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At least 559 records · Page 31

Submicron particle mass concentrations and sources in the Amazonian wet season (AMAZE-08)

Real-time mass spectra of non-refractory component of submicron aerosol particles were recorded in a tropical rainforest in the central Amazon basin during the wet season of 2008, as a part of the Amazonian Aerosol Characterization Experiment (AMAZE-08). Organic components accounted on average for more than 80% of the non-refractory submicron particle mass concentrations during the period of measurements. Ammonium was present in sufficient quantities to halfway neutralize sulfate. In this acidic, isoprene-dominated, low-NOx environment the high-resolution mass spectra as well as mass closures with ion chromatography measurements did not provide evidence for significant contributions of organosulfate species, at least at concentrations above uncertainty levels. Positive-matrix factorization of the time series of particle mass spectra identified four statistical factors to account for the variance of the signal intensities of the organic constituents: a factor HOA having a hydrocarbon-like signature and identified as regional emissions of primary organic material, a factor OOA-1 associated with fresh production of secondary organic material by a mechanism of BVOC oxidation followed by gas-to-particle conversion, a factor OOA-2 consistent with reactive uptake of isoprene oxidation products, especially epoxydiols by acidic particles, and a factor OOA-3 associated with long range transport and atmospheric aging. The OOA-1, -2, and -3 factors had progressively more oxidized signatures. Diameter-resolved mass spectral markers also suggested enhanced reactive uptake of isoprene oxidation products to the accumulation mode for the OOA-2 factor, and such size partitioning can be indicative of in-cloud process. The campaign-average factor loadings were in a ratio of 1.1:1.0 for the OOA-1 compared to the OOA-2 pathway, suggesting the comparable importance of gas-phase compared to particle-phase (including cloud waters) production pathways of secondary organic material during the study period.

Chen, Q.↗

Determining Best Estimates and Uncertainties in Cloud Microphysical Parameters from ARM Field Data: Implications for Models, Retrieval Schemes and Aerosol-Cloud-Radiation Interactions

We proposed to analyze in-situ cloud data collected during ARM/ASR field campaigns to create databases of cloud microphysical properties and their uncertainties as needed for the development of improved cloud parameterizations for models and remote sensing retrievals, and for evaluation of model simulations and retrievals. In particular, we proposed to analyze data collected over the Southern Great Plains (SGP) during the Mid-latitude Continental Convective Clouds Experiment (MC3E), the Storm Peak Laboratory Cloud Property Validation Experiment (STORMVEX), the Small Particles in Cirrus (SPARTICUS) Experiment and the Routine AAF Clouds with Low Optical Water Depths (CLOWD) Optical Radiative Observations (RACORO) field campaign, over the North Slope of Alaska during the Indirect and Semi-Direct Aerosol Campaign (ISDAC) and the Mixed-Phase Arctic Cloud Experiment (M-PACE), and over the Tropical Western Pacific (TWP) during The Tropical Warm Pool International Cloud Experiment (TWP-ICE), to meet the following 3 objectives; derive statistical databases of single ice particle properties (aspect ratio AR, dominant habit, mass, projected area) and distributions of ice crystals (size distributions SDs, mass-dimension m-D, area-dimension A-D relations, mass-weighted fall speeds, single-scattering properties, total concentrations N, ice mass contents IWC), complete with uncertainty estimates; assess processes by which aerosols modulate cloud properties in arctic stratus and mid-latitude cumuli, and quantify aerosol’s influence in context of varying meteorological and surface conditions; and determine how ice cloud microphysical, single-scattering and fall-out properties and contributions of small ice crystals to such properties vary according to location, environment, surface, meteorological and aerosol conditions, and develop parameterizations of such effects.In this report we describe the accomplishments that we made on all 3 research objectives.

