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An Optical Streaking Method for Measuring Femtosecond Electron Bunches

The measurement of the ultra-short electron bunch length on the femtosecond time scale constitutes a very challenging problem. In the x-ray free electron laser facilities such as the Linac Coherent Light Source, generation of a sub-ten femtoseconds electron beam with 20pC charge is possible, but direct measurements are very difficult due to the resolution limit of the present diagnostics. We propose a new method here based on the measurement of the electron beam energy modulation induced from laser-electron interaction in a short wiggler. A typical optical streaking method requires a laser wavelength much longer than the electron bunch length. In this paper a laser with its wavelength shorter than the electron bunch length has been adopted, while the slope on the laser intensity envelope is used to distinguish the different periods. With this technique it is possible to reconstruct the bunch longitudinal profile from a single shot measurement. Generation of ultrashort x-ray pulses at femtoseconds (fs) scale is of great interest within synchrotron radiation and free electron laser (FEL) user community. One of the simple methods is to operate the FEL facility at low charge. At the Linac Coherent Light Source (LCLS), we have demonstrated the capability of generating ultrashort electron-beam (e-beam) with a duration of less than 10 fs fwhm using 20 pC charge. The x-ray pulses have been delivered to the x-ray users with a similar or even shorter pulse duration. However, The measurement of such short electron or x-ray pulse length at the fs time-scale constitutes a challenging problem. A standard method using an S-band radio-frequency (rf) transverse deflector has been established at LCLS, which works like a streak camera for electrons and is capable of resolving bunch lengths as short as 25 fs fwhm. With this device, the electrons are transversely deflected by the high-frequency time-variation of the deflecting fields. Increasing the deflecting voltage and rf frequency are the right direction to achieve a better resolution. For example, by choosing an X-band transverse deflecting cavity, the expected resolution for LCLS beam with 4.3 GeV is about 1 fs rms. Typically the rf breakdown threshold and the power source availability prevent going to even higher voltage and frequency. With the highly-developed laser techniques, we can choose to streak the beam at optical frequencies. By jumping from rf to optical frequency, the wavelength is shortening by 4 to 5 orders. With an electron bunch length shorter than half period of the laser, we can apply the similar rf deflecting or zero-phasing method for e-beam bunch length measurements using a high-power laser. A short wiggler is required to provide interaction between the electron and the laser. For example, to measure the e-beam at the order of 1 m rms length, a laser with its wavelength of 10 {mu}m may be considered. For a typical few GeV e-beam, the wiggler period has to be large to satisfy the resonance condition. Also, if the e-beam is longer than one laser period, the different modulation periods will overlap and we cannot distinguish them. So this method is so far limited by the achievable long-wavelength laser power. To get an effective modulation on an e-beam of 4.3 GeV, the required laser power is about a few tens GW. In this paper we propose to adopt a high-power Ti:Sapphire laser (wavelength of 800 nm), and use the slope in the intensity envelope to distinguish the different modulation periods. First an ultrashort electron beam interacts with the Ti:Sapphire laser in a wiggler, where the electron energy is modulated at the same periods of the laser. If the laser pulse is long and the short electron bunch is overlapped (in time) with the middle part of the laser, such as the setup at LCLS laser heater, the different energy modulation periods on the electron beam will be overlapped on the energy profile. In this conditionwe typically have a double-horn distribution of the energy profile, and the electron-bunch length information cannot be retrieved. But if the laser pulse (with a Gaussian temporal shape) is relatively short, we can synchronize the e-beam with the laser at the slope region of the intensity envelope, and the amplitude of each energy modulation period will be different. Then these electrons pass through a dispersive section such as a spectrometer, after that this periodically-modulated energy profile can be observed in a transverse screen. By properly choosing the laser parameters, each modulation period will show as a separate streak on the screen. This modulation period in energy dimension correlates to the laser wavelength in time dimension. Since the laser wavelength is a known parameter, no additional calibration is needed. This provides a single shot, self-calibrated method for ultrashort electron bunch length measurements.

