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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Application of a temporal multiscale method for efficient simulation of degradation in PEM Water Electrolysis under dynamic operating conditions

Hydrogen is emerging as a vital energy carrier, driven by the need to reduce carbon emissions. Proton Electrolyte Membrane Water Electrolysis (PEMWE) enables hydrogen production under fluctuating renewable power conditions but requires improved understanding and stability of the anode catalyst layer under dynamic operating conditions, especially with low noble metal loadings. Long-term degradation experiments are both time-consuming and costly; therefore, a systematic, model-aided approach is essential. In the present work, a temporal multiscale method is applied to reduce the computational effort of simulating long-term degradation processes in PEMWE, with an exemplary focus on catalyst dissolution. A mechanistic model incorporating the oxygen evolution reaction, catalyst dissolution, and hydrogen permeation from the cathode to the anode was hypothesized and implemented. In this way, the local periodicity of transport and reaction processes in dynamic PEMWE operation, which influence the gradual degradation of the catalyst layer, is captured. The temporal multiscale method significantly reduces the computational effort of simulation, decreasing processing time from hours to mere minutes. This efficiency gain is attributed to the limited evolution of Slow-Scale variables during each period of time P of the Fast-Scale variables. Consequently, simulation is required only until local periodicity is achieved within each Slow-Scale time step. Hence, the fully resolved dynamic problem is decoupled into these two scales, employing a heterogeneous multiscale technique. The developed approach effectively accelerates parameter estimation and predictive simulations, supporting systematic modeling of PEMWE degradation under dynamic conditions.

08 HYDROGEN↗
DOE OSTI2021

A pathway to unveiling neutrinoless ββ decay nuclear matrix elements via γγ decay

We investigate the experimental feasibility of detecting second-order double-magnetic dipole (γγ-M1M1) decays from double isobaric analog states (DIAS), which have recently been found to be strongly correlated with the nuclear matrix elements of neutrinoless ββ decay. Using the nuclear shell model, we compute theoretical branching ratios for γγ-M1M1 decays and compare them with other competing processes, such as single-γ decay and proton emission, which represent the dominant decay channels. We also estimate the potential competition from internal conversion and internal pair creation, which can influence the decay dynamics. Additionally, we propose an experimental strategy based on using LaBr3 scintillators to identify γγ-M1M1 transitions from the DIAS amidst the background of the competing processes. Our approach emphasizes the challenges of isolating the rare γγ-M1M1 decay and suggests ways to enhance the experimental detection sensitivity. Our simulations suggest that it may be possible to access experimentally γγ-M1M1 decays from DIAS, shedding light on the neutrinoless ββ decay nuclear matrix elements.

Romeo, Beatriz↗
DOE OSTI2020

Mirror-symmetry violation in bound nuclear ground states

Conservation laws are deeply related to any symmetry present in a physical system. Analogously to electrons in atoms exhibiting spin symmetries, it is possible to consider neutrons and protons in the atomic nucleus as projections of a single fermion with an isobaric spin (isospin) of t = 1/2. Every nuclear state is thus characterized by a total isobaric spin T and a projection T z —two quantities that are largely conserved in nuclear reactions and decays. A mirror symmetry emerges from this isobaric-spin formalism: nuclei with exchanged numbers of neutrons and protons, known as mirror nuclei, should have an identical set of states, including their ground state, labelled by their total angular momentum J and parity π. In this work, we report evidence of mirror-symmetry violation in bound nuclear ground states within the mirror partners strontium-73 and bromine-73. We find that a J π = 5/2 - spin assignment is needed to explain the proton-emission pattern observed from the T = 3/2 isobaric-analogue state in rubidium-73, which is identical to the ground state of strontium-73. Therefore the ground state of strontium-73 must differ from its J π = 1/2 - mirror bromine-73. This observation offers insights into charge-symmetry-breaking forces acting in atomic nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Saturn-ring proton backlighters for the National Ignition Facility

