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At least 559 records · Page 31

A new non-diffusional gas bubble production route in used nuclear fuel: Implications for fission gas release, cladding corrosion, and next generation fuel design

The relationship between noble metal phase particles and fission gas bubble production in used nuclear fuel is described. The majority of Te atoms within noble metal phase undergo radioactive decay to form stable Xe within a few hours after particle formation. This results in the production of clusters of Xe atoms contained within the solid metal matrix exhibiting an equivalent gas bubble pressure approaching 1 GPa. These high pressure bubbles are stabilized by the UO2 within the bulk of the fuel. However, when these bubbles form near the fuel / cladding interface, in combination with local and temporal damage caused by fission recoil, they are capable of overcoming the fracture strength of the UO2 and rupturing catastrophically. The force of the resulting bubble rupture is sufficient to eject noble metal phase particles several microns into the cladding. This proposed mechanism explains the observance of noble metal phase in cladding and is consistent with a host of morphological features found near the fuel / cladding interface.

Schwantes, Jon M.↗

Electrochemical Dilatometry of Si-Bearing Electrodes: Dimensional Changes and Experiment Design

The severe volumetric changes in Si particles during the Li (de)alloying process cause expansion and contraction of the electrodes, which along with excessive electrolyte reduction and solid electrolyte interphase formation brings about rapid decay in cell capacity. In this work, we use operando electrochemical dilatometry to quantify the (de)lithiation-induced expansion/contraction of Si-based and graphite-rich electrodes during electrochemical cycling. We evaluate the relationship between electrode capacity and dilation and observe that by increasing the Si contribution to the electrode capacity, the swelling is aggravated upon lithiation. For silicon-rich anodes, the electrode dilation can be higher than 300%, and the expansion profile consists of a combination of slow swelling at low lithiation followed by an accelerated increase at higher lithium contents. We investigate how electrode properties, such as porosity, affect the dilation profile and quantify the irreversible expansion of the electrodes. Finally, we discuss some of the challenges associated with the dilatometry technique and suggest experimental approaches for obtaining consistent and reliable data.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Physical conditions for conducting radiobiological experiments in beams of accelerated particles with high linear energy transfer

The design and construction of an accelerator to conduct radiobiological experiments is reported that uses aluminum filters to control the accelerated ion beam while preserving its stability, and a vacuum chamber to conduct the ion beam with the help of a collector through a lavsan exit port to the target. Depth distribution of the absorbed dose from a monodirectional ion beam is practically completely represented by the change in the energy spectrum of the biological object.

Kudryashov, Y. I.↗

Particle contamination from Martin Optical Black

The design of the barrel baffle of the Infrared Astronomical Satellite (IRAS) Optical Subsystem to minimize production of particulate contamination is described. The configuration of the 50-inch long, 28.5-inch diameter baffle required pop-rivet assembly after coating with Martin Optical Black for stray light suppression. An experiment to determine the contamination produced at assembly led to the modification of the baffle construction to preclude such damage to the coated surfaces.

Young, P. J.↗

Automated calibration of a flight particle spectrometer

An automatic calibration system was designed for use in the vacuum facility at the Space Science Laboratory of the Marshall Space Flight Center. That system was developed and used in the intervening winter to calibrate the ion spectrometer that eventually flew in May 1986 aboard the NASA project, CRIT 1. During this summer, it is planned to implement the calibration of both an ion and electron spectrometer of a new design whose basic elements were conceived during the winter of 1985 to 1986. This spectrometer was completed in the summer and successfully mounted in the vacuum tank for calibration. However, the source gate valve malfunctioned, and, at the end of the summer, it still needed a replacement. During the inevitable delays in the experimental research, the numerical model of the Critical Velocity effect was completed and these results were presented.