54 ENVIRONMENTAL SCIENCES↗

Diurnal, Seasonal, and Interannual Variations of Cloud Properties Derived for CERES From Imager Data

Simultaneous measurement of the radiation and cloud fields on a global basis is a key component in the effort to understand and model the interaction between clouds and radiation at the top of the atmosphere, at the surface, and within the atmosphere. The NASA Clouds and Earth s Radiant Energy System (CERES) Project, begun in 1998, is meeting this need. Broadband shortwave (SW) and longwave radiance measurements taken by the CERES scanners at resolutions between 10 and 20 km on the Tropical Rainfall Measuring Mission (TRMM), Terra, and Aqua satellites are matched to simultaneous retrievals of cloud height, phase, particle size, water path, and optical depth OD from the TRMM Visible Infrared Scanner (VIRS) and the Moderate Resolution Imaging Spectroradiometer (MODIS) on Terra and Aqua. Besides aiding the interpretation of the broadband radiances, the CERES cloud properties are valuable for understanding cloud variations at a variety of scales. In this paper, the resulting CERES cloud data taken to date are averaged at several temporal scales to examine the temporal and spatial variability of the cloud properties on a global scale at a 1 resolution.

Minnis, Patrick↗

Non-conservation and conservation for different formulations of moist potential vorticity

Potential vorticity (PV) is one of the most important quantities in atmospheric science. In the absence of dissipative processes, the PV of each fluid parcel is known to be conserved, for a dry atmosphere. However, a parcel's PV is not conserved if clouds or phase changes of water occur. Recently, PV conservation laws were derived for a cloudy atmosphere, where each parcel's PV is not conserved but parcel-integrated PV is conserved, for integrals over certain volumes that move with the flow. Hence a variety of different statements are now possible for moist PV conservation and non-conservation, and in comparison to the case of a dry atmosphere, the situation for moist PV is more complex. Here, in light of this complexity, several different definitions of moist PV are compared for a cloudy atmosphere. Numerical simulations are shown for a rising thermal, both before and after the formation of a cloud. These simulations include the first computational illustration of the parcel-integrated, moist PV conservation laws. The comparisons, both theoretical and numerical, serve to clarify and highlight the different statements of conservation and non-conservation that arise for different definitions of moist PV.

54 ENVIRONMENTAL SCIENCES↗

A Fourier approach to cloud motion estimation

A Fourier phase-difference technique for cloud motion estimation from pairs of pictures is described, and results obtained using this technique are compared with the results of a Fourier-domain cross-correlation scheme. The phase-difference technique makes use of the phase of the cross-spectral density and allows motion estimates to be made for individual spatial frequencies, which are related to cloud pattern dimensions. When objects being tracked do not change their shape, size, and orientation to more than a limited degree, both techniques are effective. The phase difference technique is relatively sensitive to the presence of mixtures of motions, changes in cloud shape, and edge effects; in these circumstances, the cross-correlation scheme is preferable. It is suggested that the Fourier transform phase difference estimation methods can be applied in problems such as landmark matching.

Arking, A.↗

ShupeTurner cloud microphysics

This product is the ShupeTurner cloud microphysics product derived for the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition in the central Arctic. The product includes time-height derivations of the cloud type (phase type) and the condensed water content and characteristic effective particle size for liquid and ice hydrometeor populations. Additionally, it includes the vertical integral of the condensed water content for liquid and ice, i.e., the liquid water path and ice water path. These are derived using a combination of sensors, including: cloud radar, depolarization lidar, microwave radiometer, ceilometer, and radiosondes. During MOSAiC, these sensors were installed and operated onboard the Polarstern icebreaker while within the Arctic sea ice. Most data were obtained while Polarstern was moored to the MOSAiC sea ice floe, passively drifting through the Arctic. However, the data from 16 May 2020 - 17 June 2020 and 31 July 2020 - 21 August 2020 were obtained while Polarstern was underway transiting through the sea ice during relocations of the expedition. General details of the retrieval algorithm, its application, and uncertainties are provided in Shupe et al. (2015), with the cloud classification being described in more detail in Shupe (2007). General details about the MOSAiC expedition including instruments, locations, and meteorological context is provided in Shupe et al. (2022).

