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At least 559 records · Page 31

Quantification of LEU Holdup using gamma ray imaging and inverse transport solver

Holdup is the residual amount of special nuclear material (SNM) remaining in a processing facility after the bulk materials have been cleaned out. In commercial uranium processing facilities, quantification of holdup is a major challenge because of the highly variable shapes and sizes of the deposits. Any method that attempts to generalize and calibrate deposit shapes in order to quantify holdup will be prone to high uncertainties. Uncertainties on the order of ±50% are typical in holdup results. In international safeguards applications, a ±50% uncertainty can result in a large amount of material unaccounted for (MUF) thereby increasing the difficulty of detecting material diversion and facility misuse. An imaging-based methodology has been developed with the objective of significantly reducing this uncertainty by using the true deposit shape, instead of relying on oversimplified geometric assumptions. The project is a collaboration between ORNL, Y-12, and the University of Tennessee, Knoxville, TN. Uranium sources of known masses were measured using the Germanium Gamma-ray Imager (GeGI), a high-resolution imaging spectrometer, creating a pixelated map for each spectral bin. Two different gamma imaging methods are employed in this work: coded aperture imaging and Compton imaging. A validated MonteCarlo model of the detector has been developed using the GEANT4 code for determining the intrinsic response of the detector, its enclosure, and the coded aperture mask. An inverse transport solver based on the Markov Chain Monte-Carlo approach known as Differential Evolution Adaptive Metropolis (DREAM) is employed to use the measurement data from the image pixels (coded aperture or Compton) to solve for the mass of 235 U in the deposit. A reliable method based on the DREAM solver has been developed to flag the infinite thickness condition of a uranium deposit. The project team is working towards improving the image reconstruction for Compton imaging so that a better localization of the source can be achieved. Besides treating the coded aperture and Compton imaging methods independently, the project is also evaluating a combined method that uses the Compton scatter data from a coded aperture measurement. GEANT4 simulations are being performed to evaluate the combined approach. The impact on the DREAM optimization as the source thickness progressively approaches infinite thickness is being evaluated. A number of uranium sources available at ORNL have been measured, and the DREAM results have been tested and validated for the coded aperture imaging. A similar effort will be carried out to validate the Compton based method once the development of algorithms for better localization are complete. The imaging based quantification is very amenable to unattended monitoring of holdup accumulation at key measurement points. A proof of concept measurement has been completed to demonstrate this capability The current work used the high energy resolution imager GeGI. However, the approach and methodologies are applicable to other imagers such as the cadmium zin telluride (CZT) based imager manufactured by H3D, Inc.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

CRADA Number NFE-24-10110 with Qubit Engineering Inc. (CRADA Final Report)

Over the past year, the Qubit Engineering team has pushed the frontiers of power‑grid optimization, working in close collaboration with Oak Ridge National Laboratory (ORNL) and the Tennessee Valley Authority (TVA). Their progress is reflected in three newly submitted conference papers, “Unified Relational GNN Architecture for AC Optimal Power Flow Calculations in Electric Grids,” “Graph‑Based Attention Mechanisms for Solving the AC Optimal Power Flow Problem in Electrical‑Power Networks,” and “Enhanced Power‑Grid Maintenance Planning and Quantum‑Inspired Combinatorial Prospects.” These publications showcase state‑of‑the‑art graph‑neural‑network methods for AC‑OPF and novel quantum‑inspired heuristics for maintenance scheduling. Beyond the academic results, the Qubit team has converted the research into two production‑grade tools built on TVA data: Neuro‑Grid, an AI‑driven power‑flow simulator that provides instant, interactive full‑grid load‑flow visualizations, and Quanta‑Grid, a quantum‑inspired maintenance‑scheduling engine to support logistics optimization for power utilities. Together, these advances demonstrate how Qubit’s partnership with ORNL and TVA is delivering practical, physics‑grounded analytics for next‑generation grid management.

