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The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Aerosols and especially their effect on clouds are one of the key components of the climate system and the hydrological cycle [Ramanathan et al., 2001]. Yet, the aerosol effect on clouds remains largely unknown and the processes involved not well understood. A recent report published by the National Academy of Science states "The greatest uncertainty about the aerosol climate forcing - indeed, the largest of all the uncertainties about global climate forcing - is probably the indirect effect of aerosols on clouds [NRC, 2001]." The aerosol effect on clouds is often categorized into the traditional "first indirect (i.e., Twomey)" effect on the cloud droplet sizes for a constant liquid water path [Twomey, 1977] and the "semi-direct" effect on cloud coverage [e.g., Ackerman et al ., 2001]." Enhanced aerosol concentrations can also suppress warm rain processes by producing a narrow droplet spectrum that inhibits collision and coalescence processes [e.g., Squires and Twomey, 1961; Warner and Twomey, 1967; Warner, 1968; Rosenfeld, 19991. The aerosol effect on precipitation processes, also known as the second type of aerosol indirect effect [Albrecht, 1989], is even more complex, especially for mixed-phase convective clouds. Table 1 summarizes the key observational studies identifying the microphysical properties, cloud characteristics, thermodynamics and dynamics associated with cloud systems from high-aerosol continental environments. For example, atmospheric aerosol concentrations can influence cloud droplet size distributions, warm-rain process, cold-rain process, cloud-top height, the depth of the mixed phase region, and occurrence of lightning. In addition, high aerosol concentrations in urban environments could affect precipitation variability by providing an enhanced source of cloud condensation nuclei (CCN). Hypotheses have been developed to explain the effect of urban regions on convection and precipitation [van den Heever and Cotton, 2007 and Shepherd, 2005]. Please see Tao et al. (2007) for more detailed description on aerosol impact on precipitation. Recently, a detailed spectral-bin microphysical scheme was implemented into the Goddard Cumulus Ensemble (GCE) model. Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and summertime convection over a mid-latitude continent with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. The impact of atmospheric aerosol concentration on cloud and precipitation will be investigated.

Tao, Wei-Kuo↗

International Satellite Cloud Climatology Project (ISCCP) Stage D2 Monthly Cloud Product - Revised Algorithm in Hierarchical Data Format (ISCCP_D2)

Since 1983 an international group of institutions has collected and analyzed satellite radiance measurements from up to five geostationary and two polar orbiting satellites to infer the global distribution of cloud properties and their diurnal, seasonal and interannual variations. The primary focus of the first phase of the project (1983-1995) was the elucidation of the role of clouds in the radiation budget (top of the atmosphere and surface). In the second phase of the project (1995 onwards) the analysis also concerns improving understanding of clouds in the global hydrological cycle. [Location=TROPOSPHERE] [Temporal_Coverage: Start_Date=1983-07-01; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=280 Km; Longitude_Resolution=280 Km; Temporal_Resolution=Monthly].

CLOUD TOP PRESSURE↗

International Satellite Cloud Climatology Project (ISCCP) Stage DX Pixel Level Cloud Product - Revised Algorithm in Native (NAT) Format (ISCCP_DX_NAT)

Since 1983 an international group of institutions has collected and analyzed satellite radiance measurements from up to five geostationary and two polar orbiting satellites to infer the global distribution of cloud properties and their diurnal, seasonal and interannual variations. The primary focus of the first phase of the project (1983-1995) was the elucidation of the role of clouds in the radiation budget (top of the atmosphere and surface). In the second phase of the project (1995 onwards) the analysis also concerns improving understanding of clouds in the global hydrological cycle. [Location=TROPOSPHERE] [Temporal_Coverage: Start_Date=1983-07-01; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=30 Km; Longitude_Resolution=30 Km; Temporal_Resolution=3 Hourly].

CLOUD ICE↗

International Satellite Cloud Climatology Project (ISCCP) Stage B3 Reduced Radiances in Native (NAT) Format (ISCCP_B3_NAT)

Since 1983 an international group of institutions has collected and analyzed satellite radiance measurements from up to five geostationary and two polar orbiting satellites to infer the global distribution of cloud properties and their diurnal, seasonal and interannual variations. The primary focus of the first phase of the project (1983-1995) was the elucidation of the role of clouds in the radiation budget (top of the atmosphere and surface). In the second phase of the project (1995 onwards) the analysis also concerns improving understanding of clouds in the global hydrological cycle. [Location=TROPOSPHERE] [Temporal_Coverage: Start_Date=1983-07-01; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=30 Km; Longitude_Resolution=30 Km; Temporal_Resolution=3 Hourly].

