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At least 55 records · Page 3

System and method for plasmonic control of short pulses in optical fibers

The present disclosure relates to an optical waveguide system. The system may include a first waveguide having a core-guide and a material portion surrounding and encasing the core-guide. The core-guide enables a core-guide mode for an optical signal travelling through the core-guide. A second waveguide forms a lossy waveguide on an outer surface of the first waveguide. The construction of the second waveguide is such as to achieve a desired coupling between the core-guide mode and the lossy waveguide to control an energy level of the optical signal travelling through the core-guide.

42 ENGINEERING↗

Analysis of the nonlinear propagation of incoherent pulses

The nonlinear propagation of incoherent optical pulses is studied using a normalized nonlinear Schrödinger equation and statistical analysis, demonstrating various regimes that depend on the field’s coherence time and intensity. The quantification of the resulting intensity statistics using probability density functions shows that, in the absence of spatial effects, nonlinear propagation leads to an increase in the likelihood of high intensities in a medium with negative dispersion, and a decrease in a medium with positive dispersion. In the latter regime, nonlinear spatial self-focusing originating from a spatial perturbation can be mitigated, depending on the coherence time and amplitude of the perturbation. These results are benchmarked against the Bespalov–Talanov analysis applied to strictly monochromatic pulses.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Impact of the optical parametric amplification phase on laser pulse compression

Optical parametric chirped-pulse amplification (OPCPA) is an effective way to generate ultrashort pulses that has been used extensively for a variety of applications requiring high peak intensities. Precise control and measurement of a system’s spectral and spatial phases are required for Fourier transform–limited pulse compression and diffraction-limited focusing. Phase accumulated during optical parametric amplification (OPA) can degrade the compressibility and focusability of the pulse, reducing peak intensity. We used analytic and numerical analysis of OPA to study the influence of crystal parameters, wavefront of the pump and signal, and their relative optical alignment on the accumulated phase. Here, we show that the accumulated signal phase is largely independent of amplifier saturation and, with significant local wavefront gradients in the signal or pump beam, the quality of the compressed pulses can be degraded. We use first-order expressions for the pump- and signal-angle sensitivity to evaluate an OPCPA system consisting of a highly deuterated potassium dihydrogen phosphate (DKDP) amplifier designed to support bandwidth for 15 fs pulses centered at 920 nm.

47 OTHER INSTRUMENTATION↗

FORTE Measurements of Global Optical Lightning Waveforms and Implications for Optical Lightning Detection

Lightning processes generate a diverse collection of optical pulses from current traversing the lightning channels. These signals are then broadened spatially and temporally via scattering in the clouds. The resulting waveforms measured from space with instruments like the photodiode detector (PDD) on the Fast On-orbit Recording of Transient Events (FORTE) satellite have a variety of shapes. In this study, we use coincident optical and Radio-Frequency measurements to document the properties of optical PDD waveforms associated with different types of lightning, estimate delays from scattering in the clouds, and comment on how pulse shape impacts optical lightning detection. We find that the attributes of optical pulses recorded by the PDD are consistent with prior studies, but vary globally and with event amplitude. The most powerful lightning tends to be single-peaked with faster rise times (median: ~100 µs) and shorter effective widths (median: ~400 µs) than normal lightning. Particularly dim events, meanwhile, include cases of broad optical waveforms with sustained optical emission throughout the PDD record, which the pixelated FORTE Lightning Location System (LLS) instrument has difficulty detecting. We propose that this is due to the optical signal being divided between individual LLS pixels that are each, individually, not bright enough to trigger. We use PDD waveforms and Monte Carlo radiative transfer modeling to demonstrate that increasing the temporal and spatial resolution of a pixelated lightning imager will make it more difficult to detect these broad/dim pulses as their energy becomes divided between additional pixels/integration frames.

