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At least 55 records · Page 3

An analysis of the high-latitude thermospheric wind pattern calculated by a thermospheric general circulation model. II - Neutral parcel transport

A diagnostic package developed to analyze runs made by the National Center for Atmospheric Research thermosphere general circulation model is used to calculate neutral parcel trajectories in the high-latitude E and F regions. Parcel trajectories are presented for a number of different cases to illustrate the main characteristics of F region parcel transport in the winter high-latitude region. Several examples of E region parcel trajectories are similarly analyzed, concentrating on both the southern (summer) and northern (winter) regions. F region parcel trajectories are calculated backward in time from passage over a given geographical location to illustrate the 'genesis' of those parcels whose velocities can be monitored from a ground-based Fabry-Perot observatory.

Killeen, T. L.

Analysis of the Global Microwave Polarization Data of Clouds

Two NASA microwave radiometers, the satellite-borne GPM (Global Precipitation Measurement) Microwave Imager (GMI) and the aircraft-borne CoSMIR (the Conical Scanning Millimeter-wave Imaging Radiometer), measure vertically- and horizontally-polarized microwaves emitted by cloud particles and the Earth below, providing unique information on ice crystal properties in clouds. Their data reveal that non-spherical ice crystals are common and they fall in a preferred horizontally aligned orientation in convective and optically thick clouds especially near cloud top. A bin (particle-size-resolving) microphysical model with an ice crystal shape representation is developed to simulate the evolution of ice crystal properties (i.e., size, shape and orientation), where the radiation effect on microphysics (REM) is taken into account. Since REM represents the effect of all (e.g., both infrared and solar) radiation on ice crystal temperature, it relies upon the ice crystal proprieties that determine how an ice crystal receives radiation. Definitely, REM is different from the radiative effects that cause sensitivity at the microwave frequencies in the GPM and CoSMIR observations. Model results show that horizontally-oriented ice crystals grow faster than vertically-oriented (or spherical) ones due to REM. When both horizontally- and vertically-oriented ice crystals coexist in an air parcel, the model results show that the former grow by vapor deposition whereas the latter shrink by sublimation and disappear eventually. These modeling results are supported by the GMI data and the CoSMIR observations from MC3E (Midlatitude Continental Convective Clouds Experiment) and OLYMPEX (Olympic Mountains Experiment) on the prevalence of horizontally-oriented ice crystals. Moreover, the REM-induced precipitation explains the CloudSat observations of rare thin clouds in the tropical mid-troposphere as well as the common diamond dust in the high latitudes.

Xiping Zeng

A mechanistic model of Eulerian, Lagrangian mean, and Lagrangian ozone transport by steady planetary waves

Ozone transport is calculated for steady, dissipative planetary waves using the Eulerian, Lagrangian mean, and residual circulation. A Lagrangian model of parcel dynamics is used to interpret planetary wave-photochemistry interaction. In chemically active regions the mean field ozone changes are found to be significant only where there are large gradients in chemical sources and sinks along parcel trajectories. The largest changes in the mean field are found in the lower stratosphere and are due to the Lagrangian mean advection. When the Lagrangian mean advection is approximated by the residual circulation, errors in the transport velocities as large as 30 pct may occur.

Rood, R. B.

Tropospheric Ozone Pollution from Space: New Views from the TOMS (Total Ozone Mapping Spectrometer) Instrument