CLOUD PARTICLE SIZE↗

International Satellite Cloud Climatology Project (ISCCP) Stage D2 Monthly Cloud Product - Revised Algorithm in Native (NAT) Data Format (ISCCP_D2_NAT)

Since 1983 an international group of institutions has collected and analyzed satellite radiance measurements from up to five geostationary and two polar orbiting satellites to infer the global distribution of cloud properties and their diurnal, seasonal and interannual variations. The primary focus of the first phase of the project (1983-1995) was the elucidation of the role of clouds in the radiation budget (top of the atmosphere and surface). In the second phase of the project (1995 onwards) the analysis also concerns improving understanding of clouds in the global hydrological cycle. [Location=TROPOSPHERE] [Temporal_Coverage: Start_Date=1983-07-01; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=280 Km; Longitude_Resolution=280 Km; Temporal_Resolution=Monthly].

CLOUD OPTICAL THICKNESS↗

International Satellite Cloud Climatology Project (ISCCP) Stage D1 3-Hourly Cloud Product - Revised Algorithm in Hierarchical Data Format (ISCCP_D1)

Since 1983 an international group of institutions has collected and analyzed satellite radiance measurements from up to five geostationary and two polar orbiting satellites to infer the global distribution of cloud properties and their diurnal, seasonal and interannual variations. The primary focus of the first phase of the project (1983-1995) was the elucidation of the role of clouds in the radiation budget (top of the atmosphere and surface). In the second phase of the project (1995 onwards) the analysis also concerns improving understanding of clouds in the global hydrological cycle. [Location=TROPOSPHERE] [Temporal_Coverage: Start_Date=1983-07-01; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=280 Km; Longitude_Resolution=280 Km; Temporal_Resolution=3 Hourly].

CLOUD LIQUID WATER PATH↗

International Satellite Cloud Climatology Project (ISCCP) Stage D1 3-Hourly Cloud Product - Revised Algorithm in Native (NAT) Format (ISCCP_D1_NAT)

Since 1983 an international group of institutions has collected and analyzed satellite radiance measurements from up to five geostationary and two polar orbiting satellites to infer the global distribution of cloud properties and their diurnal, seasonal and interannual variations. The primary focus of the first phase of the project (1983-1995) was the elucidation of the role of clouds in the radiation budget (top of the atmosphere and surface). In the second phase of the project (1995 onwards) the analysis also concerns improving understanding of clouds in the global hydrological cycle. [Location=TROPOSPHERE] [Temporal_Coverage: Start_Date=1983-07-01; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=280 Km; Longitude_Resolution=280 Km; Temporal_Resolution=3 Hourly].

GRID DATA↗

International Satellite Cloud Climatology Project (ISCCP) TIROS Operational Vertical Sounder (TOVS) Product in Native (NAT) Format (ISCCP_TOVS_NAT)

Since 1983 an international group of institutions has collected and analyzed satellite radiance measurements from up to five geostationary and two polar orbiting satellites to infer the global distribution of cloud properties and their diurnal, seasonal and interannual variations. The primary focus of the first phase of the project (1983-1995) was the elucidation of the role of clouds in the radiation budget (top of the atmosphere and surface). In the second phase of the project (1995 onwards) the analysis also concerns improving understanding of clouds in the global hydrological cycle. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1983-07-01; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=280 degree; Longitude_Resolution=280 degree; Temporal_Resolution=Daily - < Monthly].

PRECIPITABLE WATER PROFILES↗

International Satellite Cloud Climatology Project (ISCCP) Ice Snow Product in Native (NAT) Format (ISCCP_ICESNOW_NAT)

Since 1983 an international group of institutions has collected and analyzed satellite radiance measurements from up to five geostationary and two polar orbiting satellites to infer the global distribution of cloud properties and their diurnal, seasonal and interannual variations. The primary focus of the first phase of the project (1983-1995) was the elucidation of the role of clouds in the radiation budget (top of the atmosphere and surface). In the second phase of the project (1995 onwards) the analysis also concerns improving understanding of clouds in the global hydrological cycle. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1983-07-01; Stop_Date=] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=112 Km; Longitude_Resolution=112 Km; Temporal_Resolution=5-day].