Torbert, Roy B.↗

Airborne Laser Polar Nephelometer

A polar nephelometer has been developed at NCAR to measure the angular variation of the intensity of light scattered by air molecules and particles. The system has been designed for airborne measurements using outside air ducted through a 5-cm diameter airflow tube; the sample volume is that which is common to the intersection of a collimated source beam and the detector field of view within the airflow tube. The source is a linearly polarized helium-neon laser beam. The optical system defines a collimated field-of-view (0.5deg half-angle) through a series of diaphragms located behind a I72-mm focal length objective lens. A photomultiplier tube is located immediately behind an aperture in the focal plane of the objective lens. The laser beam is mechanically chopped (on-off) at a rate of 5 Hz; a two-channel pulse counter, synchronized to the laser output, measures the photomultiplier pulse rate with the light beam both on and off. The difference in these measured pulse rates is directly proportional to the intensity of the scattered light from the volume common to the intersection of the laser beam and the detector field-of-view. Measurements can be made at scattering angles from 15deg to 165deg with reference to the direction of propagation of the light beam. Intermediate angles are obtained by selecting the angular increments desired between these extreme angles (any multiple of 0.1deg can be selected for the angular increment; 5deg is used in normal operation). Pulses provided by digital circuits control a stepping motor which sequentially rotates the detector by pre-selected angular increments. The synchronous photon-counting system automatically begins measurement of the scattered-light intensity immediately after the rotation to a new angle has been completed. The instrument has been flown on the NASA Convair 990 airborne laboratory to obtain data on the complex index of refraction of atmospheric aerosols. A particle impaction device is operated simultaneously to collect particles from the same airflow tube used to make the scattered-light measurements. A size distribution function is obtained by analysis of the particles collected by the impaction device. Calculated values of the angular variation of the scattered-light intensity are obtained by applying Mie scattering theory to the observed size distribution function and assuming different values of the complex index of refraction of the particles. The calculated values are then compared with data on the actual variation of the scattered-light intensity obtained with the polar nephelometer. The most probable value of the complex refractive index is that which provides the best fit between the experimental light scattering data and the parameters calculated from the observed size distribution function.

Grams, Gerald W.↗

Radiation Effects and Protection for Moon and Mars Missions

Manned and robotic missions to the Earth's moon and Mars are exposed to a continuous flux of Galactic Cosmic Rays (GCR) and occasional, but intense, fluxes of Solar Energetic Particles (SEP). These natural radiations impose hazards to manned exploration, but also present some constraints to the design of robotic missions. The hazards to interplanetary flight crews and their uncertainties have been studied recently by a National Research Council Committee (Space Studies Board 1996). Considering the present uncertainty estimates, thick spacecraft shielding would be needed for manned missions, some of which could be accomplished with onboard equipment and expendables. For manned and robotic missions, the effects of radiation on electronics, sensors, and controls require special consideration in spacecraft design. This paper describes the GCR and SEP particle fluxes, secondary particles behind shielding, uncertainties in radiobiological effects and their impact on manned spacecraft design, as well as the major effects on spacecraft equipment. The principal calculational tools and considerations to mitigate the radiation effects are discussed, and work in progress to reduce uncertainties is included.

Parnell, Thomas A.↗

Towards accelerating particle-resolved direct numerical simulation with neural operators

In this paper, we present our ongoing work aimed at accelerating a particle-resolved direct numerical simulation model designed to study aerosol–cloud–turbulence interactions. The dynamical model consists of two main components—a set of fluid dynamics equations for air velocity, temperature, and humidity, coupled with a set of equations for particle (i.e., cloud droplet) tracing. Rather than attempting to replace the original numerical solution method in its entirety with a machine learning (ML) method, we consider developing a hybrid approach. We exploit the potential of neural operator learning to yield fast and accurate surrogate models and, in this study, develop such surrogates for the velocity and vorticity fields. We discuss results from numerical experiments designed to assess the performance of ML architectures under consideration as well as their suitability for capturing the behavior of relevant dynamical systems.

