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At least 541 records · Page 30
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Production and Purification of Terbium-155 Using Natural Gadolinium Targets

Terbium-155 (t 1/2 = 5.32 days) is one of four medically relevant radioisotopes of terbium. It is of interest to the field as a suitable diagnostic counterpart for therapeutic radiolanthanides, as its decay scheme includes γ-rays that are suitable for single photon emission computed tomography (SPECT) imaging. Additionally, 155 Tb has an Auger electron (AE) yield that is viable for AE therapy. There are several direct and indirect production routes that can produce 155 Tb. Two possible direct routes include proton irradiation on gadolinium targets via 155 Gd(p,n) 155 Tb and 156 Gd(p,2n) 155 Tb. The 155 Gd(p,n) 155 Tb reaction is accessible at incident proton beam energies of ∼10 MeV, whereas the 156 Gd(p,2n) 155 Tb nuclear reaction requires ∼18 MeV. This study aims to investigate the production of 155 Tb from natGd through the nat Gd(p,x) nuclear reaction, wherein both (p,n) and (p,2n) reactions were leveraged, and the purification using a three-column ion chromatography method. Using this system, recoveries of radioterbium of up to 97% were achieved in addition to high recoveries of the Gd target material, illustrating the suitability of this technique for enriched targets.

36 MATERIALS SCIENCE↗
NASA NTRS1976

Magnetospheric dynamics and wave-particle interactions

It has been demonstrated that two general classes of wave-particle interactions are of great importance for magnetospheric dynamics. Electromagnetic and electrostatic plasma instabilities give rise to relatively narrow-banded spontaneous emissions (e.g., ELF hiss, chorus, three-halves noise, ion cyclotron and ion-plasma-frequency turbulence) that can scatter trapped particles into the loss cone, leading to modified pitch-angle distributions, stable trapping limits, diffuse aurora, proton precipitation events, etc. The current-driven plasma instabilities give rise to impulsive ion acoustic or Buneman mode turbulence that provides very effective energy transfer (via the anomalous conductivity mechanism) at the bow shock and in regions where strong field-aligned currents are observed. We review these interactions and identify significant open questions that must be investigated during the IMS.

Scarf, F. L.↗
NASA NTRS1985

Spectral and spatial properties of solar microflares

Solar microflares are studied using both hard ( 28 keV) and soft (3.5 to 8.0 keV) X-ray observations. The soft X-ray events have durations 3 m at 0.1x maximum intensity, and typically have similar rise and decay times. The fastest decay observed was 15 s (1/e). Soft and hard X-ray intensities are uncorrelated. The events are very compact, consistent with a projected area approximately 8 x 8 inches. They are normally not associated with H alpha or type 3 emissions and their time profiles suggest a thermal origin at the top of the chromosphere. If the primary energy release site is in the corona, an energy transfer agent consistent with the observations is a non-thermal proton beam.

Simnett, G. M.↗
NASA NTRS2016

Deep Morphological and Spectral Study of the SNR RCW 86 with Fermi-LAT

RCW 86 is a young supernova remnant (SNR) showing a shell-type structure at several wavelengths and is thought to be an efficient cosmic-ray (CR) accelerator. Earlier Fermi Large Area Telescope results reported the detection of gamma-ray emission coincident with the position of RCW 86 but its origin (leptonic or hadronic) remained unclear due to the poor statistics. Thanks to 6.5 years of data acquired by the Fermi-LAT and the new event reconstruction Pass 8, we report the significant detection of spatially extended emission coming from RCW 86. The spectrum is described by a power-law function with a very hard photon index (Gamma = 1.42 +/- 0.1(sub stat) +/- 0.06(sub syst)) in the 0.1-500 GeV range and an energy flux above 100 MeV of (2.91 +/- 0.8(sub stat) +/- 0.12(sub syst)) x 10(exp -11) erg/(sq cms). Gathering all the available multiwavelength (MWL) data, we perform a broadband modeling of the non-thermal emission of RCW 86 to constrain parameters of the nearby medium and bring new hints about the origin of the gamma-ray emission. For the whole SNR, the modeling favors a leptonic scenario in the framework of a two-zone model with an average magnetic field of 10.2 +/- 0.7 microG and a limit on the maximum energy injected into protons of 2 x 10(exp 49) erg for a density of 1 per cu cm. In addition, parameter values are derived for the north-east and south-west (SW) regions of RCW 86, providing the first indication of a higher magnetic field in the SW region.

