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At least 577 records · Page 32
All sourcesNASA NTRSDOE OSTI
DOE OSTI2013

Collocation and integration of reprocessing and repositories: implications for aqueous flowsheets and waste management

It is an accident of history that the current model of the fuel cycle is a separate set of facilities connected by transportation. The question is whether collocation and integration of reprocessing and fuel fabrication with the repository significantly reduce the costs of a closed fuel cycle while improving system performance in terms of safety and long-term repository performance. This paper examines the question in terms of higher-level functional requirements of reprocessing systems and geological repositories.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2022

Chemical Thermodynamic Modeling of Molten Salts to Support Off-Gas Abatement Systems

The reprocessing of used nuclear fuel by any means will liberate gaseous fission products, such as hydrogen ( 3 H), carbon ( 14 C), noble gases ( 85 Kr), and halogens ( 129 I), from the irradiated fuel. These elements will distribute through chemical processing operations and partition into process off-gas streams, and the specific volatile release fractions will be dictated by the chemical and physical properties of the system. A recent assessment found that there were significant knowledge gaps regarding the release quantities of volatile radionuclides from individual unit operations. These knowledge gaps limited the ability to determine what dedicated off-gas treatment technologies could be required for electrochemical-based reprocessing facilities. Unfortunately, experimental efforts to quantify release fractions are limited by the challenges associated with performing experiments using irradiated fuel. This report documents preliminary thermodynamic predictions of iodine and tritium release from chloride-based molten salts as part of an effort to better direct resources toward those experiments (both simulant and irradiated) that will be of the greatest impact. It was predicted that less than 0.5% of tritium was expected to be released and that nearly all of that amount would be released as H 2 . Thermochemical data for hydrogen (H 2 ) are of high fidelity, and no additional validation is recommended. Less than 0.05% of iodine was predicted to be released, with the primary volatile species being Cs 2 I 2 . Unlike the tritium predictions, the data underpinning the iodine release predictions are of low quality. It is recommended that a limited experimental program be dedicated to expanding the current physical property and thermodynamic property data for iodine in electrochemical processing and molten salt conditions, including vapor pressure measurements for the dimerized species predicted to comprise the majority of iodine release. Validating and improving the thermodynamic properties used in predictive modeling can reduce the need for expensive testing with irradiated fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2016

Voltammetry Method Evaluation

The purpose of the ANL MPACT Voltammetry project is to evaluate the suitability of previously developed cyclic voltammetry techniques to provide electroanalytical measurements of actinide concentrations in realistic used fuel processing scenarios. The molten salts in these scenarios are very challenging as they include high concentrations of multiple electrochemically active species, thereby creating a variety of complications. Some of the problems that arise therein include issues related to uncompensated resistance, cylindrical diffusion, and alloying of the electrodeposited metals. Improvements to the existing voltammetry technique to account for these issues have been implemented, resulting in good measurements of actinide concentrations across a wide range of adverse conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

The Electron Thermal Conductivity of Pu and Zr Substituted Gamma-Uranium

Uranium alloys are attractive recycled nuclear fuels because of their high thermal conductivity (k) and fissile density; however, the effects of alloying elements on k remain unclear. Here, the electron thermal conductivity (k_e) of U-Pu-Zr compositions are calculated using density functional theory. The electronic structure is evaluated to understand the effects of plutonium (Pu) and zirconium (Zr) substitution on the k_e of ?-U. Alloys of up to 37.5 at. % Pu and 37.5 at. % Zr are examined. Two methods are applied to calculate k_e; we find that the accuracy of each method depends on the electronic and mass similarities between the solute and solvent atoms. Specifically, when the solute atom is similar in electronic structure and mass, the method that applies the electron relaxation time of ?-U is best, while if the elements are dissimilar, a mixed method that mixes several parameters associated with k_e from each element in the alloy is best. The introduction of all alloying elements decreases k_e; however, in binary compounds, Pu and Zr have different effects. Pu generally flattens the electronic bands but compensates for this deleterious effect by increasing electron density near the Fermi level. Zr flattens the electronic bands more severely without adding electron density near the Fermi level. Therefore, Zr decreases the k_e more than Pu in binary compounds. In ternary compounds, the difference between Pu and Zr is minimal due to the phononic change from the large mass change of Zr substitution, even at 12.5 at. %. Thus, we predict that higher loadings of Pu, and potentially other actinides, can be added to U-Pu-Zr compositions for faster recycling of spent fuel with without sacrificing k. We also note that these k_e calculation methods can be applied to non-fuel alloys that require k_e predictions, such as cladding, heat exchanger, and structural materials.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Fuel cycle for a fusion neutron source

