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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 541 records · Page 30
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Effects of the electrical parameters and gas flow rate on the generation of reactive species in liquids exposed to atmospheric pressure plasma jets

In this work, an atmospheric pressure plasma jet was fabricated and studied for plasma–liquid interactions. The plasma jet consists of a quartz-covered pin electrode and outer quartz tube with a tapered nozzle. Using the current–voltage (I-V) and optical emission characteristics of the plasma jet, the plasma density and the speed of the plume were investigated. The optical emission spectra clearly indicated the excited NO, O, OH, N{sub 2}, and N{sub 2}{sup +} in the plasma plumes. Then the plasma jets were applied to the deionized water. We investigated the effects of the operating parameters such as applied voltage, pulse frequency, and gas flow rate on the generation of reactive species in the gas and liquid phases. The densities of reactive species including OH radicals were obtained at the plasma–liquid surface and inside the plasma-treated liquids using ultraviolet absorption spectroscopy and chemical probe method. The nitrite concentration was detected by Griess assay. The data are very suggestive that there is a strong correlation among the production of reactive oxygen and nitrogen species (RONS) in the plasmas and liquids.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

Radio-frequency capacitive discharge with flowing liquid electrodes at reduced gas pressures

Results are presented from experimental studies of the electrophysical and spectral characteristics of the low-temperature plasma of a radio-frequency capacitive discharge excited between two flowing liquid electrodes at gas pressures of 10{sup 3}−10{sup 5} Pa. The plasma composition, the electron density, and the vibrational and rotational temperatures of gas molecules are estimated. The types and shapes of discharge are described, and the thermal and gas-hydrodynamic processes in the discharge zone are analyzed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1977

Lower hybrid emission diagnostics on the NASA Lewis Bumpy Torus

The feasibility of using RF emission near the lower-hybrid frequency of the NASA Lewis Bumpy Torus plasma for diagnostic purposes is examined. The emission is detected using a spectrum analyzer and a 50-ohm miniature coaxial antenna that is sensitive to the polarization of the incoming signal. The frequency shift of the lower-hybrid emission peak is monitored as a function of the background pressure, electrode voltage, electrode ring configuration, and the strength of the toroidal dc magnetic field. Simultaneous measurements of the average plasma density are made with a polarization diplexing microwave interferometer. The experimental results extend previous work to include negative electrode voltages and plasma densities up to 1 trillion per cu cm. The information derived from the experiment is discussed with reference to: (1) the strength of the dc magnetic field in the emitting region, (2) a comparison of the lower-hybrid plasma density with the average plasma density, and (3) the validity of the cold-plasma lower-hybrid resonance formula in the high-density operating regime of the bumpy-torus plasma.

Mallavarpu, R.↗
DOE OSTI2020

AMPPED LDRD: Advanced Models of the Physics & Phenomena of Electrical Discharge.

This Laboratory Directed Research and Development (LDRD) project aimed at addressing an unmet need for physics-based models that enable prediction of electrical breakdown in the presence of high voltage gradients and real-world environments. This project focused on understanding coupled plasma-surface feedback phenomena critical to electrical discharge processes and design of breakdown voltages, breakdown times, and breakdown paths. New secondary electron emission and coupled plasma-surface measurement methods and models were developed. Highly reproducible discharge experiments were developed to provide current-voltage data as a function of time, and methods were developed to condition electrodes for predictable discharge. To assess plasma-surface feedback mechanisms, new surface physics capabilities, including measurement systems for local and global photoemission yield and ion-induced secondary electron emission yield were developed. Discharge models were developed to incorporate these yields for predicting discharge behavior to understand influence of surface physics on discharge current and time evolution, and methods to accelerate these simulations were demonstrated. A key finding was that the initiation process of a non-vacuum discharge appears highly dependent on photoemission at the cathode. Advanced diagnostics were developed, including spatial electrical field imaging, spectroscopy of plasmas, and high-speed imaging of discharge event s in metal and dielectric environments. These diagnostics and improved electrical models are a step toward enabling quantitative design margins, assurance of safety architectures, and implementation of novel materials and technologies for wide ranging energy and electronics applications.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Linear electromagnetic excitation of an asymmetric low pressure capacitive discharge with unequal sheath widths

It is well-known that standing waves having radially center-high radio frequency (rf) voltage profiles exist in high frequency capacitive discharges. In this work, we determine the symmetric and antisymmetric radially propagating waves in a cylindrical capacitive discharge that is asymmetrically driven at the lower electrode by an rf voltage source. The discharge is modeled as a uniform bulk plasma which at lower frequencies has a thicker sheath at the smaller area powered electrode and a thinner sheath at the larger area grounded electrode. These are self-consistently determined at a specified density using the Child law to calculate sheath widths and the electron power balance to calculate the rf voltage. The fields and the system resonant frequencies are determined. The center-to-edge voltage ratio on the powered electrode is calculated versus frequency, and central highs are found near the resonances. The results are compared with simulations in a similar geometry using a two-dimensional hybrid fluid-analytical code, giving mainly a reasonable agreement. The analytic model may be useful for finding good operating frequencies for a given discharge geometry and power.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2012