New products from the TOMS (Total Ozone Mapping Spectrometer) >satellite instrument can resolve pollution events in tropical and mid-latitudes, Over the past several years, we have developed tropospheric ozone data sets by two methods. The modified-residual technique [Hudson and Thompson, 1998; Thompson and Hudson, 1999] uses v. 7 TOMS total ozone and is applicable to tropical regimes in which the wave-one pattern in total ozone is observed. The TOMSdirect method [Hudson et at., 2000] represents a new algorithm that uses TOMS radiances to extract tropospheric ozone in regions of constant stratospheric ozone and tropospheric ozone displaying high mixing ratios and variability characteristic of pollution, Absorbing aerosols (dust and smoke; Herman et at., 1997 Hsu et al., 1999), a standard TOMS product, provide transport and/or source marker information to interpret tropospheric ozone. For the Nimbus 7/TOMS observing period (1979-1992), modified-residual TTO (tropical tropospheric ozone) appears as two maps/month at I-degree latitude 2-degree longitude resolution at a homepage and digital data are available (20S to 20N) by ftp at http://metosrv2. umd.edu/~tropo/ 14y_data.d. Preliminary modified-residual TTO data from the operational Earth-Probe/TOMS (1996- present) are posted in near-real-time at the same website. Analyses with the new tropospheric ozone and aerosol data are illustrated by the following (I)Signals in tropical tropospheric ozone column and smoke amount during ENSO (El Nino-Southern Oscillation) events, e.g. 1982-1983 and the intense ENSO induced biomass fires of 1997-1998 over the Indonesian region [Thompson et a[, 2000a, Thompson and Hudson, 1999]. (2) Trends in tropospheric ozone and smoke aerosols in various tropical regions (Atlantic, Pacific, Africa, Brazil). No significant trends were found for ozone from1980-1990 [Thompson and Hudson, 19991 although smoke aerosols increased during the period [Hsu et al.,1999]. (3) Temporal and spatial offsets ("paradoxes") in tropical tropospheric ozone and smoke aerosol in regions of greatest tropical biomass burning [Thompson et at., 1996;2000b]. (4) Trans-boundary pollution tracking. With an air parcel (trajectory) model, smoke aerosol and ozone and dust plumes can be tracked across oceans (e.g., Asia to North America; North America to Europe) and national boundaries, e.g. Indonesia to Singapore and Malaysia during the 1997 ENSO fires.

Thompson, Anne M.

Influence of Lower Tropospheric Moisture on Local Soil Moisture-Precipitation Feedback Over the U.S. Southern Great Plains

Land-atmosphere coupling (LAC) has long been studied focusing on land surface and atmospheric boundary layer processes. However, the influence of lower tropospheric (LT) humidity on LAC remains largely unexplored. In this study, we use radiosonde observations from the U.S. Southern Great Plains (SGP) site and an entrained parcel buoyancy model to investigate the impact of LT humidity on LAC there during the warm season (May–September). We quantify the effect of LT humidity on convective buoyancy by measuring the difference between the 2–4 km vertically integrated buoyancy with and without the influence of background LT humidity. Our results show that, under dry soil conditions, anomalously high LT humidity is necessary to produce the buoyancy profiles required for afternoon precipitation events (APEs). These APEs under dry soil moisture cannot be explained by commonly used local land-atmosphere coupling indices such as the convective triggering potential/low-level humidity index (CTP/HI Low ), which do not account for the influence of the LT humidity. On the other hand, consideration of LT humidity is unnecessary to explain APEs under wet soil moisture conditions, suggesting the boundary layer moisture alone could be sufficient to generate the required buoyancy profiles. These findings highlight the need to consider the impact of LT humidity, which is often decoupled from the humidity near the surface and largely controlled by moisture transport, in understanding land-atmospheric feedbacks over dry soil conditions, especially during droughts or dry spells over the SGP.

