for the dynamics of foam element heating, expansion, and stagnation largely supported the theoretical picture. Simulations using this model for laser experiments on under-dense 2 mg cc -1 SiO 2 aerogel foams reproduced the experimental data fairly well. We used the validated model in simulations of low-density structured foam-like materials (produced via additive manufacturing) with a variety of morphologies. We found that the log-pile configurations were consistent with the analytical propagation model of Gus’kov et al. Further validation of the model was obtained by simulating experiments performed at the Jupiter Laser Facility using the log-pile and octet-truss foam morphologies. Simulations of the foam-laser interaction using a wave propagation code showed that the microstructure was able to enhance stimulated Brillouin scattering (SBS) by concentrating the light energy into density holes. In turn, this promotes laser filamentation, reducing SBS and bringing the predicted values closer to the experimental data.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Magnetic field generation in a laser-irradiated thin collisionless plasma target by return current electrons carrying orbital angular momentum

Abstract Magnetized high energy density physics offers new opportunities for observing magnetic field-related physics for the first time in the laser–plasma context. We focus on one such phenomenon, which is the ability of a laser-irradiated magnetized plasma to amplify a seed magnetic field. We performed a series of fully kinetic 3D simulations of magnetic field amplification by a picosecond-scale relativistic laser pulse of intensity 4.2 × 10 18 W cm −2 incident on a thin overdense target. We observe axial magnetic field amplification from an initial 0.1 kT seed to 1.5 kT over a volume of several cubic microns, persisting hundreds of femtoseconds longer than the laser pulse duration. The magnetic field amplification is driven by electrons in the return current gaining favorable orbital angular momentum from the seed magnetic field. This mechanism is robust to laser polarization and delivers order-of-magnitude amplification over a range of simulation parameters.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Polarization and phase control of electron injection and acceleration in the plasma by a self-steepening laser pulse

Abstract We describe an interplay between two injection mechanism of background electrons into an evolving plasma bubble behind an intense laser pulse: one due to the overall bubble expansion, and another due to its periodic undulation. The two mechanisms occur simultaneously when an intense laser pulse propagating inside a plasma forms a shock-like steepened front. Periodic undulations of the plasma bubble along the laser propagation path can either inhibit or conspire with electron injection due to bubble expansion. We show that carrier-envelope-phase (CEP) controlled plasma bubble undulation induced by the self-steepening laser pulse produces a unique electron injector—expanding phase-controlled undulating bubble (EPUB). The longitudinal structure of the electron bunch injected by the EPUB can be controlled by laser polarization and power, resulting in high-charge (multiple nano-Coulombs) high-current (tens of kilo-amperes) electron beams with ultra-short (femtosecond-scale) temporal structure. Generation of high-energy betatron radiation with polarization- and CEP-controlled energy spectrum and angular distribution is analyzed as a promising application of EPUB-produced beams.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Novel signatures of radiation reaction in electron–laser sidescattering

In this article we investigate novel signatures of radiation reaction via the angular deflection of an electron beam colliding at 90 degrees with an intense laser pulse. Due to the radiation reaction effect, the electrons can be deflected towards the beam axis for plane wave backgrounds, which is not possible in the absence of radiation reaction effects. The magnitude and size of the deflection angle can be controlled by tailoring the laser pulse shapes. The effect is first derived analytically using the Landau–Lifshitz equation, which allows to determine the important scaling behavior with laser intensity and particle energy. We then move on to full scale 3D Monte Carlo simulations to verify the effect is observable with present day laser technology. We investigate the opportunities for an indirect observation of laser depletion in such side scattering scenarios.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multilayer film coating for laser ion source target for increase of low charge state production

The use of Laser Ion Source for accelerator facilities has the advantage to tune the characteristic of the produced beams by changing the laser parameters using the same primary target. The advantageous and innovative opportunity to manipulate the characteristic of charge state distributions by the use of composed target, may open new possibilities for the ion sources. In this experiment we characterize and study the plasma produced by the laser ablation of coated targets at constant laser parameters. The performed investigation has the double purpose to have a better understanding of penetration depth of laser in composed materials and understand how to tune the charge states by adding coating films. Finally, the obtained results showed that for particular thickness of coating, the low charge states were produced with higher yield than in the case of pure material.