24 POWER TRANSMISSION AND DISTRIBUTION↗

Environmental Flow Requirements from FERC Licenses Across the US

Environmental flow requirements included in Federal Energy Regulatory Commission (FERC) hydropower licenses are important for balancing natural properties and benefits of river ecosystems (e.g., healthy species, recreation, water supply, flood control) supporting hydropower production. In some cases, environmental flow requirements may limit operational flexibility given current operational schemes and make a hydropower plant less able to provide power to the electric grid on demand. Hydropower plants may gain some flexibility as hydropower scheduling time periods are made to be more responsive to the short-term needs of an energy grid increasingly reliant on intermittent renewables. However, many flow requirements focus on the daily, monthly, or seasonal flow fluctuations which matches the time scale of most paradigms linking flow alterations to the health of river ecosystems. This dataset seeks to provide a greater understanding of how flexibility in environmental requirements can be leveraged to create positive outcomes for both the power system and the environment. It contains information on environmental flow requirements from the Protection, Mitigation, and Enhancement section of 50 randomly selected FERC licenses: 25 issued from 1998-2013 that were also included in the ORNL Mitigation Database (Schramm et al. 2015) and 25 issued from 2014-present. The information on environmental flow requirements was extracted from the PM&E section of 50 randomly selected FERC licenses: 25 issued from 1998-2013 that were also included in the ORNL Mitigation Database (Schramm et al. 2015) and 25 issued from 2014-present. The flow requirements were then categorized into flow augmentation categories based on whether the license stated a specific water management purpose for the given requirement called augmentation categories (i.e., fisheries or habitat, recreation or boating, industry, and general or unspecified; Table B). Requirements were also grouped into flow type categories (e.g., minimum flow rate, maximum flow rate, ramping rate). Additional information related to flow requirements such as the augmentation time-period and whether the flow rate was continuous (i.e., condition must be present at all-times) or instantaneous (i.e., condition present at a point in time) was also extracted from the licenses. Some licenses had specific flow requirements based on whether the project was in a wet, dry, or normal water year. If that information was presented in the license, it was also included in the data set. The location within the project was noted, hereafter, zone, in the dataset for flow requirements relating to specific areas of hydropower projects (Dam, Powerhouse, Bypass Reach). Maximum discharge capacities of hydropower facilities were also extracted from both the Existing Hydropower Assets (EHA) data set and the National Inventory of Dams (NID) databases. Each facility was coded with project identification codes from the EHA dataset to facilitate cross-referencing between datasets.

13 HYDRO ENERGY↗

Thermochemical Nonequilibrium Modeling in a Continuous-Galerkin, Finite-Element Framework

The presented work discusses the implementation, verification, and validation of Park's two-temperature model in a scalable, computational fluid dynamics (CFD) code developed at the US Department of Energy's Oak Ridge National Laboratory (ORNL). The implementation of Park's two-temperature model was verified through 0D test cases involving an adiabatic reactor and a nitrogen thermal bath. The implementation was then validated through comparisons with other validated CFD codes and experimental data on a hypersonic cylinder and double cones. These are standard benchmark test cases for thermochemical non-equilibrium (TCNE) modeling, and all data are shared publicly. The verification and validation results showed that ORNL's in-house CFD code could model complex, high-speed flow problems with and without TCNE modeling. This work is essential for future research involving 3D shock wave/boundary layer interactions (SBLIs).

Nutter, Nicole↗

A galactic approach to neutron scattering science

Neutron scattering science is leading to significant advances in our understanding of materials and will be key to solving many of the challenges that society is facing today. Improvements in scientific instruments are actually making it more difficult to analyze and interpret the results of experiments due to the vast increases in the volume and complexity of data being produced and the associated computational requirements for processing that data. New approaches to enable scientists to leverage computational resources are required, and Oak Ridge National Laboratory (ORNL) has been at the forefront of developing these technologies. We recently completed the design and initial implementation of a neutrons data interpretation platform that allows seamless access to the computational resources provided by ORNL. For the first time, we have demonstrated that this platform can be used for advanced data analysis of correlated quantum materials by utilizing the world's most powerful computer system, Frontier. In particular, we have shown the end-to-end execution of the DCA++ code to determine the dynamic magnetic spin susceptibility χ(q, ω) for a single-band Hubbard model with Coulomb repulsion U/t = 8 in units of the nearest-neighbor hopping amplitude t and an electron density of n = 0.65. The following work describes the architecture, design, and implementation of the platform and how we constructed a correlated quantum materials analysis workflow to demonstrate the viability of this system to produce scientific results.