54 ENVIRONMENTAL SCIENCES↗

MPEX High Heat Flux Plasma Dump Design, Manufacture, and Articles Test

Here, the Material Plasma Exposure eXperiment (MPEX) device is a steady-state linear plasma device currently in the final design phase at the Oak Ridge National Laboratory. This device will reach ion fluences up to 10 31 m -2 and will be used to expose neutron-irradiated materials to divertor-relevant plasmas and to study the effects of plasma-material interactions. These studies will elucidate the complex effects of plasmas with divertor candidate materials capable of withstanding high heat flux and high fluences for next-generation fusion devices. Bidirectional plasma will be generated using a high-power (200 kW) helicon source. Plasma will be confined by superconducting magnets. The last plasma-facing component on the upstream side of the MPEX device is the dump, which has been designed to intercept plasma and energetic particles. The dump will have a total heat load of 9.2 kW. A copper alloy (Glidcop AL-15) was selected for use in the water-cooled flange design because of its high thermal conductivity, its retaining strength at elevated temperatures, and its ability to be used in the high-temperature braze joints used in this application. Titanium-zirconium-molybdenum (TZM) tiles are brazed to the Glidcop AL-15 flange using high-temperature braze alloy. External water-cooling channels are used on the dump flange to prevent water leakage inside the vacuum space. This article discusses the details of the high heat flux dump design, including the computational fluid dynamics (CFD) and structural analyses performed to validate the design to meet the operational requirements of the MPEX device.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

3D TRISO particle-explicit compact meshing

The TRI-structural ISOtropic (TRISO) layered fuel particle is a robust nuclear fuel form offering enhanced safety and performance for advanced reactor concepts, including high-temperature gas-cooled reactors and other Generation IV designs. These poppy-seed-sized particles are embedded in a graphite matrix to form fuel elements that must withstand elevated temperatures and high burn-up levels. The heterogeneous nature of these fuel elements — comprising thousands of randomly distributed TRISO particles — produces complex stress fields and thermal gradients that one- and two-dimensional models cannot accurately capture. While three-dimensional modeling has improved predictions of dimensional changes, internal pressure buildup, and fission product transport under irradiation, current approaches rely on homogenized material properties that are known to have considerable divergence from experimental observations. This work presents a methodology for optimized random packing of TRISO fuel compacts and full three-dimensional mesh generation within the BISON fuel performance code, with each particle coating layer individually discretized. The resulting mesh was demonstrated through heat conduction simulations under representative in-reactor operating conditions, showing strong agreement with expected behavior. This capability enables detailed analysis of particle-to-particle interactions, matrix cracking mechanisms, and the statistical distribution of coating layer failures — all of which directly govern fuel performance and safety margins.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The Orbiting Wide-Angle Light Collectors (OWL) Mission for Charged-Particle Astronomy

The space-based OWL mission is designed to perform high-statistics measurements of ultra-high-energy cosmic rays (UHECR) using the Earth's atmosphere as a vast particle calorimeter, furthering the field of charged-particle astronomy. OWL has been developed in formal NASA instrument and mission studies and is comprised of two large telescopes separated by approx.600 km in 1000 km, near-equatorial orbits to stereoscopically image the near-UV air fluorescence emitted by UHECR-induced particle cascades. The High Resolution Fly's Eye (HiRes) Collaboration, and subsequently the Pierre Auger Observatory, recently reported confirmation of the expected Greisen-Zatsepin-Kuzmin (GZK) suppression of the UHECR flux above a few times 10(exp 19) eV. This observation is consistent with the majority of UHECR originating in astrophysical objects and reduces the need to invoke exotic physical processes. Particles observed above the GZK threshold energy must have come from sources within about 100 Mpc from the Earth. The small particle deflection angles expected at UHECR energies, with standard assumptions of extragalactic magnetic fields, are on the order of 1 degree. Thus by observing particles above the GZK threshold with sufficient exposure, there is the potential of identifying and characterizing individual UHECR sources. Auger has reported significant anisotropy in the arrival directions of UHECR at energies above about 6 10(exp 19) eV observed in the South, and a correlation to AGN in the 12th VCV catalog, suggesting that the sources of UHECR are traced by the distribution of luminous matter in the Universe. However, with similar statistics and the same event selection criteria, HiRes observations in the North are consistent with isotropy. Extended observations by Auger-South, by Telescope Array in the North, and possibly by the proposed Auger-North, will further these investigations. However, much greater exposures will be required to fully identify individual sources and measure their cosmic ray spectra. A five-year OWL mission would deliver approximately 10(exp 6)sq km/sr/yr of exposure with full aperture reached at approx. 10(exp 19) eV. The baseline 3 m optical aperture OWL telescopes with 45 degree full field-of-view are easily accomodated on a single conventional launch vehicle. On orbit, the simultaneous viewing of the same volume of atmosphere allows for precise stereo event reconstruction, which is nearly independent of the inclination of the particle track and tolerant of atmospheric conditions. The availability of monocular operation provides increased reliability or can be employed to increase the instantaneous aperture. In stereo mode, OWL is also capable of fully reconstructing horizontal or upward-moving showers and so has unmatched sensitivity to neutrino-induced events. The details of the OWL mission will he presented and its science capabilities will be discussed.