43 PARTICLE ACCELERATORS↗

The chemRIXS Instrument for Solution-Phase Resonant Inelastic X-ray Scattering at the Linac Coherent Light Source

The chemRIXS instrument at the Linac Coherent Light Source (LCLS) offers new opportunities for studying solution-phase systems with time-resolved soft X-ray spectroscopic methods such as resonant inelastic X-ray scattering (RIXS) using the recently commissioned high-repetition-rate LCLS-II X-ray free electron laser. The orders-of-magnitude X-ray flux improvement provided by the superconducting accelerator, combined with corresponding advances in the optical laser system and the liquid jet recirculation system, enables studies on dilute systems with high signal-to-noise compared to what was possible with the LCLS-I copper accelerator. These capabilities open up time-resolved X-ray absorption spectroscopy and RIXS to entirely new classes of samples, as well as enabling the development of new soft X-ray spectroscopic methods on liquid samples. An overview of the beamline components and the first LCLS-II commissioning results are presented.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

FEL2026 - 42nd International Free Electron Laser Conference - Prepress

On behalf of the International Executive Committee of the FEL Conference series, we are pleased to announce the 42nd International Free Electron Laser Conference (FEL2026). The conference will be held at Li Ka Shing Center located on Stanford campus from August 23rd to August 28th, 2026. FEL2026 will focus on recent advances in free electron laser theory and experiments, electron beam, photon beam and undulator technologies, and applications of free electron lasers. FEL2026 will be hosted by SLAC National Accelerator Laboratory and Stanford PULSE Institute. Stanford is the birthplace of the free-electron laser. SLAC houses two premier X-ray FEL facilities (LCLS and LCLS‑II) in the US. The conference program will include an optional tour of the LCLS and LCLS-II. Stay tuned for more conference information by following this official conference website (www.fel2026.org). Email questions should be addressed to fel2026@slac.stanford.edu.

Summers, Tasha [SLAC National Accelerator Laborato↗

Demonstration of a diamond anvil cell platform at the Linac Coherent Light Source: capabilities and outlook

A novel X-ray free electron laser (XFEL) diffraction setup for use with diamond anvil cells (DACs) at the Linac Coherent Light Source (LCLS) is described. The new diamond window at the Matter at Extreme Conditions (MEC) instrument allows hard X-ray experiments on DACs to be performed in air. The platform is described along with alignment and calibration procedures, and details of the X-ray beam and diagnostics. Example data are presented, including a reversible XFEL-induced phase transition in CsPbI 3 . The DAC setup was commissioned at MEC, but is applicable to most LCLS instruments where the unique pulse structures available at LCLS offer access to new ultrafast experimental techniques at high pressure.

Linac Coherent Light Source (LCLS)↗

The DREAM Endstation at the Linac Coherent Light Source

Free-electron lasers (FEL), with their ultrashort pulses, ultrahigh intensities, and high repetition rates at short wavelength, have provided new approaches to Atomic and Molecular Optical Science. One such approach is following the birth of a photo electron to observe ion dynamics on an ultrafast timescale. Such an approach presents the opportunity to decipher the photon-initiated structural dynamics of an isolated atomic and molecular species. It is a fundamental step towards understanding single- and non-linear multi-photon processes and coherent electron dynamics in atoms and molecules, ultimately leading to coherent control following FEL research breakthroughs in pulse shaping and polarization control. A key aspect for exploring photoinduced quantum phenomena is visualizing the collective motion of electrons and nuclei in a single reaction process, as dynamics in atoms/ions proceed at femtosecond (10 –15 s) timescales while electronic dynamics take place in the attosecond timescale (10 –18 s). Here, we report on the design of a Dynamic Reaction Microscope (DREAM) endstation located at the second interaction point of the Time-Resolved Molecular and Optical (TMO) instrument at the Linac Coherent Light Source (LCLS) capable of following the photon–matter interactions by detecting ions and electrons in coincidence. The DREAM endstation takes advantage of the pulse properties and high repetition rate of LCLS-II to perform gas-phase soft X-ray experiments in a wide spectrum of scientific domains. With its design ability to detect multi-ions and electrons in coincidence while operating in step with the high repetition rate of LCLS-II, the DREAM endstation takes advantage of the inherent momentum conservation of reaction product ions with participating electrons to reconstruct the original X-ray photon–matter interactions. In this report, we outline in detail the design of the DREAM endstation and its functionality, with scientific opportunities enabled by this state-of-the-art instrument.

47 OTHER INSTRUMENTATION↗

Demonstration of a diamond anvil cell platform at the Linac Coherent Light Source: Capabilities and Outlook

A novel x-ray free electron laser (XFEL) diffraction setup for use with diamond anvil cells (DACs) at the Linac Coherent Light Source (LCLS) is described. Using the new diamond window at the Matter at Extreme Conditions (MEC) instrument, it allows hard x-ray experiments on DACs to be performed in air. The platform is described along with alignment and calibration procedures and details of the x-ray beam and diagnostics. Example data are presented, including a reversible XFEL induced phase transition in CsPbI3. The DAC setup was commissioned at MEC, but is applicable to most LCLS instruments where the unique pulse structures available at LCLS offer access to new ultrafast experimental techniques at high pressure.

