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Generation IV Benchmarking of TRISO Fuel Performance Models Under Accident Conditions Final Report

The Generation IV International Forum (GIF) is a co-operative international endeavor of fourteen members organized to carry out the research and development needed to establish the feasibility and performance capabilities of the next generation nuclear energy systems. GIF selected six reactor technologies, amongst which is the Very High Temperature Reactor (VHTR) that is primarily dedicated to the cogeneration of electricity and hydrogen. The technical basis for VHTR is the tristructural isotropic (TRISO)-coated particle fuel, the graphite as the core structure, helium coolant, as well as the dedicated core layout and lower power density to removal decay heat in a natural way. At the heart of safety features of the VHTR concept lie the TRISO fuel particles that are designed to keep their structural integrity and retain fission products at temperatures up to 1600°C. As part as the design and future operation of VHTRs, a key aspect is the accurate prediction of fuel performance under irradiation and accident conditions. Modeling and simulation allow prediction of TRISO fuel behavior when subject to neutron flux and in high temperature accident scenarios. The refinement of the fuel performance models and codes is performed by comparison to in-pile and out-of-pile experimental data that reproduce the expected irradiation conditions in high temperature gas-cooled reactors (HTGRs). Historically, the International Atomic Energy Agency (IAEA) developed a benchmark dedicated to the validation of predictive methods for fuel and fission product behavior through the Coordinated Research Program CRP-2 (IAEA, 1997). CRP-2 was later updated to cover fuel fabrication, quality assurance, irradiation performance, safety testing, and spent fuel. The scope of the resulting CRP-6 benchmarks focused on HTGR fuel performance and fission product release (IAEA, 2012). Taking advantage of additional TRISO fuel fabrication, irradiation, and safety testing campaigns, GIF launched a Generation IV Benchmarking of TRISO Fuel Performance Models under Accident Conditions in late 2015. This GIF benchmark is a three-year program steered by Idaho National Laboratory (INL, USA). The other participants include the Japan Atomic Energy Agency (JAEA, Japan) and the Korea Atomic Energy Research Institute (KAERI, Korea). The objectives of the benchmark are to: follow on the IAEA CRP benchmarks, (2) model fission product release under accident conditions, (3) compare results obtained by the fuel performance modeling codes of the benchmark participants, and (4) compare these code predictions to experimental data. Safety tests chosen for modeling include the first and second experiments of the Advanced Gas Reactor program (AGR-1 and AGR-2) and the High Flux Reactor (HFR) EU1bis experiment. This report presents the results obtained by the three research institutions using their respective fuel performance modeling codes. Comparisons of the corresponding fission product release predictions are made with experimental data from AGR-1, AGR-2, and HFR-EU1bis. The benchmark results show good agreements between all participants but also show a general trend of over-prediction of the experimental release data, which is mainly attributed to the use of over-estimated diffusion coefficients.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

BISON: A Finite Element-Based Nuclear Fuel Performance Code

BISON is a finite element-based nuclear fuel performance code applicable to a variety of fuel forms including light water reactor fuel rods, TRISO particle fuel, and metallic rod and plate fuel. It is a multiphysics fuel analysis tool that solves fully-coupled thermomechanical problems. BISON is based on MOOSE and can efficiently solve problems using standard workstations or very large high-performance computers in a variety of different dimensions, including full 3D, 2D-RZ axisymmetric, layered axisymmetric 1D, and spherically symmetric 1D systems. It is developed by a team of scientists and engineers at Idaho National Laboratory and by collaborators. The development of BISON is supported by various funding agencies, principally the United States Department of Energy.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Status of Multiple Channel Fuel Performance Capabilities Within the SAS4A/SASSYS-1 Safety Analysis Software

SAS4A/SASSYS-1 (SAS) is a fast-running simulation tool used to perform deterministic analysis of anticipated events as well as design basis and beyond design basis accidents for advanced liquid-metal-cooled nuclear reactors. It is a critical element of safety analysis capabilities for the U.S. Department of Energy and is utilized within industry to perform the transient safety analyses required to support the licensing of Liquid Metal-cooled Fast Reactors (LMFRs). Although SAS is exceptionally fast for most transient scenarios, fuel performance calculations, along with the associated pre-transient characterization of the fuel pin, may be required for transient scenarios where fuel pin failure is hypothesized. Both the pre-transient characterization and the transient fuel performance calculation are necessary to properly quantify margins to potential fuel failure and assess the time spent potentially exceeding such margins during events. While safety analysis calculations with fuel performance models provide a more detailed characterization of the reactor during a transient, the pre-transient characterization can be time-consuming and computationally expensive. Often, large numbers of fuel pins have been exposed to similar pre-transient irradiation conditions. Similarly, the same pre-transient fuel characterization may be applicable to numerous transient conditions. This provides an opportunity to optimize the SAS computational framework such that pre-transient fuel characterization can be shared across multiple channels (fuel pins) and across multiple simulations, thus dramatically reducing overall computational costs. This report summarizes progress toward enhancing the SAS computational framework to support shared, multiple channel fuel performance characterizations intended to significantly reduce computational costs. Preliminary testing has shown that the computational time saved by using the pre-transient sharing capability is approximately equal to the time it takes to perform the pre-transient characterization.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