54 ENVIRONMENTAL SCIENCES↗

Near-zero-index ultra-fast pulse characterization

Transparent conducting oxides exhibit giant optical nonlinearities in the near-infrared window where their linear index approaches zero. Despite the magnitude and speed of these nonlinearities, a “killer” optical application for these compounds has yet to be found. Because of the absorptive nature of the typically used intraband transitions, out-of-plane configurations with short optical paths should be considered. In this direction, we propose an alternative frequency-resolved optical gating scheme for the characterization of ultra-fast optical pulses that exploits near-zero-index aluminium zinc oxide thin films. Besides the technological advantages in terms of manufacturability and cost, our system outperforms commercial modules in key metrics, such as operational bandwidth, sensitivity, and robustness. The performance enhancement comes with the additional benefit of simultaneous self-phase-matched second and third harmonic generation. Because of the fundamental importance of novel methodologies to characterise ultra-fast events, our solution could be of fundamental use for numerous research labs and industries.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

High power handling digitizer using photonics

Devices, methods for analog-to-digital converters (ADCs) that perform high-dynamic range measurements based on optical techniques are disclosed. In one example aspect, an optical encoder includes a polarization rotator configured to receive a train of optical pulses, and an electro-optic (EO) modulator coupled to an output of the polarization rotator. The EO modulator is configured to receive a radio frequency (RF) signal and to produce a phase modulated signal in accordance with the RF signal. The optical encoder also includes a polarizing beam splitter coupled to the output of the EO modulator; and an optical hybrid configured to receive two optical signals from the polarizing beam splitter and to produce four optical outputs that are each phase shifted with respect to one another.

DeVore, Peter Thomas Setsuda↗

High power handling digitizer using photonics

Devices, methods for analog-to-digital converters (ADCs) that perform high-dynamic range measurements based on optical techniques are disclosed. In one example aspect, an optical encoder includes a polarization rotator configured to receive a train of optical pulses, and an electro-optic (EO) modulator coupled to an output of the polarization rotator. The EO modulator is configured to receive a radio frequency (RF) signal and to produce a phase modulated signal in accordance with the RF signal. The optical encoder also includes a polarizing beam splitter coupled to the output of the EO modulator; and an optical hybrid configured to receive two optical signals from the polarizing beam splitter and to produce four optical outputs that are each phase shifted with respect to one another.

DeVore, Peter Thomas Setsuda↗

MTW-OPAL: a technology development platform for ultra-intense optical parametric chirped-pulse amplification systems

Optical parametric chirped-pulse amplification implemented using multikilojoule Nd:glass pump lasers is a promising approach for producing ultra-intense pulses (>10 23 W/cm 2 ). We report on the MTW-OPAL Laser System, an optical parametric amplifier line (OPAL) pumped by the Nd:doped portion of the multi-terawatt (MTW) laser. This midscale prototype was designed to produce 0.5-PW pulses with technologies scalable to tens of petawatts. Technology choices made for MTW-OPAL were guided by the longer-term goal of two full-scale OPALs pumped by the OMEGA EP to produce 2 × 25-PW beams that would be co-located with kilojoule–nanosecond ultraviolet beams. Several MTW-OPAL campaigns that have been completed since “first light” in March 2020 show that the laser design is fundamentally sound, and optimization continues as we prepare for “first-focus” campaigns later this year.

42 ENGINEERING↗

A sensitive high repetition rate arrival time monitor for X-ray free electron lasers

X-ray free-electron laser sources enable time-resolved X-ray studies with unmatched temporal resolution. To fully exploit ultrashort X-ray pulses, timing tools are essential. However, new high repetition rate X-ray facilities present challenges for currently used timing tool schemes. Here we address this issue by demonstrating a sensitive timing tool scheme to enhance experimental time resolution in pump-probe experiments at very high pulse repetition rates. Our method employs a self-referenced detection scheme using a time-sheared chirped optical pulse traversing an X-ray stimulated diamond plate. By formulating an effective medium theory, we confirm subtle refractive index changes, induced by sub-milli-Joule intense X-ray pulses, that are measured in our experiment. The system utilizes a Common-Path-Interferometer to detect X-ray-induced phase shifts of the optical probe pulse transmitted through the diamond sample. Owing to the thermal stability of diamond, our approach is well-suited for MHz pulse repetition rates in superconducting linear accelerator-based free-electron lasers.

47 OTHER INSTRUMENTATION↗

Spectral and temporal shaping of spectrally incoherent pulses in the infrared and ultraviolet

Laser–plasma instabilities (LPIs) hinder the interaction of high-energy laser pulses with targets. Simulations show that broadband spectrally incoherent pulses can mitigate these instabilities. Optimizing laser operation and target interaction requires controlling the properties of these optical pulses. We demonstrate closed-loop control of the spectral density and pulse shape of nanosecond spectrally incoherent pulses after optical parametric amplification in the infrared (∼1053 nm) and sum–frequency generation to the ultraviolet (∼351 nm) using spectral and temporal modulation in the fiber front end. The high versatility of the demonstrated approaches can support the generation of high-energy, spectrally incoherent pulses by future laser facilities for improved LPI mitigation.