Gaoyun Wang

Photochemical trajectory modelling studies of the 1987 Antarctic spring vortex

Simulations of Antarctic ozone photochemistry performed using a photochemical model integrated along air parcel trajectories are described. This type of model has a major advantage at high latitudes of being able to simulate correctly the complex interaction between photolysis and temperature fields, which, because of the polar night cannot be represented accurately in a zonally averaged framework. Isentropic air parcel trajectories were computed using Meteorological Office global model analyses and forecast fields from positions along the ER-2 flight paths during the Airborne Antarctic Ozone Experiment in Austral Spring 1987. A photochemical model is integrated along these trajectories using the aircraft observations to initialize constituent concentrations. The model includes additional reactions of the ClO dimer and also bromine reactions, which are thought to play a significant role in Antarctica. The model also includes heterogeneous reactions which are invoked when the air parcel passes through a polar stratospheric cloud (PSC). The existence of a PSC is determined throughout the course of the model integration from the parcel temperature and the saturated vapour pressure of water over an assumed H2O/HNO3 mixture. The air parcel temperature is used to determine the saturated vapor pressure of HNO3 over the same mixture. Mixing ratios which exceed saturation result in condensation of the excess in the model and hence lead to a reduction of the amount of gas phase NO2 available for chemical reaction.

Austin, J.

A computationally efficient model for turbulent droplet dispersion in spray combustion

A novel model for turbulent droplet dispersion is formulated having significantly improved computational efficiency in comparison to the conventional point source stochastic sampling methodology. In the proposed model, a computational parcel representing a group of physical particles is considered to have a normal (Gaussian) probability density function (PDF) in three-dimensional space. The mean of each PDF is determined by Lagrangian tracking of each computational parcel, either deterministically or stochastically. The variance is represented by a turbulence-induced mean squared dispersion which is based on statistical inferences from the linearized direct modeling formulation for particle/eddy interactions. Convolution of the computational parcel PDF's produces a single PDF for the physical particle distribution profile. The validity of the new model is established by comparison with the conventional stochastic sampling method, where in each parcel is represented by a delta function distribution, for non-evaporating particles injected into simple turbulent air flows.

Litchford, Ron J.

Lagrangian Assimilation of Satellite Data for Climate Studies in the Arctic

Under this grant we have developed and tested a new Lagrangian model of sea ice. A Lagrangian model keeps track of material parcels as they drift in the model domain. Besides providing a natural framework for the assimilation of Lagrangian data, it has other advantages: 1) a model that follows material elements is well suited for a medium such as sea ice in which an element retains its identity for a long period of time; 2) model cells can be added or dropped as needed, allowing the spatial resolution to be increased in areas of high variability or dense observations; 3) ice from particular regions, such as the marginal seas, can be marked and traced for a long time; and 4) slip lines in the ice motion are accommodated more naturally because there is no internal grid. Our work makes use of these strengths of the Lagrangian formulation.

Lindsay, Ronald W.

Evaluation of an efficient statistical transport model for turbulent droplet dispersion in dilute combusting sprays

Evaluation of an efficient statistical transport model for turbulent droplet dispersion is made for a dilute spray of methanol droplets injected into a turbulent, axisymmnetric methane-fuelled diffusion flame burning in stagnant air. In the dispersion model, a computational parcel representing a group of physical particles (droplets) is considered to have a normal probability density function (pdf) in space. The mean is determined by Lagrangian tracking through a sequence of stochastically generated turbulent eddies and the variance is evaluated from a statistical formulation based on the linearized particle equations of motion. The basic validity of this model is established through comparison with available experimental data and with theoretical predictions using a conventional stochastic direct modeling approach. The conclusion of the evaluation is that the proposed dispersion model compares favorably with experimental data and provides a valid technique for simulating turbulent combusting sprays with significant computational savings over conventional methods.

Litchford, Ron J.

