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NASA NTRS1978

Barium and neodymium isotopic anomalies in the Allende meteorite

The discovery of Ba and Nd isotopic anomalies in two inclusions from the Allende meteorite is reported. The inclusions are Ca-Al-rich objects typical of the type considered as high-temperature condensation products in the solar nebula and contain distinctive Mg and O isotopic anomalies of the FUN (mass Fractionation, Unknown Nuclear processes) type. Mass-spectrometry results are discussed which show that inclusion C1 has anomalies in Ba at masses 134 and 136, while inclusion EK1-4-1 exhibits large marked negative anomalies at 130, 132, 134, and 136, as well as a positive anomaly at 137. It is also found that inclusion EK1-4-1 shows marked negative anomalies in Nd at masses 142, 146, 148, and 150, in addition to a positive anomaly at 145. These isotopic shifts are attributed to addition of r-process nuclei rather than mass fractionation. It is suggested that an onion-shell supernova explosion followed by injection into the solar nebula is the most likely generic model that may explain the observations.

Mcculloch, M. T.↗

NASA NTRS1978

On strontium isotopic anomalies and odd-A p-process abundances

Several aspects of the nucleosynthesis of Sr isotopes are considered in an attempt to shed light on the problem of the Sr isotopic anomalies discovered in an inclusion of the Allende meteorite. Decomposition of the Sr isotopes into average r-, s-, and p-process nucleosynthetic classes is performed. It is suggested that the Allende inclusion most likely has an excess of s-process Sr and that the initial Sr-87/Sr-86 isotopic ratio is probably slightly more primitive than basaltic achondrites. The results also show that Sn-115 is mostly due to the r-process and that odd-A yields are very small. It is concluded that if the Sr anomaly in the inclusion is an average s enhancement, it argues somewhat in favor of a model of gas/dust fractionation of s and r isotopes during accumulation of the inclusion parent in the protosolar cloud.

Clayton, D. D.↗

NASA NTRS1978

UH cosmic rays - Possible origin in massive stars

The origin of the Z greater than 28, ultraheavy (UH) cosmic rays in supernova explosions of massive stars, at least about 10 solar masses, is considered. For Z greater than 70, the UH data are dominated by an r-process source distribution, but for the elements just beyond iron, Z from 29 to 36, the data cannot be explained by any single process of nucleosynthesis. This problem is solved naturally in a massive-star model by secondary neutron-capture reactions occurring during core helium burning (a limited s-process) and during explosive carbon burning. Interstellar-propagation calculations have been performed with these episodes of synthesis as source distributions, and the results offer an explanation for the current UH cosmic-ray data. Further, the heavy-element synthesis during explosive carbon burning is re-examined by using more realistic initial conditions given by the post-helium-burning configuration of the star. These results are compared with earlier work and the UH cosmic-ray data. Some effects of preferential acceleration, based upon ionization potential, are considered, and experimental tests for this model are discussed.

Wefel, J. P.↗

NASA NTRS1980

Actinide crystal-liquid partitioning for clinopyroxene and Ca3/PO4/2

Coefficients for the partitioning of the actinide elements Th, U and Pu, which are used as indicators of r-process nucleosynthesis and the ages of meteorite and lunar samples, between diopsidic clinopyroxene, whitlockite and silicate liquid at 20 kbar are measured. Fission and alpha track radiography techniques are employed to detect element concentrations in synthetic crystals made using spiked starting materials, under the assumptions of equilibrium partitioning at the crystal-liquid interface and actinide zoning. Analysis of the data indicates results to be consistent with interface equilibrium except at high cooling rates. Th/U/Pu partition coefficients of about 0.002/0.002/O.06 are measured for clinopyroxene and 1.2/0.5/3.4 for whitlockite. The greater incorporation of Pu into the crystalline phases is attributed to the importance of trivalent Pu, and the similarity of its partition coefficient into clinopyroxene to that of the light rare earths supports the concept of Pu/rare earth dating.

Benjamin, T.↗

NASA NTRS1980

Nucleosynthesis of neutron-rich heavy nuclei during explosive helium burning in a 15 solar-mass supernova

The production of heavy nuclei during explosive helium burning has been calculated using the Weaver and Woosley self-consistent model of a complete 15 solar-mass star and the n-process code of Blake and Schramm. It was found that the resulting neutron-rich heavy nuclei are not produced in the relative abundances of solar-system r-process material (such as a Pt peak) nor are any actinides produced. Basically insufficient neutrons are available.

Blake, J. B.↗

NASA NTRS1981

Nucleocosmochronology

Nucleocosmochronology is analyzed on the basis of elemental isotopic abundances of radionuclides. The production and depletion mechanisms for the cosmological chronometers are investigated and model-independent theories are reviewed. Emphasis is given to the significance of the mean age of the elements and the time resolution of the last nucleosynthetic events contributing to the solar system, and it is shown how the intermediate-lived chronometers may give information on the time dependence shape of the production function. Anomalous nucleocosmochronology is investigated and galactic and cosmological constraints are described in terms of time scales for the mean age of elements and galaxies and the age of the universe. Data resulting from both model-independent and dependent analyses are compared. Results based on the mean age for the r-process elements suggest a lower limit to the age of the galaxy and the universe. It is concluded that nucleocosmochronology, when coupled with other independent determinations for the age of the universe, defines a concordant universe age of 13.5-15.5 billion years. The shape of the production function is not well determined because of the uncertainties in the xenon data.

