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Chain Dynamics in Magnetorheological Suspensions

Magnetorheological (MR) suspensions are composed of colloidal particles which acquire dipole moments when subjected to an external magnetic field. At sufficient field strengths and concentrations, the dipolar particles rapidly aggregate to form long chains. Subsequent lateral cross-linking of the dipolar chains is responsible for a rapid liquid-to-solid-like rheological transition. The unique, magnetically-activated rheological properties of MR suspensions make them ideal for interfacing mechanical systems to electronic controls. Additionally, the ability to experimentally probe colloidal suspensions interacting through tunable anisotropic potentials is of fundamental interest. Our current experimental work has focused on understanding the fluctuations of dipolar chains. It has been proposed by Halsey and Toor (HT) that the strong Landau-Peierls thermal fluctuations of dipolar chains could be responsible for long-range attractions between chains. Such interactions will govern the long-time relaxation of MR suspensions. We have synthesized monodisperse neutrally buoyant MR suspensions by density matching stabilized ferrofluid emulsion droplets with D2O. This allows us to probe the dynamics of the dipolar chains using light scattering without gravitational, interfacial, and polydispersity effects to resolve the short-wavelength dynamics of the dipolar chains. We used diffusing wave spectroscopy to measure these dynamics. The particle displacements at short times that show an independence to the field strength, but at long times exhibit a constrained, sub-diffusive motion that slows as the dipole strength is increased. The experiments are in good qualitative agreement with Brownian dynamics simulations of dipolar chains. Although there have been several important and detailed studies of the structure and interactions in MR suspensions, there has not been conclusive evidence that supports or contradicts the HT model prediction that long-range interactions exist between fluctuating chains of dipolar particles. Resolving this issue would contribute greatly to the understanding of these interesting and important materials. We have begun to test the predictions of the HT model by both examining the dynamics of individual chains and by measuring the forces between dipolar chains directly to accurately and quantitatively assess the interactions that they experience. To do so, we employ optical trapping techniques and video-microscopy to manipulate and observe our samples on the microscopic level. With these techniques, it is possible to observe chains that are fluctuating freely in three-dimensions, independent of interfacial effects. More importantly, we are able to controllably observe the interactions of two chains at various separations to measure the force-distance profile. The techniques also allow us to study the mechanical properties of individual chains and chain clusters. Our work to this point has focused on reversibly-formed dipolar chains due to field induced dipoles where the combination of this chaining, the dipolar forces, and the hydrodynamic interactions that dictate the rheology of the suspensions. One can envision, however, many situations where optical, electronic, or rheological behavior may be optimized with magneto-responsive anisotropic particles. Chains of polarizable particles may have the best properties as they can coil and flex in the absence of a field and stiffen and orient when a field is applied. We have recently demonstrated a synthesis of stable, permanent paramagnetic chains by both covalently and physically linking paramagnetic colloidal particles. The method employed allows us to create monodisperse chains of controlled length. We observed the stability, field-alignment, and rigidity of this new class of materials. The chains may exhibit unique rheological properties in an applied magnetic field over isotropic suspensions of paramagnetic particles. They are also useful rheological models as bead-spring systems. These chains form the basis for our current experiments with optical traps.

Gast, A. P.↗

Linear Polarization Measurements of Chromospheric Emission Lines

We have used the Zurich Imaging Stokes Polarimeter (ZIMPOL I) with the McMath-Pierce 1.5 m main telescope on Kitt Peak to obtain linear polarization measurements of the off-limb chromosphere with a sensitivity better than 1 x 10(exp -5). We found that the off-disk observations require a combination of good seeing (to show the emission lines) and a clean heliostat (to avoid contamination by scattered light from the Sun's disk). When these conditions were met, we obtained the following principal results: 1. Sometimes self-reversed emission lines of neutral and singly ionized metals showed linear polarization caused by the transverse Zeeman effect or by instrumental cross talk from the longitudinal Zeeman effect in chromospheric magnetic fields. Otherwise, these lines tended to depolarize the scattered continuum radiation by amounts that ranged up to 0.2%. 2. Lines previously known to show scattering polarization just inside the limb (such as the Na I lambda5889 D2 and the He I lambda5876 D3 lines) showed even more polarization above the Sun's limb, with values approaching 0.7%. 3. The O I triplet at lambda7772, lambda7774, and lambda7775 showed a range of polarizations. The lambda7775 line, whose maximum intrinsic polarizability, P(sub max), is less than 1%, revealed mainly Zeeman contributions from chromospheric magnetic fields. However, the more sensitive lambda7772 (P(sub max) = 19%) and lambda7774 (P(sub max) = 29%) lines had relatively strong scattering polarizations of approximately 0.3% in addition to their Zeeman polarizations. At times of good seeing, the polarization spectra resolve into fine structures that seem to be chromospheric spicules.