The concept of a tokamak-based stationary fusion neutron source (FNS) for scientific research (neutron diffraction, etc.), tests of structural materials for future fusion reactors, nuclear waste transmutation, fission reactor fuel production, and control of subcritical nuclear systems (fusion–fission hybrid reactor) is being developed in Russia. The fuel cycle system is one of the most important systems of FNS that provides circulation and reprocessing of the deuterium–tritium fuel mixture in all fusion reactor systems: the vacuum chamber, neutral injection system, cryogenic pumps, tritium purification system, separation system, storage system, and tritium-breeding blanket. The existing technologies need to be significantly upgraded since the engineering solutions adopted in the ITER project can be only partially used in the FNS (considering the capacity factor higher than 0.3, tritium flow up to 200 m{sup 3}Pa/s, and temperature of reactor elements up to 650°C). The deuterium–tritium fuel cycle of the stationary FNS is considered. The TC-FNS computer code developed for estimating the tritium distribution in the systems of FNS is described. The code calculates tritium flows and inventory in tokamak systems (vacuum chamber, cryogenic pumps, neutral injection system, fuel mixture purification system, isotope separation system, tritium storage system) and takes into account tritium loss in the fuel cycle due to thermonuclear burnup and β decay. For the two facility versions considered, FNS-ST and DEMO-FNS, the amount of fuel mixture needed for uninterrupted operation of all fuel cycle systems is 0.9 and 1.4 kg, consequently, and the tritium consumption is 0.3 and 1.8 kg per year, including 35 and 55 g/yr, respectively, due to tritium decay.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

The TRANSCEND University Consortium: Theme 4: Nuclear Materials - 20431

The safe and secure management of Pu is a matter of international concern, with ∼250 t of separated Pu currently stockpiled worldwide. The UK's civil inventory of nuclear materials contains significant stocks of separated Pu from the reprocessing of Magnox and AGR spent fuels. The preferred option for the 138.5 tonnes of Pu is re-use as mixed oxide (MOx) fuel, although 5% is not suitable for re-use and is recommended for direct disposal. However, it will take more than 15 years to implement re-use, requiring that the Pu be kept in interim storage in its current state for that period, i.e. as PuO{sub 2} powder within inert steel storage cans at Sellafield. The focus of the work presented here is thus plutonium storage and the direct disposal of plutonium. The Research and Development needs of both are now pressing: in the case of storage due to it being the current default; in the case of immobilization and disposal because of a comparative lack of Research and Development on Pu conditioning and packaging due to policy uncertainty as to whether it would be disposed of in a Geologic Disposal Facility (GDF). Addressing these needs is complicated by Pu's high radioactivity, decay heat and radiotoxicity, criticality, nuclear safeguard requirements and, for some UK Pu contaminated materials targeted for disposal, poor inventory. Thus, there is also a critical requirement for underpinning research on Pu bearing materials in these two contexts. In response to these needs, the TRANSCEND Consortium (Transformative Science and Engineering for Nuclear Decommissioning, a multi-disciplinary collaboration of 11 universities and 8 key industry partners from across the UK's civil nuclear sector) is seeking to provide technical underpinning to ongoing option development for the UK's civil Pu stockpile. Whilst understanding the behaviour of plutonium during its re-use as MOx is beyond the scope of the TRANSCEND Consortium work plan, the main objectives of the work are: (1) For interim storage: to understand how the surface structure and properties of pristine and radiation damaged PuO{sub 2} change with time in the absence and presence of water; and (2) For immobilization and disposal: to understand the mechanisms of incorporation of Pu into ceramic and glass-ceramic waste-forms, as well as the effect on these of self-induced radiation damage. Each objective is being addressed through separate work packages, the details of which are discussed in this paper. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2016

