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At least 559 records · Page 31

Mass Determinations of the Three Mini-Neptunes Transiting TOI-125

The Transiting Exoplanet Survey Satellite, TESS, is currently carrying out an all-sky search for small planets transiting bright stars. In the first year of the TESS survey, a steady progress was made in achieving the mission’s primary science goal of establishing bulk densities for 50 planets smaller than Neptune. During that year, the TESS’s observations were focused on the southern ecliptic hemisphere, resulting in the discovery of three mini-Neptunes orbiting the star TOI-125, a V = 11.0 K0 dwarf. We present intensive HARPS radial velocity observations, yielding precise mass measurements for TOI-125b, TOI-125c, and TOI-125d. TOI-125b has an orbital period of 4.65 d, a radius of 2.726 ± 0.075 R(E), a mass of 9.50 ± 0.88 M(E), and is near the 2:1 mean motion resonance with TOI-125c at 9.15 d. TOI-125c has a similar radius of 2.759 ± 0.10 R(E) and a mass of 6.63 ± 0.99 M(E), being the puffiest of the three planets. TOI-125d has an orbital period of 19.98 d and a radius of 2.93 ± 0.17 R(E) and mass 13.6 ± 1.2 M(E). For TOI-125b and d, we find unusual high eccentricities of 0.19 ± 0.04 and 0.17(sup +0.08, sub −0.06), respectively. Our analysis also provides upper mass limits for the two low-SNR planet candidates in the system; for TOI-125.04 (R(P) = 1.36 R(E), P = 0.53 d), we find a 2σ upper mass limit of 1.6 M(E), whereas TOI-125.05 (R(P) = 4.2(sup +2.4, sub −1.4 R(E), P = 13.28 d) is unlikely a viable planet candidate with an upper mass limit of 2.7 M(E). We discuss the internal structure of the three confirmed planets, as well as dynamical stability and system architecture for this intriguing exoplanet system.

L D Nielsen↗

Isochronal Age-mass Discrepancy of Young Stars: SCExAO/CHARIS Integral Field Spectroscopy of the HIP 79124 Triple System

We present SCExAO/CHARIS 1.1-2.4 μm integral field direct spectroscopy of the young HIP 79124 triple system. HIP 79124 is a member of the Scorpius-Centaurus association, consisting of an A0V primary with two low-mass companions at a projected separation of < 1″. Thanks to the high quality wavefront corrections provided by SCExAO, both companions are decisively detected without the employment of any PSF-subtraction algorithm to eliminate quasi-static noise. The spectrum of the outer C object is very well matched by Upper Scorpius M4 ± 0.5 standard spectra, with a T(eff) = 2945 ± 100 K and a mass of ∼350 M(Jup). HIP 79124 B is detected at a separation of only 180 mas in a highly-correlated noise regime, and it falls in the spectral range M6 ± 0.5 with T(eff) = 2840 ± 190 K and ∼100 M(Jup). Previous studies of stellar populations in Sco-Cen have highlighted a discrepancy in isochronal ages between the lower-mass and higher-mass populations. This could be explained either by an age spread in the region, or by conventional isochronal models failing to reproduce the evolution of low-mass stars. The HIP 79124 system should be coeval, and therefore it provides an ideal laboratory to test these scenarios. We place the three components in a color-magnitude diagram and find that the models predict a younger age for the two low-mass companions (∼3 Myr) than for the primary star (∼6 Myr). These results imply that the omission of magnetic effects in conventional isochronal models inhibit them from reproducing early low-mass stellar evolution, which is further supported by the fact that new models that include such effects provide more consistent ages in the HIP 79124 system.