97 MATHEMATICS AND COMPUTING↗

AGR-3/4 Compact 1-4 Examination Plan

This plan describes the post irradiation examination (PIE) activities to be performed by Oak Ridge National Laboratory (ORNL) on irradiated Compact 1-4 taken from the Advanced Gas Reactor (AGR) experiment, AGR-3/4. This work will be performed in accordance with the general objectives outlined in the AGR 3/4 PIE Plan and guidance in the ORNL PIE Statement of Work.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Single-Bar SMT Testing on Alloy 617 using Software Controls

INL has performed simplified model testing using a variable in the software control program to compare with the testing performed at ORNL, which uses hardware to modify the control signal. The INL tests compared well with the ORNL tests, showing similar stress and strain values, as well as similarly shaped hysteresis loops. This demonstrates that possibility of performing simplified model testing without any hardware modifications.

36 MATERIALS SCIENCE↗

AGR 3/4 Compact 7 4 Examination Plan

This plan describes the post irradiation examination (PIE) activities to be performed by Oak Ridge National Laboratory (ORNL) on irradiated Compact 7 4 taken from the Advanced Gas Reactor (AGR) experiment, AGR 3/4. This work will be performed in accordance with the general objectives outlined in the AGR 3/4 PIE Plan and guidance in the ORNL PIE Statement of Work.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR 3/4 Compact 8 4 Examination Plan

This plan describes the post irradiation examination (PIE) activities to be performed by Oak Ridge National Laboratory (ORNL) on irradiated Compact 8 4 taken from the Advanced Gas Reactor (AGR) experiment, AGR 3/4. This work will be performed in accordance with the general objectives outlined in the AGR 3/4 PIE Plan and guidance in the ORNL PIE Statement of Work.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

FITT OXIDATION TEST PLAN

This plan describes the post irradiation examination (PIE) oxidation testing activities to be performed by Oak Ridge National Laboratory (ORNL) on individual particles from Compact 5 4 2 taken from the Advanced Gas Reactor (AGR) experiment, AGR 2. This work will be performed in accordance with the general objectives outlined in the AGR 2 PIE Plan1 and guidance in the ORNL PIE Statement of Work.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Feasibility Study for a Proposed Subcritical Assembly at Oak Ridge National Laboratory

Nuclear Criticality Safety (NCS) staff use the guidelines in the ANSI/ANS-8.26 standard to establish and maintain their training and qualifications. Section 7.4 of the standard requires NCS staff to participate in hands-on experiments meant to “…demonstrate how varying the properties of a fissionable material system can affect neutron multiplication.” This training is performed to ensure NCS and operations staff are aware of the risks involved with conducting operations with fissionable materials outside reactors. A new, inherently safe, subcritical assembly, to be housed at Oak Ridge National Laboratory (ORNL) is being considered to augment the current training capabilities of the US Department of Energy/National Nuclear Security Administration (DOE/NNSA) Nuclear Criticality Safety Program (NCSP), which conducts hands-on subcritical and critical experiments to support the training and qualifications of NCS staff. This paper reports the results of a feasibility study performed by ORNL.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Effects of Lithium-ion Battery Recycling Wastes on Ammonia-Oxidizing Bacteria

Increased demand for lithium-ion batteries (LIB) necessitates development of effective recycling methods for critical battery materials. Oak Ridge National Laboratory (ORNL) is exploring membrane solvent extraction (MSX) for the hydrometallurgical recycling of LIB materials. In this study, waste from MSX was investigated for its impact on the ammonia-oxidizing organism, Nitrosomonas europaea—a model organism for nitrogen removal during wastewater treatment. It was found that Raffinate 4 from ORNL was inhibitory to the growth and nitrite production of N. europaea, likely due to its nickel content. Further investigation is currently underway.

