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All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Scalar and tensor resonances in $J/\psi $ radiative decays

We perform a systematic analysis of the J/ψ → γπ 0 π 0 and → γ$K$$^{0}_{S}$$K$$^{0}_{S}$ partial waves measured by BESIII. We use a large set of amplitude parametrizations to reduce the model bias. We determine the physical properties of seven scalar and tensor resonances in the 1–2.5GeV mass range. These include the well known f 0 (1500) and f 0 (1710), that are considered to be the primary glueball candidates. The hierarchy of resonance couplings determined from this analysis favors the latter as the one with the largest glueball component.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1986

Pion-decay radiation and two-phase acceleration in the June 3, 1982 solar flare

The June 3, 1982 flare is unique in the wealth of observed neutron, gamma-ray and energetic-particle emission that it produced. Using calculations of high-energy emissions to fit the various time-dependent gamma-ray fluxes, a self-consistent interaction model for the June 3 flare is constructed in which the observed fluxes are produced by two distinct particle populations with different acceleration and interaction time histories as well as different but time-independent energy spectra. The two populations are associated with first- and second-phase particle acceleration, respectively.

Ramaty, R.↗
DOE OSTI2021

Non-radiative luminescence decay with self-trapped hole migration in strontium titanate: Interplay between optical and transport properties

A novel model for the non-radiative decay of self-trapped excitons (STEs) in the advanced functional oxide SrTiO3 is proposed and supported by experimental observations. The study is based on the initial ionoluminescence stage for STE emission at 2.5 eV, and its dependence on temperature and electronic excitation rate under energetic heavy-ion irradiation. For all temperatures, this initial stage reaches rapidly a quasi-steady level, and then decreases as induced-structural damage increases. The quasi-steady luminescence exhibits a linear dependence on the excitation rate, suggesting a constant efficiency for STEs formation. An activation energy of 55 meV, essentially independent of the incident ion mass and energy of projectile-ion, is deduced from an Arrhenius-type relationship with irradiation temperature. This energy is in good agreement with experimental values, measured for non-radiative STE decay under ns-laser pulse excitation, and reasonably consistent with density functional theory calculations for migration of self-trapped holes (STHs) described by a small-polaron adiabatic hopping model. A new mechanism dealing with a non-radiative contribution to the STE transition is discussed, consisting of STH migration through thermally-activated hopping and annihilation with the STE-electron. Luminescence kinetics from the chromium intrinsic impurity strongly supports this model, being consistent with the annihilation of Cr 3+ centers through recombination with migrating STHs.

luminescence↗
DOE OSTI2022

Low-Energy Supernovae Severely Constrain Radiative Particle Decays

The hot and dense core formed in the collapse of a massive star is a powerful source of hypothetical feebly interacting particles such as sterile neutrinos, dark photons, axionlike particles (ALPs), and others. Radiative decays such as a→2γ deposit this energy in the surrounding material if the mean free path is less than the radius of the progenitor star. For the first time, we use a supernova (SN) population with particularly low explosion energies as the most sensitive calorimeters to constrain this possibility. These SNe are observationally identified as low-luminosity events with low ejecta velocities and low masses of ejected 56 Ni. Their low energies limit the energy deposition from particle decays to less than about 0.1 B, where 1 B(bethe) = 10 51 erg. For 1–500 MeV-mass ALPs, this generic argument excludes ALP-photon couplings G aγγ in the 10 -10 -10 -8 GeV -1 range.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Efficient lattice QCD computation of radiative-leptonic-decay form factors at multiple positive and negative photon virtualities

In previous work [D. Giusti, Methods for high-precision determinations of radiative-leptonic decay form factors using lattice QCD, Phys. Rev. D 107, 074507 (2023)], we showed that form factors for radiative leptonic decays of pseudoscalar mesons can be determined efficiently and with high precision from lattice QCD using the “three-dimensional (3D) method,” in which three-point functions are computed for all values of the current insertion time and the time integral is performed at the data-analysis stage. Here, we demonstrate another benefit of the 3D method: the form factors can be extracted for any number of nonzero photon virtualities from the same three-point functions at no extra cost. We present results for the $D_s → ℓνγ*$ vector form factor as a function of photon energy and photon virtuality, for both positive and negative virtuality, for a single ensemble with 340 MeV pion mass and 0.11 fm lattice spacing. In our analysis, we separately consider the two different time orderings and the different quark flavors in the electromagnetic current. We discuss in detail the behavior of the unwanted exponentials contributing to the three-point functions, as well as the choice of fit models and fit ranges used to remove them for various values of the virtuality. While positive photon virtuality is relevant for decays to multiple charged leptons, negative photon virtuality suppresses soft contributions and is of interest in QCD-factorization studies of the form factors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Hint of a new scalar interaction in LHCb data?