Ruben Asensio-Torres↗

A 10,000-solar-mass black hole in the nucleus of a bulgeless dwarf galaxy

The motions of gas and stars in the nuclei of nearby galaxies have demonstrated that massive black holes are common1 and that their masses correlate with the stellar velocity dispersion σ⁎ of the bulge. This correlation suggests that massive black holes and galaxies influence each other’s growth. Dynamical measurements are less reliable when the sphere of influence is unresolved; thus, it remains unknown whether this correlation exists in galaxies much smaller than the Milky Way. Light echoes from photoionized clouds around accreting black holes, in combination with the velocity of these clouds, yield a direct mass measurement that circumvents this difficulty. Here we report an exceptionally low reverberation delay of 83 ± 14 min between variability in the accretion disk and Hα emission from the nucleus of the dwarf galaxy NGC 4395. Combined with the Hα velocity dispersion σline = 426 ± 1 km/s, this lag determines a mass of about 10,000 M⊙ for the black hole (M(BH)). This mass is among the smallest central black hole masses reported, near the low end of expected masses for heavy ‘seeds’, and the best direct mass measurement for a galaxy of this size. Despite the lack of a bulge, NGC 4395 is consistent with the M(BH–σ⁎) relation, indicating that the relation need not originate from hierarchical galaxy assembly nor from black hole feedback.

Jong-Hak Woo↗

Near future MeV telescopes can discover asteroid-mass primordial black hole dark matter

Primordial black holes (PBHs), formed out of large over densities in the early Universe, are a viable dark matter (DM) candidate over a broad range of masses. Ultralight, asteroid-mass PBHs with masses around1017g are particularly interesting as current observations allow them to constitute the entire DM density. PBHs in this mass range emit∼MeV photons via Hawking radiation which can directly be detected by the gamma ray telescopes, such as the upcoming AMEGO. In this work we forecast how well an instrument with the sensitivity of AMEGO will be able to detect, or rule out, PBHs as a DM candidate, by searching for their evaporating signature when marginalizing over the Galactic and extra-Galactic gamma-ray back-grounds. We find that an instrument with the sensitivity of AMEGO could exclude nonrotating PBHs as the only DM component for masses up to7×1017g at 95% confidence level for a monochromatic mass distribution, improving upon current bounds by nearly an order of magnitude. The forecasted constraints are more stringent for PBHs that have rotation, or which follow extended mass distributions

Anupam Ray↗

Populating the brown dwarf and stellar boundary: Five stars with transiting companions near the hydrogen-burning mass limit

We report the discovery of five transiting companions near the hydrogen-burning mass limit in close orbits around main sequence stars originally identified by the Transiting Exoplanet Survey Satellite (TESS) as TESS objects of interest (TOIs): TOI-148, TOI-587, TOI-681, TOI-746, and TOI-1213. Using TESS and ground-based photometry as well as radial velocities from the CORALIE, CHIRON, TRES, and FEROS spectrographs, we found the companions have orbital periods between 4.8 and 27.2 days, masses between 77 and 98 MJup , and radii between 0.81 and 1.66 RJup . These targets have masses near the uncertain lower limit of hydrogen core fusion (~73-96 MJup ), which separates brown dwarfs and low-mass stars. We constrained young ages for TOI-587 (0.2 ± 0.1 Gyr) and TOI-681 (0.17 ± 0.03 Gyr) and found them to have relatively larger radii compared to other transiting companions of a similar mass. Conversely we estimated older ages for TOI-148 and TOI-746 and found them to have relatively smaller companion radii. With an effective temperature of 9800 ± 200 K, TOI-587 is the hottest known main-sequence star to host a transiting brown dwarf or very low-mass star. We found evidence of spin-orbit synchronization for TOI-148 and TOI-746 as well as tidal circularization for TOI-148. These companions add to the population of brown dwarfs and very low-mass stars with well measured parameters ideal to test formation models of these rare objects, the origin of the brown dwarf desert, and the distinction between brown dwarfs and hydrogen-burning main sequence stars.