Lateral Shock of the R Aquarii Jet

The R Aqr jet was observed with the VLA B-configuration at two epochs separated by approximately 13.2 yr. Comparison of the resulting 6 cm continuum images show that the radio jet has undergone a lateral counterclockwise rotation of approximately 6 deg-12 deg on the plane of the sky. The model of jet parcels on independent trajectories is difficult to reconcile with these observations and leads us to consider a path-oriented jet (i.e., younger parcels follow the same path as older parcels). Comparison of the most recent radio image with a nearly contemporaneous HST/FOC ultraviolet image at approximately 2330 Angstroms suggests that the ultraviolet emission lies along the leading side of the rotating radio jet. In conjunction with a proper motion analysis of the jet material that yields empirical space-velocity and resulting acceleration-magnitude relationships as a function of distance from the central source, we evaluate the observational results in terms of a schematic model in which the jet emission consists of plane-parallel isothermal shocks along the leading edge of rotation. In such a radiating shock, the ultraviolet-emitting region is consistent with the adiabatic region in the form of a high-temperature, low-density sheath that surrounds the cooled postshock radio-emitting region. Within the context of the schematic model, we obtain the temperatures, densities, and pressures within the preshock, adiabatic, and postshock regions as a function of distance from the central source; the physical parameters so derived compare favorably to previously published estimates. We obtain a total jet mass of 3.1 x 10(exp -5) solar mass and an age of approximately 115 yr. We evaluate the model in the context of its density-boundary condition, its applicability to an episodic or quasi-continuous jet, and angular momentum considerations.

Hollis, J. M.

Distribution of Halon-1211 in the Upper Troposphere and Lower Stratosphere and the 1994 Total Bromine Budget

We report here on the details of the first, in situ, real-time measurements of H-1211 (CBrClF2) and sulfur hexafluoride (SF6) mixing ratios in the stratosphere up to 20 km. Stratospheric air was analyzed for these gases and others with a new gas chromatograph, flown aboard a National Aeronautics and Space Administration ER-2 aircraft as part of the Airborne Southern Hemisphere Ozone Experiment/Measurements for Assessing the Effects of Stratospheric Aircraft mission conducted in 1994. The mixing ratio of SF6, with its nearly linear increase in the troposphere, was used to estimate the mean age of stratospheric air parcels along the ER-2 flight path. Measurements of H-1211 and mean age estimates were then combined with simultaneous measurements of CFC-11 (CCl3F), measurements of brominated compounds in stratospheric whole air samples, and records of tropospheric organic bromine mixing ratios to calculate the dry mixing ratio of total bromine in the lower stratosphere and its partitioning between organic and inorganic forms. We estimate that the organic bromine-containing species were almost completely photolyzed to inorganic species in the oldest air parcels sampled. Our results for inorganic bromine are consistent with those obtained from a photochemical, steady state model for stratospheric air parcels with CFC- I I mixing ratios greater than 150 ppt. For stratospheric air parcels with CFC-11 mixing ratios less than 50 ppt (mean age greater than or equal to 5 years) we calculate inorganic bromine mixing ratios that are approximately 20% less than the photo-chemical, steady state model. There is a 20% reduction in calculated ozone loss resulting from bromine chemistry in old air relative to some previous estimates as a result of the lower bromine levels.

Wamsley, P. R.

Trajectory Simulations of Upper Tropospheric Humidity

We present comparisons of simulations of upper tropospheric humidity at 215 and 146 hPa with satellite measurements. Our model uses diabatic trajectories to advect water vapor from an initial condition of 100% relative humidity to the final state. The model does not allow parcels' relative humidity to exceed 100%, and in this way crudely incorporates condensation. We find that this simple model does a good job of simulating the observations. Sensitivity studies suggest that one must have realistic wind velocities in order to accurately simulate the humidity distribution; microphysical parameterizations seem to be less important. Comparisions between simulations using UKMO and NCEP horizontal winds will be discussed.

Dessler, A. E.

Simulating Droplet-Resolved Haze and Cloud Chemistry Forming Secondary Organic Aerosols in Turbulent Conditions within Laboratory and Cloud Parcels

