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All sourcesNASA NTRSDOE OSTI
NASA NTRS1986

Production of radionuclides in artificial meteorites irradiated isotropically with 600 MeV protons

The understanding of the production of cosmogenic nuclides in small meteorites (R is less than 40 cm) still is not satisfactory. The existing models for the calculation of depth dependent production rates do not distinguish between the different types of nucleons reacting in a meteorite. They rather use general depth dependent particle fluxes to which cross sections have to be adjusted to fit the measured radionuclide concentrations. Some of these models can not even be extended to zero meteorite sizes without logical contradictions. Therefore, a series of three thick target irradiations was started at the 600 MeV proton beam of the CERN isochronuous cyclotron in order to study the interactions of small stony meteorites with galactic protons. The homogeneous 4 pi irradiation technique used provides a realistic meteorite model which allows a direct comparison of the measured depth profiles with those in real meteorites. Moreover, by the simultaneous measurement of thin target production cross sections one can differentiate between the contributions of primary and secondary nucleons over the entire volume of the artificial meteorite.

Michel, R.↗
NASA NTRS1986

Compilation of cosmogenic radionuclides in meteorites

All available data for the concentration of cosmogenic nuclides Mn-53(t(1/2) = 3.7 x 10(6) years), Al-26 (7.05 x 10(5) years), Be-10 (1.6 x 10(6) years), Cl-36 (3.0 x 10(5) years) and Ne-21, and Ne-22/Ne-21 ratios in stony, iron, and stony-iron meteorites were compiled. For iron meteorites, the He-4/Ne-21 ratio was adopted instead of Ne-22/Ne-21 ratio, because the He-4/Ne-21 ratio in iron meteorites indicates the shielding condition of the sample. The compilation contains over 2000 different analyses for four cosmogenic radionuclides.

Nishiizumi, K.↗
NASA NTRS1986

Cosmogenic radionuclides and noble gases in the Wethersfield (1982) chondrite

The Wethersfield (1982) chondrite was assayed for a suite of cosmogenic radionuclides shortly after fall. Data are reported for Be-7, Na-22, All-26, Sc-46, V-48, Cr-51, Mn-54, Co-56, Co-57, and Co-60. A comparison is made with predicted results based on a scaling to the Deep River Neutron Monitor. Noble gases were also assayed in a subsample. The cosmic-ray-exposure age is estimated to be 45 Myr.

Evans, J. C.↗
NASA NTRS1991

The interactions of atmospheric cosmogenic radionuclides with spacecraft surfaces

The discovery of the cosmogenic radionuclide Be-7 on the front surface of the Long Duration Exposure Facility (LDEF) has opened new opportunities to study several unexplored regions of space science. The experiments have shown that the Be-7 found was concentrated in a thin surface layer of spacecraft material. The only reasonable source of the isotope is the atmosphere through which the spacecraft passed. It is expected that the uptake of Be in such circumstances will depend on the chemical form of the Be and the chemical nature of the substrate. It was found that the observed concentration of Be-7 does differ between metal surfaces and organic surfaces such as PTFE (Teflon). It is noted however, that (1) organic surfaces are etched by the atomic oxygen found under these orbital conditions, and (2) the relative velocity of the species is 8 km/s relative to the surface and the interaction chemistry and physics may differ from the norm. Be-7 is formed by disintegration of O and N nuclei under cosmic ray proton bombardment. Many other isotopes are produced by cosmic ray reactions, and some of these are suited to measurement by the extremely sensitive methods of accelerator mass spectrometry.

Gregory, John C.↗
NASA NTRS1991

The interactions of atmospheric cosmogenic radionuclides with spacecraft surfaces

The discovery of the cosmogenic radionuclide Be-7 on the front surface (and the front surface only) of the Long Duration Exposure Facility (LDEF) spacecraft has opened opportunities to investigate new phenomena in several disciplines of space science. The experiments performed for this work show that the Be-7 results only if the source of the isotope is the atmosphere through which the spacecraft passed. We should expect that the uptake of beryllium in such circumstances will depend on the chemical form of the Be and the chemical nature of the substrate. It was found that the observed concentration of Be-7 does, in fact, differ between metal surfaces and organic surfaces such as PTFE (teflon). It is noted, however, that: (1) organic surfaces, even PTFE, are etched by the atomic oxygen found under these orbital conditions, and (2) the relative velocity of the species is 8 km(exp -1)s relative to the surface and the interaction chemistry and physics may differ from the norm. The Be-7 is formed by spallation of O and N nuclei under cosmic ray proton bombardment. The principal source region is at altitudes of 12-15 km. While very small quantities are produced above 300 km, the amount measured on the LDEF was 3 to 4 orders of magnitude higher than expected from production at orbital attitude. The most reasonable explanation is that Be-7 is rapidly transported from low altitudes by some unknown mechanism. The process must take place on a time scale similar to the half-life of the isotope (53 days). Many other isotopes are produced by cosmic ray reactions, and some of these are suited to measurement by the extremely sensitive methods of accelerator mass spectrometry. A program was initiated to search for these isotopes and it is hoped that such studies will provide new methods for studying mixing in the upper atmosphere.