SNOW COVER↗

CERES Monthly Gridded Single Satellite TOA and Surfaces/Clouds (SFC) data in HDF (CER_SFC_Terra-FM2-MODIS_Edition2A)

The Monthly Gridded TOA/Surface Fluxes and Clouds (SFC) product contains a month of space and time averaged Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The SFC is also produced for combinations of scanner instruments. All instantaneous shortwave, longwave, and window fluxes at the Top-of-the-Atmosphere (TOA) and surface from the CERES SSF product for a month are sorted by 1-degree spatial regions and by the local hour of observation. The mean of the instantaneous fluxes for a given region-hour bin is determined and recorded on the SFC along with other flux statistics and scene information. These average fluxes are given for both clear-sky and total-sky scenes. The regional cloud properties are column averaged and are included on the SFC. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2003-12-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=100] [Data_Resolution: Latitude_Resolution=1 degree; Longitude_Resolution=1 degree; Horizontal_Resolution_Range=100 km - < 250 km or approximately 1 degree - < 2.5 degrees; Temporal_Resolution=1 hour; Temporal_Resolution_Range=Hourly - < Daily].

ICE PARTICLE DIAMETER↗

Spatial and Temporal Distribution of Clouds Observed by MODIS Onboard the Terra and Aqua Satellites

The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched aboard the Terra spacecraft on December 18, 1999 and Aqua spacecraft on May 4, 2002. A comprehensive set of remote sensing algorithms for the retrieval of cloud physical and optical properties have enabled over twelve years of continuous observations of cloud properties from Terra and over nine years from Aqua. The archived products from these algorithms include 1 km pixel-level (Level-2) and global gridded Level-3 products. In addition to an extensive cloud mask, products include cloud-top properties (temperature, pressure, effective emissivity), cloud thermodynamic phase, cloud optical and microphysical parameters (optical thickness, effective particle radius, water path), as well as derived statistics. Results include the latitudinal distribution of cloud optical and radiative properties for both liquid water and ice clouds, as well as latitudinal distributions of cloud top pressure and cloud top temperature. MODIS finds the cloud fraction, as derived by the cloud mask, is nearly identical during the day and night, with only modest diurnal variation. Globally, the cloud fraction derived by the MODIS cloud mask is approx.67%, with somewhat more clouds over land during the afternoon and less clouds over ocean in the afternoon, with very little difference in global cloud cover between Terra and Aqua. Overall, cloud fraction over land is approx.55%, with a distinctive seasonal cycle, whereas the ocean cloudiness is much higher, around 72%, with much reduced seasonal variation. Cloud top pressure and temperature have distinct spatial and temporal patterns, and clearly reflect our understanding of the global cloud distribution. High clouds are especially prevalent over the northern hemisphere continents between 30 and 50 . Aqua and Terra have comparable zonal cloud top pressures, with Aqua having somewhat higher clouds (cloud top pressures lower by 100 hPa) over land due to afternoon deep convection. The coldest cloud tops (colder than 230 K) generally occur over Antarctica and the high clouds in the tropics (ITCZ and the deep convective clouds over the western tropical Pacific and Indian sub-continent).

King, Michael D.↗

Changing Characteristics of Tropical Extreme Precipitation–Cloud Regimes in Warmer Climates

In this study, we investigated the changing characteristics of climatic scale (monthly) tropical extreme precipitation in warming climates using the Energy Exascale Earth System Model (E3SM). The results are from Atmospheric Model Intercomparison Project (AMIP)-type simulations driven by (a) a control experiment with the present-day sea surface temperature (SST) and CO 2 concentration, (b) P4K, the same as in (a) but with a uniform increase of 4K in the SST globally, and (c) the same as in (a), but with an imposed SST and CO 2 concentration from the outputs of the coupled E3SM forced by a 4xCO 2 concentration. We found that as the surface warmed under P4K and 4xCO 2 , both convective and stratiform rain increased. Importantly, there was an increasing fractional contribution of stratiform rain as a function of the precipitation intensity, with the most extreme but rare events occurring preferentially over land more than the ocean, and more so under 4xCO 2 than P4K. Extreme precipitation was facilitated by increased precipitation efficiency, reflecting accelerated rates of recycling of precipitation cloud water (both liquid and ice phases) in regions with colder anvil cloud tops. Changes in the vertical profiles of clouds, condensation heating, and vertical motions indicate increasing precipitation–cloud–circulation organization from the control and P4K to 4xCO 2 . The results suggest that large-scale ocean warming, that is, P4K, was the primary cause contributing to an organization structure resembling the well-known mesoscale convective system (MCS), with increased extreme precipitation on shorter (hourly to daily) time scales. Additional 4xCO 2 atmospheric radiative heating and dynamically consistent anomalous SST further amplified the MCS organization under P4K. Analyses of the surface moist static energy distribution show that increases in the surface moisture (temperature) under P4K and 4xCO 2 was the key driver leading to enhanced convective instability over tropical ocean (land). However, a fast and large increase in the land surface temperature and lack of available local moisture resulted in a strong reduction in the land surface relative humidity, reflecting severe drying and enhanced convective inhibition (CIN). It is argued that very extreme and rare “record-breaking” precipitation events found over land under P4K, and more so under 4xCO 2 , are likely due to the delayed onset of deep convection, that is, the longer the suppression of deep convection by CIN, the more severe the extreme precipitation when it eventually occurs, due to the release of a large amount of stored surplus convective available potential energy in the lower troposphere during prolonged CIN.