Abstract We explain recent LHCb measurements of the lepton universality ratios, $$R_{D^{(*)}}^{\tau /\ell }\equiv \frac{\mathcal {B}(\bar{B} \rightarrow D^{(*)+} \tau ^- \bar{\nu }_\tau )}{\mathcal {B}(\bar{B} \rightarrow D^{(*)+}\ell ^- \bar{\nu }_\ell )}$$ R D ( ∗ ) τ / ℓ ≡ B ( B ¯ → D ( ∗ ) + τ - ν ¯ τ ) B ( B ¯ → D ( ∗ ) + ℓ - ν ¯ ℓ ) and $${R(\Lambda _c^+)}^{\tau /\ell } \equiv \frac{\mathcal {B}(\Lambda _b \rightarrow \Lambda _c^+ \tau ^- \bar{\nu }_{\tau })}{\mathcal {B}(\Lambda _b \rightarrow \Lambda _c^+ \ell ^- \bar{\nu }_{\ell })}$$ R ( Λ c + ) τ / ℓ ≡ B ( Λ b → Λ c + τ - ν ¯ τ ) B ( Λ b → Λ c + ℓ - ν ¯ ℓ ) with $$\ell =\mu $$ ℓ = μ , via new physics that affects $$R_D^{\tau /\ell }$$ R D τ / ℓ and $$R(\Lambda _c^+)^{\tau /\ell }$$ R ( Λ c + ) τ / ℓ but not $$R_{D^*}^{\tau /\ell }$$ R D ∗ τ / ℓ . The scalar operator in the effective theory for new physics is indicated. We find that the forward-backward asymmetry and $$\tau $$ τ polarization in $$\bar{B} \rightarrow D^+ \tau ^{-} \bar{\nu }_{\tau }$$ B ¯ → D + τ - ν ¯ τ and $$\Lambda _b \rightarrow \Lambda _c^+ \tau ^- \bar{\nu }_{\tau }$$ Λ b → Λ c + τ - ν ¯ τ decays are significantly affected by the scalar interaction. We construct a simple two Higgs doublet model as a realization of our scenario and consider lepton universality in semileptonic charm and top decays, radiative B decay, B -mixing, and $$Z \rightarrow b \bar{b}$$ Z → b b ¯ .

Physics↗
DOE OSTI2026

Lattice calculation of light meson radiative leptonic decays

In this work, we perform a lattice QCD calculation of the branching ratios and the form factors\r\nof radiative leptonic decays P →ℓνℓγ (P= π,K) using Nf = 2+1 domain wall fermion ensembles\r\ngenerated by the RBC and UKQCD collaborations at the physical pion mass. We adopt the\r\ninfinite-volume reconstruction (IVR) method, which extends lattice data to infinite volume and\r\neffectively controls the finite-volume effects. This study represents a first step toward a complete\r\ncalculation of radiative corrections to leptonic decays using the IVR method, including both real\r\nphoton emissions and virtual photon loops. For decays involving a final-state electron, collinear\r\nradiative corrections, enhanced by the large logarithmic factors such as ln(m2\r\nπ/m2e) and ln(m2K/m2e), can reach the level of O(10%) and are essential at the current level of theoretical and experimental precision. After including these corrections, our result for π →eνeγ agrees with the PIBETA measurement; for K →eνeγ, our results are consistent with the KLOE data and exhibit a 1.7σtension with E36; and for K →µνµγ, where radiative corrections are negligible, our results confirm the previously observed discrepancies between lattice results and the ISTRA/OKA measurements at large photon energies, and with the E787 results at large muon–photon angles.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Decoupling excitons from high-frequency vibrations in organic molecules

The coupling of excitons in π-conjugated molecules to high-frequency vibrational modes, particularly carbon–carbon stretch modes (1,000–1,600 cm -1 ) has been thought to be unavoidable. These high-frequency modes accelerate non-radiative losses and limit the performance of light-emitting diodes, fluorescent biomarkers and photovoltaic devices. Here, by combining broadband impulsive vibrational spectroscopy, first-principles modelling and synthetic chemistry, we explore exciton–vibration coupling in a range of π-conjugated molecules. We uncover two design rules that decouple excitons from high-frequency vibrations. First, when the exciton wavefunction has a substantial charge-transfer character with spatially disjoint electron and hole densities, we find that high-frequency modes can be localized to either the donor or acceptor moiety, so that they do not significantly perturb the exciton energy or its spatial distribution. Second, it is possible to select materials such that the participating molecular orbitals have a symmetry-imposed non-bonding character and are, thus, decoupled from the high-frequency vibrational modes that modulate the π-bond order. We exemplify both these design rules by creating a series of spin radical systems that have very efficient near-infrared emission (680–800 nm) from charge-transfer excitons. We show that these systems have substantial coupling to vibrational modes only below 250 cm -1 , frequencies that are too low to allow fast non-radiative decay. This enables non-radiative decay rates to be suppressed by nearly two orders of magnitude in comparison to π-conjugated molecules with similar bandgaps. Our results show that losses due to coupling to high-frequency modes need not be a fundamental property of these systems.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1985