Gregory, John C.↗
NASA NTRS1992

The interactions of atmospheric cosmogenic radionuclides with spacecraft surfaces

The discovery of the cosmogenic radionuclide Be-7 on the front surface of the Long Duration Exposure Facility (LDEF) spacecraft has opened opportunities to investigate new phenomena in several disciplines of space science. The experiments performed for this work show that the Be-7 results only if the source of the isotope is the atmosphere through which the spacecraft passed. We should expect that the uptake of beryllium in such circumstances will depend on the chemical form of the Be and the chemical nature of the substrate. It was found that the observed concentration of Be-7 does, in fact, differ between metal surfaces and organic surfaces such as PTFE (teflon). It is noted, however, that: (1) organic surfaces, even PTFE, are etched by the atomic oxygen found under these orbital conditions, and (2) the relative velocity of the species is 8 km(exp -1)s relative to the surface and the interaction chemistry and physics may differ from the norm. The Be-7 is formed by spallation of O and N nuclei under cosmic ray proton bombardment. The principal source region is at altitudes of 12-15 km. While very small quantities are produced above 300 km, the amount measured on the LDEF was 3 to 4 orders of magnitude higher than expected from production at orbital altitude. The most reasonable explanation is that Be-7 is rapidly transported from low altitudes by some unknown mechanism. The process must take place on a time scale similar to the half-life of the isotope (53 days). Many other isotopes are produced by cosmic ray reactions, and some of these are suited to measurement by the extremely sensitive methods of accelerator mass spectrometry. A program was initiated to search for these isotopes and it is hoped that such studies will provide new methods for studying mixing in the upper atmosphere.

Gregory, J. C.↗
NASA NTRS1993

Cosmogenic radionuclides on LDEF: An unexpected Be-10 result

Following the discovery of the atmospheric derived cosmogenic radionuclide Be-7 on the Long Duration Exposure Facility (LDEF), a search began for other known nuclides produced by similar mechanisms. None of the others have the narrow gamma-ray line emission of Be-7 decay which enabled its rapid detection and quantification. A search for Be-10 atoms on LDEF clamp plates using accelerator mass spectrometry is described. An unexpected result was obtained.

Gregory, J. C.↗
NASA NTRS1994

Use of radon and cosmogenic radionuclides as indicators of exchange between troposphere and stratosphere

This research grant covered participation in the operational phase of NASA's Stratosphere-Troposphere Exchange Project (STEP), a multi-agency airborne science program conducted aboard NASA U-2 and ER-2 high altitude research aircraft. The primary goals of STEP were to investigate the mechanisms of irreversible movement of mass, trace gases, and aerosols from the troposphere into the stratosphere, and to explain the observed dryness of the stratosphere. Three flight experiments were conducted to address these questions: two extratropical experiments, in 1984 and 1986, and a tropical experiment, in 1987. The cosmogenic radionuclides Be-7 and P-32, produced in the stratosphere by cosmic rays, and Rn-222 (radon), emitted from continental soils, were well-suited as tracers of intra-stratospheric air mass movements, and to follow episodes of troposphere to stratosphere exchange. Measurements of Be-7 and P-32 were made in all three STEP experiments. Measurements of radon were made in the tropical experiment only. The equipment worked well, and produced a valuable data set in support of the STEP objectives, as indicated by the 'quick-look' results outlined.

Kritz, Mark A.↗
NASA NTRS1999

Cosmogenic Radionuclides in Hot Desert Chondrites with Low C-14 Activities: A Progress Report

Terrestrial ages of meteorites from hot deserts provide an important tool to estimate meteorite fluxes to the Earth. Most desert meteorites have terrestrial ages less than 40 ky, but a few achondrites from the Sahara region were recently shown to have significantly higher ages, up to approx. 100 ky. In general, C-14 (half-life = 5730 y) is the most suited radionuclide to determine terrestrial ages for desert meteorites. However for meteorites with ages greater than 35 ky, the concentration of cosmogenic C-14 has decreased to a level at which it becomes difficult to distinguish between cosmogenic C-14 and terrestrial contamination. These meteorites may therefore be much older than 35 ky. We selected chondrites with low C-14 activities (less than or equal to 2 dpm/kg) for measurements of the concentrations of cosmogenic Cl-36 (half-life= 3.01 x 10 (exp 5) y) and Ca-41 (half-life= 1.04 x 10 (exp 5) y) in the metal phase. Since the ratio of Ca-14/Cl-36 in the metal phase of chondrites is relatively constant and well known, the measured ratio is a direct measure of the terrestrial age. A major problem is that most or sometimes all of the metal in these old "hot desert" meteorites has been oxidized to hydrated Fe-Ni-oxides. Therefore, we also measured the concentrations of Be-10, Al-26 and Cl-36 in the stony phase in order to constrain the terrestrial age as much as possible.