43 PARTICLE ACCELERATORS↗

Linear colliders based on laser-plasma accelerators

Laser-plasma accelerators are capable of sustaining accelerating fields of 10–100 GeV/m, 100–1000 times that of conventional technology and the highest fields produced by any of the widely researched advanced accelerator concepts. Laser-plasma accelerators also intrinsically accelerate short particle bunches, several orders of magnitude shorter than that of conventional technology, which leads to reductions in beamstrahlung and, hence, savings in the overall power consumption to reach a desired luminosity. These properties make laser-plasma accelerators a promising accelerator technology for a more compact, less expensive high-energy linear collider providing multi-TeV polarized leptons. In this submission to the Snowmass 2021 Accelerator Frontier, we discuss the motivation for a laser-plasma-accelerator-based linear collider, the status of the field, and potential linear collider concepts up to 15 TeV. Herein, we outline the research and development path toward a collider based on laser-plasma accelerator technology, and highlight near-term and mid-term applications of this technology on the collider development path. The required experimental facilities to carry out this research are described. We conclude with community recommendations developed during Snowmass.

43 PARTICLE ACCELERATORS↗

Optimized matching conditions for self-guided laser wakefield accelerators

We revisit the matching conditions for self-guided laser pulse propagation in plasma and refine their formulation to maximize the energy of electrons produced via laser wakefield acceleration. Bayesian optimization, combined with particle-in-cell simulations carried out in a quasi-three-dimensional geometry and a Lorentz-boosted frame, is employed. The optimization identifies the maximum electron energy that a self-guided laser wakefield accelerator, driven by a laser of a given energy, can produce, together with the corresponding acceleration distance. Our results further demonstrate that electrons with energies close to the maximum value can be obtained across a relatively wide range of input parameters and without the need for their precise tuning. This provides substantial flexibility for experimental implementation and significantly relaxes the operational constraints associated with self-guided laser wakefield accelerators.

43 PARTICLE ACCELERATORS↗

Nonlinear transmission of laser light through coronal plasma due to self-induced incoherence

The success of direct laser-driven inertial con nement fusion (ICF) relies critically on the efficient coupling of laser light to plasma. At ignition scale, the absolute stimulated Raman scattering (SRS) instability can severely inhibit this coupling by redirecting and strongly depleting laser light. This article describes a new dynamic saturation regime of the absolute SRS instability near one quarter of the critical density. The saturation occurs when spatiotemporal ion-acoustic fluctuations in the plasma density detune the instability resonance. Here, the dynamic saturation mitigates the strong depletion of laser light and enhances its transmission through the instability region, explaining the coupling of laser light to ICF targets at higher plasma densities.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laser melting modes in metal powder bed fusion additive manufacturing

In laser powder bed fusion additive manufacturing of metals, extreme thermal conditions create many highly dynamic physical phenomena such as vaporization and recoil, Marangoni convection, and protrusion and keyhole instability. Collectively however, the full set of phenomena is too complicated for practical applications and, in reality, the melting modes are used as a guideline for printing. With increasing local material temperature beyond the boiling point, the mode can change from conduction to keyhole. These mode designations ignore laser-matter interaction details but in many cases are adequate to determine the approximate microstructures and hence the properties of the build. To date, no consistent, common, and coherent definitions have been agreed upon because of historic limitations in melt pool and vapor depression morphology measurements. Here, we distinguish process-based definitions of different melting modes from those based on postmortem evidence. The latter are mainly derived from the transverse cross-sections of the fusion zone, whereas the former come directly from time-resolved x-ray imaging of melt pool and vapor depression morphologies. These process-based definitions are more strict and physically sound, and they offer new guidelines for laser additive manufacturing practices and create new research directions. Further, we highlight the significance of the keyhole, which substantially enhances the laser energy absorption by the melt pool. Recent studies strongly suggest that stable-keyhole laser melting enables efficient, sustainable, and robust additive manufacturing. The realization of this scenario demands the development of multiphysics models, signal translations from morphology to other feasible signals, and in-process metrology across platforms and scales.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A portable on-axis laser-heating system for near-90° X-ray spectroscopy: application to ferropericlase and iron silicide