BISON fuel performance modeling optimization for experiment X447 and X447A using axial swelling and cladding strain measurements

With the recent need to qualify new reactor designs such as the Versatile Test Reactor (VTR), fuel performance calculations need to be performed to determine safety criteria of the proposed designs. In order to validate the fuel performance results obtained by a fuel performance code, BISON, for new reactor designs, legacy fuel from EBR-II and FFTF MFF with Post -Irradiation Examination (PIE) data need to be used as validation cases to benchmark models. Here in this work, BISON has been paired with the Fuels Irradiation & Physics Database (FIPD) and IFR Materials Information System (IMIS) to supply PIE data for comparison with simulations of EBR-II experiments X447/X447A. X447/X447A were assessed by implementing models for Fuel Cladding Chemical Interaction (FCCI) within BISON and optimizing the friction coefficient between the fuel surface and the cladding, the anisotropic swelling factor, and the HT9 first thermal creep scalar (which scales the first term in the HT9 creep equation) to best match the PIE axial fuel swelling height and cladding profilometry for all pins in X447/X447A. The optimal values were found using a generic algorithm developed to select different values for the three parameters until end criteria was met and error couldn’t be reduced further. The BISON-simulated cladding profilometry was evaluated using Standard Error of the Estimate (SEE) to account for the profile shape of the cladding profilometry. Optimal values for the friction coefficient, anisotropic fuel swelling factor, and HT9 first thermal creep scalar were found to best fit the BISON simulation results to the PIE measurements found in IMIS and FIPD. Improvements to current models are suggested to account for the underprediction of fuel swelling at low burnups and the overprediction of fuel swelling at higher burnups observed for the axial fuel swelling height. Although two pins in EBR-II X447/X447A (DP70 and DP75) were known to fail due to FCCI, none of the pins simulated in BISON reached a cumulative damage fraction (CDF) above 0.008 with FCCI correlations coupled in the BISON simulations. The error estimate generated for all pins in X447/X447A using optimal values was 209 µm, which is deemed acceptable.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sensitivity of UO 2 fuel performance to microstructural evolutions driven by dilute additives

Use of dilute additives to nuclear fuel is being considered to increase the security of commercial fuel management through traceability of fabricated fuel elements. Taggants, as additives are denoted when included for traceability purposes, may also improve fuel performance, as demonstrated in Cr-containing uranium dioxide as described in the literature, and they may also improve fuel safety. In fact, studies have shown that some additives affect fuel material properties such as grain size and density after sintering. Given the possible range of elements that could be used as additives, the impact of such fuel property variations on the fuel’s thermomechanical behavior becomes relevant. These effects can be evaluated through a sensitivity study of standard fuel models to analyze changes in these properties using a fuel performance code. In this work, the BISON code is being used to investigate these effects through a 2D axisymmetric model of smeared UO 2 fuel pellets and ZIRLO® cladding under realistic pressurized water reactor core irradiation conditions. Here, randomly sampled densities and grain sizes within specified ranges are used as input parameters in the simulations, and several fuel model-related outputs are evaluated. The thermomechanical response of the cladding is also addressed in this study. The simultaneous variation of both input parameters offers a more comprehensive path to identify key sensitivities. Outputs explored include temperature, fission gas release, creep, and radial stress. Results show that although most of these outputs are sensitive to grain size to a certain extent, density mainly affects fuel temperature and elastic strain. Furthermore, sensitivities can vary depending on the radial position within the fuel pellet.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TRISO fuel performance analysis: Uncertainty quantification toward optimization

