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DOE OSTI2025

Spectroscopy of the Hamburg Meteorite, Michigan H4

Spectroscopic studies of the Hamburg (Michigan H4) meteorite using visible–near-infrared (VNIR), mid-infrared (MIR), Raman, and Mössbauer data reproduce the results of more conventional laboratory measurements of petrology and geochemistry. This combination provides general information on the mineral modes of silicates, although spectroscopy was performed on different splits of this meteorite, and varying results may be explained by heterogeneity that is typical of ordinary chondrites. Raman also detects small features assigned to first-order D and G carbon bands, while Mössbauer data show the presence of Fe oxides and carbides. The electron microprobe (EMPA) composition of olivine in this meteorite is accurately measured to be Fo 81.3 , while MIR and Raman closely agree with Fo 80 and Fo 82 , respectively, and Mössbauer, at Fo 60 − Fo 70 , is in the ballpark. Similarly, P. R. Heck et al. report pyroxenes with compositions of Fs 16 Wo 1 , while Raman suggests a somewhat similar composition of Fs 28 Wo 0 . Both VNIR and MIR detect the presence of small amounts of feldspar, while EMPA identifies its composition as An 14 Ab 8 Or 5 . VNIR data were matched to spectral libraries of meteorite and asteroid data and shown to closely match other L and H meteorites. The best spectral matches to the Michigan H4 meteorite are to asteroid classes L/H/LL/URE, EH/EL/AUB, and CO/CV from M. D. Dyar et al.; objects in this group are intermediate in semimajor axis lengths for their orbits. The results highlight the strengths and weaknesses of each technique and show their collective strength when applied together to a single meteorite sample.

58 GEOSCIENCES↗

DOE OSTI2026

Enabling event-by-event precision in γ-ray cascades for neutron-induced reactions

Neutron-induced γ-ray spectra provide key inputs for modern active interrogation applications. A precise modeling of the nuclear reaction and subsequent emission of γ rays is challenging and often impossible due to limitations on evaluated data file formats and nuclear transport simulation codes. We present a framework that addresses these challenges by combining experimental data and reaction-model calculation outputs into an extended candidate version of the Generalized Nuclear Data Structure (GNDS) file, the successor format for the legacy Evaluated Nuclear Data File (ENDF-6). This proposed GNDS hierarchical format contains all the necessary ingredients for inline γ-ray cascade reproduction with event-by-event precision, including continuum–continuum and continuum–discrete transitions following neutron-capture and inelastic neutron scattering reactions. Cascade-event generation based on our approach demonstrates improved energy conservation on an event-by-event basis and permits the use of γ-γ coincidences in applications. This work offers, for the first time, a method to generate neutron-capture and inelastic neutron-scattering γ-ray cascades where energy conservation, correlations, and experimental primaries are fully accounted for.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2026

59 Co(p,X) spallation reaction cross sections for 250 MeV to 2 GeV protons

Cobalt is an advantageous target for probing the physics of nuclear spallation, because it is a naturally mono-isotopic element ( 59 Co), and its per-nucleon binding energy (BE/A = 8.768 MeV) is near the maximum value for all nuclei. We measured nuclear spallation cross sections for the 59 Co(p,X) reaction at five kinetic energies ranging from 250 MeV to 2 GeV. Cross sections for the production of 58 Co, 57 Co, 57 Mn, 56 Co, 56 Mn, 56 Cr, 55 Fe, 53 Fe, 54 Mn, 52 Mn, 51 Cr, 49 Cr, 48 V, 47 Sc, 46 Sc, 44 Sc, and 44 Scm are reported. Where comparable data exist in the EXFOR reaction database, we find that our measured cross sections generally agree. In many cases, we provide data for reactions or energies not currently reported in EXFOR. Our cross sections also provide evidence for the presence of α-clusters within the 59 Co nucleus, a surprising result given the asymmetry in Z (27) and N (32) for this nucleus. Finally, we use our measurements to evaluate the accuracy of spallation cross section simulations from GEANT4-based radiation transport toolkit, performed with the INCLXX-, Bertini-, and Binary-ion-cascade (BIC) based physics lists. This benchmarking activity revealed that the simulations overestimated the cross sections by a factor of ∼2–4 on average, and that the INCL-XX physics list provides the most reliable results. This evaluation informs the selection of the GEANT4 physics lists used for the analysis of data from NASA’s Psyche mission, which will measure γ rays and neutrons resulting from spallation reactions occurring on the surface of an asteroid whose surface is thought to be rich in iron-nickel metal.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Spectroscopic Measurements and Models of Energy Deposition in the Substrate of Quantum Circuits by Natural Ionizing Radiation