Diamond Anvil Cells, LCLS, XFEL, High-Pressure↗

Real‐time XFEL data analysis at SLAC and NERSC: A trial run of nascent exascale experimental data analysis

X‐ray scattering experiments using free electron lasers (XFELs) are a powerful tool to determine the molecular structure and function of unknown samples (such as COVID‐19 viral proteins). XFEL experiments are a challenge to computing in two ways: (i) due to the high cost of running XFELs, a fast turnaround time from data acquisition to data analysis is essential to make informed decisions on experimental protocols; (ii) data‐collection rates are growing exponentially, requiring new scalable algorithms. Here we report our experiences analyzing data from two experiments at the Linac Coherent Light Source (LCLS) during September 2020. Raw data were analyzed on NERSC's Cori XC40 system, using the Superfacility paradigm: our workflow automatically moves raw data between LCLS and NERSC, where it is analyzed using the software package CCTBX. We achieved real time data analysis with a turnaround time from data acquisition to full molecular reconstruction in as little as 10 min—sufficient time for the experiment's operators to make informed decisions. By hosting the data analysis on Cori, and by automating LCLS‐NERSC interoperability, we achieved a data analysis rate which matches the data acquisition rate. Completing data analysis within 10 min is a first for XFEL experiments and an important milestone if we are to keep up with data‐collection trends.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Isolation, Characterization, and Depolymerization of L -Cysteine Substituted Eucalyptus Lignin

Lignin condensation reactions are hard to avoid or control during separation, which is a deterrent to lignin isolation and post-conversation, especially for the full utilization of lignocelluloses. Selective protection of β-aryl ether linkages in the isolation process is crucial to lignin valorization. Herein, a two-step acid/alkali separation method assisted with l-cysteine for eucalyptus lignin separation is developed, and the isolated L -cysteine lignins (LCLs) are comprehensively characterized by 2D NMR, 31 P NMR, thioacidolysis, etc. Compared to the two-step control treatment, a much higher β-O-4 content is preserved without reducing the separation efficiency assisted by L -cysteine, which is also significantly higher than alkali lignin and kraft lignin. The results of hydrogenolysis show that LCLs generate a much higher monomer yield than that of control sample. Structural analysis of LCLs suggests that lignin condensation reaction, to some extent, is suppressed by adding L -cysteine during the two-step acid/alkali separation. Further, mechanistic studies using dimeric model compound reveals that L -cysteine may be the α-carbon protective agent in the two-step separation. The role of L -cysteine in the two-step lignin isolation method provides novel insights to the selective fractionation of lignin from biomass, especially for the full valorization of lignocellulosic biomass.

09 BIOMASS FUELS↗

Coherent-Radiation Spectroscopy of Few-Femtosecond Electron Bunches Using a Middle-Infrared Prism Spectrometer

Modern, high-brightness electron beams such as those from plasma wakefield accelerators and free-electron laser linacs continue the drive to ever-shorter bunch durations. In low-charge operation ( ~ 20 pC ), bunches shorter than 10 fs are reported at the Linac Coherent Light Source (LCLS). Though suffering from a loss of phase information, spectral diagnostics remain appealing as compact, low-cost bunch duration monitors suitable for deployment in beam dynamics studies and operations instrumentation. Progress in middle-infrared (MIR) imaging has led to the development of a single-shot, MIR prism spectrometer to characterize the corresponding LCLS coherent beam radiation power spectrum for few-femtosecond scale bunch length monitoring. In this Letter, we report on the spectrometer installation as well as the temporal reconstruction of 3 to 60 fs-long LCLS electron bunch profiles using single-shot coherent transition radiation spectra.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The Macromolecular Femtosecond Crystallography Instrument at the Linac Coherent Light Source

The Macromolecular Femtosecond Crystallography (MFX) instrument at the Linac Coherent Light Source (LCLS) is the seventh and newest instrument at the world's first hard X-ray free-electron laser. It was designed with a primary focus on structural biology, employing the ultrafast pulses of X-rays from LCLS at atmospheric conditions to overcome radiation damage limitations in biological measurements. It is also capable of performing various time-resolved measurements. The MFX design consists of a versatile base system capable of supporting multiple methods, techniques and experimental endstations. The primary techniques supported are forward scattering and crystallography, with capabilities for various spectroscopic methods and time-resolved measurements. The location of the MFX instrument allows for utilization of multiplexing methods, increasing user access to LCLS by running multiple experiments simultaneously.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