54 ENVIRONMENTAL SCIENCES↗

Optimizing cloud motion estimation on the edge with phase correlation and optical flow

Abstract. Phase correlation (PC) is a well-known method for estimating cloud motion vectors (CMVs) from infrared and visible spectrum images. Commonly, phase shift is computed in the small blocks of the images using the fast Fourier transform. In this study, we investigate the performance and the stability of the blockwise PC method by changing the block size, the frame interval, and combinations of red, green, and blue (RGB) channels from the total sky imager (TSI) at the United States Atmospheric Radiation Measurement user facility's Southern Great Plains site. We find that shorter frame intervals, followed by larger block sizes, are responsible for stable estimates of the CMV, as suggested by the higher autocorrelations. The choice of RGB channels has a limited effect on the quality of CMVs, and the red and the grayscale images are marginally more reliable than the other combinations during rapidly evolving low-level clouds. The stability of CMVs was tested at different image resolutions with an implementation of the optimized algorithm on the Sage cyberinfrastructure test bed. We find that doubling the frame rate outperforms quadrupling the image resolution in achieving CMV stability. The correlations of CMVs with the wind data are significant in the range of 0.38–0.59 with a 95 % confidence interval, despite the uncertainties and limitations of both datasets. A comparison of the PC method with constructed data and the optical flow method suggests that the post-processing of the vector field has a significant effect on the quality of the CMV. The raindrop-contaminated images can be identified by the rotation of the TSI mirror in the motion field. The results of this study are critical to optimizing algorithms for edge-computing sensor systems.

54 ENVIRONMENTAL SCIENCES↗

Phase Doppler Interferometry for Efficient Cloud Drop Size Distribution, Number Density, and LWC Measurements

Threats to aviation safety as a result of super-cooled large drops (SLD) has been addressed by the FAA rules change (14 CFR Part 25) with the additional icing certification requirement. SLD clouds often consist of bi-modal drop size spectra leading to significant problems in simulating and characterizing these conditions in situ and in icing wind tunnels. Legacy instrumentation for measuring drop size distributions and liquid water content are challenged under these conditions. The large size range measurement problem is addressed with the development of the Phase Doppler Interferometer, Flight Probe Dual-Range (PDI FPDR). The method is described in this report along with the measurement capabilities including the dynamic measurement range and overall working size range. The PDI instrument bases drop size measurements on the light wavelength as the measurement length scale. The light wavelength is a much more robust scale, especially as compared to the light scattering intensity. Additionally, methods for accurately characterizing the sample volume in situ based on measured drop velocity and transit time are reviewed, given the importance of this parameter for merging results and measuring LWC. Droplet coincidence in the sample volume can be problematic so this condition is treated with an innovative signal parsing approach. Measurement examples acquired in the NASA IRT are provided. Measurements of LWC showed good agreement with the Artium Particle Imaging (PI) instrument but diverged from the tunnel calibration results for larger MVD values.

42 ENGINEERING↗

The application of satellite data in the determination of ocean temperatures and cloud characteristics and statistics

The author has identified the following significant results. The major shortcoming of the data was the loss of the infrared radiances from the S191 spectrometer. The cloud thermodynamic phase determination procedure was derived and tested with the data collected by the S192 multispectral scanner. Results of the test indicate a large fraction of the data could be classified thermodynamically. An added bonus was the inclusion of snow in the classification approach. The conclusion to be drawn from this portion of the effort is that in most cases considered ice clouds, liquid water droplet clouds, and snow fields can be spectroscopically separated to a high degree of accuracy.

Curran, R. J.↗

Overview of the Field Phase of the NASA Tropical Cloud Systems and Processes (TCSP)Experiment

The Tropical Cloud Systems and Processes experiment is sponsored by the National Aeronautics and Space Administration (NASA) to investigate characteristics of tropical cyclone genesis, rapid intensification and rainfall using a three-pronged approach that emphasizes satellite information, suborbital observations and numerical model simulations. Research goals include demonstration and assessment of new technology, improvements to numerical model parameterizations, and advancements in data assimilation techniques. The field phase of the experiment was based in Costa Rica during July 2005. A fully instrumented NASA ER-2 high altitude airplane was deployed with Doppler radar, passive microwave instrumentation, lightning and electric field sensors and an airborne simulator of visible and infrared satellite sensors. Other assets brought to TCSP were a low flying uninhabited aerial vehicle, and a surface-based radiosonde network. In partnership with the Intensity Forecasting Experiment of the National Oceanic and Atmospheric Administration (NOAA) Hurricane Research Division, two NOAA P-3 aircraft instrumented with radar, passive microwave, microphysical, and dropsonde instrumentation were also deployed to Costa Rica. The field phase of TCSP was conducted in Costa Rica to take advantage of the geographically compact tropical cyclone genesis region of the Eastern Pacific Ocean near Central America. However, the unusual 2005 hurricane season provided numerous opportunities to sample tropical cyclone development and intensification in the Caribbean Sea and Gulf of Mexico as well. Development of Hurricane Dennis and Tropical Storm Gert were each investigated over several days in addition to Hurricane Emily as it was close to Saffir-Simpson Category 5 intensity. An overview of the characteristics of these storms along with the pregenesis environment of Tropical Storm Eugene in the Eastern Pacific will be presented.