Naturally occurring background radiation is a potential source of correlated decoherence events in superconducting qubits that will challenge error-correction schemes. In order to characterize the radiation environment in an unshielded laboratory representative of superconducting qubits’ environments, we performed broadband, spectroscopic measurements of background radiation events inside a millikelvin refrigerator. The spectrometer was designed to mimic the size and composition of a quantum circuit. Specifically, we measured the background radiation spectra in silicon substrates of two thicknesses, 500 and 1500 µm, and one area, 25 mm 2 . The observed spectra span energies from a few kilo-electron-volts up to nearly 10 MeV, are nearly featureless, and decrease in intensity by a factor of 40 000 between 100 keV and 3 MeV for the 500-µm substrate. We integrate the spectra to obtain the average event rates and deposited power levels. These quantities correspond to a rate of 0.023 events per second and a power of 4.9 keV s -1 , when counting events that deposit at least 40 keV for the 500-µm-thick substrate. We find that the cryogenic measurements are in good agreement with predictions based on simple measurements of the terrestrial gamma-ray flux outside the refrigerator, published models of cosmic-ray fluxes, a crude model of the cryostat, and radiation-transport simulations. This model requires no free parameters to predict the background radiation spectra in the silicon substrates. The agreement between measurements and predictions demonstrates that the model we present can be used to assess the relative contributions of terrestrial and cosmic-ray sources to background radiation interactions in silicon substrates of varying thickness. These spectroscopic measurements are performed with a novel combination of superconducting microresonators located on micromachined silicon islands that define the interaction volume with background radiation. The resonators transduce deposited energy to a readily detectable electrical signal. Microresonator readout closely resembles dispersive superconducting qubit readout, so similar devices—with or without micromachined islands—are suitable for integration with superconducting quantum circuits as detectors for background radiation events. For our specific laboratory conditions, we find that gamma-ray emissions from radioisotopes are responsible for the majority of events that deposit E < 1 ⁢Me⁢V. We present results demonstrating that the background radiation spectrum contains relevant contributions from cosmic-ray particles other than muons, particularly a tail of multi-mega-electron-volt events due to protons and neutrons. These observations suggest several paths to reducing the impact of background radiation on quantum circuits, supported by an empirically validated model for generating reliable predictions of radiation interactions with silicon substrates.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2026

Data-Driven Performance Optimization of Gamma Spectrometers With Many Channels

In gamma spectrometers with variable spectroscopic performance across many channels (e.g., many pixels or voxels), a tradeoff exists between including data from successively worse-performing readout channels and increasing efficiency. Brute-force calculation of the optimal set of included channels is exponentially infeasible as the number of channels grows, and approximate methods are required. In this work, we present a data-driven framework for attempting to find near-optimal sets of included detector channels. The framework leverages non-negative matrix factorization (NMF) to learn the behavior of gamma spectra across the detector and clusters similarly-performing detector channels together. Performance comparisons are then made between spectra with channel clusters removed, which is more feasible than brute force. The framework is general and can be applied to arbitrary, user-defined performance metrics depending on the application. We apply this framework to optimizing gamma spectra measured by H3D M400 CdZnTe (CZT) spectrometers, which exhibit variable performance across their crystal volumes. In particular, we show several examples optimizing various performance metrics for uranium and plutonium gamma spectra in non-destructive assay (NDA) for nuclear safeguards, and explore trends in performance versus parameters such as clustering algorithm type. We also compare the NMF + clustering pipeline to several non-machine-learning (ML) algorithms, including several greedy algorithms. Although, we find that the NMF + clustering pipeline tends to find the best-performing set of detector voxels, significantly improving over the unoptimized spectra, but that a greedy accumulation of spectra segmented by detector depth can, in some cases, give similar performance improvements in much less computation time.

Energy resolution↗

NASA NTRS1969

The cosmic gamma-ray spectrum from secondary- particle production in the metagalaxy.