Sheeley, N. R., Jr.↗

Spatially-and Temporally-Resolved Multi-Parameter Interferometric Rayleigh Scattering System and Method

A system that simultaneously measures the translational temperature, bulk velocity, and density in gases by collecting, referencing, and analyzing nanosecond time-scale Rayleigh scattered light from molecules is described. A narrow-band pulsed laser source is used to probe two largely separated measurement locations, one of which is used for reference. The elastically scattered photons containing information from both measurement locations are collected at the same time and analyzed spectrally using a planar Fabry-Perot interferometer. A practical means of referencing the measurement of velocity using the laser frequency, and the density and temperature using the information from the reference measurement location maintained at constant properties is provided.

Bivolaru, Daniel↗

An ASCA observation of the Seyfert 2 galaxy Markarian 3

We report preliminary results of an ASCA observation of the Seyfert 2 galaxy Markarian 3 (Mkn 3). Comparison with previous Ginga and Broad-Band X-ray Telescope (BBXRT) observations shows that the observed hard X-ray luminosity above 4 keV decreased by a factor of approximately 3 (intrinsic luminosity by almost a factor of 6) in a period of approximately 3.6 yr. On the other hand, the soft luminosity has not varied significantly in approximately 13 yr, lending support to the extended nature of the soft emission, perhaps dominated by scattering of the nuclear X-rays. ASCA resolves the Fe K line emission into at least two components for the first time. The dominant component at 6.4 keV has an equivalent width of approximately 860 eV and full width at half maximum (FWHM) approximately equals 10(exp 4) km/sec, while the second component has an equivalent width of approximately 190 eV and appears to be narrower than the first. The total intensity of the Fe K emission decreased by factor of over 3 in response to the decrease in the continuum level, implying that a substantial part of the dominant Fe K emission must originate in a region smaller than that responsible for the soft emission. The variability provides direct evidence that the hard X-ray continuum and Fe K line in this Seyfert 2 are being observed directly through the nuclear obscuring material, not in scattered light.

Iwasawa, Kazushi↗

Possible Detection of an Emission Cyclotron Resonance Scattering Feature from the Accretion-Powered Pulsar 4U 1626-67

We present analysis of 4U 1626-67, a 7.7 s pulsar in a low-mass X-ray binary system, observed with the hard X-ray detector of the Japanese X-ray satellite Suzaku in 2006 March for a net exposure of ~88 ks. The source was detected at an average 10-60 keY flux of approx 4 x 10-10 erg / sq cm/ s. The phase-averaged spectrum is reproduced well by combining a negative and positive power-law times exponential cutoff (NPEX) model modified at approx 37 keY by a cyclotron resonance scattering feature (CRSF). The phase-resolved analysis shows that the spectra at the bright phases are well fit by the NPEX with CRSF model. On the other hand. the spectrum in the dim phase lacks the NPEX high-energy cutoff component, and the CRSF can be reproduced by either an emission or an absorption profile. When fitting the dim phase spectrum with the NPEX plus Gaussian model. we find that the feature is better described in terms of an emission rather than an absorption profile. The statistical significance of this result, evaluated by means of an F test, is between 2.91 x 10(exp -3) and 1.53 x 10(exp -5), taking into account the systematic errors in the background evaluation of HXD-PIN. We find that the emission profile is more feasible than the absorption one for comparing the physical parameters in other phases. Therefore, we have possibly detected an emission line at the cyclotron resonance energy in the dim phase.

Iwakiri, W. B.↗

The X-ray Halo of GX5-1

Using Chandra observations we have measured the energy-resolved dust-scattered X-ray halo around the low-mass X-ray binary GX5-1, detecting for the first time multiply scattered X-rays from interstellar dust. % e compared the observed X-ray halo at various energies to predictions from a range of dust models. These fits used both smoothly-distributed dust as well as dust in clumped clouds, with CO and 21 cm observations helping to determine the position of the clouds along the line of sight. We found that the BARE-GR-B model of Zubko, Dwek & Arendt (2004) generally led to the best results, although inadequacies in both the overall model and the data limit our conclusions. We did find that the composite dust models of Zubko, Dwek & Arendt (2004), especially the "no carbon" models, gave uniformly poor results. Although models using cloud positions and densities derived naively from CO and 21 cm data gave generally poor results, plausible adjustments to the distance of the largest cloud and the mass of a cloud in the expanding 3 kpc Arm lead to significantly improved fits. We suggest that combining X-ray halo, CO, and 21 cm observations will be a fruitful method to improve our understanding of both the gas and dust phases of the interstellar medium.

