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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3

Spatio-temporal electric field distributions in an atmospheric plasma jet impinging on a microchannel array surface

The electric field distribution in the ionization waves (IWs) propagating over a microchannel array dielectric surface, with the channels either empty or filled with distilled water, is measured by ps electric field induced second harmonic generation. The surface IW is initiated by the atmospheric pressure N 2 –Ar plasma jet impinging on the surface vertically and powered by ns pulse discharge bursts. The results show that the electric field inside the microchannels, specifically its horizontal component, is enhanced by up to a factor of 2. The field enhancement region is localized within the channels. The vertical electric field inside the channels lags in time compared to the field measured at the ridges, indicating the transient reversal of the IW propagation direction across the channels (toward the jet). This is consistent with the phase-locked plasma emission images and confirmed by the kinetic modeling predictions, which show that the IW ‘jumps’ over the empty channels and propagates into the channels only after the jump between the adjacent ridges. When the channels are filled with water, the wave speed increases by up to 50%, due to the higher effective dielectric constant of the surface. No evidence of a significant electric field enhancement near the dielectric surface (ceramic or water) has been detected, within the spatial resolution of the present diagnostic, ~100 μ m.

plasmas and liquids↗

Simulating energetic particle losses in JET plasmas with a reverse integration biasing scheme

We report that an integrated energetic particle transport model has been constructed in JET plasmas constrained by experimental fast ion loss measurements. The model incorporates a synthetic fast ion loss detector identical to JET’s thin-foil Faraday cup fast ion loss detector array. The loss model combines analyses from the TRANSP and ORBIT-kick codes with enhanced features for producing the synthetic diagnostic. Extensions to the ORBIT code framework allow a full-orbit representation within the vacuum region that can map particles directly to an installed detector geometry. Since synthetic fast ion loss detectors are plagued by weak loss statistics, a novel reverse integration biasing scheme has been implemented to boost computational efficiency. The model is validated against experimental loss measurements induced by long-lived kink modes and is found to be in good agreement. This confirms the development of a fully integrated transport/loss model which can be quantitatively verified against experiment allowing for future validation and predictive studies. The model is particularly useful for more complicated plasma scenarios that involve multiple fast ion species such as JET’s 2021 DT-campaign.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Mega-Gauss Plasma Jet Creation Using a Ring of Laser Beams

Using 20 OMEGA laser beams at the Laboratory for Laser Energetics, University of Rochester, to irradiate a flat plastic target in a hollow ring configuration, we created supersonic cylindrical stable plasma jets with self-generated megagauss magnetic fields extending out to >4 mm. These well-collimated magnetized jets possess a number of distinct and novel properties that will allow us to study the dynamics, physical processes, and scaling properties of astrophysical jets with a dynamic range exceeding those of previous laboratory settings. The dimensionless parameters of these laboratory jets fall in the same regime as those of young stellar object jets. These jets will also provide new versatile laser-based platforms to study magnetized shocks, shear flows, and other plasma processes under controllable conditions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Molecular beam mass spectrometry measurements of vibrationally excited N 2 in the effluent of an atmospheric plasma jet: a comparison with a state-to-state kinetic model

Vibrationally excited N 2 molecules are suggested to be one of the possible key species responsible for the observed synergistic effects in plasma catalysis for NH 3 synthesis. To assess the impact of vibrationally excited species in plasma-catalysis, quantitative measurements near interfaces are required, which remains challenging. In this letter, we report spatially resolved measurements of vibrationally excited N 2 in the effluent of an atmospheric pressure plasma jet by molecular beam mass spectrometry (MBMS). The mass spectrometry signals as a function of electron energy of the ionizer were fitted with the effective electron-impact ionization cross section of N 2 (v) considering the vibrational distribution function as determined by a detailed vibrational level resolved plasma kinetic calculation. Here, the reported method presented in this letter shows the capability of MBMS to measure vibrationally excited species of N 2 near interfaces when the vibrational distribution function is known or assumed and shows excellent agreement with state-to-state kinetic models of N 2 (v).