Nolan Grieves↗

Secure Mass Measurements From Transit Timing: 10 Kepler Exoplanets Between 3 and 8M⊕ with Diverse Densities and Incident Fluxes

We infer dynamical masses in eight multiplanet systems using transit times measured from Keplerʼs complete dataset, including short-cadence data where available. Of the 18 dynamical masses that we infer, 10 pass multiple tests for robustness. These are in systems Kepler-26 (KOI-250), Kepler-29 (KOI-738), Kepler-60 (KOI-2086), Kepler-105 (KOI-115), and Kepler-307 (KOI-1576). Kepler -105 c has a radius of 1.3R⊕ and a density consistent with an Earth-like composition. Strong transit timing variation (TTV) signals were detected from additional planets, but their inferred masses were sensitive to outliers or consistent solutions could not be found with independently measured transit times, including planets orbiting Kepler-49 (KOI-248), Kepler-57 (KOI-1270), Kepler-105 (KOI-115), and Kepler-177 (KOI-523). Nonetheless, strong upper limits on the mass of Kepler-177 cimply an extremely low density of 0.1 g cm−3. In most cases, individual orbital eccentricities were poorly constrained owing to degeneracies in TTV inversion. For five planet pairs in our sample, strong secular interactions imply a moderate to high likelihood of apsidal alignment over a wide range of possible eccentricities. We also find solutions for the three planets known to orbit Kepler-60 in a Laplace-like resonance chain. However, nonlibrating solutions also match the transit timing data. For six systems, we calculate more precise stellar parameters than previously known, enabling useful constraints on planetary densities where we have secure mass measurements. Placing these exoplanets on the mass–radius diagram, we find that a wide range of densities is observed among sub-Neptune-mass planets and that the range in observed densities is anticorrelated with incident flux.

Stars individual↗

Secure Mass Measurements From Transit Timing: 10 Kepler Exoplanets Between 3 and 8 M⊕ With Diverse Densities and Incident Fluxes

We infer dynamical masses in eight multiplanet systems using transit times measured from Keplerʼs complete data set, including short-cadence data where available. Of the 18 dynamical masses that we infer, 10 pass multiple tests for robustness. These are in systems Kepler-26 (KOI-250), Kepler-29 (KOI-738), Kepler-60 (KOI-2086), Kepler-105 (KOI-115), and Kepler-307 (KOI-1576). Kepler-105 c has a radius of 1.3 R(sub ⨁) and a density consistent with an Earth-like composition. Strong transit timing variation (TTV) signals were detected from additional planets, but their inferred masses were sensitive to outliers or consistent solutions could not be found with independently measured transit times, including planets orbiting Kepler-49 (KOI-248), Kepler-57 (KOI-1270), Kepler-105 (KOI-115), and Kepler-177 (KOI-523). Nonetheless, strong upper limits on the mass of Kepler-177 c imply an extremely low density of ∽0.1 g cm(exp −3). In most cases, individual orbital eccentricities were poorly constrained owing to degeneracies in TTV inversion. For five planet pairs in our sample, strong secular interactions imply a moderate to high likelihood of apsidal alignment over a wide range of possible eccentricities. We also find solutions for the three planets known to orbit Kepler-60 in a Laplace-like resonance chain. However, nonlibrating solutions also match the transit timing data. For six systems, we calculate more precise stellar parameters than previously known, enabling useful constraints on planetary densities where we have secure mass measurements. Placing these exoplanets on the mass–radius diagram, we find that a wide range of densities is observed among sub-Neptune-mass planets and that the range in observed densities is anticorrelated with incident flux.

Individual stars↗

A Wind-Driven Snow Redistribution Module for Alpine3d V3.3.0: Adaptations Designed for Downscaling Ice Sheet Surface Mass Balance

Ice sheets gain mass via snow accumulation at the ice sheet surface, which is the primary component of surface mass balance. On the Antarctic ice sheet, winds redistribute snow resulting in surface mass balance that is variable in both space and time. Representing wind-driven snow redistribution processes in models is critical for local assessments of surface mass balance, repeat altimetry studies, and interpretation of ice core accumulation records. To this end, we have adapted Alpine3D, an existing distributed snow modeling framework, to downscale Antarctic surface mass balance to horizontal resolutions up to 1 km. In particular, we have introduced a new two-dimensional advection-based wind-driven snow redistribution module that is driven by an offline coupling between WindNinja, a wind downscaling model, and Alpine3D. We then show that large accumulation variability can be at least partially explained by terrain-induced wind speed variations which subsequently redistribute snow around rolling topography. By comparing Alpine3D to airborne-derived snow accumulation measurements within a testing domain over Pine Island Glacier in West Antarctica, we demonstrate that our Alpine3D downscaling approach improves surface mass balance estimates when compared to MERRA-2, a global atmospheric reanalysis which we use as atmospheric forcing. In particular, when compared to MERRA-2, Alpine3D reduces simulated surface mass balance root mean squared error by 23.4 mm w.e.yr−1 (13%) and increases variance explained by 24%. Despite these improvements, Alpine3D still underestimates observed accumulation variability, thus providing an opportunity for future model improvement.