47 OTHER INSTRUMENTATION↗

Noncollinear, inelastic four-wave mixing in the extreme ultraviolet

Driving four-wave mixing (FWM) processes with extreme ultraviolet (EUV) pulses could enable experimental approaches that have the potential to provide unique information on dynamics and correlations. In this work, we demonstrate inelastic FWM obtained by noncollinear mixing of two EUV pulses with different photon energies and an optical pulse in a diamond sample. This three-pulse interaction leads to the emission of an optical signal, propagating in the phase-matching direction and blue shifted by the photon energy difference of the two EUV pulses. The presented results demonstrate the feasibility of experiments such as the soft X-ray analogue of coherent anti-Stokes Raman scattering, so far only theoretically conceived [ Phys. Rev. Lett. 89 , 043001 ( 2002 ) PRLTAO 0031-9007 10.1103/PhysRevLett.89.043001 ], which can be further extended for studying vibrational and electronics dephasing in solid, liquid, or gaseous samples.

Mincigrucci, R. (ORCID:0000000163436256)↗

Unifying femtosecond and picosecond single-pulse magnetic switching in Gd-Fe-Co

Many questions are still open regarding the physical mechanisms behind the magnetic switching in Gd-Fe-Co alloys by single optical pulses. Phenomenological models suggest a femtosecond scale exchange relaxation between sublattice magnetization as the driving mechanism for switching. The recent observation of thermally induced switching in Gd-Fe-Co by using both several picosecond optical laser pulse as well as electric current pulses has questioned this previous understanding. This has raised the question of whether or not the same switching mechanics are acting at the femtosecond and picosecond scales. In this work, we aim at filling this gap in the understanding of the switching mechanisms behind thermal single-pulse switching. To that end, we have studied experimentally thermal single-pulse switching in Gd-Fe-Co alloys, for a wide range of system parameters, such as composition, laser power, and pulse duration. We provide a quantitative description of the switching dynamics using atomistic spin dynamics methods with excellent agreement between the model and our experiments across a wide range of parameters and timescales, ranging from femtoseconds to picoseconds. Furthermore, we find distinct element-specific damping parameters as a key ingredient for switching with long picosecond pulses and argue that switching with pulse durations as long as 15 ps is possible due to a low damping constant of Gd. Our findings can be easily extended to speed up dynamics in other contexts where ferrimagnetic Gd-Fe-Co alloys have been already demonstrated to show fast and energy-efficient processes, e.g., domain-wall motion in a track and spin-orbit torque switching in spintronics devices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Ultrafast electron dynamics in platinum and gold thin films driven by optical and terahertz fields

Here, we investigate the ultrafast electron dynamics triggered by terahertz and optical pulses in thin platinum and gold films by probing their transient optical reflectivity. The response of the platinum film to an intense terahertz pulse is similar to the optically induced one and can be described by a two-temperature model with a 20% larger electron–phonon coupling for the terahertz-driven dynamics compared to the optically induced one, ascribed to an additional nonthermal electron–phonon coupling contribution. Surprisingly, gold films exhibit a much smaller terahertz pulse-induced reflectivity change and with a sign opposite to the optical case. Additionally we explain this remarkable observation with field emission of electrons due to Fowler–Nordheim tunneling, enabled in samples with thicknesses below the structural percolation threshold, where nanostructuring promotes near-field enhancement. Our results provide a fundamental insight into the ultrafast processes relevant to modern electro- and magneto-optical applications.

74 ATOMIC AND MOLECULAR PHYSICS↗

Broadband sum-frequency generation of spectrally incoherent pulses

We study and demonstrate the nonlinear frequency conversion of broadband optical pulses from 1053 nm to 351 nm using sum-frequency generation with a narrowband pulse at 526.5 nm. The combination of angular dispersion and noncollinearity cancels out the wave-vector mismatch and its frequency derivative, yielding an order-of-magnitude increase in spectral acceptance compared to conventional tripling. This scheme can support the nonlinear frequency conversion of broadband spectrally incoherent nanosecond pulses generated by high-energy lasers and optical parametric amplifiers to mitigate laser−plasma instabilities occurring during interaction with a target. The experimental results obtained with KDP crystals are in excellent agreement with modeling, demonstrating the generation of spectrally incoherent pulses with a bandwidth larger than 10 THz at 351 nm.

47 OTHER INSTRUMENTATION↗