acceleration of particles – cosmic rays – ISM:↗
DOE OSTI2021

A Review on Bioinspired Proton Exchange Membrane Fuel Cell: Design and Materials

With the climate crisis gathering recognition, there has been significant interest in clean energy. As a reliable and clean energy solution, markets transitioning toward sustainable energy have identified polymer electrolyte membrane fuel cells (PEMFCs) as a critical technology. The increasing interest in PEMFCs is primarily due to their high energy density, high efficiency and zero greenhouse gas emission. However, additional development is required to overcome the current barriers associated with fuel cell component design, high manufacturing cost, and insufficient stability. Bioinspired designs have the potential to provide new and valuable insights using novel techniques for extracting design inspirations from biological structures. Applying these design concepts to develop materials and structures for various fuel cell components can be transformative. The well–adapted structures and functional features of biological systems have been proven to greatly enhance the performance of current designs through novel and optimized pathways. Bioinspired designs have indeed lived up to performance expectations and even exceed them. Herein, the potential and value of using these bioinspired designs are discussed. Recent studies and advancements based on nature–inspired structures for components of PEMFCs and how these design considerations substantiate their claim as an attractive alternative to conventional designs are discussed.

25 ENERGY STORAGE↗
DOE OSTI2026

Can ferric-oxyl excited states explain elongated iron-oxygen bonds in heme peroxidase catalytic intermediates?

The use of X-ray structures to determine and interpret the ferryl iron-oxygen bond order in molecular oxygen-activating heme enzymes has, in the past, been controversial. This has mainly stemmed from the susceptibility of ferryl species to X-ray-induced electronic state changes. In this work we establishe using time-resolved serial femtosecond X-ray crystallography (tr-SFX) on a dye-decolourising peroxidase that the ferryl intermediate species (Compounds I and II) captured following in situ mixing of microcrystals with H 2 O 2 have single, rather than the double bond character expected. X-ray emission validated tr-SFX data with quantum refinement, time-dependent-DFT calculations and QM/MM geometry optimizations together support the concept that the single iron-oxygen bond character is not an indication of ferryl reduction or a protonated form (Fe IV -OH) but is instead attributed to the existence of accessible excited states possessing ferric-oxyl (Fe III –O •– ) character. Such states offer insight into the nature of ferryl heme.

Williams, Lewis J. [University of Essex, Colcheste↗
NASA NTRS1982

X-ray emission from young stars and implications for the early solar system

Recent observations of soft X-ray emission from solar-type stars obtained with the Einstein X-Ray Observatory indicate that X-ray luminosity is inversely correlated with stellar age. If this result is applied to the sun and if X-ray emission is a valid indicator of other manifestations of solar activity, then past solar wind and flare levels can be inferred. It can qualitatively explain the excess xenon and nitrogen found in the lunar regolith compared to the level expected from the contemporary solar wind. X-ray emission from T Tauri and other low-mass pre-main-sequence stars is both highly luminous and variable, indicating the presence of flares approximately 4000 times stronger than the largest flares seen in the contemporary sun. The proton flux from such solar flares during the one to ten million-year pre-main-sequence phase would be sufficient to account for the Al-26 anomaly in meteorites.

Feigelson, E. D.↗
NASA NTRS1991

Outflows driven by cosmic-ray pressure in broad absorption line QSOs

It is shown how the escape of ultrarelativistic neutrons from the central engine of an AGN can lead to the production of a strong fast wind with most of the acceleration occurring outside the broad emission line region. This feature is required in order to explain observations of broad absorption line (BAL) QSOs, in which the blue wings of the broad emission lines are often absorbed. The dynamical and thermal structure of the wind is determined, and the formation of BALs in such an outflow is modeled, deriving line profiles and constraining the rate at which the energy or relativistic protons has be be converted to thermal energy in order to provide pressure confinement for the BAL clouds. The problem of acceleration and survival of the clouds is discussed.