Eric Keenan↗

Effect of Engine Thrust and Isp Tradeoffs and Alternate Propellants on ΔV Budget and Architecture Mass for 1st Generation Nuclear Thermal Propulsion Flight Test Systems

Following the first Nuclear Thermal Propulsion (NTP) system test, also known as DRACO, the next NTP system to be developed would be the 1st Generation NTP system. An analysis was conducted to determine the performance of different vehicle configurations utilizing hydrogen (H-NTP), ammonia (A-NTP), and methane (M-NTP) as propellants launched onboard commercial launch vehicles. This was enabled by a quasi-steady-state power balance engine model and vehicle component physics that sized the vehicle system using Master Equipment List (MEL) parameters. The analysis considered configuration cases outlined by a matrix of different mission classes and vehicle configurations that covered the design space of the 1st Generation NTP system to explore various propellant options, engine architectures, and mission scopes. Four mission classes were evaluated which included single burn missions performing maneuvers having a ΔV of 1 km/s and 2.5 km/s followed by 2-burn and 4-burn missions that aimed to exhaust the launch vehicles volume or mass limitations. In all cases, the NTP systems with the lowest thrust class had the longest burn time of which A-NTP and M-NTP systems provided the longest and shortest burn times depending on the launch vehicle used while H-NTP systems tended to cluster together in the middle. Longer burn times could be useful as a testing platform to increase the time for data accumulation. Across the multi-burn cases, H-NTP systems were found to be volume limited while A-NTP and M-NTP systems were mass limited. Both single burn missions showed that A-NTP configurations provided the lowest dry mass given that ammonia had the highest density with comparable performance to M-NTP systems and no requirement for cryocoolers. The results showed that beyond the propellant selection type, the launch vehicle selection, which included Starship, New Glenn, Vulcan, Falcon 9 (recoverable), and Falcon Heavy (recoverable), was a primary driving factor in the test vehicle’s capabilities. Trends were determined based on a set of dimensionless parameters that included the mass ratio of inert mass to initial wetted mass, ratio of specific impulse to burn time, and a dimensionless engine parameter (ratio of impulse to engine momentum). These relationships found the “knees-in-the-curves” that could be a significant point of reference for the designer as they indicate a change in the trend which is located at a specific impulse to burn time ratio of 1, a mass ratio of 0.6, and an engine performance parameter of 4. This study did not attempt to make a recommendation rather provide the tools for the reader to select their own configuration based on their needs.

Propellant↗

Effect of Engine Thrust and Isp Tradeoffs and Alternate Propellants on ΔV Budget and Architecture Mass for 1st Generation Nuclear Thermal Propulsion Flight Test Systems

