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At least 559 records · Page 31

Rossi-alpha Analysis of Thermal/Epithermal eXperiments Optimized for Polyethylene Thermal Neutron Scattering

Accurate nuclear data is the foundation for predictive simulations and design of new experimental in the nuclear community. The criticality safety community has particular interest in benchmarking assemblies with thermal neutron data. To address such needs the Nuclear Criticality Safety Program (NCSP) funded the Thermal/Epithermal eXperiments (TEX) campaigns that were to be completed between Lawrence Livermore National Laboratory (LLNL) and Los Alamos National Laboratory (LANL). Specifically, analysis of plutonium with a thermal neutron spectrum expands on previous work to help validate thermal scattering law data, which can have larger impacts in thermal applications. The first of these experiments were successfully conducted in 2018, but this paper will focus on the 2021 measurement focused on investigating the the thermal scattering law (TSL) for polyethylene. These experiments were successfully conducted at the National Criticality Experiments Research Center (NCERC) using the Planet vertical lift critical assembly machine. Polethylene plates were layered with trays of Zero Power Physics Reactor (ZPPR) 24 plates in a 12" by 12" square. The ZPPR plates were 2" by 3" by 0.125" bearing weapons grade plutonium. The polyethylene moderator was either 2" or 1.6875" thick. This work builds on the Rossi-alpha calculations done by McKenzie et al. for the same detector-assembly system and will only focus on the Rossi-alpha neutron noise method. This work will aim to further validate the results of the experiment through a novel neutron noise python package. Following similar methodology to the previous analysis, analysis of TEX evaluated the prompt neutron decay constant at delayed critical, $α_{DC}$ using Rossi-alpha for different polyethylene moderator thicknesses. These results will help improve understanding of TSL in critical experiments. Alpha (α), is the prompt neutron decay constant of the measured system and allows for the evaluation of a systems propensity to sustain fission chains via prompt neutrons. The single value description of the assemblies allow for comparison between experiments regardless of composition, geometry, and reflectors/moderators. Rossi-alpha measurements were performed on the polyethylene moderated TEX experiments to estimate $α_{DC}$.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Search for hadronic decays of feebly-interacting particles at NA62

The NA62 experiment at CERN has the capability to collect data in a beam-dump mode, where 400 GeV protons are dumped on an absorber. In this configuration, New Physics particles, including dark photons, dark scalars, and axion-like particles, may be produced in the absorber and decay in the instrumented volume beginning approximately 80 m downstream of the dump. A search for these particles decaying in flight to hadronic final states is reported, based on an analysis of a sample of 1.4 x 10 17 protons on dump collected in 2021. No evidence of a New Physics signal is observed, excluding new regions of parameter spaces of multiple models.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for Neutrino-Induced Neutral Current Delta Radiative Decay in MicroBooNE and a First Test of the MiniBooNE Low Energy Excess Under a Single Photon Hypothesis (submitted to PRL)

We report results from a search for neutrino-induced neutral current (NC) resonant Δ(1232) baryon production followed by Δ radiative decay, with a h0.8i GeV neutrino beam. Data corresponding to MicroBooNE’s first three years of operations (6.80×10 20 protons on target) are used to select single-photon events with one or zero protons and without charged leptons in the final state (1γ1p and 1γ0p, respectively). The background is constrained via an in-situ high-purity measurement of NC π 0 events, made possible via dedicated 2γ1p and 2γ0p selections. A total of 16 and 153 events are observed for the 1γ1p and 1γ0p selections, respectively, compared to a constrained background prediction of 20.5 ± 3.65(sys.) and 145.1 ± 13.8(sys.) events. The data lead to a bound on an anomalous enhancement of the normalization of NC Δ radiative decay of less than 2.3 times the predicted nominal rate for this process at the 90% confidence level (CL). The measurement disfavors a candidate photon interpretation of the MiniBooNE low-energy excess as a factor of 3.18 times the nominal NC Δ radiative decay rate at the 94.8% CL, in favor of the nominal prediction, and represents a greater than 50-fold improvement over the world’s best limit on single-photon production in NC interactions in the sub-GeV neutrino energy range.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Modeling quasielastic interactions of monoenergetic kaon decay-at-rest neutrinos