A high-power, high-repetition-rate THz source for pump–probe experiments at Linac Coherent Light Source II

Experiments using a THz pump and an X-ray probe at an X-ray free-electron laser (XFEL) facility like the Linac Coherent Light Source II (LCLS II) require frequency-tunable (3 to 20 THz), narrow bandwidth (~10%), carrier-envelope-phase-stable THz pulses that produce high fields (>1 MV cm –1 ) at the repetition rate of the X-rays and are well synchronized with them. Herein, a two-bunch scheme to generate THz radiation at LCLS II is studied: the first bunch produces THz radiation in an electromagnet wiggler immediately following the LCLS II undulator that produces X-rays from the second bunch. The initial time delay between the two bunches is optimized to compensate for the path difference in THz transport. The two-bunch beam dynamics, the THz wiggler and radiation are described, as well as the transport system bringing the THz pulses from the wiggler to the experimental hall.

42 ENGINEERING↗

Development and calibration of mirrors and gratings for the Soft X-ray materials science beamline at the Linac Coherent Light Source free-electron laser

This article discusses the development and calibration of the x-ray reflective and diffractive elements for the Soft X-ray Materials Science (SXR) beamline of the Linac Coherent Light Source (LCLS) free-electron laser (FEL), designed for operation in the 500 – 2000 eV region. The surface topography of three Si mirror substrates and two Si diffraction grating substrates was examined by atomic force microscopy (AFM) and optical profilometry. The figure of the mirror substrates was also verified via surface slope measurements with a long trace profiler. A boron carbide (B 4 C) coating especially optimized for the LCLS FEL conditions was deposited on all SXR mirrors and gratings. Coating thickness uniformity of 0.14 nm root mean square (rms) across clear apertures extending to 205 mm length was demonstrated for all elements, as required to preserve the coherent wavefront of the LCLS source. The reflective performance of the mirrors and the diffraction efficiency of the gratings were calibrated at beamline 6.3.2 at the Advanced Light Source synchrotron. To verify the integrity of the nanometer-scale grating structure, the grating topography was examined by AFM before and after coating. This is to our knowledge the first time B 4 C-coated diffraction gratings are demonstrated for operation in the soft x-ray region.

36 MATERIALS SCIENCE↗

AN OSCILLATOR CONFIGURATION FOR FULL REALIZATION OF HARD X-RAY FREE ELECTRON LASER*

An x-ray free electron laser oscillator (XFELO) is feasible by employing an X-ray cavity with Bragg mirrors such as diamond crystals. An XFELO at the 5th harmonic frequency may be implemented at the LCLS II using its 4 GeV superconducting linac, producing stable, fully coherent, high-spectral-purity hard x-rays. In addition, its output can be a coherent seed to the LCLS amplifier for stable, high-power, femto-second x-ray pulses. We summarize the recent progress in various R&D efforts addressing critical issues for realizing an XFELO at LCLS II.

Kim, K. -J.↗

Undulator Radiation Generated by a Single Electron

The facilities providing single electron beams are currently being commissioned at Fermilab and will be at SLAC. Recently, Fermilab’s IOTA ring routinely demonstrated circulation of a single electron at 100 MeV beam energy. Alternatively, SLAC is working on constructing LCLS-II an X-ray FEL driven by a 4 GeV SRF linac. A parasitic beamline, S30XL, is planned that will extract 4 GeV dark current from between the primary LCLS-II electron bunches. The dark current will be delivered to End Station A and can work independently of LCLS-II experiments. The dark current will be bunched at a frequency of 46 MHz while extracted current varied from single electrons to 10’s of nA. In the present paper, we estimate the feasibility of propagating single electron beams through a conventional undulator, placed in the IOTA and S30XL beamlines. We explore the possible observable effects and experimental parameters range. In addition, we focus on potential applications of such beams in systems for high fidelity quantum measurements.