Following the first Nuclear Thermal Propulsion (NTP) system test, also known as DRACO, the next NTP system to be developed would be the 1st Generation NTP system. An analysis was conducted to determine the performance of different vehicle configurations utilizing hydrogen (H-NTP), ammonia (A-NTP), and methane (M-NTP) as propellants launched onboard commercial launch vehicles. This was enabled by a quasi-steady-state power balance engine model and vehicle component physics that sized the vehicle system using Master Equipment List (MEL) parameters. The analysis considered configuration cases outlined by a matrix of different mission classes and vehicle configurations that covered the design space of the 1st Generation NTP system to explore various propellant options, engine architectures, and mission scopes. Four mission classes were evaluated which included single burn missions performing maneuvers having a ΔV of 1 km/s and 2.5 km/s followed by 2-burn and 4-burn missions that aimed to exhaust the launch vehicles volume or mass limitations. In all cases, the NTP systems with the lowest thrust class had the longest burn time of which A-NTP and M-NTP systems provided the longest and shortest burn times depending on the launch vehicle used while H-NTP systems tended to cluster together in the middle. Longer burn times could be useful as a testing platform to increase the time for data accumulation. Across the multi-burn cases, H-NTP systems were found to be volume limited while A-NTP and M-NTP systems were mass limited. Both single burn missions showed that A-NTP configurations provided the lowest dry mass given that ammonia had the highest density with comparable performance to M-NTP systems and no requirement for cryocoolers. The results showed that beyond the propellant selection type, the launch vehicle selection, which included Starship, New Glenn, Vulcan, Falcon 9 (recoverable), and Falcon Heavy (recoverable), was a primary driving factor in the test vehicle’s capabilities. Trends were determined based on a set of dimensionless parameters that included the mass ratio of inert mass to initial wetted mass, ratio of specific impulse to burn time, and a dimensionless engine parameter (ratio of impulse to engine momentum). These relationships found the “knees-in-the-curves” that could be a significant point of reference for the designer as they indicate a change in the trend which is located at a specific impulse to burn time ratio of 1, a mass ratio of 0.6, and an engine performance parameter of 4. This study did not attempt to make a recommendation rather provide the tools for the reader to select their own configuration based on their needs.

Propellant↗

Effect of Engine Thrust and Isp Tradeoffs and Alternate Propellants on ΔV Budget and Architecture Mass for 1st Generation Nuclear Thermal Propulsion Flight Test Systems

Following the first Nuclear Thermal Propulsion (NTP) system test, also known as DRACO, the next NTP system to be developed would be the 1st Generation NTP system. An analysis was conducted to determine the performance of different vehicle configurations utilizing hydrogen (H-NTP), ammonia (A-NTP), and methane (M-NTP) as propellants launched onboard commercial launch vehicles. This was enabled by a quasi-steady-state power balance engine model and vehicle component physics that sized the vehicle system using Master Equipment List (MEL) parameters. The analysis considered configuration cases outlined by a matrix of different mission classes and vehicle configurations that covered the design space of the 1st Generation NTP system to explore various propellant options, engine architectures, and mission scopes. Four mission classes were evaluated which included single burn missions performing maneuvers having a ΔV of 1 km/s and 2.5 km/s followed by 2-burn and 4-burn missions that aimed to exhaust the launch vehicles volume or mass limitations. In all cases, the NTP systems with the lowest thrust class had the longest burn time of which A-NTP and M-NTP systems provided the longest and shortest burn times depending on the launch vehicle used while H-NTP systems tended to cluster together in the middle. Longer burn times could be useful as a testing platform to increase the time for data accumulation. Across the multi-burn cases, H-NTP systems were found to be volume limited while A-NTP and M-NTP systems were mass limited. Both single burn missions showed that A-NTP configurations provided the lowest dry mass given that ammonia had the highest density with comparable performance to M-NTP systems and no requirement for cryocoolers. The results showed that beyond the propellant selection type, the launch vehicle selection, which included Starship, New Glenn, Vulcan, Falcon 9 (recoverable), and Falcon Heavy (recoverable), was a primary driving factor in the test vehicle’s capabilities. Trends were determined based on a set of dimensionless parameters that included the mass ratio of inert mass to initial wetted mass, ratio of specific impulse to burn time, and a dimensionless engine parameter (ratio of impulse to engine momentum). These relationships found the “knees-in-the-curves” that could be a significant point of reference for the designer as they indicate a change in the trend which is located at a specific impulse to burn time ratio of 1, a mass ratio of 0.6, and an engine performance parameter of 4. This study did not attempt to make a recommendation rather provide the tools for the reader to select their own configuration based on their needs.