Monoenergetic muon neutrinos at 236 MeV are readily produced in intense medium-energy proton facilities (≳2–3GeV) when a positive kaon decays at rest (KDAR; K + →μ + ν μ ). These neutrinos provide a unique opportunity to both study the neutrino interaction and probe the nucleus with a monoenergetic weak-interaction-only tool. We present cross-section calculations for quasielastic scattering of these 236-MeV neutrinos off 12 C and 40 Ar, paying special attention to low-energy aspects of the scattering process. Our model takes the description of the nucleus in a mean-field approach as the starting point, where we solve Hartree-Fock equations using a Skyrme type nucleon-nucleon interaction. Thereby, we introduce long-range nuclear correlations by means of a continuum random-phase approximation (CRPA) framework where we solve the CRPA equations using a Green's function method. The model successfully describes (e,e') data on 12 C and 40 Ca in the kinematic region that overlaps with the KDAR ν μ phase space. In addition to these results, we present future prospects for precision KDAR cross-section measurements and applications of our calculations in current and future experiments that will utilize these neutrinos.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Space-based Measurements of Neutron Lifetime: A Novel Approach to a Long-standing Problem

Free neutrons decay via the weak interaction with a mean lifetime of around 15 minutes. Knowledge of this lifetime is important as it provides constraints on the unitarity of the CKM matrix and is a key parameter for studies of Big-Bang nucleosynthesis. However, current laboratory measurements differ by as much as 5σ. We are investigating a new technique to measure neutron lifetime: space-based neutron spectroscopy. We will complete a proof-of-principle demonstration using data from NASA’s MESSENGER mission to Mercury.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Use of Sensors and Machine Learning for Signal Discovery in a Solvent Extraction Process – 23280

Reprocessing is an important step in the nuclear fuel cycle where usable nuclear materials are extracted from spent fuel for recycling. The extraction of materials for reuse simultaneously reduces not only the volume of nuclear waste, but its decay time to radioactivity levels similar to that of the originating uranium ore. As part of an initiative to steward research, development, and innovation into the nuclear fuel cycle, Idaho National Laboratory is designing and constructing a solvent extraction testbed named Beartooth. Beartooth will allow researchers to refine extraction processes, test innovative extraction processes, and give early career scientists opportunities to gain skills in performing separations chemistry that uses centrifugal contactors. In addition, the Beartooth testbed is being uniquely designed to enable novel technologies including machine learning capabilities for the characterization of chemical process operations in near real-time. To aid in the design of Beartooth, a team of researchers are installing a variety of atypical sensors into a system of contactors for signal discovery. The team will implement machine learning methods on sensor data to determine signal features with the goal of providing a process operator with a deeper understanding of the chemical process and equipment usage. This work will summarize sensors utilized and preliminary results from an infrared camera.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Opportunities for detailed fission studies using light charged particle reactions

Since its discovery in 1939, the nuclear fission process has provided much insight into the behavior of nuclei under many different conditions. As part of the nuclear chain reaction, the fission process has had a profound impact on modern society and it has consequently attracted much attention to the field of nuclear physics. In this talk, I will argue that the time is ripe for a resumption of studies of the fission process induced by light charged particle reactions. Although fission can be induced in heavy nuclei by several means, in some cases these methods suffer from the complication that fission can occur at several points during the decay chain thus mixing up contributions from different excitation energies. Using instead light charged particle reactions to excite the nuclei in question, the precise excitation energy from which fission takes place, can be determined. In fact, a number of such studies were carried out previously, and a first set of results on fission barrier heights, mass, energy and angular distributions were obtained. Applying detection techniques developed over the last decades will allow researchers to obtain detailed, high-quality data from which to probe and refine our present understanding of the process. Based on these observations, I suggest that substantial advances in the study of this process can be achieved by using simple light charged particle reactions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Use of Sensors and Machine Learning for Signal Discovery in a Solvent Extraction Process