Proton radiography is a well-established technique for measuring electromagnetic fields in high-energy-density plasmas. Fusion reactions producing monoenergetic particles, such as D 3 He, are commonly used as a source, produced by a capsule implosion. Using smaller capsules for radiography applications is advantageous as the source size decreases, but on the National Ignition Facility (NIF), this can introduce complications from increasing blow-by light, since the phase plate focal spot size is much larger than the capsules. In this article, we report a demonstration of backlighter targets where a “Saturn” ring is placed around the capsule to block this light. The nuclear performance of the backlighters is unperturbed by the addition of a ring. We also test a ring with an equatorial cutout, which severely affects the proton emission and is not viable for radiography applications. These results demonstrate the general viability of Saturn ring backlighter targets for use on the NIF.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Measurement of the Ar ( e , e ' p ) and Ti ( e , e ' p ) cross sections in Jefferson Lab Hall A

The E12-14-012 experiment, performed in Jefferson Lab Hall A, has collected exclusive electron-scattering data ( e , e ' p ) in parallel kinematics using natural argon and natural titanium targets. In this study we report the first results of the analysis of the data set corresponding to beam energy 2222 GeV, electron scattering angle 21 . 5 ° , and proton emission angle – 50 ° . The differential cross sections, measured with ≈ 4 % uncertainty, have been studied as a function of missing energy and missing momentum, and compared to the results of Monte Carlo simulations, obtained from a model based on the distorted-wave impulse approximation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Convenient Location of a Near-Threshold Proton-Emitting Resonance in B 11

The presence of cluster-like narrow resonances in the vicinity of reaction/decay thresholds is a ubiquitous phenomenon with profound consequences. Here, we argue that the continuum coupling, present in the open quantum system description of the atomic nucleus, can profoundly impact the nature of near-threshold states. In this Letter, we discuss the structure of the recently observed near-threshold resonance in 11 B, whose very existence explains the puzzling beta-delayed proton emission of the neutron-rich 11 Be.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

All-optical nanoscopic spatial control of molecular reaction yields on nanoparticles

Molecular adsorbate reactions on nanoparticles play a fundamental role in areas such as nano-photocatalysis, atmospheric, and astrochemistry. They can be induced, enhanced, and controlled by field localization and enhancement on the nanoparticle surface. In particular, the ability to perform highly controlled near-field-mediated reactions is key to deepening our understanding of surface photoactivity on nanosystems. Here, using reaction nanoscopy, we experimentally demonstrate all-optical nanoscopic control of surface reaction yields by tailoring the near fields on nanoparticles with waveform-controlled linear and bicircular two-color laser pulses, respectively. We observe site-selective proton emission from the dissociative ionization of adsorbate molecules on Si O 2 nanoparticles as a function of the polarization and relative phase of the two-color pulses. The angularly resolved close-to-uniform mapping between the surface reaction yields and the measured ion momentum enables the observation and spatial control of molecular reactions on the nanoparticle surface with nanoscopic resolution. The experimental results are modeled and reproduced qualitatively by classical trajectory Monte Carlo simulations. Our work paves the way toward reliable all-optical control of photocatalytic chemical reactions on nanoscale surfaces.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Enhanced Nuclear Binding near the Proton Drip Line Opens Possible Bypass of the 64 Ge Rapid Proton Capture Process Waiting Point

Abstract We performed astrophysics model calculations with updated nuclear data to identify a possible bypass of the 64 Ge waiting point, a defining feature of the rapid proton capture (rp) process that powers type I X-ray bursts on accreting neutron stars. We find that the rp-process flow through the 64 Ge bypass could be up to 36% for astrophysically relevant conditions. Our results call for new studies of 65 Se, including the nuclear mass, β -delayed proton emission branching, and nuclear structure as it pertains to the 64 As( p , γ ) reaction rate at X-ray burst temperatures.

Nuclear astrophysics↗
NASA NTRS1982

Parity nonconservation and the origin of cosmic magnetic fields

Three mechanisms of cosmic magnetic field generation are discussed: (1) asymmetric decay of particles emitted by rotating black holes; (2) asymmetric proton emission by black holes due to weak radiative corrections, and (3) equilibrium parity-violating currents. It is shown that all three mechanisms can produce a seed field sufficiently strong to account for the present galactic fields.