Begelman, Mitchell↗
NASA NTRS1993

Electrotastic wave excitation in planetary magnetospheres: Application to Neptune

Voyager 2 observations of electrostatic electron and ion harmonic waves in Neptune's magnetosphere are addressed. A model of electron Bernstein modes generated by a loss cone distribution of superthermal electrons is scaled to Neptune parameters and a comparison of theory with the observed electron flux shows good agreement. A model of proton Bernstein modes generated by a ring distribution of Tritonogenic nitrogen ions is also investigated and satisfactory agreement with the data are obtained compatible with known properties of the magnetosphere. The success of the model in accounting for electrostatic emission observed by Voyager over a wide range of sampled parameters recommends its general applicability to planetary magnetospheres.

Barbosa, D. D.↗
NASA NTRS2013

Status of the GAMMA-400 Project

The preliminary design of the new space gamma-ray telescope GAMMA-400 for the energy range 100 MeV-3 TeV is presented. The angular resolution of the instrument, 1-2 deg at E(gamma) approximately 100 MeV and approximately 0.01 at E(gamma) greater than 100 GeV, its energy resolution is approximately 1% at E(gamma) greater than 100 GeV, and the proton rejection factor is approximately 10(exp 6) are optimized to address a broad range of science topics, such as search for signatures of dark matter, studies of Galactic and extragalactic gamma-ray sources, Galactic and extragalactic diffuse emission, gamma-ray bursts, as well as high-precision measurements of spectra of cosmic-ray electrons, positrons, and nuclei.

Galper, A. M.↗
NASA NTRS2021

A Ring Accelerator? Unusual Jet Dynamics in the IceCube Candidate PKS 1502+106

On 2019/07/30.86853 UT, IceCube detected a high-energy astrophysical neutrino can-didate. The Flat Spectrum Radio Quasar PKS 1502+106 is located within the 50 percent uncertainty region of the event. Our analysis of 15 GHz Very Long Baseline Ar-ray (VLBA) and astrometric 8 GHz VLBA data, in a time span prior and after theIceCube event, reveals evidence for a radio ring structure which develops with time.Several arc-structures evolve perpendicular to the jet ridge line. We find evidence forprecession of a curved jet based on kinematic modelling and a periodicity analysis.An outflowing broad line region (BLR) based on the C IV line emission (Sloan Dig-ital Sky Survey, SDSS) is found. We attribute the atypical ring to an interaction ofthe precessing jet with the outflowing material.We discuss our findings in thecontext of a spine-sheath scenario where the ring reveals the sheath andits interaction with the surroundings (NLR clouds).We find that the radioemission is correlated with theγ-ray emission, with radio lagging theγ-rays. Basedon theγ-ray variability timescale, we constrain theγ-ray emission zone to the BLR(30-200rg) and within the jet launching region. We discuss that the outflowing BLRprovides the external radiation field forγ-ray production via external Compton scat-tering.The neutrino is most likely produced by proton-proton interactionin the blazar zone (beyond the BLR), enabled by episodic encounters ofthe jet with dense clouds, i.e. some molecular cloud in the NLR.