Tri-structural isotropic (TRISO) fuel particles are a fuel form being considered for potential use in next-generation nuclear reactors (i.e., high-temperature gas-cooled reactors). Though the TRISO fuel manufacturing process has continually advanced in recent years, particle comparisons still reveal statistical variations and uncertainties in terms of geometric configurations and material properties. Given that the physical processes ongoing in TRISO fuel particles during reactor operation are highly correlated with each other, a small degree of uncertainty in one model may lead to significant uncertainty in another. This makes appropriate uncertainty quantification of TRISO fuel particles essential. However, one may wonder about the extent to which the current version of TRISO particles has been optimized, and whether any room remains for further improvements. This paper quantifies TRISO fuel performance model uncertainties that stem from geometric and material data. For this analysis, the BISON code was used, and the Advanced Gas Reactor (AGR)-2 experiment served as a reference case. A total of 10 5 calculations was performed for the uncertainty and optimization analysis, altering the geometric and material data within their uncertainty range. Lastly, the optimization potential of TRISO particles is evaluated from a fuel performance perspective.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR TRISO Fuel Performance Modeling in FY-25

This report summarizes the activities performed in FY-25 to support fuel performance modeling for the Advanced Gas Reactor (AGR) Fuel Development and Qualification Program. This includes implementation of a new uranium oxycarbide (UCO) kernel swelling rate model, inner pyrolytic carbon (IPyC) cracking behavior and failure predictions, development of new UCO and silicon carbide (SiC) cesium diffusion parameters, and the thermomechanical behavior of particle layers using experimental data from micro-tensile strength testing.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Coupled fuel performance calculations in VERA and demonstration on Watts Bar unit 1, cycle 1

As the core simulator capabilities in the Virtual Environment for Reactor Applications (VERA) have become more mature and stable, increased attention has been focused on coupling Bison to provide fuel performance simulations. This technique has been a very important driver for the pellet-clad interaction challenge problem being addressed by the Consortium for Advanced Simulation of Light Water Reactors (CASL). Here, two coupling approaches are demonstrated on quarter core problems based on Watts Bar Nuclear Plant Unit 1, Cycle 1: (1) an inline approach in which a one-way coupling is used between neutronics/thermal hydraulics (through MPACT/CTF) and fuel performance (through Bison) but no fuel temperature information is passed back to MPACT/CTF, and (2) a two-way approach (coupled) in which the fuel temperature is passed from Bison to MPACT/CTF. In both approaches, power and temperature distributions from MPACT/CTF are used to inform the Bison simulations for each rod in the core.The demonstrations presented here are the first integrated fuel performance simulations in VERA, which opens many possibilities for future work, including applications to accident-tolerant fuel efforts and transient simulations, which are of critical importance to CASL. These demonstrations also highlight the potential to move away from the current Bison-informed fuel temperature lookup table approach, which is the default in MPACT/CTF simulations, if performance improvements are made in the near future.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

OECD/NEA MPCMIV Benchmark - Preliminary fuel performance results

The on-going OECD/NEA Multi-physics Pellet Cladding Mechanical Interaction Validation (MPCMIV) benchmark aims to provide guidance on multi-physics validation through the modelling of two cold ramps. In this paper, the first results for the base irradiation of the father rod and fuel rodlet (refabricated from the father rod), and the first cold ramp are presented. The base irradiation consists of 3 years of irradiation in the Forsmark-2 reactor. The cold ramp encompasses a steady-state pre-ramp period of less than one hour at a low constant linear heat rate (LHR) followed by a ramp test (< 1 min) with a much higher maximal LHR. The base irradiation is modelled using the fuel performance codes FRAPCON and FAST, while the cold ramp modeling is using the fuel performance code FRAPTRAN. Several missing parameters for FRAPCON/FAST base irradiation models have been selected using multiple references such as the OECD/NEA light water reactor Uncertainty Analysis in Modelling (UAM) benchmark specifications and the FRAPCON Integral Assessment report. The obtained results for the base irradiation such as the cladding outer diameter show reasonable agreement with the experimental measurements. The results for the cold ramp show larger differences with the experimental measurements (e.g., cladding axial elongation). However, such differences have been observed as well in other studies involving pellet cladding mechanical interaction analyses and are attributed to the fuel performance modelling assumptions and to the tuned modelling parameters that were not covered by the specifications. Uncertainty and sensitivity analysis might allow a better quantification of these missing parameters. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Fuel performance evaluation of two high burnup PWR core designs during normal operation, control rod withdrawal, and control rod ejection scenarios