43 PARTICLE ACCELERATORS↗

Incident IR Bandwidth Effects on Efficiency and Shaping for Third Harmonic Generation of Quasi-Rectangular UV Longitudinal Profiles

The photocathode of the proposed LCLS RF Photoinjector will be irradiated by uv laser light which is generated as the third harmonic of incident fundamental ir laser light. We have investigated quantitatively the effect of input ir spectral bandwidth on the exiting longitudinal intensity profiles, energy conversion efficiencies and spectral bandwidths that characterize the third harmonic generation (THG) process with a pair of crystals. These profiles, efficiencies and bandwidths include the residual fundamental and residual second harmonic light exiting the second crystal. The intrinsic acceptance bandwidth for THG is determined by crystal material and thickness as well as the type of phase matching that is used. For our case of BBO material with type I phase matching these bandwidths are approximately 0.9 nm*cm and 0.1 nm*cm for second and third harmonic generation respectively. Consequently for fixed crystal thicknesses and a fixed input ir longitudinal profile, the specified input ir bandwidth will determine the profiles, efficiencies and bandwidths exiting the second crystal. The results reported here are predictions of the SNLO code that is available as 'freeware' from the Sandia National Laboratories. It has been modified for this work. It is critical to note that this modification has enabled us to generate SNLO predictions of the 'coupled' case in which the output of the first crystal is used as input to the second crystal. Our focus is the dependence of uv longitudinal intensity profile and THG efficiency on the input ir bandwidth and crystal thicknesses. We include here cases that best illustrate input bandwidth effects. The criteria for selection of reported cases are highest efficiency generation of quasi-rectangular uv profiles with proportional intensity ripple less than 5% rms on the plateau of the pulse. Maximizing THG efficiency typically amounts to maximizing the crystal thicknesses with the longitudinal profile constraint. The specified incident ir longitudinal profile is quasi-rectangular (i.e. nonzero risetime and falltime with small intensity variation on the plateau) with a 10 psec pulse duration (FWHM). By assumption, this profile has been established upstream of the crystals at the fundamental ir wavelength. The simplest possible optical configuration is used in this work as shown in figure 1. The first crystal is the site of second harmonic generation (SHG) driven by the incident ir irradiation of central wavelength, 800nm. Downstream of the first crystal, the second crystal is the site of third harmonic generation (THG) which occurs by sum frequency mixing. Inter-crystal optics (such as a half waveplate) are assumed to be lossless at the fundamental and second harmonic wavelengths. As shown in figure 1, a portion of the incident ir irradiation is not sequestered from the first crystal for subsequent THG in the second crystal. Also, quasi-phase matching configurations and other complex compensation schemes have not been investigated at this point. The simplistic geometry better elucidates the intrinsic acceptance bandwidth limitations imposed by the crystals. Our goal in this endeavor has been to conduct a quantitative assessment of incident ir bandwidth effects on the THG process for BBO material of varied thicknesses and not, at this stage, to comply with all uv pulse specifications for the LCLS RF Photoinjector. Nonetheless, our results can be compared with LCLS photoinjector uv pulse requirements which call for a nominal 10 psec FWHM with 1 psec risetime and falltime and a nominally flat plateau (allowing for slope adjustments) with no more than a 5% rms proportional intensity variation. Furthermore, the results of this work can be used to suggest crystal thicknesses that would likely comply with all uv pulse requirements given the appropriate longitudinal profile and bandwidth for an input ir pulse.

43 PARTICLE ACCELERATORS↗

Optical tailoring of xFEL beams

There is an inherent flexibility unique to free electron lasers (FELs) that lends well to experimental approaches normally too difficult for other light sources to accomplish. This includes the ability to optically shape the electron bunch prior to final its acceleration for the final FEL process. Optical pulse shaping of the electron bunch can enable both femtosecond and attosecond level FEL pulse control. Pulse shaping is currently implemented, not optically but mechanically, in LCLS-I with an adjustable foil slit that physically spoils the momentum phase of the electron bunch. This selectively suppresses the downstream FEL process of spoiled electrons. Such a mechanical spoiling method fails for both the soft x-ray regime as well as the high repetition rates that are planned in LCLS-II. Our proposed optical spoiling method circumvents this limitation by making use of the existing ultrafast laser beam that is typically used for adjusting the energy spread for the initial electron bunch. Using Fourier domain shaping we can nearly arbitrarily shape the laser pulses to affect the electron bunch. This can selectively spoil electrons within each bunch. Here we demonstrate the viability of this approach with a programmable acousto-optic dispersive filter. This method is not only well suited for LCLS-II but also has several advantages over mechanical spoiling, including lack of radiation concerns, experiment specific FEL pulse shapes, and real-time adjustment for applications that require high duty-cycle variation such as lock-in amplification of small signals.

43 PARTICLE ACCELERATORS↗