S Britzen↗
DOE OSTI2022

Search for Lepton Flavor Violation in Two Body Muon and Pion Decay at Rest

The ability of the Mu2e experiment to probe, or discover beyond the Standard Model physics in direct Charged Lepton Flavor Violation $\mu^+$ and $\pi^+$ decay modes is estimated. These direct modes are searched for simultaneously with proposed Mu2e detector validation runs, and are complementary to the Mu2e main search goal, an indirect search for $\mu^- \to e^-$ conversion at the sensitivity level of $\sim 10^{-17}$. The $\mu^+$ validation run will operate at 50% nominal magnetic field and reduced proton beam intensity to less than 1/100th nominal, in order to observe the e+ spectrum from $\mu^+$ decay, at and below the Michel edge Ee . 53 MeV. The $\pi^+$ validation run, based on measuring the mono-energetic e+ emission in the decay $\pi^+ \to e+\nu$, at 76% of nominal magnetic field and reduced beam intensity less than 1/5th nominal. Both of these runs can be used to fix the momentum scale for the Mu2e conversion search. In addition the muon validation dataset can be used to correct for systematic errors in the detector response by mapping the well known to O(\u03B13) corrected theoretical Michel spectrum, to the observed spectrum. One direct search is for two-body Charged Lepton Flavor Violation $\mu^+ \to e^+X$ decay, where $X$ is a light new physics particle. This allows Mu2e to explore well motivated models including axion like particles with flavor violating couplings and massive $Z^0$ bosons with more sensitivity then present astrophysical and laboratory constraints. In two weeks of data-taking, Mu2e can achieve direct mode 90% confidence level branching ratio limits of $10^{-7}$ over the mass range $20 \le m_X \le 50$ MeV, improving the current experimental limit at $10^{-5}$ by two orders of magnitude. In the mass range $m_X \le 20$ MeV, assuming systematic error corrections can be made by correcting the Monte Carlo mapping, the achievable search sensitivity is found to be $2.3\times 10^{-7}$ for $m_X =0$, an order of magnitude improvement over the current best limit at $2.6\times 10^{-6}$, when assuming $V+A$ or isotropic coupling. The $\pi^+$ validation run, allows searching for $\pi^+ \to e^+N$ decay, where $N$ is a heavy neutral lepton such as a heavy sterile neutrino, in the mass region $20 \le m_N \le 65$ MeV. A branching ratio limit at 90% confidence level of $3\times 10^{-8}$ can be achieved in two weeks, an improvement of the current search sensitivity limit by an order of magnitude.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1991

Evidence for particle acceleration in AE Aqr from radio and X-ray observations

The novalike cataclysmic variable AE Aquarii shows evidence for radio synchrotron emission from expanding magnetized clouds. The radio and UV flare timescales are similar indicating that the central engine is located close to the white dwarf. A collisionless shock may develop above the polar cap, which may explain the observed temperature. Protons and ions accelerated up to energies of more than 1 TeV can diffuse away from the central engine, enter magnetized clouds, and generate waves which in turn heat and accelerate electrons. An embarrassing situation exists where reprocessed optical and X-ray pulsations (33 s) are observed, but the expected direct X-ray pulse from the white dwarf is absent. The standard theory for CVs cannot explain this, and one possible explanation is that a beam of relativistic protons and ions from the polar cap may give the observed reprocessed optical to X-rays in a thick target fixed in the system.

De Jager, O. C.↗
NASA NTRS2003

Self-Consistent Model of Magnetospheric Ring Current and Electromagnetic Ion Cyclotron Waves: The May 2-7, 1998, Storm

Complete description of a self-consistent model for magnetospheric ring current interacting with electromagnetic ion cyclotron waves is presented. The model is based on the system of two kinetic equations; one equation describes the ring current ion dynamics, and another equation describes the wave evolution. The effects on ring current ions interacting with electromagnetic ion cyclotron waves, and back on waves, are considered self-consistently by solving both equations on a global magnetospheric scale under non steady-state conditions. In the paper by Khazanov et al. [2002] this self-consistent model has only been shortly outlined, and discussions of many the model related details have been omitted. For example, in present study for the first time a new algorithm for numerical finding of the resonant numbers for quasilinear wave-particle interaction is described, or it is demonstrated that in order to describe quasilinear interaction in a multi-ion thermal plasma correctly, both e and He(+) modes of electromagnetic ion cyclotron waves should be employed. The developed model is used to simulate the entire May 2-7, 1998 storm period. Trapped number fluxes of the ring current protons are calculated and presented along with their comparison with the data measured by the 3D hot plasma instrument Polar/HYDRA. Examining of the wave (MLT, L shell) distributions produced during the storm progress reveals an essential intensification of the wave emissions in about two days after main phase of storm. This result is well consistent with the earlier ground-based observations. Also the theoretical shapes and the occurrence rates for power spectral densities of electromagnetic ion cyclotron waves are studied. It is found that in about 2 days after the storm main phase on May 4, mainly non Gaussian shapes of power spectral densities are produced.