Smith, Randall K.↗

Thermodynamic measurements in a high pressure hydrogen-oxygen flame using Raman scattering from a broadband excimer laser

Raman scattering is an inelastic molecular scattering process in which incident radiation is reemitted at a fixed change in frequency. Raman spectroscopy can be used to measure the number density and temperature of the irradiated species. The strength of the Raman signal is inversely proportional to the wavelength raised to the fourth power. Consequently, high signal to noise ratios are obtained by using ultraviolet (UV) excitation sources. Using UV sources for Raman Spectroscopy in flames is complicated by the fact that some of the primary constituents in hydrogen-oxygen combustion absorb and reemit light in the UV and these fluorescence processes interfere with the Raman signals. This problem has been handled in atmospheric pressure flames in some instances by using a narrowband tunable excimer laser as a source. This allows for detuning from absorption transitions and the elimination of interfering fluorescence signals at the Raman wavelengths. This approach works well in the atmospheric pressure flame; however, it has two important disadvantages. First, injection-locked narrowband tunable excimer lasers are very expensive. More importantly, however, is the fact that at the high pressures characteristic of rocket engine combustion chambers, the absorption transitions are broadened making it difficult to tune to a spectral location at which substantial absorption would not occur. The approach taken in this work is to separate the Raman signal from the fluorescence background by taking advantage of the fact that Raman signal has nonisotropic polarization characteristics while the fluorescence signals are unpolarized. Specifically, for scattering at right angles to the excitation beam path, the Raman signal is completely polarized. The Raman signal is separated from the fluorescence background by collecting both horizontally and vertically polarized signals separately. One of the polarizations has both the Raman signal and the fluorescence background while the other has only the fluorescence signal. The Raman scatter is the difference between the signals. By choosing an appropriate optical setup, both signals can be obtained simultaneously with the same monochromator; hence, time resolved measurements are possible using this approach.

Hartfield, Roy, Jr.↗

HST/ACS Coronagraphic Observations of the HD 163296 Circumstellar Disk: Evidence of Time-Variable Self-Shadowing?

We present Hubble Space Telescope Advanced Camera for Surveys (HST/ACS) coronagraphic observations of the Herbig Ae star HD 163296. HD 163296's scattered light disk was resolved in the F606W and F814W filters in observations obtained In 2003 and in the F435W filter in observations obtained in 2004. Analysis of single-epoch data indicates that the disk (V-I) color is redder than the observed stellar (V-I) color. This spatially uniform red disk color might be indicative of either an evolution in the grain size distribution (i.e. grain growth) and/or composition. Both of these processes would be consistent with the observed flat geometry of the outer disk, as diagnosed by the observed r$(exp -3)$ power law behavior of its median azimuthally averaged disk surface brightness, which suggest that grain evolution is occurring. Comparison of ACS and STIS epoch scattered light data reveals differences in the observed disk surface brightnesses, of order 1 mag arcsec$(exp -2)$, in both V and white-light filter bandpasses. Along with the observed variability in the visibility and surface brightness of the ansa(e) in the disk, and spectropolarimetric variability of the system, these results suggest that the resolved scattered light disk is variable, a phenomenon not previously observed in any other Herbig protoplanetary system We speculate that the observed behavior might be attributable to the variable inflation of the scale height of the inner disk wall, which results in variable self-shadowing of the outer disk.

Wisniewski, J.↗

Optical Coronagraphic Spectroscopy of AU Mic: Evidence of Time Variable Colors?

We present coronagraphic long slit spectra of AU Mic's debris disk taken with the STIS instrument aboard the Hubble Space Telescope. Our spectra are the first spatially-resolved, scattered light spectra of the system's disk, which we detect at projected distances between approximately 10 and 45 au. Our spectra cover a wavelength range between 5200 and 10200 Angstrom. We find that the color of AU Mic's debris disk is bluest at small (12-17 au) projected separations. These results both confirm and quantify the findings qualitatively noted by Krist et al. and are different than IR observations that suggested a uniform blue or gray color as a function of projected separation in this region of the disk. Unlike previous literature, which reported that the color of AU Mic's disk became increasingly more blue as a function of projected separation beyond approx. 30 au, we find the disk's optical color between 35 and 45 au to be uniformly blue on the southeast side of the disk and decreasingly blue on the northwest side. We note that this apparent change in disk color at larger projected separations coincides with several fast, outward moving ''features'' that are passing through this region of the southeast side of the disk. We speculate that these phenomenon might be related and that the fast moving features could be changing the localized distribution of sub-micron-sized grains as they pass by, thereby reducing the blue color of the disk in the process. We encourage follow-up optical spectroscopic observations of AU Mic to both confirm this result and search for further modifications of the disk color caused by additional fast moving features propagating through the disk.