There is interest among utilities to extend the current, 18-month operating cycle to 24 months. Economically, this extension would require greater than 5 % enrichment and peak rod average discharge burnup levels above 62 GWd/MTU. A notable challenge of increasing enrichment is the resulting additional excess reactivity encountered during the early stages of fuel life. To accommodate, burnable absorbers beyond soluble boron are introduced into the fuel system. In high burnup fuels, the possibilities of cladding lift-off and fuel melting increase due, in part, to increased rod internal pressures and limited fuel thermal conductivity, respectively. This work collaboratively employs PARCS, RELAP5-3D, and BISON to compare the fuel performance of two high burnup fuel candidates with higher than 5 % enrichment. Here, the fuel performance parameters were compared to current NRC guidance. The results demonstrate an annular fuel design with homogenously blended gadolinium as a burnable absorber operates with greater safety margins during normal operation, allowing for additional operational flexibility. During normal operation, the core design utilizing Integral Fuel Burnable Absorber pins contained fuel pins which reached plenum pressures above 15.5 MPa by the end of the first fuel cycle and fuel pins experienced cladding hoop strains above 1 %. In the Gd core design, only two observed pins experienced plenum pressures above 15.5 MPa and no pins exceeded 1 % cladding hoop strain. During the control rod withdrawal scenario, plenum pressures for pins in both designs marginally exceeded system pressure, however neither experienced excessive hoop strain. The Gd core design experienced a maximum fuel temperature of 2418 K, which is significantly higher than the Integral Fuel Burnable Absorber design at 2157 K, but still within regulatory guidance. We predicted that the fuel in both could return to service after the CRW event. We also predicted that cladding would not fail during the Control Rod Ejection in either core design. Generally, the Integral Fuel Burnable Absorber core design performed with greater safety margin with regards to temperature during normal operation and the transient events. However, the Gd core design performed with greater safety margin regarding plenum pressure and hoop strain limits during normal operation and both transient events.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

BISON Simulation of MARVEL Fuel Performance

BISON simulation of MARVEL fuel rod performance was conducted for normal operation. Fuel temperatures, plenum pressures and cumulative damage factors were calculated for five core zones. This report presents the results. BISON simulation for transient cases are planned. When the results are available, this report will be updated.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Fuel Performance Modeling Plan to Support the Advance Gas Reactor Program

This report documents the current status of the fuel performance modeling initiative to support the Advanced Gas Reactor (AGR) Fuel Development and Qualification Program in the development of tristructural-isotropic-coated fuel particles. It includes a brief summary of the codes that have been developed to support tristructural isotropic modeling along with a summary of the behavior of fuel particles during irradiation and the modeling used to capture these effects. In addition, this report identifies further modeling and material property needs for further development based on experience from previously performed AGR experiments. In general, the remaining activities to support fuel performance modeling for the AGR program include continued AGR experiment support for AGR-3/4 and AGR-5/6/7 as well as modeling improvements identified throughout the course of the program. These modeling improvements can be summarized as thermomechanical particle behavior and fission product transport. Additional modeling needs may be identified while processing the data collected during the AGR post-irradiation examination campaign and may lead to further improvements that are not included in this report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advancing SiC clad fuel performance model: bridging micro- and macro-scale models and experimental validation

This report presents a workflow for advancing fuel performance modeling of SiC composite cladding for light-water reactors by linking microscale, experimental data-informed finite element analysis with rod-scale fuel performance codes such as BISON. The workflow uses X-ray computed tomography (XCT) to capture the actual geometry and processing-induced defects of as-fabricated SiC composite tube specimens, particularly porosity and wall-thickness variations, and converts the segmented XCT volumes into image-based finite element meshes for high fidelity structural analysis.

Koyanagi, Takaaki [Oak Ridge National Laboratory (↗

25-Pin metallic fuel performance benchmark case based on the EBR-II X430 experiments series

A metallic fuel benchmark case was developed for the fuel performance code BISON based on 25 uranium-zirconium and uranium-plutonium-zirconium pins of the Experimental Breeder Reactor II X430 experiment series. Results of the benchmarks were compared with measurements and calculations made at the time of the experiment as well as subsequent measurements reported in 2019. The comparisons were used to quantify the accuracy of the BISON predictions and to identify patterns in the BISON differences.BISON predicted burnup, plenum pressure, and fission gas release fractions accurately. BISON temperature predictions were somewhat cooler than the temperatures determined at the time of the experiment but appeared to be reasonably accurate considering uncertainties in the legacy temperature calculations, uncertainties in the legacy linear heat rate calculations, and the high sensitivities of the BISON-predicted temperatures to BISON inputs. Fuel axial elongation predictions had errors correlated to fuel composition; BISON tended to underpredict the elongation of binary fuels and overpredict the elongation of ternary fuels. BISON cladding radial dilation predictions were also significantly lower than legacy PIE measurements.Recommendations were made to improve the BISON fuel gaseous swelling model to account for fuel composition, to add additional capabilities to the coolant channel temperature model to ease benchmark development, and to continue developing benchmark cases based on a wide range of experiments in several reactors. Once a wide array of benchmarks is developed, an attempt can be made to enhance or calibrate BISON models to improve the cladding dilation predictions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Multiscale, mechanistic modeling of cesium transport in silicon carbide for TRISO fuel performance prediction