Reprocessing is an important step in the nuclear fuel cycle where usable nuclear materials are extracted from used fuel for recycling. The separation of materials for reuse simultaneously reduces not only the volume of nuclear waste, but its decay time to radioactivity levels similar to that of the originating uranium ore. As part of an initiative to steward research, development, and innovation into the nuclear fuel cycle, Idaho National Laboratory is designing and constructing a solvent extraction testbed named Beartooth. This testbed will allow researchers to refine separation processes, test innovative extraction processes, and give early career scientists opportunities to gain skills in performing separations chemistry utilizing centrifugal contactors. In addition, the Beartooth testbed is being uniquely designed to enable novel technologies including machine learning capabilities for the characterization of chemical process operations in near real-time. To aid in the design of Beartooth, a team of researchers are installing a variety of atypical sensors into a system of contactors for signal discovery. The team will implement machine learning methods on acquired sensor data to extract signal features. The goal is to provide a process operator with a deeper understanding of the chemical process and equipment usage. This work will summarize sensors utilized and preliminary results from an infrared camera.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Scalable modular dynamic molten salt reactor system model with decay heat

Nodal dynamic models allow rapid reduced-order simulations of complex systems. This paper presents a publicly available system dynamic model of a molten salt reactor system with a topology of the Molten Salt Reactor Experiment (MSRE), in MATLAB/Simulink, building upon a model previously published and validated with MSRE data. It adds scaling of nominal power, dynamic representation of decay heat generation, a generic decay heat removal system, improved documentation, modularity, and test cases. One hour of system transient runs in less than 10 min on a laptop. This model is intended for first order engineering calculations, developing insights into system transient behavior, equipment sizing, parameter sensitivity studies. The model contains an easy to use toolkit which can be customized and expanded to describe any molten salt reactor system. Finally, scenarios involving off-normal transients are presented. Relation between shutdown reactivity insertions, decay heat removal, core recriticality, and safe shutdown conditions are discussed.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Investigation of post-breakup Coulomb acceleration using a trajectory model

Intermediate mass fragments ejected during the deexcitation of excited projectilelike fragments may promptly decay following ejection; the daughter particles that are subsequently produced are subject to interactions with the residual nucleus that affect final-state observables, a process herein referred to as post-breakup Coulomb acceleration. A simple classical Coulomb interaction model was used to study modification of 8 Be (2 + ), 5 Li (3/2 – ), 7 Li (7/2 – ), 7 Be (7/2 – ), and states in 12 B emitted following heavy-ion collisions of 28 Si + 12 C at 35 MeV/nucleon. Here, in contrast to previous work studying 8 Be (2 + ), excellent agreement between simulation and experiment was obtained using only Coulomb forces when either a Lorentzian or R-matrix line shape was used to describe the initial relative energy rather than a Gaussian. In consideration of the obtained results, improvements to the model and evaluation of experimental data are discussed as future directions, but it was concluded that the effects observed in the present data can be accurately described using only elements of classical mechanics and that the process is largely understood for a wide range of state lifetimes and mass and charge (a)symmetries.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

K*(892) 0 meson production in inelastic p+p interactions at 158 GeV/ c beam momentum measured by NA61/SHINEat the CERN SPS

The measurement of Κ*(892) 0 resonance production via its Κ⁺π⁻ decay mode in inelastic p+p collisions at beam momentum 158 Ge V/c (√ S ΝΝ = 17.3 Ge V) is presented. The data were recorded by the NA61/SHINE hadron spectrometer at the CERN Super Proton Synchrotron. The template method was used to extract the K*(892) 0 signal and double-differential transverse momentum and rapidity spectra were obtained. The full phase-space mean multiplicity of K*(892) 0 mesons was found to be (78.44 ± 0.38(stat) ± 6.0(sys)) ∙ 10 -3 . The NA61/SHINE results are compared with the EPOS1.99 and Hadron Resonance Gas models as well as with world data from p+p and nucleus-nucleus collisions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Status and plans for measurements of Neutrino-Argon interactions at ICARUS

