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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 541 records · Page 30
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

A search for prompt lepton-jets in pp collisions at √s = 8 TeV with the ATLAS detector

We present a search for a new, light boson with a mass of about 1 GeV and decaying promptly to jets of collimated electrons and/or muons (lepton-jets). The analysis is performed with 20.3 fb -1 of data collected by the ATLAS detector at the Large Hadron Collider in proton-proton collisions at a centre-of-mass energy of 8 TeV. Events are required to contain at least two lepton-jets. This study finds no statistically significant deviation from predictions of the Standard Model and places 95% confidence-level upper limits on the contribution of new phenomena beyond the SM, incuding SUSY-portal and Higgs-portal models, on the number of events with lepton-jets.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2012

CO2/light gas separation performance of cross-linked poly(vinylimidazolium) gel membranes as a function of ionic liquid loading and cross-linker content

A series of cross-linked poly(vinylimidazolium)-RTIL gel membranes was synthesized and evaluated for room-temperature, ideal CO2/N-2, CO2/CH4, and CO2/H-2 separation performance. The membranes were formed by photo-polymerization of oligo(ethylene glycol)-functionalized cross-linking (i.e., di-functional) and non-cross-linking (i.e., mono-functional) vinylimidazolium RTIL monomers with nonpolymerizable, "free RTIL." The effect of free RTIL ([emim][Tf2N]) loading on CO2 separation performance was evaluated by varying RTIL loading at three levels (45, 65, and 75 wt.%). The effect of cross-linker content on CO2 separation performance was also evaluated by varying the copolymer composition of cross-linked membranes from 5 to 100 mol% di-functional monomer. The substituent on the monofunctional RTIL monomer was also varied to investigate the effect of substituent structure and chemistry on CO2 separation performance. CO2 permeability was dramatically increased with higher loading of free RTIL. Increased RTIL loading had no effect on CO2/N-2 or CO2/CH4 permeability selectivity, but significantly improved CO2/H-2 permeability selectivity. Reducing the cross-linking monomer concentration generally improved CO2 permeability. However, anomalous permeability and selectivity behavior was observed below critical concentrations of cross-linker. The effect of the substituent on the monofunctional monomer on CO2 separation performance was minimal compared to the effects of RTIL loading and copolymer composition. (C) 2012 Elsevier B.V. All rights reserved.

Carlisle, TK↗
DOE OSTI2013

Effect of composition and nanostructure on CO2/N-2 transport properties of supported alkyl-imidazolium block copolymer membranes

Polymerized room-temperature ionic liquids (poly(RTIL)s) have garnered attention as new and interesting membrane materials for CO2/light gas separations because they combine the high CO2 affinity and thermal and chemical stability of RTILs, with the physical and mechanical properties of polymeric materials. Our group recently synthesized a new type of block copolymer (BCP) combining an imidazolium-based poly(RTIL) and an alkyl non-ionic polymer. These alkyl-b-ionic BCPs phase-separate into ordered nanostructures. Prior work investigating gas transport through phase-separated BCPs is very limited, and none has included RTIL-based BCP systems. However it has been shown that nanoscale phase-separation could facilitate gas transport via nanostructure orientation control or phase connectivity improvement. We have successfully made defect-free, thin-film composite membranes with these novel alkyl-imidazolium BCPs as a 3-20 mu m thick top layer, and determined their CO2/N-2 separation properties via single-gas permeability measurements and selectivity calculations. These new BCP materials were found to have distinct advantages over the analogous physical blends of the parent homopolymers with respect to membrane fabrication. The composition of the BCP top layer, which is directly connected to the type of nanostructure formed, was found to have a significant effect on CO2 permeability (i.e., it can increase CO2 permeability by two orders of magnitude up to an observed value of 9300 barrer). This improvement is mainly due to a large increase in the diffusion coefficient in the ordered nanostructures compared to amorphous BCP materials. (C) 2012 Elsevier B.V. All rights reserved.