Hood, Robbie E.↗

An underestimated negative cloud feedback from cloud lifetime changes

As the atmosphere warms, part of the cloud population shifts from ice and mixed phase (“cold”) to liquid (“warm”) clouds. Because warm clouds are more reflective and longerlived, this phase change reduces the solar flux absorbed by Earth and constitutes a negative radiative feedback. This cooling feedback is weaker in CMIP6 than in CMIP5, contributing to greater greenhouse warming. While this change is often attributed to improvements in simulated cloud phase, another model bias persists: warm clouds precipitate too readily, potentially leading to underestimated negative lifetime feedbacks. In this work, we modify a climate model to better simulate warm rain probability and find it exhibits a cloud lifetime feedback nearly three times larger than the default model. This suggests model errors in cloud-precipitation processes may bias cloud feedbacks as much as CMIP5–CMIP6 climate sensitivity differences. Reliable climate model projections therefore require improved cloud process realism guided by process-oriented observations and observational constraints.

54 ENVIRONMENTAL SCIENCES↗

Ground-based remote sensing of ice clouds

A ground-based cloud water phased discriminating spectroradiometer was designed, built, and employed to obtain reflectance from the sides and tops of cumuliform towers during the Arizona summer monsoons from 1984 through 1987 (Pileaskie and Twomey, 1987 and 1988). The experimental procedure was designed to observe the upper regions of rapidly ascending turrets as they matured, obtaining spectra every two minutes to determine the onset of glaciation. Occasionally, conditions permitted continuous observations from time of cloud conception to full maturation, i.e., an advanced cumulonimbus marked by anvil growth, lightning, and precipitation.

Pilewskie, Peter↗

Continuous Lidar Monitoring of Polar Stratospheric Clouds at the South Pole

Polar stratospheric clouds (PSC) play a primary role in the formation of annual ozone holes over Antarctica during the austral sunrise. Meridional temperature gradients in the lower stratosphere and upper troposphere, caused by strong radiative cooling, induce a broad dynamic vortex centered near the South Pole that decouples and insulates the winter polar airmass. PSC nucleate and grow as vortex temperatures gradually fall below equilibrium saturation and frost points for ambient sulfate, nitrate, and water vapor concentrations (generally below 197 K). Cloud surfaces promote heterogeneous reactions that convert stable chlorine and bromine-based molecules into photochemically active ones. As spring nears, and the sun reappears and rises, photolysis decomposes these partitioned compounds into individual halogen atoms that react with and catalytically destroy thousands of ozone molecules before they are stochastically neutralized. Despite a generic understanding of the ozone hole paradigm, many key components of the system, such as cloud occurrence, phase, and composition; particle growth mechanisms; and denitrification of the lower stratosphere have yet to be fully resolved. Satellite-based observations have dramatically improved the ability to detect PSC and quantify seasonal polar chemical partitioning. However, coverage directly over the Antarctic plateau is limited by polar-orbiting tracks that rarely exceed 80 degrees S. In December 1999, a NASA Micropulse Lidar Network instrument (MPLNET) was first deployed to the NOAA Earth Systems Research Laboratory (ESRL) Atmospheric Research Observatory at the Amundsen-Scott South Pole Station for continuous cloud and aerosol profiling. MPLNET instruments are eye-safe, capable of full-time autonomous operation, and suitably rugged and compact to withstand long-term remote deployment. With only brief interruptions during the winters of 2001 and 2002, a nearly continuous data archive exists to the present.