Symbalisty, E. M. D.↗

NASA NTRS1981

Cosmic-ray abundances of elements with atomic number 26 less than or equal to 40 measured on HEAO 3

Individual elements in the cosmic radiation of even atomic number (Z) in the interval 26-40 have been resolved and their relative abundances measured. The results are inconsistent with a cosmic-ray source whose composition in this charge interval is dominated by r-process nucleosynthesis. The ratios of cosmic-ray source abundances to solar system abundances in this interval follow the same general correlation with first ionization potential as for the lighter elements, although there are deviations in detail.

Binns, W. R.↗

NASA NTRS1982

Abundances of cosmic ray nuclei heavier than 50 Sn

Preliminary results are reported from 430 days of exposure of the heavy nuclei experiment on the HEAO-3 spacecraft. These results are confined to the heavy nuclei with Z equal to or greater than 50 and emphasize the conclusions obtained on the relative numbers of actinides and heavy stable elements in the lead-platinum region. The extreme paucity of actinides found is inconsistent with the predictions of a cosmic ray source that is highly enriched in r-process material, but quite consistent with a source whose composition is similar to that of normal solar system material. An upper limit, at the 95 percent confidence level, is placed in the ratio of nuclei with Z equal to or greater than 88/(Z in the range from 74 to 87) of 0.03.

Waddington, C. J.↗

NASA NTRS1982

Ultraheavy cosmic rays - HEAO-3 results

The instrumentation and results from the Heavy Nuclei experiment on the HEAO 3 satellite are described. Six independently analyzed dual-gap ionization chambers measured the energy loss of the cosmic rays while a Cerenkov counter with 8 independently analyzed photomultipliers viewed two sheets of Pilot 425 plastic in a white box. Trajectories of the cosmic ray nuclei were determined in multiwire ionization hodoscopes. Variations in abundances were observed to be imperfectly ordered in terms of the first ionization potential, and volatility was also ruled out as the controlling factor. A predicted drop in abundance after Ba-56 was found, along with another sharp fall above Pb-82. Only one actinide-type event was detected during the 14 mos of viewing, a result consistent with other findings but which testifies against r-process formation.

Israel, M. H.↗

NASA NTRS1983

The propagation of ultraheavy cosmic ray nuclei

The propagation of ultraheavy cosmic ray nuclei (Z greater than 30) has been studied using a model based on the leaky-box formalism. This model has been used to examine the possible composition of the source, the path length distribution, and the mean escape length of the confinement region. Various abundance ratios have been found that have a sensitive dependence on one or more of these factors. Comparison of the theoretical values of these ratios with published data suggests that the source composition is similar to that of solar system matter, but that in the Pt-Pb region, enrichment in material produced by the r-process cannot be ruled out. Data for the secondary-to-primary ratio (Ru-44 - Cd-48)/(Sn-50 - Ba-56) show the presence of significantly more secondaries than are predicted, even when a truncated path length distribution is used in the model.

Brewster, N. R.↗

NASA NTRS1983

Cosmic-ray abundances of Sn, Te, Xe, and Ba nuclei measured on HEAO 3

The results of an analysis of HEAO 3 Heavy Nuclei Experimental data covering 440 days of observations of Sn-Ba nuclei in cosmic rays are reported. The particles were detected by a Cernkov counter, and a Z-squared ceiling was calculated to normalize the histograms produced. The observed large abundance of Sn and Ba relative to other elements in the region of interest indicated a predominance of the s-process in the source of the particles. When account was taken of first ionization potential effects, the data indicated that the material could be solar system in origin. A source dominated by the r-process nucleosynthesis was ruled out at the 0.93 confidence level.

Binns, W. R.↗

NASA NTRS1982

Chemical evolution of OB associations

It is determined that the existence of Al-26 and Pd-107 in meteorites in the early solar system indicates that our solar system probably formed inside an OB association that had been contaminated by the debris of at least one supernova. In addition to these radioactive tracers, the contamination of the material out of which the solar system formed would have significantly enriched the heavy element composition of the solar system relative to that of the average interstellar medium. It is found that the solar system would be enriched in those isotopes which are produced by the more massive stars, such as O-16, C-12, Ne-20, and some other r-process material. It is proposed that specific isotopic ratios and elemental ratios reflecting these differences would include the Ne-20/Ne-22 ratio, which would be higher in the solar system than in the interstellar medium and the cosmic rays, the C-12/C-13 ratio which would be higher in the solar system than in the interstellar medium, and the oxygen-to-carbon ratio, which would also be higher in the solar system than in the typical interstellar medium.