Nguyen, PT↗
DOE OSTI2011

Search for neutral MSSM Higgs bosons decaying to tau(+)tau(-) pairs in proton-proton collisions root s=7 TeV with the ATLAS detector

A search for neutral Higgs bosons decaying to pairs of {tau} leptons with the ATLAS detector at the LHC is presented. The analysis is based on proton-proton collisions at a center-of-mass energy of 7 TeV, recorded in 2010 and corresponding to an integrated luminosity of 36 pb{sup -1}. After signal selection, 276 events are observed in this data sample. The observed number of events is consistent with the total expected background of 269 {+-} 36 events. Exclusion limits at the 95% confidence level are derived for the production cross section of a generic Higgs boson {phi} as a function of the Higgs boson mass and for A/H/h production in the Minimal Supersymmetric Standard Model (MSSM) as a function of the parameters m{sub A} and tan {beta}.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2011

Measurement of the inclusive isolated prompt photon cross-section in pp collisions at root s=7 TeV using 35 pb(-1) of ATLAS data

A measurement of the differential cross-section for the inclusive production of isolated prompt photons in pp collisions at a center-of-mass energy {radical}s = 7 TeV is presented. The measurement covers the pseudorapidity ranges |{eta}| < 1.37 and 1.52 {le} |{eta}| < 2.37 in the transverse energy range 45 {le} E{sub T} < 400 GeV. The results are based on an integrated luminosity of 35 pb{sup -1}, collected with the ATLAS detector at the LHC. The yields of the signal photons are measured using a data-driven technique, based on the observed distribution of the hadronic energy in a narrow cone around the photon candidate and the photon selection criteria. The results are compared with next-to-leading order perturbative QCD calculations and found to be in good agreement over four orders of magnitude in cross-section.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2012

Measurement of the top quark pair production cross-section with ATLAS in the single lepton channel

A measurement of the production cross-section for top quark pairs ($t\bar{t}$) in pp collisions at $\sqrt{s} = 7TeV is presented using data recorded with the ATLAS detector at the Large Hadron Collider. Events are selected in the single lepton topology by requiring an electron or muon, large missing transverse momentum and at least three jets. With a data sample of 35 pb -1 , two different multivariate methods, one of which uses b-quark jet identification while the other does not, use kinematic variables to obtain cross-section measurements of σ $t\bar{t}$ = 187±11 (stat.) $+18\atop{-17}$ (syst.) ± 6 (lumi.) pb and σ $t\bar{t}$ =173 ± 17 (stat.) $+18\atop{-16}$ (syst.) ± 6 (lumi.) pb respectively. In conclusion, the two measurements are in agreement with each other and with QCD calculations. The first measurement has a better a priori sensitivity and constitutes the main result of this Letter.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Ordered, microphase-separated, noncharged-charged diblock copolymers via the sequential ATRP of styrene and styrenic imidazolium monomers

A series of imidazolium-based noncharged-charged diblock copolymers (1) was synthesized by the direct, sequential ATRP of styrene and styrenic imidazolium bis(trifluoromethyl)sulfonamide monomers with methyl, n-butyl, and n-decyl side-chains. Small-angle X-ray scattering studies on initial examples of 1 with a total of 50 repeat units and styrene:imidazolium-styrene repeat unit ratios of 25:25, 20:30, and 15:35 showed that their ability to form ordered nanostructures (i.e., sphere and cylinder phases) in their neat states depends on both the block ratio and the length of the alkyl side-chain on the imidazolium monomer. To our knowledge, the synthesis of imidazolium-based BCPs that form ordered, phase-separated nanostructures via direct ATRP of immiscible co-monomers is unprecedented. (C) 2014 Elsevier Ltd. All rights reserved.

Shi, ZX↗
DOE OSTI2012

Modified normal-phase ion-pair chromatographic methods for the facile separation and purification of imidazolium-based ionic compounds

lmidazolium- and oligo(imidazolium)-based ionic organic compounds are important in the design of room-temperature ionic liquid materials; however, the chromatographic analysis and separation of such compounds are often difficult. A convenient and inexpensive method for effective thin-layer chromatography (TLC) analysis and column chromatography separation of imidazolium-based ionic compounds is presented. Normal-phase ion-pair TLC is used to effectively analyze homologous mixtures of these ionic compounds. Subsequent separation of the mixtures is performed using ion-pair flash chromatography on normal-phase silica gel, yielding high levels of recovery. This method also results in a complete exchange of the counter anion on the imidazolium compounds to the anion of the ion-pair reagent. (C) 2012 Elsevier Ltd. All rights reserved.

Urban, ND↗