Wear behavior of AISI 1090 steel modified by pulse plasma technique

AISI 1090 steel was pulse plasma treated (PPT) using a Molybdenum electrode. Two different pulse numbers were chosen to obtain modified layers of 20{+-}5 {mu}m thickness. The dry sliding wear studies performed on this steel with and without PPT against an alumina ball counterpart showed that the PPT improved the wear resistance. The pulse number of the PPT modified layer was found to be highly influential in imparting the wear resistance to this steel, due to enhancement of surface hardness depending on treatment time.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Measuring characteristic differences between high- and low-performing discharges on the MegaJOuLe Neutron Imaging Radiography (MJOLNIR) DPF

A dense plasma focus (DPF) is a compact coaxial plasma gun, which completes its discharge as a Z-pinch, producing short (<100 ns) pulses of ions, x rays, and/or neutrons. Lawrence Livermore National Laboratory recently constructed and began operating a new device, the MJOLNIR (MegaJOuLe Neutron Imaging Radiography) DPF, which is designed for single-pulse flash neutron radiography. This device has achieved neutron yields of up to 4.1×10 11 neutrons/pulse at 3.3 MA peak current, and higher-current commissioning is under way. Like most DPFs, MJOLNIR exhibits variable yields in some configurations. Here, we present evidence of the role of parasitic current paths within the gun in stochastically influencing the yield. First through “conditioning shots,” where new hardware has been introduced, we show that increased run-down and run-in speeds correlate with higher yields. These observations are consistent with current being delivered to the electrodes but not to the main plasma sheath, degrading the implosion-driving force. Once nominal conditions are established, we correlate low-performing discharges with smaller current dip and associated voltage spike for a fixed machine configuration. A snow-plow model is able to recreate small-magnitude current dips through the introduction of a parasitic current path, and particle-in-cell simulations establish how parasitic current paths lower the ion beam energy available to produce neutrons. Finally, we observe an increased likelihood of shots with low yield and smaller current dip with increasing fill pressure.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Experimental studies of the difference between plasma potentials measured by Langmuir probes and emissive probes in presheaths

The plasma potential measured by cylindrical and planar Langmuir probes has been shown to differ from the plasma potential measured by emissive probes in the neighborhood of the presheath near a negatively biased electrode immersed in a weakly collisional low temperature argon plasma. There are two principal results demonstrated in this paper. First, while it is well known that Langmuir probes cannot reliably measure plasma potentials inside of sheaths, results presented here demonstrate that the problem persists in presheaths, the quasineutral plasma bordering sheaths. It is known that emissive probes analyzed in the limit of zero emission accurately measure the plasma potential in the sheath. It is now clear that they are the only known electrostatic probe technique able to measure the plasma potential accurately throughout the presheath. Second, it is shown that the difference between potential measurements made by Langmuir probes and emissive probes in the body of the plasma, farther than a presheath distance from the boundary, is not proportional to T e , as has been previously claimed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Experiments with biased side electrodes in electron cyclotron resonance ion sources

The output of highly charged ions from an electron cyclotron resonance ion source (ECRIS) consists of ionic losses from a highly confined plasma. Therefore, an increase of the output of the ions of interest always is a compromise between an increase in the confinement and an increase of the losses. One route towards a solution consists of attacking the losses in directions – i.e., radial directions – that do not contribute to the required output. This was demonstrated in an experiment (using the Kei ECRIS at NIRS, Japan) where radial losses were electrostatically reduced by positively biasing one set of six “side” electrodes surrounding the plasma in side-ward directions attached (insulated) to the cylindrical wall of the plasma chamber. Recently new studies were performed in two laboratories using two essentially different ion sources. At the BioNano ECRIS (Toyo University, Japan) various sets of electrodes were used; each of the electrodes could be biased individually. At the Atomki ECRIS (Hungary), one movable, off-axis side electrode was applied in technically two versions. The measurements show indeed a decrease of ionic losses but different effectivities as compared to the biased disk.