Far-ultraviolet background observations at high galactic latitude. I - The Coma Cluster

A series of high-galactic-latitude observations made with the Voyager 2 ultraviolet spectrometer are used to place stringent upper limits on the far-ultraviolet emissions from the central regions of the Coma Cluster of galaxies. In particular, consideration of the 912-1150 A region yields lower limits upon the radiative decay lifetimes of any neutrino species with masses in the range 22.1-27.8 eV, assuming massless decay products. Limits on the radiative decay lifetimes of such neutrinos are found to vary from 2.4 x 10 to the 25th to 7.1 x 10 to the 24th s, respectively, as a function of neutrino rest mass. This represents a substantial improvement over previous measurements.

Holberg, J. B.↗
NASA NTRS1993

A search for radiative neutrino decay from supernovae

This document presents the data analysis procedures proposed for use with the COMPTEL instrument aboard the Compton Gamma Ray Observatory (GRO) in the search for radiative neutrino decay from supernovae. The proposed analysis methodology is an extension of a standard procedure used by the COMPTEL team in searching for a variety of source types. We have applied the procedures to a set of simulated data to demonstrate the feasibility of the method to this project.

Miller, Richard S.↗
NASA NTRS1992

Can neutrino decay-driven mock gravity save hot dark matter?

The radiative decay of a 30 eV neutrino with a lifetime of order 10 exp 23-24 s has recently been shown to yield a satisfactory explanation of a wide range of problems in astrophysics. In this paper, it is investigated whether the photon flux generated by the radiative decay of a massive neutrino is capable of generating sufficient radiation pressure to cause a 'mock gravitational' collapse of primordial hydrogen clouds. It is shown that when using neutral hydrogen as a source of opacity for mock gravity the time scale for mock gravitational collapse is significantly larger than the expansion time scale. Thus, the model fails as a source of galactic seed perturbations. Furthermore, it is argued that nonlinear feedback mechanisms will be unable to increase the collapse rate of the cloud under mock gravity.

Splinter, Randall J.↗
NASA NTRS1993

A search for radiative neutrino decay from supernovae

Two supernovae have been identified in the COMPTEL data base as being the best sources to investigate for evidence of gamma-ray emission caused by radiative neutrino decay. These are SN1987a and SN1993J. A detailed simulation has shown us that we can expect a gain in sensitivity 1-3 orders of magnitude (depending on neutrino mass) over previous results. Instrument response is now being modeled using a SPARC10 computer acquired for this study. A library of simulated gamma-ray lines is being produced for COMPTEL as a by-product of this effort.

Svoboda, Robert C.↗
NASA NTRS1993

Radiative lifetimes of the 2s2p2(4P) metastable levels of N III

The radiative decay rates of N III 175 nm intersystem lines were measured in the laboratory by recording the time dependence of photon intensities emitted as the 2s2p2(4P) metastable term of N(2+) ions decay to the 2s22p(2P0) ground term. A cylindrical radio frequency ion trap was used to store the electron impact-produced N(2+) ions. The radiative decay signals were analyzed by multiexponential least-squares fits to the data. The measured radiative decay rates to the ground term are 1019(+/- 64)/s for 4P sub 1/2, 74.5(+/- 5.4)/s for 4P sub 3/2, and 308( +/- 22)/s for 4P sub 5/2. Comparisons of the measured values with theoretical values are presented.