OZONE DESTRUCTION↗

Persistent Supercooled Drizzle at Temperatures Below -25 °C Observed at McMurdo Station, Antarctica

The rarity of reports in the literature of brief and spatially limited observations of drizzle at temperatures below -20 degrees C suggest that riming and other temperature-dependent cloud microphysical processes such as heterogeneous ice nucleation and ice crystal depositional growth prevent drizzle persistence in cold environments. In this study, we report on a persistent drizzle event observed by ground-based remote sensing measurements at McMurdo Station, Antarctica. The temperatures in the drizzle-producing cloud were below -25 degrees C and the drizzle persisted for a period exceeding 7.5 hr. Using ground-based, satellite, and reanalysis data, we conclude that drizzle was likely present in parts of a widespread cloud field, which stretched more than similar to 1,000 km along the Ross Ice Shelf coast. Parameter space sensitivity tests using two-moment bulk microphysics in large eddy simulations constrained by the observations suggest that activated ice freezing nuclei and accumulation-mode aerosol number concentrations aloft during this persistent drizzle period were likely on the order of 0.2 L-1 and 20 cm -3 , respectively. In such constrained simulations, the drizzle moisture flux through cloud base exceeds that of ice. The simulations also indicate that drizzle can lead to the formation of multiple peaks in cloud water content profiles. This study suggests that persistent drizzle at these low temperatures may be common at the low aerosol concentrations typical of the Antarctic and Southern Ocean atmospheres.

54 ENVIRONMENTAL SCIENCES↗

The NASA ACTIVATE Mission

The NASA Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE) conducted 162 joint flights with two aircraft over the northwest Atlantic to study aerosol–cloud interactions (ACIs), which represent the largest uncertainty in estimating total anthropogenic radiative forcing. The combination of a high-flying King Air and low-flying HU-25 Falcon, equipped with remote sensing and in situ instruments, characterized trace gases, aerosol particles, clouds, and meteorological variables with data collected nearly simultaneously below, within, and above marine boundary layer (MBL) clouds. Flights spanning warm and cold seasons across 3 years (2020–22) provided a broad range of conditions associated with aerosol particles, cloud properties (including particle size and phase), and meteorology, ideally suited for robust ACI calculations and assessing how well models simulate a wide range of MBL clouds from stratiform to cumulus. ACTIVATE data suggest that drivers of cloud droplet number concentration N d , including aerosol particles and MBL dynamics, vary between winter and summer months with a stronger potential to convert aerosol particles into cloud droplets in winter. Models of varying complexity not only highlight some skills in simulating winter and summer cloud types but also identify challenges that still need to be addressed such as treatment of turbulence, wet scavenging, and mesoscale organization. Remote sensing advances range from new retrieval methods for N d , cloud phase classification, vertically resolved aerosol and cloud condensation nuclei number concentration, and ocean surface wind speed. This work describes these scientific and technological advances along with efforts in outreach and open data science.

aerosol indirect effect↗

Habit–Dependent Vapor Growth Modulates Arctic Supercooled Water Occurrence

We present an analysis of long-term data collected at Utqiagvik, Alaska, to explore the impacts of cloud processes on the probability of finding supercooled water given cloud temperature, P(L|T), in the topmost unseeded liquid-bearing layers. P(L|T) has local minima at temperatures around –6°C and –15°C. Simulations using habit-evolving ice microphysics models suggest that these minima are the result of efficient vapor growth by non-isometric habits found at these temperatures. Here, we conclude that habit-dependent vapor growth of ice crystals modulates the macrophysical occurrence of supercooled water in polar clouds, the effect of which should be included in model parametrizations to avoid biases and/or error compensation. Our methodology is adaptable for spherical ice treatments implemented in models (example parametrizations provided), amenable for use with satellite measurements to give global impartial observational targets for model evaluations, and may allow empirical characterization of bulk responses to seeding and possibly secondary ice effects.

54 ENVIRONMENTAL SCIENCES↗

Development of a phase Doppler based probe for icing cloud droplet characterization

The development and evaluation of a compact optical fiber probe (OFP) for airborne and wind tunnel icing cloud characterizations is described. This probe was based upon the proven phase Doppler technique for measuring the size and velocity of spherical drops. Direct comparisons of the size distributions from the standard PDPA with the OFP were used to confirm the reliability of the probe. After some improvements in the fiber coupling efficiency, the number density and liquid water content data agreed to within 15 percent.

Rudoff, R. C.↗