43 PARTICLE ACCELERATORS↗
DOE OSTI2024

Effect of V Content on Corrosion Behavior of Al-V Alloys Produced by Mechanical Alloying and Subsequent Spark Plasma Sintering

Al-V alloys produced via high-energy ball milling have been reported to show simultaneous improvement of corrosion resistance and mechanical properties compared to traditional Al alloys. In these alloys, V content plays a crucial role in increasing or decreasing the corrosion resistance. Therefore, the effect of V and microstructure on corrosion of high-energy ball milled and subsequently spark plasma sintered Al-xV alloys (x = 2, 5, 10 at%) has been studied. Cyclic potentiodynamic polarization tests and electrochemical impedance spectroscopic analysis revealed the increment of V content up to 5 at% enhanced the corrosion resistance of the alloy. However, highly heterogeneous microstructure in Al-10 at%V resulted in significant localized corrosion over the immersion time. The electrochemical impedance spectroscopy studies over 14 days of immersion revealed underlying corrosion mechanisms.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Pulsed power accelerator surface Joule heating models

Understanding the effects of contaminant plasmas generated within the Z machine at Sandia is critical to understanding current loss mechanisms. The plasmas are generated at the accelerator electrode surfaces and include desorbed species found in the surface and substrate of the walls. These desorbed species can become ionized. The timing and location of contaminant species desorbed from the wall surface depend non-linearly on the local surface temperature. For accurate modeling, it is necessary to utilize wall heating models to estimate the amount and timing of material desorption. One of these heating mechanisms is Joule heating. In this paper, we propose several extended semi-analytic magnetic diffusion heating models for computing surface Joule heating and demonstrate their effects for several representative current histories. We quantitatively assess under what circumstances these extensions to classical formulas may provide a validatable improvement to the understanding of contaminant desorption timing.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Electrochemical Structure of the Plasma–Liquid Interface

Nonthermal atmospheric pressure plasma in contact with a liquid yields a variety of energetic photons, ions, and electrons, which can be transported into the plasma–liquid interface (PLI). Similar to the electrochemical interface formed between a solid electrode and electrolyte in conventional electrochemical systems, the charge-transfer process across the PLI is able to promote reduction–oxidation (redox) reactions. However, in the case of free plasma jets in contact with liquids, the absence of solid electrodes obscures the spatial locations of the electrochemical half-reactions. Herein, we present a spatial electrochemical measurement technique used to characterize an aqueous solution in contact with an atmospheric pressure plasma jet. The technique is based on measuring the potential difference between two identical Ag/AgCl electrochemical electrodes positioned at different locations within the solution. More specifically, electrochemical maps were made by measuring the potential of one electrochemical electrode positioned at different locations near the PLI with respect to the other electrochemical electrode positioned far away from the PLI in the bulk solution. Regions in the map with negative and positive potential differences between these electrochemical electrodes were used to identify the electrodeless cathode and anode, respectively. Here, visualization of the spatial distribution of molecular colorimetric redox indicators by multispectral imaging revealed that reduction was occurring near the plasma jet centerline while oxidation was occurring further away in solution, which constitutes an independent confirmation of the electrochemical maps.

Absorption↗
DOE OSTI2013

Influence of the gas-flow Reynolds number on a plasma column in a glass tube

Atmospheric-plasma generation inside a glass tube is influenced by gas stream behavior as described by the Reynolds number (Rn). In experiments with He, Ne, and Ar, the plasma column length increases with an increase in the gas flow rate under laminar flow characterized by Rn < 2000. The length of the plasma column decreases as the flow rate increases in the transition region of 2000 < Rn < 4000. For a turbulent flow beyond Rn > 4000, the length of the plasma column is short in front of the electrode, eventually leading to a shutdown.

42 ENGINEERING↗
DOE OSTI2012

Development of a dielectric barrier discharge enhanced plasma jet in atmospheric pressure air

A plasma jet equipped with dielectric barrier discharge (DBD) is developed to generate diffuse air plasma with fairly large gap and cross sectional area. The diffuse air plasma has two discharge modes under different gap widths from the nozzle to the ground plate electrode. For large gap width, a diffuse plume fills the whole space between the nozzle and the plate electrode after coaxial DBD is ignited when the applied voltage reaches a certain value. Rather than diffuse plasma plume, a bright plasma column bridges the nozzle and the plate electrode with further increasing the applied voltage under small gap width. By optical and electrical measurement, results show that the macroscopically diffuse discharge in air is obtained by the superimposition of radially distributed streamers that appear at different cycles of the applied voltage, and the bright plasma column belongs to atmospheric pressure glow discharge. The molecular vibrational temperature and the gas temperature are given as functions of the peak value of the applied voltage.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1978

A dense plasma ultraviolet source

The intense ultraviolet emission from the NASA Hypocycloidal-Pinch (HCP) plasma is investigated. The HCP consists of three disk electrodes whose cross section has a configuration similar to the cross section of a Mather-type plasma focus. Plasma foci were produced in deuterium, helium, xenon, and krypton gases in order to compare their emission characteristics. Time-integrated spectra in the wavelength range from 200 nm to 350 nm and temporal variations of the uv emission were obtained with a uv spectrometer and a photomultiplier system. Modifications to enhance uv emission in the iodine-laser pump band (250 to 290 nm) and preliminary results produced by these modifications are presented. Finally, the advantages of the HCP as a uv over use of conventional xenon lamps with respect to power output limit, spectral range, and lifetime are discussed.