Top Fuel 2016 Proceedings

Top Fuel, also called Light Water Reactor (LWR) Fuel Performance Meeting, is an annual topical meeting whose primary objective is to bring together leading specialists in LWR fuel from around the world to analyze advances in nuclear fuel technology and to use the findings of the latest cutting-edge research to help manufacture high performance nuclear fuels of today and tomorrow. The conference hosts 2 plenary sessions, 2 special sessions, and numerous technical sessions organized into 5 technical track ares: Track 1 - Fuel performance reliability, operations and maintenance experience; Track 2 - Advances in fuel technologies (e.g., enhanced accident tolerant fuel); Track 3 - Transient and off-normal fuel behavior; Track 4 - Used fuel storage, transportation, and reuse/recovery; and Track 5 - Fuel modeling and analysis. These proceedings gather 169 papers.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2019

Separation of Xenon from Krypton in UNF Reprocessing Off-Gas

Reprocessing of used nuclear fuel (UNF) results emits several volatile radionuclides that must be removed from the bulk off gas prior to release in order to meet U.S. regulatory emission requirements. After other volatile radionuclides have been removed, krypton (Kr) remains, along with associated with xenon (Xe) in the gas stream. The half-life of Xe is short enough that by the time UNF is sufficiently cooled to be reprocessed Xe is no longer a radiological concern and it may be release to atmosphere or collected for other purposes. Kr, however, must be placed in long term storage. In order to ensure the smallest practical volume for long term storage, the Xe, which is nearly ten times the volume of Kr, must be separated from the Kr. Although cryogenic distillation has been used successfully for this purpose, high capital and operational cost, along with safety considerations, made development of gas adsorption processes for separation of Xe and Kr attractive. INL developed an engineered form sorbent consisting of silver mordenite in a polyacrylonitrile matrix (AgZ-PAN) capable of complete separation of Xe from Kr in a single pass, allowing Kr to be captured downstream with no detectable Xe present.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2015

Solutions for management of defective fuel assemblies - 15318

Defective fuel management is a major challenge for nuclear operators when the time comes for finding a long-term solution for their used (or spent) fuel assemblies. This question of defective fuel management can be raised in several cases: - For optimizing the remaining operating costs of shutdown reactors, the spent fuel pools must be emptied as soon as possible; a solution needs therefore to be found for evacuating all the spent fuel assemblies, defective fuel assemblies and in particular defective fuel rods included; - Some utilities are today facing a saturation of their reactor spent fuel pool; evacuating the defective fuel assemblies and extracted defective fuel rods allows optimizing the space in the pool. Whereas the solutions for managing intact used fuel assemblies are well-known, a specific technical solution must be implemented for managing the defective spent fuel assemblies as well. The purpose of this paper is to describe the existing solutions for the management of all types of defective fuel assemblies. Interim Dry Storage Solution Interim dry storage of defective spent fuel assemblies is being implemented for decades in the USA. Specific operations are performed for preparing the defective fuel assemblies for interim dry storage and they are then stored with intact used fuel assemblies in the dry storage cask. The advantage of such a solution is its short-term cost effectiveness. The paper presents the existing dry interim storage solutions for defective used fuel rods, the way they are implemented, the associated operational experience. Long-term Dry Storage Solution A long-term dry storage solution for defective fuel assemblies is being developed, compliant with direct disposal requirements. The solution is based on the encapsulation of each defective fuel rod into a fuel rod capsule and an associated specific dry storage licensing approach: this is the best available technology regarding long term storage safety requirements. The paper presents this unique capsule technology, the transport and storage casks that can be used for transportation of defective fuel rods to the storage facility, and the associated transport licensing approach currently used in Europe. Treatment Solution. The most definitive way to get rid of defective fuel assemblies is their treatment (or reprocessing) in a treatment plant. There is then no need to assess the behaviour of these specific used fuel assemblies as for an interim storage facility or a final repository. The advantage of such a solution is its sustainable approach. The paper presents the existing transport and treatment solutions, the way they are implemented, the associated operational experience. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2015