A portable IR fiber laser-heating system, optimized for X-ray emission spectroscopy (XES) and nuclear inelastic scattering (NIS) spectroscopy with signal collection through the radial opening of diamond anvil cells near 90°with respect to the incident X-ray beam, is presented. The system offers double-sided on-axis heating by a single laser source and zero attenuation of incoming X-rays other than by the high-pressure environment. A description of the system, which has been tested for pressures above 100 GPa and temperatures up to 3000 K, is given. The XES spectra of laser-heated Mg 0.67 Fe 0.33 O demonstrate the potential to map the iron spin state in the pressure–temperature range of the Earth's lower mantle, and the NIS spectra of laser-heated FeSi give access to the sound velocity of this candidate of a phase inside the Earth's core. This portable system represents one of the few bridges across the gap between laser heating and high-resolution X-ray spectroscopies with signal collection near 90°.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Laser-damage performance of gallium-alloy liquid metal mirrors

We explore the characteristics and laser-damage behavior of gallium-based liquid metal alloy mirrors under exposure to ns laser pulses. One of the key advantages of using liquid metal mirrors is the self-healing potential following perturbations arising from exposure to high-power laser pulses. In this work, key performance metrics, such as reflectivity and the laser-damage initiation mechanism and initiation threshold, were investigated using fused-silica cells filled with three different liquid metal Ga alloys. The results suggest that irreversible modification (damage) under 355-nm, 6-ns pulses are associated with the formation of gallium oxide, taking place at a fluence significantly higher than that for damage initiation in conventional metal mirrors. This behavior is believed to arise from the different damage initiation mechanism in liquid metal mirrors requiring increased laser absorbed energy for an irreversible modification of the material surface to occur. As a result, this exploratory work is the first of its kind and highlights some favorable performance characteristics of gallium-alloy metal mirrors.

47 OTHER INSTRUMENTATION↗

Depth-Resolved Lithiated Gradients in Pristine and Laser-Ablated Anodes During Fast Charging

Laser ablating 3D electrode microstructures is a technique to improve Li-ion battery fast-charge performance. This technique has been theoretically proposed and electrochemically validated previously in the literature. The fundamental principle underlying laser ablation is that the ablated features reduce Li-ion transport pathways, improving access to the electrode active material near the current collector. This, in turn, promotes more homogeneous electrode utilization. The present study seeks to directly affirm the physics attributed to laser ablation using operando high-speed synchrotron X-ray diffraction. In this study, depth-resolved graphite lithiation gradients are measured operando during high-rate (15 min) charging. The depth-resolved lithiation dynamics of both ablated and non-ablated anodes are compared. The results highlight that the laser-ablated graphite electrode has notably more homogeneous utilization as compared to the non-ablated electrode. Additionally, the ablated electrode has a significant delay in reaching the maximum graphite lithiation at the separator, indicating less propensity for lithium plating. During low rate delithiation/discharge (2 hr), the two cells' lithiation gradients converge. Notably, a calibrated physics-based electrochemical model accurately reflects experimental findings, suggesting the potential to use pseudo-4D models not only to optimize laser ablation parameters in fast-charge capable electrodes but also to guide fast charging protocols that avoid lithium plating.

25 ENERGY STORAGE↗

High-energy X-ray radiography with apodized petawatt laser beams

We have produced laser wakefield-accelerated electron beams with energies of 2 GeV in Target Area 1 of the ZEUS facility. These electron beams oscillate in the accelerating structure that is produced in the wake of an ultrashort laser pulse (25 fs). These ’betatron’ oscillations result in the emission of a collimated (4 mrad divergence) beam of high-energy X-ray/gamma photons (on the order of several hundred keV). In this work, we demonstrate the capabilities of the ZEUS laser system by showing that apodizing the laser beam in the near field allows for the production of high-quality betatron X-rays for radiography purposes. This demonstrates that a high-power, large-aperture laser beam could be split into multiple parts to drive betatron X-ray sources from multiple angles or temporal delays into a High Energy Density (HED) target to be probed, enabling pump-probe measurements at multiple temporal delays or tomography on a single shot.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laser-based Adhesion Strength Measurements for Advanced Manufactured Sensor Adhesion Characterization