42 ENGINEERING↗

Atmospheric Cold Plasma Jet Coating and Surface Treatment for Improved Adhesive Bonding Performance of Dissimilar Material Joints Subject to Harsh Environmental Exposure

The program goal was the development and demonstration of a novel material coating system using an innovative atmospheric cold microwave plasma jet to enable surface functionalization for corrosion protection, wear resistance and improved bonding strength. The technical approach was directed towards proof-of-concept demonstration of advanced point-of-manufacturing material bonding to improve adhesive joint performance subject to harsh environmental exposure. The assembled team, consisting of the researchers at the University of Illinois, end-users at General Motors and small business manufacturer Starfire Industries, successfully demonstrated a single, cost-effective, high-volume production process that meets the requirements of multi-material combinations relevant to the energy-intensive transportation industry (e.g. Al-steel, Mg-steel, Al-Mg and Al-CFRP joints for body-in-white structures) while eliminating offline pretreatment for Al and Mg alloy substrates that are energy intensive, have chemical waste disposal issues, and add cost. Technical demonstration of dissimilar material joining while maintaining bonding strength and cohesion after long-duration environmental exposure was accomplished for all materials of interest. This novel approach has broad applicability for manufacturing in automotive, aerospace, marine, railcar, and specialty consumer goods, etc.

36 MATERIALS SCIENCE↗

Observations of a plectonemic configuration in a stable magnetized plasma jet

Astrophysical jets are collimated high-speed outflows emerging from spinning and accreting matter around celestial objects and may spontaneously result from self-organized processes. Magnetic self-organization is commonly observed in laboratory plasma physics experiments; however, they require close-fitting flux conservers to constrain and stabilize the toroidal or cylindrical structures. Here we report the first observations of a long, stable, free-boundary plasma jet far from chamber walls, embedding a double-helix magnetic structure resembling a force-free plectonemic Taylor state. The jets arise from an experimental setup that mimics an accretion disk and has no close-fitting solid flux conserver. The results support the hypothesis that self-organization could be a universal, intrinsic explanation for jet formation, collimation, and stability and may help explain double-helix features in celestial observations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Spatially resolved density measurements of singlet delta oxygen in a non-equilibrium atmospheric pressure plasma jet by molecular beam mass spectrometry

Singlet delta oxygen (O 2 (a 1 Δ g )), the first electronically excited state of O 2 , plays an important role in many applications. We report the first measurements of absolute densities of O 2 (a 1 Δ g ) in an atmospheric pressure plasma jet (APPJ) by molecular beam mass spectrometry (MBMS). The ability to measure axial and radial profiles of O 2 (a 1 Δ g ) impinging on a substrate in the effluent of the APPJ is a key advantage of the MBMS diagnostic method over previously reported optical methods. Here, the measured large O 2 (a 1 Δ g ) densities in the APPJ effluent, up to one order of magnitude higher than the O density, underline the potential importance of O 2 (a 1 Δ g ) in many applications using APPJs.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Theoretical Modeling of Reactor Relevant Conditions for Plasma Jet Driven Magneto-Inertial Fusion

The Charger Advanced Power and Propulsion Laboratory (CAPP), a laboratory within the Propulsion Research Center (PRC) at the University of Alabama in Huntsville (UAH) is working with Los Alamos National Laboratory (LANL). to develop models and inform on promising paths for high gain magneto-inertial fusion (MIF) conditions. This report provides a framework for identifying promising conditions for achieving ignition in plasma-jet-driven magneto-inertial fusion (PJMIF)[1]. As proposed, for the first part of the contract, UAH proposes to develop a gain over unity set of stagnation conditions to provide a state of plasma conditions to achieve to set long terms goals for the PJMIF program. Specifically, UAH will model PJMIF stagnation conditions to include radiation, heat transfer, two temperature energy equations, fusion reactivity and nonlocal fusion product deposition, but no hydrodynamics for these purposes. These calculations will use a stationary plasma model to reduce simulation complexity—focusing on a DT target at 10 keV. Subsequent work will include a DD plasma layer acting as an afterburner. UAH will assume an initial magnetic field without any consideration of the topology, just assume a field strength, most likely scaled with consideration of the local hall parameter. This effort will inform the team on the tradeoff between mass, peak target field, etc and the achievable gain.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

In Situ Infrared Spectroscopy of a Plasma Jet and Data-Driven Solution of Multi-Scale Plasma Chemistry Problems

Multi-scale problems are commonly known in many scientific and engineering fields where microscopic behaviors are coupled with macroscopic processes. This is also an unsolved problem in low-temperature plasma chemistry where hundreds of chemical species are involved in thousands of chemical reactions. To address this problem, a physics-informed data-driven modeling is developed to solve such a multi-scale problem using the experimental Fourier-transform infrared spectroscopy (FTIR) measurements of several species’ concentrations. The modeling based on modern machine learning techniques provides concentrations of other relevant species along with the electron temperature and gas temperature at the location of FTIR measurements. For example, the concentrations O, OH, and H 2 O 2 play key roles in plasma-based cancer therapy. This approach overcomes the multi-scale difficulties of microscopic low-temperature plasma chemistry coupling with macroscopic gas flow and allows the acquisition of a full picture of output species concentrations. Presented here for the helium-air jet at atmospheric pressure, the ML-based modeling can be used to describe and possibly control multiscale systems using partial experimental data sets.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Quantification of complex protective surface oxide layer formed during plasma jet exposure of multicomponent ultra-high temperature carbides