Cosmic gamma rays spectrum from neutral pions production and decay in metagalactic cosmic ray p-p collisions, deriving models based on Einstein general relativity theory

Stecker, F. W.↗

NASA NTRS1975

High-energy gamma-ray results from the second small astronomy satellite

Data are reported which were obtained with a high-energy (exceeding 35 Mev) gamma-ray telescope flown on the second Small Astronomy Satellite (SAS-2). The high-energy galactic gamma radiation is observed to dominate over the general diffuse radiation along the entire galactic plane, and its longitudinal and latitudinal distributions appear to be generally correlated with galactic structural features, particularly with arm segments. Principally on the basis of its angular distribution and magnitude, it is suggested that this radiation results primarily from cosmic-ray interactions with interstellar matter. A uniform celestial gamma radiation appears to have been detected; the form of its differential spectrum over the energy range from about 35 to 170 MeV is obtained, and a cosmological origin is suggested for this radiation. In addition to the general galactic emission, high-energy gamma radiation was detected from the Crab Nebula, Vela X, a general region toward the galactic center, and a region located a few degrees north of the galactic plane. Upper limits to the high-energy gamma ray fluxes are set for a number of localized sources.

Fichtel, C. E.↗

NASA NTRS1975

Gamma ray astronomy

A review is given of recent papers in the field of gamma-ray astronomy. It is mentioned that the strongest feature of the gamma ray sky is the general radiation from the galactic plane which is superimposed on what appears to be a general diffuse radiation, whose properties are not yet defined. The observation of high-energy galactic gamma radiation by the SAS-2 satellite is considered as is the observation of point and localized sources (the Crab Nebula, Vela, etc.). The observation of diffusive gamma radiation is discussed.

Fichtel, C. E.↗

NASA NTRS1977

Very high-energy gamma ray astronomy

Recent results in ground-based very high-energy (less than 10 to the eleventh power eV) gamma-ray astronomy are reviewed. The various modes of the atmospheric Cerenkov technique are described, and the importance of cosmic ray rejection methods is stressed. The positive detections (at approximately less than 10 to the 12th power eV) of the Crab pulsar that suggest a very flat spectrum and time-variable pulse phase are discussed. Observations of other pulsars (particularly Vela) suggest that these features may be general. The steady flux upper limits for the Crab Nebula are thus reconsidered, and a new value of the implied (Compton-synchrotron) magnetic field in the Nebula is reported. Evidence that a 4.8-hour modulated effect was detected at E sub gamma is less than 10 to the 12th power eV from Cyg X-3 is strengthened in that the exact period originally proposed agrees well with a recent determination of the X-ray period. The southern sky observations are reviewed, and the significance of the detection of an active galaxy (NGC 5128) is considered for source models and future observations.

Grindlay, J. E.↗

NASA NTRS1977

X-ray and gamma-ray line production by nonthermal ions

X-ray production was calculated at approximately 6.8 keV by the 2p to 1s transition in fast hydrogen- and helium-like iron ions, following both electron capture to excited levels and collisional excitation. A refinement of the OBK approximation was used to obtain an improved charge exchange cross section. This, and the corresponding ionization cross section were used to determine equilibrium charge fractions for iron ions as functions of their energy. The effective X-ray line production cross section was found to be sharply peaked in energy at about 8 to 12 MeV/amu. Because fast ions of similar energies can also excite nuclear levels, the ratio of selected strong gamma ray line emissivities to the X-ray line emissivity was also calculated. Limits set by this method on the intensity of gamma ray line emission from the galactic center and the radio galaxy Centaurus A are generally lower than those reported in the literature.

Bussard, R. W.↗

NASA NTRS1977

Diffuse gamma radiation

An examination of the intensity, energy spectrum, and spatial distribution of the diffuse gamma-radiation observed by SAS-2 satellite away from the galactic plane in the energy range above 35 MeV has shown that it consists of two components. One component is generally correlated with galactic latitudes, the atomic hydrogen column density was deduced from 21 cm measurements, and the continuum radio emission, believed to be synchrotron emission. It has an energy spectrum similar to that in the plane and joins smoothly to the intense radiation from the plane. It is therefore presumed to be of galactic origin. The other component is apparently isotropic, at least on a coarse scale, and has a steep energy spectrum. No evidence is found for a cosmic ray halo surrounding the galaxy in the shape of a sphere or oblate spheroid with galactic dimensions. Constraints for a halo model with significantly larger dimensions are set on the basis of an upper limit to the gamma-ray anisotropy.