Khazanov, G. V.↗
NASA NTRS2012

Design and Performance of the GAMMA-400 Gamma-Ray Telescope for Dark Matter Searches

The GAMMA-400 gamma-ray telescope is designed to measure the fluxes of gamma-rays and cosmic-ray electrons + positrons, which can be produced by annihilation or decay of the dark matter particles, as well as to survey the celestial sphere in order to study point and extended sources of gamma-rays, measure energy spectra of Galactic and extragalactic diffuse gamma-ray emission, gamma-ray bursts, and gamma-ray emission from the Sun. GAMMA-400 covers the energy range from 100 MeV to 3000 GeV. Its angular resolution is approx. 0.01 deg (E(sub gamma) > 100 GeV), the energy resolution approx. 1% (E(sub gamma) > 10 GeV), and the proton rejection factor approx 10(exp 6). GAMMA-400 will be installed on the Russian space platform Navigator. The beginning of observations is planned for 2018.

Dark Matter↗
NASA NTRS1984

Voyager 1 evidence for ion-cyclotron instability in the vicinity of the Io plasma Torus

The Voyager 1 traversal of the Io plasma torus was marked by pronounced enhancement in low frequency wave activity with especially strong wave intensification below the proton gyrofrequency, suggesting the excitation of ion-cyclotron waves over the same radial range in which the energetic ring current ions exhibit phase space density depletion due to strong pitch angle scattering loss to the atmosphere. If the more intense emissions observed intermittently by Voyager 1 are representative of waves in the high latitude source region, the resulting pitch angle scattering would be sufficiently rapid to explain the observed energetic ion losses and the excitation of intense Jovian auroral emissions of field lines passing through the torus.

Thorne, R. M.↗
NASA NTRS1994

Proton-induced fragmentation of carbon at energies below 100 MeV

Radiation effects caused by single cosmic ray particles have been studied for many years in radiobiological experiments for different biological objects and biological end-points. Additionally, single event effects in microelectronic devices have gained large interest. There are two fundamental mechanisms by which a single particle can cause radiation effects. On the one hand, a cosmic ray ion with high linear energy transfer can deposit a high dose along its path. On the other hand, in a nuclear collision, a high dose can be deposited by short range particles emitted from the target nucleus. In low earth orbits a large contribution to target fragmentation events originates from trapped protons which are encountered in the South Atlantic Anomaly. These protons have energies up to a few hundred MeV. We study the fragmentation of C, O and Si nuclei - the target nuclei of biological material and microelectronic devices - in nuclear collisions. Our aim is to measure production cross sections, energy spectra, emission directions and charge correlations of the emitted fragments. The present knowledge concerning these data is rather poor. M. Alurralde et al. have calculated cross sections and average energies of fragments produced from Si using the cascade-evaporation model. D.M. Ngo et al. have used the semiempirical cross section formula of Silberberg and Tsao to calculate fragment yields and the statistical model of Goldhaber to describe the reaction kinematics. Cross sections used in these models have uncertainties within a factor of two. Our data will help to test and improve existing models especially for energies below 300 MeV/nucleon. Charge correlations of fragments emitted in the same interaction are of particular importance, since high doses can be deposited if more than one heavy fragment with a short range is produced.

Schmitz, M.↗
DOE OSTI2020

Valence-to-core X-ray emission spectroscopy of titanium compounds using energy dispersive detectors

X-ray emission spectroscopy (XES) of transition metal compounds is a powerful tool for investigating the spin and oxidation state of the metal centers. Valence-to-core (vtc) XES is of special interest, as it contains information on the ligand nature, hybridization, and protonation. To date, most vtc-XES studies have been performed with high-brightness sources, such as synchrotrons, due to the weak fluorescence lines from vtc transitions. Here, we present a systematic study of the vtc-XES for different titanium compounds in a laboratory setting using an X-ray tube source and energy dispersive microcalorimeter sensors. With a full-width at half-maximum energy resolution of approximately 4 eV at the Ti Kβ lines, we measure the XES features of different titanium compounds and compare our results for the vtc line shapes and energies to previously published and newly acquired synchrotron data as well as to new theoretical calculations. Finally, we report simulations of the feasibility of performing time-resolved vtc-XES studies with a laser-based plasma source in a laboratory setting. Our results show that microcalorimeter sensors can already perform high-quality measurements of vtc-XES features in a laboratory setting under static conditions and that dynamic measurements will be possible in the future after reasonable technological developments.

36 MATERIALS SCIENCE↗