Multicomponent ultra-high temperature ceramics (MC-UHTCs) has garnered attention due to their improved thermo-mechanical and oxidation properties. MC-UHTC was progressively formed by adding a UHTC component at each step, producing binary, ternary and quaternary UHTC systems, processed by spark plasma sintering (SPS). Here, we investigate the role of multi-elements and thermochemical stability of the surface oxide layer formed during plasma arc jet exposure (T > 2500 °C) of MC-UHTCs using core-level X-ray photoelectron spectroscopy (XPS) correlated with the structural investigation. The results indicate that adding a UHTC component improves oxidation resistance due to the assemblage of refractory phases forming complex mixed oxides via preferential oxidation. XPS spectra of Ta4f, Nb3d, Ti1p, and Hf4f showed that the nature of the chemical bonds switched from metal carbides to metal oxides (metal oxy-carbides) in the binary system with retained metal carbides in ternary and quaternary UHTCs. The absence of a metal carbide peak in the high-resolution C1s scan of the binary system also supports this finding. The principal complex mixed oxide phases emanate in the exiguous oxidation of MC-UHTCs are quantified using Rietveld analysis. Overall, this study suggests that MC-UHTC is a promising material for possible application in thermal protection systems (TPS).

36 MATERIALS SCIENCE↗

Interpretation of electromagnetic modes in the sub-TAE frequency range in JET plasmas with elevated monotonic q-profiles

Recent JET deuterium experiments with an advanced tokamak scenario using an internal transport barrier (ITB) have been performed to clearly observe destabilized toroidicity-induced Alfvén eigenmodes (TAEs) by fast ions; interestingly, these also exhibit unstable electromagnetic (EM) perturbations in the sub-TAE frequency range. We identify such EM perturbations to be beta-induced ion temperature gradient (BTG) eigenmodes and not beta-induced Alfvén eigenmodes nor beta-induced Alfvén acoustic eigenmodes, which are often unstable in such high-beta plasmas with high-power neutral beam injection (NBI). The BTG modes are the most unstable modes due to the high thermal ion temperature gradient related to the ITB, high thermal ion temperature compared to thermal electron temperature (high T i /T⁠ e ), and a high ion beta regime. BTG mode experimental characteristics match the analytical theory, i.e., location in the vicinity of a rational magnetic surface with a low magnetic shear, mode frequency scaling with the ion diamagnetic frequency (⁠ω$^*_i$⁠), and a coupling among Alfvén and drift waves. We also perform linear gyrokinetic simulations with validated plasma profiles and equilibrium, and find a mode kinetically driven by thermal ions with similar characteristics as the experimental BTG modes.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

2D photofragmentation LIF imaging of H 2 O 2 and HO 2 in the effluent of an atmospheric-pressure plasma jet: effects of solid and liquid interfaces

Two-dimensional (2D) absolute measurements of hydrogen peroxide (H 2 O 2 ) and approximations of the hydroperoxyl radical (HO 2 ) in the effluent of a COST Reference Microplasma Jet operated with a He/H 2 O feed gas are presented. Gas-phase densities are mapped using photofragmentation laser-induced fluorescence (PF-LIF) under three boundary conditions: open effluent, a solid target, and a liquid target. A novel method is presented for separating PF-LIF signals from H 2 O 2 and HO 2 using comparative measurements in oxygen-rich and oxygen-free environments to exploit the preferential formation of HO 2 in the presence of molecular oxygen. This separation strategy is supported by results from a plug-flow plasma chemistry model. Measured densities agree closely with model predictions in both magnitude and trend, while the 2D experimental distributions provide additional insight into the spatial dependencies of these species. In particular, the results show distinct differences in species transport depending on the target type: solid surfaces induce lateral deflection and reduced centerline densities, whereas liquid interfaces promote axial accumulation and higher near-axis concentrations.