Propellant↗

Beyond $Δm^2$: Absolute Mass Sensitivity in Neutrino Oscillations

Conventional wisdom says that neutrino oscillations measure only mass-squared differences and not the absolute neutrino mass scale. This is true, however, only at leading order in the expansion parameters $m_i/E$, the ratios of the neutrino masses $m_i$ ($i=1,2,3$) to the neutrino energy $E$. At next-to-leading order, the oscillation phase includes terms proportional to $m_i^4-m_j^4 = Δm^2_{ij}(m_i^2+m_j^2)$, and is therefore sensitive to the absolute mass scale. In this paper, we derive the next-to-leading-order corrections using a wave-packet treatment and taking into account the neutrino-production kinematics. We then apply this result to reactor antineutrinos and find that the JUNO experiment is sensitive to neutrino masses of a few hundred keV. While not competitive with existing bounds from beta decay, electron capture, and cosmology, neutrino oscillations provide a novel, complementary probe of the neutrino mass scale, with sensitivity to a different combination of neutrino masses.

Alves, Gustavo F.S. [Fermilab; Argonne; Northweste↗

High and Ultra-High Temperature Reaction Kinetics by Single Nanoparticle Mass Spectrometry

Methodology is presented for non-destructive, optically-detected single nanoparticle (NP) mass spectrometry, with the goal of extracting surface reaction kinetics for single NPs at high temperatures. Methods for determining the NP charge, mass, and temperature as a function of time are discussed, and the data are used to extract both the absolute kinetics for mass change, as well as the efficiencies of the surface processes that cause them. Factors that contribute to the uncertainties in absolute and relative mass determination, and in the resulting kinetic parameters, are discussed. The method allows the NP-to-NP variations in initial reactivity to be measured directly, along with the time evolution of reactivity resulting from NP structural/compositional changes that occur under reaction conditions. The strengths and limitations of single nanoparticle mass spectrometry as a high temperature surface kinetics tool are discussed in the context of sublimation and O2 oxidation kinetics experiments for single hafnium (Hf) NPs at temperatures ranging above 2400 K. The Hf oxidation kinetics are compared to analogous oxidation experiments for silicon, graphite, and carbon black NPs. In all four cases, the oxidation chemistry was dominated by processes that result in net mass loss, and the distinct mechanisms responsible are discussed. All four NPs also eventually passivated, i.e., the efficiencies for oxidative etching decreased by at least two orders of magnitude, relative to the initial efficiencies. Furthermore, the passivation mechanisms, which are quite different for carbon, compared to silicon or hafnium, are discussed. Carbon NP passivation is attributed to structural isomerization leading to fully coordinated, fullerene-like NP surfaces, while for silicon and hafnium, passivation results from delayed formation of an oxide layer, triggered by accumulation of oxygen in the NP sub-surface region.

36 MATERIALS SCIENCE↗

Investigating nuclear structure near N=32 and N=34: Precision mass measurements of neutron-rich Ca, Ti, and V isotopes

Nuclear mass measurements of isotopes are key to improving our understanding of nuclear structure across the chart of nuclides, in particular, for the determination of the appearance or disappearance of nuclear shell closures. Here, we present high-precision mass measurements of neutron-rich Ca, Ti, and V isotopes performed at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN) and the Low Energy Beam and Ion Trap (LEBIT) facilities. These measurements were made using the TITAN multiple-reflection time-of-flight mass spectrometer (MR-ToF-MS) and the LEBIT 9.4T Penning trap mass spectrometer. In total, 13 masses were measured, 8 of which represent increases in precision over previous measurements. These measurements refine trends in the mass surface around N=32 and N=34, and support the disappearance of the N=32 shell closure with increasing proton number. Additionally, our data do not support the presence of a shell closure at N=34.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Small Body GN and C Research Report: G-SAMPLE - An In-Flight Dynamical Method for Identifying Sample Mass [External Release Version]

G-SAMPLE is an in-flight dynamical method for use by sample collection missions to identify the presence and quantity of collected sample material. The G-SAMPLE method implements a maximum-likelihood estimator to identify the collected sample mass, based on onboard force sensor measurements, thruster firings, and a dynamics model of the spacecraft. With G-SAMPLE, sample mass identification becomes a computation rather than an extra hardware requirement; the added cost of cameras or other sensors for sample mass detection is avoided. Realistic simulation examples are provided for a spacecraft configuration with a sample collection device mounted on the end of an extended boom. In one representative example, a 1000 gram sample mass is estimated to within 110 grams (95% confidence) under realistic assumptions of thruster profile error, spacecraft parameter uncertainty, and sensor noise. For convenience to future mission design, an overall sample-mass estimation error budget is developed to approximate the effect of model uncertainty, sensor noise, data rate, and thrust profile error on the expected estimate of collected sample mass.