Most of our existing knowledge of cloud chemistry in regards to forming secondary organic aerosols (SOA) is based on measurements in bulk aqueous solutions. However, SOA reaction kinetics derived from bulk solution measurements might differ from the kinetics in actual cloud droplets, since turbulent mixing and ionic strengths, and ratio of surface area to volume in individual cloud droplets might vary substantially from bulk solutions in the real atmosphere. Three-dimensional models at various scales have been used to simulate aqueous chemistry. However, most of these models do not resolve turbulence down to the smallest length scales of 1 mm and do not simulate cloud chemistry in individual cloud droplets due to large computational costs. Here we incorporate the formation of isoprene epoxydiol SOA (IEPOX-SOA) in individual droplets within a one-dimensional explicit mixing parcel model (EMPM-Chem). We apply EMPM-Chem to simulate turbulence and droplet-resolved IEPOX-SOA formation using a configuration based on the Michigan Tech Pi chamber. We find that the dissolution of IEPOX gases is weighted more towards larger cloud droplets due to their large liquid water content (compared to smaller droplets), while the conversion of dissolved IEPOX to IEPOX-SOA is much greater within smaller deliquesced haze particles due to their higher acidity and ionic strengths compared to cloud droplets. We also find that as droplet residence times increase in the chamber, e.g., due to increasing ammonium bisulfate seed aerosol injection rates and/or increasing heights of the chamber, formation of IEPOX-SOA increases substantially. Thus, our EMPM-Chem model could be used to design future cloud chambers to maximize SOA production from cloud chemistry. We also apply the EMPM-Chem model to simulate how IEPOX-SOA formation evolves in individual cloud droplets within rising cloudy parcels in the atmosphere. We find that as subsaturated air is entrained into and turbulently mixed with the cloud parcel, evaporation causes a reduction in droplet sizes, which leads to corresponding increases in per droplet ionic strength and acidity. Increased droplet acidity in turn greatly accelerates the kinetics of IEPOX-SOA formation. In conclusion, our results provide key insights into single-cloud-droplet chemistry, suggesting that entrainment mixing may be an important process that increases SOA formation in the real atmosphere.

54 ENVIRONMENTAL SCIENCES

A Lagrangian Simulation of Subsonic Aircraft Exhaust Emissions

To estimate the effect of subsonic and supersonic aircraft exhaust on the stratospheric concentration of NO(y), we employ a trajectory model initialized with air parcels based on the standard release scenarios. The supersonic exhaust simulations are in good agreement with 2D and 3D model results and show a perturbation of about 1-2 ppbv of NO(y) in the stratosphere. The subsonic simulations show that subsonic emissions are almost entirely trapped below the 380 K potential temperature surface. Our subsonic results contradict results from most other models, which show exhaust products penetrating above 380 K, as summarized. The disagreement can likely be attributed to an excessive vertical diffusion in most models of the strong vertical gradient in NO(y) that forms at the boundary between the emission zone and the stratosphere above 380 K. Our results suggest that previous assessments of the impact of subsonic exhaust emission on the stratospheric region above 380 K should be considered to be an upper bound.

Schoeberl, M. R.

Sensitivity of Cirrus Simulations in Idealized Situations: The WG2 Test Cases

GCSS Cirrus Cloud Systems Working Group (WG2) is presently conducting a comparison of cirrus cloud models for idealized initial conditions. The experiments involve binary (off/on) tests of model sensitivity to infrared radiative processes, and thermal stratification, and vertical wind shear for situations of weakly forced (3 cm/s uplift) cold (-60 to -70 C) and warm (-35 to -50 C) cirrus clouds. A range of model types are involved including parcel, SCM, 2-D CRM, 3-D CRM and LES models. The test cases will be described and results from 2-dimensional cirrus cloud models with bulk microphysics (implicit second moment scheme) and explicit bin microphysics will be compared. Vertical ice mass flux (particle fall speed) is a critical model component leading to significant intermodel differences. Efforts are ongoing to better quantify this aspect. Future plans of WG2 will also be briefly described and include model comparisons for a well-observed case of cold (ARM IOP) cirrus and of warm (EUCREX) cirrus, as well as, a joint activity with WG4 to consider the treatment of anvil cirrus in a variety of models.

Starr, David OC.