Lomax, Jamie R.↗

VLBI observations of the Crab nebula pulsar

Observations were made at meter wave-lengths using very long base-line interferometry techniques. At 196.5 MHz no resolution of the pulsar are observed; all the pulse shapes observed with the interferometers are similar to single dish profiles, and all the power pulsates. At 111.5 MHz besides the pulsing power there is always a steady component, presumably due to interstellar scattering. The pulsar is slightly resolved at 111.5 MHz with an apparent angular diameter of 0.07 sec ? 0.01 sec. A 50 percent linear polarization of the time-averaged power is noted at 196.5 MHz; at 111.5 MHz, 20 percent of the total time-averaged power is polarized, 35 percent of the pulsing power is polarized, and the steady component is unpolarized.

Vandenberg, N. R.↗

Introductory remarks: Photometry section

The principal goals of photometry and polarimetry are summarized. These goals include studies of the emission features of gaseous species of comets, the wavelength depenence of albedo, the phase function of scatter distribution, and time variation of rotation. Recent advances in photometric techniques were reviewed and include: use of proper filters, extension to the shortest and longest wavelengths, higher spectral resolving power, and polarizaton techniques.

Ahearn, M. F.↗

Aircraft laser sensing of sound velocity in water - Brillouin scattering

A real-time data source for sound speed in the upper 100 m has been proposed for exploratory development. This data source is planned to be generated via a ship- or aircraft-mounted optical pulsed laser using the spontaneous Brillouin scattering technique. The system should be capable (from a single 10 ns 500 mJ pulse) of yielding range resolved sound speed profiles in water to depths of 75-100 m to an accuracy of 1 m/s. The 100 m profiles will provide the capability of rapidly monitoring the upper-ocean vertical structure. They will also provide an extensive, subsurface-data source for existing real-time, operational ocean nowcast/forecast systems.

Hickman, G. D.↗

Active Neutron and Gamma-Ray Instrumentation for In Situ Planetary Science Applications

We describe the development of an instrument capable of detailed in situ bulk geochemical analysis of the surface of planets, moons, asteroids, and comets. This instrument technology uses a pulsed neutron generator to excite the solid materials of a planet and measures the resulting neutron and gamma-ray emission with its detector system. These time-resolved neutron and gamma-ray data provide detailed information about the bulk elemental composition, chemical context, and density distribution of the soil within 50 cm of the surface. While active neutron scattering and neutron-induced gamma-ray techniques have been used extensively for terrestrial nuclear well logging applications, our goal is to apply these techniques to surface instruments for use on any solid solar system body. As described, experiments at NASA Goddard Space Flight Center use a prototype neutron-induced gamma-ray instrument and the resulting data presented show the promise of this technique for becoming a versatile, robust, workhorse technology for planetary science, and exploration of any of the solid bodies in the solar system. The detection of neutrons at the surface also provides useful information about the material. This paper focuses on the data provided by the gamma-ray detector.

Parsons, A.↗

Nd:YAG Laser-Based Dual-Line Detection Rayleigh Scattering and Current Efforts on UV, Filtered Rayleigh Scattering

Ongoing research in Rayleigh scattering diagnostics for variable density low speed flow applications and for supersonic flow measurements are described. During the past several years, the focus has been on the development and use of a Nd:YAG-based Rayleigh scattering system with improved signal-to-noise characteristics and with applicability to complex, confined flows. This activity serves other research projects in the Aerodynamics Laboratory which require the non-contact, accurate, time-frozen measurement of gas density, pressure, and temperature (each separately), in a fairly wide dynamic range of each parameter. Recently, with the acquisition of a new seed-injected Nd:YAG laser, effort also has been directed to the development of a high-speed velocity probe based on a spectrally resolved Rayleigh scattering technique.

Otugen, M. Volkan↗

Atomic collisions in the presence of laser radiation - Time dependence and the asymptotic wave function

A time-dependent, wave-packet description of atomic collisions in the presence of laser radiation is extracted from the more conventional time-independent, stationary-state description. This approach resolves certain difficulties of interpretation in the time-independent approach which arise in the case of asymptotic near resonance. In the two-state model investigated, the approach predicts the existence of three spherically scattered waves in this asymptotically near-resonant case.