Bulk characterization of (U, Pu) mixed carbide fuel for distribution of plutonium

Homogeneous distribution of plutonium in (U, Pu) mixed fuels is important from fuel performance as well as reprocessing point of view. Radiation imaging and assay techniques are employed for the detection of Pu rich agglomerates in the fuel. A simulation study of radiation transport was carried out to analyse the technique of autoradiography so as to estimate the minimum detectability of Pu agglomerates in MC fuel with nominal PuC content of 70% using Monte Carlo simulations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Steam Oxidation and Burst Testing in the Severe Accident Test Station

Within six months of the March 2011 nuclear accident at Fukushima Daiichi, research began at Oak Ridge National Laboratory (ORNL) to simulate the high temperature steam oxidation accident conditions and identify potential accident tolerant fuel (ATF) cladding [1-14]. The ORNL laboratory equipment for steam oxidation equipment was expanded and made available to the entire ATF research community as the Severe Accident Test Station (SATS) in 2012 [5,1 5], including the capability to conduct the standard integral loss of coolant accident (LOCA) experiment [9]. A second SATS has now been deployed in an ORNL hot cell for handling irradiated specimens including reprocessed UO 2 /Zr fuel [16].

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2025

Estimating Potential Tritium and Plutonium Production in North Korea’s Experimental Light Water Reactor

Our work explores North Korea's 100 MW-th Experimental Light Water Reactor (ELWR) and its potential contributions to the country's nuclear weapons program. Built at the Yongbyon Nuclear Research Center, the ELWR began operations in October 2023 and represents North Korea's first attempts at a light-water reactor using domestically-enriched, ceramic fuel. Our study examines possible configurations for energy, tritium, and tritium-plutonium co-production. Assuming a single-batch core, the ELWR can be used to annually produce 48-82 grams of tritium, which can supply 2-4 new boosted warheads each year, up to a maximum arsenal of 88-150 warheads total. Concurrent production of tritium and weapon-grade plutonium is also possible but requires reprocessing of spent ceramic fuel. Furthermore, these findings underscore how North Korea's nuclear capabilities may be advanced through the ELWR's dual-use potential.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2016

Going from Closed to Open and Then Back Again: How to Keep a Level Head

Nuclear Energy is a mature, reliable low carbon technology with a secure and abundant fuel source and is an essential contributor to the energy mix. The UK has a long history of using nuclear energy and has a long standing world class expertise in the recycling of used nuclear fuel with three generations of industrial scale reprocessing plant operating on the Sellafield site, as well as the Thorp Miniature Pilot Plant in the 1980's, and a vibrant, internationally recognised R and D capability at the National Nuclear Laboratory (NNL). However, the reprocessing plants at Sellafield are both scheduled to finish around 2020 with Thorp and Magnox plants moving to post operational clean out (POCO). This will move the UK from a closed fuel cycle to an open one. Within the UK a decision has been made to refresh the current nuclear energy plants to at least replacement of the existing nuclear fleet. This will mean the building of new nuclear power plant to ensure energy production of 16 GWe per annum. With the closure of the UK's reprocessing plants, these new nuclear power plants will operate on an open fuel cycle with long term storage of used fuel followed by disposal. However it is also recognised that this may not be enough and as such expansion scenarios ranging from 16 to 75 GWe nuclear energy production are being considered through the development of a UK Road map. Within these energy scenarios, a variety of options are being evaluated including electricity generation only, electricity generation plus heat, open versus closed fuel cycles, Generation III versus Generation IV systems and combinations of the above. What is clear is that the deciding factor on the type and mix of any energy programme will not be on technology choice alone. Instead a complex mix of Government policy, relative cost of nuclear power, market decisions and public opinion will influence the rate and direction of growth of any future energy programme. At the ANS Winter Meeting 2013 a number of these techniques were presented. What was clear from the fuel cycle scenario modelling was the requirement for the utilisation of a closed fuel cycle to enable the expansion beyond 16 GWe. It is therefore a necessity for the UK to keep options open for a potential return to a closed fuel cycle in the future. The requirement to maintain the skills and capabilities to do so will be an essential part of any future nuclear strategy. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2015