Fichtel, C. E.↗

NASA NTRS1978

Thermal limit for spherical accretion and X-ray bursts

A mechanism is described whereby the rate of spherical accretion on a collapsed object and the resulting X-ray luminosity can be limited by thermal heating and evaporation of the accreting gas. The luminosity limit can be a factor of the order of 100 below the corresponding Eddington limit. Steady accretion flow is not possible within a range above this limit, and X-ray bursts can be produced by accretion surges resulting from the cooling and collapse of a heated gas shell above a critical optical depth. The luminosity and approximate recurrence rate of the bursts from NGC 6624 and other burst sources may then be understood. A general model for bursters is proposed in which massive (about 10 to 100 solar masses) black holes, from massive stars and the cores of disrupted globular clusters, undergo supercritical spherical accretion in interstellar clouds. Both X-ray and gamma-ray bursts are predicted to have similar hard X-ray (about 200 keV) spectra, though high average accretion rates and central optical depths also yield a comparable luminosity at around 5 keV from a Comptonized blackbody spectrum in the X-ray bursts and associated steady sources.

Grindlay, J. E.↗

NASA NTRS1979

Detection of 6.13 MeV gamma-rays within and at the top of the atmosphere

A measurement of the 6.13 MeV gamma-radiation from excited O-16 in the atmosphere has been made with a high-resolution Ge(Li) spectrometer flown from Palestine, Texas, 1974 June 10, on a high-altitude balloon. This measurement, made both within and near the top of the atmosphere, is found to have the same general profile as predicted by a semiempirical model, but gives a flux about a factor of 2 higher than predicted. Certain variations in the intensity at float altitude have led to the hypothesis of an extraterrestrial source of 6.13 MeV gamma-radiation from the galactic anticenter. The 3 sigma upper limits for a number of other astrophysically significant line fluxes are also given. The data presented here are consistent with either a source or a no-source hypothesis.

Willett, J. B.↗

NASA NTRS1981

Relativistic astrophysics - The view from Texas in Baltimore /Review/

Recent observational and theoretical work presented at the Tenth Texas Symposium on Relativistic Astrophysics held in Baltimore, Maryland from December 15-19, 1980, is outlined. Areas covered include the theoretical foundations of relativistic astrophysics in general relativity, quantum gravitational theory and the association of grand unification with astronomical and cosmological issues, the cosmic microwave, X-ray, gamma-ray, UV, cosmic ray and gravitational wave backgrounds, the current expansion rate and average mass-energy density of the universe, and mechanisms of galaxy formation. Also discussed are the characteristics of active galaxies and clusters emitting in the gamma-ray and X-ray regions, and compact objects formed from supernova explosions, including pulsars, X-ray-emitting neutron stars, Sco X-1 and SS 433, gamma-ray sources, and X-ray and gamma-ray bursters.

Trimble, V. L.↗

NASA NTRS1981

Thermonuclear processes on accreting neutron stars

Theoretical models for X-ray burst sources that invoke thermonuclear flashes on the surface layers of an accreting neutron star are discussed. The historical development of X-ray burst observation is summarized, and a physical picture of a neutron star undergoing accretion is drawn. Detailed numerical computations of the evolution of the surface layers of such a star are reviewed. The need for general relativistic corrections to the model is pointed out. Finally, comparisons are made with observations of X-ray bursts, the rapid burster, fast X-ray transients, X-ray pulsars, and gamma-ray burst sources.

Joss, P. C.↗

NASA NTRS1982

On the nature of 2 gamma bursts with spectral evolutions observed by the Konus experiment

Several unique features of the evolving spectra of the April 2, 1979B, and November 11, 1979 gamma-ray bursts observed by the Konus experiment can be used to determine a number of critical parameters of the sources, within the context of the thermal synchrotron model, including their luminosity distance. These results shed much light on the origin of these events and possibly gamma bursts in general.

Liang, E. P.↗

NASA NTRS1983

On the nature of two gamma bursts with spectral evolutions observed by the KONUS experiment

Liang, E. P.↗

NASA NTRS1983

Status and future of high energy diffuse gamma-ray astronomy

There are two distinctly different high energy diffuse gamma-ray components, one well correlated with broad galactic features and the other apparently isotropic and presumably extragalactic. The observed diffuse galactic high energy gamma radiation is generally thought to be produced in interactions between the cosmic rays and the interstellar matter and photons. It should then ultimately be possible to obtain from the diffuse galactic emission a detailed picture of the galactic cosmic-ray distribution, a high contrast view of the general structure of the galaxy, and further insight into molecular clouds. Two of the candidates for the explanation of the extragalactic diffuse radiation are the sum of emission from active galaxies and matter-antimatter annihilation. A major advancement in the study of the properties of both galactic and extragalactic gamma radiation should occur over the next decade.

Fichtel, C. E.↗