The ICARUS experiment, utilizing Liquid Argon Time Projection Chamber (LAr TPC) technology, has been installed at Fermilab (USA), following its initial operation in Italy and subsequent refurbishment at CERN. ICARUS has successfully been taking physics data at Fermilab since June 2022. While the experiment’s primary objective is to function as the far detector of the Short Baseline Neutrino program (SBN), searching for hints of physics beyond three-flavour PMNS neutrino oscillations, ICARUS also offers other diverse physics capabilities, including searches beyond the standard model and measurements of cross-sections. In addition to being exposed to the common Booster Neutrino (BNB) beamline of the SBN experiment, ICARUS receives neutrinos from the Main Injector (NuMI) beam. Due to the off-axis angle between NuMI and ICARUS, coupled with contributions from both pion and kaon decays to neutrino fluxes, interactions of NuMI neutrinos within ICARUS can be detected over a range of several GeV in energy. Measurements of these interactions present unique opportunities to infer neutrino interaction cross sections on an argon nuclear target within an energy range that overlaps both the SBN oscillation search and a significant portion of the DUNE spectrum. This presentation will summarise the current status of ICARUS’ neutrino cross-section measurements.

Roy, Promita [Fermilab] (ORCID:0000000164958937)↗

Extraction of the non-spin- and spin-transfer isovector responses via the 12 C ⁡( 10 Be, 10 B + 𝛾)⁢ 12 B reaction

The isovector response in 12 B was investigated via the 12 C ⁡( 10 Be, 10 B + 𝛾)⁢ 12 B* reaction at 100⁢𝐴MeV. By utilizing the 𝛾-decay properties of the 1.74 MeV 0 + and 0.718 MeV 1 + states in 10 B, the separate extraction of the non-spin-transfer (Δ⁢𝑆 = 0) and spin-transfer (Δ⁢𝑆 = 1) isovector responses up to an excitation energy of 50 MeV in 12 B in a single measurement is demonstrated. The experimental setup employed the S800 spectrometer to detect and analyze the 10 B ejectiles and the Gamma-Ray Energy Tracking In-beam Nuclear Array (GRETINA) for obtaining the Doppler-reconstructed spectrum for 𝛾 rays emitted in flight by 10 B. A 12 C foil was placed at the pivot point of the spectrograph. Here, the 12 B reaction product was not detected. Contributions from transitions associated with the transfer of different units of angular momentum in the non-spin- and spin-transfer responses were analyzed using a multipole decomposition analysis. The extracted non-spin-dipole (Δ⁢𝑆 = 0, Δ⁢𝐿 = 1) and spin-dipole (Δ⁢𝑆 = 1, Δ⁢𝐿 = 1) responses were found to be consistent with available data from other charge-exchange probes, validating the non-spin- and spin-transfer filters used. While statistical uncertainties and experimental resolutions were relatively large due to the modest intensity of the 10 Be secondary beam, the results show that, with the much higher intensities that will be available at new rare-isotope beam facilities, the ( 10 Be, 10 B + 𝛾) reaction and its Δ⁢𝑇 𝑧 = −1 partner, the ( 10 C, 10 B + 𝛾) reaction, are powerful tools for elucidating the isovector non-spin- and spin-transfer responses in nuclei.