Stationary Liquid Fuel Fast Reactor

For effective burning of hazardous transuranic (TRU) elements of used nuclear fuel, a transformational advanced reactor concept named SLFFR (Stationary Liquid Fuel Fast Reactor) was proposed based on stationary molten metallic fuel. The fuel enters the reactor vessel in a solid form, and then it is heated to molten temperature in a small melting heater. The fuel is contained within a closed, thick container with penetrating coolant channels, and thus it is not mixed with coolant nor flow through the primary heat transfer circuit. The makeup fuel is semi- continuously added to the system, and thus a very small excess reactivity is required. Gaseous fission products are also removed continuously, and a fraction of the fuel is periodically drawn off from the fuel container to a processing facility where non-gaseous mixed fission products and other impurities are removed and then the cleaned fuel is recycled into the fuel container. A reference core design and a preliminary plant system design of a 1000 MWt TRU- burning SLFFR concept were developed using TRU-Ce-Co fuel, Ta-10W fuel container, and sodium coolant. Conservative design approaches were adopted to stay within the current material performance database. Detailed neutronics and thermal-fluidic analyses were performed to develop a reference core design. Region-dependent 33-group cross sections were generated based on the ENDF/B-VII.0 data using the MC2-3 code. Core and fuel cycle analyses were performed in theta-r-z geometries using the DIF3D and REBUS-3 codes. Reactivity coefficients and kinetics parameters were calculated using the VARI3D perturbation theory code. Thermo-fluidic analyses were performed using the ANSYS FLUENT computational fluid dynamics (CFD) code. Figure 0.1 shows a schematic radial layout of the reference 1000 MWt SLFFR core, and Table 0.1 summarizes the main design parameters of SLFFR-1000 loop plant. The fuel container is a 2.5 cm thick cylinder with an inner radius of 87.5 cm. The fuel container is penetrated by twelve hexagonal control assembly (CA) guide tubes, each of which has 3.0 mm thickness and 69.4 mm flat-to-flat outer distance. The distance between two neighboring CA guide tube is selected to be 26 cm to provide an adequate space for CA driving systems. The fuel container has 18181 penetrating coolant tubes of 6.0 mm inner diameter and 2.0 mm thickness. The coolant tubes are arranged in a triangular lattice with a lattice pitch of 1.21 cm. The fuel, structure, and coolant volume fractions inside the fuel container are 0.386, 0.383, and 0.231, respectively. Separate steel reflectors and B4C shields are used outside of the fuel container. Six gas expansion modules (GEMs) of 5.0 cm thickness are introduced in the radial reflector region. Between the radial reflector and the fuel container is a 2.5 cm sodium gap. The TRU inventory at the beginning of equilibrium cycle (BOEC) is 5081 kg, whereas the TRU inventory at the beginning of life (BOL) was 3541 kg. This is because the equilibrium cycle fuel contains a significantly smaller fissile fraction than the LWR TRU feed. The fuel inventory at BOEC is composed of 34.0 a/o TRU, 41.4 a/o Ce, 23.6 a/o Co, and 1.03 a/o solid fission products. Since uranium-free fuel is used, a theoretical maximum TRU consumption rate of 1.011 kg/day is achieved. The semi-continuous fuel cycle based on the 300-batch, 1- day cycle approximation yields a burnup reactivity loss of 26 pcm/day, and requires a daily reprocessing of 32.5 kg of SLFFR fuel. This yields a daily TRU charge rate of 17.45 kg, including a makeup TRU feed of 1.011 kg recovered from the LWR used fuel. The charged TRU-Ce-Co fuel is composed of 34.4 a/o TRU, 40.6 a/o Ce, and 25.0 a/o Co.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2013