Mitchell, John↗

The Magnetospheric Multiscale Mission...Resolving Fundamental Processes in Space Plasmas

The Magnetospheric Multiscale (MMS) mission is a multiple-spacecraft Solar-Terrestrial Probe designed to study the microphysics of magnetic reconnection, charged particle acceleration, and turbulence in key boundary regions of Earth's magnetosphere. These three processes, which control the flow of energy, mass, and momentum within and across plasma boundaries, occur throughout the universe and are fundamental to our understanding of astrophysical and solar system plasmas. Only in Earth's magnetosphere, however, are they readily accessible for sustained study through in-situ measurement. MMS will employ five co-orbiting spacecraft identically instrumented to measure electric and magnetic fields, plasmas, and energetic particles. The initial parameters of the individual spacecraft orbits will be designed so that the spacecraft formation will evolve into a three-dimensional configuration near apogee, allowing MMS to differentiate between spatial and temporal effects and to determine the three dimensional geometry of plasma, field, and current structures. In order to sample all of the magnetospheric boundary regions, MMS will employ a unique four-phase orbital strategy involving carefully sequenced changes in the local time and radial distance of apogee and, in the third phase, a change in orbit inclination from 10 degrees to 90 degrees. The nominal mission operational lifetime is two years. Launch is currently scheduled for 2006.

Curtis, S.↗

Artificial Intelligence for imaging Cherenkov detectors at the EIC

Abstract Imaging Cherenkov detectors form the backbone of particle identification (PID) at the future Electron Ion Collider (EIC). Currently all the designs for the first EIC detector proposal use a dual Ring Imaging CHerenkov (dRICH) detector in the hadron endcap, a Detector for Internally Reflected Cherenkov (DIRC) light in the barrel, and a modular RICH (mRICH) in the electron endcap. These detectors involve optical processes with many photons that need to be tracked through complex surfaces at the simulation level, while for reconstruction they rely on pattern recognition of ring images. This proceeding summarizes ongoing efforts and possible applications of AI for imaging Cherenkov detectors at EIC. In particular we will provide the example of the dRICH for the AI-assisted design and of the DIRC for simulation and particle identification from complex patterns and discuss possible advantages of using AI.

Instruments & Instrumentation↗

Magellan star scanner experiences - What a long, stange trip it's been

Since its launch to Venus in 1989, the Magellan spacecraft has encountered a variety of interesting phenomena - several related to its star scanner. After much concentration, it was determined that the scanner events were due to environmental effects on the instrument - in particular, its response to solar protons and an unanticipated amount of thermal blanket dust (this dust is, in turn, generated and moved by other environmental forces). In short, while those phenomena were originally an operational nuisance, our scanner has unexpectedly shown new use as a particle and fields detector. Since its simple design makes Magellan's star scanner a good proton detector, a brief description of the charged-particle environment (particularly proton propagation) is also included. Short- and long-term trends in sensor behavior are presented, as are their correlations to the local environment. A summary of results to date is provided in the hope that these may be of help to future operations teams diagnosing similar phenomena. A summary is also given of methods found to reduce the operational impact of these phenomena.