54 ENVIRONMENTAL SCIENCES↗

Warm boundary-layer cloud properties and cloud susceptibilities product at the ARM ENA observatory

Cloud liquid water path, albedo, and cloud fraction susceptibilities for marine warm boundary-layer clouds are quantified using the Meteosat retrieved cloud microphysical properties at the ARM Eastern North Atlantic (ENA) observatory in the Azores. The Meteosat cloud retrievals are based on the methods applied by the Clouds and the Earth’s Radiant Energy System (CERES) project, which are specifically tailored to support the ARM user facility over the ARM ground-based observation sites (enavisstpx2dm11minnisX1.c1). Cloud susceptibility is quantified as the slope between cloud properties and Nd within a 1-degree-by-1-degree grid box at each satellite time step using a least-square regression. To reduce uncertainties associated with the adiabatic assumption in the Nd retrieval, for each cloud object, we exclude cloudy pixels at the cloud edge, defined as those adjacent to cloud-free pixels. To minimize influence of cloud heterogeneity and co-variability on the retrieved cloud susceptibility, cloud properties are averaged to 0.25-degree resolution using the 3-km pixel-level retrieval, and the 1-degree cloud susceptibilities are estimated using the smoothed data. Cloud type classification is applied to distinct cloud object, labeling all contiguous cloudy pixels. Marine warm boundary-layer clouds are defined as clouds with 90% of cloud tops below 3km, and Meteosat retrieved cloud phase as liquid.

54 ENVIRONMENTAL SCIENCES↗

minimpl (b1)

The micropulse lidar (MPL) is a ground-based, optical, remote-sensing system designed primarily to determine the altitude of clouds; however, it is also used for detection of atmospheric aerosols. The physical principle is the same as for radar. Pulses of energy are transmitted into the atmosphere; the energy scattered back to the transceiver is collected and measured as a time-resolved signal, thereby detecting clouds and aerosols in real time. From the time delay between each outgoing pulse and the backscattered signal, the distance to the scatterer is inferred. Post-processing of the lidar return characterizes the extent and properties of aerosols or other particles in a region.

54 ENVIRONMENTAL SCIENCES↗

Early Results from the MODIS Atmosphere Cloud Algorithms

The Moderate Resolution Imaging Spectroradiometer (MODIS) is one of five instruments aboard the Terra Earth Observing System platform launched in December 1999. With 36 spectral bands from the visible through the infrared, and spatial resolution from 250m to 1km, the instrument provides an unprecedented opportunity for global cloud studies. A comprehensive set of remote sensing algorithms for cloud masking and retrieval of cloud physical and optical properties have been developed by members of the MODIS atmosphere team. The archived products from these algorithms have applications in climate change studies, climate modeling, numerical weather prediction, as well as fundamental atmospheric research. In addition to an extensive cloud mask, products include cloud top physical parameters (temperature, pressure, emissivity), cloud phase, cloud optical parameters (optical depth, effective particle radius, water path), visible cirrus reflectance, a contrail flag, and other derived parameters. All products are archived into two categories: pixel-level retrievals at a 1 km or 5 km spatial resolution at nadir (referred to as Level-2 products) and 1 degree global gridded statistics (Level-3 products). An overview of the MODIS atmosphere algorithms and products, their status, validation activities, and early level-2 and -3 results will be presented.

Platnick, S.↗

The 1996 Subsonic Aircraft: Contrail and Cloud Effects Special Study

During April 1996 NASA, in conjunction with the DOE, will sponsor a multi-aircraft field campaign to better understand the microphysical and radiative properties of cirrus clouds, the origins of ice nuclei and cloud condensation nuclei in the upper troposphere, and the possible role that the commercial subsonic aircraft fleet might play in altering cloud or aerosol properties. The NASA ER-2 aircraft will be used as a remote sensing platform, while the NASA DC-8 aircraft will be used as an in situ measurement platform. In situ observations will include a full set of size distribution measurements from nano-meter to millimeter sizes, ice water content measurements, gas phase and condensed phase chemical measurements, ice crystal optical phase function measurements, lidar observations of cloud top and cloud base, and atmospheric state measurement. The ER-2 will have lidar, microwave ice water path measurements, as well as visible and infrared spectral measurement. In this presentation the highlights of the mission will be presented. The goal will be to address fundamental questions such as the mode of nucleation of cirrus clouds, the composition of the nuclei on which cirrus form, the degree to which aircraft impact cirrus cloud properties.