The Viability of Trajectory Analysis for Diagnosing Dynamical and Chemical Influences on Ozone Concentrations in the UTLS

The viability of trajectory analysis for diagnosing the interplay between chemistry and dynamics is investigated by comparing ozone mixing ratios modelled using air-parcel pathways to values observed along flight tracks during ATTREX (Airborne Tropical TRopopause EXperiment). Trajectories are initiated at the locations of ozone observations and tracked backward in time to their sources at termini of backward trajectories. The modelled values of ozone utilize 3-dimensional analysis fields from WACCM (Whole Atmosphere Community Climate Model) (a chemical-climate model with dynamical fields nudged towards MERRA (Modern-Era Retrospective Analysis and Research Applications) reanalysis) and ERA-interim (product of ECMWF - the European Centre for Medium-Range Weather Forecasts) to determine source mixing ratios with chemical production and loss terms derived from the ozone chemistry used in WACCM. A statistical base of modelled ozone is constructed with 6 trajectory platforms (adiabatic, diabatic, and kinematic forced by ERA-interim and MERRA), two chemical models (WACCM chemistry and no chemistry), and 4 trajectory lengths (5, 10, 20, and 30 days). Linear regression is employed to separate systematic errors from random errors and to characterize the impact of source mixing ratios, path length, vertical motion, and chemistry on modelled ozone errors. Errors in the analysis ozone fields are large, if not dominant, contributors to model error. Random errors are particularly large for point-by-point comparisons, however averaging over 800 km (75 minutes) flight segments substantially reduces random error and exposes systematic errors. Of the two analysis ozone data sets, WACCM, which incorporates detailed chemistry, provides the smaller systematic errors while ERA-interim, which has crude chemistry but assimilates observational data, has the smaller random errors. Of the different trajectory platforms, adiabatic calculations produce the smaller random errors (irrespective of the use of chemistry) but both vertical motion and chemistry are required to optimally reduce systematic errors. These results suggest that meaningful analysis of dynamical and chemical interactions that control ozone mixing ratios are viable on spatial scales larger than a few reanalysis grid spaces, that errors in the analyzed ozone data sets are large but not prohibitively so, and that vertical velocities and heating rates from reanalysis data, while problematic, contain useful information [on the ozone concentrations in the UTLS (Upper Troposphere/Lower Stratosphere)].

ozone

Studies on fuel spray characteristics in high-pressure environment

The present study deals with several issues involving the improvement of physical submodels and the computational efficiency in modeling dense fuel sprays. To improve the computational efficiency, a parcel PDF approach is implemented which can account for turbulent dispersion within each computational parcel. The advantage of a parcel PDF tracking method is to reduce the number of computational parcels representing the spray dynamics as well as to obtain grid-independent solutions for two-phase flows. To account for the dense spray effects, an existing drop collision and coalescence model, two breakup models, and a Reitz's wave instability model were used. These models were incorporated into a state-of-the-art multiphase all-speed transient flow solution procedure. Comparative performance for two breakup models as well as the turbulence modulation effects are also studied. Validation cases include the nonevaporating and evaporating solid-cone dense sprays. The predictions show a reasonably good agreement with available experimental results in terms of spray penetration, drop sizes, gas and drop mean velocities, and gas and drop rms velocities. The numerical results indicate that the present parcel PDF model has the capability of accurately representing drop dispersion in dense sprays with manageable number of computational parcels.

Shang, H. M.

Short-term variability of nitrogen dioxide in the winter stratosphere

Measurements of limb radiance from the Solar Mesosphere Explorer (SME) satellite are used to infer the NO2 density at the 10- and 16-mbar pressure levels from January 1 to March 31 of 1982. A photochemical-dynamical model is developed using the presently accepted chemistry of the NO(x) family. The dynamical model produces isentropic trajectories which simulate the history of air parcels. From the trajectories the photochemical model calculates NO2 densities, which are compared to those observed by SME. Although the model generally reproduces the spatial and temporal variations rather well, some disagreement was noted for conditions of exceptionally low temperatures. Further analysis indicates that the temperature sensitivity of the N2O5 photolysis cross sections may be overestimated at low temperatures.

Zawodny, J. M.