Seale, Eric H.↗

Cell and Particle Interactions and Aggregation During Electrophoretic Motion

The objectives of this research were (i) to perform experiments for observing and quantifying electrophoretic aggregation, (ii) to develop a theoretical description to appropriately analyze and compare with the experimental results, (iii) to study the combined effects of electrophoretic and gravitational aggregation of large particles, and the combined effects of electrophoretic and Brownian aggregation of small particles, and (iv) to perform a preliminary design of a potential future flight experiment involving electrophoretic aggregation. Electrophoresis refers to the motion of charged particles, droplets or molecules in response to an applied electric field. Electrophoresis is commonly used for analysis and separation of biological particles or molecules. When particles have different surface charge densities or potentials, they will migrate at different velocities in an electric field. This differential migration leads to the possibility that they will collide and aggregate, thereby preventing separation.

Davis, Robert H.↗

Co-optimizing water-alternating-carbon dioxide injection projects using a machine learning assisted computational framework

In this report, a robust machine-learning-based computational framework that couples multi-layer neural network (MLNN) proxies and a multi-objective particle swarm optimizer (MOPSO) to design water-alternating-carbon dioxide injection (CO 2 -WAG) projects is presented. The proposed optimization protocol considers various objectives, including oil recovery and CO 2 storage volume. Expert MLNN systems are trained and employed as surrogate models of the high-fidelity compositional simulator in the optimization workflow. When multiple objective functions are considered, two approaches are employed to treat the objectives: the weighted sum method and the Pareto-front-based scheme. A field-scale implementation focusing on tertiary recovery in the Morrow B formation at Farnsworth Unit (FWU) is presented. The developed Pareto-optimal solutions indicate the maximal available oil production can be 1.64 × 10 7 barrels and maximal carbon storage can achieve 2.35 × 10 7 tons. Trade-offs factor is defined to divide the constructed Pareto front into 4 sections with the trade-off factors’ value ranges from 0.35 to 49.9. This work also compares the optimum solution found by the aggregative objective function and the solution repository covered by the Pareto front that considers the physical and operational constraints and reduces uncertainties involved by the multi-objective optimization process. Our comparison indicates multiple solutions exist to satisfy the objective criteria of the WAG design, and these results cannot be found using the traditional weighted sum method. The Pareto front solution can provide more options for project designers, but decisions regarding necessary trade-offs must be made using the solution repository to balance the project economics and CO 2 storage amount.

10 SYNTHETIC FUELS↗

Post-irradiation examination of AGR-3/4 TRISO fuel compacts using three-dimensional X-ray computed tomography

The AGR-3/4 irradiation tests combined the third and fourth planned irradiation experiments in the US Department of Energy’s Advanced Gas Reactor (AGR) testing campaign of tri-structural isotropic (TRISO) fuel compacts. In this article, we present post-irradiation examination (PIE) using X-ray computed tomography (XCT) of two unirradiated and two irradiated compacts from the AGR-3/4 irradiation tests. The irradiated compacts studied (compact 7–1 and compact 12–4) represent the upper and lower limit of burnup within the AGR-3/4 irradiation experiment. This article presents a detailed quantitative analysis on the post-irradiation structure of TRISO fuel compacts. Various quantitative parameters including shape, size, and packing of kernels, and their spatial distribution, were utilized to gain insights into the structural changes caused by irradiation. The equivalent diameter and sphericity were found to increase and decrease, respectively, in irradiated compact 7–1 due to its higher burnup. Nearest neighbor distance between fuel kernels decreased after irradiation, suggesting irradiation-induced shrinkage of graphitic matrix. Furthermore, each compact in AGR-3/4 irradiation tests contained 20 designed-to-fail (DTF) fuel particles that were meant to act as a source of fission product release to the experiment test train. Furthermore, in the present work, all DTF fuel particles in the four compacts studied were identified, and it was found that they exhibited larger kernel swelling in compact 12–4 and smaller kernel swelling in compact 7–1, compared to the driver particles.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