Schramm, D. N.↗

NASA NTRS1984

A high-resolution study of ultra-heavy cosmic-ray nuclei (A0178)

The main objective of the experiment is a detailed study of the charge spectra of ultraheavy cosmic-ray nuclei from zinc (Z = 30) to uranium (Z = 92) and beyond using solid-state track detectors. Special emphasis will be placed on the relative abundances in the region Z or - 65, which is thought to be dominated by r-process nucleosynthesis. Subsidiary objectives include the study of the cosmic-ray transiron spectrum a search for the postulated long-lived superheavy (SH) nuclei (Z or = 110), such as (110) SH294, in the contemporary cosmic radiation. The motivation behind the search for super-heavy nuclei is based on predicted half-lives that are short compared to the age of the Earth but long compared to the age of cosmic rays. The detection of such nuclei would have far-reaching consequences for nuclear structure theory. The sample of ultraheavy nuclei obtained in this experiment will provide unique opportunities for many tests concerning element nucleosynthesis, cosmic-ray acceleration, and cosmic-ray propagation.

Osullivan, D.↗

NASA NTRS1984

Elemental advances of ultraheavy cosmic rays

The elemental composition of the cosmic-ray source is different from that which has been generally taken as the composition of the solar system. No general enrichment of products of either r-process or s-process nucleosynthesis accounts for the differences over the entire range of ultraheavy (Z 30) elements; specific determination of nucleosynthetic contributions to the differences depends upon an understanding of the nature of any acceleration fractionation. Comparison between the cosmic-ray source abundances and the abundances of C1 and C2 chondritic meteorites suggests that differences between the cosmic-ray source and the standard (C1) solar system may not be due to acceleration fractionation of the cosmic rays, but rather to a fractionation of the C1 abundances with respect to the interstellar abundances.

Source record↗

NASA NTRS1985

A very important process of nucleosynthesis in stars

When some nuclei are free from strong gravitational field, they are unstable and will become stable nuclei by competitions of following processes: (1) neutron-evaporation; (2) spontaneous fission; and (3) beta prime 3-decay. At the initial stage, (1) and (2) are important and (3) can be ignored. The qualitative results are as follows: (1) it seems that nuclei with A 100 come from the spontaneous fission and beta prime decay of neutron-evaporated nuclei with A similiar to 140-440, which can replace the r-process; (2) the super-heavy elements with Z=114--126 (A similiar to 330--360) can be formed. They can be observed in cosmic rage if they have the halftime T 10 to the 7th poweer years; (3) the peak in the rare-earth elements comes from the symmetric fission of super-heavy elements; (4) there are more neutron-rich nuclei in the fragments; and (5) the abundances of a 83 elements in cosmic rays are one order of magnitude higher than that in the solar system.

Yu, C.↗

NASA NTRS1984

Elemental abundances of ultraheavy cosmic rays

The elemental composition of the cosmic-ray source is different from that which has been generally taken as the composition of the solar system. No general enrichment of products of either r-process or s-process nucleosynthesis accounts for the differences over the entire range of ultraheavy elements; specific determination of nucleosynthetic contributions to the differences depends upon an understanding of the nature of any acceleration fractionation. Comparison between the cosmic-ray source abundances and the abundances of C1 and C2 chondritic meteorites suggests the possibility that differences between the cosmic-ray source and the 'standard (C1) solar system' may not be due to acceleration fractionation of the cosmic rays, but may be due instead to a fractionation of the C1 abundances with respect to the interstellar abundances.

Binns, W. R.↗

NASA NTRS1983

Cosmic ray elemental abundances for Z = 26-42 measured on HEAO-3

An analysis is presented of 454 days of data from the Heavy Nuclei Experiment aboard the HEAO-3 satellite using an improved charge estimation algorithm is presented. A more precise normalization of Z = 32-42 abundances relative to iron is obtained, and more accurate detector response maps are used to recognize and reject a small class of events which was previously misidentified. The resulting abundances are in generally good agreement with solar system abundances with the first ionization potential (FIP) and with the Cameron solar system r-process (1982) with and without an applied FIP bias. The simplest interpretation of the results is that the cosmic ray source has solar system abundances modified by an FIP and/or volatility-dependent bias.

Binns, W. R.↗

NASA NTRS1985

Solar abundances and the role of nucleogenesis in low-to-medium mass stars in the galaxy

The pattern of solar elemental abundances agrees well with that shown by Cl chondrites for nonvolatile elements. For metals of the iron peak, the chief source of uncertainty seems to be the structure of the solar atmosphere. Lines of rare elements are frequently masked by atomic and molecular lines of abundant species. The vast majority of stars (including the sun) will do little to change the bulk composition of the interstellar medium from which new stars are formed. He, C, and N in small quantities are supplied by stars from 1 to 8 solar masses as they evolve and produce nebular envelopes that dissipate into the interstellar medium, but as has long been recognized, oxygen, heavier elements, and all r-process and proton-rich nuclides are made in massive stars.

Aller, L. H.↗