Fang, Z.↗
DOE OSTI2024

MicroBooNE investigations on the photon interpretation of the MiniBooNE low energy excess

The MicroBooNE experiment is a liquid argon time projection chamber with 85-ton active volume at Fermilab, operated from 2015 to 2020 to collect neutrino data from Fermilab's Booster Neutrino Beam. One of MicroBooNE's physics goals is to investigate possible explanations of the low-energy excess observed by the MiniBooNE experiment in $\nu_{\mu}\rightarrow \nu_{e}$ neutrino oscillation measurements. MicroBooNE has performed searches to test hypothetical interpretations of the MiniBooNE low-energy excess, including the underestimation of the photon background or instrinic $\nu_{e}$ background. This thesis presents MicroBooNE's searches for two neutral current (NC) single-photon production processes that contribute to the photon background of the MiniBooNE measurement: NC $\Delta$ resonance production followed by $\Delta$ radiative decay: $\Delta \rightarrow N\gamma$, and NC coherent single-photon production. Both searches take advantage of boosted decision trees to yield efficient background rejection, and a high-statistic NC $\pi^0$ measurement to constrain dominant background, and make use of MicroBooNE's first three years of data. The NC $\Delta \rightarrow N\gamma$ measurement yielded a bound on the $\Delta$ radiative decay process at 2.3 times the predicted nominal rate at 90\% confidence level(C.L.), disfavoring a candidate photon interpretation of the MiniBooNE low-energy excess as a factor of 3.18 times the nominal NC Δ radiative decay rate at the 94.8\% C.L. The NC coherent single photon measurement leads to the world's first experimental limit on the cross-section of this process below 1 GeV, of $1.49 \times 10^{-41} \text{cm}^2$ at 90\% C.L., corresponding to 24.0 times the nominal prediction.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Search for diphoton decays of an axionlike particle in radiative J / ψ decays

We search for the diphoton decay of a light pseudoscalar axionlike particle, a , in radiative J / ψ decays, using 10 10 J / ψ events collected with the BESIII detector. We find no evidence of a signal and set upper limits at the 95% confidence level on the product branching fraction B ( J / ψ → γ a ) × B ( a → γ γ ) and the axionlike particle photon coupling constant g a γ γ in the ranges of ( 3.7 – 48.5 ) × 10 − 8 and ( 2.2 – 101.8 ) × 10 − 4 GeV − 1 , respectively, for 0.18 ≤ m a ≤ 2.85 GeV / c 2 . These are the most stringent limits to date in this mass region. Published by the American Physical Society 2024

Astronomy & Astrophysics↗
DOE OSTI2023

Chapter 14: Surface plasmon resonance enhanced artificial photosynthesis of chemical fuels for energy storage

Nanostructured noble metals such as Au, Ag, and Cu have interesting optical properties because of the oscillation motions of their surface electrons upon strong coupling with light under resonance conditions. This resonant oscillation motion of conduction electrons refers to surface plasmon resonance (SPR) and localized SPR (LSPR) when localized near the surface of a nanoparticle. The extinction spectrum of a solution of plasmonic nanoparticles has tunable wavelength responses from UV to NIR due to strong light scattering and absorption which are highly sensitive to the permittivity of the nanoparticles, their sizes and shapes, and chemical environment. Strong light scattering due to the LSPR of plasmonic nanoparticles creates a strong localized and far-field intensity capable of enhancing light absorption characteristics of a chromophore near a plasmonic surface. Engineering the chromophores’ radiative decay dynamics can be done by 1) increasing its radiative decay rate to increase its photoluminescence intensity and 2) increasing its nonradiative decay rates associated to direct charge transfer to the metal surface. Such interesting photophysical properties of a chromophore can be extended to other light-absorbing materials such as semiconductor thin films and nanostructures. This plasmonic effect on the photophysics of a light-absorbing material can be theoretically and experimentally validated. The phenomenon has also been applied to advanced optoelectronic devices such as organic light-emitting diodes (OLED)1 and organic photovoltaics (OPV).2-4 The local field created by the SPR can provide an intense EM field to enhance photoluminescence emission of an organic chromophore5-8 and Raman scattering of an organic molecule, and single-molecule Raman9-10 can be detected on specially designed LSPR substrate. (Figure 1 on SPR for energy) Recent studies suggest that LSPR can be incorporated in light-harvesting and conversion systems to increase energy conversion in a solar cell and photoelectrochemical cell and chemical transformations of CO2 to chemical fuels.11-12 Plasmonic active metals naturally exhibit catalytic activities for electrochemical fuel conversion that can be enhanced by engineering their structures to form unique catalytic structures such as symmetry-broken Au-Cu Janus nanocrystals.13 These studies are critical to addressing the global challenges of energy14-15 and CO2 emission from nonrenewable sources such as coal, petroleum, and natural gas.16-17 Electrochemical systems comprised of unique photonic structures and functions that enable efficient and affordable energy harvesting/conversion/storage are highly desired for providing safe and environment-friendly energy sources. This chapter reviews our recent work of LSPR enabled photoelectrochemical water splitting and recent advances in LSPR-enabled CO2 reduction and photochemical reactions reported in the literature. Scientific and technical challenges of applying LSPR to enhance these energy conversion and storage systems are discussed at the conclusion of this chapter.

Pan, Shanlin↗