Toon, Owen B.↗

Understanding Differences Between Co-Incident CloudSat, Aqua/MODIS and NOAA18 MHS Ice water Path Retrievals Over the Tropical Oceans

Accurate measurement of the physical and radiative properties of clouds and their representation in climate models continues to be a challe nge. Model parameterizations are still subject to a large number of t unable parameters; furthermore, accurate and representative in situ o bservations are very sparse, and satellite observations historically have significant quantitative uncertainties, particularly with respect to particle size distribution (PSD) and cloud phase. Ice Water Path (IWP), or amount of ice present in a cloud column, is an important cl oud property to accurately quantify, because it is an integral measur e of the microphysical properties of clouds and the cloud feedback pr ocesses in the climate system. This paper investigates near co-incident retrievals of IWP over tropical oceans using three diverse measurem ent systems: radar from CloudSat, Vis/IR from Aqua/MODIS, and microwa ve from NOAA-18IMHS. CloudSat 94 GHz radar measurements provide high resolution vertical and along-orbit structure of cloud reflectivity a nd enable IWP (and IWC) retrievals. Overlapping MODIS measurements of cloud optical thickness and phase allow estimates of IWP when cloud tops are identified as being ice. Periodically, NOAA18 becomes co-inci dent in space I time to enable comparison of A-Train measurements to IWP inferred from the 157 and 89 GHz channel radiances. This latter m easurement is effective only for thick convective anvil systems. We s tratify these co-incident data (less than 4 minutes separation) into cirrus only, cirrus overlying liquid water clouds, and precipitating d eep convective clouds. Substantial biases in IWP and ice effective ra dius are found. Systematic differences in these retrievals are consid ered in light of the uncertainties in a priori assumptions ofPSDs, sp ectral sensitivity and algorithm strategies, which have a direct impact on the IWP product.

Pittman, Jasna↗

Changing Characteristics of Tropical Extreme Precipitation-Cloud Regimes in Warmer Climates

In this paper, we have investigated the changing characteristics of climatic scale (monthly) tropical extreme precipitation in warming climates using the Energy Exascale Earth System Model (E3SM). Results are from Atmospheric Model Intercomparison Project (AMIP)-type simulations driven by a) control experiment with present-day sea surface temperature (SST) and CO 2 concentration, b) P4K, same as in a) but with uniform increase by 4K in SST globally, and c) same as in a), but with imposed SST and CO 2 concentration from outputs of coupled E3SM forced by 4xCO 2 concentration. We find that as the surface warms under P4K and 4xCO 2 , both convective and stratiform rain increase. Importantly, there is increasing fractional contribution of stratiform rain as a function of precipitation intensity, with the most extreme but rare events occurring preferentially over land more than ocean, more so under 4xCO 2 than P4K. Extreme precipitation is facilitated by increased precipitation efficiency, reflecting accelerated rates of recycling of precipitation-cloud water (both liquid and ice phases) in regions with colder anvil cloud tops. Changes in vertical profiles of clouds, condensation heating and vertical motions indicate increasing precipitation-cloud-circulation organization from control, P4K to 4xCO 2 . Results suggest that large-scale ocean warming, i.e., P4K, is the primary cause contributing to organization structure resembling the well-known Mesoscale Convective System (MCS) for increased extreme precipitation on shorter (hourly to daily) time scales. Additional 4xCO 2 atmospheric radiative heating, and dynamically consistent anomalous SST further amplifies the MCS organization under P4K. Analyses of the surface moist static energy distribution show that increase in surface moisture (temperature) under P4K and 4xCO 2 is the key driver leading to enhanced convective instability over tropical ocean (land). However, the fast and large increase in land surface temperature and lack of available local moisture result in strong reduction in land surface relative humidity, reflecting severe drying and enhanced convective inhibition (CIN). It is argued that very extreme and rare “record-breaking” precipitation events found over land under P4K, more so under 4xCO 2 , are likely due to the delayed onset of deep convection, i.e., the longer the suppression of deep convection by CIN, the more severe the extreme precipitation when eventually occur, due to the release of large amount of stored surplus convective available potential energy in the lower troposphere during prolonged CIN.

climate-scale extreme tropical precipitation↗