Welten, Kees↗
NASA NTRS2000

Cosmogenic Radionuclides in Hot Desert Chondrites With Low C-14 Activities

Terrestrial ages of meteorites from hot deserts provide an important tool to estimate meteorite fluxes to the Earth. Most desert meteorites have terrestrial ages less than 40 ky, but a few achondrites from the Sahara region were recently shown to have significantly higher ages, up to approx.100 ky. In general, C-14 (half-life = 5730 y) is the most suited radionuclide to determine terrestrial ages for desert meteorites. However for meteorites with ages >35 ky, the concentration of cosmogenic C-14 has decreased to a level at which it becomes difficult to distinguish between cosmogenic C-14 and terrestrial contamination. These meteorites may therefore be much older than 35 ky. We selected chondrites with low C-14 activities (less than or equal to 2 dpm/kg) for measurements of the concentrations of cosmogenic Cl-36 (half-life= 3.01 x 10(exp 5) y) and Ca-41 (half-life= 1.04 x 10(exp 5) y) in the metal phase. Since the ratio of Ca-41/Cl-36 in the metal phase of chondrites is relatively constant and well known, the measured ratio is a direct measure of the terrestrial age]. A major problem is that most or sometimes all. of the metal in these old "hot desert" meteorites has been oxidized to hydrated Fe-Ni-oxides. Therefore, we also measured the concentrations of Be-10, Al-26 and Cl-36 in the stony phase in order to constrain the terrestrial age as much as possible.

Welten, K. C.↗
NASA NTRS2004

Constraints on the Origin of Chondrules and CAIs from Short-lived and Long-lived Radionuclides

In order to understand the timing of events in the early solar system, we rely on the radio-nuclide-based chronometers applied to materials in primitive meteorites. Because the time scale of early-solar system evolution was on the order of a few million years (Myr), we focus on so-called "short-lived radionuclides" with mean lives of less than 10 Myr (Table 1), as well as on the long-lived U-Pb system where high precision 207Pb-206Pb ages are applied. Note that the validity of some systems as chronometers (e.g., Be-B, Fe-Ni) has yet to be established. We summarize literature data for chondrules and CAIs and discuss how these chronometers constrain formation time scales in the early solar system.

Kita, N. T.↗
NASA NTRSDate not supplied

Surface Exposure History of Asteroid Bennu Based on Cosmogenic Radionuclides in OSIRIS-Rex Samples

The surface of asteroid Bennu changes over time because of impacts, mass movement, and particle ejections [1-4]. The OSIRIS-REx samples were collected from a 20-m-diameter crater on Bennu called Hokioi. One of the driving hypotheses of the mission is that Hokioi is part of a population of small (<25 m) craters that are less than 0.1 Myr old and contain relatively unweathered material [1,4]. Our goal is to understand the recent surface exposure history of Bennu, utilizing radionuclides (10Be, 26Al, 36Cl, 41Ca) produced by both galactic and solar cosmic rays. We received ~12 mg of aggregate sample OREX-803014-0. We picked five of the larger particles with masses ranging from 0.24 to 0.68 mg. We dissolved each particle, along with 0.15 mg Be and 1.0 mg Cl carrier, in HF/HNO3 mixture, and did the same for the remaining aggregate sample of 9.8 mg. After dissolution, we took a small aliquot for chemical analysis, added 0.7 mg of Al carrier, and separated Be, Al, and Cl for analysis of cosmogenic 10Be, 26Al, and 36Cl by accelerator mass spectrometry [5]. Preliminary 26Al results show concentrations of 21–27 dpm/kg for the Bennu samples, with an average of 22.5 ± 0.6 dpm/kg for the five particles and 21.1 ± 0.7 dpm/kg for the remaining aggregate. These values are close to the expected 26Al saturation values of 25–30 dpm/kg for the top 1 m of Bennu’s regolith, suggesting a minimum exposure age of 1.5–2.0 Myr near the surface. Our initial Bennu results also resemble those found for Ryugu samples [6,7]; thus, we can hypothesize that the two asteroids have had similar surface exposure histories.

K C Welten↗