Devries, P. L.↗

DC-8 scanning lidar characterization of aircraft contrails and cirrus clouds

A Subsonic Assessment (SASS) element of the overall Atmospheric Effects of Aviation Project (AEAP) was initiated by NASA to assess the atmospheric impact of subsonic aircraft. SRI was awarded a project to develop and test a scanning backscatter lidar for installation on the NASA DC-8 (year 1), participate in the Subsonic Aircraft: Contrail and Cloud Effects Special Study (SUCCESS) field program (year 2), and conduct a comprehensive analysis of field data (year 3). A scanning mirror pod attached to the DC-8 aircraft provides for scanning lidar observations ahead of the DC-8 and fixed-angle upward or downward observations. The lidar system installed within the DC-8 transmits 275 MJ at 1.06 gm wavelength or about 130 mJ at 1.06 and 0.53 gm simultaneously. Range-resolved aerosol backscatter is displayed in real time in terms of cloud/contrail spatial distributions. The objectives of the project are to map contrail/cloud vertical distributions ahead of DC-8; provide DC-8 guidance into enhanced scattering layers; document DC-8 flight path intersection of contrail and cloud geometries (in-situ measurement positions relative to cloud/contrail shape and an extension of in-situ measurements into the vertical -- integrated contrail/cloud properties); analyze contrail/cloud radiative properties with LIRAD (combined lidar and radiometry) technique; evaluate mean particle sizes of aircraft emissions from two-wavelength observations; study contrail/cloud interactions, diffusion, and mass decay/growth; and make observations in the near-field of aircraft engine emissions. The scanning mirror pod may also provide a scanning capability for other remote sensing instruments.

Nielsen, Norman B.↗

Time resolved density measurements in premixed turbulent flames

Premixed, turbulent flames are important in connection with investigations of fundamental, turbulent-reacting-flow processes and the study of practical combustion devices, such as spark ignition engines and premixed, prevaporized gas turbine combustors which burn premixed reactants. The considered investigation is concerned with the application of laser induced Rayleigh scattering to measure the gas density in premixed, methane-air flames. A description is provided of the results of density and velocity measurements in an open, lean, premixed methane-air flame stabilized in grid turbulence of low Reynolds number. It is found that where applicable, Rayleigh scattering can be used to good advantage to measure molecular number density. Mean and rms density results show that the mean flame thickens with axial distance but that the maximum in rms does not change appreciably.

Dandekar, K. V.↗

Multi-epoch Direct Imaging and Time-variable Scattered Light Morphology of the HD 163296 Protoplanetary Disk

We present H-band polarized scattered light imagery and JHK high-contrast spectroscopy of the protoplanetary disk around HD 163296 observed with the High-Contrast Coronographic Imager for Adaptive Optics (HiCIAO) and Subaru Coronagraphic Extreme Adaptive Optics (SCExAO)/Coronagraphic High Angular Resolution Imaging Spectrograph (CHARIS) instruments at Subaru Observatory. The polarimetric imagery resolve a broken ring structure surrounding HD 163296 that peaks at a distance along the major axis of 0 65 (66 au) and extends out to 0 98 (100 au) along the major axis. Our 2011 H-band data exhibit clear axisymmetry, with the NW and SE side of the disk exhibiting similar intensities. Our data are clearly different from 2016 epoch H-band observations of the Very Large Telescope (VLT)/Spectro-Polarimetric High-contrast Exoplanet REsearch (SPHERE), which found a strong 2.7 x asymmetry between the NW and SE side of the disk. Collectively, these results indicate the presence of time-variable, non-azimuthally symmetric illumination of the outer disk. While our SCExAO/CHARIS data are sensitive enough to recover the planet candidate identified from NIRC2 in the thermal infrared (IR), we fail to detect an object with JHK brightness nominally consistent with this object. This suggests that the candidate is either fainter in JHK bands than model predictions, possibly due to extinction from the disk or atmospheric dust/ clouds, or that it is an artifact of the data set/data processing, such as a residual speckle or partially subtracted disk feature. Assuming standard hot-start evolutionary models and a system age of 5Myr, we set new, direct mass limits for the inner (outer) Atacama Large Millimeter/submillimeter Array (ALMA)-predicted protoplanet candidate along the major (minor) disk axis of of 1.5 (2) M(J).

Evan A. Rich↗