in-flight sample-mass identification↗

The structure of quark mass corrections in the gg → HH amplitude at high-energy

The leading and next-to-leading order QCD predictions for Higgs boson pair production at hadron colliders suffer from a significant mass renormalisation scheme uncertainty related to the choice of the top-quark mass. The functional dependence of the result on the value of the intermediate quark mass can be understood in the high-energy limit using the Method of Regions and the tools of Soft-Collinear Effective Theory. In this work, we study the origin of the sizeable logarithmic mass corrections in the gg → HH amplitudes at leading and next-to-leading power in the limit s, |t|, |u| ≫ ${m}_t^2$ ≫ ${m}_H^2$. We argue that the mass corrections follow a predictable factorised pattern that can be exploited to simplify their computation. We present results for the leading power leading logarithmic corrections, our analysis leads to a significant reduction in the theoretical uncertainty of the double Higgs production amplitudes at scattering energies ≳ 1 TeV due to the top-quark mass scheme.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Development, feasibility, and uncertainty of radioactive 22 Na tracer dilution and gamma spectroscopy for mass determination of molten salt for pyroprocessing spent nuclear fuels

Accurate knowledge of the total mass of molten salts both for pyroprocessing spent nuclear fuels and for molten salt reactors is necessary for safeguards purposes. However, it is challenging to know or measure the total mass of molten salt due to the complicated shapes as well as the compositional—and thus density—changes that occur over time during operation. Here, we investigated radioactive tracer dilution (RTD) as a potential safeguards technique for application to the total mass measurement of LiCl–KCl–UCl 3 salt used for uranium electrorefining, with a focus on the feasibility, uncertainty, and fission product effect of RTD for salt mass measurement. To this end, experimental-scale RTD tests (600–700 g of total mass) were initially carried out by adding 22 Na tracer salt into LiCl–KCl salt containing 0, 5, and 28wt% radioactive salts from an electrorefiner (ER) for refining uranium. Upon the completion of the experimental-scale RTD tests, we performed a scale-up RTD test by directly adding 22 Na tracer salts to the ER, which uses about 12 kg of LiCl–KCl–UCl 3 salt during normal operation. This paper reports the main features of RTD for total mass measurement of molten salt and summarizes the results of the experimental-scale and scale-up RTD tests.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Analysis of an irradiated uranium sample for source attribution without chemical separation using microplasma ionization and ultrahigh resolution mass spectrometry

The use of element isotope ratios has great potential in not only determining the reactor type used to produce plutonium (Pu) but also in determining the burnup and the time since irradiation. While a powerful nuclear forensic technique, determining element isotope ratios is complicated by severe isobaric interferences when performed on typical inductively coupled plasma mass spectrometers. Such analyses require extensive chemical separations prior to analysis to alleviate the inter-elemental isobars. Ultrahigh mass resolution spectrometry provides a potential alternative, greatly reducing the complexity of sample preparation and turnaround times for these critical measurements. To demonstrate the power of the approach, a sample of irradiated, depleted uranium was analyzed with the liquid sampling—atmospheric pressure glow discharge ion source coupled to an Orbitrap mass spectrometer. The Orbitrap is augmented with an external data acquisition system, Spectroswiss’s FTMS-Booster X2T, allowing collection of extended ion transients, providing higher mass resolution. In using this approach, the 150 Sm/ 149 Sm and 152 Sm/ 149 Sm isotope ratios were found to be within 20% of predicted values without any chemical separations and without mass bias corrections. In addition, the 240 Pu/ 239 Pu isotope ratio was determined, free from the 238 UH + interferences common to the ICP-MS platforms, while at the same time allowing for the determination of U isotopic signatures. While these demonstrative results are from a single sample, the advantages of the microplasma/ultrahigh mass resolution approach to intra-element isotope ratio determinations are clear.

Fuel burnup↗