Understanding cesium (Cs) transport in TRistructural ISOtropic (TRISO) particle fuel is crucial for predicting fission product release in high-temperature reactors. However, current challenges include significant scatter in diffusivity data and unexplained temperature-dependent diffusion regimes in the silicon carbide layer. This study addresses these challenges by developing a multiscale, mechanistic Cs transport model integrating atomistic simulations and phase field modeling. Our model quantifies temperature and grain size effects on Cs diffusivity, attributing experimentally observed regimes to a transition from bulk-dominated diffusivity at high temperatures to grain boundary-dominated diffusivity at lower temperatures. The model, validated against diffusion measurements and advanced gas reactor (AGR)-1 and AGR-2 post-irradiation fission product release data, enhances the predictive capability of the BISON fuel performance code. This study advances our understanding of Cs release from TRISO particles and its dependence on temperature and silicon carbide grain size, with implications for the safety and efficiency of high-temperature nuclear reactors.

BISON↗

Review of the Technical Basis for Properties and Fuel Performance Data Used in HEU to LEU Conversion Analysis for U-10Mo Monolithic Alloy Fuel

This report provides the technical basis for properties and fuel performance data used in conversion analysis for U.S. High Performance Research Reactors (USHPRR) that will convert from highly enriched uranium (HEU) to low-enriched uranium (LEU) using a new U-10Mo monolithic alloy fuel that is being qualified. The conditions that the fuel experiences changes between an HEU and LEU fuel element design due to many causes, including the density of the fuel, the presence of U-238 resonant absorber, changes to the plate and coolant channel dimensions, and changes in fuel management due to reactivity or optimization. These types of changes have been documented in operational and safety analyses conducted for conversions over decades for over 70 reactors. These conversions have all, or almost all, required recalculation of safety-related values as well as establishing operational characteristics of the core, including power distribution, reactor core power level, and cycle length between required fuel management. An overall objective of conversion is to change the reactor core design as little as possible while maintaining the reactors’ scientific, isotope production, medical, and engineering missions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fuel Performance Modeling Plan to Support the Advance Gas Reactor Program

This report documents the current status of the fuel performance modeling initiative to support the Advanced Gas Reactor (AGR) program in the development of tristructural isotropic (TRISO) coated fuel particles. A brief summary of the modeling codes that have been developed to support TRISO modeling is included along with a summary of the behavior of fuel particles during irradiation and the modeling used to capture these effects. In addition, this report identifies further modeling and material property needs that have been identified for further development based on experience from previously performed AGR experiments. In general, the remaining activities to support fuel performance modeling for the AGR program include continued AGR experiment support for AGR-3/4 and AGR-5/6/7 as well as modeling improvements identified throughout the course of the program. These modeling improvements can be summarized as the following: Fission product transport Thermomechanical particle behavior Additional modeling needs may be identified during the processing the data collected during the AGR post-irradiation examination (PIE) campaign and may lead to further modeling improvements that are not included in this report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Full-core high-burnup BWR LOCA fuel performance analysis and FFRD susceptibility

The susceptibility of the boiling water reactor (BWR) Limerick Unit 1 to fuel fragmentation, relocation, and dispersal during a postulated large-break loss-of-coolant accident (LBLOCA) was calculated using a multiphysics framework. The simulations include full-core, rod-resolved neutronic, thermal hydraulic, and fuel performance models using the VERA, TRACE, and BISON codes. This work focused on the transient BISON simulations, which include both the normal operation and LBLOCA periods in the same simulations. Cladding integrity was assessed using two correlations that are included with BISON. make page break Several new BWR-specific features were recently added to BISON. This work represents the first time these features have been included in a core-scale set of simulations. This study hence evaluates the performance of these new models for an operating reactor with realistic operating conditions. Simulation results showed that cladding integrity was maintained (i.e., no rods burst). Finally, future work to improve BWR and PWR predictions using this framework is suggested.

BISON↗