Neutronics of accelerator-driven subcritical fission for burning transuranics in used nuclear fuel

We report the development of a conceptual design for accelerator-driven subcritical fission in a molten salt core (ADSMS). ADSMS is capable of destroying all of the transuranics at the same rate and proportion as they are produced in a conventional nuclear power plant. The ADSMS core is fueled solely by transuranics extracted from used nuclear fuel and reduces its radiotoxicity by a factor 10,000. ADSMS offers a way to close the nuclear fuel cycle so that the full energy potential in the fertile fuels uranium and thorium can be recovered.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2017

Experience in Decommissioning of Nuclear Fuel Cycle Facilities in Germany - 17195

Several nuclear fuel cycle facilities have been decommissioned in Germany and the sites released from regulatory control. There is an overview of past and current decommissioning projects of fuel cycle facilities, either past fuel element fabrication facilities or past and current (experimental) reprocessing facilities. Several examples of technological advances are given, being developed due to obstacles, which occurred during conduct of these decommissioning projects. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2017

Delayed gamma-ray spectroscopy with lanthanum bromide detector for non-destructive assay of nuclear material

High-energy delayed γ-ray spectroscopy is a potential technique for directly assaying spent fuel assemblies and achieving the safeguards goal of quantifying nuclear material inventories for spent fuel handling, interim storage, reprocessing facilities, repository sites, and final disposal. Requirements for the γ-ray detection system, up to ~6 MeV, can be summarized as follows: high efficiency at high γ-ray energies, high energy resolution, good linearity between γ-ray energy and output signal amplitude, ability to operate at very high count rates, and ease of use in industrial environments such as nuclear facilities. High Purity Germanium Detectors (HPGe) are the state of the art and provide excellent energy resolution but are limited in their count rate capability. Lanthanum Bromide (LaBr 3 ) scintillation detectors offer significantly higher count rate capabilities at lower energy resolution. Thus, LaBr 3 detectors may be an effective alternative for nuclear spent-fuel applications, where count-rate capability is a requirement. This paper documents the measured performance of a 2” (length) × 2” (diameter) of LaBr3 scintillation detector system, coupled to a negatively biased PMT and a tapered active high voltage divider, with count-rates up to ~3 Mcps. An experimental methodology was developed that uses the average current from the PMT’s anode and a dual source method to characterize the detector system at specific very high count rate values. Delayed γ-ray spectra were acquired with the LaBr 3 detector system at the Idaho Accelerator Center, Idaho State University, where samples of ~3g of 235 U were irradiated with moderated neutrons from a photo-neutron source. Results of the spectroscopy characterization and analysis of the delayed γ-ray spectra acquired indicate the possible use of LaBr3 scintillation detectors when high count rate capability may outweigh the lower energy resolution.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Molten Salt Reactors and Electrochemical Reprocessing: Synthesis and Chemical Durability of Potential Waste Forms for Metal and Salt Waste Streams

The molten salt reactor (MSR) is one of the leading advanced nuclear reactor candidates to replace current nuclear reactor technologies in the U.S. Besides having more economical and reliable designs, MSRs have are amenable to a closed fuel cycle, in which electrochemical reprocessing can be performed to recycle the used nuclear fuel. This review intends to provide information about potential waste forms for metal and salt waste streams from these salt-based nuclear processes. Metal waste streams arise from reactor components and structural materials. Salt waste streams are generated during reactor operations as fission products build up in salt-fueled systems. Waste forms that have the highest waste loading and/or have shown the most commercial promise are discussed with an emphasis on the current state of efforts to understand the synthesis and chemical durability of metal and ceramic waste forms.

molten salt reactors, electrochemical reprocessing↗