Charge-exchange reactions↗

A New Measurement of the 60 keV Emission from Am-241 Using Metallic Magnetic Calorimeters

Here, we report a new measurement of the 60 keV transition from 241 Am. It uses a metallic magnetic calorimeter gamma-ray detector calibrated in the region around 60 keV by four accurately known X-rays and gamma rays from the decay of 169 Yb. We determine an energy of 59,539.3 ± 0.3 (stat) ± 0.3 (syst) eV, which is 1.6 ± 0.4 eV lower than the current literature value of 59,540.9 ± 0.1 eV. We discuss the sources of this uncertainty and approaches to address them.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Long Term Assessment of Radiocesium in Deer, Fish, Soil, and Vegetation at the Savannah River Site

Throughout the Savannah River Site's (SRS) operational history, many radionuclides have been released into the environment. However, due to fallout from weapons testing, the amount released from SRS, its persistence in the environment, and the seclusion of the Site, radiocesium (Cs-137) is one of the most critical radionuclides in the SRS environment. The Effective half-life (Te) is the time it takes for a radionuclide in the environment to decrease by 50% of its initial amount. There are three means of radionuclide removal: Physical: Radioactive decay, sedimentation, and washout; Chemical: Changes in pH, oxidation state or adsorption; Biological: Changes in the food web or translocation. Effective half-life (T{sub e}) = log{sub e}2/λ{sub e} Where λ{sub e} is estimated from the slopes of loge-transformed Cs-137 activity concentrations regressed on year. The objective of this work was to calculate the effective half-life of Cs-137 in various biota at SRS and to perform an assessment of the changes in the effective half life over time. Compared to 2013 data, there is a slight increase in the effective half-lives for fish at most sampling locations. This effective half-life increase is an indication that the rate of Cs-137 loss is starting to plateau. The effective half-life of Cs-137 in SRS fish ranges from 4-11 years. The effective half-life of Cs-137 in soil at the Creek plantation is about 15 years. The effective half-life of Cs-137 in grassy vegetation at the Creek Plantation is about 14 years. The effective half-life of deer hunted on the SRS is about 15.5 years. After termination of all reactor activity by 1980, the Cs-137 activity began to drop drastically.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

nEXO: neutrinoless double beta decay search beyond 10 28 year half-life sensitivity

The nEXO neutrinoless double beta (0νββ) decay experiment is designed to use a time projection chamber and 5000 kg of isotopically enriched liquid xenon to search for the decay in 136 Xe. Progress in the detector design, paired with higher fidelity in its simulation and an advanced data analysis, based on the one used for the final results of EXO-200, produce a sensitivity prediction that exceeds the half-life of 10 28 years. Specifically, improvements have been made in the understanding of production of scintillation photons and charge as well as of their transport and reconstruction in the detector. The more detailed knowledge of the detector construction has been paired with more assays for trace radioactivity in different materials. In particular, the use of custom electroformed copper is now incorporated in the design, leading to a substantial reduction in backgrounds from the intrinsic radioactivity of detector materials. Furthermore, a number of assumptions from previous sensitivity projections have gained further support from interim work validating the nEXO experiment concept. Together these improvements and updates suggest that the nEXO experiment will reach a half-life sensitivity of 1.35 × 10 28 yr at 90% confidence level in 10 years of data taking, covering the parameter space associated with the inverted neutrino mass ordering, along with a significant portion of the parameter space for the normal ordering scenario, for almost all nuclear matrix elements. Furthermore, the effects of backgrounds deviating from the nominal values used for the projections are also illustrated, concluding that the nEXO design is robust against a number of imperfections of the model.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

2022 Report - SRNL Aging and Lifetimes program tritium aging studies on structural alloys

This report documents work performed in fiscal year 2022 at SRNL in support of the Aging and Lifetimes program. This work is an enduring collaboration between SRNL and SNL to study tritium embrittlement of structural metals used in Gas Transfer System reservoirs. The measured data inform component lifetime assessments and predictions. Test coupons are thermally pre-charged with tritium and allowed to age at cryogenic temperatures to freeze out tritium diffusion and minimize off-gassing while allowing for decay helium levels to build. Coupons are removed and tested at planned intervals to measure how mechanical properties degrade as helium levels increase. This report summarizes test results from coupons which are in various stages of aging as they were tritium pre-charged in previous years, as well as documenting one new charging run.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