As part of the advanced manufacturing (AM) focus of the Nuclear Energy Enabling Technologies (NEET) Advanced Sensors and Instrumentation (ASI) Program, new in-house capabilities to fabricate and test novel active and passive in-pile sensors are being developed at the Idaho National Laboratory (INL). These advanced-manufactured sensors, such as peak temperature monitors and strain gauges, must be miniaturized and be able to provide real-time feedback, all while withstanding the coupled extremes of temperature and radiation typically observed in the environment of a nuclear test reactor. Fabricating durable and robust in-pile sensors with high fidelity requires a fundamental understanding of the optimal process parameters required in the AM technique, as well as the effect of deviations from optimal process parameters on the sensor-substrate adhesion and the ultimate robustness of the sensor. This report presents the use of a laser-based, non-contact approach for characterizing the adhesion of sensors manufactured using aerosol jet printing (AJP) that comprise of silver nanoparticle inks deposited and sintered on austenitic stainless steel (SS) 316L substrates. The effect of substrate surface roughness, surface energy, ink sintering time and sintering temperature on the printed sensor topography and the sensor-substrate adhesion has been systematically investigated. The sensor-substrate interfacial adhesion strength was determined from the critical laser pulse energy required to ablate/ detach the printed sensor from the substrate. Measurements of the sensor topography using optical profilometry revealed that post-deposition sintering at 400°C for 60 minutes resulted in a reduced sensor thickness, while plasma treating the substrate prior to printing yielded sensors with uniform thickness profiles transverse to the print direction. Sintering temperature and time were found to be the dominant parameters that affected sensor-substrate adhesion, followed by substrate surface roughness. The laser-based and locally-destructive approach for adhesion strength measurements shows promise in overcoming the challenges and limitations of current standardized peel tests and can be developed into a post-fabrication process control protocol for evaluating the durability of AM printed sensors in a high throughput fashion. Future studies will investigate the use of laser-induced spallation techniques as well as non-destructive laser ultrasonic methods for sensor-substrate adhesion characterization on sensors manufactured using AJP and other AM techniques such as plasma jet printing (PJP).

42 ENGINEERING↗

Direct Laser Impulse (DLI) System Alignment: Requirements Engineering Project

The National Ignition Facility (NIF) is the world’s largest and most energetic laser, and it is comprised of 192 laser beams that must align onto one target for the purpose of learning about Internal Confinement Fusion (ICF) and High Energy Density (HED) physics. A new NIF capability under development is the Direct Laser Impulse (DLI). The DLI capability will provide a test environment where high pulsed laser energy is delivered to a three-dimensional target. Achieving this delivery to target relies on a precision alignment and positioning of the two redirected NIF beams, as shown in Figure 1. When aligned, the two combined beams—with a frequency converted from infrared (IR) to green laser light, at a fluence (energy per unit area) of roughly 20 joules per square centimeter—will be capable of delivering up to 30 kilojoules of direct, unfocused energy to a one cubic foot target. The 40-cm x 40-cm aligned impulse area at the DLI target interaction plane (TIP) is achieved by using a beam path comprised of pickoff and transport mirrors, frequency conversion crystals, optics serving as environmental barriers, and debris shields. A separate aligned diagnostic beam path is also required for impulse to TIP characterization. Final in-situ alignment is required for the two populated diverted NIF beam paths onto the DLI target as well as the diagnostic optical beam path. Existing NIF alignment subsystems do not offer references that meet DLI’s unique demand. The new DLI Red Box, which has been designed to allow for alignment, has been shown to require deviation from the intended configuration and operational use case to obtain adequate functionality. A systems engineering evaluation has identified a solution that meets the stakeholder requirements while optimizing key performance parameters. The solution, referred to in this document as the Red Box “+” Rotated, was determined to be an improved version of the current DLI Red Box. This system offers improved system repeatability and alignment stability while maintaining similar interfaces and decreasing the demand for engineer/operator interaction.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

High-Efficiency, High-Current Laser-Driven Electron Injector

This final report describes research conducted under DOE Award DE-SC0021132, "High-Efficiency, High-Current Laser-Driven Electron Injector," during the period 09/01/2020–08/31/2023. The project investigates a largely unexplored regime of short-pulse laser–plasma interaction near the quarter-critical density in ultrathin gas targets as a novel electron injection mechanism for laser–wakefield acceleration (LWFA). The overarching goal is to develop high-efficiency, high-current electron sources driven by modest peak-intensity lasers at high repetition rate, suitable as compact injectors or front-ends for future laser-based accelerators.

43 PARTICLE ACCELERATORS↗