atmospheric-pressure plasma jet (APPJ)↗

Interpenetration and kinetic effects in converging, high-energy plasma jets

In this work, we report on numerical simulations of laser-driven convergent plasma fusion targets. These “inverted corona” fusion targets are useful for the study of counter-streaming and converging rarefied plasma flows, and previous experiments have demonstrated their potential as neutron sources. The scheme consists of a fuel layer lined along the interior surface of a hollow plastic shell that is laser-ablated and expands inward towards the target center. The plasma streams generated in these targets are initially nearly collisionless as they converge, leading to wide interaction length scales and long interaction time scales as the jets interpenetrate. Such kinetic effects impact mixing of constituent ions - a phenomenon not properly captured by single-fluid hydrodynamic simulations. Here we conduct numerical simulations using two different methods: (1) single-fluid simulations in HYDRA, and (2) kinetic-ion, fluid-electron hybrid particle-in-cell (PIC) simulations in the code Chicago. It is shown that the initially nearly collisionless plasma fronts interpenetrate deeply and lead to broader interaction regions in space and time resulting in significant beam-beam fusion. The two approaches make different, testable predictions for the effect of fuel-layer thickness on neutron yield.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Role of collisionality and radiative cooling in supersonic plasma jet collisions of different materials

Currently there is considerable interest in creating scalable laboratory plasmas to study the mechanisms behind the formation and evolution of astrophysical phenomena such as Herbig-Haro objects and supernova remnants. Laboratory-scaled experiments can provide a well diagnosed and repeatable supplement to direct observations of these extraterrestrial objects if they meet similarity criteria demonstrating that the same physics govern both systems. Here, we present a study on the role of collision and cooling rates on shock formation using colliding jets from opposed conical wire arrays on a compact pulsed-power driver. These diverse conditions were achieved by changing the wire material feeding the jets, since the ion-ion mean free path (λmfp-ii) and radiative cooling rates (Prad) increase with atomic number. Low Z carbon flows produced smooth, temporally stable shocks. Weakly collisional, moderately cooled aluminum flows produced strong shocks that developed signs of thermal condensation instabilities and turbulence. Weakly collisional, strongly cooled copper flows collided to form thin shocks that developed inconsistently and fragmented. Effectively collisionless, strongly cooled tungsten flows interpenetrated, producing long axial density perturbations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

How do magnetized HED flows transition to collimated plasma jets? (Final Report)

We present results from a pulsed-power experiment designed to generate accretion-like flows in the laboratory that may be used to study the dynamics of astrophysical accretion-driven outflows. To emulate systems like Young Stellar Object (YSO) outflows, we create radially converging plasma flows in a short disk that transition into much longer bipolar outflows. Our experiment uses a ~1 MA pulsed-power driver to generate plasma from an array of thin aluminum wires mounted to a 3D-printed current path that controls the angular momentum and magnetic field topology. In this paper, we show that experimental data scale favorably to observed properties of YSO jets. This set of experiments tests the simplest version of our possible plasma dynamics, where outflows are generated without rotation or axial magnetic field present. The temperature, velocity and density of the disk and outflows are characterized using interferometry, gated optical and ultraviolet imaging, and Thomson scattering diagnostics. We discuss the Reynolds number, magnetic Reynolds number and Mach numbers calculated in three different stages of the experiment, and compare our results to 3D numerical simulations in the PERSEUS magnetohydrodynamics code. This report is a summary of the work done by the graduate students who were supported by the project.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Exploring applications of laser-produced relativistic pair plasma jets for high-energy-density physics and astrophysics (LDRD Final Report)

We have successfully completed the ER project on the relativistic electron-positron “pair” plasmas which have unique physics property fundamental to High Energy Density (HED) plasma physics and laboratory astrophysics. Over the three-year span, we completed three discovery science experiments on NIF ARC, established a new NIF platform for the pair plasma experiments which also benefited a range of other science and HED experiments using ARC. Additional 5 experimental campaigns on Omega and Gekko facilities have also been executed successfully. Our results on the pair physics and pair-plasma interactions have been published in journal and conferences and highlighted on the Lab’s Newsline.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Observation of a magneto-Rayleigh-Taylor instability in magnetically collimated plasma jets

We present the direct experimental observation of the formation of a diamagnetic cavity and magneto-Rayleigh-Taylor (MRT) instability in a β ≈ 1 high energy density plasma. Proton radiography is used to measure the two dimensional path-integrated magnetic field in a laser-produced plasma propagating parallel to a preimposed magnetic field. Flutelike structures, associated with the MRT instability, are observed to grow at the surface of the cavity, with a measured wavelength of 1.2 mm and growth time of 4 ns. These measurements are in good agreement with predictions of three dimensional magnetohydrodynamic simulations using the GORGON code. Published by the American Physical Society 2024

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