99 GENERAL AND MISCELLANEOUS↗

AGR-3/4 Compact 10-4 Examination Plan

This plan describes the post irradiation examination (PIE) activities to be performed by Oak Ridge National Laboratory (ORNL) on irradiated Compact 10 4 taken from the Advanced Gas Reactor (AGR) experiment, AGR 3/4. This work will be performed in accordance with the general objectives outlined in the AGR 3/4 PIE Plan and guidance in the ORNL PIE Statement of Work.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

FITT OXIDATION TEST PLAN

This plan describes the post irradiation examination (PIE) oxidation testing activities to be performed by Oak Ridge National Laboratory (ORNL) on individual particles from Compact 5 4 2 taken from the Advanced Gas Reactor (AGR) experiment, AGR 2. This work will be performed in accordance with the general objectives outlined in the AGR 2 PIE Plan1 and guidance in the ORNL PIE Statement of Work.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Pu-238 Production Calculator and Estimation Tool

A MS Excel tool was created to help track Pu-238 production, Np-237 feedstock use, estimate production scenarios, and coordinate planning for shipments. As-run estimates were used as a basis for beginning and end of life isotopic concentrations. Multiple target types were created to demonstrate a proof of concept while actual results were not yet available The initial goals of this production tool were: • Track unirradiated, currently irradiated, and irradiated targets at the Advanced Test Reactor (ATR) • Estimate production yields from irradiated targets in various positions for each cycle • Provide past, current, and future year quantities of Np-237 and Pu-238 at ATR, amounts shipped to ATR and amounts shipped from ATR • Estimate production from current and future target designs based on data from numerical modeling (values will be provided by Idaho National Laboratory (INL)) • After proof of principle, additional work is planned that will further enhance the tool with: o Incorporate the High Flux Isotope Reactor (HFIR) reactor at Oak Ridge National Laboratory (ORNL) for irradiation o Incorporate irradiations and target shipments from ORNL to INL and back to track Np-237 transfers across the Department of Energy (DOE) Complex

07 ISOTOPE AND RADIATION SOURCES↗

A Subcritical Assembly for Training and Education Use at the Oak Ridge National Laboratory

A near-final design has been completed for a new subcritical assembly at Oak Ridge National Laboratory (ORNL). This subcritical assembly will support the Nuclear Criticality Safety Program (NCSP) training and education program to augment current subcritical assembly capabilities at Sandia National Laboratories (SNL) and at the National Criticality Experiments Research Center (NCERC). Other collaborations have been proposed with the Sunrise Consortium and others. This proposed subcritical assembly uses legacy AGN-201M research reactor fuel plates that are available from the Y-12 National Security Complex. This subcritical assembly contains approximately 620 grams of 235 U as UO 2 particulates distributed homogeneously in radiation-stabilized polyethylene. The fuel plates will have a graphite neutron reflector to obtain a core multiplication, M, from 10 to 50, corresponding to a k eff of 0.9 to 0.95, respectively. The subcritical assembly will be able to support at least four experiments for the training courses: (1) the addition of fissile material to increase neutron multiplication (mass), (2) a core separation experiment (interaction), (3) the effect of adding moderators to the core (moderation), and (4) the effect of adding neutron absorbers to the core (poison/absorption). The proposed ORNL subcritical assembly will provide additional student bandwidth to support NCSP training courses and to provide for some backup capacity if nuclear facility operations are disrupted at SNL or NCERC due to some unforeseen issue. The subcritical assembly will be designed to be an inherently safe subcritical assembly—subcritical under all normal and abnormal conditions—and it will provide the capability to conduct hands-on training to support NCSP and general nuclear criticality safety (NCS) staff training and qualification goals.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Evaluation of Oak Ridge National Laboratory Health Physics Research Reactor Operation Data for Critical Benchmark Creation [Abstract]