Vilenkin, A.↗
DOE OSTI2025

$\mathcal{R}$ -matrix analysis of η + nat Cl reactions relevant to molten-salt reactor designs [Abstract]

Performed with support from the U.S. Nuclear Criticality Safety Program in an effort to provide improved chlorine cross section and corresponding covariance data, the R-matrix analysis of neutron induced reactions for two stable chlorine isotopes, 35,37 Cl, was performed in the energy range of thermal up to 1.2 MeV. Starting from the repository of the ENDF/B-VIII.0 library and following recent measurement campaigns, this work represents a significant improvement in the evaluation of the ( η , p ) reaction channel. The evaluation methodology uses the $\mathcal{R}$ -matrix code SAMMY to generate a set of Reich-Moore resonance parameters. As predicted by recently measured 35 Cl( η , p ) data, the presented evaluation features a dramatic increase in the magnitude of the ( η , p ) reaction channel over the ENDF/B-VIII.0 and previous nuclear data ENDF/B released libraries. Together with details of the evaluation procedure, the impact of the updates in the outgoing proton emissions on reactivity coefficients for different molten-salt reactor designs is presented and discussed.

charged-particle↗
NASA NTRS1999

Space Environment Effects: Model for Emission of Solar Protons (ESP)--Cumulative and Worst-Case Event Fluences

The effects that solar proton events have on microelectronics and solar arrays are important considerations for spacecraft in geostationary and polar orbits and for interplanetary missions. Designers of spacecraft and mission planners are required to assess the performance of microelectronic systems under a variety of conditions. A number of useful approaches exist for predicting information about solar proton event fluences and, to a lesser extent, peak fluxes. This includes the cumulative fluence over the course of a mission, the fluence of a worst-case event during a mission, the frequency distribution of event fluences, and the frequency distribution of large peak fluxes. Naval Research Laboratory (NRL) and NASA Goddard Space Flight Center, under the sponsorship of NASA's Space Environments and Effects (SEE) Program, have developed a new model for predicting cumulative solar proton fluences and worst-case solar proton events as functions of mission duration and user confidence level. This model is called the Emission of Solar Protons (ESP) model.

Xapsos, M. A.↗
NASA NTRS1999

Space Environment Effects: Model for Emission of Solar Protons (ESP): Cumulative and Worst Case Event Fluences

The effects that solar proton events have on microelectronics and solar arrays are important considerations for spacecraft in geostationary and polar orbits and for interplanetary missions. Designers of spacecraft and mission planners are required to assess the performance of microelectronic systems under a variety of conditions. A number of useful approaches exist for predicting information about solar proton event fluences and, to a lesser extent, peak fluxes. This includes the cumulative fluence over the course of a mission, the fluence of a worst-case event during a mission, the frequency distribution of event fluences, and the frequency distribution of large peak fluxes. Naval Research Laboratory (NRL) and NASA Goddard Space Flight Center, under the sponsorship of NASA's Space Environments and Effects (SEE) Program, have developed a new model for predicting cumulative solar proton fluences and worst-case solar proton events as functions of mission duration and user confidence level. This model is called the Emission of Solar Protons (ESP) model.

Xapsos, M. A.↗
NASA NTRS1985

Ly-alpha and H-alpha emission by superthermal proton beams

Simnett and Harrison (1984) have presented a model in which 100-1000 keV protons are an energy transfer agent linking coronal mass ejections and solar flares. Orrall and Zirker (1976) suggested that such protons, incident upon the chromosphere, would produce nonthermal Ly-alpha emission after charge exchange with ambient chromospheric hydrogen atoms. The present investigation is concerned with a study of the charge-exchange mechanism proposed by Orral and Zirker. The physical theory of the formation of nonthermal Ly-alpha (and H-alpha) emission is considered, taking into account photon emission, atomic transitions, atomic equilibrium, the dominant atomic processes, and the stopping of superthermal protons. Computational results presented by Orrall and Zirker are extended.

Canfield, R. C.↗
NASA NTRS1973

Approximations for neutron emission spectra from proton collisions between 20 and 500 MeV on nuclei of A greater than or equal to 12

When high energy protons from solar proton events or trapped radiation belts impinge on spacecraft structures, secondary particles are emitted. The most pernicious secondaries, from either a biological or physical standpoint, are the cascade and evaporation neutrons because of their reaction with matter leading to radioactive materials in the spacecraft structures. Empirically determined cascade and evaporation neutron emission spectra for protons of energy between 20 and 500 MeV incident on all materials at or above carbon in mass number are presented.

Burrell, M. O.↗