Lee, J. H.↗
DOE OSTI2021

Mitigation of breathing oscillations and focusing of the plume in a segmented electrode wall-less Hall thruster

We report in the absence of the channel walls bounding the plasma, a wall-less Hall thruster is a promising configuration with a potentially longer lifetime and easier scalability than conventional Hall thrusters. Because the ion acceleration takes place in the fringing magnetic field with a strong axial component, the operation of a typical wall-less thruster is characterized by a large beam divergence of the plasma flow, which reduces the thrust. In this work, the addition of a biased segmented electrode to the wall-less thruster is shown to significantly narrow the plasma plume and suppress large amplitude breathing oscillations of the discharge current commonly associated with ionization instability. Both effects result in improvements to the thruster performance. Physical mechanisms responsible for these effects are unclear, but they are apparently associated with the reduction of the electron cross field transport to the anode and a transition in the breathing mode frequency.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2011

Thrust Stand Measurements Using Alternative Propellants in the Microwave Assisted Discharge Inductive Plasma Accelerator

Storable propellants (for example water, ammonia, and hydrazine) are attractive for deep space propulsion due to their naturally high density at ambient interplanetary conditions, which obviates the need for a cryogenic/venting system. Water in particular is attractive due to its ease of handling and availability both terrestrially and extra-terrestrially. While many storable propellants are reactive and corrosive, a propulsion scheme where the propellant is insulated from vulnerable (e.g. metallic) sections of the assembly would be well-suited to process these otherwise incompatible propellants. Pulsed inductive plasma thrusters meet this criterion because they can be operated without direct propellant-electrode interaction. During operation of these devices, electrical energy is capacitively stored and then discharged through an inductive coil creating a time-varying current in the coil that interacts with a plasma covering the face of the coil to induce a plasma current. Propellant is accelerated and expelled at a high exhaust velocity (O(10-100 km/s)) by the Lorentz body force arising from the interaction of the magnetic field and the induced plasma current. While this class of thruster mitigates the life-limiting issues associated with electrode erosion, many pulsed inductive plasma thrusters require high pulse energies to inductively ionize propellant. The Microwave Assisted Discharge Inductive Plasma Accelerator (MAD-IPA) is a pulsed inductive plasma thruster that addressees this issue by partially ionizing propellant inside a conical inductive coil before the main current pulse via an electron cyclotron resonance (ECR) discharge. The ECR plasma is produced using microwaves and a static magnetic field from a set of permanent magnets arranged to create a thin resonance region along the inner surface of the coil, restricting plasma formation, and in turn current sheet formation, to a region where the magnetic coupling between the plasma and the theta-pinch coil is high. The use of a conical theta-pinch coil also serves to provide neutral propellant containment and plasma plume focusing that is improved relative to the more common planar geometry of the Pulsed Inductive Thruster (PIT). In this paper, we describe thrust stand measurements performed to evaluate the specific impulse and thrust efficiency of the MAD-IPA for a variety of propellants. Propellants tested include both widely-used, non-reactive noble gases like argon, and rarely-used propellants such as water, hydrazine and ammonia. Dependencies of impulse data on propellant species are discussed in the context of the current sheet formation and electromagnetic plasma acceleration processes.

Hallock, Ashley K.↗
DOE OSTI2023

Effects of oxidant gas for atomic layer deposition on crystal structure and fatigue of ferroelectric Hf x Zr 1-x O 2 thin films

TiN/Hf x Zr 1-x O 2 (HZO)/TiN capacitors were prepared using two types of HZO films fabricated by atomic layer deposition using H 2 O or O 2 plasma as an oxidant gas, and post-deposition annealing at 400 °C was performed before the TiN top-electrode fabrication. The ferroelectric orthorhombic phase was dominantly formed for the O 2 plasma-based capacitor due to the strongly oxidizing source of O 2 plasma, resulted in higher remanent polarization (2P r = 20 µC/cm 2 ) than that (13 µC/cm 2 ) of the H 2 O-based capacitor. The fatigue properties for the O 2 plasma-based capacitor were improved by 14 % after 106 cycles compared to the H 2 O-based capacitor. This could be attributed to an oxygen-rich interface reaction layer (IRL) including TiO x between the HZO film and TiN bottom-electrode for the O 2 plasma-based capacitor. In conclusion, based on these results, superior 2P r and fatigue properties can be obtained using O 2 plasma-based HZO films.

36 MATERIALS SCIENCE↗