The Oak Ridge National Laboratory (ORNL) Health Physics Research Reactor (HPRR) was a research reactor designed and built at ORNL in 1961. The critical assembly was using a highly enriched uranium and molybdenum alloy as the fuel, and it could be operated in steady-state or burst modes. The reactor was used for about 25 years to produce a lot of publications related to dosimetry, radiobiology and radiation detectors testing before its decommissioning in 1987. In recent years, the idea of using legacy operation data from the to create a valuable critical accident alarm system shielding benchmark arose. Such a benchmark has been submitted to the International Criticality Safety Benchmark Experiment Project (ICSBEP) Technical Review Group for a potential inclusion in the 2022 version of the handbook. Another way to use the valuable data from the operation of the HPRR is to evaluate the feasibility of the creation of a subcritical or prompt supercritical benchmark for inclusion in the ICSBEP or the International Reactor Physics Experiments Evaluation Project (IRPhEP) handbooks. To initiate a burst, the HPRR had to be operated in a slightly subcritical state for a few minutes. Then, the insertion of the burst control rod would greatly increase the reactivity of the system and start the burst. No critical configuration of the HPRR critical assembly could be located. The only information available concerns stable subcritical and prompt supercritical states, found in a burst experiments’ logbook. In the recovered logbook pages, information about 8 different bursts is available. The information includes the rods positions before and during a burst, the recorded subcritical reactor period and reactivity, and the burst fission yield derived from the temperature elevation sulfur pellet irradiation analysis. By using the HPRR logbook information and the as-built drawings of the critical assembly, a highly detailed model of the HPRR was created with SCALE 6.2.4/KENO-VI. Eight KENO-VI models were created to replicate the sub-critical assembly configurations described in the eight bursts from the recovered logbook pages. KENO-VI calculates k eff and it can be linked to a reactivity value in cents by using the delayed neutron fraction B eff , also calculated by KENO-VI. KENO-VI can also be used to model the prompt super-critical configurations of the HPRR and to assess the similarity with the burst measurements by comparing the calculated k eff and the measured fission yields between each burst. Unfortunately, high uncertainty exist and the obtained discrepancies between experiments and calculation results are high, compromising the creation of a valuable critical benchmark from HPRR operation data. The reasons of the discrepancies and potential ways to solve them are explored.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

A Subcritical Assembly for Training and Education Use at the Oak Ridge National Laboratory [Abstract]

A near-final design has been completed for a new subcritical assembly at Oak Ridge National Laboratory (ORNL). This subcritical assembly will support the Nuclear Criticality Safety Program (NCSP) training and education program to augment current subcritical assembly capabilities at Sandia National Laboratories (SNL) and at the National Criticality Experiments Research Center (NCERC). Other collaborations have been proposed with the Sunrise Consortium and others. This proposed subcritical assembly uses legacy AGN-201M research reactor fuel plates that are available from the Y-12 National Security Complex. This subcritical assembly contains approximately 620 grams of 235 U as UO 2 particulates distributed homogeneously in radiation-stabilized polyethylene. The fuel plates will have a graphite neutron reflector to obtain a core multiplication, M, from 10 to 50, corresponding to a k eff of 0.9 to 0.95, respectively. The subcritical assembly will be able to support at least four experiments for the training courses: (1) the addition of fissile material to increase neutron multiplication (mass), (2) a core separation experiment (interaction), (3) the effect of adding moderators to the core (moderation), and (4) the effect of adding neutron absorbers to the core (poison/absorption). The proposed ORNL subcritical assembly will provide additional student bandwidth to support NCSP training courses and to provide for some backup capacity if nuclear facility operations are disrupted at SNL or NCERC due to some unforeseen issue. The subcritical assembly will be designed to be an inherently safe subcritical assembly—subcritical under all normal and abnormal conditions—and it will provide the capability to conduct hands-on training to support NCSP and general nuclear criticality safety (NCS) staff training and qualification goals.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